FN Thomson Reuters Web of Science™ VR 1.0 PT J AU McIntyre, JI Agusbudiman, A Cameron, IM Dumais, JR Eslinger, PW Gheddou, A Khrustalev, K Marsoem, P Miley, HS Nikkinen, M Prinke, AM Ripplinger, MD Schrom, BT Sliger, WA Stoehlker, U Suhariyono, G Warren, GA Widodo, S Woods, VT AF McIntyre, Justin I. Agusbudiman, Agung Cameron, Ian M. Dumais, Johannes R. Eslinger, Paul W. Gheddou, Abdelhakim Khrustalev, Kirill Marsoem, Pujadi Miley, Harry S. Nikkinen, Mika Prinke, Amanda M. Ripplinger, Michael D. Schrom, Brian T. Sliger, William A. Stoehlker, Ulrich Suhariyono, Gatot Warren, Glen A. Widodo, Susilo Woods, Vincent T. TI Real-time stack monitoring at the BaTek medical isotope production facility SO JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY LA English DT Article DE Medical isotope production; International monitoring system (IMS); Stack monitoring; Radioxenon; CTBTO ID NUCLEAR-EXPLOSIONS AB Radioxenon emissions from fission-based radiopharmaceutical production are a major source of background concentrations affecting the radioxenon detection systems of the international monitoring system (IMS). Collection of real-time emissions data from production facilities makes it possible to screen out some medical isotope signatures from the IMS radioxenon data sets. This paper describes an effort to obtain and analyze real-time stack emissions data with the design, construction and installation of a small stack monitoring system developed by a joint CTBTO-IDC, BATAN, and Pacific Northwest National Laboratory team at the BaTek medical isotope production facility near Jakarta, Indonesia. C1 [McIntyre, Justin I.; Cameron, Ian M.; Eslinger, Paul W.; Miley, Harry S.; Prinke, Amanda M.; Ripplinger, Michael D.; Schrom, Brian T.; Sliger, William A.; Warren, Glen A.; Woods, Vincent T.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Agusbudiman, Agung; Dumais, Johannes R.; Marsoem, Pujadi; Suhariyono, Gatot; Widodo, Susilo] Natl Nucl Energy Agcy, BATAN, Jakarta, Indonesia. [Gheddou, Abdelhakim; Khrustalev, Kirill] CTBTO, Int Data Ctr, Vienna, Austria. [Nikkinen, Mika] IAEA, A-1400 Vienna, Austria. [Stoehlker, Ulrich] Fed Off Radiat Protect, Freiburg, Germany. RP Eslinger, PW (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM paul.w.eslinger@pnnl.gov FU U.S. Office of Multilateral and Nuclear Affairs in the Bureau of Arms Control, Verification and Compliance Nuclear, at the Department of State; U.S. Nuclear Arms Control Technology Program, at the Defense Threat Reduction Agency; European Union [2008/588/CFSP] FX The authors wish to acknowledge the funding support of the U.S. Office of Multilateral and Nuclear Affairs in the Bureau of Arms Control, Verification and Compliance Nuclear, at the Department of State and the U.S. Nuclear Arms Control Technology Program, at the Defense Threat Reduction Agency. The stack monitor equipment and data analysis to support the CTBTO in implementing the noble gas verification regime were funded by the European Union through Council Joint Action 2008/588/CFSP of 15 July 2008. NR 13 TC 1 Z9 1 U1 0 U2 0 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0236-5731 EI 1588-2780 J9 J RADIOANAL NUCL CH JI J. Radioanal. Nucl. Chem. PD APR PY 2016 VL 308 IS 1 BP 311 EP 316 DI 10.1007/s10967-015-4348-2 PG 6 WC Chemistry, Analytical; Chemistry, Inorganic & Nuclear; Nuclear Science & Technology SC Chemistry; Nuclear Science & Technology GA DG7MQ UT WOS:000372268800035 ER PT J AU Pasha, MFK Yang, M Yeasmin, D Saetern, S Kao, SC Smith, B AF Pasha, M. Fayzul K. Yang, Majntxov Yeasmin, Dilruba Saetern, Sen Kao, Shih-Chieh Smith, Brennan TI Identifying High Power-Density Stream Reaches through Refined Geospatial Resolution in Hydropower Resource Assessment SO JOURNAL OF WATER RESOURCES PLANNING AND MANAGEMENT LA English DT Article AB Aided by the rapid development of multiple geospatial data sets for topography, hydrology, and existing energy-water infrastructures, reconnaissance-level hydropower resource assessment can now be conducted using geospatial models in all regions of the United States. The updated techniques can be used to estimate the total undeveloped hydropower potential across all regions, and they may eventually help to identify additional hydropower resources that were previously overlooked. To enhance the characterization of higher power-density stream reaches, this paper explored how the degree of geospatial resolution affects the identification of hydropower stream reaches, using the geospatial merit matrix-based hydropower resource assessment (GMM-HRA) model. GMM-HRA model simulation was conducted at eight different spatial resolutions on six USGS eight-digit hydrologic units with terrains classified as flat, mild, and steep. The results showed that more hydropower potential from higher power-density stream reaches can be identified with increasing spatial resolution. Both flat and mild terrains exhibited lower impacts from resolution differences than did the steep terrain. The findings indicate that greater care should be taken in selecting the discretization resolution for hydropower resource assessments in future studies. C1 [Pasha, M. Fayzul K.; Yang, Majntxov; Saetern, Sen] Calif State Univ Fresno, Dept Civil & Geomat Engn, 2320E San Ramon Ave M-S EE94, Fresno, CA 93740 USA. [Yeasmin, Dilruba] Calif State Univ Fresno, Calif Water Inst, Fresno, CA 93740 USA. [Yeasmin, Dilruba] Calif State Univ Fresno, Ctr Irrigat Technol, Fresno, CA 93740 USA. [Kao, Shih-Chieh] Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. [Smith, Brennan] Oak Ridge Natl Lab, Div Environm Sci, Energy Water Ecosyst Engn Grp, POB 2008, Oak Ridge, TN 37831 USA. RP Pasha, MFK (reprint author), Calif State Univ Fresno, Dept Civil & Geomat Engn, 2320E San Ramon Ave M-S EE94, Fresno, CA 93740 USA. EM mpasha@csufresno.edu RI Kao, Shih-Chieh/B-9428-2012 OI Kao, Shih-Chieh/0000-0002-3207-5328 FU Wind and Water Power Technologies Office, Office of Energy Efficiency and Renewable Energy of the U.S. Department of Energy (DOE); California State University-Fresno; U.S. DOE [DE-AC05-00OR22725] FX This research was sponsored by the Wind and Water Power Technologies Office, Office of Energy Efficiency and Renewable Energy of the U.S. Department of Energy (DOE). Support from California State University-Fresno is also acknowledged. This paper was co-authored by employees of Oak Ridge National Laboratory, managed by UT Battelle, under contract DE-AC05-00OR22725 with the U.S. DOE. Accordingly, the publisher, by accepting the article for publication, acknowledges that the U.S. government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for U.S. government purposes. The U.S. DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 9 TC 1 Z9 1 U1 0 U2 0 PU ASCE-AMER SOC CIVIL ENGINEERS PI RESTON PA 1801 ALEXANDER BELL DR, RESTON, VA 20191-4400 USA SN 0733-9496 EI 1943-5452 J9 J WATER RES PLAN MAN JI J. Water Resour. Plan. Manage.-ASCE PD APR PY 2016 VL 142 IS 4 AR 06016001 DI 10.1061/(ASCE)WR.1943-5452.0000599 PG 6 WC Engineering, Civil; Water Resources SC Engineering; Water Resources GA DH5DD UT WOS:000372804500001 ER PT J AU Seth, A Klise, KA Siirola, JD Haxton, T Laird, CD AF Seth, Arpan Klise, Katherine A. Siirola, John D. Haxton, Terranna Laird, Carl D. TI Testing Contamination Source Identification Methods for Water Distribution Networks SO JOURNAL OF WATER RESOURCES PLANNING AND MANAGEMENT LA English DT Article DE Drinking water distribution system; Source identification; Testing ID DISTRIBUTION-SYSTEMS; OPTIMIZATION; ALGORITHM; SECURITY; DESIGN; MODEL AB In the event of contamination in a water distribution network (WDN), source identification (SI) methods that analyze sensor data can be used to identify the source location(s). Knowledge of the source location and characteristics are important to inform contamination control and cleanup operations. Various SI strategies that have been developed by researchers differ in their underlying assumptions and solution techniques. The following manuscript presents a systematic procedure for testing and evaluating SI methods. The performance of these SI methods is affected by various factors including the size of WDN model, measurement error, modeling error, time and number of contaminant injections, and time and number of measurements. This paper includes test cases that vary these factors and evaluates three SI methods on the basis of accuracy and specificity. The tests are used to review and compare these different SI methods, highlighting their strengths in handling various identification scenarios. These SI methods and a testing framework that includes the test cases and analysis tools presented in this paper have been integrated into EPA's Water Security Toolkit (WST), a suite of software tools to help researchers and others in the water industry evaluate and plan various response strategies in case of a contamination incident. Finally, a set of recommendations are made for users to consider when working with different categories of SI methods. C1 [Seth, Arpan; Laird, Carl D.] Purdue Univ, Sch Chem Engn, 480 Stadium Mall, W Lafayette, IN 47907 USA. [Klise, Katherine A.] Sandia Natl Labs, Geosci Res & Applicat Grp, POB 5800,MS 0751, Albuquerque, NM 87185 USA. [Siirola, John D.] Sandia Natl Labs, Ctr Res Comp, POB 5800 MS,1326, Albuquerque, NM 87185 USA. [Haxton, Terranna] US EPA, Natl Homeland Secur Res Ctr, 26 W Martin Luther King Dr, Cincinnati, OH 45268 USA. RP Laird, CD (reprint author), Purdue Univ, Sch Chem Engn, 480 Stadium Mall, W Lafayette, IN 47907 USA. EM haxton.terra@epa.gov; lairdc@purdue.edu FU Sandia National Laboratories; U.S. Environmental Protection Agency; Lockheed Martin Corporation for the U.S. Department of Energy's National Nuclear Security Administration [DE-AC04 94AL85000]; U.S. Environmental Protection Agency (EPA) through its Office of Research and Development [DW8992192801]; Department of Energy's Sandia National Laboratories; [SAND2014-20020 J] FX The authors gratefully acknowledge financial support provided by Sandia National Laboratories and U.S. Environmental Protection Agency. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04 94AL85000. SAND Number SAND2014-20020 J. The U.S. Environmental Protection Agency (EPA) through its Office of Research and Development funded and collaborated in the research described here under an Interagency Agreement (IA # DW8992192801) with the Department of Energy's Sandia National Laboratories. It has been subject to an administrative review but does not necessarily reflect the views of the Agency. No official endorsement should be inferred. EPA does not endorse the purchase or sale of any commercial products or services. NR 32 TC 1 Z9 1 U1 3 U2 11 PU ASCE-AMER SOC CIVIL ENGINEERS PI RESTON PA 1801 ALEXANDER BELL DR, RESTON, VA 20191-4400 USA SN 0733-9496 EI 1943-5452 J9 J WATER RES PLAN MAN JI J. Water Resour. Plan. Manage.-ASCE PD APR PY 2016 VL 142 IS 4 AR 04016001 DI 10.1061/(ASCE)WR.1943-5452.0000619 PG 11 WC Engineering, Civil; Water Resources SC Engineering; Water Resources GA DH5DD UT WOS:000372804500003 ER PT J AU Fernandez-Moreno, JP Malitsky, S Lashbrooke, J Biswal, AK Racovita, RC Mellerowicz, EJ Jetter, R Orzaez, D Aharoni, A Granell, A AF Fernandez-Moreno, Josefina-Patricia Malitsky, Sergey Lashbrooke, Justin Biswal, Ajaya Kumar Racovita, Radu C. Mellerowicz, Ewa J. Jetter, Reinhard Orzaez, Diego Aharoni, Asaph Granell, Antonio TI An efficient method for medium throughput screening of cuticular wax composition in different plant species SO METABOLOMICS LA English DT Article DE Metabolic profiling; Cuticular waxes; Fruit surface; Fleshy fruit ID TRANSPIRATION BARRIER PROPERTIES; TOMATO FRUIT; SURFACE WAX; MICRO-TOM; CUTICLE; IDENTIFICATION; TRITERPENOIDS; COMPONENTS; DIVERSITY; CULTIVARS AB Introduction Most aerial plant organs are covered by a cuticle, which largely consists of cutin and wax. Cuticular waxes are mixtures of dozens of compounds, mostly very-long-chain aliphatics that are easily extracted by solvents. Over the last four decades, diverse cuticular wax analysis protocols have been developed, most of which are complex and time-consuming, and need to be adapted for each plant species or organ. Plant genomics and breeding programs often require mid-throughput metabolic phenotyping approaches to screen large numbers of individuals and obtain relevant biological information. Objectives To generate a fast, simple and user-friendly methodology able to capture most wax complexity independently of the plant, cultivar and organ. Methods Here we present a simple GC-MS method for screening relatively small wax amounts, sampled by short extraction with a versatile, uniform solvent. The method will be tested and validated in leaves and fruits from three different crop species: tomato (Solanum lycopersicum), apple (Malus domestica) and hybrid aspen (Populus tremula x tremuloides). Results Consistent results were obtained in tomato cultivar M82 across three consecutive years (2010-2012), two organs (leaf and fruit), and also in two different tomato (M82 and MicroTom) and apple (Golden Delicious and Granny Smith) cultivars. Our results on tomato wax composition match those reported previously, while our apple and hybrid aspen analyses provide the first comprehensive cuticular wax profile of these species. Conclusion This protocol allows standardized identification and quantification of most cuticular wax components in a range of species. C1 [Fernandez-Moreno, Josefina-Patricia; Orzaez, Diego; Granell, Antonio] Univ Politecn Valencia, Fruit Genom & Biotechnol Lab, Inst Biol Mol & Celular Plantas CSIC UPV, Ciudad Politecn Innovac, Ave Ingn Fausto Elio S-N, E-46022 Valencia, Spain. [Malitsky, Sergey; Lashbrooke, Justin; Aharoni, Asaph] Weizmann Inst Sci, Dept Plants & Environm Sci, Ullmann Bldg Life Sci,Room 105,POB 26, IL-76100 Rehovot, Israel. [Biswal, Ajaya Kumar] Univ Georgia, Complex Carbohydrate Res Ctr, 315 Riverbend Rd, Athens, GA 30602 USA. [Biswal, Ajaya Kumar] DOE BioEnergy Sci Ctr BESC, Oak Ridge, TN USA. [Racovita, Radu C.] Univ British Columbia, Dept Chem, Fac Sci, 3529-6270 Univ Blvd, Vancouver, BC V6T 1Z4, Canada. [Mellerowicz, Ewa J.] Swedish Univ Agr Sci, Dept Forest Genet & Plant Physiol, Umea Plant Sci Ctr, S-90183 Umea, Sweden. [Jetter, Reinhard] Univ British Columbia, Dept Bot, Fac Sci, 3529-6270 Univ Blvd, Vancouver, BC V6T 1Z4, Canada. [Jetter, Reinhard] Univ British Columbia, Dept Chem, Fac Sci, 3529-6270 Univ Blvd, Vancouver, BC V6T 1Z4, Canada. RP Granell, A (reprint author), Univ Politecn Valencia, Fruit Genom & Biotechnol Lab, Inst Biol Mol & Celular Plantas CSIC UPV, Ciudad Politecn Innovac, Ave Ingn Fausto Elio S-N, E-46022 Valencia, Spain.; Aharoni, A (reprint author), Weizmann Inst Sci, Dept Plants & Environm Sci, Ullmann Bldg Life Sci,Room 105,POB 26, IL-76100 Rehovot, Israel. EM asaph.aharoni@weizmann.ac.il; agranell@ibmcp.upv.es RI ORZAEZ, DIEGO/H-3457-2012; Racovita, Radu/Q-8089-2016; Lashbrooke, Justin/B-3732-2017; Granell, Antonio/G-3664-2010 OI ORZAEZ, DIEGO/0000-0003-1662-5403; Racovita, Radu/0000-0002-6396-9869; Lashbrooke, Justin/0000-0003-4511-4215; FU MINECO [BIO2013-42193-R]; EC [SFS7a-2014, 634561]; FPU-MECD [AP-2007-01905]; Israel Science Foundation (ISF) [646/11]; COST [FA1106] FX Research at the IBMCP was supported by MINECO Grant BIO2013-42193-R and from EC H2020 TRADITOM SFS7a-2014-(contract 634561) to Antonio Granell and by FPU-MECD personal Grant to Josefina Patricia Fernandez Moreno (AP-2007-01905). Research at the Weizmann Institute of Sciences was supported by the Israel Science Foundation (ISF) personal Grant to Asaph Aharoni (ISF Grant No. 646/11). We also thank COST FA1106 Quality Fruit for funding networking activities. NR 33 TC 1 Z9 1 U1 7 U2 26 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1573-3882 EI 1573-3890 J9 METABOLOMICS JI Metabolomics PD APR PY 2016 VL 12 IS 4 AR UNSP 73 DI 10.1007/s11306-016-0982-0 PG 13 WC Endocrinology & Metabolism SC Endocrinology & Metabolism GA DG5YD UT WOS:000372156700014 ER PT J AU Stewart, R Urban, M Duchscherer, S Kaufman, J Morton, A Thakur, G Piburn, J Moehl, J AF Stewart, Robert Urban, Marie Duchscherer, Samantha Kaufman, Jason Morton, April Thakur, Gautam Piburn, Jesse Moehl, Jessica TI A Bayesian machine learning model for estimating building occupancy from open source data SO NATURAL HAZARDS LA English DT Article DE Population; Building; Occupancy; Bayesian; Uncertainty; Open source; Elicitation ID EXPERT OPINIONS; POPULATION AB Understanding building occupancy is critical to a wide array of applications including natural hazards loss analysis, green building technologies, and population distribution modeling. Due to the expense of directly monitoring buildings, scientists rely in addition on a wide and disparate array of ancillary and open source information including subject matter expertise, survey data, and remote sensing information. These data are fused using data harmonization methods, which refer to a loose collection of formal and informal techniques for fusing data together to create viable content for building occupancy estimation. In this paper, we add to the current state of the art by introducing the population data tables (PDT), a Bayesian model and informatics system for systematically arranging data and harmonization techniques into a consistent, transparent, knowledge learning framework that retains in the final estimation uncertainty emerging from data, expert judgment, and model parameterization. PDT aims to estimate ambient occupancy in units of people/1000 ft(2) for a number of building types at the national and sub-national level with the goal of providing global coverage. We present the PDT model, situate the work within the larger community, and report on the progress of this multi-year project. C1 [Stewart, Robert; Urban, Marie; Thakur, Gautam; Piburn, Jesse] Oak Ridge Natl Lab, 1 Bethel Valley Rd,MS-6017,POB 2008, Oak Ridge, TN 37831 USA. [Duchscherer, Samantha; Kaufman, Jason; Morton, April; Moehl, Jessica] Oak Ridge Associated Univ, 1 Bethel Valley Rd,MS-6017,POB 2008, Oak Ridge, TN 37831 USA. RP Stewart, R (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd,MS-6017,POB 2008, Oak Ridge, TN 37831 USA. EM stewartrn@ornl.gov RI Thakur, Gautam/S-8694-2016; OI Thakur, Gautam/0000-0002-8341-4596; Stewart, Robert/0000-0002-8186-7559; Duchscherer, Samantha/0000-0002-2023-3106 FU UT-Battelle, LLC [DE-AC05-00OR22725]; U.S. Department of Energy FX This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 61 TC 0 Z9 0 U1 8 U2 15 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0921-030X EI 1573-0840 J9 NAT HAZARDS JI Nat. Hazards PD APR PY 2016 VL 81 IS 3 BP 1929 EP 1956 DI 10.1007/s11069-016-2164-9 PG 28 WC Geosciences, Multidisciplinary; Meteorology & Atmospheric Sciences; Water Resources SC Geology; Meteorology & Atmospheric Sciences; Water Resources GA DG7TC UT WOS:000372285600026 ER PT J AU Wright, AT AF Wright, Aaron T. TI HOST-PATHOGEN INTERACTIONS A cholera surveillance system SO NATURE CHEMICAL BIOLOGY LA English DT News Item AB Bacterial pathogen-secreted proteases may have a key role in inhibiting a potentially widespread host-pathogen interaction. Activity-based protein profiling enabled the identification of a major Vibrio cholerae serine protease that limits the ability of a host-derived intestinal lectin to bind to the bacterial pathogen in vivo. C1 [Wright, Aaron T.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. RP Wright, AT (reprint author), Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. EM aaron.wright@pnnl.gov OI Wright, Aaron/0000-0002-3172-5253 NR 5 TC 0 Z9 0 U1 1 U2 4 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1552-4450 EI 1552-4469 J9 NAT CHEM BIOL JI Nat. Chem. Biol. PD APR PY 2016 VL 12 IS 4 BP 203 EP 204 DI 10.1038/nchembio.2039 PG 3 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DH2DA UT WOS:000372593200002 PM 26900864 ER PT J AU Grimm, SS Isacoff, EY AF Grimm, Sasha S. Isacoff, Ehud Y. TI Allosteric substrate switching in a voltage-sensing lipid phosphatase SO NATURE CHEMICAL BIOLOGY LA English DT Article ID SHAKER K+ CHANNEL; GATED PROTON CHANNELS; TENSIN HOMOLOG PTEN; CI-VSP; POTASSIUM CHANNEL; SENSITIVE PHOSPHATASE; ION-CHANNEL; SENSOR; DOMAIN; ACTIVATION AB Allostery provides a critical control over enzyme activity, biasing the catalytic site between inactive and active states. We found that the Ciona intestinalis voltage-sensing phosphatase (Ci-VSP), which modifies phosphoinositide signaling lipids (PIPs), has not one but two sequential active states with distinct substrate specificities, whose occupancy is allosterically controlled by sequential conformations of the voltage-sensing domain (VSD). Using fast fluorescence resonance energy transfer (FRET) reporters of PIPs to monitor enzyme activity and voltage-clamp fluorometry to monitor conformational changes in the VSD, we found that Ci-VSP switches from inactive to a PIP3-preferring active state when the VSD undergoes an initial voltage-sensing motion and then into a second PIP2-preferring active state when the VSD activates fully. This two-step allosteric control over a dual-specificity enzyme enables voltage to shape PIP concentrations in time, and provides a mechanism for the complex modulation of PIP-regulated ion channels, transporters, cell motility, endocytosis and exocytosis. C1 [Grimm, Sasha S.; Isacoff, Ehud Y.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Isacoff, Ehud Y.] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [Isacoff, Ehud Y.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Isacoff, Ehud Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Isacoff, EY (reprint author), Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA.; Isacoff, EY (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA.; Isacoff, EY (reprint author), Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA.; Isacoff, EY (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. EM ehud@berkeley.edu FU US National Institutes of Health [R01GM117051, T32GM008295]; UC Berkeley Chancellors Fellowship for Graduate Study FX We thank Y. Okamura (Osaka University) for Ci-VSP, M. Matsuda (Kyoto University) for Fllip-pm, T. Meyer (Stanford University) for GFP-PLC-PH, T. Balla (US National Institutes of Health) for GFP-TAPP-PH, H. Okada, C. Stanley and Z. Fu for technical support, as well as A. Reiner, S. Bharill, S. Kohout, E. Carroll and other current and former members of the Isacoff laboratory for guidance on analysis and helpful discussions. This work was supported by the US National Institutes of Health (R01GM117051 and T32GM008295; E.Y.I.) as well as fellowship support for provided by the UC Berkeley Chancellors Fellowship for Graduate Study (S.S.G.). NR 60 TC 3 Z9 3 U1 7 U2 12 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 1552-4450 EI 1552-4469 J9 NAT CHEM BIOL JI Nat. Chem. Biol. PD APR PY 2016 VL 12 IS 4 BP 261 EP + DI 10.1038/NCHEMBIO.2022 PG 8 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DH2DA UT WOS:000372593200013 PM 26878552 ER PT J AU Ascherl, L Sick, T Margraf, JT Lapidus, SH Calik, M Hettstedt, C Karaghiosoff, K Doblinger, M Clark, T Chapman, KW Auras, F Bein, T AF Ascherl, Laura Sick, Torben Margraf, Johannes T. Lapidus, Saul H. Calik, Mona Hettstedt, Christina Karaghiosoff, Konstantin Doeblinger, Markus Clark, Timothy Chapman, Karena W. Auras, Florian Bein, Thomas TI Molecular docking sites designed for the generation of highly crystalline covalent organic frameworks SO NATURE CHEMISTRY LA English DT Article ID FILMS; CONSTRUCTION; PORES AB Covalent organic frameworks (COFs) formed by connecting multidentate organic building blocks through covalent bonds provide a platform for designing multifunctional porous materials with atomic precision. As they are promising materials for applications in optoelectronics, they would benefit from a maximum degree of long-range order within the framework, which has remained a major challenge. We have developed a synthetic concept to allow consecutive COF sheets to lock in position during crystal growth, and thus minimize the occurrence of stacking faults and dislocations. Hereby, the three-dimensional conformation of propeller-shaped molecular building units was used to generate well-defined periodic docking sites, which guided the attachment of successive building blocks that, in turn, promoted long-range order during COF formation. This approach enables us to achieve a very high crystallinity for a series of COFs that comprise tri- and tetradentate central building blocks. We expect this strategy to be transferable to a broad range of customized COFs. C1 [Ascherl, Laura; Sick, Torben; Calik, Mona; Hettstedt, Christina; Karaghiosoff, Konstantin; Doeblinger, Markus; Auras, Florian; Bein, Thomas] Univ Munich LMU, Dept Chem, Butenandtstr 5-13, D-81377 Munich, Germany. [Ascherl, Laura; Sick, Torben; Calik, Mona; Hettstedt, Christina; Karaghiosoff, Konstantin; Doeblinger, Markus; Auras, Florian; Bein, Thomas] Univ Munich LMU, Ctr NanoSci CeNS, Butenandtstr 5-13, D-81377 Munich, Germany. [Margraf, Johannes T.; Clark, Timothy] Univ Erlangen Nurnberg, Comp Chem Ctr, Nagelsbachstr 25, D-91052 Erlangen, Germany. [Lapidus, Saul H.; Chapman, Karena W.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Auras, F; Bein, T (reprint author), Univ Munich LMU, Dept Chem, Butenandtstr 5-13, D-81377 Munich, Germany. EM florian.auras@cup.lmu.de; bein@lmu.de FU German Science Foundation (Research Cluster Nanosystems Initiative Munich); Free State of Bavaria (Research Network SolTech); European Research Council under the European Union's Seventh Framework Programme (FP7)/ERC Grant Agreement [321339]; DOE Office of Science [DE-AC02-06CH11357] FX We are grateful for funding from the German Science Foundation (Research Cluster Nanosystems Initiative Munich) and the Free State of Bavaria (Research Network SolTech). The research leading to these results received funding from the European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013)/ERC Grant Agreement 321339. This research used beamlines 11-BM and 11-ID-B at the Advanced Photon Source, a US Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 35 TC 22 Z9 22 U1 67 U2 179 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1755-4330 EI 1755-4349 J9 NAT CHEM JI Nat. Chem. PD APR PY 2016 VL 8 IS 4 BP 310 EP 316 DI 10.1038/NCHEM.2444 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA DH0WT UT WOS:000372505500008 ER PT J AU Rotter, P Lechner, BAJ Morherr, A Chisnall, DM Ward, DJ Jardine, AP Ellis, J Allison, W Eckhardt, B Witte, G AF Rotter, Paul Lechner, Barbara A. J. Morherr, Antonia Chisnall, David M. Ward, David J. Jardine, Andrew P. Ellis, John Allison, William Eckhardt, Bruno Witte, Gregor TI Coupling between diffusion and orientation of pentacene molecules on an organic surface SO NATURE MATERIALS LA English DT Article ID THIN-FILM GROWTH; JUMP DIFFUSION; SCATTERING; NEUTRON; MOTION AB The realization of efficient organic electronic devices requires the controlled preparation of molecular thin films and heterostructures. As top-down structuring methods such as lithography cannot be applied to van der Waals bound materials(1), surface diffusion becomes a structure-determining factor that requires microscopic understanding. Scanning probe techniques provide atomic resolution, but are limited to observations of slow movements, and therefore constrained to low temperatures. In contrast, the helium-3 spin-echo (HeSE) technique achieves spatial and time resolution on the nm and ps scale, respectively, thus enabling measurements at elevated temperatures(2). Here we use HeSE to unveil the intricate motion of pentacene admolecules diffusing on a chemisorbed monolayer of pentacene on Cu(110) that serves as a stable, well-ordered organic model surface(3). We find that pentacene moves along rails parallel and perpendicular to the surface molecules. The experimental data are explained by admolecule rotation that enables a switching between diffusion directions, which extends our molecular level understanding of diffusion in complex organic systems. C1 [Rotter, Paul; Morherr, Antonia; Eckhardt, Bruno; Witte, Gregor] Univ Marburg, Fachbereich Phys, Renthof 5, D-35032 Marburg, Germany. [Lechner, Barbara A. J.; Chisnall, David M.; Ward, David J.; Jardine, Andrew P.; Ellis, John; Allison, William] Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England. [Lechner, Barbara A. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Witte, G (reprint author), Univ Marburg, Fachbereich Phys, Renthof 5, D-35032 Marburg, Germany. EM gregor.witte@physik.uni-marburg.de RI Lechner, Barbara/F-4963-2013; Eckhardt, Bruno/D-5948-2012; OI Lechner, Barbara/0000-0001-9974-1738; Eckhardt, Bruno/0000-0003-4050-3254; Ward, David/0000-0002-1587-7011 FU EPSRC [EP/E0049621]; Austrian Academy of Sciences; Royal Society; E.U. ERASMUS programme; Deutsche Forschungsgemeinschaft [GRK 1782] FX The authors acknowledge financial support from the EPSRC (EP/E0049621, B.A.J.L., D.J.W., D.M.C., A.P.J., J.E., W.A.), the Austrian Academy of Sciences (B.A.J.L.), the Royal Society (A.P.J.), the E.U. ERASMUS programme (A.M.) and the Deutsche Forschungsgemeinschaft (GRK 1782, P.R.). Underlying data are available at the University of Cambridge Research data repository (https://www.repository.cam.ac.uk). NR 30 TC 4 Z9 4 U1 12 U2 59 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD APR PY 2016 VL 15 IS 4 BP 397 EP + DI 10.1038/NMAT4575 PG 5 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA DH2CL UT WOS:000372591700012 PM 26901514 ER PT J AU Gu, J Yan, Y Young, JL Steirer, KX Neale, NR Turner, JA AF Gu, Jing Yan, Yong Young, James L. Steirer, K. Xerxes Neale, Nathan R. Turner, John A. TI Water reduction by a p-GaInP2 photoelectrode stabilized by an amorphous TiO2 coating and a molecular cobalt catalyst SO NATURE MATERIALS LA English DT Article ID ATOMIC LAYER DEPOSITION; SENSITIZED SOLAR-CELLS; VISIBLE-LIGHT; HYDROGEN-PRODUCTION; H-2 PRODUCTION; PHOTOANODES; CONVERSION; SILICON; PHOSPHONATE; CARBOXYLATE AB Producing hydrogen through solar water splitting requires the coverage of large land areas. Abundant metal-based molecular catalysts offer scalability, but only if they match noble metal activities. We report on a highly active p-GaInP2 photocathode protected through a 35-nm TiO2 layer functionalized by a cobaloxime molecular catalyst (GaInP2-TiO2-cobaloxime). This photoelectrode mediates H-2 production with a current density of similar to 9mAcm(-2) at a potential of 0V versus RHE under 1-sun illumination at pH 13. The calculated turnover number for the catalyst during a 20-h period is 139,000, with an average turnover frequency of 1.9 s(-1). Bare GaInP2 shows a rapid current decay, whereas the GaInP2-TiO2-cobaloxime electrode shows <= 5% loss over 20 min, comparable to a GaInP2-TiO2-Pt catalyst particle-modified interface. The activity and corrosion resistance of the GaInP2-TiO2-cobaloxime photocathode in basic solution is made possible by an atomic layer-deposited TiO2 and an attached cobaloxime catalyst. C1 [Gu, Jing; Yan, Yong; Young, James L.; Steirer, K. Xerxes; Neale, Nathan R.; Turner, John A.] Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. [Young, James L.] Univ Colorado, Mat Sci & Engn Program, Boulder, CO 80309 USA. RP Turner, JA (reprint author), Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. EM john.turner@nrel.gov FU US Department of Energy, Office of Science, Office of Basic Energy Sciences, Solar Photochemistry Program [DE-AC36-08GO28308]; NSF [DGE 1144083] FX We gratefully acknowledge H. Doscher for supplying the GaInP2 wafers, C. Xiao for AFM measurements, L. Gedvilas for ATR-IR measurements, C. Macomber for ICP-MS measurements, S. George for advice on ALD and H. Wang and T. Deutsch for useful discussions. This material is based on work supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, Solar Photochemistry Program under Contract Number DE-AC36-08GO28308. J.L.Y. acknowledges NSF Graduate Research Fellowship Grant No. DGE 1144083. NR 50 TC 28 Z9 28 U1 47 U2 128 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD APR PY 2016 VL 15 IS 4 BP 456 EP + DI 10.1038/NMAT4511 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA DH2CL UT WOS:000372591700022 PM 26689139 ER PT J AU Tantakitti, F Boekhoven, J Wang, X Kazantsev, RV Yu, T Li, JH Zhuang, E Zandi, R Ortony, JH Newcomb, CJ Palmer, LC Shekhawat, GS de la Cruz, MO Schatz, GC Stupp, SI AF Tantakitti, Faifan Boekhoven, Job Wang, Xin Kazantsev, Roman V. Yu, Tao Li, Jiahe Zhuang, Ellen Zandi, Roya Ortony, Julia H. Newcomb, Christina J. Palmer, Liam C. Shekhawat, Gajendra S. de la Cruz, Monica Olvera Schatz, George C. Stupp, Samuel I. TI Energy landscapes and functions of supramolecular systems SO NATURE MATERIALS LA English DT Article ID NANOFIBERS; PATHWAY; CELL; NANOSTRUCTURES; POLYMERIZATION; BIOACTIVITY; PEPTIDES; MICELLES; MATRIX; GELS AB By means of two supramolecular systems-peptide amphiphiles engaged in hydrogen-bonded beta-sheets, and chromophore amphiphiles driven to assemble by pi-orbital overlaps-we show that the minima in the energy landscapes of supramolecular systems are defined by electrostatic repulsion and the ability of the dominant attractive forces to trap molecules in thermodynamically unfavourable configurations. These competing interactions can be selectively switched on and off, with the order of doing so determining the position of the final product in the energy landscape. Within the same energy landscape, the peptide-amphiphile system forms a thermodynamically favoured product characterized by long bundled fibres that promote biological cell adhesion and survival, and a metastable product characterized by short monodisperse fibres that interfere with adhesion and can lead to cell death. Our findings suggest that, in supramolecular systems, functions and energy landscapes are linked, superseding the more traditional connection between molecular design and function. C1 [Tantakitti, Faifan; Boekhoven, Job; Ortony, Julia H.; Newcomb, Christina J.; Palmer, Liam C.; Stupp, Samuel I.] Northwestern Univ, Simpson Querrey Inst BioNanotechnol, 303 East Super St, Chicago, IL 60611 USA. [Tantakitti, Faifan; Wang, Xin; Ortony, Julia H.; Shekhawat, Gajendra S.; de la Cruz, Monica Olvera; Stupp, Samuel I.] Northwestern Univ, Dept Mat Sci & Engn, 2220 Campus Dr, Evanston, IL 60208 USA. [Boekhoven, Job; Kazantsev, Roman V.; Yu, Tao; Zhuang, Ellen; Zandi, Roya; Palmer, Liam C.; de la Cruz, Monica Olvera; Schatz, George C.; Stupp, Samuel I.] Northwestern Univ, Dept Chem, 2220 Campus Dr, Evanston, IL 60208 USA. [Li, Jiahe; de la Cruz, Monica Olvera; Schatz, George C.] Dept Chem & Biol Engn, 2145 Sheridan Rd, Evanston, IL 60208 USA. [de la Cruz, Monica Olvera] Northwestern Univ, Dept Phys & Astron, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Stupp, Samuel I.] Northwestern Univ, Dept Biomed Engn, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Stupp, Samuel I.] Northwestern Univ, Dept Med, 251 East Huron St, Chicago, IL 60611 USA. [Boekhoven, Job] Tech Univ Munich, Inst Adv Study, Lichtenbergstr 2A, D-85748 Garching, Germany. [Boekhoven, Job] Tech Univ Munich, Dept Chem, Lichtenbergstr 2A, D-85748 Garching, Germany. [Newcomb, Christina J.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. RP Stupp, SI (reprint author), Northwestern Univ, Simpson Querrey Inst BioNanotechnol, 303 East Super St, Chicago, IL 60611 USA.; Stupp, SI (reprint author), Northwestern Univ, Dept Mat Sci & Engn, 2220 Campus Dr, Evanston, IL 60208 USA.; Stupp, SI (reprint author), Northwestern Univ, Dept Chem, 2220 Campus Dr, Evanston, IL 60208 USA.; Stupp, SI (reprint author), Northwestern Univ, Dept Biomed Engn, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Stupp, SI (reprint author), Northwestern Univ, Dept Med, 251 East Huron St, Chicago, IL 60611 USA. EM s-stupp@northwestern.edu RI Stupp, Samuel/B-6737-2009; Wang, Xin /J-7089-2014; Palmer, Liam/E-2975-2010; OI Wang, Xin /0000-0001-8358-3536; Palmer, Liam/0000-0003-0804-1168; Boekhoven, Job/0000-0002-9126-2430 FU Center for Bio-Inspired Energy Sciences (CBES), an Energy Frontiers Research Center (EFRC) - US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0000989]; National Institutes of Health NIDCR grant [R01DE015920]; Rubicon Fellowship of the Netherlands Organisation for Scientific Research (NWO); Royal Thai Government scholarship; Northwestern University Bioscientist Program; Northwestern University Office for Research FX Synthesis of PAs, their morphological assessments, MD simulations and free energy calculations were supported by the Center for Bio-Inspired Energy Sciences (CBES), an Energy Frontiers Research Center (EFRC) funded by the US Department of Energy, Office of Science, Office of Basic Energy Sciences under award number DE-SC0000989. The biological studies were supported by National Institutes of Health NIDCR grant (R01DE015920). J.B., F.T. and J.L. are grateful for support by a Rubicon Fellowship of the Netherlands Organisation for Scientific Research (NWO), the Royal Thai Government scholarship and the Northwestern University Bioscientist Program, respectively. We acknowledge the following core facilities at Northwestern University: the Peptide Synthesis Core at the Simpson Querrey Institute for BioNanotechnology, the Biological Imaging Facility (supported by the Northwestern University Office for Research), the Center for Advanced Microscopy (NCI CCSG P30 CA060553), Keck Biophysics Facility, the EPIC, SPID facility (NUANCE Center- NSF DMR-1121262 and NSF EEC-0647560). The authors thank M. Seniw for help with graphics. NR 35 TC 19 Z9 19 U1 39 U2 101 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 1476-1122 EI 1476-4660 J9 NAT MATER JI Nat. Mater. PD APR PY 2016 VL 15 IS 4 BP 469 EP + DI 10.1038/NMAT4538 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA DH2CL UT WOS:000372591700024 PM 26779883 ER PT J AU Stephens, J Fierro, A Beeson, S Laity, G Trienekens, D Joshi, RP Dickens, J Neuber, A AF Stephens, J. Fierro, A. Beeson, S. Laity, G. Trienekens, D. Joshi, R. P. Dickens, J. Neuber, A. TI Photoionization capable, extreme and vacuum ultraviolet emission in developing low temperature plasmas in air SO PLASMA SOURCES SCIENCE & TECHNOLOGY LA English DT Article DE low temperature plasma; streamer; photoionization; spectroscopy; VUV; EUV; breakdown ID DIELECTRIC SURFACE FLASHOVER; ELECTRON-IMPACT; CROSS-SECTIONS; ATMOSPHERIC CONDITIONS; STREAMER PROPAGATION; OSCILLATOR-STRENGTH; WAVELENGTH REGION; MEDIUM-RESOLUTION; N-2; ABSORPTION AB Experimental observation of photoionization capable extreme ultraviolet and vacuum ultraviolet emission from nanosecond timescale, developing low temperature plasmas (i.e. streamer discharges) in atmospheric air is presented. Applying short high voltage pulses enabled the observation of the onset of plasma formation exclusively by removing the external excitation before spark development was achieved. Contrary to the common assumption that radiative transitions from the b(1)Pi(u) (Birge-Hopfield I) and b'(1)Sigma(+)(u) (Birge-Hopfield II) singlet states of N-2 are the primary contributors to photoionization events, these results indicate that radiative transitions from the c'(1)(4)Sigma(+)(u) (Carroll-Yoshino) singlet state of N-2 are dominant in developing low temperature plasmas in air. In addition to c'(4) transitions, photoionization capable transitions from atomic and singly ionized atomic oxygen were also observed. The inclusion of c'(1)(4)Sigma(+)(u) transitions into a statistical photoionization model coupled with a fluid model enabled streamer growth in the simulation of positive streamers. C1 [Stephens, J.; Fierro, A.; Beeson, S.; Laity, G.; Trienekens, D.; Joshi, R. P.; Dickens, J.; Neuber, A.] Texas Tech Univ, Ctr Pulsed Power & Power Elect, Lubbock, TX 79407 USA. [Fierro, A.; Laity, G.] Sandia Natl Labs, Albuquerque, NM 87123 USA. [Beeson, S.] Air Force Res Lab, Kirtland AFB, NM 87117 USA. [Trienekens, D.] Eindhoven Univ Technol, Elementary Proc Gas Discharges, POB 513, NL-5600 MB Eindhoven, Netherlands. RP Neuber, A (reprint author), Texas Tech Univ, Ctr Pulsed Power & Power Elect, Lubbock, TX 79407 USA. EM andreas.neuber@ttu.edu RI Dickens, James/H-5993-2016 FU AT&T Professorship in ECE at Texas Tech University; SMART scholarship; Dutch Technology Foundation STW [12119] FX This work was partially funded by the AT&T Professorship in ECE at Texas Tech University. Author (S.B.) was supported by the SMART scholarship and author (DT) was supported by project 12119 of the Dutch Technology Foundation STW. NR 81 TC 0 Z9 0 U1 3 U2 8 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0963-0252 EI 1361-6595 J9 PLASMA SOURCES SCI T JI Plasma Sources Sci. Technol. PD APR PY 2016 VL 25 IS 2 AR 025024 DI 10.1088/0963-0252/25/2/025024 PG 11 WC Physics, Fluids & Plasmas SC Physics GA DG8MI UT WOS:000372337900026 ER PT J AU Greene, GL Geltenbort, P AF Greene, Geoffrey L. Geltenbort, Peter TI the neutron enigma SO SCIENTIFIC AMERICAN LA English DT Article C1 [Greene, Geoffrey L.] Univ Tennessee, Phys, Knoxville, TN 37996 USA. [Greene, Geoffrey L.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN USA. [Geltenbort, Peter] Inst Laue Langevin, Grenoble, France. RP Greene, GL (reprint author), Univ Tennessee, Phys, Knoxville, TN 37996 USA. NR 0 TC 0 Z9 0 U1 2 U2 5 PU NATURE PUBLISHING GROUP PI NEW YORK PA 75 VARICK ST, 9TH FLR, NEW YORK, NY 10013-1917 USA SN 0036-8733 J9 SCI AM JI Sci.Am. PD APR PY 2016 VL 314 IS 4 BP 37 EP 41 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH0NX UT WOS:000372482000025 ER PT J AU D'Elia, M Gunzburger, M AF D'Elia, M. Gunzburger, M. TI Identification of the Diffusion Parameter in Nonlocal Steady Diffusion Problems SO APPLIED MATHEMATICS AND OPTIMIZATION LA English DT Article DE Nonlocal diffusion; Nonlocal operator; Fractional operator; Vector calculus; Control theory; Optimization; Parameter estimation; Finite element methods ID SYMMETRIC JUMP-PROCESSES; BOUNDARY-VALUE-PROBLEMS; LONG-RANGE FORCES; PERIDYNAMIC MODELS; VECTOR CALCULUS; APPROXIMATION; EQUATIONS; DYNAMICS AB The problem of identifying the diffusion parameter appearing in a nonlocal steady diffusion equation is considered. The identification problem is formulated as an optimal control problem having a matching functional as the objective of the control and the parameter function as the control variable. The analysis makes use of a nonlocal vector calculus that allows one to define a variational formulation of the nonlocal problem. In a manner analogous to the local partial differential equations counterpart, we demonstrate, for certain kernel functions, the existence of at least one optimal solution in the space of admissible parameters. We introduce a Galerkin finite element discretization of the optimal control problem and derive a priori error estimates for the approximate state and control variables. Using one-dimensional numerical experiments, we illustrate the theoretical results and show that by using nonlocal models it is possible to estimate non-smooth and discontinuous diffusion parameters. C1 [D'Elia, M.; Gunzburger, M.] Florida State Univ, Dirac Sci Lib 400, Tallahassee, FL 32306 USA. [D'Elia, M.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP D'Elia, M (reprint author), Florida State Univ, Dirac Sci Lib 400, Tallahassee, FL 32306 USA.; D'Elia, M (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM mdelia@fsu.edu FU US National Science Foundation [DMS-1315259] FX This work was supported in part by the US National Science Foundation Grant DMS-1315259. NR 42 TC 1 Z9 1 U1 1 U2 8 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0095-4616 EI 1432-0606 J9 APPL MATH OPT JI Appl. Math. Optim. PD APR PY 2016 VL 73 IS 2 BP 227 EP 249 DI 10.1007/s00245-015-9300-x PG 23 WC Mathematics, Applied SC Mathematics GA DG7HH UT WOS:000372254900002 ER PT J AU Buchko, GW Perkins, A Parsonage, D Poole, LB Karplus, PA AF Buchko, Garry W. Perkins, Arden Parsonage, Derek Poole, Leslie B. Karplus, P. Andrew TI Backbone chemical shift assignments for Xanthomonas campestris peroxiredoxin Q in the reduced and oxidized states: a dramatic change in backbone dynamics SO BIOMOLECULAR NMR ASSIGNMENTS LA English DT Article DE Plant diseases; Peroxidase; Drug design; Conformational change ID CATALYSIS AB Peroxiredoxins (Prx) are ubiquitous enzymes that reduce peroxides as part of antioxidant defenses and redox signaling. While Prx catalytic activity and sensitivity to hyperoxidative inactivation depend on their dynamic properties, there are few examples where their dynamics has been characterized by NMR spectroscopy. Here, we provide a foundation for studies of the solution properties of peroxiredoxin Q from the plant pathogen Xanthomonas campestris (XcPrxQ) by assigning the observable H-1(N), N-15, C-13(alpha), C-13(beta), and C-13' chemical shifts for both the reduced (dithiol) and oxidized (disulfide) states. In the reduced state, most of the backbone amide resonances (149/152, 98 %) can be assigned in the XcPrxQ H-1-N-15 HSQC spectrum. In contrast, a remarkable 51 % (77) of these amide resonances are not visible in the H-1-N-15 HSQC spectrum of the disulfide state of the enzyme, indicating a substantial change in backbone dynamics associated with the formation of an intramolecular C48-C84 disulfide bond. C1 [Buchko, Garry W.] Pacific NW Natl Lab, Earth & Biol Sci Directorate, Richland, WA 99352 USA. [Perkins, Arden; Karplus, P. Andrew] Oregon State Univ, Dept Biochem & Biophys, Corvallis, OR 97331 USA. [Parsonage, Derek; Poole, Leslie B.] Wake Forest Sch Med, Dept Biochem, Winston Salem, NC 27157 USA. RP Buchko, GW (reprint author), Pacific NW Natl Lab, Earth & Biol Sci Directorate, Richland, WA 99352 USA.; Karplus, PA (reprint author), Oregon State Univ, Dept Biochem & Biophys, Corvallis, OR 97331 USA. EM garry.buchko@pnnl.gov; karplusp@science.oregonstate.edu RI Buchko, Garry/G-6173-2015 OI Buchko, Garry/0000-0002-3639-1061 FU National Institute of Health [GM050389]; US Department of Energy's Office of Biological and Environmental Research (BER) program FX This research was supported by the National Institute of Health R01 Grant number GM050389 (LBP and PAK). Part of this research was performed at the W.R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility located at Pacific Northwest National Laboratory (PNNL) and sponsored by US Department of Energy's Office of Biological and Environmental Research (BER) program. Battelle operates PNNL for the US Department of Energy. NR 13 TC 0 Z9 0 U1 0 U2 1 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1874-2718 EI 1874-270X J9 BIOMOL NMR ASSIGN JI Biomol. NMR Assign. PD APR PY 2016 VL 10 IS 1 BP 57 EP 61 DI 10.1007/s12104-015-9637-8 PG 5 WC Biophysics; Spectroscopy SC Biophysics; Spectroscopy GA DG6WX UT WOS:000372227900011 PM 26438558 ER PT J AU Zhang, F Hager, R Ku, SH Chang, CS Jardin, SC Ferraro, NM Seol, ES Yoon, E Shephard, MS AF Zhang, Fan Hager, Robert Ku, Seung-Hoe Chang, Choong-Seock Jardin, Stephen C. Ferraro, Nathaniel M. Seol, E. Seegyoung Yoon, Eisung Shephard, Mark S. TI Mesh generation for confined fusion plasma simulation SO ENGINEERING WITH COMPUTERS LA English DT Article DE Geometric model; Automatic mesh generation; Tokamak fusion reactor ID FINITE-ELEMENT; ADAPTATION AB XGC1 and M3D-C (1) are two fusion plasma simulation codes being developed at Princeton Plasma Physics Laboratory. XGC1 uses the particle-in-cell method to simulate gyrokinetic neoclassical physics and turbulence (Chang et al. Phys Plasmas 16(5):056108, 2009; Ku et al. Nucl Fusion 49:115021, 2009; Admas et al. J Phys 180(1):012036, 2009). M3D- solves the two-fluid resistive magnetohydrodynamic equations with the finite elements (Jardin J comput phys 200(1):133-152, 2004; Jardin et al. J comput Phys 226(2):2146-2174, 2007; Ferraro and Jardin J comput Phys 228(20):7742-7770, 2009; Jardin J comput Phys 231(3):832-838, 2012; Jardin et al. Comput Sci Discov 5(1):014002, 2012; Ferraro et al. Sci Discov Adv Comput, 2012; Ferraro et al. International sherwood fusion theory conference, 2014). This paper presents the software tools and libraries that were combined to form the geometry and automatic meshing procedures for these codes. Specific consideration has been given to satisfy the mesh configuration and element shape quality constraints of XGC1 and M3D-C-1. C1 [Zhang, Fan; Seol, E. Seegyoung; Yoon, Eisung; Shephard, Mark S.] Rensselaer Polytech Inst, Sci Computat Res Ctr, Troy, NY 12180 USA. [Hager, Robert; Ku, Seung-Hoe; Chang, Choong-Seock; Jardin, Stephen C.] Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. [Ferraro, Nathaniel M.] Gen Atom Co, San Diego, CA 92121 USA. RP Seol, ES (reprint author), Rensselaer Polytech Inst, Sci Computat Res Ctr, Troy, NY 12180 USA. EM seols@rpi.edu RI Ku, Seung-Hoe/D-2315-2009 OI Ku, Seung-Hoe/0000-0002-9964-1208 FU U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences and Office of Advanced Scientific Computing Research [DE-SC0008449, DE-SC0006618, DE-SC0006617] FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences and Office of Advanced Scientific Computing Research under Award Numbers DE-SC0008449 (Partnership for Edge Physics Simulations), DE-SC0006618 (Center for Extended Magnetohydrodynamic Modeling), and DE-SC0006617 (Frameworks, Algorithms, and Scalable Technologies for Mathematics). NR 28 TC 1 Z9 1 U1 2 U2 9 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0177-0667 EI 1435-5663 J9 ENG COMPUT-GERMANY JI Eng. Comput. PD APR PY 2016 VL 32 IS 2 BP 285 EP 293 DI 10.1007/s00366-015-0417-y PG 9 WC Computer Science, Interdisciplinary Applications; Engineering, Mechanical SC Computer Science; Engineering GA DG7WM UT WOS:000372294400008 ER PT J AU Hansen, GA Xavier, PG Mish, SP Voth, TE Heinstein, MW Glass, MW AF Hansen, Glen A. Xavier, Patrick G. Mish, Sam P. Voth, Thomas E. Heinstein, Martin W. Glass, Micheal W. TI An MPI plus X implementation of contact global search using Kokkos SO ENGINEERING WITH COMPUTERS LA English DT Article DE Partial differential equations; Finite element analysis; Contact problems; Spatial searching ID PARALLEL; ALGORITHM; PATTERNS; GPUS AB This paper describes an approach that seeks to parallelize the spatial search associated with computational contact mechanics. In contact mechanics, the purpose of the spatial search is to find "nearest neighbors," which is the prelude to an imprinting search that resolves the interactions between the external surfaces of contacting bodies. In particular, we are interested in the contact global search portion of the spatial search associated with this operation on domain-decomposition-based meshes. Specifically, we describe an implementation that combines standard domain-decomposition-based MPI-parallel spatial search with thread-level parallelism (MPI-X) available on advanced computer architectures (those with GPU coprocessors). Our goal is to demonstrate the efficacy of the MPI-X paradigm in the overall contact search. Standard MPI-parallel implementations typically use a domain decomposition of the external surfaces of bodies within the domain in an attempt to efficiently distribute computational work. This decomposition may or may not be the same as the volume decomposition associated with the host physics. The parallel contact global search phase is then employed to find and distribute surface entities (nodes and faces) that are needed to compute contact constraints between entities owned by different MPI ranks without further inter-rank communication. Key steps of the contact global search include computing bounding boxes, building surface entity (node and face) search trees and finding and distributing entities required to complete on-rank (local) spatial searches. To enable source-code portability and performance across a variety of different computer architectures, we implemented the algorithm using the Kokkos hardware abstraction library. While we targeted development towards machines with a GPU accelerator per MPI rank, we also report performance results for OpenMP with a conventional multi-core compute node per rank. Results here demonstrate a 47 % decrease in the time spent within the global search algorithm, comparing the reference ACME algorithm with the GPU implementation, on an 18M face problem using four MPI ranks. While further work remains to maximize performance on the GPU, this result illustrates the potential of the proposed implementation. C1 [Hansen, Glen A.; Voth, Thomas E.] Sandia Natl Labs, Computat Multiphys Dept 1443, POB 5800, Albuquerque, NM 87185 USA. [Xavier, Patrick G.; Mish, Sam P.] Sandia Natl Labs, Simulat Modeling Sci Dept 1543, POB 5800, Albuquerque, NM 87185 USA. [Heinstein, Martin W.] Sandia Natl Labs, Computat Solid Mech & Struct Dynam Dept 1542, POB 5800, Albuquerque, NM 87185 USA. [Glass, Micheal W.] Sandia Natl Labs, Computat Simulat Infrastruct Dept 1545, POB 5800, Albuquerque, NM 87185 USA. RP Hansen, GA (reprint author), Sandia Natl Labs, Computat Multiphys Dept 1443, POB 5800, Albuquerque, NM 87185 USA. EM gahanse@sandia.gov OI Hansen, Glen/0000-0002-1786-9285 FU U.S. Department of Energy through NNSA Advanced Scientific Computing (ASC) Integrated Codes (IC) program; Lockheed Martin Corporation; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was funded by the U.S. Department of Energy through the NNSA Advanced Scientific Computing (ASC) Integrated Codes (IC) program. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The authors would like to thank Tero Karras of NVIDIA Corporation for his CUDA code and suggestions. NR 35 TC 0 Z9 0 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0177-0667 EI 1435-5663 J9 ENG COMPUT-GERMANY JI Eng. Comput. PD APR PY 2016 VL 32 IS 2 BP 295 EP 311 DI 10.1007/s00366-015-0418-x PG 17 WC Computer Science, Interdisciplinary Applications; Engineering, Mechanical SC Computer Science; Engineering GA DG7WM UT WOS:000372294400009 ER PT J AU Rood, AS Sondrup, AJ Ritter, PD AF Rood, Arthur S. Sondrup, A. Jeffrey Ritter, Paul D. TI QUANTITATIVE EVALUATION OF AN AIR-MONITORING NETWORK USING ATMOSPHERIC TRANSPORT MODELING AND FREQUENCY OF DETECTION METHODS SO HEALTH PHYSICS LA English DT Article DE air sampling; modeling; dose assessment; modeling; meteorological; monitoring; air ID VALIDATION AB A methodology has been developed to quantify the performance of an air-monitoring network in terms of frequency of detection. Frequency of detection is defined as the fraction of events that result in a detection at either a single sampler or network of samplers. An event is defined as a release to the atmosphere of a specified amount of activity over a finite duration that begins on a given day and hour of the year. The methodology uses an atmospheric transport model to predict air concentrations of radionuclides at the samplers for a given release time and duration. Another metric of interest determined by the methodology is called the network intensity, which is defined as the fraction of samplers in the network that have a positive detection for a given event. The frequency of detection methodology allows for evaluation of short-term releases that include effects of short-term variability in meteorological conditions. The methodology was tested using the U.S. Department of Energy Idaho National Laboratory Site ambient air-monitoring network consisting of 37 low-volume air samplers in 31 different locations covering a 17,630 km(2) region. Releases from six major facilities distributed over an area of 1,435 km(2) were modeled and included three stack sources and eight ground-level sources. A Lagrangian Puff air dispersion model (CALPUFF) was used to model atmospheric transport. The model was validated using historical Sb-125 releases and measurements. Relevant 1-wk release quantities from each emission source were calculated based on a dose of 1.9x10(-4) mSv at a public receptor (0.01 mSv assuming release persists over a year). Important radionuclides were Am-241, Cs-137, Pu-238, Pu-239, Sr-90, and tritium. Results show the detection frequency was over 97.5% for the entire network considering all sources and radionuclides. Network intensity results ranged from 3.75% to 62.7%. Evaluation of individual samplers indicated some samplers were poorly located and added little to the overall effectiveness of the network. Using the frequency of detection methods, alternative sampler placements were simulated that could substantially improve the performance and efficiency of the network. C1 [Rood, Arthur S.] K Spar Inc, 4835 W Foxtrail Lane, Idaho Falls, ID 83402 USA. [Sondrup, A. Jeffrey] Idaho Natl Lab, Idaho Falls, ID USA. [Ritter, Paul D.] Bechtel BWTX Idaho LLC, Idaho Falls, ID USA. RP Rood, AS (reprint author), K Spar Inc, 4835 W Foxtrail Lane, Idaho Falls, ID 83402 USA. EM asr@kspar.com NR 23 TC 0 Z9 0 U1 1 U2 3 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0017-9078 EI 1538-5159 J9 HEALTH PHYS JI Health Phys. PD APR PY 2016 VL 110 IS 4 BP 311 EP 327 DI 10.1097/HP.0000000000000466 PG 17 WC Environmental Sciences; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA DG1MZ UT WOS:000371833500001 PM 26910025 ER PT J AU Strom, DJ AF Strom, Daniel J. TI Why We Need Nuclear Power. SO HEALTH PHYSICS LA English DT Book Review C1 [Strom, Daniel J.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Strom, DJ (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. NR 1 TC 0 Z9 0 U1 3 U2 3 PU LIPPINCOTT WILLIAMS & WILKINS PI PHILADELPHIA PA TWO COMMERCE SQ, 2001 MARKET ST, PHILADELPHIA, PA 19103 USA SN 0017-9078 EI 1538-5159 J9 HEALTH PHYS JI Health Phys. PD APR PY 2016 VL 110 IS 4 BP 395 EP 395 DI 10.1097/HP.0000000000000455 PG 1 WC Environmental Sciences; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Nuclear Science & Technology; Radiology, Nuclear Medicine & Medical Imaging GA DG1MZ UT WOS:000371833500009 ER PT J AU Brunet, JPL Li, L Karpyn, ZT Huerta, NJ AF Brunet, Jean-Patrick Leopold Li, Li Karpyn, Zuleima T. Huerta, Nicolas J. TI Fracture opening or self-sealing: Critical residence time as a unifying parameter for cement-CO2-brine interactions SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Well integrity; Carbon storage; Reactive transport modeling; Cement fracture alteration; CO2 leakage ID GEOLOGIC SEQUESTRATION CONDITIONS; CARBONATED BRINE; CO2-RICH BRINE; WELL CEMENT; CO2 LEAKAGE; HYDROTHERMAL SYSTEMS; REACTIVE FLOW; DISSOLUTION; MODEL; INTEGRITY AB Understanding long-term property evolution of cement fractures is essential for assessing well integrity during geological carbon sequestration (GCS). Cement fractures represent preferential leakage pathways in abandoned wells upon exposure to CO2-rich fluid. Contrasting self-sealing and fracture opening behavior have been observed while a unifying framework is still missing. Here we developed a process-based reactive transport model that explicitly simulates flow and multi-component reactive transport in fractured cement by reproducing experimental observation of sharp flow rate reduction during exposure to carbonated water. The simulation shows similar reaction network as in diffusion-controlled systems without flow. That is, the CO2-rich water accelerates the portlandite dissolution, releasing calcium that further reacted with carbonate to form calcite. The calibrated model was used for CO2-flooding numerical experiments in 250 cement fractures with varying initial hydraulic aperture (b) and residence time (tau) defined as the ratio of fracture volume over flow rate. A long tau leads to slow replenishment of carbonated water, calcite precipitation, and self-sealing. The opposite occurs when tau is small with short fracture and fast flow rates. Simulation results indicate a critical residence time tau(c) the minimum tau required for self-sealing - divides the conditions that trigger the opening and self-sealing behavior. The tau(c) value depends on the initial aperture size through tau(c) = 9.8 x 10(-4) x b(2) + 0.254 x b.Among the 250 numerical experiments, significant changes in effective permeability - self-healing or opening - typically occur within hours to a day, thus providing supporting argument for the extrapolation of short-term laboratory observation (hours to months) to long-term prediction at relevant GCS time scales (years to hundreds of years). (C) 2016 Elsevier Ltd. All rights reserved. C1 [Brunet, Jean-Patrick Leopold; Li, Li; Karpyn, Zuleima T.] Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA. [Li, Li; Karpyn, Zuleima T.] Penn State Univ, EMS Energy Inst, University Pk, PA 16802 USA. [Li, Li] Penn State Univ, Earth & Environm Syst Inst, University Pk, PA 16802 USA. [Huerta, Nicolas J.] US DOE, Natl Energy Technol Lab, Albany, OR 97321 USA. RP Li, L (reprint author), Penn State Univ, John & Willie Leone Family Dept Energy & Mineral, University Pk, PA 16802 USA.; Li, L (reprint author), Penn State Univ, EMS Energy Inst, University Pk, PA 16802 USA.; Li, L (reprint author), Penn State Univ, Earth & Environm Syst Inst, University Pk, PA 16802 USA. EM lili@eme.psu.edu RI Li, Li/A-6077-2008 OI Li, Li/0000-0002-1641-3710 FU National Energy Technology Laboratory (NETL), U.S. Department of Energy, an agency of the United States Government [RES1000026]; URS Energy and Construction, Inc. FX This project was funded by the National Energy Technology Laboratory (NETL), U.S. Department of Energy, an agency of the United States Government, through a support contract through Project RES1000026 with URS Energy and Construction, Inc. We acknowledge the stimulating discussions with Brian Strazisar in early stage of the project that has helped formulate the idea. We appreciate the careful and insightful reviews from two anonymous reviewers and the associate editor Susan Carroll. NR 66 TC 4 Z9 4 U1 3 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD APR PY 2016 VL 47 BP 25 EP 37 DI 10.1016/j.ijggc.2016.01.024 PG 13 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DG3SB UT WOS:000371989100004 ER PT J AU Szecsody, JE Zhong, LR Vermeul, VR McKinley, JP Bowden, M Williams, MD Eisenhauer, E AF Szecsody, Jim E. Zhong, Lirong Vermeul, Vince R. McKinley, James P. Bowden, Mark Williams, Mark D. Eisenhauer, Emalee TI Laboratory study of the influence of scCO(2) injection on metals migration, precipitation, and microbial growth SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Carbon storage; Saline aquifer; Mineral dissolution-precipitation; Microbial growth; Particulate movement ID GEOLOGICAL CARBON SEQUESTRATION; CO2 STORAGE; SALINE AQUIFERS; POROUS-MEDIA; REACTIVE TRANSPORT; SUPERCRITICAL CO2; ROCK INTERACTIONS; TRACE-ELEMENTS; POWER-PLANTS; DEGREES-C AB Laboratory experiments were conducted to evaluate the impact of supercritical carbon dioxide (scCO(2)) injection on aqueous and solid phase geochemistry, and subsequent changes in permeability. These experiments showed that brine displacement from the Mount Simon Sandstone cores (similar to 1200m depth) by scCO(2) was inefficient by advection, because the low viscosity scCO(2) flows predominantly in larger pores, leaving a significant amount of brine in smaller pores. Acidification caused by scCO2 injection resulted in significant increases in Mg2+, Na+, SO42- Al3+, and silica concentrations are likely from differing rates of carbonate, clay, albite, and K-feldspar dissolution. The mass of precipitates that formed over 1.2 years (NaCl, KCl, lead oxide, and forsterite) was small, as observed by electron microprobe analysis and did not influence permeability. Trace metals that increased during scCO(2) injection included Ba, Mn, Sr, Ni, Sn, Bi, Cu, Li, P, and Zn, and trace metals that decreased included Hg, Pb, and Co. The scCO(2) injection experiments also showed a moderate amount of particulate (iron oxide) movement correlated with the fraction of scCO2, but the sandstone permeability did not change, even after substantial (i.e., 115 pore volumes) scCO2 injection. Anaerobic and aerobic microbial growth was observed (23 and 14 times, respectively) correlated with higher scCO(2) concentration, but the calculated change in pore space occupied by the increase in biomass is insignificant. The small observed geochemical and microbial changes are not expected to reduce the ability to inject scCO(2) into the reservoir, but significant increases in trace metal concentrations could magnify the water quality impact of a potential leak of reservoir fluids into an overlying aquifer. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Szecsody, Jim E.; Zhong, Lirong; Vermeul, Vince R.; McKinley, James P.; Bowden, Mark; Williams, Mark D.; Eisenhauer, Emalee] Pacific NW Natl Lab, POB 999,K3-61,K7-73,K8-96,K8-73,K3-62, Richland, WA 99354 USA. RP Szecsody, JE (reprint author), Pacific NW Natl Lab, POB 999,K3-61,K7-73,K8-96,K8-73,K3-62, Richland, WA 99354 USA. EM jim.szecsody@pnnl.gov; lirong.zhong@pnnl.gov; vince.vermeul@pnnl.gov; james.mckiniey@pnnl.gov; Mark.Bowden@pnnl.gov; mark.d.williams@pnnl.gov; emalee.eisenhauer@pnnl.gov FU FutureGen Industrial Alliance, Inc. (Alliance); U.S. Department of Energy (DOE); U.S. DOE [DE-AC06-76RL0 1830] FX Funding of this research was provided by the FutureGen Industrial Alliance, Inc. (Alliance) and the U.S. Department of Energy (DOE). The FutureGen 2.0 Project is implemented under Cooperative Agreement DE-FE0001882 between the U.S. Department of Energy and the Alliance. The Alliance is a non-profit membership organization created to benefit the public interest and the interests of science through research, development, and demonstration of near-zero emissions coal technology. The Pacific Northwest National Laboratory is operated by Battelle for the U.S. DOE under Contract DE-AC06-76RL0 1830. NR 60 TC 0 Z9 0 U1 4 U2 11 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD APR PY 2016 VL 47 BP 71 EP 85 DI 10.1016/j.ijggc.2016.01.029 PG 15 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DG3SB UT WOS:000371989100008 ER PT J AU Yonkofski, CMR Gastelum, JA Porter, EA Rodriguez, LR Bacon, DH Brown, CF AF Yonkofski, Catherine M. R. Gastelum, Jason A. Porter, Ellen A. Rodriguez, Luke R. Bacon, Diana H. Brown, Christopher F. TI An optimization approach to design monitoring schemes for CO2 leakage detection SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE CO2 storage; Carbon capture and sequestration; CO2 leakage detection; Monitoring verification and accounting; MVA; Monitoring systems design; Risk and uncertainty ID CARBON SEQUESTRATION; WELL PLACEMENT; AQUIFERS AB This paper demonstrates an approach to identify optimal monitoring designs that minimize the time to first detection of CO2 leakage from a subsurface storage formation. This research is part of the National Risk Assessment Partnership (NRAP), a DOE project tasked with conducting risk and uncertainty analysis in the areas of reservoir performance, natural leakage pathways, wellbore integrity, groundwater protection, monitoring, and systems level modeling. Our approach applies a simulated annealing algorithm that searches the solution space by iteratively mutating potential monitoring designs. A user-defined leakage signature based on change from initial conditions is implemented to infer CO2 leakage had occurred. An example application was performed to demonstrate the effectiveness and efficiency of this method compared to an exhaustive search of the entire solution space. We accounted for uncertainty in the example by evaluating the performance of potential monitoring designs across a set of simulated leakage realizations. The example application approached the optimal time to leakage detection in a few minutes using a standard workstation, which was several orders of magnitude faster than an exhaustive search of the solution space, thus exhibiting efficiency and effectiveness. A user-friendly tool, DREAM (Designs for Risk Evaluation and Management), is being developed for use on personal computers to make this method accessible to stakeholders, regulators, and researchers. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Yonkofski, Catherine M. R.; Gastelum, Jason A.; Porter, Ellen A.; Rodriguez, Luke R.; Bacon, Diana H.; Brown, Christopher F.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Yonkofski, CMR (reprint author), Pacific NW Natl Lab, Battelle Seattle Res Ctr, 1100 Dexter Ave N,Suite 400, Seattle, WA 98109 USA. EM catherine.yonkofski@pnnl.gov FU U.S. Department of Energy (DOE) [AC05-76RL01830] FX PNNL is operated by Battelle for the U.S. Department of Energy (DOE) under Contract DE-AC05-76RL01830. This research is part of the National Risk Assessment Partnership, an initiative within DOE's Office of Fossil Energy. NR 20 TC 1 Z9 1 U1 1 U2 5 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD APR PY 2016 VL 47 BP 233 EP 239 DI 10.1016/j.ijggc.2016.01.040 PG 7 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DG3SB UT WOS:000371989100020 ER PT J AU Kirk, MF Altman, SJ Santillan, EFU Bennett, PC AF Kirk, Matthew F. Altman, Susan J. Santillan, Eugenio-Felipe U. Bennett, Philip C. TI Interplay between microorganisms and geochemistry in geological carbon storage SO INTERNATIONAL JOURNAL OF GREENHOUSE GAS CONTROL LA English DT Article DE Carbon trapping; Porous media; Subsurface microbiology; Bioenergetics; Capnophile; Bioreactor experiments ID HIGH-PRESSURE; GEOBACILLUS-STEAROTHERMOPHILUS; MICROBIAL DIVERSITY; SUPERCRITICAL CO2; CALCIUM-CARBONATE; SALINE AQUIFERS; DEEP SUBSURFACE; WATER-QUALITY; DIOXIDE; INACTIVATION AB Researchers at the Center for Frontiers of Subsurface Energy Security (CFSES) have conducted laboratory and modeling studies to better understand the interplay between microorganisms and geochemistry for geological carbon storage (GCS). We provide evidence of microorganisms adapting to high pressure CO2 conditions and identify factors that may influence survival of cells to CO2 stress. Factors that influenced the ability of cells to survive exposure to high-pressure CO2 in our experiments include mineralogy, the permeability of cell walls and/or membranes, intracellular buffering capacity, and whether cells live planktonically or within biofilm. Column experiments show that, following exposure to acidic water, biomass can remain intact in porous media and continue to alter hydraulic conductivity. Our research also shows that geochemical changes triggered by CO2 injection can alter energy available to populations of subsurface anaerobes and that microbial feedbacks on this effect can influence carbon storage. Our research documents the impact of CO2 on microorganisms and in turn, how subsurface microorganisms can influence GCS. We conclude that microbial presence and activities can have important implications for carbon storage and that microorganisms should not be overlooked in further GCS research. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Kirk, Matthew F.] Kansas State Univ, Dept Geol, Manhattan, KS 66506 USA. [Altman, Susan J.] Sandia Natl Labs, Dept Geochem, Albuquerque, NM 87185 USA. [Santillan, Eugenio-Felipe U.; Bennett, Philip C.] Univ Texas Austin, Dept Geol Sci, Jackson Sch Geosci, Austin, TX USA. [Santillan, Eugenio-Felipe U.] Smithsonian Environm Res Ctr, POB 28, Edgewater, MD 21037 USA. RP Altman, SJ (reprint author), Sandia Natl Labs, POB 5800 MS0754, Albuquerque, NM 87185 USA. EM sjaltma@sandia.gov FU Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001114]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This material is based upon work supported as part of the Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001114. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. Matthew Kirk conducted the laboratory and modeling work presented in this paper while at Sandia National Laboratories. NR 83 TC 1 Z9 1 U1 6 U2 13 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1750-5836 EI 1878-0148 J9 INT J GREENH GAS CON JI Int. J. Greenh. Gas Control PD APR PY 2016 VL 47 BP 386 EP 395 DI 10.1016/j.ijggc.2016.01.041 PG 10 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels; Engineering, Environmental SC Science & Technology - Other Topics; Energy & Fuels; Engineering GA DG3SB UT WOS:000371989100034 ER PT J AU Hu, JZ Xu, SC Kwak, JH Hu, MY Wan, C Zhao, ZC Szanyi, J Bao, XH Han, XW Wang, Y Peden, CHF AF Hu, Jian Zhi Xu, Suochang Kwak, Ja Hun Hu, Mary Y. Wan, Chuan Zhao, Zhenchao Szanyi, Janos Bao, Xinhe Han, Xiuwen Wang, Yong Peden, Charles H. F. TI High field Al-27 MAS NMR and TPD studies of active sites in ethanol dehydration using thermally treated transitional aluminas as catalysts SO JOURNAL OF CATALYSIS LA English DT Article DE Penta-coordinated alumina; Al-27 MAS NMR; High magnetic field; TPD ID PENTACOORDINATED AL3+ IONS; GAMMA-ALUMINA; PHASE-TRANSFORMATION; DELTA-ALUMINA; GAMMA-AL2O3; SURFACE; MORPHOLOGY; MECHANISM; SUPPORT; ACIDITY AB High field quantitative Al-27 single pulse (SP) MAS NMR combined with temperature programmed desorption (TPD) of ethanol is used to study the surface of gamma-Al2O3 during phase transformation processes induced by calcination in the temperature range of 500-1300 degrees C. Following ethanol adsorption, ethylene is generated during TPD with a desorption temperature above 200 degrees C. The amount of ethylene decreases monotonically with increasing calcination temperature prior to TPD. Significantly, Al-27 SP MAS NMR reveals that the amount of penta-coordinated Al3+ ions also decreases with increasing calcination temperature. A quantitative (within experimental error) correlation between the amount of penta-coordinated Al3+ ions and the amount of strongly adsorbed ethanol molecules (i.e., the ones that convert to ethylene during TPD) is obtained. These results provide good evidence for a proposal that the penta-coordinated aluminum sites are the catalytic active sites on alumina surfaces during ethanol dehydration reaction across the entire course of gamma-to-alpha Al2O3 phase transformations. (C) 2016 Published by Elsevier Inc. C1 [Hu, Jian Zhi; Xu, Suochang; Kwak, Ja Hun; Hu, Mary Y.; Wan, Chuan; Zhao, Zhenchao; Szanyi, Janos; Peden, Charles H. F.] Pacific NW Natl Lab, Inst Integrated Catalysis Fundamental & Computat, Richland, WA 99354 USA. [Kwak, Ja Hun] UNIST, Ulsan 689798, South Korea. [Xu, Suochang; Bao, Xinhe; Han, Xiuwen] Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China. [Wang, Yong] Washington State Univ, Voiland Sch Chem Engn & Bioengn, Pullman, WA 99163 USA. RP Hu, JZ; Peden, CHF (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis Fundamental & Computat, Richland, WA 99354 USA. EM Jianzhi.Hu@pnnl.gov; Chuck.Peden@pnnl.gov RI Hu, Jian Zhi/F-7126-2012; Wan, Chuan/I-4657-2016 OI Wan, Chuan/0000-0002-8226-7619 FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences; DOE's Office of Biological and Environmental Research; DOE [DE-AC06-76RLO 1830] FX This research was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences. All of the NMR experiments were performed in the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research, and located at Pacific Northwest National Laboratory (PNNL). PNNL is a multi-program national laboratory operated for the DOE by Battelle Memorial Institute under Contract DE-AC06-76RLO 1830. Dr. Ju Feng is acknowledged for assisting with the NMR measurements; Dr. Libor Kovarik and Dr. Mark Bowden are acknowledged for assisting acquiring the XRD data in Fig. 1. NR 40 TC 4 Z9 4 U1 14 U2 37 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9517 EI 1090-2694 J9 J CATAL JI J. Catal. PD APR PY 2016 VL 336 BP 85 EP 93 DI 10.1016/j.jcat.2016.01.006 PG 9 WC Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA DG3BI UT WOS:000371944100009 ER PT J AU Pakhare, D Schwartz, V Abdelsayed, V Haynes, D Shekhawat, D Poston, J Spivey, J AF Pakhare, Devendra Schwartz, Viviane Abdelsayed, Victor Haynes, Daniel Shekhawat, Dushyant Poston, James Spivey, James TI Erratum to "Kinetic and mechanistic study of dry (CO2) reforming of methane over Rh-substituted La2Zr2O7 pyrochlores" (vol 316, pg 78, 2014) SO JOURNAL OF CATALYSIS LA English DT Correction C1 [Pakhare, Devendra; Spivey, James] Louisiana State Univ, Dept Chem Engn, Baton Rouge, LA 70803 USA. [Schwartz, Viviane] Oak Ridge Natl Lab, Dept Energy, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Abdelsayed, Victor; Haynes, Daniel; Shekhawat, Dushyant; Poston, James] US DOE, Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Abdelsayed, Victor] URS Corp, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. RP Spivey, J (reprint author), Louisiana State Univ, Dept Chem Engn, Baton Rouge, LA 70803 USA. EM jjspivey@lsu.edu NR 1 TC 0 Z9 0 U1 8 U2 20 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9517 EI 1090-2694 J9 J CATAL JI J. Catal. PD APR PY 2016 VL 336 BP 135 EP 135 DI 10.1016/j.jcat.2016.02.018 PG 1 WC Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA DG3BI UT WOS:000371944100016 ER PT J AU Ren, JH Tian, Y Hossain, E Connolly, MD AF Ren, Jianhua Tian, Yuan Hossain, Ekram Connolly, Michael D. TI Fragmentation Patterns and Mechanisms of Singly and Doubly Protonated Peptoids Studied by Collision Induced Dissociation SO JOURNAL OF THE AMERICAN SOCIETY FOR MASS SPECTROMETRY LA English DT Article DE Peptoid; N-alkylated glycine; CID; Fragmentation pattern; Protonated; Fragmentation mechanism; Y-ion formation mechanism ID MASS-SPECTROMETRIC CHARACTERISTICS; AROMATIC SIDE-CHAINS; SECONDARY STRUCTURE; PEPTIDE HYBRIDS; NONBIOLOGICAL POLYMER; OLIGOMERS; LIBRARIES; PATHWAYS; GLYCINE; DESIGN AB Peptoids are peptide-mimicking oligomers consisting of N-alkylated glycine units. The fragmentation patterns for six singly and doubly protonated model peptoids were studied via collision-induced dissociation tandem mass spectrometry. The experiments were carried out on a triple quadrupole mass spectrometer with an electrospray ionization source. Both singly and doubly protonated peptoids were found to fragment mainly at the backbone amide bonds to produce peptoid B-type N-terminal fragment ions and Y-type C-terminal fragment ions. However, the relative abundances of B- versus Y-ions were significantly different. The singly protonated peptoids fragmented by producing highly abundant Y-ions and lesser abundant B-ions. The Y-ion formation mechanism was studied through calculating the energetics of truncated peptoid fragment ions using density functional theory and by controlled experiments. The results indicated that Y-ions were likely formed by transferring a proton from the C-H bond of the N-terminal fragments to the secondary amine of the C-terminal fragments. This proton transfer is energetically favored, and is in accord with the observation of abundant Y-ions. The calculations also indicated that doubly protonated peptoids would fragment at an amide bond close to the N-terminus to yield a high abundance of low-mass B-ions and high-mass Y-ions. The results of this study provide further understanding of the mechanisms of peptoid fragmentation and, therefore, are a valuable guide for de novo sequencing of peptoid libraries synthesized via combinatorial chemistry. C1 [Ren, Jianhua; Tian, Yuan; Hossain, Ekram] Univ Pacific, Dept Chem, 3601 Pacific Ave, Stockton, CA 95211 USA. [Connolly, Michael D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Ren, JH (reprint author), Univ Pacific, Dept Chem, 3601 Pacific Ave, Stockton, CA 95211 USA. EM jren@pacific.edu FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [CHE-1301505] FX The authors thank Dr. David Robinson (Sandia National Laboratories) for providing peptoid samples, and Dr. Ronald Zuckermann (The Molecular Foundry, Lawrence Berkeley National Laboratory) for supporting the peptoid synthesis. All peptoids, including deuterium labeled peptoids, were synthesized at the Molecular Foundry. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract no. DE-AC02-05CH11231. J.R. acknowledges the support from the National Science Foundation (CHE-1301505). The authors thank Dr. Patrick Jones (University of the Pacific) for proof-reading the manuscript. All mass spectrometry experiments were conducted at the Chemistry Mass Spectrometry Facility at the University of the Pacific. NR 57 TC 1 Z9 1 U1 2 U2 8 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1044-0305 EI 1879-1123 J9 J AM SOC MASS SPECTR JI J. Am. Soc. Mass Spectrom. PD APR PY 2016 VL 27 IS 4 BP 646 EP 661 DI 10.1007/s13361-016-1341-0 PG 16 WC Biochemical Research Methods; Chemistry, Analytical; Chemistry, Physical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA DG7DT UT WOS:000372245700012 PM 26832347 ER PT J AU Zhang, MQ Groves, R Counce, RM Watson, JS Zawodzinski, TA AF Zhang, Mengqi Groves, Richard Counce, Robert M. Watson, Jack S. Zawodzinski, Thomas A. TI Melting/freezing points of high concentrations of AlCl3 in a saturated chloroaluminate ionic liquid SO JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY LA English DT Article DE Ionic liquids; DSC; AlCl3; Energy storage ID MOLTEN-SALTS; ELECTROCHEMISTRY AB Melting/freezing points of AlCl3 in saturated chloroaluminate ionic liquids [molar ratio 2:1 AlCl3:1-ethyl-3-methyl imidazolium chloride (EMIC)] are measured by differential scanning calorimetry (DSC). A critical range of temperature data (50-130 A degrees C) for AlCl3 dissolution and precipitation from saturated chloroaluminate ionic liquids is obtained. This range of temperature data is of significance to control phase transition of AlCl3 in saturated chloroaluminate ionic liquids. By applying the chloroaluminate ionic liquids to electrolytes for energy storage usage, solid AlCl3 can be partially dissolved and precipitated out during the charging/discharging cycle of energy storage equipment. Therefore, the energy density of the electrolytes is expected to be greatly improved. C1 [Zhang, Mengqi; Counce, Robert M.; Watson, Jack S.; Zawodzinski, Thomas A.] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Groves, Richard] Clean Energy Events, Wilmington, NC 28409 USA. [Zawodzinski, Thomas A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Zhang, MQ (reprint author), Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. EM seventh_zmq@hotmail.com FU NSF [EPS-1004083]; TN-SCORE program FX We thank the TN-SCORE program, NSF EPS-1004083, for funding this work. NR 17 TC 0 Z9 0 U1 6 U2 9 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1388-6150 EI 1572-8943 J9 J THERM ANAL CALORIM JI J. Therm. Anal. Calorim. PD APR PY 2016 VL 124 IS 1 BP 395 EP 398 DI 10.1007/s10973-015-5154-3 PG 4 WC Thermodynamics; Chemistry, Analytical; Chemistry, Physical SC Thermodynamics; Chemistry GA DG7JZ UT WOS:000372261900041 ER PT J AU Guo, Y Lambert, S Wallen, R Errichello, R Keller, J AF Guo, Yi Lambert, Scott Wallen, Robb Errichello, Robert Keller, Jonathan TI Theoretical and experimental study on gear-coupling contact and loads considering misalignment, torque, and friction influences SO MECHANISM AND MACHINE THEORY LA English DT Article DE Gear coupling; Contact; Load; Misalignment; Friction AB A new analytic model addresses the tooth contact and induced loads of gear couplings that are affected by misalignment, torque, and friction. The contact model accounts for Hertzian, bending, and shear deformations of coupling teeth considering crown modifications. For a specified torque and shaft misalignment, the model calculates the number of teeth in contact, tooth load, stiffness, stress, deformation, and safety factors. The tooth load distribution around the circumference compares well with high fidelity finite-element/contact-mechanics analyses. Simulation time with the analytic model is orders of magnitude less. Using the local contact characteristics, the model computes coupling loads that are primarily caused by the disrupted tooth contact and sliding friction caused by axial motions. This analytic model was validated by experiments. The load amplitude depends on the misalignment, torque, and friction. At low torque, coupling motion was induced by the eccentricity between the hub and sleeve even with nearly perfect alignment. This eccentricity was caused by its self-weight. When torque was larger than a threshold, the motion amplitude was greatly reduced. This torque threshold was analytically derived and validated by experiments. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Guo, Yi; Lambert, Scott; Wallen, Robb; Keller, Jonathan] Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. [Errichello, Robert] GEARTECH Townsend, Townsend, MT USA. RP Guo, Y (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM yi.guo@nrel.gov FU U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory; DOE Office of Energy Efficiency and Renewable Energy, Wind and Water Power Technologies Office FX This work was supported by the U.S. Department of Energy under Contract Number DE-AC36-08GO28308 with the National Renewable Energy Laboratory. Funding for the work was provided by the DOE Office of Energy Efficiency and Renewable Energy, Wind and Water Power Technologies Office. NR 26 TC 0 Z9 0 U1 5 U2 12 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0094-114X J9 MECH MACH THEORY JI Mech. Mach. Theory PD APR PY 2016 VL 98 BP 242 EP 262 DI 10.1016/j.mechmachtheory.2015.11.015 PG 21 WC Engineering, Mechanical SC Engineering GA DG2LE UT WOS:000371897800018 ER PT J AU Tu, QC Zhou, XS He, ZL Xue, K Wu, LY Reich, P Hobbie, S Zhou, JZ AF Tu, Qichao Zhou, Xishu He, Zhili Xue, Kai Wu, Liyou Reich, Peter Hobbie, Sarah Zhou, Jizhong TI The Diversity and Co-occurrence Patterns of N-2-Fixing Communities in a CO2-Enriched Grassland Ecosystem SO MICROBIAL ECOLOGY LA English DT Article DE nifH; Soil diazotrophs; Community structure; Co-occurrence patterns; Elevated CO2 ID PROGRESSIVE NITROGEN LIMITATION; ELEVATED CO2; MICROBIAL COMMUNITIES; FOREST PRODUCTIVITY; GENE DIVERSITY; CARBON-DIOXIDE; SOIL; FIXATION; AZOSPIRILLUM; NETWORK AB Diazotrophs are the major organismal group responsible for atmospheric nitrogen (N-2) fixation in natural ecosystems. The extensive diversity and structure of N-2-fixing communities in grassland ecosystems and their responses to increasing atmospheric CO2 remain to be further explored. Through pyrosequencing of nifH gene amplicons and extraction of nifH genes from shotgun metagenomes, coupled with co-occurrence ecological network analysis approaches, we comprehensively analyzed the diazotrophic community in a grassland ecosystem exposed to elevated CO2 (eCO(2)) for 12 years. Long-term eCO(2) increased the abundance of nifH genes but did not change the overall nifH diversity and diazotrophic community structure. Taxonomic and phylogenetic analysis of amplified nifH sequences suggested a high diversity of nifH genes in the soil ecosystem, the majority belonging to nifH clusters I and II. Co-occurrence ecological network analysis identified different co-occurrence patterns for different groups of diazotrophs, such as Azospirillum/Actinobacteria, Mesorhizobium/Conexibacter, and Bradyrhizobium/Acidobacteria. This indicated a potential attraction of non-N-2-fixers by diazotrophs in the soil ecosystem. Interestingly, more complex co-occurrence patterns were found for free-living diazotrophs than commonly known symbiotic diazotrophs, which is consistent with the physical isolation nature of symbiotic diazotrophs from the environment by root nodules. The study provides novel insights into our understanding of the microbial ecology of soil diazotrophs in natural ecosystems. C1 [Tu, Qichao] Zhejiang Univ, Ocean Coll, Dept Marine Sci, Hangzhou 310058, Zhejiang, Peoples R China. [Tu, Qichao; Zhou, Xishu; Zhou, Jizhong] Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA. [Tu, Qichao; Zhou, Xishu; Zhou, Jizhong] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Zhou, Xishu; He, Zhili; Xue, Kai; Wu, Liyou] Cent S Univ, Sch Minerals Proc & Bioengn, Changsha 410083, Hunan, Peoples R China. [Reich, Peter; Hobbie, Sarah] Univ Minnesota, Dept Forest Resources, St Paul, MN 55455 USA. [Reich, Peter] Univ Western Sydney, Hawkesbury Inst Environm, Richmond, NSW 2753, Australia. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. [Zhou, Jizhong] Tsinghua Univ, State Key Joint Lab Environm Simulat & Pollut Con, Sch Environm, Beijing 100084, Peoples R China. RP Zhou, JZ (reprint author), Univ Oklahoma, Inst Environm Genom, Norman, OK 73019 USA.; Zhou, JZ (reprint author), Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA.; Zhou, JZ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA.; Zhou, JZ (reprint author), Tsinghua Univ, State Key Joint Lab Environm Simulat & Pollut Con, Sch Environm, Beijing 100084, Peoples R China. EM jzhou@ou.edu OI Hobbie, Sarah/0000-0001-5159-031X FU U.S. Department of Agriculture through NSF-USDA Microbial Observatories Program [2007-35319-18305]; Department of Energy through Genomics: GTL Foundational Science [DE-SC0004601]; Office of Biological and Environmental Research; National Science Foundation [DEB-0716587, DEB-0620652, DEB-0322057, DEB-0080382]; Cedar Creek Long Term Ecological Research project; BioComplexity project; LTER project; LTREB project [DEB-0716587, DEB-0218039, DEB-0219104, DEB-0217631]; DOE Program for Ecosystem Research; Minnesota Environment and Natural Resources Trust Fund FX We thank James W. Voordeckers for editing this paper. This work is supported by the U.S. Department of Agriculture (project 2007-35319-18305) through the NSF-USDA Microbial Observatories Program, by the Department of Energy under contract DE-SC0004601 through Genomics: GTL Foundational Science, Office of Biological and Environmental Research, and by the National Science Foundation under grants DEB-0716587 and DEB-0620652 as well as grants DEB-0322057, DEB-0080382 (the Cedar Creek Long Term Ecological Research project), DEB-0218039, DEB-0219104, DEB-0217631, and DEB-0716587 (BioComplexity, LTER and LTREB projects), the DOE Program for Ecosystem Research, and the Minnesota Environment and Natural Resources Trust Fund. NR 66 TC 4 Z9 4 U1 17 U2 55 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0095-3628 EI 1432-184X J9 MICROB ECOL JI Microb. Ecol. PD APR PY 2016 VL 71 IS 3 BP 604 EP 615 DI 10.1007/s00248-015-0659-7 PG 12 WC Ecology; Marine & Freshwater Biology; Microbiology SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Microbiology GA DG7LO UT WOS:000372266000009 PM 26280746 ER PT J AU Schreiber, S Vogel, J Schwimmer, HD Marks, SM Schreiber, F Jagust, W AF Schreiber, Stefanie Vogel, Jacob Schwimmer, Henry D. Marks, Shawn M. Schreiber, Frank Jagust, William TI Impact of lifestyle dimensions on brain pathology and cognition SO NEUROBIOLOGY OF AGING LA English DT Article DE Aging; Amyloid; APOE; Hippocampus; PIB ID NORMAL OLDER-ADULTS; ALZHEIMERS-DISEASE; RISK-FACTORS; DEMENTIA; ASSOCIATION; COMPENSATION; INFLAMMATION; POPULATION; DEPOSITION; REGIONS AB Single lifestyle factors affect brain biomarkers and cognition. Here, we addressed the covariance of various lifestyle elements and investigated their impact on positron emission tomography-based beta-amyloid (A beta), hippocampal volume, and cognitive function in aged controls. Lower A beta burden was associated with a lifestyle comprising high cognitive engagement and low vascular risk, particularly in apolipoprotein E epsilon 4 carriers. Although cognitive function was related to high lifetime cognitive engagement and low vascular risk, A beta load had no relation to current cognitive function. The covariance between high adult socioeconomic status, high education, and low smoking prevalence predicted better cognitive function and this was mediated by larger hippocampal volume. Our data show that lifestyle is a complex construct composed of associated variables, some of which reflect factors operating over the life span and others which may be developmental. These factors affect brain health via different pathways, which may reinforce one another. Our findings moreover support the importance of an intellectually enriched lifestyle accompanied by vascular health on both cognition and presumed cerebral mediators of cognitive function. (C) 2016 Elsevier Inc. All rights reserved. C1 [Schreiber, Stefanie; Vogel, Jacob; Schwimmer, Henry D.; Marks, Shawn M.; Jagust, William] Univ Calif Berkeley, Helen Wills Neurosci Inst, 132 Barker Hall, Berkeley, CA 94720 USA. [Schreiber, Stefanie] Otto Von Guericke Univ, Dept Neurol, Magdeburg, Germany. [Schreiber, Stefanie] German Ctr Neurodegenerat Dis DZNE, Magdeburg, Germany. [Schreiber, Frank] Tech Univ Carolo Wilhelmina Braunschweig, Dept Control Engn, D-38106 Braunschweig, Germany. [Jagust, William] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Schreiber, S (reprint author), Univ Calif Berkeley, Helen Wills Neurosci Inst, 132 Barker Hall, Berkeley, CA 94720 USA. EM stefanie.schreiber@med.ovgu.de OI Schwimmer, Henry/0000-0002-6055-6401 FU German Research Foundation (DFG) [SCHR 1418/3-1]; NIH [AG034570] FX This work was supported by a German Research Foundation (DFG) research fellowship (SCHR 1418/3-1) offered to Stefanie Schreiber and NIH grant AG034570. NR 44 TC 0 Z9 0 U1 2 U2 7 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 0197-4580 EI 1558-1497 J9 NEUROBIOL AGING JI Neurobiol. Aging PD APR PY 2016 VL 40 BP 164 EP 172 DI 10.1016/j.neurobiolaging.2016.01.012 PG 9 WC Geriatrics & Gerontology; Neurosciences SC Geriatrics & Gerontology; Neurosciences & Neurology GA DG2OZ UT WOS:000371908400018 PM 26973116 ER PT J AU Lincoln, D AF Lincoln, Don TI The Nature of the Electron SO PHYSICS TEACHER LA English DT Editorial Material C1 [Lincoln, Don] Fermilab Natl Accelerator Lab, Batavia, IL USA. RP Lincoln, D (reprint author), Fermilab Natl Accelerator Lab, Batavia, IL USA. EM lincoln@fnal.gov NR 4 TC 1 Z9 1 U1 1 U2 1 PU AMER ASSN PHYSICS TEACHERS PI COLLEGE PK PA 5110 ROANOKE PLACE SUITE 101, COLLEGE PK, MD 20740 USA SN 0031-921X J9 PHYS TEACH JI Phys. Teach. PD APR PY 2016 VL 54 IS 4 BP 203 EP 208 DI 10.1119/1.4944357 PG 6 WC Physics, Multidisciplinary SC Physics GA DG7SG UT WOS:000372283400006 ER PT J AU Armijo, KM Johnson, J Harrison, RK Thomas, KE Hibbs, M Fresquez, A AF Armijo, Kenneth M. Johnson, Jay Harrison, Richard K. Thomas, Kara E. Hibbs, Michael Fresquez, Armando TI Quantifying photovoltaic fire danger reduction with arc-fault circuit interrupters SO PROGRESS IN PHOTOVOLTAICS LA English DT Article; Proceedings Paper CT 29th European Photovoltaic Solar Energy Conference and Exhibition (EU PVSEC) CY 2014 CL Amsterdam, NETHERLANDS DE arc-fault; PV fire; characterization; modeling; spectroscopy; reliability ID FREE-BURNING ARCS; AIR; TEMPERATURE AB Unmitigated arc-faults present fire dangers, shock hazards, and cause system downtime in photovoltaic (PV) systems. The 2011 National Electrical Code (R) added section 690.11 to require a listed arc-fault protection device on new PV systems. Underwriters Laboratories created the outline of investigation for PV DC arc-fault circuit protection, UL 1699B, for certifying arc-fault circuit interrupters (AFCIs) for arc suppression. Unfortunately, little is known about appropriate trip times for arc-faults generated at different locations in the PV system, with different electrode and polymer encapsulant geometries and materials. In this investigation, a plasma model was developed, which determines fire danger with UL 1699B-listed AFCIs and consequences of arc-fault discharges sustained beyond UL 1699B trip time requirements. This model predicts temperatures for varying system configurations and was validated by 100 and 300W arc-faults experiments where combustion times and temperatures were measured. This investigation then extrapolated burn characteristics using this model to predict polymer ignition times for exposure to arc-power levels between 100 and 1200W. The numerical results indicate AFCI maximum trip times required by UL 1699B are sufficient to suppress 100-1200W arc-faults prior to fire initiation. Optical emission spectroscopy and thermochemical decomposition analysis were also conducted to assess spectral and chemical degradation of the polymer sheath. Published 2014. This article has been contributed to by US Government employees and their work is in the public domain in the USA. C1 [Armijo, Kenneth M.; Johnson, Jay; Harrison, Richard K.; Hibbs, Michael; Fresquez, Armando] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Thomas, Kara E.] George Washington Univ, Dept Chem, 725 21st St NWWA, Washington, DC 20052 USA. RP Armijo, KM (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM kmarmij@sandia.gov NR 32 TC 0 Z9 0 U1 6 U2 6 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 EI 1099-159X J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD APR PY 2016 VL 24 IS 4 BP 507 EP 516 DI 10.1002/pip.2561 PG 10 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA DG2IP UT WOS:000371890900008 ER PT J AU Spataru, SV Sera, D Hacke, P Kerekes, T Teodorescu, R AF Spataru, Sergiu Viorel Sera, Dezso Hacke, Peter Kerekes, Tamas Teodorescu, Remus TI Fault identification in crystalline silicon PV modules by complementary analysis of the light and dark current-voltage characteristics SO PROGRESS IN PHOTOVOLTAICS LA English DT Article; Proceedings Paper CT 29th European Photovoltaic Solar Energy Conference and Exhibition (EU PVSEC) CY 2014 CL Amsterdam, NETHERLANDS DE fault identification; degradation; dark I-V characteristic; series resistance; cell cracks; optical losses; potential-induced degradation ID PHOTOVOLTAIC MODULE; SOLAR-CELLS; DEGRADATION; PERFORMANCE; SYSTEMS; CRACKS AB This article proposes a fault identification method, based on the complementary analysis of the light and dark current-voltage (I-V) characteristics of the photovoltaic (PV) module, to distinguish between four important degradation modes that lead to power loss in PV modules: (i) degradation of the electrical circuit of the PV module (cell interconnect breaks; corrosion of the junction box, module cables, and connectors); (ii) mechanical damage to the solar cells (cell microcracks and fractures); (iii) potential-induced degradation (PID) sustained by the module; and (iv) optical losses affecting the module (soiling, shading, and discoloration). The premise of the proposed method is that different degradation modes affect the light and dark I-V characteristics of the PV module in different ways, leaving distinct signatures. This work focuses on identifying and correlating these specific signatures present in the light and dark I-V measurements to specific degradation modes; a number of new dark I-V diagnostic parameters are proposed to quantify these signatures. The experimental results show that these dark I-V diagnostic parameters, complemented by light I-V performance and series-resistance measurements, can accurately detect and identify the four degradation modes discussed. Copyright (c) 2015 John Wiley & Sons, Ltd. C1 [Spataru, Sergiu Viorel; Sera, Dezso; Kerekes, Tamas; Teodorescu, Remus] Aalborg Univ, Energy Technol, Pontoppidanstr 101, DK-9220 Aalborg, Denmark. [Hacke, Peter] Natl Renewable Energy Lab, 15013 Denver W Pkwy, Golden, CO 80401 USA. RP Spataru, SV (reprint author), Aalborg Univ, Energy Technol, Pontoppidanstr 101, DK-9220 Aalborg, Denmark. EM ssp@et.aau.dk RI Kerekes, Tamas/B-8647-2016; Teodorescu, Remus/O-5224-2015; OI Kerekes, Tamas/0000-0001-7594-3298; Teodorescu, Remus/0000-0002-2617-7168; Sera, Dezso/0000-0001-9050-2423; Spataru, Sergiu/0000-0001-8112-2779 NR 44 TC 0 Z9 0 U1 2 U2 7 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 EI 1099-159X J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD APR PY 2016 VL 24 IS 4 BP 517 EP 532 DI 10.1002/pip.2571 PG 16 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA DG2IP UT WOS:000371890900009 ER PT J AU Fthenakis, V Atia, AA Morin, O Bkayrat, R Sinha, P AF Fthenakis, Vasilis Atia, Adam A. Morin, Olivier Bkayrat, Raed Sinha, Parikhit TI New prospects for PV powered water desalination plants: case studies in Saudi Arabia SO PROGRESS IN PHOTOVOLTAICS LA English DT Article; Proceedings Paper CT 29th European Photovoltaic Solar Energy Conference and Exhibition (EU PVSEC) CY 2014 CL Amsterdam, NETHERLANDS DE photovoltaics; desalination; Middle East; Saudi Arabia; business prospects ID REVERSE-OSMOSIS; OPPORTUNITIES AB Increased water demand and increased drought episodes in the Middle East and other regions necessitate an expansion in desalination projects and create a great market opportunity for photovoltaics (PV). PV-powered desalination has previously been regarded as not being a cost-competitive solution when compared with conventionally powered desalination; however, the decline in PV costs over the last few years has changed this outlook. This paper presents up-to-date performance and cost analysis of reverse osmosis (RO) desalination powered with PV connected to the Saudi Arabian grid. Reference cases include relatively small (i.e., producing 6550m(3) water per day) and large (i.e., 190000m(3)/day) desalination plants using seawater at a salinity of 40000ppm. We used data from a King Abdullah University for Science and Technology presentation and Hybrid Optimization Model for Electric Renewables 2.81 Energy Modeling Software (HOMER Energy LLC) in tandem with Desalination Economic Evaluation Program 4.0 (International Atomic Energy Agency) desalination software to analyze the techno-economic feasibility of these plants. The first phase of our work entailed a comparison between dual-axis high concentration PV (CPV) equipped with triple junction III/V solar cells and CdTe PV-powered RO systems. The estimated levelized cost of electricity from CPV is $0.16/kWh, whereas that from CdTe PV is $0.10/kWh and $0.09/kWh for fixed-tilt and one-axis tracking systems, respectively. These costs are higher than the price of diesel-based grid electricity in the region because diesel fuel is heavily subsidized in Saudi Arabia. In the second phase, we determined the cost of producing desalinated water from the two RO plant sizes powered with CdTe PV. Assuming that the grid acts as zero-loss storage, the total water cost ranges from a high cost of $1.39/m(3) for the small RO plant coupled with latitude-tilt, fixed PV to $0.85/m(3) for the large RO plant coupled with optimally positioned one-axis tracking systems; these PV power plants would displace 1158987 and 33579763l of diesel per year, respectively. Furthermore, the corresponding savings in diesel subsidies enabled by PV are $1.5m and $43.2m per year. Applying these savings to the PV system calls for a levelized cost of electricity of $0.21/kWh, justifying a feed-in-tariff at this level. The avoided CO2 emissions by displacing diesel fuel would be 3115 and 90241tonnes per year for the small and large Photovoltaics Powered Reverse Osmosis Water Desalination (PV-RO) plants, respectively. On the basis of the results of this study, we infer that there are great business prospects associated with large deployment of PV-RO plants in the greater Middle East, and we estimate the reduction in regional CO2 emissions from such deployment. Copyright (c) 2015 John Wiley & Sons, Ltd. C1 [Fthenakis, Vasilis; Atia, Adam A.; Morin, Olivier] Columbia Univ, Ctr Life Cycle Anal, New York, NY USA. [Fthenakis, Vasilis] Brookhaven Natl Lab, Renewable Energy Grp, Upton, NY 11973 USA. [Bkayrat, Raed; Sinha, Parikhit] First Solar Int Middle East, Dubai, U Arab Emirates. RP Fthenakis, V (reprint author), Brookhaven Natl Lab, Ctr PV Environm Res, Upton, NY 11973 USA. EM vmf5@columbia.edu NR 26 TC 3 Z9 3 U1 6 U2 20 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1062-7995 EI 1099-159X J9 PROG PHOTOVOLTAICS JI Prog. Photovoltaics PD APR PY 2016 VL 24 IS 4 BP 543 EP 550 DI 10.1002/pip.2572 PG 8 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA DG2IP UT WOS:000371890900011 ER PT J AU Lasri, K Mahmoud, A Saadoune, I Sougrati, MT Stievano, L Lippens, PE Hermann, RP Ehrenberg, H AF Lasri, Karima Mahmoud, Abdelfattah Saadoune, Ismael Sougrati, Moulay Tahar Stievano, Lorenzo Lippens, Pierre-Emmanuel Hermann, Raphael Pierre Ehrenberg, Helmut TI Toward understanding the lithiation/delithiation process in Fe0.5TiOPO4/C electrode material for lithium-ion batteries SO SOLAR ENERGY MATERIALS AND SOLAR CELLS LA English DT Article; Proceedings Paper CT 2nd International Renewable and Sustainable Energy Conference (IRSEC) CY OCT 17-19, 2014 CL Ouarzazate, MOROCCO SP Mediterranean Space Technol & Innovat DE Lithium-ion batteries; Anode material; Fe0.5TiOPO4; Reaction mechanism; In situ XRD; In situ XANES ID POTASSIUM TITANYL PHOSPHATE; CRYSTAL-GROWTH; ELECTROCHEMICAL PROPERTIES; STRUCTURE REFINEMENT; ANODE MATERIALS; M0.5TIOPO4 M; CAPACITY; FE; NI0.5TIOPO4; INSERTION AB Fe0.5TiOPO4/C composite was used as anode material for LIB and exhibits excellent cycling performance when the electrode is cycled in two different voltage ranges [3.0-13 V] and [3.0-0.02 V] where different insertion mechanisms were involved. A detailed in situ XANES spectroscopy study coupled to the electrochemical analyses, clearly established that the structure of Fe(0.)5TiOPO(4)/C electrode materials is preserved when cycled between 3.0 and 1.3 V. Furthermore, a formation of new phase at the end of first discharge was evidenced, with a reversible capacity of 100 mA h g(-1) after 50 cycles at C/5 rate. At highly lithiated states, [3.0-0.02 V] voltage range, a reduction-decomposition reaction highlights the Li-insertion/extraction behaviors, and low phase crystallinity is observed during cycling, in addition an excellent rate behavior and a reversible capacity of 250 mA h g(-1) can still be maintained after 50 cycles at high cycling rate 5C. (C) 2015 Elsevier E.V. All rights reserved. C1 [Lasri, Karima; Saadoune, Ismael] Cadi Ayyad Univ, FST Marrakech, LCME, BP549,Ave A Khattabi, Marrakech, Morocco. [Mahmoud, Abdelfattah; Hermann, Raphael Pierre] Forschungszentrum Julich, JCNS, D-52425 Julich, Germany. [Mahmoud, Abdelfattah; Hermann, Raphael Pierre] Forschungszentrum Julich, JARA FIT, PGI, D-52425 Julich, Germany. [Saadoune, Ismael] Univ Mohammed VI Polytech, Ctr Adv Mat, Lot 660 Hay Moulay Rachid, Ben Guerir, Morocco. [Sougrati, Moulay Tahar; Stievano, Lorenzo; Lippens, Pierre-Emmanuel] Univ Montpellier, CNRS, UMR 5253, Inst Charles Gerhardt, Pl Eugene Bataillon, F-34095 Montpellier 5, France. [Sougrati, Moulay Tahar; Stievano, Lorenzo; Lippens, Pierre-Emmanuel] FR CNRS 3459, Reseau Stockage Electrochim Energie RS2E, Paris, France. [Hermann, Raphael Pierre] Univ Liege, Fac Sci, B-4000 Liege, Belgium. [Hermann, Raphael Pierre] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Ehrenberg, Helmut] KIT, IAM, Hermann von Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany. RP Mahmoud, A (reprint author), Forschungszentrum Julich, JCNS 2, PGI 4, Leo Brandt Str 1, D-52428 Julich, Germany. EM mahmoudrca@gmail.com RI Ehrenberg, Helmut/M-7090-2013; Hermann, Raphael/F-6257-2013; Sougrati, Moulay Tahar/B-6283-2011 OI Ehrenberg, Helmut/0000-0002-5134-7130; Hermann, Raphael/0000-0002-6138-5624; Sougrati, Moulay Tahar/0000-0003-3740-2807 NR 38 TC 2 Z9 2 U1 9 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0248 EI 1879-3398 J9 SOL ENERG MAT SOL C JI Sol. Energy Mater. Sol. Cells PD APR PY 2016 VL 148 SI SI BP 11 EP 19 DI 10.1016/j.solmat.2015.11.021 PG 9 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA DG3BM UT WOS:000371944500003 ER PT J AU Lin, CY Li, QZ Tunlaya-Anukit, S Shi, R Sun, YH Wang, JP Liu, J Loziuk, P Edmunds, CW Miller, ZD Peszlen, I Muddiman, DC Sederoff, RR Chiang, VL AF Lin, Chien-Yuan Li, Quanzi Tunlaya-Anukit, Sermsawat Shi, Rui Sun, Ying-Hsuan Wang, Jack P. Liu, Jie Loziuk, Philip Edmunds, Charles W. Miller, Zachary D. Peszlen, Ilona Muddiman, David C. Sederoff, Ronald R. Chiang, Vincent L. TI A cell wall-bound anionic peroxidase, PtrPO21, is involved in lignin polymerization in Populus trichocarpa SO TREE GENETICS & GENOMES LA English DT Article DE Lignin polymerization; Populus trichocarpa; Lignin peroxidase; LC-MS/MS; Lignin systems biology ID CINNAMYL-ALCOHOL-DEHYDROGENASE; TRACHEARY ELEMENT DIFFERENTIATION; ANTISENSE DOWN-REGULATION; FERMENTABLE SUGAR YIELDS; MUTANT PINE DEFICIENT; PHASEOLUS-VULGARIS L; SPRUCE PICEA-ABIES; ARABIDOPSIS-THALIANA; MOLECULAR-CLONING; LIGNIFYING XYLEM AB Class III peroxidases are members of a large plant-specific sequence-heterogeneous protein family. Several sequence-conserved homologs have been associated with lignin polymerization in Arabidopsis thaliana, Oryza sativa, Nicotiana tabacum, Zinnia elegans, Picea abies, and Pinus sylvestris. In Populus trichocarpa, a model species for studies of wood formation, the peroxidases involved in lignin biosynthesis have not yet been identified. To do this, we retrieved sequences of all PtrPOs from Peroxibase and conducted RNA-seq to identify candidates. Transcripts from 42 PtrPOs were detected in stem differentiating xylem (SDX) and four of them are the most xylem-abundant (PtrPO12, PtrPO21, PtrPO42, and PtrPO64). PtrPO21 shows xylem-specific expression similar to that of genes encoding the monolignol biosynthetic enzymes. Using protein cleavage-isotope dilution mass spectrometry, PtrPO21 is detected only in the cell wall fraction and not in the soluble fraction. Downregulated transgenics of PtrPO21 have a lignin reduction of similar to 20 % with subunit composition (S/G ratio) similar to wild type. The transgenics show a growth reduction and reddish color of stem wood. The modulus of elasticity (MOE) of the stems of the downregulated PtrPO21-line 8 can be reduced to similar to 60 % of wild type. Differentially expressed gene (DEG) analysis of PtrPO21 downregulated transgenics identified a significant overexpression of PtPrx35, suggesting a compensatory effect within the peroxidase family. No significant changes in the expression of the 49 P. trichocarpa laccases (PtrLACs) were observed. C1 [Lin, Chien-Yuan; Shi, Rui; Wang, Jack P.; Liu, Jie; Sederoff, Ronald R.; Chiang, Vincent L.] N Carolina State Univ, Dept Forestry & Environm Resources, Forest Biotechnol Grp, Raleigh, NC 27695 USA. [Lin, Chien-Yuan] Natl Renewable Energy Lab, Biosci Ctr, Golden, CO 80401 USA. [Li, Quanzi] Chinese Acad Forestry, State Key Lab Tree Genet & Breeding, Beijing 100091, Peoples R China. [Tunlaya-Anukit, Sermsawat] SCG Packaging PLC, 19 Moo 19,Saeng Xuto Rd, Ban Pong 70110, Ratchaburi, Thailand. [Sun, Ying-Hsuan] Natl Chung Hsing Univ, Dept Forestry, Taichung 40227, Taiwan. [Wang, Jack P.; Chiang, Vincent L.] Northeast Forestry Univ, State Key Lab Tree Genet & Breeding, Harbin 150040, Peoples R China. [Loziuk, Philip; Muddiman, David C.] N Carolina State Univ, Dept Chem, WM Keck FTMS Lab, Raleigh, NC 27695 USA. [Edmunds, Charles W.; Miller, Zachary D.; Peszlen, Ilona] N Carolina State Univ, Dept Forest Biomat, Raleigh, NC 27695 USA. RP Sederoff, RR; Chiang, VL (reprint author), N Carolina State Univ, Dept Forestry & Environm Resources, Forest Biotechnol Grp, Raleigh, NC 27695 USA.; Chiang, VL (reprint author), Northeast Forestry Univ, State Key Lab Tree Genet & Breeding, Harbin 150040, Peoples R China. EM ron_sederoff@ncsu.edu; vchiang@ncsu.edu OI Wang, Jack P./0000-0002-5392-0076 FU National Science Foundation (USA), Plant Genome Research Program [DBI-0922391]; NC State University Jordan Family Endowment, NIH/NCSU Molecular Biotechnology Training Program [5T32GM00-8776-08]; NC State University Forest Biotechnology Industrial Research Consortium FX The National Science Foundation (USA), Plant Genome Research Program (Grant DBI-0922391) to V.L.C., the NC State University Jordan Family Endowment, NIH/NCSU Molecular Biotechnology Training Program (Grant 5T32GM00-8776-08), and the NC State University Forest Biotechnology Industrial Research Consortium supported this work. NR 148 TC 0 Z9 0 U1 11 U2 44 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 1614-2942 EI 1614-2950 J9 TREE GENET GENOMES JI Tree Genet. Genomes PD APR PY 2016 VL 12 IS 2 AR 22 DI 10.1007/s11295-016-0978-y PG 18 WC Forestry; Genetics & Heredity; Horticulture SC Forestry; Genetics & Heredity; Agriculture GA DG7NZ UT WOS:000372272300008 ER PT J AU Ichter, B Steele, A Loth, E Moriarty, P Selig, M AF Ichter, Brian Steele, Adam Loth, Eric Moriarty, Patrick Selig, Michael TI A morphing downwind-aligned rotor concept based on a 13-MW wind turbine SO WIND ENERGY LA English DT Article DE wind energy; extreme-scale; turbine; morphing; MoDaR ID DESIGN AB To alleviate the mass-scaling issues associated with conventional upwind rotors of extreme-scale wind turbines (10MW), a morphing downwind-aligned rotor (MoDaR) concept is proposed herein. The concept employs a downwind rotor with blades whose elements are stiff (no intentional flexibility) but with hub-joints that can be unlocked to allow for moment-free downwind alignment. Aligning the combination of gravitational, centrifugal and thrust forces along the blade path reduces downwind cantilever loads, resulting in primarily tensile loading. For control simplicity, the blade curvature can be fixed with a single morphing degree of freedom using a near-hub joint for coning angle: 22 degrees at rated conditions. The conventional baseline was set as the 13.2-MW Sandia 100-m all glass blade in a three-bladed upwind configuration. To quantify potential mass savings, a downwind load-aligning, two-bladed rotor was designed. Because of the reduced number of blades, the MoDaR concept had a favorable 33% mass reduction. The blade reduction and coning led to a reduction in rated power, but morphing increased energy capture at lower speeds such that both the MoDaR and conventional rotors have the same average power: 5.4MW. A finite element analysis showed that quasi-steady structural stresses could be reduced, over a range of operating wind speeds and azimuthal angles, despite the increases in loading per blade. However, the concept feasibility requires additional investigation of the mass, cost and complexity of the morphing hinge, the impact of unsteady aeroelastic influence because of turbulence and off-design conditions, along with system-level Levelized Cost of Energy analysis. Copyright (c) 2015 John Wiley & Sons, Ltd. C1 [Ichter, Brian; Steele, Adam; Loth, Eric] Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. [Moriarty, Patrick] Natl Renewable Energy Lab, Natl Wind Technol Ctr, Golden, CO 80401 USA. [Selig, Michael] Univ Illinois, Dept Aerosp Engn, Urbana, IL 61801 USA. RP Loth, E (reprint author), Univ Virginia, Dept Mech & Aerosp Engn, Charlottesville, VA 22904 USA. EM loth@virginia.edu NR 18 TC 0 Z9 0 U1 3 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1095-4244 EI 1099-1824 J9 WIND ENERGY JI Wind Energy PD APR PY 2016 VL 19 IS 4 BP 625 EP 637 DI 10.1002/we.1855 PG 13 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA DG3XL UT WOS:000372004300004 ER PT J AU Mirocha, JD Simpson, MD Fast, JD Berg, LK Baskett, RL AF Mirocha, J. D. Simpson, M. D. Fast, J. D. Berg, L. K. Baskett, R. L. TI Investigation of boundary-layer wind predictions during nocturnal low-level jet events using the Weather Research and Forecasting model SO WIND ENERGY LA English DT Article DE mesoscale simulation; low-level jet; Weather Research and Forecasting model; Wind Forecast Improvement Project; lidar wind profiler ID SOUTHERN GREAT-PLAINS; LARGE-EDDY SIMULATION; INERTIAL OSCILLATIONS; WRF MODEL; PART I; IMPLEMENTATION; CLIMATOLOGY; TURBULENCE; VERIFICATION; SENSITIVITY AB The accuracy of boundary-layer wind profiles occurring during nocturnal low-level jet (LLJ) events, and their sensitivities to variations of user-specifiable model configuration parameters within the Weather Research and Forecasting model, was investigated. Simulations were compared against data from a wind-profiling lidar, deployed to the Northern Great Plains during the U.S. Department of Energy-supported Weather Forecast Improvement Project. Two periods during the autumn of 2011 featuring LLJs of similar magnitudes and durations occurring during several consecutive nights were selected for analysis. Simulated wind speed and direction at 80 and 180m above the surface, the former a typical wind turbine hub height, bulk vertical gradients between 40 and 120m, a typical rotor span, and the maximum wind speeds occurring at 80 and 180m, and their times of occurrence, were compared with the observations. Sensitivities of these parameters to the horizontal and vertical grid spacing, planetary boundary layer and land surface model physics options, and atmospheric forcing dataset, were assessed using ensembles encompassing changes of each of these configuration parameters. Each simulation captured the diurnal cycle of wind speed and stratification, producing LLJs during each overnight period; however, large discrepancies in relation to the observations were frequently observed, with each ensemble producing a wide range of distributions, reflecting highly variable representations of stratification during the weakly stable overnight conditions. Root mean square error and bias values computed over the LLJ cycle (late evening through the following morning) revealed that, while some configurations performed better or worse in different aspects and at different times, none exhibited definitively superior performance. The considerable root mean square error and bias values, even among the best' performing simulations, underscore the need for improved simulation capabilities for the prediction of near-surface winds during LLJ conditions. Copyright (c) 2015 John Wiley & Sons, Ltd. C1 [Mirocha, J. D.; Simpson, M. D.; Baskett, R. L.] Lawrence Livermore Natl Lab, POB 808,L-103, Livermore, CA 94551 USA. [Fast, J. D.; Berg, L. K.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Mirocha, JD (reprint author), Lawrence Livermore Natl Lab, POB 808,L-103, Livermore, CA 94551 USA. EM jmirocha@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; US DOE Office of Energy Efficiency and Renewable Energy (EERE); EERE at Pacific Northwest National Laboratory (PNNL); DOE [DE-AC06-76RL01830] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under contract DE-AC52-07NA27344 and was supported by the US DOE Office of Energy Efficiency and Renewable Energy (EERE). Jerome Fast and Larry Berg were also supported by EERE at Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for the DOE under contract DE-AC06-76RL01830. NR 51 TC 1 Z9 1 U1 1 U2 6 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1095-4244 EI 1099-1824 J9 WIND ENERGY JI Wind Energy PD APR PY 2016 VL 19 IS 4 BP 739 EP 762 DI 10.1002/we.1862 PG 24 WC Energy & Fuels; Engineering, Mechanical SC Energy & Fuels; Engineering GA DG3XL UT WOS:000372004300011 ER PT J AU Tannenbaum, LV Beasley, JC AF Tannenbaum, Lawrence V. Beasley, James C. TI Validating mammalian resistance to stressor-mediated reproductive impact using rodent sperm analysis SO ECOTOXICOLOGY LA English DT Article DE Reproduction; Sperm; Rodent Sperm Analysis; Ecological risk assessmemt ID METHOXYCHLOR; SPERMATOGENESIS; ATRESIA; RISK; RATS; MICE AB Small rodents from chemically and radiologically contaminated areas on the Savannah River Site, SC were evaluated for sensitive reproductive parameters in a dual purpose study. The primary intent was to observe if established reproductive thresholds-for effect could be exceeded in animals that, due to their restricted home ranges, are maximally exposed to local contamination. Secondarily, validation was sought for a principal element of the Rodent Sperm Analysis method that is used in support of ecological risk assessments for contaminated terrestrial properties. The method's fundamental underlying premise is that during decades of elapsed time between contamination release events and ecological assessments being conducted, rodents develop a resilience to potential stressors, evidenced by their continuing presence. During spring 2014 we collected 89 cotton mice (Peromyscus gossypinus) across three contaminated locations and one reference location, and quantified important male and female reproductive parameters (sperm counts and sperm morphology, and ovarian follicle counts, respectively) and organ weights. The outcome of the comprehensive sperm parameter review, in conjunction with the parallel female reproduction review and other corroborative population and tissue-based information gathered, suggests that mammalian assessments at contaminated sites are unnecessary in the common case. C1 [Tannenbaum, Lawrence V.] Army Publ Hlth Ctr Provis, MCHB IP REH, Bldg 1675,APG EA, Aberdeen, MD 21010 USA. [Beasley, James C.] Univ Georgia, Warnell Sch Forestry & Nat Resources, Savannah River Ecol Lab, PO Drawer E, Aiken, SC 29802 USA. RP Tannenbaum, LV (reprint author), Army Publ Hlth Ctr Provis, MCHB IP REH, Bldg 1675,APG EA, Aberdeen, MD 21010 USA. EM lawrence.v.tannenbaum.civ@mail.mil FU U.S. Army Environmental Command; Department of Energy [DE-FC09-07SR22506] FX This material is based upon work supported by the U.S. Army Environmental Command (Mr. J. Daniel) and the Department of Energy under Award Number DE-FC09-07SR22506 to the University of Georgia Research Foundation. We thank Mr. Lincoln Oliver for his rodent trapping assistance; Pathology Associates, Maryland, Charles River Laboratories (Mr. Fred Les) for their sperm quality analyses; and Dr. Jodi Flaws, Department of Comparative Biosciences, University of Illinois, for her ovarian follicle analyses. The manuscript review assistance of Jeffrey Leach and Sherri Hutchens is greatly appreciated. NR 26 TC 0 Z9 0 U1 0 U2 2 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0963-9292 EI 1573-3017 J9 ECOTOXICOLOGY JI Ecotoxicology PD APR PY 2016 VL 25 IS 3 BP 584 EP 593 DI 10.1007/s10646-016-1617-y PG 10 WC Ecology; Environmental Sciences; Toxicology SC Environmental Sciences & Ecology; Toxicology GA DF8WA UT WOS:000371640000016 PM 26879951 ER PT J AU You, ST Hadley, SW Shankar, M Liu, YL AF You, Shutang Hadley, Stanton W. Shankar, Mallikarjun Liu, Yilu TI Co-optimizing generation and transmission expansion with wind power in large-scale power grids-Implementation in the US Eastern Interconnection SO ELECTRIC POWER SYSTEMS RESEARCH LA English DT Article DE Generation and transmission co-optimized expansion; Wind power; Multiple regions; Scenario creation; Mixed-integer programming (MIP) ID PSO BASED APPROACH; NSGA-II ALGORITHM; PLANNING PROBLEM; MULTIOBJECTIVE MODEL; TRANSPORTATION MODEL; ELECTRICITY MARKETS; PART I; SYSTEMS; UNCERTAINTIES; DEMAND AB This paper studies the generation and transmission expansion co-optimization problem with a high wind power penetration rate in large-scale power grids. In this paper, generation and transmission expansion co-optimization is modelled as a mixed-integer programming (MIP) problem. A scenario creation method is proposed to capture the variation and correlation of both load and wind power across regions for large-scale power grids. Obtained scenarios that represent load and wind uncertainties can be easily introduced into the MIP problem and then solved to obtain the co-optimized generation and transmission expansion plan. Simulation results show that the proposed planning model and the scenario creation method can improve the expansion result significantly through modelling more detailed information of wind and load variation amongregions in the US El system. The improved expansion plan that combines generation and transmission will aid system planners and policy makers to maximize the social welfare in large-scale power grids. (C) 2015 Elsevier B.V. All rights reserved. C1 [You, Shutang; Liu, Yilu] Univ Tennessee, Knoxville, TN 37996 USA. [Hadley, Stanton W.; Shankar, Mallikarjun; Liu, Yilu] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP You, ST (reprint author), Univ Tennessee, Knoxville, TN 37996 USA. EM syou3@utk.edu FU U.S. Department of Energy; Engineering Research Center Program of the U.S. National Science Foundation under NSF [EEC-1041877]; CURENT Industry Partnership Program FX This work was supported primarily by the U.S. Department of Energy. This work was also supported by the Engineering Research Center Program of the U.S. National Science Foundation under NSF Award Number EEC-1041877 and the CURENT Industry Partnership Program. In addition, the authors would like to thank reviewers for their constructive comments on this paper. NR 49 TC 3 Z9 3 U1 2 U2 4 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0378-7796 EI 1873-2046 J9 ELECTR POW SYST RES JI Electr. Power Syst. Res. PD APR PY 2016 VL 133 BP 209 EP 218 DI 10.1016/j.epsr.2015.12.023 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA DF2RM UT WOS:000371191500024 ER PT J AU Liu, LL Wang, X Lajeunesse, MJ Miao, GF Piao, SL Wan, SQ Wu, YX Wang, ZH Yang, S Li, P Deng, MF AF Liu, Lingli Wang, Xin Lajeunesse, Marc J. Miao, Guofang Piao, Shilong Wan, Shiqiang Wu, Yuxin Wang, Zhenhua Yang, Sen Li, Ping Deng, Meifeng TI A cross-biome synthesis of soil respiration and its determinants under simulated precipitation changes SO GLOBAL CHANGE BIOLOGY LA English DT Article DE apparent Q(10); aridity index; drought; meta-analysis; precipitation regime; soil moisture; soil temperature; wet ID CLIMATE-CHANGE; TERRESTRIAL ECOSYSTEMS; MANIPULATION EXPERIMENTS; TEMPERATURE SENSITIVITY; GRASSLAND ECOSYSTEM; SEMIARID GRASSLAND; CO2 EFFLUX; RESPONSES; PULSES; METAANALYSIS AB Soil respiration (R-s) is the second-largest terrestrial carbon (C) flux. Although R-s has been extensively studied across a broad range of biomes, there is surprisingly little consensus on how the spatiotemporal patterns of R-s will be altered in a warming climate with changing precipitation regimes. Here, we present a global synthesis R-s data from studies that have manipulated precipitation in the field by collating studies from 113 increased precipitation treatments, 91 decreased precipitation treatments, and 14 prolonged drought treatments. Our meta-analysis indicated that when the increased precipitation treatments were normalized to 28% above the ambient level, the soil moisture, R-s,R- and the temperature sensitivity (Q(10)) values increased by an average of 17%, 16%, and 6%, respectively, and the soil temperature decreased by -1.3%. The greatest increases in R-s and Q(10) were observed in arid areas, and the stimulation rates decreased with increases in climate humidity. When the decreased precipitation treatments were normalized to 28% below the ambient level, the soil moisture and R-s values decreased by an average of -14% and -17%, respectively, and the soil temperature and Q(10) values were not altered. The reductions in soil moisture tended to be greater in more humid areas. Prolonged drought without alterations in the amount of precipitation reduced the soil moisture and R-s by -12% and -6%, respectively, but did not alter Q(10). Overall, our synthesis suggests that soil moisture and R-s tend to be more sensitive to increased precipitation in more arid areas and more responsive to decreased precipitation in more humid areas. The responses of R-s and Q(10) were predominantly driven by precipitation-induced changes in the soil moisture, whereas changes in the soil temperature had limited impacts. Finally, our synthesis of prolonged drought experiments also emphasizes the importance of the timing and frequency of precipitation events on ecosystem C cycles. Given these findings, we urge future studies to focus on manipulating the frequency, intensity, and seasonality of precipitation with an aim to improving our ability to predict and model feedback between R-s and climate change. C1 [Liu, Lingli; Wang, Xin; Wang, Zhenhua; Yang, Sen; Li, Ping; Deng, Meifeng] Chinese Acad Sci, State Key Lab Vegetat & Environm Change, Inst Bot, Beijing 100093, Peoples R China. [Wang, Xin; Wang, Zhenhua; Yang, Sen; Li, Ping; Deng, Meifeng] Univ Chinese Acad Sci, Beijing 100049, Peoples R China. [Lajeunesse, Marc J.] Univ S Florida, Dept Integrat Biol, Tampa, FL 33620 USA. [Miao, Guofang] N Carolina State Univ, Dept Forestry & Environm Resources, Raleigh, NC 27659 USA. [Piao, Shilong] Peking Univ, Dept Ecol, Coll Urban & Environm Sci, Beijing 100871, Peoples R China. [Wan, Shiqiang] Henan Univ, State Key Lab Cotton Biol, Key Lab Plant Stress Biol, Coll Life Sci, Kaifeng 475004, Henan, Peoples R China. [Wu, Yuxin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Liu, LL (reprint author), Chinese Acad Sci, State Key Lab Vegetat & Environm Change, Inst Bot, Beijing 100093, Peoples R China. EM lingli.liu@ibcas.ac.cn RI Wan, Shiqiang/B-5799-2009; Liu, Lingli/A-7771-2008; Wu, Yuxin/G-1630-2012 OI Liu, Lingli/0000-0002-5696-3151; Wu, Yuxin/0000-0002-6953-0179 FU Chinese National Key Development Program for Basic Research [2013CB956304, 2014CB954003]; National Natural Science Foundation of China [31522011]; National Science Foundation (USA) [DEB-1451031]; National 1000 Young Talents Program FX The authors would like to thank anonymous reviewers for their thoughtful comments. This study was supported financially by Chinese National Key Development Program for Basic Research (2013CB956304, 2014CB954003), the National Natural Science Foundation of China (31522011), the National Science Foundation (USA) to M.J.L. (DEB-1451031), and National 1000 Young Talents Program. NR 39 TC 4 Z9 4 U1 47 U2 133 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1354-1013 EI 1365-2486 J9 GLOBAL CHANGE BIOL JI Glob. Change Biol. PD APR PY 2016 VL 22 IS 4 BP 1394 EP 1405 DI 10.1111/gcb.13156 PG 12 WC Biodiversity Conservation; Ecology; Environmental Sciences SC Biodiversity & Conservation; Environmental Sciences & Ecology GA DF7CN UT WOS:000371515300007 PM 26554753 ER PT J AU Spasojevic, MJ Bahlai, CA Bradley, BA Butterfield, BJ Tuanmu, MN Sistla, S Wiederholt, R Suding, KN AF Spasojevic, Marko J. Bahlai, Christie A. Bradley, Bethany A. Butterfield, Bradley J. Tuanmu, Mao-Ning Sistla, Seeta Wiederholt, Ruscena Suding, Katharine N. TI Scaling up the diversity-resilience relationship with traitdatabases and remote sensing data: the recovery ofproductivity after wildfire SO GLOBAL CHANGE BIOLOGY LA English DT Article DE fire resistance; fire tolerance; functional diversity; Landfire; MODIS; NatureServe; path analysis; resprout ability; seed mass; southwest United States ID PLANT-SPECIES RICHNESS; FUNCTIONAL DIVERSITY; ECOLOGICAL RESILIENCE; RESPONSE DIVERSITY; INTRASPECIFIC VARIABILITY; ENVIRONMENTAL-CHANGE; CLIMATIC GRADIENTS; COMMUNITY ECOLOGY; ECOSYSTEM HEALTH; LANDSCAPE-SCALE AB Understanding the mechanisms underlying ecosystem resilience - why some systems have an irreversible response to disturbances while others recover - is critical for conserving biodiversity and ecosystem function in the face of global change. Despite the widespread acceptance of a positive relationship between biodiversity and resilience, empirical evidence for this relationship remains fairly limited in scope and localized in scale. Assessing resilience at the large landscape and regional scales most relevant to land management and conservation practices has been limited by the ability to measure both diversity and resilience over large spatial scales. Here, we combined tools used in large-scale studies of biodiversity (remote sensing and trait databases) with theoretical advances developed from small-scale experiments to ask whether the functional diversity within a range of woodland and forest ecosystems influences the recovery of productivity after wildfires across the four-corner region of the United States. We additionally asked how environmental variation (topography, macroclimate) across this geographic region influences such resilience, either directly or indirectly via changes in functional diversity. Using path analysis, we found that functional diversity in regeneration traits (fire tolerance, fire resistance, resprout ability) was a stronger predictor of the recovery of productivity after wildfire than the functional diversity of seed mass or species richness. Moreover, slope, elevation, and aspect either directly or indirectly influenced the recovery of productivity, likely via their effect on microclimate, while macroclimate had no direct or indirect effects. Our study provides some of the first direct empirical evidence for functional diversity increasing resilience at large spatial scales. Our approach highlights the power of combining theory based on local-scale studies with tools used in studies at large spatial scales and trait databases to understand pressing environmental issues. C1 [Spasojevic, Marko J.] Washington Univ, Dept Biol, St Louis, MO 63130 USA. [Spasojevic, Marko J.] Washington Univ, Tyson Res Ctr, St Louis, MO 63130 USA. [Bahlai, Christie A.] Michigan State Univ, Dept Entomol, E Lansing, MI 48915 USA. [Bahlai, Christie A.] Michigan State Univ, Great Lakes Bioenergy Res Ctr, E Lansing, MI 48915 USA. [Bradley, Bethany A.] Univ Massachusetts, Dept Environm Conservat, Amherst, MA 01003 USA. [Butterfield, Bradley J.] No Arizona Univ, Dept Biol Sci, Flagstaff, AZ 86011 USA. [Butterfield, Bradley J.] No Arizona Univ, Merriam Powell Ctr Environm Res, Flagstaff, AZ 86011 USA. [Tuanmu, Mao-Ning] Yale Univ, Dept Ecol & Evolutionary Biol, New Haven, CT 06520 USA. [Sistla, Seeta] Univ Calif Irvine, Dept Ecol & Evolutionary Biol, Irvine, CA 92697 USA. [Wiederholt, Ruscena] Univ Arizona, Sch Nat Resources & Environm, Tucson, AZ 85721 USA. [Suding, Katharine N.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. RP Spasojevic, MJ (reprint author), Washington Univ, Dept Biol, St Louis, MO 63130 USA.; Spasojevic, MJ (reprint author), Washington Univ, Tyson Res Ctr, St Louis, MO 63130 USA. EM mspaso@gmail.com OI Bahlai, Christie/0000-0002-8937-8709 NR 90 TC 2 Z9 2 U1 27 U2 68 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1354-1013 EI 1365-2486 J9 GLOBAL CHANGE BIOL JI Glob. Change Biol. PD APR PY 2016 VL 22 IS 4 BP 1421 EP 1432 DI 10.1111/gcb.13174 PG 12 WC Biodiversity Conservation; Ecology; Environmental Sciences SC Biodiversity & Conservation; Environmental Sciences & Ecology GA DF7CN UT WOS:000371515300009 PM 26599833 ER PT J AU Yang, JY He, YJ Aubrey, DP Zhuang, QL Teskey, RO AF Yang, Jinyan He, Yujie Aubrey, Doug P. Zhuang, Qianlai Teskey, Robert O. TI Global patterns and predictors of stem CO2 efflux in forest ecosystems SO GLOBAL CHANGE BIOLOGY LA English DT Article DE gross primary production; leaf area index; respiration; root CO2 efflux; stem CO2 efflux ID GROSS PRIMARY PRODUCTION; NET PRIMARY PRODUCTION; ANNUAL CARBON COST; LEAF-AREA INDEX; SOIL RESPIRATION; MAINTENANCE RESPIRATION; AUTOTROPHIC RESPIRATION; CONSTANT FRACTION; RAIN-FORESTS; TREE STEMS AB Stem CO2 efflux (E-S) plays an important role in the carbon balance of forest ecosystems. However, its primary controls at the global scale are poorly understood and observation-based global estimates are lacking. We synthesized data from 121 published studies across global forest ecosystems and examined the relationships between annual E-S and biotic and abiotic factors at individual, biome, and global scales, and developed a global gridded estimate of annual E-S. We tested the following hypotheses: (1) Leaf area index (LAI) will be highly correlated with annual E-S at biome and global scales; (2) there will be parallel patterns in stem and root CO2 effluxes (R-A) in all forests; (3) annual E-S will decline with forest age; and (4) LAI coupled with mean annual temperature (MAT) and mean annual precipitation (MAP) will be sufficient to predict annual E-S across forests in different regions. Positive linear relationships were found between E-S and LAI, as well as gross primary production (GPP), net primary production (NPP), wood NPP, soil CO2 efflux (R-S), and R-A. Annual E-S was correlated with R-A in temperate forests after controlling for GPP and MAT, suggesting other additional factors contributed to the relationship. Annual E-S tended to decrease with stand age. Leaf area index, MAT and MAP, predicted 74% of variation in E-S at global scales. Our statistical model estimated a global annual E-S of 6.7 +/- 1.1PgCyr(-1) over the period of 2000-2012 with little interannual variability. Modeled mean annual E-S was 71 +/- 43, 270 +/- 103, and 420 +/- 134gCm(2)yr(-1) for boreal, temperate, and tropical forests, respectively. We recommend that future studies report E-S at a standardized constant temperature, incorporate more manipulative treatments, such as fertilization and drought, and whenever possible, simultaneously measure both aboveground and belowground CO2 fluxes. C1 [Yang, Jinyan; Aubrey, Doug P.; Teskey, Robert O.] Univ Georgia, Warnell Sch Forestry & Nat Resources, Athens, GA 30602 USA. [He, Yujie; Zhuang, Qianlai] Purdue Univ, Dept Earth Atmospher & Planetary Sci, W Lafayette, IN 47907 USA. [He, Yujie] Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA 92697 USA. [Aubrey, Doug P.] Univ Georgia, Savannah River Ecol Lab, Aiken, SC 29802 USA. [Zhuang, Qianlai] Purdue Univ, Dept Agron, W Lafayette, IN 47907 USA. RP Yang, JY (reprint author), Univ Georgia, Warnell Sch Forestry & Nat Resources, Athens, GA 30602 USA. EM yangjy@uga.edu RI He, Yujie/E-2514-2017 OI He, Yujie/0000-0001-8261-5399 FU PINEMAP; USDA National Institute of Food and Agriculture [2011-68002-30185]; NSF Division of Information AMP; Intelligent Systems project [NSF-1028291] FX We thank Dr. Jeffrey Dukes and Dr. Chris A. Maier for their constructive comments on an earlier version of the manuscript. We also thank two anonymous reviewers' constructive comments. We thank all site investigators and their funding agencies, whose support was essential for this meta-analysis. This study was supported by PINEMAP, a coordinated Agricultural Project funded by the USDA National Institute of Food and Agriculture (#2011-68002-30185). This study was also partially supported by a NSF Division of Information & Intelligent Systems project (NSF-1028291). NR 67 TC 0 Z9 0 U1 11 U2 36 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1354-1013 EI 1365-2486 J9 GLOBAL CHANGE BIOL JI Glob. Change Biol. PD APR PY 2016 VL 22 IS 4 BP 1433 EP 1444 DI 10.1111/gcb.13188 PG 12 WC Biodiversity Conservation; Ecology; Environmental Sciences SC Biodiversity & Conservation; Environmental Sciences & Ecology GA DF7CN UT WOS:000371515300010 PM 26667780 ER PT J AU Fedorov, SS Rohatgi, US Barsukov, IV Gubynskyi, MV Barsukov, MG Wells, BS Livitan, MV Gogotsi, OG AF Fedorov, Sergiy S. Rohatgi, Upendra Singh Barsukov, Igor V. Gubynskyi, Mykhailo V. Barsukov, Michelle G. Wells, Brian S. Livitan, Mykola V. Gogotsi, Oleksiy G. TI Ultrahigh-Temperature Continuous Reactors Based on Electrothermal Fluidized Bed Concept SO JOURNAL OF FLUIDS ENGINEERING-TRANSACTIONS OF THE ASME LA English DT Article; Proceedings Paper CT 15th International Symposium on Gas-Particle Flows to the Memory of Professor Clayton T. Crowe CY AUG, 2014 CL Chicago, IL ID CARBONS AB Authors introduce an ultrahigh-temperature (i.e., 2500-3000 degrees C) continuous fluidized bed furnace, in which the key operating variable is specific electrical resistance of the bed. A correlation has been established to predict the specific electrical resistance for the natural graphite-based precursors. Fluid dynamics models have been validated with the data from a fully functional prototype reactor. Data collected demonstrated that the difference between the calculated and measured values of specific resistance is approximately 25%; due to chaotic nature of electrothermal fluidized bed processes, this discrepancy was deemed acceptable. Optimizations proposed allow producing natural graphite-based end product with the purity level of 99.98+wt.%C for battery markets. C1 [Fedorov, Sergiy S.; Gubynskyi, Mykhailo V.; Livitan, Mykola V.] Natl Met Acad Ukraine, UA-49600 Dnepropetrovsk, Ukraine. [Rohatgi, Upendra Singh] Brookhaven Natl Lab, Mem ASME, Upton, NY 11973 USA. [Barsukov, Igor V.; Barsukov, Michelle G.; Wells, Brian S.] Amer Energy Technol Co, Arlington Hts, IL 60004 USA. [Gogotsi, Oleksiy G.] Mat Res Ctr Ltd, UA-03680 Kiev, Ukraine. RP Barsukov, IV (reprint author), Amer Energy Technol Co, Arlington Hts, IL 60004 USA. EM fedorov.pte@gmail.com; rohatgi@bnl.gov; ibarsukov@usaenergytech.com; gubinm58@gmail.com; Michelle.Barsukov@usaenergytech.com; Brian.Wells@usaenergytech.com; nvlivitan@gmail.com; alex@dom.ua RI Gogotsi, Oleksiy/M-8937-2015 OI Gogotsi, Oleksiy/0000-0002-3173-4432 FU U.S. Department of Energy, NNSA under the Global Initiatives for Proliferation Prevention [BNL-T2-372-UA, STCU-P482]; Dr. Joseph E. Doninger of Dontech Global, Inc., in Lake Forest, IL FX Dr. Rohatgi has submitted this paper in honor of Professor Clayton Crowe. The support for Dr. Rohatgi and team from Ukraine came from the U.S. Department of Energy, NNSA under the Global Initiatives for Proliferation Prevention ( Project Nos. BNL-T2-372-UA and STCU-P482). The support on various stages of this project from Dr. Joseph E. Doninger of Dontech Global, Inc., in Lake Forest, IL, is greatly appreciated. Additionally, we would like to acknowledge scientific contributions by the engineering group represented by Leonid M. Usatiuk, Vitaliy I. Lutsenko, Yaroslav O. Tyrygin, Konstantyn A. Nikitenko, and Vadim Yu. Pisarenko of M. K. Yangel Special Design Bureau "Yuzhnoe" in Dniepropetrovsk, Ukraine who took part in this project. Author I. B. submits this work in an eternal memoriam of Mr. Wesley Krueger of South Holland, IL, whose dogged persistence, technical acumen, and deep understanding of electrothermal fluidized bed reactors for carbon refining made this technology viable in the marketplace. This paper also recognizes contributions of many colleagues from Ukraine. NR 42 TC 0 Z9 0 U1 1 U2 4 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0098-2202 EI 1528-901X J9 J FLUID ENG-T ASME JI J. Fluids Eng.-Trans. ASME PD APR PY 2016 VL 138 IS 4 SI SI AR 044502 DI 10.1115/1.4031689 PG 11 WC Engineering, Mechanical SC Engineering GA DF9WT UT WOS:000371713800012 ER PT J AU Aughterson, RD Lumpkin, GR de los Reyes, M Gault, B Baldo, P Ryan, E Whittle, KR Smith, KL Cairney, JM AF Aughterson, R. D. Lumpkin, G. R. de los Reyes, M. Gault, B. Baldo, P. Ryan, E. Whittle, K. R. Smith, K. L. Cairney, J. M. TI The influence of crystal structure on ion-irradiation tolerance in the Sm(x)Yb(2-x)TiO5 series SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID INDUCED AMORPHIZATION; ORTHORHOMBIC LN(2)TIO(5); RADIATION TOLERANCE; RESISTANCE; CERAMICS; DAMAGE; PYROCHLORES; TITANATES; DISORDER; LA AB This ion-irradiation study covers the four major crystal structure types in the Ln(2)TiO(5) series (Ln = lanthanide), namely orthorhombic Pnma, hexagonal P63/mmc, cubic (pyrochlore-like) Fd-3m and cubic (fluorite-like) Fm-3m. This is the first systematic examination of the complete Ln(2)TiO(5) crystal system and the first reported examination of the hexagonal structure. A series of samples, based on the stoichiometry Sm(x)Yb(2-x)TiO5 (where x = 2, 1.4, 1, 0.6, and 0) have been irradiated using 1 MeV Kr2+ ions and characterised in-situ using a transmission electron microscope. Two quantities are used to define ion-irradiation tolerance: critical dose of amorphisation (D-c), which is the irradiating ion dose required for a crystalline to amorphous transition, and the critical temperature (T-c), above which the sample cannot be rendered amorphous by ion irradiation. The structure type plus elements of bonding are correlated to ion-irradiation tolerance. The cubic phases, Yb2TiO5 and Sm0.6Yb1.4TiO5, were found to be the most radiation tolerant, with Tc values of 479 and 697 K respectively. The improved radiation tolerance with a change in symmetry to cubic is consistent with previous studies of similar compounds. (C) 2016 Elsevier B.V. All rights reserved. C1 [Aughterson, R. D.; Lumpkin, G. R.; de los Reyes, M.] Australian Nucl Sci & Technol Org, Inst Mat Engn, PMB 1, Menai, NSW 2234, Australia. [Aughterson, R. D.; Cairney, J. M.] Univ Sydney, Australian Ctr Microscopy & Microanal, Sydney, NSW 2006, Australia. [Gault, B.] Univ Oxford, Dept Mat, Parks Rd, Oxford OX1 3PH, England. [Baldo, P.; Ryan, E.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Whittle, K. R.] Univ Liverpool, Sch Engn, Ctr Mat & Struct, Liverpool L69 3GH, Merseyside, England. [Smith, K. L.] Australian Nucl Sci & Technol Org, Govt Int & External Relat, PMB 1, Menai, NSW 2234, Australia. RP Aughterson, RD (reprint author), Australian Nucl Sci & Technol Org, Inst Mat Engn, PMB 1, Menai, NSW 2234, Australia.; Aughterson, RD (reprint author), Univ Sydney, Australian Ctr Microscopy & Microanal, Sydney, NSW 2006, Australia. EM roa@ansto.gov.au RI Lumpkin, Gregory/A-7558-2008; OI Aughterson, Robert/0000-0002-1704-024X; Gault, Baptiste/0000-0002-4934-0458 NR 32 TC 0 Z9 0 U1 2 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 17 EP 24 DI 10.1016/j.jnucmat.2015.12.036 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400003 ER PT J AU Squires, LN Lessing, P AF Squires, Leah N. Lessing, Paul TI Direct chemical reduction of neptunium oxide to neptunium metal using calcium and calcium chloride SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID DIOXIDE; CACL2 AB A process of direct reduction of neptunium oxide to neptunium metal using calcium metal as the reducing agent is discussed. After reduction of the oxide to metal, the metal is separated by density from the other components of the reaction mixture and can be easily removed upon cooling. The direct reduction technique consistently produces high purity (98%-99% pure) neptunium metal. (C) 2016 Elsevier B.V. All rights reserved. C1 [Squires, Leah N.; Lessing, Paul] Idaho Natl Lab, 2525 Fremont Ave, Idaho Falls, ID 83415 USA. RP Squires, LN (reprint author), Idaho Natl Lab, 2525 Fremont Ave, Idaho Falls, ID 83415 USA. EM leah.squires@inl.gov NR 8 TC 1 Z9 1 U1 2 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 65 EP 68 DI 10.1016/j.jnucmat.2016.01.007 PG 4 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400009 ER PT J AU Spicer, JB Olasov, LR Zeng, FW Han, KR Gallego, NC Contescu, CI AF Spicer, James B. Olasov, Lauren R. Zeng, Fan W. Han, Karen Gallego, Nidia C. Contescu, Cristian I. TI Laser ultrasonic assessment of the effects of porosity and microcracking on the elastic moduli of nuclear graphites SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE Laser ultrasonics; Nuclear graphite; Porosity; Microcracking ID ORIENTATION DISTRIBUTION FUNCTION; WAVE VELOCITY-MEASUREMENTS; MICROSTRUCTURAL CHARACTERIZATION; ANISOTROPIC MATERIAL; ISOTROPIC GRAPHITE; YOUNGS MODULUS; CRACKS; IRRADIATION; ROCKS; IG-110 AB Laser ultrasonic methods have been used to measure the elastic moduli of various nuclear graphites. Measurements were made to assess wavespeeds for longitudinal and shear waves in different propagation directions and these were used along with density measurements to compute the longitudinal and shear moduli as well as Young's modulus. All moduli decreased with increasing graphite porosity and these variations could be interpreted using models describing the effect of porosity on material stiffness. Extrapolations for these models to zero porosity were used to infer the moduli for theoretically dense graphite; the results were far below predicted values reported in the literature for fully dense, polycrystalline, isotropic graphite. Differences can be attributed to microcracking in the graphite microstructure. Using models for the effects of microcracking on modulus, estimates for microcrack populations indicate that the number of cracks per unit volume must be much greater than the number of pores per unit volume. Experimental results reported in the literature for irradiated graphites as well as for the stress dependence of graphite modulus are consistent with the influence of microcracking on elastic behavior and could be interpreted using concepts developed here. Results in this work for graphite structure- property relationships should allow for more sophisticated characterization of nuclear graphites using ultrasonic methods. (C) 2015 Elsevier B.V. All rights reserved. C1 [Spicer, James B.; Olasov, Lauren R.; Zeng, Fan W.; Han, Karen] Johns Hopkins Univ, Whiting Sch Engn, Dept Mat Sci & Engn, Baltimore, MD 21218 USA. [Gallego, Nidia C.; Contescu, Cristian I.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Carbon & Composites Grp, Oak Ridge, TN 37831 USA. RP Spicer, JB (reprint author), Johns Hopkins Univ, Whiting Sch Engn, Dept Mat Sci & Engn, Baltimore, MD 21218 USA. EM spicer@jhu.edu RI Spicer, James/A-3312-2010; OI Spicer, James/0000-0002-3512-5503; Contescu, Cristian/0000-0002-7450-3722; Gallego, Nidia/0000-0002-8252-0194 NR 48 TC 1 Z9 1 U1 12 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 80 EP 91 DI 10.1016/j.jnucmat.2015.12.015 PG 12 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400012 ER PT J AU Snead, LL Katoh, Y Koyanagi, T Terrani, K Specht, ED AF Snead, Lance L. Katoh, Yutai Koyanagi, Takaaki Terrani, Kurt Specht, Eliot D. TI Dimensional isotropy of 6H and 3C SiC under neutron irradiation SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article ID BEAM-INDUCED AMORPHIZATION; PHYSICAL-PROPERTY CHANGE; SILICON-CARBIDE; INDUCED CRYSTALLINE; AMORPHOUS TRANSITION; RADIATION-DAMAGE; SINGLE-CRYSTALS; IMPLANTED IONS; CERAMICS; STRENGTH AB This investigation experimentally determines the as-irradiated crystal axes dimensional change of the common polytypes of SiC considered for nuclear application. Single crystal alpha-SiC (6H), beta-SiC (3C), CVD beta-SiC, and single crystal Si have been neutron irradiated near 60 degrees C from 2 x 10(23) to 2 x 10(26) n/m(2) (E > 0.1 MeV), or about 0.02-20 dpa, in order to study the effect of irradiation on bulk swelling and strain along independent crystalline axes. Single crystal, powder diffractometry and density measurement have been carried out. For all neutron doses where the samples remained crystalline all SiC materials demonstrated equivalent swelling behavior. Moreover the 6H-SiC expanded isotropically. The magnitude of the swelling followed a similar to 0.77 power law against dose consistent with a microstructure evolution driven by single interstitial (carbon) mobility. Extraordinarily large similar to 7.8% volume expansion in SiC was observed prior to amorphization. Above similar to 0.9 similar to 10(25) n/m(2) (E > 0.1 MeV) all SiC materials became amorphous with an identical swelling: a 11.7% volume expansion, lowering the density to 2.84 g/cm(3). The as-amorphized density was the same at the 2 x 10(25) and 2 x 10(26) n/m(2) (E > 0.1 MeV) dose levels. (C) 2016 Elsevier B.V. All rights reserved. C1 [Snead, Lance L.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Katoh, Yutai; Koyanagi, Takaaki; Terrani, Kurt; Specht, Eliot D.] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Snead, LL (reprint author), MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. EM Snead@MIT.edu RI Koyanagi, Takaaki/D-9841-2017 OI Koyanagi, Takaaki/0000-0001-7272-4049 NR 46 TC 4 Z9 4 U1 6 U2 25 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 92 EP 96 DI 10.1016/j.jnucmat.2016.01.010 PG 5 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400013 ER PT J AU White, JT Nelson, AT Dunwoody, JT Byler, DD McClellan, KJ AF White, J. T. Nelson, A. T. Dunwoody, J. T. Byler, D. D. McClellan, K. J. TI Thermophysical properties of USi to 1673 K SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE Uranium silicide; USi; Laser flash analysis; Thermal conductivity; Accident tolerant fuels ID URANIUM; U3SI2 AB Consideration of uranium silicide compounds as candidate nuclear reactor fuels requires the accurate knowledge of their thermophysical properties as a function of temperature. Stoichiometric USi has received little attention in the literature with regard to property characterization. This absence of data prevents modeling and simulation communities from predicting performance of uranium silicide fuels that are either nominally USi itself, or are designed with other uranium silicide phases but may include appreciable fractions of USi introduced as a result of the fuel synthesis or fabrication process. This study was undertaken to quantify the thermal expansion coefficient, specific heat capacity, thermal diffusivity, and thermal conductivity of USi from ambient conditions to just below the peritectic decomposition of the compound. Stoichiometric samples that were prepared by arc melting and powder metallurgical routes for thermophysical property measurements exhibited 94% USi phase, with the balance being U3Si5 phase that likely formed during the solidification process. An energetic phase transformation was observed at 723 K, which is attributed to the inclusion of the secondary U3Si5 phase. (C) 2016 Elsevier B.V. All rights reserved. C1 [White, J. T.; Nelson, A. T.; Dunwoody, J. T.; Byler, D. D.; McClellan, K. J.] Los Alamos Natl Lab, Los Alamos, NM USA. RP White, JT (reprint author), Los Alamos Natl Lab, Los Alamos, NM USA. EM jtwhite@lanl.gov OI Nelson, Andrew/0000-0002-4071-3502 NR 20 TC 1 Z9 1 U1 7 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 129 EP 135 DI 10.1016/j.jnucmat.2016.01.013 PG 7 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400018 ER PT J AU Marcum, WR Wachs, DM Robinson, AB Lillo, MA AF Marcum, W. R. Wachs, D. M. Robinson, A. B. Lillo, M. A. TI Aluminum cladding oxidation of prefilmed in-pile fueled experiments SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article AB A series of fueled irradiation experiments were recently completed within the Advanced Test Reactor Full size plate In center flux trap Position (AFIP) and Gas Test Loop (GTL) campaigns. The conduct of the AFIP experiments supports ongoing efforts within the global threat reduction initiative (GTRI) to qualify a new ultra-high loading density low enriched uranium-molybdenum fuel. This study details the characterization of oxide growth on the fueled AFIP experiments and cross-correlates the empirically measured oxide thickness values to existing oxide growth correlations and convective heat transfer correlations that have traditionally been utilized for such an application. This study adds new and valuable empirical data to the scientific community with respect to oxide growth measurements of highly irradiated experiments, of which there is presently very limited data. Additionally, the predicted oxide thickness values are reconstructed to produce an oxide thickness distribution across the length of each fueled experiment (a new application and presentation of information that has not previously been obtainable in open literature); the predicted distributions are compared against experimental data and in general agree well with the exception of select outliers. Published by Elsevier B.V. C1 [Marcum, W. R.] Oregon State Univ, Sch Nucl Sci & Engn, 116 Radiat Ctr, Corvallis, OR 97331 USA. [Wachs, D. M.; Robinson, A. B.; Lillo, M. A.] Idaho Natl Lab, Nucl Fuels & Mat Dept, 2525 Fremont Ave, Idaho Falls, ID 83415 USA. RP Marcum, WR (reprint author), Oregon State Univ, Sch Nucl Sci & Engn, 116 Radiat Ctr, Corvallis, OR 97331 USA. EM marcumw@engr.orst.edu OI Marcum, Wade/0000-0003-2031-5758 NR 33 TC 1 Z9 1 U1 1 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 136 EP 148 DI 10.1016/j.jnucmat.2016.01.011 PG 13 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400019 ER PT J AU Xu, ZJ Joshi, V Hu, SY Paxton, D Lavender, C Burkes, D AF Xu, Zhijie Joshi, Vineet Hu, Shenyang Paxton, Dean Lavender, Curt Burkes, Douglas TI Modeling the homogenization kinetics of as-cast U-10wt% Mo alloys SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article DE Uranium; Molybdenum; omogenization modeling; Diffusion; Microstructure characterization; BSE-SEM ID URANIUM-MOLYBDENUM ALLOY; NICKEL-BASE SUPERALLOY; MICROSTRUCTURE EVOLUTION; HIGH-DENSITY; PHASE; DIFFUSION; BEHAVIOR; FUEL AB Low-enriched U-22at% Mo (U-10Mo) alloy has been considered as an alternative material to replace the highly enriched fuels in research reactors. For the U-10Mo to work effectively and replace the existing fuel material, a thorough understanding of the microstructure development from as-cast to the final formed structure is required. The as-cast microstructure typically resembles an inhomogeneous microstructure with regions containing molybdenum-rich and -lean regions, which may affect the processing and possibly the in-reactor performance. This as-cast structure must be homogenized by thermal treatment to produce a uniform Mo distribution. The development of a modeling capability will improve the understanding of the effect of initial microstructures on the Mo homogenization kinetics. In the current work, we investigated the effect of as-cast microstructure on the homogenization kinetics. The kinetics of the homogenization was modeled based on a rigorous algorithm that relates the line scan data of Mo concentration to the gray scale in energy dispersive spectroscopy images, which was used to generate a reconstructed Mo concentration map. The map was then used as realistic microstructure input for physics-based homogenization models, where the entire homogenization kinetics can be simulated and validated against the available experiment data at different homogenization times and temperatures. (C) 2016 Elsevier B.V. All rights reserved. C1 [Xu, Zhijie] Pacific NW Natl Lab, Computat Math Grp, Richland, WA 99352 USA. [Hu, Shenyang] Pacific NW Natl Lab, Reactor Mat & Mech Design, Richland, WA 99352 USA. [Joshi, Vineet; Lavender, Curt] Pacific NW Natl Lab, Energy Proc & Mat Div, Richland, WA 99352 USA. [Paxton, Dean; Burkes, Douglas] Pacific NW Natl Lab, Nucl Engn & Anal Grp, Richland, WA 99352 USA. RP Xu, ZJ (reprint author), Pacific NW Natl Lab, Computat Math Grp, Richland, WA 99352 USA. EM zhijie.xu@pnnl.gov RI Xu, Zhijie/A-1627-2009; OI Xu, Zhijie/0000-0003-0459-4531; Joshi, Vineet/0000-0001-7600-9317; HU, Shenyang/0000-0002-7187-3082 NR 30 TC 1 Z9 1 U1 5 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 154 EP 164 DI 10.1016/j.jnucmat.2015.11.026 PG 11 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400021 ER PT J AU Byun, TS Morgan, D Jiao, ZJ Almer, J Brown, D AF Byun, Thak Sang Morgan, Dane Jiao, Zhijie Almer, Jonathan Brown, Donald TI Microstructural processes in irradiated materials Preface SO JOURNAL OF NUCLEAR MATERIALS LA English DT Editorial Material C1 [Byun, Thak Sang] Pacific NW Natl Lab, Richland, WA 99352 USA. [Morgan, Dane] Univ Wisconsin, Madison, WI 53706 USA. [Jiao, Zhijie] Univ Michigan, Ann Arbor, MI 48109 USA. [Almer, Jonathan] Argonne Natl Lab, Argonne, IL 60439 USA. [Brown, Donald] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Byun, TS (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM thaksang.byun@pnnl.gov NR 0 TC 0 Z9 0 U1 2 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 165 EP 166 DI 10.1016/j.jnucmat.2016.01.015 PG 2 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400022 ER PT J AU Chen, WY Li, MM Kirk, MA Baldo, PM Lian, TG AF Chen, Wei-Ying Li, Meimei Kirk, Marquis A. Baldo, Peter M. Lian, Tiangan TI Effect of heavy ion irradiation on microstructural evolution in CF8 cast austenitic stainless steel SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS DE Cast austenitic stainless steel; CASS; Irradiation; Aging; G-phase; Dislocation loops; Ferrite; Austenite; Nuclear; Synergistic effect; TEM ID REACTOR PRESSURE-VESSELS; NEUTRON-IRRADIATION; SPINODAL DECOMPOSITION; DAMAGE EVOLUTION; THIN-FOILS; FE; RADIATION; METALS; ALLOYS; EMBRITTLEMENT AB The microstructural evolution in ferrite and austenitic in cast austenitic stainless steel (CASS) CF8, as received or thermally aged at 400 degrees C for 10,000 h, was followed under TEM with in situ irradiation of 1 MeV Kr ions at 300 and 350 degrees C to a fluence of 1.9 x 10(15) ions/cm(2) (similar to 3 dpa) at the IVEM-Tandem Facility. For the unaged CF8, the irradiation-induced dislocation loops appeared at a much lower dose in the austenite than in the ferrite. At the end dose, the austenite formed a well-developed dislocation network microstructure, while the ferrite exhibited an extended dislocation structure as line segments. Compared to the unaged CF8, the aged specimen appeared to have lower rate of damage accumulation. The rate of microstructural evolution under irradiation in the ferrite was significantly lower in the aged specimen than in the unaged. This difference is attributed to the different initial microstructures in the unaged and aged specimens, which implies that thermal aging and irradiation are not independent but interconnected damage processes. Published by Elsevier B.V. C1 [Chen, Wei-Ying; Li, Meimei; Kirk, Marquis A.; Baldo, Peter M.] Argonne Natl Lab, Argonne, IL 60436 USA. [Lian, Tiangan] Elect Power Res Inst, Palo Alto, CA 94304 USA. RP Chen, WY (reprint author), Argonne Natl Lab, Argonne, IL 60436 USA. EM wychen@anl.gov OI Chen, Wei-Ying/0000-0002-6583-4204 NR 33 TC 0 Z9 0 U1 3 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 184 EP 192 DI 10.1016/j.jnucmat.2015.08.032 PG 9 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400025 ER PT J AU Jin, K Bei, H Zhang, Y AF Jin, K. Bei, H. Zhang, Y. TI Ion irradiation induced defect evolution in Ni and Ni-based FCC equiatomic binary alloys SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS DE Metal and alloys; Ion irradiation; Solid solution; Defects; Energy dissipation ID SOLID-SOLUTION ALLOYS; HIGH-ENTROPY ALLOY; MATERIALS CHALLENGES; RADIATION-DAMAGE; ELECTRICAL-RESISTIVITY; TEMPERATURE-DEPENDENCE; MECHANICAL-PROPERTIES; STRUCTURAL-MATERIALS; IMPLANTATION; SYSTEMS AB In order to explore the chemical effects on radiation response of alloys with multi-principal elements, defect evolution under Au ion irradiation was investigated in the elemental Ni, equiatomic NiCo and NiFe alloys. Single crystals were successfully grown in an optical floating zone furnace and their (100) surfaces were irradiated with 3 MeV Au ions at fluences ranging from 1 x 10(13) to 5 x 10(15) ions cm(-2) at room temperature. The irradiation-induced defect evolution was analyzed by using ion channeling technique. Experiment shows that NiFe is more irradiation-resistant than NiCo and pure Ni at low fluences. With continuously increasing the ion fluences, damage level is eventually saturated for all materials but at different dose levels. The saturation level in pure Ni appears at relatively lower irradiation fluence than the alloys, suggesting that damage accumulation slows down in the alloys. Under high-fluence irradiations, pure Ni has wider damage ranges than the alloys, indicating that defects in pure Ni have high mobility. (C) 2015 Published by Elsevier B.V. C1 [Jin, K.; Bei, H.; Zhang, Y.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Jin, K.; Zhang, Y.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Zhang, Y (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM zhangy1@ornl.gov OI Bei, Hongbin/0000-0003-0283-7990 NR 39 TC 3 Z9 3 U1 12 U2 34 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 193 EP 199 DI 10.1016/j.jnucmat.2015.09.009 PG 7 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400026 ER PT J AU Short, MP Gaston, DR Jin, M Shao, L Garner, FA AF Short, M. P. Gaston, D. R. Jin, M. Shao, L. Garner, F. A. TI Modeling injected interstitial effects on void swelling in self-ion irradiation experiments SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS ID TEMPERATURE SHIFT; RADIATION-DAMAGE; CHARGED-PARTICLE; PURE IRON; DOSE-RATE; NEUTRON; SIMULATION; NICKEL; DEFECTS; PURITY AB Heavy ion irradiations at high dose rates are often used to simulate slow and expensive neutron irradiation experiments. However, many differences in the resultant modes of damage arise due to unique aspects of heavy ion irradiation. One such difference was recently shown in pure iron to manifest itself as a double peak in void swelling, with both peaks located away from the region of highest displacement damage. In other cases involving a variety of ferritic alloys there is often only a single peak in swelling vs. depth that is located very near the ion-incident surface. We show that these behaviors arise due to a combination of two separate effects: 1) suppression of void swelling due to injected interstitials, and 2) preferential sinking of interstitials to the ion-incident surface, which are very sensitive to the irradiation temperature and displacement rate. Care should therefore be used in collection and interpretation of data from the depth range outside the Bragg peak of ion irradiation experiments, as it is shown to be more complex than previously envisioned. (C) 2015 Elsevier B.V. All rights reserved. C1 [Short, M. P.; Jin, M.] MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. [Gaston, D. R.] Idaho Natl Lab, Idaho Falls, ID USA. [Shao, L.] Texas A&M Univ, Dept Nucl Engn, College Stn, TX 77843 USA. [Garner, F. A.] Radiat Effects Consulting, Idaho Falls, ID USA. RP Short, MP (reprint author), MIT, Dept Nucl Sci & Engn, Cambridge, MA 02139 USA. EM hereiam@mit.edu NR 46 TC 4 Z9 4 U1 8 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 200 EP 207 DI 10.1016/j.jnucmat.2015.10.002 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400027 ER PT J AU Mei, ZG Yacout, AM Kim, YS Hofman, G Stan, M AF Mei, Zhi-Gang Yacout, Abdellatif M. Kim, Yeon Soo Hofman, Gerard Stan, Marius TI First-principles study of transition-metal nitrides as diffusion barriers against Al SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS ID FUSION-REACTOR MATERIALS; TITANIUM NITRIDE; URANIUM-MOLYBDENUM; ZIRCONIUM NITRIDE; DISPERSION FUEL; ATOMIC-SCALE; ZRN; METALLIZATION; COMBUSTION; SCHEMES AB Using density-functional theory based first-principles calculations we provided a comparative study of the diffusion barrier properties of TiN, ZrN, and HfN against Al for U-Mo dispersion fuel applications. We firstly examined the thermodynamic stability of these transition-metal nitrides with Al. The calculated heats of reaction show that both TiN and ZrN are thermodynamically unstable diffusion barrier materials, which might be decomposed by Al at relatively high temperatures. As a comparison, HfN is a stable diffusion barrier material for Al. To evaluate the kinetic stability of these nitride systems against Al diffusion, we investigated the diffusion mechanisms of Al in TiN, ZrN and HfN using atomic scale simulations. The effect of non-stoichiometry on the defect formation and Al migration was systematically studied. (C) 2015 ELSEVIER B.V. All rights reserved. C1 [Mei, Zhi-Gang; Yacout, Abdellatif M.; Kim, Yeon Soo; Hofman, Gerard; Stan, Marius] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Mei, ZG (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM zmei@anl.gov NR 33 TC 0 Z9 0 U1 4 U2 18 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 208 EP 213 DI 10.1016/j.jnucmat.2015.10.048 PG 6 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400028 ER PT J AU Leng, B Ko, H Gerczak, TJ Deng, J Giordani, AJ Hunter, JL Morgan, D Szlufarska, I Sridharan, K AF Leng, Bin Ko, Hyunseok Gerczak, Tyler J. Deng, Jie Giordani, Andrew J. Hunter, Jerry L., Jr. Morgan, Dane Szlufarska, Izabela Sridharan, Kumar TI Effect of carbon ion irradiation on Ag diffusion in SiC SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS DE Silicon carbide; TRISO; Radiation; Diffusion; Silver ID RADIATION-ENHANCED DIFFUSION; CUBIC SILICON-CARBIDE; AMORPHOUS METALLIC ALLOYS; TOTAL-ENERGY CALCULATIONS; GRAIN-BOUNDARY DIFFUSION; TRISO COATED PARTICLES; AUGMENTED-WAVE METHOD; FUEL-PARTICLES; MOLECULAR-DYNAMICS; ULTRASOFT PSEUDOPOTENTIALS AB Transport of Ag fission product through the silicon-carbide (SiC) diffusion barrier layer in TRISO fuel particles is of considerable interest given the application of this fuel type in high temperature gas-cooled reactor (HTGR) and other future reactor concepts. The reactor experiments indicate that radiation may play an important role in release of Ag; however so far the isolated effect of radiation on Ag diffusion has not been investigated in controlled laboratory experiments. In this study, we investigate the diffusion couples of Ag and polycrystalline 3C-SiC, as well as Ag and single crystalline 4H-SiC samples before and after irradiation with C2+ ions. The diffusion couple samples were exposed to temperatures of 1500 degrees C, 1535 degrees C, and 1569 degrees C, and the ensuing diffusion profiles were analyzed by secondary ion mass spectrometry (SIMS). Diffusion coefficients calculated from these measurements indicate that Ag diffusion was greatly enhanced by carbon irradiation due to a combined effect of radiation damage on diffusion and the presence of grain boundaries in polycrystalline SiC samples. (C) 2015 Elsevier B.V. All rights reserved. C1 [Leng, Bin; Morgan, Dane; Szlufarska, Izabela; Sridharan, Kumar] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. [Ko, Hyunseok; Gerczak, Tyler J.; Morgan, Dane; Szlufarska, Izabela; Sridharan, Kumar] Univ Wisconsin, Mat Sci Program, Madison, WI 53706 USA. [Deng, Jie; Morgan, Dane; Szlufarska, Izabela; Sridharan, Kumar] Univ Wisconsin, Mat Sci & Engn Dept, Madison, WI 53706 USA. [Giordani, Andrew J.; Hunter, Jerry L., Jr.] Virginia Tech, Nanoscale Characterizat & Fabricat Lab, Blacksburg, VA 24061 USA. [Hunter, Jerry L., Jr.] Univ Wisconsin, Ctr Mat Sci, Madison, WI 53706 USA. [Leng, Bin] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Gerczak, Tyler J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Sridharan, K (reprint author), Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA.; Szlufarska, I (reprint author), Univ Wisconsin, Mat Sci & Engn Dept, Madison, WI 53706 USA. EM szlufarska@wisc.edu; kumars@cae.wisc.edu NR 82 TC 1 Z9 1 U1 8 U2 23 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 220 EP 232 DI 10.1016/j.jnucmat.2015.11.017 PG 13 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400030 ER PT J AU Chung, BW Lema, KE Allen, PG AF Chung, B. W. Lema, K. E. Allen, P. G. TI Effects of self-irradiation in plutonium alloys SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS ID STABILIZED DELTA-PLUTONIUM; DENSITY CHANGES; PU-238 ENRICHMENT; HELIUM BUBBLES; RADIATION; DAMAGE; PU AB In this paper, we present updated results of self-irradiation effects on Pu-238-enriched Pu-239 alloys measured by immersion density, dilatometry, and tensile tests. We obtained the self-irradiation equivalent time of nearly 200 years, nearly 100 years longer than in our previous papers. At this extended aging, we find the rate of decrease in density has slowed significantly, stabilizing around 15.73 g/cc, without signs of void swelling. The volume expansion measured at 35 degrees C also shows apparent saturation at less than 0.25%. Quasi-static tensile measurement still show gradual increase in the strength of plutonium alloys with age. (C) 2015 Elsevier B.V. All rights reserved. C1 [Chung, B. W.; Lema, K. E.; Allen, P. G.] Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. RP Chung, BW (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. EM chung7@llnl.gov RI Chung, Brandon/G-2929-2012 NR 23 TC 1 Z9 1 U1 7 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 239 EP 242 DI 10.1016/j.jnucmat.2015.09.028 PG 4 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400032 ER PT J AU Hoelzer, DT Unocic, KA Sokolov, MA Byun, TS AF Hoelzer, D. T. Unocic, K. A. Sokolov, M. A. Byun, T. S. TI Influence of processing on the microstructure and mechanical properties of 14YWT SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS ID FERRITIC ALLOY 14YWT; STRENGTHENING MECHANISMS; TEMPERATURE-DEPENDENCE; FRACTURE-TOUGHNESS; ODS STEELS; STABILITY; NITROGEN; TENSILE; OXYGEN AB The investigation of the mechanical alloying (MA) conditions for producing the advanced oxide dispersion strengthened (ODS) 14YWT ferritic alloy led to significant improvements in balancing the strength, ductility and fracture toughness properties while still maintaining the salient microstructural features consisting of ultra-fine grains and high concentration of Y-, Ti- and O-enriched nanoclusters. The implemented changes to the processing conditions included reducing the contamination of the powder during ball milling, applying a pre-extrusion annealing treatment on the ball milled powder and exploring different extrusion temperatures at 850 degrees C (SM170 heat), 1000 degrees C (SM185) and 1150 degrees C (SM200). The microstructural studies of the three 14YWT heats showed similarities in the dispersion of nanoclusters and sub-micron size grains, indicating the microstructure was insensitive to the different extrusion conditions. Compared to past 14YWT heats, the three new heats showed lower strength, but higher ductility levels between 25 and 800 degrees C and significantly higher fracture toughness values between 25 degrees C and 700 degrees C. The lower contamination levels of O, C and N achieved with improved ball milling conditions plus the slightly larger grain size were identified as important factors for improving the balance in mechanical properties of the three heats of 14YWT. (C) 2015 Elsevier B.V. All rights reserved. C1 [Hoelzer, D. T.; Unocic, K. A.; Sokolov, M. A.] Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Byun, T. S.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Hoelzer, DT (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM hoelzerd@ornl.gov RI Hoelzer, David/L-1558-2016 NR 47 TC 3 Z9 3 U1 3 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 251 EP 265 DI 10.1016/j.jnucmat.2015.12.011 PG 15 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400034 ER PT J AU Pellin, MJ Yacout, AM Mo, K Almer, J Bhattacharya, S Mohamed, W Seidman, D Ye, B Yun, D Xu, RQ Zhu, SF AF Pellin, M. J. Yacout, Abdellatif M. Mo, Kun Almer, Jonathan Bhattacharya, S. Mohamed, Walid Seidman, D. Ye, Bei Yun, D. Xu, Ruqing Zhu, Shaofei TI MeV per nucleon ion irradiation of nuclear materials with high energy synchrotron X-ray characterization SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS DE Radiation damage; Characterization; x-ray; energetic ion; nuclear fuels; UMo ID MO/AL DISPERSION FUEL; AIRCRAFT; BEHAVIOR AB The combination of MeV/Nucleon ion irradiation (e.g. 133 MeV Xe) and high energy synchrotron x-ray characterization (e.g. at the Argonne Advanced Photon Source, APS) provides a powerful characterization method to understand radiation effects and to rapidly screen materials for the nuclear reactor environment. Ions in this energy range penetrate similar to 10 mu m into materials. Over this range, the physical interactions vary (electronic stopping, nuclear stopping and added interstitials). Spatially specific x-ray (and TEM and nanoindentation) analysis allow individual quantification of these various effects. Hard x-rays provide the penetration depth needed to analyze even nuclear fuels. Here, this combination of synchrotron x-ray and MeV/Nucleon ion irradiation is demonstrated on U-Mo fuels. A preliminary look at HT-9 steels is also presented. We suggest that a hard x-ray facility with in situ MeV/nucleon irradiation capability would substantially accelerate the rate of discovery for extreme materials. (C) 2016 Published by Elsevier B.V. C1 [Pellin, M. J.; Bhattacharya, S.] Div Mat Sci, New York, NY 10010 USA. [Yacout, Abdellatif M.; Mo, Kun; Mohamed, Walid; Ye, Bei; Yun, D.] Nucl Engn Div, New York, NY USA. [Almer, Jonathan; Xu, Ruqing] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Bhattacharya, S.; Seidman, D.] Northwestern Univ, Dept Mat Sci & Engn, 2220 Campus Dr, Evanston, IL 60208 USA. [Zhu, Shaofei] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Pellin, MJ (reprint author), Div Mat Sci, New York, NY 10010 USA. EM Pellin@anl.gov RI Pellin, Michael/B-5897-2008; Seidman, David/B-6697-2009 OI Pellin, Michael/0000-0002-8149-9768; NR 32 TC 2 Z9 2 U1 0 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 266 EP 271 DI 10.1016/j.jnucmat.2016.01.004 PG 6 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400035 ER PT J AU Yun, D Miao, YB Xu, RQ Mei, ZG Mo, K Mohamed, W Ye, B Pellin, MJ Yacout, AM AF Yun, Di Miao, Yinbin Xu, Ruqing Mei, Zhigang Mo, Kun Mohamed, Walid Ye, Bei Pellin, Michael J. Yacout, Abdellatif M. TI Characterization of high energy Xe ion irradiation effects in single crystal molybdenum with depth-resolved synchrotron microbeam diffraction SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS DE Microbeam X-ray diffraction; Heavy ion irradiation; Molecular dynamics; Depth-resolved X-ray diffraction ID MICROSCOPY; STRAIN; DEFORMATION; COMPOSITES; DYNAMICS; SCALE AB Microbeam X-ray diffraction experiments were conducted at beam line 34-ID of the Advanced Photon Source (APS) on fission fragment energy Xe heavy ion irradiated single crystal Molybdenum (Mo). Lattice strain measurements were obtained with a depth resolution of 0.7 mu m, which is critical in resolving the peculiar heterogeneity of irradiation damage associated with heavy ion irradiation. Q-space diffraction peak shift measurements were correlated with lattice strain induced by the ion irradiations. Transmission electron microscopy (TEM) characterizations were performed on the as-irradiated materials as well. Nanometer sized Xe bubble microstructures were observed via TEM. Molecular Dynamics (MD) simulations were performed to help interpret the lattice strain measurement results from the experiment. This study showed that the irradiation effects by fission fragment energy Xe ion irradiations can be collaboratively understood with the depth resolved X-ray diffraction and TEM measurements under the assistance of MD simulations. (c) 2015 Elsevier B.V. All rights reserved. C1 [Yun, Di; Xu, Ruqing; Mei, Zhigang; Mo, Kun; Mohamed, Walid; Ye, Bei; Pellin, Michael J.; Yacout, Abdellatif M.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Yun, Di] Xi An Jiao Tong Univ, 28 West Xian Ning Rd, Xian 710049, Peoples R China. [Miao, Yinbin] Univ Illinois, 104 South Wright St, Urbana, IL 61801 USA. RP Yun, D (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA.; Yun, D (reprint author), Xi An Jiao Tong Univ, 28 West Xian Ning Rd, Xian 710049, Peoples R China. EM diyun1979@xjtu.edu.cn RI Pellin, Michael/B-5897-2008; Yun, Di/K-6441-2013; OI Pellin, Michael/0000-0002-8149-9768; Yun, Di/0000-0002-9767-3214; Miao, Yinbin/0000-0002-3128-4275 NR 22 TC 2 Z9 2 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 272 EP 279 DI 10.1016/j.jnucmat.2015.12.007 PG 8 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400036 ER PT J AU Zhang, X Park, JS Almer, J Li, MM AF Zhang, Xuan Park, Jun-Sang Almer, Jonathan Li, Meimei TI Characterization of neutron-irradiated HT-UPS steel by high-energy X-ray diffraction microscopy SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS DE Austenitic steel; High-energy X-ray diffraction microscopy; Irradiation effect; Meso-scale ID GRAIN-SIZE DISTRIBUTION; AUSTENITIC STAINLESS-STEELS; LATTICE-PARAMETER VARIATION; MICROSTRUCTURAL EVOLUTION; POLYCRYSTALLINE MATERIALS; TENSILE DEFORMATION; INDIVIDUAL GRAINS; MATERIALS SCIENCE; PLASTIC BEHAVIOR; FAST METHODOLOGY AB This paper presents the first measurement of neutron-irradiated microstructure using far-field high-energy X-ray diffraction microscopy (FF-HEDM) in a high-temperature ultrafine-precipitate-strengthened (HT-UPS) austenitic stainless steel. Grain center of mass, grain size distribution, crystallographic orientation (texture), diffraction spot broadening and lattice constant distributions of individual grains were obtained for samples in three different conditions: non-irradiated, neutron-irradiated (3dpa/500 degrees C), and irradiated + annealed (3dpa/500 degrees C + 600 degrees C/1 h). It was found that irradiation caused significant increase in grain-level diffraction spot broadening, modified the texture, reduced the grain-averaged lattice constant, but had nearly no effect on the average grain size and grain size distribution, as well as the grain size-dependent lattice constant variations. Post-irradiation annealing largely reversed the irradiation effects on texture and average lattice constant, but inadequately restored the microstrain. Published by Elsevier B.V. C1 [Zhang, Xuan; Li, Meimei] Argonne Natl Lab, Nucl Engn Div, Lemont, IL 60439 USA. [Park, Jun-Sang; Almer, Jonathan] Argonne Natl Lab, Adv Photon Source, Lemont, IL 60439 USA. RP Zhang, X (reprint author), Argonne Natl Lab, Nucl Engn Div, Lemont, IL 60439 USA. EM xuanzhang@anl.gov NR 57 TC 1 Z9 1 U1 4 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 280 EP 288 DI 10.1016/j.jnucmat.2015.11.063 PG 9 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400037 ER PT J AU Lin, JL Mo, K Yun, D Miao, YB Liu, X Zhao, HJ Hoelzer, DT Park, JS Almer, J Zhang, GM Zhou, ZJ Stubbins, JF Yacout, AM AF Lin, Jun-Li Mo, Kun Yun, Di Miao, Yinbin Liu, Xiang Zhao, Huijuan Hoelzer, David T. Park, Jun-Sang Almer, Jonathan Zhang, Guangming Zhou, Zhangjian Stubbins, James F. Yacout, Abdellatif M. TI In situ synchrotron tensile investigations on 14YWT, MA957, and 9-Cr ODS alloys SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS DE Advanced ODS alloys; Dislocation density; Deformation In-situ tensile test; High-energy X-ray diffraction ID X-RAY-DIFFRACTION; POLYCRYSTALLINE ALPHA-FE; ATOM-PROBE TOMOGRAPHY; DISLOCATION MODEL; FERRITIC ALLOY; MARTENSITIC STEEL; SINGLE CRYSTALS; STAINLESS-STEEL; METAL CRYSTALS; ENERGY AB Advanced ODS alloys provide exceptional radiation tolerance and high-temperature mechanical properties when compared to traditional ferritic and ferritic/martensitic 9F/M) steels. Their remarkable properties result from ultrahigh density and ultrafine size of Y-Ti-O nanoclusters within the ferritic matrix. In this work, we applied a high-energy synchrotron radiation X-ray to study the deformation process of three advanced ODS materials including 14YWT, MA957, and 9-Cr ODS steel. Only the relatively large nanoparticles in the 9-Cr ODS were observed in the synchrotron X-ray diffraction. The nanoclusters in both 14YWT and MA957 were invisible in the measurement due to their non-stoichiometric nature. Due to the different sizes of nanoparticles and nanoclusters in the materials, the Orowan looping was considered to be the major strengthening mechanism in the 9-Cr ODS, while the dispersed-barrier-hardening is dominant strengthening mechanism in both 14YWT and MA957, This analysis was inferred from the different build-up rates of dislocation density when plastic deformation was initiated. Finally, the dislocation densities interpreted from the X-ray measurements were successfully modeled using the Bergstrom's dislocation models. (C) 2016 Elsevier B.V. All rights reserved. C1 [Lin, Jun-Li; Miao, Yinbin; Liu, Xiang; Stubbins, James F.] Univ Illinois, Urbana, IL USA. [Mo, Kun; Yun, Di; Yacout, Abdellatif M.] Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Hoelzer, David T.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN USA. [Park, Jun-Sang; Almer, Jonathan] Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. [Zhao, Huijuan] Clemson Univ, Dept Mech Engn, Clemson, SC USA. [Zhang, Guangming; Zhou, Zhangjian] Univ Sci & Technol Beijing, Sch Mat Sci & Engn, Beijing 10083, Peoples R China. RP Mo, K (reprint author), Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM kunmo@anl.gov RI Hoelzer, David/L-1558-2016; Liu, Xiang/D-2005-2017; OI Liu, Xiang/0000-0002-2634-1888; Miao, Yinbin/0000-0002-3128-4275 NR 70 TC 3 Z9 3 U1 2 U2 19 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 289 EP 298 DI 10.1016/j.jnucmat.2015.10.049 PG 10 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400038 ER PT J AU Lin, JL Han, XC Heuser, BJ Almer, JD AF Lin, Jun-li Han, Xiaochun Heuser, Brent J. Almer, Jonathan D. TI Study of the mechanical behavior of the hydride blister/rim structure in Zircaloy-4 using in-situ synchrotron X-ray diffraction SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS DE Synchrotron diffraction; Zirconium alloys; Zirconium hydride; Lattice strain; Rietveld refinement ID SECOND-PHASE PARTICLES; WT-PERCENT NB; ZIRCONIUM HYDRIDE; PRECIPITATION KINETICS; REORIENTATION; STRESS; STRAIN; MATRIX; ALLOY; EMBRITTLEMENT AB High-energy synchrotron X-ray diffraction was utilized to study the mechanical response of the f.c.c delta hydride phase, the intermetallic precipitation with hexagonal C14 lave phase and the alpha-Zr phase in the Zircaloy-4 materials with a hydride rim/blister structure near one surface of the material during in-situ uniaxial tension experiment at 200 degrees C. The f.c.c delta was the only hydride phase observed in the rim/blister structure. The conventional Rietveld refinement was applied to measure the macro-strain equivalent response of the three phases. Two regions were delineated in the applied load versus lattice strain measurement: a linear elastic strain region and region that exhibited load partitioning. Load partitioning was quantified by von Mises analysis. The three phases were observed to have similar elastic modulus at 200 degrees C. (C) 2016 Elsevier B.V. All rights reserved. C1 [Lin, Jun-li; Han, Xiaochun; Heuser, Brent J.] Univ Illinois, Dept Nucl Plasma & Radiol Engn, Urbana, IL USA. [Almer, Jonathan D.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. RP Heuser, BJ (reprint author), Univ Illinois, Dept Nucl Plasma & Radiol Engn, Urbana, IL USA. EM bheuser@illinois.edu OI Han, Xiaochun/0000-0003-2775-4905 NR 45 TC 0 Z9 0 U1 5 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 299 EP 307 DI 10.1016/j.jnucmat.2015.12.048 PG 9 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400039 ER PT J AU Reiche, HM Vogel, SC Tang, M AF Reiche, H. Matthias Vogel, Sven C. Tang, Ming TI In situ synthesis and characterization of uranium carbide using high temperature neutron diffraction SO JOURNAL OF NUCLEAR MATERIALS LA English DT Article; Proceedings Paper CT 7th Symposium on Microstructural Processes in Irradiated Materials (MPIM) and Characterization of Nuclear Reactor Materials and Components with Neutron and Synchrotron Radiation held in the TMS 144th Annual Meeting and Exhibition CY MAR 15-19, 2015 CL Orlando, FL SP TMS DE Delta UC2; Cubic uranium dicarbide; High temperature; Nuclear reactor fuel; UO2; UC; In situ; Neutron diffraction ID THERMAL-CONDUCTIVITY; OXIDE NANOPARTICLES; SODIUM-NITRATE; TRANSITION; ELEMENTS; CARBON; FUELS; UO2; PERFORMANCE AB We investigated the formation of UCx from UO2+x and graphite in situ using neutron diffraction at high temperatures with particular focus on resolving the conflicting reports on the crystal structure of nonquenchable cubic UC2. The agents were UO2 nanopowder, which closely imitates nano grains observed in spent reactor fuels, and graphite powder. In situ neutron diffraction revealed the onset of the UO2 + 2C -> UC + CO2 reaction at 1440 degrees C, with its completion at 1500 degrees C. Upon further heating, carbon diffuses into the uranium carbide forming C-2 groups at the octahedral sites. This resulting high temperature cubic UC2 phase is similar to the NaCl-type structure as proposed by Bowman et al. Our novel experimental data provide insights into the mechanism and kinetics of formation of UC as well as characteristics of the high temperature cubic UC2 phase which agree with proposed rotational rehybridization found from simulations by Wen et al. Published by Elsevier B. V. C1 [Reiche, H. Matthias; Vogel, Sven C.; Tang, Ming] Los Alamos Natl Lab, MST Div Mat Sci Radiat & Dynam Extremes 8, Los Alamos, NM 87545 USA. RP Vogel, SC (reprint author), Los Alamos Natl Lab, MST Div Mat Sci Radiat & Dynam Extremes 8, Los Alamos, NM 87545 USA. EM sven@lanl.gov OI Vogel, Sven C./0000-0003-2049-0361 NR 47 TC 0 Z9 0 U1 5 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-3115 EI 1873-4820 J9 J NUCL MATER JI J. Nucl. Mater. PD APR 1 PY 2016 VL 471 BP 308 EP 316 DI 10.1016/j.jnucmat.2015.12.044 PG 9 WC Materials Science, Multidisciplinary; Nuclear Science & Technology SC Materials Science; Nuclear Science & Technology GA DG0ZS UT WOS:000371795400040 ER PT J AU Lee, PS Kim, D Nam, SE Bhave, RR AF Lee, Pyung-Soo Kim, Daejin Nam, Seung-Eun Bhave, Ramesh R. TI Carbon molecular sieve membranes on porous composite tubular supports for high performance gas separations SO MICROPOROUS AND MESOPOROUS MATERIALS LA English DT Article DE Carbon molecular sieve membrane; Gas separation; Porous stainless steel support; Intermediate alumina layer ID HOLLOW-FIBER MEMBRANES; PHENOLIC RESIN; AIR SEPARATION; ETHYLENE/ETHANE SEPARATION; OLEFIN/PARAFFIN SEPARATION; PYROLYSIS CONDITIONS; CO2/CH4 SEPARATION; POLYIMIDE; POLYETHERIMIDE; MATRIMID(R) AB Carbon molecular sieve (CMS) membranes on the inside of porous composite stainless steel supports were developed for gas separation in this research effort. The intermediate alumina layer was introduced to reduce the pore size of the porous stainless steel tube and subsequently provide uniform surface roughness. Viscosity of the phenolic polymer solution was varied from 10 to 30 centipoises (cP) to maximize performance of the CMS membranes. Pyrolysis temperature was also varied from 700 degrees C to 900 degrees C to optimize the fabrication of uniform CMS membranes on porous composite stainless steel supports. High performance CMS membranes were obtained from triple coatings and subsequent pyrolysis at 700 degrees C. The viscosity of precursor solutions played a critical role to determine the performance of CMS membranes in terms of gas permeance and ideal gas separation factor. The highest separation performance of the CMS membranes was shown with viscosity of 20 cP, resulting in gas separation factor of 462 for He/N-2, 97 for CO2/N-2, and 15.4 for O-2/N-2. (C) 2016 Elsevier Inc. All rights reserved. C1 [Lee, Pyung-Soo; Nam, Seung-Eun] Korea Res Inst Chem Technol, Adv Mat Div, 100 Jang Dong, Daejeon, South Korea. [Kim, Daejin; Bhave, Ramesh R.] Oak Ridge Natl Lab, Mat Sci & Technol Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. RP Bhave, RR (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM bhaverr@ornl.gov OI Bhave, Ramesh/0000-0003-3430-9914 NR 42 TC 3 Z9 3 U1 6 U2 33 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-1811 EI 1873-3093 J9 MICROPOR MESOPOR MAT JI Microporous Mesoporous Mat. PD APR PY 2016 VL 224 BP 332 EP 338 DI 10.1016/j.micromeso.2015.12.054 PG 7 WC Chemistry, Applied; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DG1PW UT WOS:000371841000041 ER PT J AU Mauger, SA Steirer, KX Boe, J Ostrowski, DP Olson, DC Hammond, SR AF Mauger, Scott A. Steirer, K. Xerxes Boe, Jonas Ostrowski, David P. Olson, Dana C. Hammond, Scott R. TI Effects of humidity during formation of zinc oxide electron contact layers from a diethylzinc precursor solution SO ORGANIC ELECTRONICS LA English DT Article DE Organic photovoltaics; Zinc oxide; Processing; Humidity; Contact layer ID ORGANIC SOLAR-CELLS; ENERGY-LEVEL ALIGNMENT; PHOTOVOLTAIC CELLS; OPTICAL-PROPERTIES; POLYMER; PERFORMANCE; DEPOSITION; STABILITY; FILMS AB This work focuses on the role of humidity in the formation of ZnO thin films from a reactive diethylzinc precursor solution for use as the electron contact layer (ECL) in organic photovoltaic (OPV) devices. This method is well suited for flexible devices because the films are annealed at 120 degrees C, making the process compatible with polymer substrates. ZnO films were prepared by spin coating and annealing at different relative humidity (RH) levels. It is found that RH during coating and annealing affects the chemical and physical properties of the ZnO films. Using x-ray photoelectron spectroscopy it is found that increasing RH during the formation steps produces a more stoichiometric oxide and a higher Zn/O ratio. Spectroscopic ellipsometry data shows a small decrease in the optical band gap with increased humidity, consistent with a more stoichiometric oxide. Kelvin probe measurements show that increased RH during formation results in a larger work function (i.e. further from vacuum). Consistent with these data, but counter to what might be expected, when these ZnO films are used as ECLs in OPV devices those with ZnO ECLs processed in low RH (less stoichiometric) had higher power conversion efficiency than those with high-RH processed ZnO due to improved open-circuit voltage. The increase in open-circuit voltage with decreasing humidity was observed with two different donor polymers and fullerene acceptors, which shows the trend is due to changes in ZnO. The observed changes in open-circuit voltage follow the same trend as the ZnO work function indicating that the increase in open-circuit voltage with decreasing humidity is the result of improved energetics at the interface between the bulk-heterojunction and the ZnO layer due to a vacuum level shift. (c) 2016 Elsevier B.V. All rights reserved. C1 [Mauger, Scott A.; Boe, Jonas; Olson, Dana C.] Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO USA. [Steirer, K. Xerxes] Natl Renewable Energy Lab, Ctr Mat Sci, Golden, CO USA. [Boe, Jonas; Ostrowski, David P.] Univ Colorado, Dept Elect Engn, Boulder, CO 80309 USA. [Boe, Jonas] Univ Erlangen Nurnberg, D-91054 Erlangen, Germany. [Hammond, Scott R.] SolarWindow Technol Inc, Columbia, MD USA. RP Hammond, SR (reprint author), SolarWindow Technol Inc, Columbia, MD USA. EM scott@solarwindow.com FU Solar Window Technologies, Inc.; U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory FX Funding for this work provided was by Solar Window Technologies, Inc. This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. S.A.M. would like to acknowledge Dr. Bradley A. MacLeod and Dr. Stefan Oosterhout for thoughtful discussions related to this work. S.R.H. would like to acknowledge Dr. Martin Drees for helpful discussions related to this work. NR 35 TC 0 Z9 0 U1 11 U2 32 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1566-1199 EI 1878-5530 J9 ORG ELECTRON JI Org. Electron. PD APR PY 2016 VL 31 BP 63 EP 70 DI 10.1016/j.orgel.2016.01.012 PG 8 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA DG1CE UT WOS:000371802000009 ER PT J AU Li, TW Zhang, YM Hernandez-Jimenez, F AF Li, Tingwen Zhang, Yongmin Hernandez-Jimenez, Fernando TI Investigation of particle-wall interaction in a pseudo-2D fluidized bed using CFD-DEM simulations SO PARTICUOLOGY LA English DT Article DE Gas-solid flow; Fluidized bed; Computational fluid dynamics; Discrete element method; Particle-wall interaction; Two-dimensional flow ID DIGITAL IMAGE-ANALYSIS; BOUNDARY-CONDITIONS; GRANULAR FLOWS; NUMERICAL-SIMULATION; FRICTIONAL FORCES; VELOCIMETRY PIV; BEHAVIOR; MODEL; MFIX; HYDRODYNAMICS AB We report on discrete element method simulations of a pseudo-two-dimensional (pseudo-2D) fluidized bed to investigate particle-wall interactions. Detailed information on macroscopic flow field variables, including solids pressure, granular temperature, and normal and tangential wall stresses are analyzed. The normal wall stress differs from the solids pressure because of the strong anisotropic flow behavior in the pseudo-2D system. A simple linear relationship exists between normal wall stress and solids pressure. In addition, an effective friction coefficient can be derived to characterize particle-wall flow interaction after evaluating the normal and tangential wall stresses. The effects of inter-particle and particle-wall friction coefficients are evaluated. Strong anisotropic flow behavior in the pseudo-2D system needs to be considered to validate the two-fluid model where the boundary condition is usually developed based on an isotropic assumption. The conclusion has been confirmed by simulation with different particle stiffnesses. Assumptions in the newly developed model for 2D simulation are further examined against the discrete element method simulation. (C) 2015 Chinese Society of Particuology and Institute of Process Engineering, Chinese Academy of Sciences. Published by Elsevier B.V. All rights reserved. C1 [Li, Tingwen] Natl Energy Technol Lab, Morgantown, WV 26507 USA. [Li, Tingwen] AECOM, Morgantown, WV 26507 USA. [Zhang, Yongmin] China Univ Petr, State Key Lab Heavy Oil Proc, Beijing 102249, Peoples R China. [Hernandez-Jimenez, Fernando] Univ Carlos III Madrid, Dept Thermal & Fluid Engn, Ave Univ 30, Madrid 28911, Spain. RP Li, TW (reprint author), Natl Energy Technol Lab, Morgantown, WV 26507 USA. EM tingwen.li@contr.netl.doe.gov RI Hernandez-Jimenez, Fernando/K-6447-2014; OI Hernandez-Jimenez, Fernando/0000-0002-1310-3389; Li, Tingwen/0000-0002-1900-308X FU National Energy Technology Laboratory's ongoing research in advanced numerical simulation of multiphase flow under RES [DE-FE0004000] FX This technical report was produced in support of the National Energy Technology Laboratory's ongoing research in advanced numerical simulation of multiphase flow under RES contract DE-FE0004000. NR 47 TC 0 Z9 0 U1 14 U2 36 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 1674-2001 EI 2210-4291 J9 PARTICUOLOGY JI Particuology PD APR PY 2016 VL 25 BP 10 EP 22 DI 10.1016/j.partic.2015.06.001 PG 13 WC Engineering, Chemical; Materials Science, Multidisciplinary SC Engineering; Materials Science GA DG1OJ UT WOS:000371837100002 ER PT J AU Duke, DJ Kastengren, AL Mason-Smith, N Chen, Y Young, PM Traini, D Lewis, D Edgington-Mitchell, D Honnery, D AF Duke, Daniel J. Kastengren, Alan L. Mason-Smith, Nicholas Chen, Yang Young, Paul M. Traini, Daniela Lewis, David Edgington-Mitchell, Daniel Honnery, Damon TI Temporally and Spatially Resolved x-ray Fluorescence Measurements of in-situ Drug Concentration in Metered-Dose Inhaler Sprays SO PHARMACEUTICAL RESEARCH LA English DT Article DE fluorescence; pressurized metered dose inhaler; synchrotron radiation; x-ray ID FLUID-DYNAMICS; PARTICLE-SIZE; RADIOGRAPHY; DESIGN; IMPACTOR AB Drug concentration measurements in MDI sprays are typically performed using particle filtration or laser scattering. These techniques are ineffective in proximity to the nozzle, making it difficult to determine how factors such as nozzle design will affect the precipitation of co-solvent droplets in solution-based MDIs, and the final particle distribution. In optical measurements, scattering from the constituents is difficult to separate. We present a novel technique to directly measure drug distribution. A focused x-ray beam was used to stimulate x-ray fluorescence from the bromine in a solution containing 85% HFA, 15% ethanol co-solvent, and 1 / IPBr. Instantaneous concentration measurements were obtained with 1 ms temporal resolution and 5 spatial resolution, providing information in a region that is inaccessible to many other diagnostics. The drug remains homogeneously mixed over time, but was found to be higher at the centerline than at the periphery. This may have implications for oropharyngeal deposition in vivo. Measurements in the dynamic, turbulent region of MDIs allow us to understand the physical links between formulation, inspiration, and geometry on final particle size and distribution. This will ultimately lead to a better understanding of how MDI design can be improved to enhance respirable fraction. C1 [Duke, Daniel J.] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Kastengren, Alan L.] Argonne Natl Lab, XRay Sci Div, Lemont, IL USA. [Mason-Smith, Nicholas; Edgington-Mitchell, Daniel; Honnery, Damon] Monash Univ, Dept Mech & Aerosp Engn, Lab Turbulence Res Aerosp Combust, Melbourne, Vic 3004, Australia. [Chen, Yang; Young, Paul M.; Traini, Daniela] Univ Sydney, Woolcock Inst Med Res, Resp Technol, Sydney, NSW 2006, Australia. [Lewis, David] Chiesi Ltd, Chippenham, England. RP Duke, DJ (reprint author), Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. EM dduke@anl.gov OI Honnery, Damon/0000-0003-2925-3602 FU Australian Research Council; U.S. Department of Energy (DOE) [DE-AC02-06CH11357]; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX The authors thank Dr. Christopher Powell and Dr. Andrew Swantek from the Energy Systems Division at Argonne National Laboratory for their assistance. The authors acknowledge funding support from the Australian Research Council. This research was performed at the 7-BM beam line of the Advanced Photon Source at Argonne National Laboratory. Use of the APS is supported by the U.S. Department of Energy (DOE) under Contract No. DE-AC02-06CH11357.; The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 39 TC 2 Z9 2 U1 3 U2 8 PU SPRINGER/PLENUM PUBLISHERS PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0724-8741 EI 1573-904X J9 PHARM RES-DORDR JI Pharm. Res. PD APR PY 2016 VL 33 IS 4 BP 816 EP 825 DI 10.1007/s11095-015-1828-6 PG 10 WC Chemistry, Multidisciplinary; Pharmacology & Pharmacy SC Chemistry; Pharmacology & Pharmacy GA DF8VO UT WOS:000371638600002 PM 26563204 ER PT J AU Ziebert, F Aranson, IS AF Ziebert, Falko Aranson, Igor S. TI Nonlinear Models in Molecular and Cell Biology SO PHYSICA D-NONLINEAR PHENOMENA LA English DT Editorial Material ID ACTIVE POLAR GELS AB Nonlinear models are important to rationalize and understand self-organization, pattern formation and emergent behavior in molecular and cell biological systems. This special issue focuses on recent developments, that go beyond the classical modeling ideas of biochemical reactions and diffusion processes by including several effects identified recently as being crucial, for instance: elasticity/deformablity, anisotropy, multi-phase flow and 'active' behavior. (C) 2016 Published by Elsevier B.V. C1 [Ziebert, Falko] Univ Freiburg, Inst Phys, D-79104 Freiburg, Germany. [Aranson, Igor S.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Aranson, Igor S.] Northwestern Univ, Engn Sci & Appl Math, 2145 Sheridan Rd, Evanston, IL 60202 USA. RP Ziebert, F (reprint author), Univ Freiburg, Inst Phys, D-79104 Freiburg, Germany.; Aranson, IS (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA.; Aranson, IS (reprint author), Northwestern Univ, Engn Sci & Appl Math, 2145 Sheridan Rd, Evanston, IL 60202 USA. EM falko.ziebert@physik.uni-freiburg.de; aronson@anl.gov NR 25 TC 1 Z9 1 U1 6 U2 20 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2789 EI 1872-8022 J9 PHYSICA D JI Physica D PD APR 1 PY 2016 VL 318 BP 1 EP 2 DI 10.1016/j.physd.2016.02.002 PG 2 WC Mathematics, Applied; Physics, Multidisciplinary; Physics, Mathematical SC Mathematics; Physics GA DG3AY UT WOS:000371943100001 ER PT J AU Winkler, B Aranson, IS Ziebert, F AF Winkler, Benjamin Aranson, Igor S. Ziebert, Falko TI Membrane tension feedback on shape and motility of eukaryotic cells SO PHYSICA D-NONLINEAR PHENOMENA LA English DT Article DE Motility; Bending rigidity; Cytoskeleton ID RAPIDLY MOVING CELLS; SELF-POLARIZATION; RETROGRADE FLOW; LEADING-EDGE; MIGRATION; MODEL; DYNAMICS; FORCE; POLYMERIZATION; LOCOMOTION AB In the framework of a phase field model of a single cell crawling on a substrate, we investigate how the properties of the cell membrane affect the shape and motility of the cell. Since the membrane influences the cell dynamics on multiple levels and provides a nontrivial feedback, we consider the following fundamental interactions: (i) the reduction of the actin polymerization rate by membrane tension; (ii) area conservation of the cell's two-dimensional cross-section vs. conservation of the circumference (i.e. membrane inextensibility); and (iii) the contribution from the membrane's bending energy to the shape and integrity of the cell. As in experiments, we investigate two pertinent observables - the cell's velocity and its aspect ratio. We find that the most important effect is the feedback of membrane tension on the actin polymerization. Bending rigidity has only minor effects, visible mostly in dynamic reshaping events, as exemplified by collisions of the cell with an obstacle. (C) 2015 Elsevier B.V. All rights reserved. C1 [Winkler, Benjamin; Ziebert, Falko] Univ Freiburg, Inst Phys, D-79104 Freiburg, Germany. [Aranson, Igor S.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Aranson, Igor S.] Northwestern Univ, Engn Sci & Appl Math, 2145 Sheridan Rd, Evanston, IL 60202 USA. RP Aranson, IS (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM aronson@anl.gov FU German Science Foundation (DFG) [ZI 1232/2-1]; US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division FX B.W. and F.Z. acknowledge funding from the German Science Foundation (DFG) via project ZI 1232/2-1. I.S.A. was supported by the US Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), Materials Science and Engineering Division. The numerical work was in part performed on the Northern Illinois University GPU cluster GAEA. NR 56 TC 1 Z9 1 U1 5 U2 11 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0167-2789 EI 1872-8022 J9 PHYSICA D JI Physica D PD APR 1 PY 2016 VL 318 BP 26 EP 33 DI 10.1016/j.physd.2015.09.011 PG 8 WC Mathematics, Applied; Physics, Multidisciplinary; Physics, Mathematical SC Mathematics; Physics GA DG3AY UT WOS:000371943100004 ER PT J AU Kolesnichenko, YI Lutsenko, VV Yakovenko, YV Lepiavko, BS Grierson, B Heidbrink, WW Nazikian, R AF Kolesnichenko, Ya I. Lutsenko, V. V. Yakovenko, Yu V. Lepiavko, B. S. Grierson, B. Heidbrink, W. W. Nazikian, R. TI Manifestations of the geodesic acoustic mode driven by energetic ions in tokamaks SO PLASMA PHYSICS AND CONTROLLED FUSION LA English DT Article DE tokamak; energetic ions; geodesic acoustic mode; neutron emission ID N=0 CHIRPING MODE; TRANSPORT; PLASMA; STELLARATORS; EXPLANATION; DIFFUSION; SYSTEMS; WAVES AB Effects of the energetic-ion-driven Geodesic Acoustic modes (GAM and E-GAM) on the toroidally passing energetic ions and the concomitant change of the neutron yield of beam-plasma fusion reactions in tokamaks are considered. It is shown that due to large perturbations of the plasma density, the resonant energetic ions driving the instability can be considerably slowed down for a few tens of the particle transit periods, which is much less than the collisional slowing down time. The time of the collisionless slowing down is actually determined by the period of the particle motion within the resonance island arising because of the GAM / E-GAM. Being trapped in the island, the resonant particles can not only lose their energy but also gain it. One more effect of GAMs is the flattening on the distribution function of the resonant particles. Due to conservation of the canonical angular momentum during a GAM / E-GAM instability, the change of the particle energy is accompanied by a radial displacement of the resonant particle for a distance up to the poloidal Larmor radius of energetic ions. The particles are displaced inwards or outwards, depending on the direction of their motion along the magnetic field. Expressions describing the change of the neutron yield due to GAM modes are derived. It is found that the distortion of the velocity distribution of the resonant particles can lead to a considerable drop of the neutron emission even when effects of the particle radial displacement are small. The developed theory is applied to an E-GAM experiment on the DIII-D tokamak. Relations for the period of the motion within the resonance island of passing (both well passing and marginally passing) particles and the width of the resonance of the energetic particles with GAM modes and low-frequency Alfven modes are derived. C1 [Kolesnichenko, Ya I.; Lutsenko, V. V.; Yakovenko, Yu V.; Lepiavko, B. S.] Inst Nucl Res, Prospekt Nauky 47, UA-03680 Kiev, Ukraine. [Grierson, B.; Nazikian, R.] Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. [Heidbrink, W. W.] Univ Calif Irvine, Irvine, CA 92697 USA. RP Kolesnichenko, YI (reprint author), Inst Nucl Res, Prospekt Nauky 47, UA-03680 Kiev, Ukraine. EM yk@kinr.kiev.ua OI Yakovenko, Yuriy/0000-0002-3499-5275 FU Science and Technology Center in Ukraine [6058]; National Academy of Sciences of Ukraine (NASU) [0114U000678] FX This work was supported in part by the Project No. 6058 of the Science and Technology Center in Ukraine and the National Academy of Sciences of Ukraine (NASU) and the Project No. 0114U000678 of NASU. NR 29 TC 0 Z9 0 U1 0 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0741-3335 EI 1361-6587 J9 PLASMA PHYS CONTR F JI Plasma Phys. Control. Fusion PD APR PY 2016 VL 58 IS 4 AR 045024 DI 10.1088/0741-3335/58/4/045024 PG 16 WC Physics, Fluids & Plasmas SC Physics GA DG1IA UT WOS:000371818600039 ER PT J AU Li, EZ Igochine, V Xu, L Shi, T Zhao, H Liu, Y Ti, A White, R Zhang, J Zhu, Y Huang, J Shen, B Lin, S Qian, J Gong, X Hu, L AF Li, Erzhong Igochine, V. Xu, L. Shi, T. Zhao, H. Liu, Y. Ti, A. White, R. Zhang, J. Zhu, Y. Huang, J. Shen, B. Lin, S. Qian, J. Gong, X. Hu, L. CA EAST Contributors TI The dynamics of a neoclassical tearing mode (NTM) influenced by energetic ions on EAST SO PLASMA PHYSICS AND CONTROLLED FUSION LA English DT Article DE neoclassical tearing mode (NTM); energetic ion; tokamak ID CYCLOTRON CURRENT DRIVE; INTERNAL KINK MODES; DIII-D; MAGNETIC ISLANDS; TOKAMAK PLASMA; ASDEX UPGRADE; STABILIZATION; DISCHARGES; FREQUENCY; JT-60U AB In the 2014 year's campaign of experimental advanced superconducting tokamak (EAST), a series of Magnetohydrodynamics (MHD) instabilities were observed as the launching of Neutral Beam Injection (NBI), the most interesting one of which is the neoclassical tearing mode (NTM). Evidence clearly shows that a kink mode present after a strong sawtooth-like (ST-like) crash leaves a perturbation near the location of the magnetic island, providing the initial seed. The interaction of energetic ions makes the magnetic island oscillate both in island width and in rotation frequency. Analysis indicates that the bulk plasma still dominates the dynamics of NTM, and the orbit excursion of energetic ions induces a polarization current and modifies the width and rotation frequency of the neoclassical magnetic island. C1 [Li, Erzhong; Xu, L.; Shi, T.; Zhao, H.; Liu, Y.; Ti, A.; Zhang, J.; Huang, J.; Shen, B.; Lin, S.; Qian, J.; Gong, X.; Hu, L.] Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Peoples R China. [Igochine, V.] MPI Plasmaphys, D-85748 Garching, Germany. [White, R.] Princeton Univ, Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. [Zhu, Y.] Univ Calif Irvine, Irvine, CA 92697 USA. RP Li, EZ (reprint author), Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Peoples R China. EM rzhonglee@ipp.ac.cn RI White, Roscoe/D-1773-2013 OI White, Roscoe/0000-0002-4239-2685 FU National Natural Science Foundation of China [11405216, 11575249, 11175209]; JSPS-NRF-NSFC A3 Foresight Program in the field of Plasma Physics (NSFC) [11261140328]; National Magnetic Confinement Fusion Energy Research Program [2015GB110005, 2015GB101000] FX This work is supported by the National Natural Science Foundation of China under Grant No. 11405216, 11575249, 11175209, partially by the JSPS-NRF-NSFC A3 Foresight Program in the field of Plasma Physics (NSFC No 11261140328) and by the National Magnetic Confinement Fusion Energy Research Program under Grant Nos. 2015GB110005, 2015GB101000. NR 53 TC 0 Z9 0 U1 9 U2 25 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0741-3335 EI 1361-6587 J9 PLASMA PHYS CONTR F JI Plasma Phys. Control. Fusion PD APR PY 2016 VL 58 IS 4 AR 045012 DI 10.1088/0741-3335/58/4/045012 PG 15 WC Physics, Fluids & Plasmas SC Physics GA DG1IA UT WOS:000371818600027 ER PT J AU Pablant, NA Satake, S Yokoyama, M Gates, DA Bitter, M Bertelli, N Delgado-Aparicio, L Dinklage, A Goto, M Hill, KW Igamai, S Kubo, S Lazerson, S Matsuoka, S Mikkelsen, DR Morita, S Oishi, T Seki, R Shimozuma, T Suzuki, C Suzuki, Y Takahashi, H Yamada, H Yoshimura, Y AF Pablant, N. A. Satake, S. Yokoyama, M. Gates, D. A. Bitter, M. Bertelli, N. Delgado-Aparicio, L. Dinklage, A. Goto, M. Hill, K. W. Igamai, S. Kubo, S. Lazerson, S. Matsuoka, S. Mikkelsen, D. R. Morita, S. Oishi, T. Seki, R. Shimozuma, T. Suzuki, C. Suzuki, Y. Takahashi, H. Yamada, H. Yoshimura, Y. CA LHD Expt Grp TI Investigation of ion and electron heat transport of high-T-e ECH heated discharges in the large helical device SO PLASMA PHYSICS AND CONTROLLED FUSION LA English DT Article DE stellarator; transport; radial electric field; neoclassical; large helical device; x-ray imaging crystal spectrometer; core electron-root confinement ID NEOCLASSICAL TRANSPORT; LHD; STELLARATOR; BARRIERS; PLASMAS; SYSTEM; POWER AB An analysis of the radial electric field and heat transport, both for ions and electrons, is presented for a high-T-e electron cyclotron heated (ECH) discharge on the large helical device (LHD). Transport analysis is done using the task3d transport suite utilizing experimentally measured profiles for both ions and electrons. Ion temperature and perpendicular flow profiles are measured using the recently installed x-ray imaging crystal spectrometer diagnostic (XICS), while electron temperature and density profiles are measured using Thomson scattering. The analysis also includes calculated ECH power deposition profiles as determined through the travis ray-tracing code. This is the first time on LHD that this type of integrated transport analysis with measured ion temperature profiles has been performed without NBI, allowing the heat transport properties of plasmas with only ECH heating to be more clearly examined. For this study, a plasma discharge is chosen which develops a high central electron temperature (T-eo = 9 keV) at moderately low densities (n(eo) = 1.5 x 10(19) m(-3)). The experimentally determined transport properties from task3d are compared to neoclassical predictions as calculated by the gsrake and fortec-3d codes. The predicted electron fluxes are seen to be an order of magnitude less than the measured fluxes, indicating that electron transport is largely anomalous, while the neoclassical and measured ion heat fluxes are of the same magnitude. Neoclassical predictions of a strong positive ambipolar electric field (E-r) in the plasma core are validated through comparisons to perpendicular flow measurements from the XICS diagnostic. This provides confidence that the predictions are producing physically meaningful results for the particle fluxes and radial electric field, which are a key component in correctly predicting plasma confinement. C1 [Pablant, N. A.; Gates, D. A.; Bitter, M.; Bertelli, N.; Delgado-Aparicio, L.; Hill, K. W.; Lazerson, S.; Mikkelsen, D. R.] Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. [Satake, S.; Yokoyama, M.; Goto, M.; Igamai, S.; Kubo, S.; Morita, S.; Oishi, T.; Seki, R.; Shimozuma, T.; Suzuki, C.; Suzuki, Y.; Takahashi, H.; Yamada, H.; Yoshimura, Y.] Natl Inst Nat Sci, Natl Inst Fus Sci, 322-6 Oroshicho, Toki, Gifu 5095292, Japan. [Satake, S.; Yokoyama, M.; Morita, S.; Oishi, T.; Suzuki, Y.; Yamada, H.] SOKENDAI Grad Univ Adv Studies, Toki, Gifu 5095292, Japan. [Dinklage, A.] Max Planck Inst Plasma Phys, D-17491 Greifswald, Germany. [Matsuoka, S.] Res Org Informat Sci & Technol, Kobe, Hyogo 6500047, Japan. RP Pablant, NA (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. EM npablant@pppl.gov RI Lazerson, Samuel/E-4816-2014 OI Lazerson, Samuel/0000-0001-8002-0121 FU US DOE [DE-AC02-09CH11466]; NIFS collaborative Research Programs [NIFS14KNTT025, NIFS13KNST051]; Princeton University FX Research supported by the US DOE under Contract No. DE-AC02-09CH11466 with Princeton University. Development of TASK3D is supported by NIFS collaborative Research Programs NIFS14KNTT025. Part of simulations have been carried out on Plasma Simulator in NIFS under the support by NIFS collaborative Research Programs NIFS13KNST051. NR 36 TC 1 Z9 1 U1 0 U2 12 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0741-3335 EI 1361-6587 J9 PLASMA PHYS CONTR F JI Plasma Phys. Control. Fusion PD APR PY 2016 VL 58 IS 4 AR 045004 DI 10.1088/0741-3335/58/4/045004 PG 10 WC Physics, Fluids & Plasmas SC Physics GA DG1IA UT WOS:000371818600019 ER PT J AU Smith, DR Fonck, RJ McKee, GR Diallo, A Kaye, SM LeBlanc, BP Sabbagh, SA AF Smith, D. R. Fonck, R. J. McKee, G. R. Diallo, A. Kaye, S. M. LeBlanc, B. P. Sabbagh, S. A. TI Evolution patterns and parameter regimes in edge localized modes on the National Spherical Torus Experiment SO PLASMA PHYSICS AND CONTROLLED FUSION LA English DT Article DE edge localized modes; time series analysis; unsupervised machine learning; national spherical torus experiment (NSTX) ID PHYSICS; STABILITY; PEDESTAL; NSTX AB We implement unsupervised machine learning techniques to identify characteristic evolution patterns and associated parameter regimes in edge localized mode (ELM) events observed on the National Spherical Torus Experiment. Multi-channel, localized measurements spanning the pedestal region capture the complex evolution patterns of ELM events on Alfven timescales. Some ELM events are active for less than 100 mu s, but others persist for up to 1 ms. Also, some ELM events exhibit a single dominant perturbation, but others are oscillatory. Clustering calculations with time-series similarity metrics indicate the ELM database contains at least two and possibly three groups of ELMs with similar evolution patterns. The identified ELM groups trigger similar stored energy loss, but the groups occupy distinct parameter regimes for ELM-relevant quantities like plasma current, triangularity, and pedestal height. Notably, the pedestal electron pressure gradient is not an effective parameter for distinguishing the ELM groups, but the ELM groups segregate in terms of electron density gradient and electron temperature gradient. The ELM evolution patterns and corresponding parameter regimes can shape the formulation or validation of nonlinear ELM models. Finally, the techniques and results demonstrate an application of unsupervised machine learning at a data-rich fusion facility. C1 [Smith, D. R.; Fonck, R. J.; McKee, G. R.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. [Diallo, A.; Kaye, S. M.; LeBlanc, B. P.] Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. [Sabbagh, S. A.] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. RP Smith, DR (reprint author), Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. EM drsmith8@wisc.edu FU US Department of Energy, Office of Science, Office of Fusion Energy Sciences [DE-FG02-89ER53296, DE-SC0001288, DE-AC02-09CH11466] FX The author DRS acknowledges helpful discussions with R Maingi. This material is based upon work supported by the US Department of Energy, Office of Science, Office of Fusion Energy Sciences under Award Numbers DE-FG02-89ER53296, DE-SC0001288, and DE-AC02-09CH11466. This research used resources of the National Spherical Torus Experiment-Upgrade, which is a DOE Office of Science User Facility. The digital data for this paper can be found in [13]. NR 25 TC 0 Z9 0 U1 1 U2 6 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0741-3335 EI 1361-6587 J9 PLASMA PHYS CONTR F JI Plasma Phys. Control. Fusion PD APR PY 2016 VL 58 IS 4 AR 045003 DI 10.1088/0741-3335/58/4/045003 PG 16 WC Physics, Fluids & Plasmas SC Physics GA DG1IA UT WOS:000371818600018 ER PT J AU Zweben, SJ Myra, JR Davis, WM D'Ippolito, DA Gray, TK Kaye, SM LeBlanc, BP Maqueda, RJ Russell, DA Stotler, DP AF Zweben, S. J. Myra, J. R. Davis, W. M. D'Ippolito, D. A. Gray, T. K. Kaye, S. M. LeBlanc, B. P. Maqueda, R. J. Russell, D. A. Stotler, D. P. CA NSTX-U Team TI Blob structure and motion in the edge and SOL of NSTX SO PLASMA PHYSICS AND CONTROLLED FUSION LA English DT Article DE tokamak; turbulence; edge ID SCRAPE-OFF LAYER; DIII-D TOKAMAK; COHERENT STRUCTURES; TURBULENCE; TRANSPORT; BOUNDARY AB The structure and motion of discrete plasma blobs (a.k.a. filaments) in the edge and scrape-off layer of NSTX is studied for representative Ohmic and H-mode discharges. Individual blobs were tracked in the 2D radial versus poloidal plane using data from the gas puff imaging diagnostic taken at 400 000 frames s(-1). A database of blob amplitude, size, ellipticity, tilt, and velocity was obtained for similar to 45000 individual blobs. Empirical relationships between various properties are described, e.g. blob speed versus amplitude and blob tilt versus ellipticity. The blob velocities are also compared with analytic models. C1 [Zweben, S. J.; Davis, W. M.; Kaye, S. M.; LeBlanc, B. P.; Maqueda, R. J.; Stotler, D. P.] Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. [Myra, J. R.; D'Ippolito, D. A.; Russell, D. A.] Lodestar Res Corp, Boulder, CO 80301 USA. [Gray, T. K.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Maqueda, R. J.] X Sci LLC, Plainsboro, NJ 08536 USA. RP Zweben, SJ (reprint author), Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. EM szweben@pppl.gov FU USDOE [DE-AC02-09CH11466, DE-FG02-02ER54678] FX We thank for their contributions to this paper and this study in general: J W Ahn, S Banerjee, J A Boedo, O E Garcia, R W Gould, O Grulke, S I Krasheninnikov, S Kubota, R Maingi, T Munsat, S Sabbagh, Y Sechrest, J L Terry. This work was supported by #USDOE Contract DE-AC02-09CH11466 and DE-FG02-02ER54678. The digital data for this paper can be found at: http://arks.princeton.edu/ark:/88435/dsp01vx021h49j. NR 56 TC 7 Z9 7 U1 3 U2 12 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0741-3335 EI 1361-6587 J9 PLASMA PHYS CONTR F JI Plasma Phys. Control. Fusion PD APR PY 2016 VL 58 IS 4 AR 044007 DI 10.1088/0741-3335/58/4/044007 PG 18 WC Physics, Fluids & Plasmas SC Physics GA DG1IA UT WOS:000371818600010 ER PT J AU Yang, ZM Wullschleger, SD Liang, LY Graham, DE Gu, BH AF Yang, Ziming Wullschleger, Stan D. Liang, Liyuan Graham, David E. Gu, Baohua TI Effects of warming on the degradation and production of low-molecular-weight labile organic carbon in an Arctic tundra soil SO SOIL BIOLOGY & BIOCHEMISTRY LA English DT Article DE Soil carbon degradation; Climate warming; Anaerobic fermentation; Methanogenesis; Biogeochemistry; Arctic tundra ID PERMAFROST CARBON; METHANE PRODUCTION; CLIMATE-CHANGE; TEMPERATURE SENSITIVITY; ACIDIC PEAT; METHANOGENESIS; SUBSTRATE; PATHWAYS; MATTER; MINERALIZATION AB The fate of soil organic carbon (SOC) stored in the Arctic permafrost is a key concern as temperatures continue to rise in the northern hemisphere. Studies and conceptual models suggest that degradation of SOC is affected by its composition, but it is unclear exactly which SOC fractions are vulnerable to rapid breakdown and what mechanisms may be controlling SOC degradation upon permafrost thaw. Here, we examine the dynamic consumption and production of labile SOC in an anoxic incubation experiment using soil samples from the active layer at the Barrow Environmental Observatory, Barrow, Alaska, USA. Free-reducing sugars, alcohols, and low-molecular-weight (LMW) organic acids were analyzed during incubation at either -2 or 8 degrees C for up to 240 days. Results show that degradation of simple sugar and alcohol in SOC largely accounts for the initial rapid release of CO2 and CH4 through anaerobic fermentation, whereas the fermentation products, acetate and formate, are subsequently utilized as primary substrates for methanogenesis. Iron(III) reduction is correlated with acetate production and methanogenesis, suggesting its important role as an electron acceptor in SOC respiration in tundra environment. These observations are further supported in a glucose addition experiment, in which rapid CO2 and CH4 production occurred concurrently with rapid production and consumption of labile organics such as acetate. However, addition of tannic acid, as a more complex organic substrate, showed little influence on the overall production of CO2 and CH4 and organic acids. Together our study shows that LIVIW labile SOC controls the initial rapid release of green-house gases upon warming of permafrost soils. We present a conceptual framework for the labile SOC transformations and their relations to fermentation, iron reduction and methanogenesis, thereby providing the basis for improved model prediction of climate feedbacks in the Arctic. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Yang, Ziming; Wullschleger, Stan D.; Liang, Liyuan; Gu, Baohua] Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. [Wullschleger, Stan D.; Graham, David E.] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN USA. [Graham, David E.] Oak Ridge Natl Lab, Biosci Div, Oak Ridge, TN USA. RP Gu, BH (reprint author), Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. EM gub1@ornl.gov RI Graham, David/F-8578-2010; Wullschleger, Stan/B-8297-2012; OI Graham, David/0000-0001-8968-7344; Wullschleger, Stan/0000-0002-9869-0446; Gu, Baohua/0000-0002-7299-2956 FU Office of Biological and Environmental Research in the DOE Office of Science; US DOE [DE-AC05-00OR22725] FX The authors would like to thank Wei Fang, Taniya Roy Chowdhury, Hongmei Chen, Xiangping Yin, and Tonia Mehlhorn for technical assistance and chemical analysis. The Next Generation Ecosystem Experiments (NGEE-Arctic) project is supported by the Office of Biological and Environmental Research in the DOE Office of Science. All data are available in an online data repository (NGEE-Arctic Data Portal, DOI:10.5440/1235032). Oak Ridge National Laboratory is managed by UT-Battelle LLC for US DOE under contract DE-AC05-00OR22725. NR 45 TC 3 Z9 3 U1 30 U2 70 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-0717 J9 SOIL BIOL BIOCHEM JI Soil Biol. Biochem. PD APR PY 2016 VL 95 BP 202 EP 211 DI 10.1016/j.soilbio.2015.12.022 PG 10 WC Soil Science SC Agriculture GA DF7TR UT WOS:000371561000023 ER PT J AU Jiang, YJ Liang, YT Li, CM Wang, F Sui, YY Suvannang, N Zhou, JZ Sun, B AF Jiang, Yuji Liang, Yuting Li, Changming Wang, Feng Sui, Yueyu Suvannang, Nopmanee Zhou, Jizhong Sun, Bo TI Crop rotations alter bacterial and fungal diversity in paddy soils across East Asia SO SOIL BIOLOGY & BIOCHEMISTRY LA English DT Article DE Bacteria; Diversity; Fungi; Network; Paddy soil; Rice-base crop rotations ID MICROBIAL COMMUNITIES; AMMONIA OXIDIZERS; GLOBAL PATTERNS; NETWORKS; BIOGEOGRAPHY; PH; BIODIVERSITY; ABUNDANCE; ECOLOGY; ARCHAEA AB Rice ecosystems are distributed broadly from temperate to tropical regions, but little is known about the underlying mechanisms shaping microbial communities and their network structure in paddy soils at the continental scale. Soil samples were collected from paddy fields across East Asia representing four types of crop rotations: single rice, rice-wheat rotation, double rice, and rice-legume-rice rotation. Here, we describe the roles that crop rotations, environmental heterogeneity and geographical distance play in determining the spatial distribution of microbial communities in paddy soils across East Asia. Our survey revealed remarkable differences in the diversity and composition of microbial operational taxonomic units (OTUs) among four crop rotations. The shared cosmopolitan OTUs Rhizobiales bacterium (genus Bradyrhizobium) and Hypocreales fungus played key-species roles in the ecological networks. A steeper slope of distance decay for the fungal samples compared with the bacterial samples implies a faster turnover in fungal OTU composition across geographical zones. Bacterial communities were affected by soil environmental heterogeneity to an extent that overwhelmed the effect of geographical distance, whereas fungal communities were better predicted by geographical distance. The diversity and composition of bacterial and fungal communities corresponded strongly to soil pH but less strongly to total nitrogen. Remarkably, crop rotations played a key role in determining the changes in microbial diversity, community composition and networks. Taken together, these results provide a baseline ecological framework with which to pursue future research on soil microbial function in paddy soils. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Jiang, Yuji; Liang, Yuting; Li, Changming; Wang, Feng; Sun, Bo] Chinese Acad Sci, Inst Soil Sci, State Key Lab Soil & Sustainable Agr, Nanjing 210008, Jiangsu, Peoples R China. [Li, Changming] Univ Chinese Acad Sci, Beijing 100049, Peoples R China. [Wang, Feng] Ningbo Acad Agr Sci, Ningbo 315040, Zhejiang, Peoples R China. [Sui, Yueyu] Chinese Acad Sci, Northeast Inst Geog & Agr Ecol, Harbin 150040, Peoples R China. [Suvannang, Nopmanee] Land Dev Dept, Off Sci Land Dev, Bangkok 10900, Thailand. [Zhou, Jizhong] Univ Oklahoma, Dept Bot & Microbiol, Inst Environm Genom, Norman, OK 73019 USA. [Zhou, Jizhong] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Sun, B (reprint author), Chinese Acad Sci, Inst Soil Sci, 71 East Beijing Rd, Nanjing 210008, Jiangsu, Peoples R China. EM bsun@issas.ac.cn RI Jiang, Yuji/E-4383-2017 FU Strategic Priority Research Program (B) of the Chinese Academy of Sciences [XDB15010100, XDB15030200]; National Basic Research Program of China [2014CB441003]; National Science Foundation of China [41430856, 41530856]; Science and Technology Service Network Initiative from Chinese Academy of Sciences [KFJ-SW-STS-142] FX We thank Dechen Li, Yongtao Li, Sai Zhou and Chen Jin for their assistance with soil sampling and analysis. This research was supported by grants from the Strategic Priority Research Program (B) of the Chinese Academy of Sciences (XDB15010100, XDB15030200), National Basic Research Program of China (2014CB441003), National Science Foundation of China (41430856, 41530856), and Science and Technology Service Network Initiative from Chinese Academy of Sciences (KFJ-SW-STS-142). NR 104 TC 1 Z9 2 U1 18 U2 80 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0038-0717 J9 SOIL BIOL BIOCHEM JI Soil Biol. Biochem. PD APR PY 2016 VL 95 BP 250 EP 261 DI 10.1016/j.soilbio.2016.01.007 PG 12 WC Soil Science SC Agriculture GA DF7TR UT WOS:000371561000028 ER PT J AU Stenfeldt, C Pacheco, JM Smoliga, GR Bishop, E Pauszek, SJ Hartwig, EJ Rodriguez, LL Arzt, J AF Stenfeldt, C. Pacheco, J. M. Smoliga, G. R. Bishop, E. Pauszek, S. J. Hartwig, E. J. Rodriguez, L. L. Arzt, J. TI Detection of Foot-and-mouth Disease Virus RNA and Capsid Protein in Lymphoid Tissues of Convalescent Pigs Does Not Indicate Existence of a Carrier State SO TRANSBOUNDARY AND EMERGING DISEASES LA English DT Article DE foot-and-mouth disease; FMD; FMDV; virus; persistence; carriers; pigs ID FOLLICULAR DENDRITIC CELL; MONOCLONAL-ANTIBODIES; GERMINAL-CENTERS; INFECTED CATTLE; VIRAL PATHWAYS; SECRETORY IGA; SWINE; PATHOGENESIS; SHEEP; TRANSMISSION AB A systematic study was performed to investigate the potential of pigs to establish and maintain persistent foot-and-mouth disease virus (FMDV) infection. Infectious virus could not be recovered from sera, oral, nasal or oropharyngeal fluids obtained after resolution of clinical infection with any of five FMDV strains within serotypes A, O and Asia-1. Furthermore, there was no isolation of live virus from tissue samples harvested at 28-100 days post-infection from convalescent pigs recovered from clinical or subclinical FMD. Despite lack of detection of infectious FMDV, there was a high prevalence of FMDV RNA detection in lymph nodes draining lesion sites harvested at 35 days post-infection, with the most frequent detection recorded in popliteal lymph nodes (positive detection in 88% of samples obtained from non-vaccinated pigs). Likewise, at 35 dpi, FMDV capsid antigen was localized within follicles of draining lymph nodes, but without concurrent detection of FMDV non-structural protein. There was a marked decline in the detection of FMDV RNA and antigen in tissue samples by 60 dpi, and no antigen or viral RNA could be detected in samples obtained at 100 dpi. The data presented herein provide the most extensive investigation of FMDV persistence in pigs. The overall conclusion is that domestic pigs are unlikely to be competent long-term carriers of infectious FMDV; however, transient persistence of FMDV protein and RNA in lymphoid tissues is common following clinical or subclinical infection. C1 [Stenfeldt, C.; Pacheco, J. M.; Smoliga, G. R.; Bishop, E.; Pauszek, S. J.; Hartwig, E. J.; Rodriguez, L. L.; Arzt, J.] USDA ARS, Plum Isl Anim Dis Ctr, Foreign Anim Dis Res Unit, POB 848, Greenport, NY 11944 USA. [Stenfeldt, C.] Oak Ridge Inst Sci & Educ, PIADC Res Participat Program, Oak Ridge, TN USA. RP Arzt, J (reprint author), USDA ARS, Plum Isl Anim Dis Ctr, Foreign Anim Dis Res Unit, POB 848, Greenport, NY 11944 USA. EM Jonathan.Arzt@ars.usda.gov OI Pacheco, Juan/0000-0001-5477-0201; Arzt, Jonathan/0000-0002-7517-7893 FU National Pork Board, USA (NPB) [11-174]; Plum Island Animal Disease Center Research Participation Program FX This project was funded through a grant financed by The National Pork Board, USA (NPB project identification number: 11-174). CS is a recipient of a Plum Island Animal Disease Center Research Participation Program fellowship, administered by the Oak Ridge Institute for Science and Education (ORISE) through an inter-agency agreement with the US Department of Energy. None of the funding sources had influence upon design or performance of experimental study, interpretation of results or writing of the manuscript. The Korean FMDV isolates were provided by Dr. Kwang-Nyeong Lee, Animal and Plant Quarantine Agency, Minstry of Agriculture, Food and Rural Affairs Republic of Korea. NR 53 TC 5 Z9 5 U1 2 U2 4 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1865-1674 EI 1865-1682 J9 TRANSBOUND EMERG DIS JI Transbound. Emerg. Dis. PD APR PY 2016 VL 63 IS 2 BP 152 EP 164 DI 10.1111/tbed.12235 PG 13 WC Infectious Diseases; Veterinary Sciences SC Infectious Diseases; Veterinary Sciences GA DF9ZJ UT WOS:000371720900021 PM 24943477 ER PT J AU Chang, CY Zhang, W AF Chang, Chin-Yao Zhang, Wei TI Distributed control of inverter-based lossy microgrids for power sharing and frequency regulation under voltage constraints SO AUTOMATICA LA English DT Article DE Microgrid control; Droop control; Frequency synchronization; Power sharing; Voltage regulation ID DROOP CONTROL METHOD; ISLANDED MICROGRIDS; SYSTEMS; GENERATION; DESIGN; STABILITY; OPTIMIZATION; DEFINITION; STRATEGY; STORAGE AB This paper presents a new distributed control framework to coordinate inverter-interfaced distributed energy resources (DERs) in island microgrids. We show that under bounded load uncertainties, the proposed control method can steer the microgrid to a desired steady state with synchronized inverter frequency across the network and proportional sharing of both active and reactive powers among the inverters. We also show that such convergence can be achieved while respecting constraints on voltage magnitude and branch angle differences. The controller is robust under various contingency scenarios, including loss of communication links and failures of DERs. The proposed controller is applicable to lossy mesh microgrids with heterogeneous R/X distribution lines and reasonable parameter variations. Simulations based on various microgrid operation scenarios are also provided to show the effectiveness of the proposed control method. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Chang, Chin-Yao; Zhang, Wei] Ohio State Univ, Dept Elect & Comp Engn, Columbus, OH 43210 USA. [Zhang, Wei] Pacific NW Natl Lab, Elect Infrastruct Grp, Richland, WA 99354 USA. RP Chang, CY; Zhang, W (reprint author), Ohio State Univ, Dept Elect & Comp Engn, Columbus, OH 43210 USA.; Zhang, W (reprint author), Pacific NW Natl Lab, Elect Infrastruct Grp, Richland, WA 99354 USA. EM chang.981@osu.edu; zhang@ece.osu.edu RI Zhang, Wei/B-3219-2013; Zhang, Wei/L-2407-2016 OI Zhang, Wei/0000-0002-7511-2870 FU Laboratory Directed Research and Development under Control of Complex Systems Initiative at Pacific Northwest National Laboratory [DE-AC05-76RL01830] FX This work was funded by Laboratory Directed Research and Development funding under the Control of Complex Systems Initiative at Pacific Northwest National Laboratory, which is operated for the US Department of Energy by Battelle Memorial Institute under Contract DE-AC05-76RL01830. The material in this paper was partially presented at the 2015 American Control Conference, July 1-3, 2015, Chicago, IL, USA. This paper was recommended for publication in revised form by Associate Editor Shun-ichi Azuma under the direction of Editor Toshiharu Sugie. NR 49 TC 0 Z9 0 U1 4 U2 16 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0005-1098 EI 1873-2836 J9 AUTOMATICA JI Automatica PD APR PY 2016 VL 66 BP 85 EP 95 DI 10.1016/j.automatica.2015.12.014 PG 11 WC Automation & Control Systems; Engineering, Electrical & Electronic SC Automation & Control Systems; Engineering GA DF1KT UT WOS:000371099300011 ER PT J AU TerAvest, MA Ajo-Franklin, CM AF TerAvest, Michaela A. Ajo-Franklin, Caroline M. TI Transforming exoelectrogens for biotechnology using synthetic biology SO BIOTECHNOLOGY AND BIOENGINEERING LA English DT Review DE microbial electrochemistry; microbial electrosynthesis; abiotic-biotic interface; anode-respiring bacteria; extracellular electron transfer ID MICROBIAL FUEL-CELLS; SHEWANELLA-ONEIDENSIS MR-1; EXTRACELLULAR ELECTRON-TRANSFER; GEOBACTER-SULFURREDUCENS; ESCHERICHIA-COLI; ANAEROBIC RESPIRATION; CLOSTRIDIUM-LJUNGDAHLII; PSEUDOMONAS-AERUGINOSA; GENE-EXPRESSION; ENHANCEMENT AB Extracellular electron transfer pathways allow certain bacteria to transfer energy between intracellular chemical energy stores and extracellular solids through redox reactions. Microorganisms containing these pathways, exoelectrogens, are a critical part of microbial electrochemical technologies that aim to impact applications in bioenergy, biosensing, and biocomputing. However, there are not yet any examples of economically viable microbial electrochemical technologies due to the limitations of naturally occurring exoelectrogens. Here we first briefly summarize recent discoveries in understanding extracellular electron transfer pathways, then review in-depth the creation of customized and novel exoelectrogens for biotechnological applications. We analyze engineering efforts to increase current production in native exoelectrogens, which reveals that modulating certain processes within extracellular electron transfer are more effective than others. We also review efforts to create new exoelectrogens and highlight common challenges in this work. Lastly, we summarize work utilizing engineered exoelectrogens for biotechnological applications and the key obstacles to their future development. Fueled by the development of genetic tools, these approaches will continue to expand and genetically modified organisms will continue to improve the outlook for microbial electrochemical technologies. (c) 2015 Wiley Periodicals, Inc. C1 [TerAvest, Michaela A.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Ajo-Franklin, Caroline M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Ajo-Franklin, Caroline M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Ajo-Franklin, Caroline M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Synthet Biol Inst, Berkeley, CA 94720 USA. RP Ajo-Franklin, CM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.; Ajo-Franklin, CM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Ajo-Franklin, CM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Synthet Biol Inst, Berkeley, CA 94720 USA. EM cajo-franklin@lbl.gov FU Office of Naval Research [N000141310551]; Office of Science, Office of Basic Energy Sciences [DE-AC02-05CH11231] FX Contract grant sponsor: Office of Naval Research; Contract grant number: N000141310551; Contract grant sponsor: Office of Science, Office of Basic Energy Sciences; Contract grant number: DE-AC02-05CH11231 NR 83 TC 10 Z9 11 U1 12 U2 82 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0006-3592 EI 1097-0290 J9 BIOTECHNOL BIOENG JI Biotechnol. Bioeng. PD APR PY 2016 VL 113 IS 4 BP 687 EP 697 DI 10.1002/bit.25723 PG 11 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA DF5YT UT WOS:000371429700001 PM 26284614 ER PT J AU Regnier, D Litaize, O Serot, O AF Regnier, D. Litaize, O. Serot, O. TI An improved numerical method to compute neutron/gamma deexcitation cascades starting from a high spin state SO COMPUTER PHYSICS COMMUNICATIONS LA English DT Article DE Hauser-Feshbach; Statistical model; Deexcitation; Cascade; FIFRELIN ID SPONTANEOUS FISSION; ANGULAR-MOMENTUM; CROSS-SECTION; GAMMA-RAYS; SIMULATION; EMISSION; CAPTURE; NUCLEI; CF-252; ASSIGNMENT AB Numerous nuclear processes involve the deexcitation of a compound nucleus through the emission of several neutrons, gamma-rays and/or conversion electrons. The characteristics of such a deexcitation are commonly derived from a total statistical framework often called "Hauser Feshbach" method. In this work, we highlight a numerical limitation of this kind of method in the case of the deexcitation of a high spin initial state. To circumvent this issue, an improved technique called the Fluctuating Structure Properties (FSP) method is presented. Two FSP algorithms are derived and benchmarked on the calculation of the total radiative width for a thermal neutron capture on U-238. We compare the standard method with these FSP algorithms for the prediction of particle multiplicities in the deexcitation of a high spin level of Ba-143. The gamma multiplicity turns out to be very sensitive to the numerical method. The bias between the two techniques can reach 1.5 gamma/cascade. Finally, the uncertainty of these calculations coming from the lack of knowledge on nuclear structure is estimated via the FSP method. (C) 2016 Elsevier B.V. All rights reserved. C1 [Regnier, D.; Litaize, O.; Serot, O.] Cadarache, SPRC, DER, CEA,DEN, F-13108 St Paul Les Durance, France. [Regnier, D.] Lawrence Livermore Natl Lab, Nucl & Chem Sci Div, Livermore, CA 94551 USA. RP Litaize, O (reprint author), Cadarache, SPRC, DER, CEA,DEN, F-13108 St Paul Les Durance, France. EM olivier.litaize@cea.fr FU U.S. Department of Energy [DE-AC52-07NA27344] FX This work was partly performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 34 TC 0 Z9 0 U1 2 U2 7 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0010-4655 EI 1879-2944 J9 COMPUT PHYS COMMUN JI Comput. Phys. Commun. PD APR PY 2016 VL 201 BP 19 EP 28 DI 10.1016/j.cpc.2015.12.007 PG 10 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DF7QQ UT WOS:000371553100003 ER PT J AU Coon, ET Moulton, JD Painter, SL AF Coon, Ethan T. Moulton, J. David Painter, Scott L. TI Managing complexity in simulations of land surface and near-surface processes SO ENVIRONMENTAL MODELLING & SOFTWARE LA English DT Article DE Multiphysics; Framework; Directed acyclic graph; Land surface modeling; Thermal hydrology ID MODEL AB Increasing computing power and the growing role of simulation in Earth systems science have led to an increase in the number and complexity of processes in modern simulators. We present a multiphysics framework that specifies interfaces for coupled processes and automates weak and strong coupling strategies to manage this complexity. Process management is enabled by viewing the system of equations as a tree, where individual equations are associated with leaf nodes and coupling strategies with internal nodes. A dynamically generated dependency graph connects a variable to its dependencies, streamlining and automating model evaluation, easing model development, and ensuring models are modular and flexible. Additionally, the dependency graph is used to ensure that data requirements are consistent between all processes in a given simulation. Here we discuss the design and implementation of these concepts within the Arcos framework, and demonstrate their use for verification testing and hypothesis evaluation in numerical experiments. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Coon, Ethan T.] Los Alamos Natl Lab, Computat Earth Sci, Los Alamos, NM 87545 USA. [Moulton, J. David] Los Alamos Natl Lab, Appl Math & Plasma Phys, Los Alamos, NM 87545 USA. [Painter, Scott L.] Oak Ridge Natl Lab, Div Environm Sci, Climate Change Sci Inst, Oak Ridge, TN USA. RP Coon, ET (reprint author), Los Alamos Natl Lab, Computat Earth Sci, Los Alamos, NM 87545 USA. EM ecoon@lanl.gov RI Painter, Scott/C-2586-2016 OI Painter, Scott/0000-0002-0901-6987 FU Los Alamos National Laboratory LDRD [20110068DR]; Department of Energy's Office of Science Next Generation Ecosystem Experiment (NGEE) Arctic project; Department of Energy's Office of Science Interoperable Design for Extreme-scale Application Software (IDEAS) [LA-UR-14-25386] FX This work was supported by the Los Alamos National Laboratory LDRD project 20110068DR, the Department of Energy's Office of Science Next Generation Ecosystem Experiment (NGEE) Arctic project, and the Department of Energy's Office of Science Interoperable Design for Extreme-scale Application Software (IDEAS). LA-UR-14-25386. NR 19 TC 5 Z9 5 U1 0 U2 3 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1364-8152 EI 1873-6726 J9 ENVIRON MODELL SOFTW JI Environ. Modell. Softw. PD APR PY 2016 VL 78 BP 134 EP 149 DI 10.1016/j.envsoft.2015.12.017 PG 16 WC Computer Science, Interdisciplinary Applications; Engineering, Environmental; Environmental Sciences SC Computer Science; Engineering; Environmental Sciences & Ecology GA DF5FS UT WOS:000371377800011 ER PT J AU Tandon, P Huggins, P Maclachlan, R Dubrawski, A Nelson, K Labov, S AF Tandon, Prateek Huggins, Peter Maclachlan, Rob Dubrawski, Artur Nelson, Karl Labov, Simon TI Detection of radioactive sources in urban scenes using Bayesian Aggregation of data from mobile spectrometers SO INFORMATION SYSTEMS LA English DT Article DE Machine learning; Data fusion; Bayesian methods ID LOCALIZATION AB Mobile radiation detector systems aim to help identify dangerous sources of radiation while minimizing frequency of false alarms caused by non-threatening nuisance sources prevalent in cluttered urban scenes. We develop methods for spatially aggregating evidence from multiple spectral observations to simultaneously detect and infer properties of threatening radiation sources. Our Bayesian Aggregation (BA) framework allows sensor fusion across multiple measurements to boost detection capability of a radioactive point source, providing several key innovations previously unexplored in the literature. Our method learns the expected Signal-to-Noise Ratio (SNR) trend as a function of source exposure using Bayesian non-parametrics to enable robust detection. The method scales well in spatial search by leveraging conditional independence and locality in Bayesian updates. The framework also allows modeling of source parameters such as intensity or type to enable property characterization of detected sources. Approaches for incorporating modeling information into BA are compared and benchmarked with respect to other data fusion techniques. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Tandon, Prateek; Huggins, Peter; Maclachlan, Rob; Dubrawski, Artur] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Nelson, Karl; Labov, Simon] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Tandon, P (reprint author), Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. EM prateekt@andrew.cmu.edu FU United States Department of Homeland Security, Domestic Nuclear Detection Office [2010-DN-077-ARI040-02]; United States Department of Defense, Defense Threat Reduction Agency [HDTRA1-13-1-0026]; United States Department of Energy [DE-NA0001736]; National Science Foundation [0911032, 1320347]; United States Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344] FX This work has been partially supported by the United States Department of Homeland Security, Domestic Nuclear Detection Office, under competitively awarded Grant 2010-DN-077-ARI040-02; the United States Department of Defense, Defense Threat Reduction Agency, under Award HDTRA1-13-1-0026; the United States Department of Energy, under Grant DE-NA0001736; and the National Science Foundation under Awards 0911032 and 1320347. Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the United States Department of Energy, National Nuclear Security Administration under Contract DE-AC52-07NA27344. This support does not constitute an express or implied endorsement on the part of the United States Government. NR 18 TC 0 Z9 0 U1 3 U2 13 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4379 EI 1873-6076 J9 INFORM SYST JI Inf. Syst. PD APR PY 2016 VL 57 BP 195 EP 206 DI 10.1016/j.is.2015.10.006 PG 12 WC Computer Science, Information Systems SC Computer Science GA DF4YR UT WOS:000371358900013 ER PT J AU Wang, X Wraith, M Burke, S Rathbun, H DeVlugt, K AF Wang, Xuan Wraith, Matthew Burke, Stephen Rathbun, Howard DeVlugt, Kyle TI Densification of W-Ni-Fe powders using laser sintering SO INTERNATIONAL JOURNAL OF REFRACTORY METALS & HARD MATERIALS LA English DT Article DE Additive manufacturing; Laser sintering; Densification; Microstructure; Tungsten-nickel-iron ID TUNGSTEN; MICROSTRUCTURE; ALLOYS; TEMPERATURE; MECHANISMS AB In this paper, Laser Sintering (IS) of 90%W-7%Ni-3%Fe (wt.%) powders have been investigated, with the goal to understand the influence of final density by laser power, scanning speed, laser trace width, and the number of scanning passes. The results suggest that the laser power and scanning speed are the most important factors influencing density; the influence of trace width and number of scanning passes are not significant. With the increase of laser power and decrease of scanning speed, higher density can be achieved. The microstructure analysis indicated that the porosity changed from open porosity to closed porosity with higher laser energy input. Energy-Dispersive X-ray Spectroscopy (EDX) analysis shows that during the sintering process, W was not melted but dissolved into the Ni-Fe matrix. Contact flattening and grain accommodation of W grains have been observed. It suggests that both rearrangement and solution-reprecipitation mechanisms are responsible for the densification. The sintered density with respect to laser power and scanning speed was modeled by continuum modeling theory and compared with experimental results. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Wang, Xuan; DeVlugt, Kyle] Calif Polytech State Univ San Luis Obispo, Ind & Mfg Dept, 1 Grand Ave, San Luis Obispo, CA 93407 USA. [Wraith, Matthew; Burke, Stephen; Rathbun, Howard] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. RP Wang, X (reprint author), Calif Polytech State Univ San Luis Obispo, Ind & Mfg Dept, 1 Grand Ave, San Luis Obispo, CA 93407 USA. EM xwang12@calpoly.edu; wraith1@llnl.gov; burke24@llnl.gov; rathbun4@llnl.gov; ktdevlug@calpoly.edu FU R-IDC; College of Engineering from California Polytechnic State University San Luis Obispo FX The author would greatly thank the experimental support by Lawrence Livermore National Laboratory, and the support from R-IDC and College of Engineering from California Polytechnic State University San Luis Obispo. The sample preparation and SEM work has been supported Dr. Katherine Chen from Materials Engineering Department, and Dr. Richard Savage from Biomedical & General Engineering at Cal Poly. NR 25 TC 1 Z9 1 U1 5 U2 9 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0263-4368 J9 INT J REFRACT MET H JI Int. J. Refract. Met. Hard Mat. PD APR PY 2016 VL 56 BP 145 EP 150 DI 10.1016/j.ijrmhm.2016.01.006 PG 6 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DF2QA UT WOS:000371187700020 ER PT J AU Srivastava, S Kishore, S Narayanan, S Sandy, AR Bhatia, SR AF Srivastava, Sunita Kishore, Suhasini Narayanan, Suresh Sandy, Alec R. Bhatia, Surita R. TI Multiple Dynamic Regimes in Colloid-Polymer Dispersions: New Insight Using X-Ray Photon Correlation Spectroscopy SO JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS LA English DT Article DE colloids; gels; nanoparticles ID LAPONITE-PEO MIXTURES; POLY(ETHYLENE OXIDE); LIGHT-SCATTERING; NANOCOMPOSITE HYDROGELS; AQUEOUS DISPERSIONS; GLASS-TRANSITION; AGING BEHAVIOR; SHAKE-GELS; CLAY; SUSPENSIONS AB We present an X-ray photon correlation spectroscopy (XPCS) study of dynamic transitions in an anisotropic colloid-polymer dispersion with multiple arrested states. The results provide insight into the mechanism for formation of repulsive glasses, attractive glasses, and networked gels of colloids with weakly adsorbing polymer chains. In the presence of adsorbing polymer chains, we observe three distinct regimes: a state with slow dynamics consisting of finite particles and clusters, for which interparticle interactions are predominantly repulsive; a second dynamic regime occurring above the saturation concentration of added polymer, in which small clusters of nanoparticles form via a short-range depletion attraction; and a third regime above the overlap concentration in which dynamics of clusters are independent of polymer chain length. The observed complex dynamic state diagram is primarily governed by the structural reorganization of a nanoparticle cluster and polymer chains at the nanoparticle-polymer surface and in the concentrated medium, which in turn controls the dynamics of the dispersion. (C) 2015 Wiley Periodicals, Inc. C1 [Srivastava, Sunita; Kishore, Suhasini; Bhatia, Surita R.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Srivastava, Sunita] Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA. [Kishore, Suhasini] Univ Massachusetts, Dept Chem Engn, Amherst, MA 01003 USA. [Narayanan, Suresh; Sandy, Alec R.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Bhatia, Surita R.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Srivastava, S; Bhatia, SR (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.; Srivastava, S (reprint author), Natl Inst Stand & Technol, Gaithersburg, MD 20899 USA.; Bhatia, SR (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM sunita.srivastava@nist.gov; surita.bhatia@stonybrook.edu RI Bhatia, Surita/B-4536-2008 FU National Science Foundation [CBET-1335787]; U.S. Department of Energy Office of Science [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-98CH10886] FX This work was supported by the National Science Foundation, Award No. CBET-1335787. Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy Office of Science under contract DE-AC02-06CH11357. Research carried out in part at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NR 65 TC 2 Z9 2 U1 5 U2 27 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0887-6266 EI 1099-0488 J9 J POLYM SCI POL PHYS JI J. Polym. Sci. Pt. B-Polym. Phys. PD APR 1 PY 2016 VL 54 IS 7 BP 752 EP 760 DI 10.1002/polb.23973 PG 9 WC Polymer Science SC Polymer Science GA DF6UQ UT WOS:000371492800007 ER PT J AU Mardkhe, MK Huang, BY Bartholomew, CH Alam, TM Woodfield, BF AF Mardkhe, Maryam Khosravi Huang, Baiyu Bartholomew, Calvin H. Alam, Todd M. Woodfield, Brian F. TI Synthesis and characterization of silica doped alumina catalyst support with superior thermal stability and unique pore properties SO JOURNAL OF POROUS MATERIALS LA English DT Article DE Silica-doped alumina; Thermally stable; Large pore size; High surface area ID HIGH-TEMPERATURE STABILITY; MESOPOROUS GAMMA-ALUMINA; LARGE SURFACE-AREA; HYDROTHERMAL TREATMENT; ELEVATED-TEMPERATURES; SIZE DISTRIBUTION; GEL SURFACE; ACID; AEROGEL; NMR AB A facile, solvent-deficient, one-pot synthesis of a thermally stable silica-doped alumina, having high surface area, large pore volume and uniquely large pores, has been developed. Silica-doped alumina (SDA) was synthesized by adding 5 wt% silica from tetraethyl orthosilicate (TEOS) to aluminum isoproxide (AIP), a 1:5 mol ratio AIP to water, and a 1:2 mol ratio TEOS to water in the absence of a template. The structure of silica-doped alumina was studied by in situ high-temperature powder XRD, nitrogen adsorption, thermogravimetric analysis, solid-state NMR, and TEM. The addition of silica significantly increases the stability of gamma-Al2O3 phase to 1200 A degrees C while maintaining a high surface area, a large pore volume and a large pore diameter. After calcination at 1100 A degrees C for 2 h, a surface area of 160 m(2)/g, pore volume of 0.99 cm(3)/g, and a bimodal pore size distribution of 23 and 52 nm are observed. Compared to a commercial silica-doped alumina, after calcination for 24 h at 1100 A degrees C, the surface area, pore volume, and pore diameter SDA are higher by 46, 155, and 94 %, respectively. Results reveal that Si stabilizes the porous structure of gamma-Al2O3 up to 1200 A degrees C, while unstabilized alumina is stable to only 900 A degrees C. From our data, we infer that Si enters tetrahedral vacancies in the defect spinel structure of alumina without moving Al from tetrahedral positions and forms a silica-alumina interface. C1 [Mardkhe, Maryam Khosravi; Huang, Baiyu; Woodfield, Brian F.] Brigham Young Univ, Dept Chem & Biochem, Provo, UT 84602 USA. [Bartholomew, Calvin H.] Brigham Young Univ, Dept Chem Engn, Provo, UT 84602 USA. [Alam, Todd M.] Sandia Natl Labs, Dept Elect Opt & Nanostruct Mat, Albuquerque, NM 87185 USA. RP Woodfield, BF (reprint author), Brigham Young Univ, Dept Chem & Biochem, Provo, UT 84602 USA. EM Brian_woodfield@byu.edu RI Huang, Baiyu/N-2739-2016 OI Huang, Baiyu/0000-0001-9472-2765 FU U.S. Department of Energy [DE-FG02-05ER15666]; National Science Foundation [CHE-0959862]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the U.S. Department of Energy under grant DE-FG02-05ER15666 and National Science Foundation under CHE-0959862. The solid state NMR (TMA) was performed at Sandia National Laboratories which is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. We also thank Dr. Jeff Farrer and the BYU microscopy lab for their assistance with the TEM imaging. NR 55 TC 1 Z9 1 U1 9 U2 47 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 1380-2224 EI 1573-4854 J9 J POROUS MAT JI J. Porous Mat. PD APR PY 2016 VL 23 IS 2 BP 475 EP 487 DI 10.1007/s10934-015-0101-z PG 13 WC Chemistry, Applied; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DF4DN UT WOS:000371297700021 ER PT J AU Manjasetty, BA Halavaty, AS Luan, CH Osipiuk, J Mulligan, R Kwon, K Anderson, WF Joachimiak, A AF Manjasetty, Babu A. Halavaty, Andrei S. Luan, Chi-Hao Osipiuk, Jerzy Mulligan, Rory Kwon, Keehwan Anderson, Wayne F. Joachimiak, Andrzej TI Loop-to-helix transition in the structure of multidrug regulator AcrR at the entrance of the drug-binding cavity SO JOURNAL OF STRUCTURAL BIOLOGY LA English DT Article DE Transcription regulator; TetR/AcrR; Multidrug resistance; Loop-to-helix transition ID ENTERICA SEROVAR TYPHIMURIUM; ORGANIC-SOLVENT TOLERANCE; ESCHERICHIA-COLI; CRYSTAL-STRUCTURE; TETR FAMILY; MYCOBACTERIUM-TUBERCULOSIS; TRANSCRIPTIONAL REGULATOR; ANTIBIOTIC-RESISTANCE; UNITED-STATES; REPRESSOR AB Multidrug transcription regulator AcrR from Salmonella enterica subsp. enterica serovar Typhimurium str. LT2 belongs to the tetracycline repressor family, one of the largest groups of bacterial transcription factors. The crystal structure of dimeric AcrR was determined and refined to 1.56 angstrom resolution. The tertiary and quaternary structures of AcrR are similar to those of its homologs. The multidrug binding site was identified based on structural alignment with homologous proteins and has a di(hydroxyethyl)ether molecule bound. Residues from helices alpha 4 and alpha 7 shape the entry into this binding site. The structure of AcrR reveals that the extended helical conformation of helix alpha 4 is stabilized by the hydrogen bond between Glu67 (helix alpha 4) and Gln130 (helix alpha 7). Based on the structural comparison with the closest homolog structure, the Escherichia coli AcrR, we propose that this hydrogen bond is responsible for control of the loop-to-helix transition within helix alpha 4. This local conformational switch of helix alpha 4 may be a key step in accessing the multidrug binding site and securing ligands at the binding site. Solution small molecule binding studies suggest that AcrR binds ligands with their core chemical structure resembling the tetracyclic ring of cholesterol. (C) 2016 Published by Elsevier Inc. C1 [Manjasetty, Babu A.] European Mol Biol Lab, Grenoble Outstn, 71 Ave Martyrs, F-38042 Grenoble, France. [Manjasetty, Babu A.] Univ Grenoble Alpes, UVHCI, F-38042 Grenoble, France. [Halavaty, Andrei S.; Anderson, Wayne F.] Northwestern Univ, Feinberg Sch Med, Biochem & Mol Genet, 303 East Chicago Ave, Chicago, IL 60611 USA. [Halavaty, Andrei S.; Luan, Chi-Hao; Osipiuk, Jerzy; Mulligan, Rory; Kwon, Keehwan; Anderson, Wayne F.; Joachimiak, Andrzej] Ctr Struct Genom Infect Dis, 303 East Chicago Ave, Chicago, IL 60626 USA. [Luan, Chi-Hao] Northwestern Univ, High Throughput Anal Lab, 2205 Tech Dr, Evanston, IL 60208 USA. [Osipiuk, Jerzy; Mulligan, Rory; Joachimiak, Andrzej] Univ Chicago, Computat Inst, 5735 S Ellis Ave, Chicago, IL 60637 USA. [Osipiuk, Jerzy; Mulligan, Rory; Joachimiak, Andrzej] Argonne Natl Lab, Struct Biol Ctr, 9700 S Cass Ave, Argonne, IL 60439 USA. [Kwon, Keehwan] J Craig Venter Inst, Infect Dis, 9714 Med Ctr Dr, Rockville, MD 20850 USA. RP Halavaty, AS (reprint author), Northwestern Univ, Feinberg Sch Med, Biochem & Mol Genet, 303 East Chicago Ave, Chicago, IL 60611 USA.; Joachimiak, A (reprint author), Univ Chicago, Computat Inst, 5735 S Ellis Ave, Chicago, IL 60637 USA. EM a-halavaty@northwestern.edu; andrzejj@anl.gov OI Luan, Chi-Hao/0000-0002-2131-379X; Manjasetty, Dr. Babu/0000-0002-8229-4748 FU National Institute of Allergy and Infectious Diseases, National Institutes of Health, U.S. Department of Health and Human Services [HHSN272200700058C, HHSN272201200026C]; U.S. Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357] FX The CSGID project has been funded in whole or in part with Federal funds from the National Institute of Allergy and Infectious Diseases, National Institutes of Health, U.S. Department of Health and Human Services, under Contracts No. HHSN272200700058C and HHSN272201200026C. We thank Sankar Krishnna for the human ENO1 sample. The authors wish to thank members of the Structural Biology Center (SBC) at Argonne National Laboratory for their help with X-ray diffraction data collection. The operation of SBC beamlines is supported by the U.S. Department of Energy, Office of Biological and Environmental Research under contract DE-AC02-06CH11357. NR 56 TC 1 Z9 1 U1 1 U2 9 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 1047-8477 EI 1095-8657 J9 J STRUCT BIOL JI J. Struct. Biol. PD APR PY 2016 VL 194 IS 1 BP 18 EP 28 DI 10.1016/j.jsb.2016.01.008 PG 11 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA DF2SH UT WOS:000371193600003 PM 26796657 ER PT J AU Ajayi, OO Lorenzo-Martin, C Fenske, G Corlett, J Murphy, C Przesmitzki, S AF Ajayi, Oyelayo O. Lorenzo-Martin, Cinta Fenske, George Corlett, John Murphy, Chris Przesmitzki, Steve TI Bioderived Fuel Blend Dilution of Marine Engine Oil and Impact on Friction and Wear Behavior SO JOURNAL OF TRIBOLOGY-TRANSACTIONS OF THE ASME LA English DT Article ID SPARK-IGNITION ENGINE; ETHANOL-GASOLINE; BUTANOL; INJECTION; EMISSIONS; VISCOSITY; MIXTURES AB To reduce the amount of petroleum-derived fuel used in vehicles and vessels powered by internal combustion engines (ICEs), the addition of bioderived fuel extenders is a common practice. Ethanol is perhaps the most common bioderived fuel used for blending, and butanol is being evaluated as a promising alternative. The present study determined the fuel dilution rate of three lubricating oils (pure gasoline (E0), gasoline-10% ethanol blend (E10), and gasoline-16% isobutanol blend (i-B16)) in a marine engine operating in on-water conditions with a start-and-stop cycle protocol. The level of fuel dilution increased with the number of cycles for all three fuels. The most dilution was observed with i-B16 fuel, and the least with E10 fuel. In all cases, fuel dilution substantially reduced the oil viscosity. The impacts of fuel dilution and the consequent viscosity reduction on the lubricating capability of the engine oil in terms of friction, wear, and scuffing prevention were evaluated by four different tests protocols. Although the fuel dilution of the engine oil had minimal effect on friction, because the test conditions were under the boundary lubrication regime, significant effects were observed on wear in many cases. Fuel dilution was also observed to reduce the load-carrying capacity of the engine oils in terms of scuffing load reduction. C1 [Ajayi, Oyelayo O.; Lorenzo-Martin, Cinta; Fenske, George] Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. [Corlett, John; Murphy, Chris] Yamaha Motor Corp USA, Kennesaw, GA 30144 USA. [Przesmitzki, Steve] DOE HQ, Fuels & Lube Technol Program VTO, Washington, DC 20585 USA. RP Ajayi, OO (reprint author), Argonne Natl Lab, Div Energy Syst, Argonne, IL 60439 USA. EM ajayi@anl.gov FU U.S. Department of Energy, Energy Efficiency and Renewable Energy, Office of Vehicle Technologies [DE-AC02-06CH11357]; UChicago Argonne, LLC [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, under Contract No. DE-AC02-06CH11357. The electron microscopy was accomplished at the Electron Microscopy Center at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC. NR 16 TC 2 Z9 2 U1 4 U2 10 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0742-4787 EI 1528-8897 J9 J TRIBOL-T ASME JI J. Tribol.-Trans. ASME PD APR PY 2016 VL 138 IS 2 AR 021603 DI 10.1115/1.4031781 PG 11 WC Engineering, Mechanical SC Engineering GA DF5JU UT WOS:000371388800019 ER PT J AU Buchheit, TE Susan, DF Massad, JE Mcelhanon, JR Noebe, RD AF Buchheit, Thomas E. Susan, Donald F. Massad, Jordan E. Mcelhanon, James R. Noebe, Ronald D. TI Mechanical and Functional Behavior of High-Temperature Ni-Ti-Pt Shape Memory Alloys SO METALLURGICAL AND MATERIALS TRANSACTIONS A-PHYSICAL METALLURGY AND MATERIALS SCIENCE LA English DT Article AB A series of Ti-rich Ni-Ti-Pt ternary alloys with 13 to 18 at. pct Pt were processed by vacuum arc melting and characterized for their transformation behavior to identify shape memory alloys (SMA) that undergo transformation between 448 K and 498 K (175 A degrees C and 225 A degrees C) and achieve recoverable strain exceeding 2 pct. From this broader set of compositions, three alloys containing 15.5 to 16.5 at. pct Pt exhibited transformation temperatures in the vicinity of 473 K (200 A degrees C), thus were targeted for more detailed characterization. Preliminary microstructural evaluation of these three compositions revealed a martensitic microstructure with small amounts of Ti-2(Ni,Pt) particles. Room temperature mechanical testing gave a response characteristic of martensitic de-twinning followed by a typical work-hardening behavior to failure. Elevated mechanical testing, performed while the materials were in the austenitic state, revealed yield stresses of approximately 500 MPa and 3.5 pct elongation to failure. Thermal strain recovery characteristics were more carefully investigated with unbiased incremental strain-temperature tests across the 1 to 5 pct strain range, as well as cyclic strain-temperature tests at 3 pct strain. The unbiased shape recovery results indicated a complicated strain recovery path, dependent on prestrain level, but overall acceptable SMA behavior within the targeted temperature and recoverable strain range. C1 [Buchheit, Thomas E.; Susan, Donald F.; Massad, Jordan E.; Mcelhanon, James R.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Noebe, Ronald D.] NASA, Glenn Res Ctr, Cleveland, OH 44135 USA. RP Buchheit, TE (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM tebuchh@sandia.gov FU NASA Transformative Aeronautics Concepts Program (TACP), Transformational Tools and Technologies Project FX The authors wish to thank Mark Reece for expertise in arc button melting. Bonnie McKenzie and Alice Kilgo are acknowledged for SEM work and metallographic sample preparation. Thanks also to Don Bradley for DSC analysis, Dave Schmale for expert mechanical testing, and Dereck Johnson for the ICP analyses. Thanks to Dr. Anita Garg for helpful discussions and detailed microstructural characterization and Dr. Ken Eckelmeyer for careful review of the manuscript. RDN would like to acknowledge additional support from the NASA Transformative Aeronautics Concepts Program (TACP), Transformational Tools and Technologies Project. NR 23 TC 0 Z9 0 U1 1 U2 7 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1073-5623 EI 1543-1940 J9 METALL MATER TRANS A JI Metall. Mater. Trans. A-Phys. Metall. Mater. Sci. PD APR PY 2016 VL 47A IS 4 BP 1587 EP 1599 DI 10.1007/s11661-016-3324-y PG 13 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DF4HA UT WOS:000371307400011 ER PT J AU Demas, NG Lorenzo-Martin, C Ajayi, OO Erck, RA Shareef, I AF Demas, Nicholaos G. Lorenzo-Martin, Cinta Ajayi, Oyelayo O. Erck, Robert A. Shareef, Iqbal TI Measurement of Thin-film Coating Hardness in the Presence of Contamination and Roughness: Implications for Tribology SO METALLURGICAL AND MATERIALS TRANSACTIONS A-PHYSICAL METALLURGY AND MATERIALS SCIENCE LA English DT Article ID MECHANICAL-PROPERTIES; WEAR-RESISTANCE; ELASTIC-MODULUS; INDENTATION; NANOINDENTATION; MICROSTRUCTURE AB Standard nanoindentation measurements on commercially available TiAlN, CrN, metal-containing diamond-like carbon, and TiN coatings, deposited on steel substrates were performed to determine coating hardness and elastic modulus. It was found that the coating surface roughness/morphology present after deposition can significantly affect the measurements of nanomechanical properties so that measurements of these properties on the as-deposited coating surface may be significantly different from the bulk. In addition, a surface measurement may produce a lower nanohardness due to the existence of a soft surface contamination layer. A simple method was developed to enable accurate measurement of the nanomechanical properties of coatings, while avoiding errors introduced by surface topography and the presence of superficial contamination layers on thin films. Friction and wear behavior, as well as the wear mechanisms in dry reciprocating sliding contact of the various coatings with a steel ball can be correlated to the surface attributes of each coating in terms of roughness and the presence of contamination layers, both of which are shown to also affect the nanohardness measurements. C1 [Demas, Nicholaos G.; Lorenzo-Martin, Cinta; Ajayi, Oyelayo O.; Erck, Robert A.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Shareef, Iqbal] Bradley Univ, 1501 W Bradley Ave, Peoria, IL 61625 USA. RP Demas, NG (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM ndemas@anl.gov FU U.S. Department of Energy, Energy Efficiency and Renewable Energy, Office of Vehicle Technologies [DE-AC02-06CH11357] FX This work was supported by U.S. Department of Energy, Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, under contract DE-AC02-06CH11357. The scanning electron microscopy was performed at the Electron Microscopy Center for Materials Research at Argonne National Laboratory, a U.S. Department of Energy Office of Science Laboratory operated by UChicago Argonne, LLC. NR 16 TC 0 Z9 0 U1 5 U2 12 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1073-5623 EI 1543-1940 J9 METALL MATER TRANS A JI Metall. Mater. Trans. A-Phys. Metall. Mater. Sci. PD APR PY 2016 VL 47A IS 4 BP 1629 EP 1640 DI 10.1007/s11661-016-3342-9 PG 12 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DF4HA UT WOS:000371307400015 ER PT J AU Unocic, KA Dryepondt, S Yamamoto, Y Maziasz, PJ AF Unocic, Kinga A. Dryepondt, Sebastien Yamamoto, Yukinori Maziasz, Philip J. TI Creep and Oxidation Behavior of Modified CF8C-Plus with W, Cu, Ni, and Cr SO METALLURGICAL AND MATERIALS TRANSACTIONS A-PHYSICAL METALLURGY AND MATERIALS SCIENCE LA English DT Article ID CAST AUSTENITIC ALLOY; WATER-VAPOR; PRECIPITATION; STEELS; PHASE; COPPER; MECHANISM AB The microstructures of modified CF8C-Plus (Fe-19Cr-12Ni-0.4W-3.8Mn-0.2Mo-0.6Nb-0.5Si-0.9C) with W and Cu (CF8CPWCu) and CF8CPWCu enhanced with 21Cr + 15Ni or 22Cr + 17.5Ni were characterized in the as-cast condition and after creep testing. When imaged at lower magnifications, the as-cast microstructure was similar among all three alloys as they all contained a Nb-rich interdendritic phase and Mn-based inclusions. Transmission electron microscopy (TEM) analysis showed the presence of nanoscale Cu-rich nanoprecipitates distributed uniformly throughout the matrix of CF8CPWCu, whereas in CF8CPWCu22/17, Cu precipitates were found primarily at the grain boundaries. The presence of these nanoscale Cu-rich particles, in addition to W-rich Cr23C6, nanoscale Nb carbides, and Z-phase (Nb2Cr2N2), improved the creep strength of the CF8CPWCu steel. Modification of CF8CPWCu with Cr and Ni contents slightly decreased the creep strength but significantly improved the oxidation behavior at 1073 K (800 A degrees C). In particular, the addition of 22Cr and 17.5Ni strongly enhanced the oxidation resistance of the stainless steel resulting in a 100 degrees or greater temperature improvement, and this composition provided the best balance between improving both mechanical properties and oxidation resistance. C1 [Unocic, Kinga A.; Dryepondt, Sebastien; Yamamoto, Yukinori; Maziasz, Philip J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Unocic, KA (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM unocicka@ornl.gov FU U.S. Department of Energy, Office of Coal and Power R&D, Office of Fossil Energy, Office of Coal and Power R&D in the Office of Fossil Energy FX The authors would like to thank G.W. Garner, T.M. Lowe, T. Geer, J.L. Moser, and K.A. Powers for assistance with the experimental work. B.A Pint, L.F. Allard, and R.R. Unocic provided helpful comments and suggestions on the results and manuscript. Research was supported by the U.S. Department of Energy, Office of Coal and Power R&D, Office of Fossil Energy, Office of Coal and Power R&D in the Office of Fossil Energy, and microscopy was supported through a user proposal by ORNL's Center for Nanophase Materials Sciences (CNMS), which is a U.S. Department of Energy, Office of Science User Facility. NR 31 TC 0 Z9 0 U1 5 U2 14 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1073-5623 EI 1543-1940 J9 METALL MATER TRANS A JI Metall. Mater. Trans. A-Phys. Metall. Mater. Sci. PD APR PY 2016 VL 47A IS 4 BP 1641 EP 1653 DI 10.1007/s11661-016-3348-3 PG 13 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Materials Science; Metallurgy & Metallurgical Engineering GA DF4HA UT WOS:000371307400016 ER PT J AU Kanarska, Y Walton, O AF Kanarska, Yuliya Walton, Otis TI Application of parallel distributed Lagrange multiplier technique to simulate coupled Fluid-Granular flows in pipes with varying Cross-Sectional area SO POWDER TECHNOLOGY LA English DT Article DE Fluid-granular flows; Pneumatic conveying; Lagrange multiplier ID IMMERSED BOUNDARY METHOD; PARTICULATE FLOWS AB Fluid-granular flows are common phenomena in nature and industry. Here, an efficient computational technique based on the distributed Lagrange multiplier method is utilized to simulate complex fluid-granular flows. Each particle is explicitly resolved on an Eulerian grid as a separate domain, using solid volume fractions. The fluid equations are solved through the entire computational domain, however, Lagrange multiplier constrains are applied inside the particle domain such that the fluid within any volume associated with a solid particle moves as an incompressible rigid body. The particle-particle interactions are implemented using explicit force-displacement interactions for frictional inelastic particles similar to the DEM method (Cundall and Strack, 1979) with some modifications using the volume of an overlapping region as an input to the contact forces. A parallel implementation of the method is based on the SAMRAI (Structured Adaptive Mesh Refinement Application Infrastructure) library. Application of this method to simulate fluid-granular flows in pipes with a step decrease in cross-sectional area is discussed. Correlations between pressure losses and solid mass fluxes in a pipe for different particle concentrations, pipe diameters and particle sizes are studied. Results of the simulations agree well with available experimental data for the mass flow ratio vs pressure drop during conveying. (C) 2015 Elsevier B.V. All rights reserved. C1 [Kanarska, Yuliya; Walton, Otis] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Kanarska, Y (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM kanarska1@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. We thank Brian Comaskey for providing experimental data. NR 13 TC 0 Z9 0 U1 1 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0032-5910 EI 1873-328X J9 POWDER TECHNOL JI Powder Technol. PD APR PY 2016 VL 291 BP 35 EP 45 DI 10.1016/j.powtec.2015.11.062 PG 11 WC Engineering, Chemical SC Engineering GA DE8QH UT WOS:000370900900005 ER PT J AU Gopalan, B Shahnam, M Panday, R Tucker, J Shaffer, F Shadle, L Mei, J Rogers, W Guenther, C Syamlal, M AF Gopalan, Balaji Shahnam, Mehrdad Panday, Rupen Tucker, Jonathan Shaffer, Frank Shadle, Lawrence Mei, Joseph Rogers, William Guenther, Chris Syamlal, Madhava TI Measurements of pressure drop and particle velocity in a pseudo 2-D rectangular bed with Geldart Group D particles SO POWDER TECHNOLOGY LA English DT Article DE Fluidization; Granular flow; Experiment; Granular temperature; High speed PIV ID SOLIDS FLUIDIZED-BEDS; EXPERIMENTAL VALIDATION; GRANULAR FLOW; CFB RISERS; SIMULATION; FIELDS; MODEL; DENSE AB A small scale pseudo 2-D bed of dimension 0.075 m x 023 m x 122 m was utilized to measure the pressure drop and velocity statistics of Geldart Group D nylon beads. The pressure drop was measured using a fast-response pressure transducer and the particle velocities were measured with high speed particle image velocimetry, with particle tracking, in a slugging flow regime for three different superficial gas velocities (2, 3 & 4 times the minimum fluidization velocity (U-mf)). At superficial gas velocity of 3 U-mf, the measured slugging frequency was about 2.5 Hz, while at conditions close to 2 U-mf and 4 U-mf, the slugging frequency was about 1.5 and 1.7 Hz. Additionally, at 3 U-mf condition, the bed exhibited a much higher root mean square (RMS) of pressure drop fluctuations than those at 2 U-mf and 4 U-mf. The varying trend suggested an existence of a complicated regime change for these shallow bed measurements that had not been previously explored. The measurement of millions of individual particle velocities at the vicinity of the wall had enabled accurate measurement of higher order statistics including RMS, granular temperature, skewness, and kurtosis of particle velocity. The measured skewness and kurtosis of the velocity distribution indicated that the particle velocity distribution deviated substantially from a normal distribution as the intersection of walls of the rectangular bed was approached. (C) 2016 Elsevier B.V. All rights reserved. C1 [Gopalan, Balaji; Shahnam, Mehrdad; Panday, Rupen; Tucker, Jonathan; Shaffer, Frank; Shadle, Lawrence; Mei, Joseph; Rogers, William; Guenther, Chris; Syamlal, Madhava] Natl Energy Technol Lab, Morgantown, WV USA. [Gopalan, Balaji] W Virginia Univ, Corp Res, Morgantown, WV 26506 USA. [Panday, Rupen] REM Engn, Morgantown, WV USA. [Tucker, Jonathan] Oak Ridge Inst Sci & Engn, Oak Ridge, TN USA. RP Gopalan, B (reprint author), Natl Energy Technol Lab, Morgantown, WV USA.; Gopalan, B (reprint author), W Virginia Univ, Corp Res, Morgantown, WV 26506 USA. NR 38 TC 2 Z9 2 U1 9 U2 30 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0032-5910 EI 1873-328X J9 POWDER TECHNOL JI Powder Technol. PD APR PY 2016 VL 291 BP 299 EP 310 DI 10.1016/j.powtec.2015.12.040 PG 12 WC Engineering, Chemical SC Engineering GA DE8QH UT WOS:000370900900032 ER PT J AU Monazam, ER Breault, RW Shadle, LJ AF Monazam, Esmail R. Breault, Ronald W. Shadle, Lawrence J. TI Pressure and apparent voidage profiles for riser with an abrupt exit (T-shape) in a CFB riser operating above fast fluidization regimes SO POWDER TECHNOLOGY LA English DT Article DE Riser; Pressure profile; Circulating fluidized bed ID BED RISERS; DYNAMIC SIMILARITY; HYDRODYNAMICS AB The influence of abrupt exit (T-shaped) configuration on the riser axial pressure profile in a large-scale circulating fluidized bed (CFB) is examined. A new analysis was developed to predict the axial voidage along the length of influence in the exit region with T-shape geometry. The exit region was characterized using non-dimensional analysis of the continuum equations (balances of masses and momenta) that described multiphase flows. In addition to deceleration length due to abrupt exit, the boundary condition for the solid fraction at the top of the riser and the fully developed regions, were measured using an industrial scale circulating fluidized bed (CFB) of 03 m diameter and 15 m tall. The operating factors affecting the flow development in the exit region were determined for three materials of various sizes and densities in core annular and dilute regimes of the riser. Performance data were taken from statistically designed experiments over a wide range of Fr (0.5-39), Re (8-600), Ar (29-3600), load ratio (0.2-28), riser to particle diameter ratio (375-5000), and gas to solid density ratio (138-1381).A series of correlations were developed to predict the voidage at the exit of the riser and length of influence due to the exit geometry. The correlations are based on gas and solid properties, operating conditions, and riser geometry. Published by Elsevier B.V. C1 [Monazam, Esmail R.] REM Engn Serv PLLC, 3537 Collins Ferry Rd, Morgantown, WV 26505 USA. [Breault, Ronald W.; Shadle, Lawrence J.] US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. RP Breault, RW (reprint author), US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. EM ronald.breault@netl.doe.gov FU Department of Energy through the Fossil Energy's Integrated Gasification Combined Cycle program FX The authors acknowledge the Department of Energy for funding the research through the Fossil Energy's Integrated Gasification Combined Cycle program. NR 29 TC 2 Z9 2 U1 3 U2 17 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0032-5910 EI 1873-328X J9 POWDER TECHNOL JI Powder Technol. PD APR PY 2016 VL 291 BP 383 EP 391 DI 10.1016/j.powtec.2015.12.041 PG 9 WC Engineering, Chemical SC Engineering GA DE8QH UT WOS:000370900900041 ER PT J AU Panday, R Breault, R Shadle, LJ AF Panday, Rupen Breault, Ronald Shadle, Lawrence J. TI Dynamic modeling of the circulating fluidized bed riser SO POWDER TECHNOLOGY LA English DT Article DE Circulating fluidized bed; Inherent feedback; Riser state model; Average residence time; Dynamic experiments ID PRESSURE BALANCE MODEL; PARTICLE-VELOCITY; FLOW; DENSITY AB Dynamic modeling is required to understand hydrodynamics of a circulating fluidized bed (CFB) riser as a function of time. The paper develops a dynamic model of the riser from the conservation of solid mass. Solid mass that flows out of the riser requires particle residence time to close the mass balance equation. The mean residence time of solids was derived as the riser length divided by the superficial riser gas velocity normalized by a ratio of solid concentration in the riser outlet to that in the riser itself. For bed materials including high-density polyethylene beads, glass beads, and cork, the percentage of solid concentration in the horizontal crossover pipe connecting the riser exit and the cyclone inlet was found to be 22% of the average concentration of solids in the riser. Upon finding the particle residence time, we calculated the solid flow rate out of the riser and along with the knowledge of solids flowing into the riser column we determined the riser inventory as a function of time. We used the estimated solid inventory to model overall pressure drop across the riser from the conservation of momentum. The momentum equation included the balance of pressure force by the hydrostatic head of solids, and the wall frictions due to gas and solids in a fully developed zone. The prediction of overall riser pressure drop compared well with its measured values at many dynamic conditions. Therefore, our dynamic model is useful for developing advanced control strategy or for improving existing control systems of the CFB plant. The residence time approach is also useful for the design of a transport reactor. The technique also comes handy when setting up the boundary condition for the overall pressure drop in the CFD modeling that can simulate incremental pressures along the riser height. Published by Elsevier B.V. C1 [Panday, Rupen; Breault, Ronald; Shadle, Lawrence J.] Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. [Panday, Rupen] REM Engn Serv PLLC, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. RP Breault, R (reprint author), Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. EM ronald.breault@netl.doe.gov NR 49 TC 1 Z9 1 U1 4 U2 34 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0032-5910 EI 1873-328X J9 POWDER TECHNOL JI Powder Technol. PD APR PY 2016 VL 291 BP 522 EP 535 DI 10.1016/j.powtec.2015.12.045 PG 14 WC Engineering, Chemical SC Engineering GA DE8QH UT WOS:000370900900054 ER PT J AU Strychalska, J Thompson, JD Cava, RJ Klimczuk, T AF Strychalska, Judyta Thompson, Joe D. Cava, Robert J. Klimczuk, Tomasz TI Superconductivity and ferromagnetism in Pd doped Y9Co7 SO INTERMETALLICS LA English DT Article DE Intermetallics; Magnetic properties; Superconducting properties ID MAGNETISM; Y4CO3; MAGNETIZATION; PHASE; ZR AB The ferromagnetic superconductor Y9Co7 was chemically doped to yield the solid solution Y9Co7-xPdx for 0 < x < 0.4. The lattice parameter a does not depend on x, whereas c increases with increasing Pd content up to x = 0.2, the palladium solubility limit. The transition from ferromagnetism (T-C = 4.25 K) to superconductivity (T-sc = 2.4 K) was observed only for the parent Y9Co7 compound. For the lowest tested Pd doping level (x = 0.05), ferromagnetism is enhanced strongly (T-C = 935 K) and superconductivity is not seen above 1.8 K. The Curie temperature rapidly increases from 4.25 K to about 10 K for a Pd concentration of x = 0.1 and remains almost unchanged for Y9Co6.8Pd0.2. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Strychalska, Judyta; Klimczuk, Tomasz] Gdansk Univ Technol, Fac Appl Phys & Math, Narutowicza 11-12, PL-80233 Gdansk, Poland. [Thompson, Joe D.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Cava, Robert J.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. RP Klimczuk, T (reprint author), Gdansk Univ Technol, Fac Appl Phys & Math, Narutowicza 11-12, PL-80233 Gdansk, Poland. EM tomasz.klimczuk@pg.gda.pl FU National Science Centre (Poland) [DEC-2012/07/E/ST3/00584]; US Department of Energy [DE-FG02-98ER45706]; US Department of Energy, Office of Science, Division of Materials Sciences and Engineering FX The research performed at Gdansk University of Technology was financially supported by the National Science Centre (Poland) Grant No. DEC-2012/07/E/ST3/00584, and the analysis of the diffraction patterns at Princeton University was supported by the US Department of Energy, grant DE-FG02-98ER45706. Work at Los Alamos was performed under the auspices of the US Department of Energy, Office of Science, Division of Materials Sciences and Engineering. NR 19 TC 0 Z9 0 U1 3 U2 16 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0966-9795 EI 1879-0216 J9 INTERMETALLICS JI Intermetallics PD APR PY 2016 VL 71 BP 73 EP 75 DI 10.1016/j.intermet.2016.01.002 PG 3 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA DE8VP UT WOS:000370915100011 ER PT J AU Cho, HH Chen-Wiegart, YCK Dunand, DC AF Cho, Hoon-Hwe Chen-Wiegart, Yu-chen Karen Dunand, David C. TI Finite element analysis of mechanical stability of coarsened nanoporous gold SO SCRIPTA MATERIALIA LA English DT Article DE Coarsened nanoporous gold; Mechanical stability; Finite element (FE) analysis; Volume fraction; Surface characteristics ID BEHAVIOR; AU; FABRICATION; FOAMS AB The mechanical stability of nanoporous gold (np-Au) at various stages of thermal coarsening is studied via finite element analysis under volumetric compression using np-Au architectures imaged via X-ray nano-tomography. As the np-Au is coarsened thermally over ligament sizes ranging from 185 to 465 nm, the pore volume fraction is determinant for the mechanical stability of the coarsened np-Au, unlike the curvature and surface orientation of the ligaments. The computed Young's modulus and yield strength of the structures are compared with the Gibson-Ashby model. The geometry of the structures determines the locations where stress concentrations occur at the onset of yielding. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Cho, Hoon-Hwe; Dunand, David C.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Chen-Wiegart, Yu-chen Karen] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. RP Dunand, DC (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. EM dunand@northwestem.edu RI Dunand, David/B-7515-2009 FU Dongbu Cultural Foundation; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This research was supported by the Dongbu Cultural Foundation. The X-ray nano-tomography data were originally collected at Advanced Photon Source (APS) as detailed in Ref. [14]. Use of APS is supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under contract no. DE-AC02-06CH11357. NR 26 TC 1 Z9 1 U1 5 U2 19 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD APR 1 PY 2016 VL 115 BP 96 EP 99 DI 10.1016/j.scriptamat.2016.01.011 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DE8NV UT WOS:000370893800022 ER PT J AU Shu, SP Zhang, X Beach, JA Bellon, P Averback, RS AF Shu, Shipeng Zhang, Xuan Beach, John A. Bellon, Pascal Averback, Robert S. TI Irradiation-induced formation of nanorod precipitates in a dilute Cu-W alloy SO SCRIPTA MATERIALIA LA English DT Article DE Ion irradiation; Precipitate morphology; Self-organization; Radiation-enhanced diffusion ID HIGH-TEMPERATURE IRRADIATION; SOLID-SOLUTIONS; STABILITY AB Radiation-enhanced precipitation of W has been investigated in dilute Cu-W alloys. While spherical W precipitates are stabilized during irradiation below similar to 300 degrees C and above similar to 600 degrees C, irradiation at 500 degrees C results in the formation of nanorods. Furthermore, use of two-step irradiations, first one at 600 degrees C followed by one at 500 degrees C, indicates that the morphological transformation is reversible. The stabilization of W nanorods is rationalized using a model introduced by Frost and Russell to explain size stabilization of precipitates formed during irradiation, but extended here to consider precipitate morphology. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Shu, Shipeng; Zhang, Xuan; Beach, John A.; Bellon, Pascal; Averback, Robert S.] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. [Shu, Shipeng] Univ Wisconsin Madison, Dept Mat Sci & Engn, Madison, WI 53706 USA. [Zhang, Xuan] Argonne Natl Lab, Nucl Engn Div, Lemont, IL 60439 USA. RP Shu, SP (reprint author), Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA.; Shu, SP (reprint author), Univ Wisconsin Madison, Dept Mat Sci & Engn, Madison, WI 53706 USA. EM shu13@illinois.edu OI Shu, Shipeng/0000-0003-3859-5014 FU US National Science Foundation [DMR-1306475] FX The authors thank Daniel Schwen and Zebo Li for valuable discussions. This research was supported by US National Science Foundation under Grant Number DMR-1306475. The work was carried out in part in the Frederick-Seitz Materials Research Laboratory Central Facilities, University of Illinois at Urbana-Champaign. NR 21 TC 0 Z9 0 U1 9 U2 21 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD APR 1 PY 2016 VL 115 BP 155 EP 158 DI 10.1016/j.scriptamat.2016.01.012 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DE8NV UT WOS:000370893800035 ER PT J AU Bostelmann, F Hammer, HR Ortensi, J Strydom, G Velkov, K Zwermann, W AF Bostelmann, Friederike Hammer, Hans R. Ortensi, Javier Strydom, Gerhard Velkov, Kiril Zwermann, Winfried TI Criticality calculations of the Very High Temperature Reactor Critical Assembly benchmark with Serpent and SCALE/KENO-VI SO ANNALS OF NUCLEAR ENERGY LA English DT Article DE HTGR; VHTRC; Serpent; SCALE/KENO-VI AB Within the framework of the IAEA Coordinated Research Project on HTGR Uncertainty Analysis in Modeling, criticality calculations of the Very High Temperature Critical Assembly experiment were performed as the validation reference to the prismatic MHTGR-350 lattice calculations. Criticality measurements performed at several temperature points at this Japanese graphite-moderated facility were recently included in the International Handbook of Evaluated Reactor Physics Benchmark Experiments, and represent one of the few data sets available for the validation of HTGR lattice physics. This work compares VHTRC criticality simulations utilizing the Monte Carlo codes Serpent and SCALE/KENO-VI. Reasonable agreement was found between Serpent and KENO-VI, but only the use of the latest ENDF cross section library release, namely the ENDF/B-VII.1 library, led to an improved match with the measured data. Furthermore, the fourth beta release of SCALE 6.2/KENO-VI showed significant improvements from the current SCALE 6.1.2 version, compared to the experimental values and Serpent. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Bostelmann, Friederike; Velkov, Kiril; Zwermann, Winfried] Gesell Anlagen & Reaktorsicherheit GRS gGmbH, D-85748 Garching, Germany. [Hammer, Hans R.] Texas A&M, Dept Nucl Engn, College Stn, TX 77840 USA. [Ortensi, Javier; Strydom, Gerhard] Idaho Natl Lab, Nucl Sci & Engn Div, Idaho Falls, ID 83401 USA. RP Bostelmann, F (reprint author), Gesell Anlagen & Reaktorsicherheit GRS gGmbH, D-85748 Garching, Germany. EM Friederike.Bostelmann@grs.de RI Ortensi, Javier/B-4712-2017; Strydom, Gerhard/B-4865-2017 OI Ortensi, Javier/0000-0003-1685-3916; Strydom, Gerhard/0000-0002-5712-8553 FU German Federal Ministry for Economic Affairs and Energy; U.S. Department of Energy, Assistant Secretary for the Office of Nuclear Energy, under DOE Idaho Operations Office [DE-AC07-05ID14517] FX This work was supported by the German Federal Ministry for Economic Affairs and Energy, and the U.S. Department of Energy, Assistant Secretary for the Office of Nuclear Energy, under DOE Idaho Operations Office Contract DE-AC07-05ID14517. NR 16 TC 0 Z9 0 U1 1 U2 3 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0306-4549 J9 ANN NUCL ENERGY JI Ann. Nucl. Energy PD APR PY 2016 VL 90 BP 343 EP 352 DI 10.1016/j.anucene.2015.12.008 PG 10 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DD7LO UT WOS:000370106200033 ER PT J AU Antonov, VE Bashkin, IO Bazhenov, AV Bulychev, BM Fedotov, VK Fursova, TN Kolesnikov, AI Kulakov, VI Lukashev, RV Matveev, DV Sakharov, MK Shulga, YM AF Antonov, V. E. Bashkin, I. O. Bazhenov, A. V. Bulychev, B. M. Fedotov, V. K. Fursova, T. N. Kolesnikov, A. I. Kulakov, V. I. Lukashev, R. V. Matveev, D. V. Sakharov, M. K. Shulga, Y. M. TI Multilayer graphane synthesized under high hydrogen pressure SO CARBON LA English DT Article ID PREPARED NANOSTRUCTURED GRAPHITE; CARBON NANOTUBES; SPECTROSCOPY; SPECTRA; MANTLE AB A new hydrocarbon - hydrographite - with the composition close to CH is shown to form from graphite and gaseous hydrogen at pressures above 2 GPa and temperatures from 450 to 700 degrees C. Hydrographite is a black solid thermally stable under ambient conditions. If heated in vacuum, it decomposes into graphite and molecular hydrogen at temperatures from 500 to 650 degrees C. Powder X-ray diffraction characterizes hydrographite as a multilayer "graphane II" phase predicted by ab initio calculations [Wen X-D et al. PNAS 2011; 108: 6833] and consisting of graphane sheets in the chair conformation stacked along the hexagonal c axis in the - ABAB - sequence. The crystal structure of the synthesized phase belongs to the P6(3)mc space group. The unit cell parameters are a = 2.53(1) angstrom c = 9.54(1) angstrom and therefore exceed the corresponding parameters of graphite by 2.4(2)% and 42.0(3)%. Stretching vibrations of C-H groups on the surface of the hydrographite particles are examined by infrared spectroscopy. (C) 2015 Published by Elsevier Ltd. C1 [Antonov, V. E.; Bashkin, I. O.; Bazhenov, A. V.; Fedotov, V. K.; Fursova, T. N.; Kulakov, V. I.; Matveev, D. V.; Sakharov, M. K.] Russian Acad Sci, Inst Solid State Phys, Chernogolovka 142432, Moscow District, Russia. [Bulychev, B. M.] Moscow MV Lomonosov State Univ, Moscow 119992, Russia. [Kolesnikov, A. I.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Lukashev, R. V.] Inst Problems Chem Phys RAS, Chernogolovka 142432, Moscow District, Russia. [Shulga, Y. M.] Natl Univ Sci & Technol MISIS, Leninsky Pr 4, Moscow 119049, Russia. RP Antonov, VE (reprint author), Russian Acad Sci, Inst Solid State Phys, Chernogolovka 142432, Moscow District, Russia. EM antonov@issp.ac.ru FU Russian Foundation for Basic Research [11-02-00401]; Russian Academy of Sciences; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX The work was supported by Grant No. 11-02-00401 from the Russian Foundation for Basic Research and by the Program "The Matter under High Pressure" of the Russian Academy of Sciences. A.I.K. greatly acknowledges the support from the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 34 TC 2 Z9 2 U1 12 U2 36 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD APR PY 2016 VL 100 BP 465 EP 473 DI 10.1016/j.carbon.2015.12.051 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DD5KC UT WOS:000369961400054 ER PT J AU Smith, MW Dallmeyer, I Johnson, TJ Brauer, CS McEwen, JS Espinal, JF Garcia-Perez, M AF Smith, Matthew W. Dallmeyer, Ian Johnson, Timothy J. Brauer, Carolyn S. McEwen, Jean-Sabin Espinal, Juan F. Garcia-Perez, Manuel TI Structural analysis of char by Raman spectroscopy: Improving band assignments through computational calculations from first principles SO CARBON LA English DT Article ID POLYCYCLIC AROMATIC-HYDROCARBONS; SODIUM-ION BATTERIES; OBSERVED SPECTRA; SCALING FACTORS; FAST PYROLYSIS; FORCE-FIELDS; BASIS-SETS; CARBON; GRAPHITE; BIOCHAR AB The complex heterogeneous nature of chars has confounded the complete analysis of the Raman spectra of these materials. The additional shoulders observed on the defect (D)-band and high intensity valley between the D and graphitic (G)-bands represent the primary regions of uncertainty. In this paper the effects of various vacancy and substitution defects in a coronene parent molecule have been systematically analyzed using density functional theory (DFT). The impacts of these defects are best understood in terms of a reduced symmetry as compared to a "parent" coronene molecule. Based on simulation results, a total of ten potential bands have been assigned between 1000 cm(-1) and 1800 cm(-1). These bands have been used to deconvolute a thermoseries of cellulose chars produced by pyrolysis at 300-700 degrees C. The shoulder observed in chars near 1200 cm(-1) has been assigned to the symmetric breathing mode of various small polyaromatic hydrocarbons (PAH) as well as rings containing seven or more carbons. Intensity between 1400 cm(-1) and 1550 cm(-1) results from a range of coupled vibrational modes from various defect structures. The deconvolution of cellulose derived chars shows consistent growth of PAH clusters, loss of oxygen, and development of non-hexoganal ring systems as pyrolysis temperature increased. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Smith, Matthew W.; Garcia-Perez, Manuel] Washington State Univ, Dept Biol Syst Engn, Pullman, WA 99164 USA. [Dallmeyer, Ian] Washington State Univ, Composite Mat & Engn Ctr, Pullman, WA 99164 USA. [Johnson, Timothy J.; Brauer, Carolyn S.] Pacific NW Natl Lab, Chem Phys & Anal, Richland, WA 99352 USA. [Smith, Matthew W.; McEwen, Jean-Sabin] Gene & Linda Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. [Espinal, Juan F.] Univ Antioquia, Insitute Chem, Chem Energy Resources & Environm, Medellin, Colombia. RP Garcia-Perez, M (reprint author), Dept Biol Syst Engn, LJ Smith,Room 205,POB 646120, Pullman, WA 99164 USA.; McEwen, JS (reprint author), Voiland Sch Chem Eng & Bioengn, Wegner 257,POB 646515, Pullman, WA 99164 USA. EM js.mcewen@wsu.edu; mgarcia-perez@wsu.edu OI Garcia-Perez, Manuel/0000-0002-9386-2632 FU US National Science Foundation [CBET-1434073, CAREER CBET-1150430]; Washington State Department of Ecology; Washington State Department of Agriculture; USDA/NIFA [WNP00807, WNP00701]; U. S. Department of Energy; U.S. DOE [DE-AC05-76RLO1830]; "Programa Sostenibilidad" of the University of Antioquia FX The authors are very thankful for the financial support provided by the US National Science Foundation (CBET-1434073, CAREER CBET-1150430), the Washington State Department of Ecology, and the Washington State Department of Agriculture (Appendix A). It was also partially funded by the USDA/NIFA through Hatch Projects #WNP00807 and # WNP00701. Part of the research described in this paper was supported in part by the U. S. Department of Energy. PNNL is operated by Battelle for the U.S. DOE under Contract DE-AC05-76RLO1830. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paidup, irrevocable, world-wide license to publish or reproduce the published form of the manuscript, or allow others to do so, for United States Government purposes. Dr. Espinal thanks partial support from the "Programa Sostenibilidad 2014-2015" of the University of Antioquia. NR 78 TC 9 Z9 9 U1 28 U2 71 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD APR PY 2016 VL 100 BP 678 EP 692 DI 10.1016/j.carbon.2016.01.031 PG 15 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DD5KC UT WOS:000369961400076 ER PT J AU Shumilova, TG Tkachev, SN Isaenko, SI Shevchuk, SS Rappengluck, MA Kazakov, VA AF Shumilova, T. G. Tkachev, S. N. Isaenko, S. I. Shevchuk, S. S. Rappenglueck, M. A. Kazakov, V. A. TI A "diamond-like star" in the lab. Diamond-like glass SO CARBON LA English DT Article ID LARGE MAGELLANIC CLOUD; EARTHS INNER-CORE; CARBON STARS; WHITE-DWARF; RAMAN-SPECTROSCOPY; EXTREME CONDITIONS; PHASE; ASTEROSEISMOLOGY; CRYSTALLIZATION; TEMPERATURE AB Tantalizing information about a possible existence of diamond stars has recently refocused attention of the scientific community on the basic properties of carbon-rich planets and stars. Since the carbon-rich star types are known for a usual presence of oxygen, it is not clear how carbon and oxygen can co-exist under extreme PT-conditions at a C/O < 1 atomic ratio. Therefore, the significance of the fact that the "star" PT-conditions (7000-13,000 K, 40 GPa) have been reached and sustained for a relatively long period of time in the oxygen-rich medium of the continuously laser heated diamond anvil cell, resulting in an optically transparent carbon glass (diamond-like glass) and, subsequently, oxygen-rich solid carbon synthesis, is hard to overestimate. Moreover, our results suggest that pure carbon can co-exist with oxygen under the extreme PT-conditions and have potential to open up a new technological way for production of novel super-refractory alloys and materials. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Shumilova, T. G.; Isaenko, S. I.; Shevchuk, S. S.] Russian Acad Sci, Inst Geol, Komi Sci Ctr, Ural Div, Pervomayskaya St 54, Syktyvkar 167982, Russia. [Shumilova, T. G.] Univ Hawaii Manoa, Hawaii Inst Geophys & Planetol, 1680 East West Rd, Honolulu, HI 96822 USA. [Tkachev, S. N.] Univ Chicago, Argonne Natl Lab, Ctr Adv Radiat Sources, 9700 South Cass Ave, Argonne, IL 60439 USA. [Rappenglueck, M. A.] Inst Interdisciplinary Sci, Bahnhofstr 1, D-82205 Gilching, Germany. [Kazakov, V. A.] SSC FSUE Keldysh Res Ctr, Onezhskaya 8, Moscow 125438, Russia. RP Shumilova, TG (reprint author), Russian Acad Sci, Inst Geol, Komi Sci Ctr, Ural Div, Pervomayskaya St 54, Syktyvkar 167982, Russia. EM shumilova@geo.komisc.ru; tkachev@cars.uchicago.edu; s.i.isaenko@gmail.com; mr@infis.org; nanocentre@kerc.msk.ru FU Russian Science Support Foundation FX The authors thank A.F.Goncharov and S.Lobanov for help in laser heating DAC experiments and "in situ" temperature measurements, Yu.Gogotsi, T.L.Evans, S. Sutton for scientific consultations, V.Prakapenka for assistance in synchrotron X-ray studies, the Russian Science Support Foundation for funding to T.Sh. and S.I., the Advanced Photon Source GSECARS (the GeoSoilEnviro Consortium for Advanced Radiation Sources) sector in Argonne National Laboratory (Chicago, Illinois, USA) for the opportunity to analyze structure of the quenched sample by synchrotron X-ray, the SSC FSUE Keldysh Research Centre (Moscow, Russian Federation) for the opportunity to use its analytical facilities. NR 47 TC 0 Z9 0 U1 10 U2 17 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD APR PY 2016 VL 100 BP 703 EP 709 DI 10.1016/j.carbon.2016.01.068 PG 7 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DD5KC UT WOS:000369961400078 ER PT J AU Dohrmann, CR Widlund, OB AF Dohrmann, Clark R. Widlund, Olof B. TI A BDDC Algorithm with Deluxe Scaling for Three-Dimensional H(curl) Problems SO COMMUNICATIONS ON PURE AND APPLIED MATHEMATICS LA English DT Article ID PRIMAL FETI METHODS; 3 DIMENSIONS; MAXWELLS EQUATIONS; ELLIPTIC PROBLEMS; DOMAIN DECOMPOSITION; SCHWARZ METHODS; PRECONDITIONERS; CONSTRAINTS; ELEMENTS; DP AB In this paper, we present and analyze a BDDC algorithm for a class of elliptic problems in the three-dimensional H(curl) space. Compared with existing results, our condition number estimate requires fewer assumptions and also involves two fewer powers of log(H/h), making it consistent with optimal estimates for other elliptic problems. Here, H/h is the maximum of H-i/h(i) over all subdomains, where H-i and hi are the diameter and the smallest element diameter for the subdomain Omega(i). The analysis makes use of two recent developments. The first is a new approach to averaging across the subdomain interfaces, while the second is a new technical tool that allows arguments involving trace classes to be avoided. Numerical examples are presented to confirm the theory and demonstrate the importance of the new averaging approach in certain cases. (C) 2016 Wiley Periodicals, Inc. C1 [Dohrmann, Clark R.] Sandia Natl Labs, Computat Solid Mech & Struct Dynam Dept, POB 5800, Albuquerque, NM 87185 USA. [Widlund, Olof B.] NYU, Courant Inst, 251 Mercer St, New York, NY 10012 USA. RP Dohrmann, CR (reprint author), Sandia Natl Labs, Computat Solid Mech & Struct Dynam Dept, POB 5800, Albuquerque, NM 87185 USA.; Widlund, OB (reprint author), NYU, Courant Inst, 251 Mercer St, New York, NY 10012 USA. EM crdohrm@sandia.gov; widlund@cims.nyu.edu FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94-AL85000]; U.S. Department of Energy [DE-FG02-06ER25718]; National Science Foundation [DMS-1216564] FX Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94-AL85000.; The work of the second author was supported in part by the U.S. Department of Energy under Contract DE-FG02-06ER25718 and in part by the National Science Foundation Grant DMS-1216564. NR 27 TC 8 Z9 8 U1 2 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0010-3640 EI 1097-0312 J9 COMMUN PUR APPL MATH JI Commun. Pure Appl. Math. PD APR PY 2016 VL 69 IS 4 BP 745 EP 770 PG 26 WC Mathematics, Applied; Mathematics SC Mathematics GA DE5JS UT WOS:000370667900006 ER PT J AU Walker, RW Ashton, NK Brown, RS Liss, SA Colotelo, AH Beirao, BV Townsend, RL Deng, ZD Eppard, MB AF Walker, Ricardo W. Ashton, Neil K. Brown, Richard S. Liss, Stephanie A. Colotelo, Alison H. Beirao, Bernardo V. Townsend, Richard L. Deng, Z. Daniel Eppard, M. Brad TI Effects of a novel acoustic transmitter on swimming performance and predator avoidance of juvenile Chinook Salmon: Determination of a size threshold SO FISHERIES RESEARCH LA English DT Article DE Behavior; Dam passage; Juvenile Salmon Acoustic Telemetry System; Migration; Telemetry ID EXTERNALLY ATTACHED TRANSMITTERS; RADIO TRANSMITTERS; MAXIMUM TAG; COHO SALMON; GROWTH; IMPLANTATION; SURVIVAL; TROUT; PHYSIOLOGY; RETENTION AB The miniaturization of acoustic transmitters enables researchers to tag smaller fish for telemetry studies, thus representing a greater proportion of the population of interest. Fish having a smaller transmitter burden (e.g., the weight of the transmitter relative to the weight of the fish) may also have fewer potential adverse transmitter effects. The development of an injectable acoustic transmitter has led to research that determined the least invasive and quickest method of implantation. Following that research, the objectives of this study were to determine the effects of transmitter implantation on swimming performance and predator avoidance, and to find a minimum size threshold of fish that can be tagged without adversely affecting those responses. To assess critical swimming speed (U-crit; an index of prolonged swimming performance) and predator avoidance for juvenile Chinook Salmon (Oncorhynchus tshawytscha), fish were split into three treatments: (1) implantation with a dummy injectable acoustic transmitter (IAT treatment), (2) implantation with a dummy injectable acoustic transmitter and passive integrated transponder tag (IAT + PIT treatment), and (3) an untagged control. IAT treatment fish had lower U-crit values than untagged controls among individuals below 79 mm fork length (transmitter burden 3.4-4.0%). U-crit values for the IAT + PIT treatment were not significantly different from untagged controls and no size threshold was found. There was no significant difference in predator avoidance between fish implanted with the IAT or IAT + PIT compared to untagged controls. These guidelines could provide researchers and managers with a powerful tool to examine behavior and survival of small salmonids. (C) 2016 Elsevier B.V. All rights reserved. C1 [Walker, Ricardo W.; Ashton, Neil K.; Brown, Richard S.; Liss, Stephanie A.; Colotelo, Alison H.] Pacific NW Natl Lab, Ecol Grp, Richland, WA 99352 USA. [Beirao, Bernardo V.] Univ Fed Sao Joao del Rei, Ouro Branco, MG, Brazil. [Townsend, Richard L.] Univ Washington, Sch Aquat & Fishery Sci, Columbia Basin Res, Seattle, WA 98101 USA. [Deng, Z. Daniel] Pacific NW Natl Lab, Hydrol Grp, Richland, WA 99352 USA. [Eppard, M. Brad] US Army Corps Engineers, Portland, OR 97208 USA. RP Liss, SA (reprint author), Pacific NW Natl Lab, Ecol Grp, Richland, WA 99352 USA. EM stephanie.liss@pnnl.gov RI Deng, Daniel/A-9536-2011 OI Deng, Daniel/0000-0002-8300-8766 FU Army Corps of Engineers, Portland District FX We would like to the thank the Army Corps of Engineers, Portland District, for providing the funding for this research. We would also like to thank the Washington Department of Fish and Wildlife Leavenworth and Priest Rapids Hatcheries for providing the salmon used in this study. We also thank John Skalski from the University of Washington for statistical advice and Thomas Hancock from Portland State University for providing assistance with the swimming chambers. We appreciate the assistance from the following PNNL staff Zach Booth, Nikki Fuller, David Geist, Jill Janak, Brian Jeide, Bryan Jones, Ki Won Jung, Tim Linley, Jun Lu, Jayson Martinez, Brett Pflugrath, Jason Reynolds, and John Stephenson. NR 30 TC 4 Z9 4 U1 4 U2 24 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0165-7836 EI 1872-6763 J9 FISH RES JI Fish Res. PD APR PY 2016 VL 176 BP 48 EP 54 DI 10.1016/j.fishres.2015.12.007 PG 7 WC Fisheries SC Fisheries GA DE0HZ UT WOS:000370307000006 ER PT J AU Markley, M Kletetschka, G AF Markley, Matthew Kletetschka, Gunther TI Nanophase iron production through laser irradiation and magnetic detection of space weathering analogs SO ICARUS LA English DT Article DE Experimental techniques asteroids; Surfaces Mercury; Surface Moon; Surface spectroscopy ID DUST PARTICLES; AIRLESS BODIES; LUNAR-SAMPLES; SIMULATION; SURFACE; NANOPARTICLES; OLIVINE; MERCURY; IMPACT AB Airless bodies are constantly exposed to space weathering. The Moon and other similar S-type asteroids physically change through comminution, melting, and agglutinate formation, while spectrally they are darkening, steepening (or reddening) the spectral slope toward longer wavelengths, and reducing silicate mineral absorption bands. In these S-type bodies the production of submicroscopic metallic iron, or nanophase iron (SMFe, npFe(0)) is a major contributor in these spectral changes. We made a qualitative estimate of both quantity and size distribution of produced metallic iron by space weathered analog, olivine irradiated by laser. Through SEM observation we confirmed that nanoparticles of metallic iron formed in the nm range. Spectroscopic and magnetic susceptibility (MS) through temperature analyses reveal an increasing trend of npFe formation, darkening, reddening, and shallowing of the 1 mu m olivine absorption band. Olivine that produced the larger end of the size range of npFe produced similar effects, except for increased reddening. The magnetic data suggests that with laser irradiation there is both a linear increase of nanoparticles and a logarithmic increase in spectral change with SW time. (C) 2015 Elsevier Inc. All rights reserved. C1 [Markley, Matthew; Kletetschka, Gunther] Charles Univ Prague, Fac Sci, Albertov 6, Prague 12800, Czech Republic. [Kletetschka, Gunther] Acad Sci Czech Republic, Inst Geol, Prague, Czech Republic. [Kletetschka, Gunther] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Markley, M (reprint author), Charles Univ Prague, Fac Sci, Albertov 6, Prague 12800, Czech Republic. FU NASA grant [NNX07AU63G]; MEYS grant [LK21303]; grant RVO [67985831] FX We thank the reviewers for their comments and helpful suggestions. We thank Dr. Jeffrey Gillis-Davis for providing his facility to do part of this work and to Dr. Michael Fuller for access to his magnetic measurement instrument. Both gave us their knowledge and expertise. This work was supported by NASA grant NNX07AU63G, MEYS grant LK21303, and grant RVO 67985831. NR 39 TC 1 Z9 1 U1 4 U2 8 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD APR PY 2016 VL 268 BP 204 EP 214 DI 10.1016/j.icarus.2015.12.022 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DD9AN UT WOS:000370218100015 ER PT J AU Wang, JJ Chen, L Kang, QJ Rahman, SS AF Wang, Junjian Chen, Li Kang, Qinjun Rahman, Sheik S. TI The lattice Boltzmann method for isothermal micro-gaseous flow and its application in shale gas flow: A review SO INTERNATIONAL JOURNAL OF HEAT AND MASS TRANSFER LA English DT Review DE Shale; Lattice Boltzmann method; Micro-gaseous flow; Slip flow ID HYDROPHOBIC MICROCHANNEL WALLS; PORE-SPACE MORPHOLOGY; ORGANIC-RICH SHALES; POROUS-MEDIA; KNUDSEN LAYER; RAREFIED-GAS; APPARENT PERMEABILITY; TRANSITION REGIME; POSIDONIA SHALE; ADSORBED GAS AB The lattice Boltzmann method (LBM) has experienced tremendous advances and been well accepted as a popular method for simulating various fluid flow problems in porous media. With the introduction of an effective relaxation time and slip boundary conditions, the LBM has been successfully extended to solve micro-gaseous transport phenomena. As a result, the LBM has the potential to become an effective numerical method for gas flow in shale matrix in slip flow and transition flow regimes. Additionally, it is very difficult to experimentally determine the permeability of extremely low permeable media like shale. In this paper an extensive review on a number of slip boundary conditions and Knudsen layer treatments used in LB models for micro-gaseous flow is carried out. Furthermore, potential applications of the LBM in flow simulation in shale gas reservoirs on pore scale and representative elementary volume (REV) scale are evaluated and summarized. Our review indicates that the LBM is capable of capturing gas flow in continuum to slip flow regimes which cover significant proportion of the pores in shale gas reservoirs and identifies opportunities for future research. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Wang, Junjian; Rahman, Sheik S.] Univ New S Wales, Sch Petr Engn, Sydney, NSW 2033, Australia. [Wang, Junjian; Chen, Li; Kang, Qinjun] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM 87545 USA. [Chen, Li] Xi An Jiao Tong Univ, Sch Energy & Power Engn, Key Lab Themofluid Sci & Engn MOE, Xian 710049, Shanxi, Peoples R China. RP Rahman, SS (reprint author), Univ New S Wales, Sch Petr Engn, Sydney, NSW 2033, Australia. EM sheik.rahman@unsw.edu.au RI Chen, Li/P-4886-2014; Kang, Qinjun/A-2585-2010 OI Chen, Li/0000-0001-7956-3532; Kang, Qinjun/0000-0002-4754-2240 FU LANL's LDRD Program; SCOPE, UNSW; China Scholarship Council (CSC) [201306400014]; National Nature Science Foundation of China [51406145, 51136004]; DOE oil gas project; LANL's Institutional Computing Program FX The authors would like to acknowledge the support from the LANL's LDRD Program and Institutional Computing Program and SCOPE, UNSW. J.W. would like to acknowledge the support from China Scholarship Council (CSC, No. 201306400014), L.C. thanks the support from National Nature Science Foundation of China (Nos. 51406145 and 51136004), and Q.K. would also like to acknowledge the support from a DOE oil & gas project. NR 151 TC 9 Z9 9 U1 22 U2 83 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0017-9310 EI 1879-2189 J9 INT J HEAT MASS TRAN JI Int. J. Heat Mass Transf. PD APR PY 2016 VL 95 BP 94 EP 108 DI 10.1016/j.ijheatmasstransfer.2015.12.009 PG 15 WC Thermodynamics; Engineering, Mechanical; Mechanics SC Thermodynamics; Engineering; Mechanics GA DD7NK UT WOS:000370111200010 ER PT J AU Crespillo, ML Graham, JT Zhang, Y Weber, WJ AF Crespillo, M. L. Graham, J. T. Zhang, Y. Weber, W. J. TI In-situ luminescence monitoring of ion-induced damage evolution in SiO2 and Al2O3 SO JOURNAL OF LUMINESCENCE LA English DT Article DE Ion beam induced luminescence; Ion-solid interaction; Irradiation effects; Silica; Quartz; Alumina ID SWIFT HEAVY-IONS; INDUCED OPTICAL-ABSORPTION; BEAM-INDUCED LUMINESCENCE; SELF-TRAPPED EXCITONS; ALPHA-QUARTZ; ELECTRONIC EXCITATION; SYNTHETIC QUARTZ; RADIATION-DAMAGE; LITHIUM-NIOBATE; SILICA GLASSES AB Real-time, in-situ ionoluminescence measurements provide information of evolution of emission bands with ion fluence, and thereby establish a correlation between point defect kinetics and phase stability. Using fast light ions (2 MeV H and 3.5 He MeV) and medium mass-high energy ions (8 MeV 0, E=0.5 MeV/amu), scintillation materials of a-SiO2, crystalline quartz, and Al2O3 are comparatively investigated at room temperature with the aim of obtaining a further insight on the structural defects induced by ion irradiation and understand the role of electronic energy loss on the damage processes. For more energetic heavy ions, the electronic energy deposition pattern offers higher rates of excitation deeper into the material and allows to evaluate the competing mechanisms between the radiative and non-radiative de-excitation processes. Irradiations with 8 MeV O ions have been selected corresponding to the electronic stopping regime, where the electronic stopping power is dominant, and above the critical amorphization threshold for quartz. The usefulness of IBIL and its specific capabilities as a sensitive tool to investigate the material characterization and evaluation of radiation effects are demonstrated. Published by Elsevier B.V. C1 [Crespillo, M. L.; Graham, J. T.; Zhang, Y.; Weber, W. J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Zhang, Y.; Weber, W. J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Crespillo, ML; Weber, WJ (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM mcrespil@utk.edu; wjweber@utk.edu RI Weber, William/A-4177-2008 OI Weber, William/0000-0002-9017-7365 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; University of Tennessee Governor's Chair program FX The authors would like to thank Mr. Haizhou Xue for operating the accelerator in the Ion Beam Materials Laboratory during the irradiation and ion beam luminescence measurements. This work was primarily supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Support for one of the authors (JTG) was provided by the University of Tennessee Governor's Chair program. NR 74 TC 5 Z9 5 U1 6 U2 30 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-2313 EI 1872-7883 J9 J LUMIN JI J. Lumines. PD APR PY 2016 VL 172 BP 208 EP 218 DI 10.1016/j.jlumin.2015.12.016 PG 11 WC Optics SC Optics GA DE1IX UT WOS:000370381600032 ER PT J AU Huang, J Wang, WH Fu, Q Yang, L Zhang, K Zhang, JY Xiang, B AF Huang, Jian Wang, Wenhui Fu, Qi Yang, Lei Zhang, Kun Zhang, Jingyu Xiang, Bin TI Stable electrical performance observed in large-scale monolayer WSe2(1-x)S2x with tunable band gap SO NANOTECHNOLOGY LA English DT Article DE monolayer WSe2(1-x)S2x; field effect transistor; tunable band gap ID TRANSITION-METAL DICHALCOGENIDES; FIELD-EFFECT TRANSISTORS; LARGE-AREA SYNTHESIS; SINGLE-LAYER MOS2; 2-DIMENSIONAL MATERIALS; MOLYBDENUM-DISULFIDE; DEVICE APPLICATIONS; WSE2; SEMICONDUCTOR; ELECTRONICS AB Two-dimensional (2D) semiconductor materials have attracted broad interest due to their unique structures and physical properties. The stability of the 2D-material-based devices plays a key role in their practical applications. Here, we report the promising stable electrical performance in the large-scale monolayer WSe2(1-x)S2x with a tunable band gap. Photoluminescence (PL) spectroscopy was utilized to verify the tunable band gap in the as-grown monolayer with a tuning capability of 120 meV. Gated field effect transistor (FET) performance confirmed the p-type transport behavior in monolayer WSe2(1-x)S2x with a high on/off ratio (>10(4)). Top-gated FET configuration improves the carrier mobility with two orders larger than that in the back-gated FET device. After exposure to air for three months, the device performance manifested excellent stability with no source-drain current drop observed. P-type WSe2(1-x)S2x with a tunable band gap is the ideal complement to n-type tunable monolayers in the application of pn junction-related flexible nanodevices. C1 [Huang, Jian; Wang, Wenhui; Fu, Qi; Yang, Lei; Xiang, Bin] Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, Synerget Innovat Ctr Quantum Informat Quantum Phy, Hefei 230026, Anhui, Peoples R China. [Zhang, Kun] Univ Sci & Technol China, Ctr Micro & Nanoscale Res & Fabricat, Hefei 230026, Anhui, Peoples R China. [Zhang, Jingyu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Xiang, B (reprint author), Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, Synerget Innovat Ctr Quantum Informat Quantum Phy, Hefei 230026, Anhui, Peoples R China. EM binxiang@ustc.edu.cn RI Xiang, Bin/C-9192-2012 FU National Natural Science Foundation of China [21373196, 11434009]; National Program for Thousand Young Talents of China; Fundamental Research Funds for the Central Universities [WK2340000050, WK2060140014] FX This work was supported by the National Natural Science Foundation of China (21373196, 11434009), the National Program for Thousand Young Talents of China and the Fundamental Research Funds for the Central Universities (WK2340000050, WK2060140014). NR 31 TC 4 Z9 4 U1 10 U2 76 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD APR 1 PY 2016 VL 27 IS 13 AR 13LT01 DI 10.1088/0957-4484/27/13/13LT01 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DE6HR UT WOS:000370735100001 PM 26901119 ER PT J AU Ristova, MM Francis, C Toma, FM Yu, KM Walukiewicz, W AF Ristova, Mimoza M. Francis, Christopher Toma, Francesca M. Yu, Kin M. Walukiewicz, Wladislaw TI Electrochemical modification of the optical and electrical properties of Cd-rich NixCd1-xO alloys SO SOLAR ENERGY MATERIALS AND SOLAR CELLS LA English DT Article DE NixCd1-xO; Conductive oxide; Electron concentration; Transmittance modification; Electrochemical coloration; XPS ID CHEMICAL BATH DEPOSITION; NICKEL-OXIDE FILMS; ELECTROCHROMIC PROPERTIES AB Enhancement of the optical and electrical properties of Cd-rich NixCd1-xO alloys was achieved through an electrochemical procedure - their biasing at a constant negative potential into an electrolyte. Depending on the conductivity of the film (correlated to x), the films changed their color from transparent-yellowish to black. For a certain bias, the coloration became permanent and irreversible. Electron concentration for some samples increased for better than two orders of magnitude upon the coloration, while as the mobility decreased for a factor of 2-10. Rutherford Back Scattering (RBS) analysis revealed oxygen deficiency for the colored samples. The XRD analysis showed that the coloration could be associated to a partial reduction of CdO2 to CdO. XPS analysis suggested complex red-ox transitions of the two Ni and two Cd-oxides within the alloy. Ni2p electrons suggested that a partial NiO (transparent) transition to Ni2O3 (black) is likely the responsible process for the occurrence of the intensive light trapping. Since the NixCd1-xO band gap is tunable with x, one may conclude that this electrochemical procedure is motivating for tuning/modification/enhancement of the both, the absorption and conductivity of NixCd1-xO films for their possible application as integrated film photoanodes (TCO and PEC cell in one) within a hybrid water splitting device. (C) 2015 Elsevier B.V. All rights reserved. C1 [Ristova, Mimoza M.; Francis, Christopher; Yu, Kin M.; Walukiewicz, Wladislaw] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Ristova, Mimoza M.] Univ Ss Cyril & Methodius, Fac Nat Sci & Math, Dept Phys, Arhimedova 10, Skopje 1000, Macedonia. [Francis, Christopher; Toma, Francesca M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Toma, Francesca M.] JCAP, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Yu, Kin M.] City Univ Hong Kong, Dept Phys & Mat Sci, Kowloon, Hong Kong, Peoples R China. RP Ristova, MM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Ristova, MM (reprint author), Univ Ss Cyril & Methodius, Fac Nat Sci & Math, Dept Phys, Arhimedova 10, Skopje 1000, Macedonia. EM mima.ristova@gmail.com OI Francis, Christopher/0000-0002-4326-954X FU Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DESC0004993]; [68130116] FX This work was performed at the EMAT, LBNL and was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Dr. Ristova kindly expresses her gratitude to the Fulbright Visiting Scholar Program at the US Department of State for supporting her stay/research at the Lawrence Berkeley National Laboratory, Grant # 68130116 during entire 2014. A portion of this work was performed at the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DESC0004993. NR 26 TC 2 Z9 2 U1 6 U2 41 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0248 EI 1879-3398 J9 SOL ENERG MAT SOL C JI Sol. Energy Mater. Sol. Cells PD APR PY 2016 VL 147 BP 127 EP 133 DI 10.1016/j.solmat.2015.12.008 PG 7 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA DE0HL UT WOS:000370305600015 ER PT J AU Wolden, CA Abbas, A Li, JJ Diercks, DR Meysing, DM Ohno, TR Beach, JD Barnes, TM Walls, JM AF Wolden, Colin A. Abbas, Ali Li, Jiaojiao Diercks, David R. Meysing, Daniel M. Ohno, Timothy R. Beach, Joseph D. Barnes, Teresa M. Walls, John M. TI The roles of ZnTe buffer layers on CdTe solar cell performance SO SOLAR ENERGY MATERIALS AND SOLAR CELLS LA English DT Article DE CdTe; ZnTe; TEM; APT; Copper telluride ID BACK-CONTACT; CADMIUM TELLURIDE; CU; EFFICIENCY; FILM; DIFFUSION; THICKNESS; PHASES; CUXTE AB The use of ZnTe buffer layers at the back contact of CdTe solar cells has been credited with contributing to recent improvements in both champion cell efficiency and module stability. To better understand the controlling physical and chemical phenomena, high resolution transmission electron microscopy (HRTEM) and atom probe tomography (APT) were used to study the evolution of the back contact region during rapid thermal processing (RTP) of this layer. After activation the ZnTe layer, initially nanocrystalline and homogenous, transforms into a bilayer structure consisting of a disordered region in contact with CdTe characterized by significant Cd-Zn interdiffusion, and a nanocrystalline layer that shows evidence of grain growth and twin formation. Copper, co-evaporated uniformly within ZnTe, is found to dramatically segregate and aggregate after RTP, either collecting near the ZnTelAu interface or forming CuxTe clusters in the CdTe layer at defects or grain boundaries near the interface. Analysis of TEM images revealed that Zn accumulates at the edge of these clusters, and three-dimensional APT images confirmed that these are core-shell nanostructures consisting of CuiATe clusters encased in Zn. These changes in morphology and composition are related to cell performance and stability. (C) 2015 Elsevier B.V. All rights reserved. C1 [Wolden, Colin A.; Meysing, Daniel M.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. [Wolden, Colin A.; Li, Jiaojiao; Diercks, David R.] Colorado Sch Mines, Mat Sci Program, Golden, CO 80401 USA. [Abbas, Ali; Walls, John M.] Univ Loughborough, Loughborough LE11 3TU, Leics, England. [Meysing, Daniel M.; Barnes, Teresa M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Ohno, Timothy R.; Beach, Joseph D.] Colorado Sch Mines, Dept Phys, Golden, CO 80401 USA. RP Wolden, CA (reprint author), Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA.; Wolden, CA (reprint author), Colorado Sch Mines, Mat Sci Program, Golden, CO 80401 USA. EM cwolden@mines.edu OI Walls, John/0000-0003-4868-2621 FU Bay Area Photovoltaic Consortium under Department of Energy Award [DE-EE0004946]; UKERC through the EPSRC Supergen SuperSolar Hub; U.S. Department of Energy through the SunShot Foundational Program to Advance Cell Efficiency (F-PACE) [DE-AC36-08-GO28308] FX CAW, JL, DRD, TRO, and JDB gratefully acknowledge the Bay Area Photovoltaic Consortium for their support of this work under Department of Energy Award no. DE-EE0004946. AA and JMW was funded by UKERC through the EPSRC Supergen SuperSolar Hub. DMM and TMB were supported by the U.S. Department of Energy through the SunShot Foundational Program to Advance Cell Efficiency (F-PACE) under Contract no. DE-AC36-08-GO28308. NR 34 TC 7 Z9 7 U1 14 U2 61 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0248 EI 1879-3398 J9 SOL ENERG MAT SOL C JI Sol. Energy Mater. Sol. Cells PD APR PY 2016 VL 147 BP 203 EP 210 DI 10.1016/j.solmat.2015.12.019 PG 8 WC Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied SC Energy & Fuels; Materials Science; Physics GA DE0HL UT WOS:000370305600025 ER PT J AU Luo, YY Lu, J Liu, FK Wan, XQ AF Luo, Yiyong Lu, Jian Liu, Fukai Wan, Xiuquan TI The positive Indian Ocean Dipole-like response in the tropical Indian Ocean to global warming SO ADVANCES IN ATMOSPHERIC SCIENCES LA English DT Article DE Indian Ocean Dipole; positive Indian Ocean Dipole-like response; global warming; Bjerknes feedback ID COUPLED MODEL; VARIABILITY; EVENTS; SURFACE; TEMPERATURE; CIRCULATION; PACIFIC; ENSO; SST AB Climate models project a positive Indian Ocean Dipole (pIOD)-like SST response in the tropical Indian Ocean to global warming. By employing the Community Earth System Model and applying an overriding technique to its ocean component (version 2 of the Parallel Ocean Program), this study investigates the similarities and differences of the formation mechanisms for the changes in the tropical Indian Ocean during the pIOD versus global warming. Results show that their formation processes and related seasonality are quite similar; in particular, wind-thermocline-SST feedback is the leading mechanism in producing the anomalous cooling over the eastern tropics in both cases. Some differences are also found, including the fact that the cooling effect of the vertical advection over the eastern tropical Indian Ocean is dominated by the anomalous vertical velocity during the pIOD but by the anomalous upper-ocean stratification under global warming. These findings are further examined through an analysis of the mixed layer heat budget. C1 [Luo, Yiyong; Liu, Fukai; Wan, Xiuquan] Ocean Univ China, Phys Oceanog Lab, Qingdao 266100, Peoples R China. [Lu, Jian] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Luo, YY (reprint author), Ocean Univ China, Phys Oceanog Lab, Qingdao 266100, Peoples R China. EM yiyongluo@ouc.edu.cn FU National Basic Research Program of China [2012CB955600]; "Strategic Priority Research Program" of the Chinese Academy of Sciences [XDA11010302]; National Natural Science Foundation of China [41376009]; Joint Program of Shandong Province and National Natural Science Foundation of China [U1406401]; National Science Foundation [AGS-1249173]; Zhufeng and Taishan Projects of the Ocean University of China; Office of Science of the U.S. Department of Energy as part of the Regional and Global Climate Modeling program FX This work is supported by the National Basic Research Program of China (Grant No. 2012CB955600), the "Strategic Priority Research Program" of the Chinese Academy of Sciences (Grant No. XDA11010302), the National Natural Science Foundation of China (Grant No. 41376009), the Joint Program of Shandong Province and National Natural Science Foundation of China (Grant No. U1406401), and the National Science Foundation (Grant No. AGS-1249173). Y. LUO would also like to acknowledge the support from the Zhufeng and Taishan Projects of the Ocean University of China. J. LU is supported by the Office of Science of the U.S. Department of Energy as part of the Regional and Global Climate Modeling program. NR 27 TC 0 Z9 0 U1 2 U2 27 PU SCIENCE PRESS PI BEIJING PA 16 DONGHUANGCHENGGEN NORTH ST, BEIJING 100717, PEOPLES R CHINA SN 0256-1530 EI 1861-9533 J9 ADV ATMOS SCI JI Adv. Atmos. Sci. PD APR PY 2016 VL 33 IS 4 SI SI BP 476 EP 488 DI 10.1007/s00376-015-5027-5 PG 13 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DD6JI UT WOS:000370030100007 ER PT J AU Sarks, C Higbee, A Piotrowski, J Xue, SS Coon, JJ Sato, TK Jin, MJ Balan, V Dale, BE AF Sarks, Cory Higbee, Alan Piotrowski, Jeff Xue, Saisi Coon, Joshua J. Sato, Trey K. Jin, Mingjie Balan, Venkatesh Dale, Bruce E. TI Quantifying pretreatment degradation compounds in solution and accumulated by cells during solids and yeast recycling in the Rapid Bioconversion with Integrated recycling Technology process using AFEX (TM) corn stover SO BIORESOURCE TECHNOLOGY LA English DT Article DE AFEX (TM); Cellulosic ethanol; Pretreatment degradation products; Saccharomyces cerevisiae; Cell recycling ID FERMENTATION INHIBITORS; ETHANOL; PRODUCTS; BIOMASS; HYDROLYSATE; SOFTWARE AB Effects of degradation products (low molecular weight compounds produced during pretreatment) on the microbes used in the RaBIT (Rapid Bioconversion with Integrated recycling Technology) process that reduces enzyme usage up to 40% by efficient enzyme recycling were studied. Chemical genomic profiling was performed, showing no yeast response differences in hydrolysates produced during RaBIT enzymatic hydrolysis. Concentrations of degradation products in solution were quantified after different enzymatic hydrolysis cycles and fermentation cycles. Intracellular degradation product concentrations were also measured following fermentation. Degradation product concentrations in hydrolysate did not change between RaBIT enzymatic hydrolysis cycles; the cell population retained its ability to oxidize/reduce (detoxify) aldehydes over five RaBIT fermentation cycles; and degradation products accumulated within or on the cells as RaBIT fermentation cycles increased. Synthetic hydrolysate was used to confirm that pretreatment degradation products are the sole cause of decreased xylose consumption during RaBIT fermentations. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Sarks, Cory; Xue, Saisi; Jin, Mingjie; Balan, Venkatesh; Dale, Bruce E.] Michigan State Univ, Dept Chem Engn & Mat Sci, BCRL, 3815 Technol Blvd, Lansing, MI 48910 USA. [Sarks, Cory; Xue, Saisi; Jin, Mingjie; Balan, Venkatesh; Dale, Bruce E.] Michigan State Univ, DOE Great Lakes Bioenergy Res Ctr GLBRC, E Lansing, MI 48824 USA. [Higbee, Alan; Piotrowski, Jeff; Sato, Trey K.] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI 53704 USA. [Coon, Joshua J.] Univ Wisconsin, Dept Chem, 1101 Univ Ave, Madison, WI 53704 USA. [Coon, Joshua J.] Univ Wisconsin, Dept Biomol Chem, Madison, WI 53704 USA. RP Sarks, C (reprint author), Michigan State Univ, Dept Chem Engn & Mat Sci, BCRL, 3815 Technol Blvd, Lansing, MI 48910 USA. EM sarkscor@egr.msu.edu; ahigbee@glbrc.wisc.edu; jpiotrowski@wisc.edu; xuesaisi@egr.msu.edu; jcoon@chem.wisc.edu; tksato@glbrc.wisc.edu; jinmingj@egr.msu.edu; balan@egr.msu.edu; bdale@egr.msu.edu OI Xue, Saisi/0000-0002-1973-0666 FU U.S. Department of Energy through the DOE Great Lakes Bioenergy Research Center (GLBRC) Grant [DE-FC02-07ER64494] FX This work was supported by U.S. Department of Energy through the DOE Great Lakes Bioenergy Research Center (GLBRC) Grant DE-FC02-07ER64494. We thank Novozymes for supplying the commercial enzymes for this work. We thank Dr. Rebecca GarlockOng and Charles Donald, Jr. for providing/preparing AFEX pretreated corn stover. We thank Christa Gunawan for HPLC analysis. Finally, we thank members of the GLBRC fermentation group from University of Wisconsin for their valuable suggestions and input. NR 26 TC 1 Z9 1 U1 3 U2 14 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD APR PY 2016 VL 205 BP 24 EP 33 DI 10.1016/j.biortech.2016.01.008 PG 10 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA DD2BM UT WOS:000369727400004 PM 26802184 ER PT J AU Schell, DJ Dowe, N Chapeaux, A Nelson, RS Jennings, EW AF Schell, Daniel J. Dowe, Nancy Chapeaux, Alexandre Nelson, Robert S. Jennings, Edward W. TI Accounting for all sugars produced during integrated production of ethanol from lignocellulosic biomass SO BIORESOURCE TECHNOLOGY LA English DT Article DE Pretreatment; Enzymatic hydrolysis; Fermentation; Ethanol; Yields ID DILUTE-ACID PRETREATMENT; CORN STOVER; ZYMOMONAS-MOBILIS; FERMENTATION; CONFIGURATIONS; SACCHAROMYCES; PERFORMANCE; SHF AB Accurate mass balance and conversion data from integrated operation is needed to fully elucidate the economics of biofuel production processes. This study explored integrated conversion of corn stover to ethanol and highlights techniques for accurate yield calculations. Acid pretreated corn stover (PCS) produced in a pilot-scale reactor was enzymatically hydrolyzed and the resulting sugars were fermented to ethanol by the glucose-xylose fermenting bacteria, Zymomonas mobilis 8b. The calculations presented here account for high solids operation and oligomeric sugars produced during pretreatment, enzymatic hydrolysis, and fermentation, which, if not accounted for, leads to overestimating ethanol yields. The calculations are illustrated for enzymatic hydrolysis and fermentation of PCS at 17.5% and 20.0% total solids achieving 80.1% and 77.9% conversion of cellulose and xylan to ethanol and ethanol titers of 63 g/L and 69 g/L, respectively. These procedures will be employed in the future and the resulting information used for techno-economic analysis. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Schell, Daniel J.; Dowe, Nancy; Nelson, Robert S.; Jennings, Edward W.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. [Chapeaux, Alexandre] P2 Sci, 4 Res Dr, Woodbridge, CT 06525 USA. RP Schell, DJ (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM dan.schell@nrel.gov FU U.S. Department of Energy's Bioenergy Technologies Office; U.S. Government FX The authors wish to thank Xiaowen Chen, Eric Kuhn, and Nick Nagle for preparing and pretreating corn stover. We would also like to thank the U.S. Department of Energy's Bioenergy Technologies Office for funding this research.; The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. NR 19 TC 2 Z9 2 U1 5 U2 25 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0960-8524 EI 1873-2976 J9 BIORESOURCE TECHNOL JI Bioresour. Technol. PD APR PY 2016 VL 205 BP 153 EP 158 DI 10.1016/j.biortech.2016.01.024 PG 6 WC Agricultural Engineering; Biotechnology & Applied Microbiology; Energy & Fuels SC Agriculture; Biotechnology & Applied Microbiology; Energy & Fuels GA DD2BM UT WOS:000369727400020 PM 26826954 ER PT J AU Permann, CJ Tonks, MR Fromm, B Gaston, DR AF Permann, Cody J. Tonks, Michael R. Fromm, Bradley Gaston, Derek R. TI Order parameter re-mapping algorithm for 3D phase field model of grain growth using FEM SO COMPUTATIONAL MATERIALS SCIENCE LA English DT Article DE PF method; Finite element; Grain growth; 3D modeling; MOOSE ID COMPUTER-SIMULATION; BOUNDARY MIGRATION; FINITE-ELEMENT; EVOLUTION; DYNAMICS AB Phase field modeling (PFM) is a well-known technique for simulating microstructural evolution. To model grain growth using PFM, typically each grain is assigned a unique non-conserved order parameter and each order parameter field is evolved in time. Traditional approaches using a one-to-one mapping of grains to order parameters present a challenge when modeling large numbers of grains due to the computational expense of using many order parameters. This problem is exacerbated when using an implicit finite element method (FEM), as the global matrix size is proportional to the number of order parameters. While previous work has developed methods to reduce the number of required variables and thus computational complexity and run time, none of the existing approaches can be applied for an implicit FEM implementation of PFM. Here, we present a modular, dynamic, scalable reassignment algorithm suitable for use in such a system. Polycrystal modeling with grain growth and stress require careful tracking of each grain's position and orientation which is lost when using a reduced order parameter set. The method presented in this paper maintains a unique ID for each grain even after reassignment, to allow the PFM to be tightly coupled to calculations of the stress throughout the polycrystal. Implementation details and comparative results of our approach are presented. (C) 2016 Elsevier B.V. All rights reserved. C1 [Permann, Cody J.; Gaston, Derek R.] Idaho Natl Lab, Modeling & Simulat, POB 1625, Idaho Falls, ID 83415 USA. [Tonks, Michael R.; Fromm, Bradley] Idaho Natl Lab, Fuel Modeling & Simulat, POB 1625, Idaho Falls, ID 83415 USA. RP Permann, CJ (reprint author), Idaho Natl Lab, Modeling & Simulat, POB 1625, Idaho Falls, ID 83415 USA. FU Battelle Energy Alliance, LLC [DE-AC07-05ID14517]; US Department of Energy FX This work was funded by the Department of Energy Nuclear Energy Advanced Modeling and Simulation program. This manuscript has been authored by Battelle Energy Alliance, LLC under Contract No. DE-AC07-05ID14517 with the US Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 27 TC 3 Z9 3 U1 6 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0927-0256 EI 1879-0801 J9 COMP MATER SCI JI Comput. Mater. Sci. PD APR 1 PY 2016 VL 115 BP 18 EP 25 DI 10.1016/j.commatsci.2015.12.042 PG 8 WC Materials Science, Multidisciplinary SC Materials Science GA DD1PB UT WOS:000369692500003 ER PT J AU Stand, L Zhuravleva, M Camarda, G Lindsey, A Johnson, J Hobbs, C Melcher, CL AF Stand, L. Zhuravleva, M. Camarda, G. Lindsey, A. Johnson, J. Hobbs, C. Melcher, C. L. TI Exploring growth conditions and Eu2+ concentration effects for KSr2I5:Eu scintillator crystals SO JOURNAL OF CRYSTAL GROWTH LA English DT Article DE Bridgman technique; Single crystal growth; Halides; Potassium compounds; Scintillator; Micro-resolution X-ray mapping ID STRONTIUM IODIDE; RESOLUTION AB Our current research is focused on understanding dopant optimization, growth rate, homogeneity and their impact on the overall performance of KSr2I5:Eu2+ single crystal scintillators. In this work we have investigated the effects of Eu2+ concentration in the potassium strontium iodide matrix, and we found that the concentration needed to maximize the light yield was 4 mol%. In order to assess the effects of the pulling rate, we grew single crystals at 12, 24 and 120 mm/day via the vertical Bridgman technique. For the sample sizes measured (5 x 5 x 5 mm(3)), we found that the crystal grown at the fastest rate of 120 mm/day showed a light yield within similar to 7% of the more slowly grown boules, and no significant change was observed in the energy resolution. Therefore, light yields from 88,000 to 96,000 ph/MeV and energy resolutions from 2.4 to 3.0% (at 662 keV) were measured for KSr2I5:Eu 4% over a relatively wide range of growth conditions. In order to assess the homogeneity of KSr2I5:Eu 4%, a newly developed micro-resolution X-ray technique was used to map the light yield as a function of excitation position. In the crystals that we studied, we did not observe any significant inhomogeneity other than a smooth gradient due to light collection and self absorption effects. (C) 2016 Elsevier B.V. All rights reserved. C1 [Stand, L.; Zhuravleva, M.; Lindsey, A.; Johnson, J.; Hobbs, C.; Melcher, C. L.] Univ Tennessee, Scintillat Mat Res Ctr, Knoxville, TN USA. [Stand, L.; Zhuravleva, M.; Lindsey, A.; Johnson, J.; Hobbs, C.; Melcher, C. L.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Camarda, G.] Brookhaven Natl Lab, Nonproliferat & Natl Secur Dept, Upton, NY 11973 USA. RP Stand, L (reprint author), 1508 Middle Dr,414 Ferris Hall, Knoxville, TN 37996 USA. EM lstand@utk.edu OI Zhuravleva, Mariya/0000-0002-7809-5404 FU Domestic Nuclear Detection Office [2014-DN-077-ARI088-01, 2012-DN-077-ARI067-04]; US Department of Homeland Security FX This work was supported by the US Department of Homeland Security, Domestic Nuclear Detection Office, under Grant # 2014-DN-077-ARI088-01 and grant # 2012-DN-077-ARI067-04. This support does not constitute an express or implied endorsement on the part of the Government. NR 23 TC 2 Z9 2 U1 5 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-0248 EI 1873-5002 J9 J CRYST GROWTH JI J. Cryst. Growth PD APR 1 PY 2016 VL 439 BP 93 EP 98 DI 10.1016/j.jcrysgro.2015.12.048 PG 6 WC Crystallography; Materials Science, Multidisciplinary; Physics, Applied SC Crystallography; Materials Science; Physics GA DD6HM UT WOS:000370025300015 ER PT J AU Wu, CY Cline, D Hayes, A Flight, RS Melchionna, AM Zhou, C Lee, IY Swan, D Fox, R Anderson, JT AF Wu, C. Y. Cline, D. Hayes, A. Flight, R. S. Melchionna, A. M. Zhou, C. Lee, I. Y. Swan, D. Fox, R. Anderson, J. T. TI CHICO2, a two-dimensional pixelated parallel-plate avalanche counter SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Parallel-plate avalanche counter; Charged-particle detection; Pixelation; Radioactive beams ID SHAPE AB CHICO2 (Compact Heavy Ion COunter), is a large solid-angle, charged-particle detector array developed to provide both theta and phi angle resolutions matching those of GRETINA (Gamma-Ray Energy Tracking In beam Nuclear Array). CHICO2 was successfully tested at the Argonne National Laboratory where it was fielded as an auxiliary detector with GRETINA for gamma-ray spectroscopic studies of nuclei using a Cf-252 spontaneous fission source, stable beams, and radioactive beams from CARIBU. In field tests of the Ge-72,Ge-76 beams on a 0.5 mg/cm(2) Pb-208 target at the sub-barrier energy, CHICO2 provided charged-particle angle resolutions (FWHM) of 1.55 degrees in theta and 2.47 degrees in phi. This achieves the design goal for both coordinates assuming a beam-spot size ( > 3 mm) and the target thickness ( > 0.5 mg/cm(2)). The combined angular resolution of GRETINA/CHICO2 resulted in a Doppler-shift corrected energy resolution of 0.60% for 1 MeV coincident de-excitation gamma-rays. This is nearly a factor of two improvements in resolution and sensitivity compared to Gammasphere/CHICO. Kinematically-coincident detection of scattered ions by CHICO2 still maintains the mass resolution (Delta M/M) of similar to 5% that enhanced isolation of scattered weak beams of interest from scattered contaminant beams. (C) 2016 Elsevier B.V. All rights reserved. C1 [Wu, C. Y.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Cline, D.; Hayes, A.; Flight, R. S.; Melchionna, A. M.; Zhou, C.] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA. [Lee, I. Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Swan, D.] Swan Res LLC, Owosso, MI 48867 USA. [Fox, R.] CAEN Technol INC, Staten Isl, NY 10305 USA. [Anderson, J. T.] Argonne Natl Lab, Div High Energy Phys, Argonne, IL 60439 USA. RP Wu, CY (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM wu24@llnl.gov FU US Department of Energy by Lawrence Livermore National Security, LLC [DE-AC52-07NA27344]; US Department of Energy, Office of Nuclear Physics; US National Science Foundation FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Security, LLC under contract DE-AC52-07NA27344 and by the US Department of Energy, Office of Nuclear Physics, and US National Science Foundation support of the Rochester group. We thank Brian Bucher of LLNL as well as Shaofei Zhu and Daniel Ayangeakaa of ANL for their efforts to set up CHICO2 and extract figures from test runs and experiments described in this paper. NR 22 TC 1 Z9 1 U1 3 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD APR 1 PY 2016 VL 814 BP 6 EP 11 DI 10.1016/j.nima.2016.01.034 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DD1OW UT WOS:000369692000002 ER PT J AU Gallmeier, FX Iverson, EB Lu, W Baxter, DV Muhrer, G Ansell, S AF Gallmeier, F. X. Iverson, E. B. Lu, W. Baxter, D. V. Muhrer, G. Ansell, S. TI Introducing single-crystal scattering and optical potentials into MCNPX: Predicting neutron emission from a convoluted moderator SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Neutron source; Neutron moderation; Transport code; Simulation ID TRANSMISSION; SILICON AB Neutron transport simulation codes are indispensable tools for the design and construction of modern neutron scattering facilities and instrumentation. Recently, it has become increasingly clear that some neutron instrumentation has started to exploit physics that is not well-modeled by the existing codes. In particular, the transport of neutrons through single crystals and across interfaces in MCNP(X), Geant4, and other codes ignores scattering from oriented crystals and refractive effects, and yet these are essential phenomena for the performance of monochromators and ultra-cold neutron transport respectively (to mention but two examples). In light of these developments, we have extended the MCNPX code to include a single-crystal neutron scattering model and neutron reflection/refraction physics. We have also generated silicon scattering kernels for single crystals of definable orientation. As a first test of these new tools, we have chosen to model the recently developed convoluted moderator concept, in which a moderating material is interleaved with layers of perfect crystals to provide an exit path for neutrons moderated to energies below the crystal's Bragg cut-off from locations deep within the moderator. Studies of simple cylindrical convoluted moderator systems of 100 mm diameter and composed of polyethylene and single crystal silicon were performed with the upgraded MCNPX code and reproduced the magnitude of effects seen in experiments compared to homogeneous moderator systems. Applying different material properties for refraction and reflection, and by replacing the silicon in the models with voids, we show that the emission enhancements seen in recent experiments are primarily caused by the transparency of the silicon and void layers. Finally we simulated the convoluted moderator experiments described by Iverson et al. and found satisfactory agreement between the measurements and the simulations performed with the tools we have developed. (C) 2016 Elsevier B.V. All rights reserved. C1 [Gallmeier, F. X.; Iverson, E. B.; Lu, W.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Baxter, D. V.] Indiana Univ, Ctr Explorat Energy & Matter, Bloomington, IN 47408 USA. [Muhrer, G.; Ansell, S.] ESS AB, European Spallat Source, Lund, Sweden. RP Gallmeier, FX (reprint author), Oak Ridge Natl Lab, Spallat Neutron Source, Instrument & Source Div, POB 2008, Oak Ridge, TN 37831 USA. EM gallmeierfz@ornl.gov RI Baxter, David /D-3769-2013; OI Baxter, David /0000-0003-2812-0904; Iverson, Erik /0000-0002-7920-705X FU U.S. Department of Energy [DE-AC05-00OR22725] FX This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 24 TC 0 Z9 0 U1 3 U2 13 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD APR 1 PY 2016 VL 814 BP 39 EP 49 DI 10.1016/j.nima.2015.12.053 PG 11 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DD1OW UT WOS:000369692000006 ER PT J AU Weinmann-Smith, R Swinhoe, MT Hendricks, J AF Weinmann-Smith, R. Swinhoe, M. T. Hendricks, J. TI Measurement and simulation of cosmic rays effects on neutron multiplicity counting SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Safeguards; Neutron detector; Multiplicty; Cosmic ray; MCNP ID SPECTRA AB Neutron coincidence and multiplicity counting is a standard technique used to measure uranium and plutonium masses in unknown samples for nuclear safeguards purposes, but background sources of radiation can obscure the results. In particular, high energy cosmic rays can produce large coincidence count contributions. Since some of the events occur in the sample itself, it is impossible to measure the background separately. This effect greatly increases the limit of detection of some low level neutron coincidence counting applications. The cosmic ray capability of MCNP6 was used to calculate the expected coincidence rates from cosmic rays for different sample configurations and experimental measurements were conducted for comparison. Uranium enriched to 66%, lead bricks, and an empty detector were measured in the mini Epithermal Neutron Multiplicity Counter, and MCNP6 simulations were made of the same measurements. The results show that the capability is adequate for predicting the expected background rates. Additional verification of MCNP6 was given by comparison of particle production rates to other publications, increasing confidence in MCNP6's use as a tool to lower the limit of detection. MCNP6 was then used to find particle and source information that would be difficult to detect experimentally. The coincidence count contribution was broken down by particle type for singles, doubles, and triples rates. The coincidence count contribution was broken down by source, from(a, n), spontaneous fission, and cosmic rays, for each multiplicity. (C) 2016 Elsevier B.V. All rights reserved. C1 [Weinmann-Smith, R.] Univ Florida, 100 Rhines Hall,549 Gale Lemerand Dr,POB 116400, Gainesville, FL 32611 USA. [Weinmann-Smith, R.; Swinhoe, M. T.; Hendricks, J.] Los Alamos Natl Lab, POB 1663,MS E540, Los Alamos, NM 87545 USA. RP Weinmann-Smith, R (reprint author), Univ Florida, 100 Rhines Hall,549 Gale Lemerand Dr,POB 116400, Gainesville, FL 32611 USA. EM rweinmann@ufl.edu OI Swinhoe, Martyn/0000-0002-7620-4654 FU National Nuclear Security Administration Office of Nonproliferation and International Security FX Funding for this work was provided by the National Nuclear Security Administration Office of Nonproliferation and International Security, which had no involvement in the execution of the work. NR 19 TC 0 Z9 0 U1 1 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD APR 1 PY 2016 VL 814 BP 50 EP 55 DI 10.1016/j.nima.2016.01.012 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DD1OW UT WOS:000369692000007 ER PT J AU Croft, S Favalli, A Swinhoe, MT Goddard, B Stewart, S AF Croft, Stephen Favalli, Andrea Swinhoe, Martyn T. Goddard, Braden Stewart, Scott TI The effect of deadtime and electronic transients on the predelay bias in neutron coincidence counting SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Predelay; Neutron coincidence counting; Deadtime AB In neutron coincidence counting using the shift register autocorrelation technique, a predelay is inserted before the opening of the (R+A)-gate. Operationally the purpose of the predelay is to ensure that the (R+A)- and A-gates have matched effectiveness, otherwise a bias will result when the difference between the gates is used to calculate the accidentals corrected net reals coincidence rate. The necessity for the predelay was established experimentally in the early practical development and deployment of the coincidence counting method. The choice of predelay for a given detection system is usually made experimentally, but even today long standing traditional values (e.g., 4.5 mu s) are often used. This, at least in part, reflects the fact that a deep understanding of why a finite predelay setting is needed and how to control the underlying influences has not been fully worked out. In this paper we attempt to gain some insight into the problem. One aspect we consider is the slowing down, thermalization, and diffusion of neutrons in the detector moderator. The other is the influence of deadtime and electronic transients. These may be classified as non-ideal detector behaviors because they are not included in the conventional model used to interpret measurement data. From improved understanding of the effect of dead time and electronic transients on the predelay bias in neutron coincidence counting, the performance of both future and current coincidence counters may be improved. Published by Elsevier B.V. C1 [Croft, Stephen; Stewart, Scott] Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Favalli, Andrea; Swinhoe, Martyn T.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Goddard, Braden] Khalifa Univ Sci Technol & Res, POB 127788, Abu Dhabi, U Arab Emirates. RP Croft, S (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. FU U.S. Department of Energy (DOE), National Nuclear Security Administration (NNSA), Office of Nonproliferation Research and Development [NA-22] FX This work was sponsored in part by the U.S. Department of Energy (DOE), National Nuclear Security Administration (NNSA), Office of Nonproliferation Research and Development (NA-22). We take this opportunity to thank Dr. Peter Santi of LANL for his encouragement throughout this project. NR 28 TC 1 Z9 1 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD APR 1 PY 2016 VL 814 BP 96 EP 103 DI 10.1016/j.nima.2016.01.022 PG 8 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DD1OW UT WOS:000369692000013 ER PT J AU Dale, VH Kline, KL Buford, MA Volk, TA Smith, CT Stupak, I AF Dale, Virginia H. Kline, Keith L. Buford, Marilyn A. Volk, Timothy A. Smith, C. Tattersall Stupak, Inge TI Incorporating bioenergy into sustainable landscape designs SO RENEWABLE & SUSTAINABLE ENERGY REVIEWS LA English DT Review DE Adaptive management; Biofuel; Planning; Resource management; Scale; Stakeholder ID AGRICULTURAL RESIDUE REMOVAL; BIOMASS FEEDSTOCK PRODUCTION; BIOETHANOL SUPPLY CHAIN; DECISION-SUPPORT TOOL; FOREST MANAGEMENT; BIODIVERSITY CONSERVATION; STAKEHOLDER ENGAGEMENT; ENERGY SECURITY; MARGINAL LAND; SYSTEMS AB The paper describes an approach to landscape design that focuses on integrating bioenergy production with other components of environmental, social and economic systems. Landscape design as used here refers to a spatially explicit, collaborative plan for management of landscapes and supply chains. Landscape design can involve multiple scales and build on existing practices to reduce costs or enhance services. Appropriately applied to a specific context, landscape design can help people assess trade-offs when making choices about locations, types of feedstock, transport, refining and distribution of bioenergy products and services. The approach includes performance monitoring and reporting along the bioenergy supply chain. Examples of landscape design applied to bioenergy production systems are presented. Barriers to implementation of landscape design include high costs, the need to consider diverse land-management objectives from a wide array of stakeholders, up-front planning requirements, and the complexity and level of effort needed for successful stakeholder involvement. A landscape design process may be stymied by insufficient data or participation. An impetus for coordination is critical, and incentives may be required to engage landowners and the private sector. Hence devising and implementing landscape designs for more sustainable outcomes require clear communication of environmental, social, and economic opportunities and concerns. (C) 2015 The Authors. Published by Elsevier Ltd. This is an open access article under the CC BY-NC-ND license (http://creativecommons.org/licenses/by-nc-nd/4.0/). C1 [Dale, Virginia H.; Kline, Keith L.] Oak Ridge Natl Lab, Div Environm Sci, Ctr Bioenergy Sustainabil, POB 2008, Oak Ridge, TN 37831 USA. [Buford, Marilyn A.] US Forest Serv Res & Dev, Washington, DC 20250 USA. [Volk, Timothy A.] SUNY Coll Environm Sci & Forestry, Syracuse, NY 13210 USA. [Smith, C. Tattersall] Univ Toronto, Toronto, ON, Canada. [Stupak, Inge] Univ Copenhagen, Copenhagen, Denmark. RP Dale, VH (reprint author), 1 Bethel Valley Rd, Oak Ridge, TN 37830 USA. EM dalevh@ornl.gov; klinekl@ornl.gov; mbuford@fs.fed.us; tavolk@esf.edu; tat.smith@utoronto.ca; ism@ign.ku.dk OI Kline, Keith/0000-0003-2294-1170 FU U.S. Department of Energy (DOE) under the Bioenergy Technologies Office; DOE [DE-AC05-00OR22725] FX This research was supported by the U.S. Department of Energy (DOE) under the Bioenergy Technologies Office. Oak Ridge National Laboratory is managed by UT-Battelle, LLC, for DOE under Contract DE-AC05-00OR22725. Comments by Ben Wigley, Arnaldo Walter, Camila Ortolan Fernandes de Oliveira, and Yetta Jager on an earlier draft are greatly appreciated. Erica Atkin edited the manuscript, and Gina Busby helped check references. This paper is dedicated to the memory of Al Lucier, who helped organize a workshop on "Incorporating Bioenergy in Sustainable Landscape Designs" held in March 2014 in New Bern, North Carolina, at which many of our ideas developed. NR 103 TC 6 Z9 6 U1 10 U2 38 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1364-0321 J9 RENEW SUST ENERG REV JI Renew. Sust. Energ. Rev. PD APR PY 2016 VL 56 BP 1158 EP 1171 DI 10.1016/j.rser.2015.12.038 PG 14 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA DC8IC UT WOS:000369462100090 ER PT J AU Fornasiero, F LeBlanc, M Charnvanichborikarn, S Kucheyev, SO Shin, SJ Gong, KP Ci, LJ Park, J Miles, R AF Fornasiero, Francesco LeBlanc, Mary Charnvanichborikarn, Supakit Kucheyev, Sergei O. Shin, Swanee J. Gong, Kuanping Ci, Lijie Park, Jinseong Miles, Robin TI Hierarchical reinforcement of randomly-oriented carbon nanotube mats by ion irradiation SO CARBON LA English DT Article ID SPIDER SILK FIBRILS; MECHANICAL-PROPERTIES; HIGH-PERFORMANCE; RAMAN-SPECTROSCOPY; WIGNER DEFECTS; HIGH-STRENGTH; COMPOSITES; FIBERS; TOUGHNESS; STIFFNESS AB Because of their outstanding mechanical properties, carbon nanotubes (CNTs) are attractive 1-D nanoscale building blocks for lightweight composites that could potentially outperform naturally occurring materials. A still unsolved challenge for fully exploiting CNT superior mechanical properties for reinforcement of macroscopic systems is control of the interfacial interaction across multiple length scales to favor load transfer. Toward overcoming this challenge, we investigate here the effect of high-energy He+ ion irradiation on the elastic modulus and tensile strength of thin films of randomly oriented double-walled nanotube (DWCNT) mats and DWCNT-epoxy composites. We correlate irradiation-induced reinforcement with the formation of cross-links at different hierarchical levels of the DWCNT network. Our measurements reveal a rapidly increasing reinforcement at low ion doses, attributed to intra-bundle CNT cross-links, followed by a slow mechanical reinforcement at higher doses, associated to inter-bundle cross-links. At the highest ion irradiation dose of this study, the strength and elastic modulus of DWCNT-epoxy composites approach similar to 900 MPa and 25 GPa, respectively, which is among the best mechanical performances reported for randomly-oriented CNT mats. We also develop a model accounting for radiation-induced hierarchical reinforcement of DWCNT films. The model is in good agreement with the experimental results across the entire dose range. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Fornasiero, Francesco; LeBlanc, Mary; Charnvanichborikarn, Supakit; Kucheyev, Sergei O.; Shin, Swanee J.; Miles, Robin] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. [Gong, Kuanping; Park, Jinseong] Samsung Cheil Ind, San Jose Lab, 2186 Bering Dr, San Jose, CA 95131 USA. [Ci, Lijie] Shandong Univ, Sch Mat Sci & Engn, Jinan 250061, Peoples R China. RP Fornasiero, F (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM fornasiero1@llnl.gov OI Fornasiero, Francesco/0000-0002-3505-5867 FU Lawrence Livermore National Laboratory; U.S. Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by Lawrence Livermore National Laboratory. Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the U.S. Department of Energy, National Nuclear Security Administration under Contract DE-AC52-07NA27344. TEM experiments were conducted at the National Center for Electron Microscopy, Molecular Foundry, Lawrence Berkeley National Lab, which is supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract # DE-AC02-05CH11231. NR 80 TC 0 Z9 0 U1 8 U2 42 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0008-6223 EI 1873-3891 J9 CARBON JI Carbon PD APR PY 2016 VL 99 BP 491 EP 501 DI 10.1016/j.carbon.2015.12.042 PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DC2TP UT WOS:000369069800059 ER PT J AU Zeng, XM Du, ZH Schuh, CA Tamura, N Gan, CL AF Zeng, Xiao Mei Du, Zehui Schuh, Christopher A. Tamura, Nobumichi Gan, Chee Lip TI Microstructure, crystallization and shape memory behavior of titania and yttria co-doped zirconia SO JOURNAL OF THE EUROPEAN CERAMIC SOCIETY LA English DT Article DE Titania doping; YDZ; Microstructure; Crystallization; Elemental analysis; Shape memory effect ID ARC-MELTED ZRO2-2MOL-PERCENT-Y2O3; PARTIALLY-STABILIZED ZIRCONIA; GRAIN BOUNDARY MOTION; TETRAGONAL ZIRCONIA; MONOCLINIC TRANSFORMATION; MARTENSITIC TRANSFORMATIONS; PHASE-TRANSFORMATION; CERAMICS; POLYCRYSTALS; PLASTICITY AB Small volume zirconia ceramics with few or no grain boundaries have been demonstrated recently to exhibit the shape memory effect. To explore the shape memory properties of yttria doped zirconia (YDZ), it is desirable to develop large, microscale grains, instead of submicron grains that result from typical processing of YDZ. In this work, we have successfully produced single crystal micro-pillars from microscale grains encouraged by the addition of titania during processing. Titania has been doped into YDZ ceramics and its effect on the grain growth, crystallization and microscale elemental distribution of the ceramics have been systematically studied. With 5 mol% titania doping, the grain size can be increased up to similar to 4 mu m, while retaining a large quantity of the desired tetragonal phase of zirconia. Micro-pillars machined from tetragonal grains exhibit the expected shape memory effects where pillars made from titania-free YDZ would not. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Zeng, Xiao Mei; Du, Zehui; Gan, Chee Lip] Nanyang Technol Univ, Temasek Labs, Singapore 637553, Singapore. [Zeng, Xiao Mei; Gan, Chee Lip] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore. [Schuh, Christopher A.] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Tamura, Nobumichi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Gan, CL (reprint author), Nanyang Technol Univ, Temasek Labs, Singapore 637553, Singapore. EM CLGan@ntu.edu.sg RI Gan, Chee Lip/A-2248-2011 OI Gan, Chee Lip/0000-0002-8420-3168 FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy; [9011102294]; [9011102296] FX We would like to thank Dr Liu Qing, Dr Jason Scott Herrin, Shahrouz Amini and Dr Ali Gilles Tchenguise Miserez at NTU for their assistance with experiments. We would like to acknowledge the project funding support under project agreements 9011102294 and 9011102296. The Advanced Light Source (ALS) is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 at the Lawrence Berkeley National Laboratory (LBNL). NR 38 TC 2 Z9 2 U1 4 U2 30 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 0955-2219 EI 1873-619X J9 J EUR CERAM SOC JI J. Eur. Ceram. Soc. PD APR PY 2016 VL 36 IS 5 BP 1277 EP 1283 DI 10.1016/j.jeurceramsoc.2015.11.042 PG 7 WC Materials Science, Ceramics SC Materials Science GA DC8GG UT WOS:000369457300018 ER PT J AU Rai, V Reeves, DC Margolis, R AF Rai, Varun Reeves, D. Cale Margolis, Robert TI Overcoming barriers and uncertainties in the adoption of residential solar PV SO RENEWABLE ENERGY LA English DT Article DE Solar photovoltaic (PV); Information channels; Peer effects; Consumer behavior; Leasing; Individual decision-making ID POWER-SYSTEMS; DIFFUSION; TECHNOLOGIES; GENERATION; CALIFORNIA; DESIGN; MODEL AB In recent years decreasing hardware costs have driven down the installed price of solar photovoltaic (PV) systems and spurred adoption. However, system cost is not the only barrier faced by solar adopters. Potential adopters also face various informational barriers, leading to high indirect costs during the information search process. There is a significant gap in the literature for empirical work on solar adoption linking how the information context (installer marketing; neighbors with solar, i.e., peer effects; etc.) interacts with a potential adopter's motivations to impact decision outcomes. To address this gap we present results of a new survey on the decision-making process of residential PV adopters in northern California. The main aspects of our analysis include: salient motivating factors, information gathering process, peer effects, role of installers, and factors driving the choice of outright purchase versus third-party ownership (e.g., leasing) modes of adoption. We find that installers and neighbors play important, but often supplementary, roles throughout the decision-making process and have influence on both the decision to adopt as well as on the mode of adoption. Furthermore, expected financial returns and concerns about operations and maintenance are the main determining factors for the mode of adoption. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Rai, Varun; Reeves, D. Cale] Univ Texas Austin, LBJ Sch Publ Affairs, 2315 Red River St, Austin, TX 78712 USA. [Rai, Varun] Univ Texas Austin, Dept Mech Engn, 2315 Red River St, Austin, TX 78712 USA. [Margolis, Robert] Natl Renewable Energy Lab, Washington, DC USA. RP Rai, V (reprint author), Univ Texas Austin, LBJ Sch Publ Affairs, 2315 Red River St, Austin, TX 78712 USA.; Rai, V (reprint author), Univ Texas Austin, Dept Mech Engn, 2315 Red River St, Austin, TX 78712 USA.; Rai, V (reprint author), Univ Texas Austin, 2315 Red River St, Austin, TX 78712 USA. EM raivarun@utexas.edu OI Rai, Varun/0000-0002-4080-9299 FU National Renewable Energy Laboratory [XGG-3-23326-01]; Elspeth Rostow Memorial Fellowship FX We thank Carolyn Davidson, Easan Drury, and Scott Robinson for valuable feedback and insights. This work was funded by the National Renewable Energy Laboratory (Subcontract # XGG-3-23326-01). VR acknowledges support from the Elspeth Rostow Memorial Fellowship. All remaining errors are ours alone. NR 38 TC 5 Z9 5 U1 12 U2 34 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0960-1481 J9 RENEW ENERG JI Renew. Energy PD APR PY 2016 VL 89 BP 498 EP 505 DI 10.1016/j.renene.2015.11.080 PG 8 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA DC4KU UT WOS:000369190600046 ER PT J AU Chang, G Ruehl, K Jones, CA Roberts, J Chartrand, C AF Chang, G. Ruehl, K. Jones, C. A. Roberts, J. Chartrand, C. TI Numerical modeling of the effects of wave energy converter characteristics on nearshore wave conditions SO RENEWABLE ENERGY LA English DT Article DE Wave energy converter (WEC); Wave modeling; Model sensitivity; Simulating WAves Nearshore (SWAN); Nearshore wave propagation ID PORTUGUESE NEARSHORE; COASTAL REGIONS; FARM; IMPACT; CLIMATE; DEVICES AB Modeled nearshore wave propagation was investigated downstream of simulated wave energy converters (WECs) to evaluate overall near- and far-field effects of WEC arrays. Model sensitivity to WEC characteristics and WEC array deployment scenarios was evaluated using a modified version of an industry standard wave model, Simulating WAves Nearshore (SWAN), which allows the incorporation of device-specific WEC characteristics to specify obstacle transmission. The sensitivity study illustrated that WEC device type and subsequently its size directly resulted in wave height variations in the lee of the WEC array. Wave heights decreased up to 30% between modeled scenarios with and without WECs for large arrays (100 devices) of relatively sizable devices (26 m in diameter) with peak power generation near to the modeled incident wave height. Other WEC types resulted in less than 15% differences in modeled wave height with and without WECs, with lesser influence for WECs less than 10 m in diameter. Wave directions and periods were largely insensitive to changes in parameters. However, additional model parameterization and analysis are required to fully explore the model sensitivity of peak wave period and mean wave direction to the varying of the parameters. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Chang, G.; Jones, C. A.] Integral Consulting Inc, 200 Washington St,Suite 101, Santa Cruz, CA 95060 USA. [Ruehl, K.; Roberts, J.; Chartrand, C.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Chang, G (reprint author), Integral Consulting Inc, 200 Washington St,Suite 101, Santa Cruz, CA 95060 USA. EM gchang@integral-corp.com; kmruehl@sandia.gov; cjones@integral-corp.com; jdrober@sandia.gov; ccchart@sandia.gov FU Department of Energy's Wind and Water Power Technologies Office - U.S. Department of Energy; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This research was made possible by support from the Department of Energy's Wind and Water Power Technologies Office, funded by the U.S. Department of Energy. Sandia is a multi-program laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. Special thanks to Ari Posner for early developmental efforts associated with SNL-SWAN and to Jason Magalen for initial SWAN model set-up and sensitivity studies. NR 28 TC 5 Z9 5 U1 8 U2 26 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0960-1481 J9 RENEW ENERG JI Renew. Energy PD APR PY 2016 VL 89 BP 636 EP 648 DI 10.1016/j.renene.2015.12.048 PG 13 WC GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY; Energy & Fuels SC Science & Technology - Other Topics; Energy & Fuels GA DC4KU UT WOS:000369190600059 ER PT J AU McMurray, JW AF McMurray, J. W. TI Characterization of urania vaporization with transpiration coupled thermogravimetry SO JOURNAL OF CHEMICAL THERMODYNAMICS LA English DT Article DE UO2 +/- x; UO3; Uranium; Urania; Volatilization; Oxygen potential; Phase equilibrium ID VAPOR-PRESSURE; FUEL AB Transpiration measurements are very useful for determining equilibrium vapor pressures of materials. However, the traditional technique involves condensing the volatiles entrained in a carrier gas outside of the hot measurement zone. One potential problem is deposition en route to a cooled collector. Thermogravimetric analysis (TGA) can be used to measure in situ mass loss due to vaporization and therefore obviate the need to analyze the entire gas train due to premature plating of vapor species. Therefore, a transpiration coupled TGA technique was used to determine equilibrium pressures of UO3 gas over fluorite structure UO2+x and U3O8 at T = (1573 and 1773) K. The results are compared to calculations from models and databases in the open literature. This study gives clarity to the thermochemical data for UO3 gas and validates the mass loss transpiration method using thermogravimetry for determining equilibrium vapor pressures of non-stoichiometric oxides. (C) 2015 Elsevier Ltd. All rights reserved. C1 [McMurray, J. W.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP McMurray, JW (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM mcmurrayjw1@ornl.gov OI McMurray, Jacob/0000-0001-5111-3054 FU US Department of Energy, Office of Nuclear Energy Fuel Cycle Technology Program FX The author would like to thank Dr. Nathan S. Jacobson of NASA Glenn Research Center for invaluable guidance and helpful comments. The author would also like to thank Wally Porter and Cristian Contescu of Oak Ridge National Laboratory. The work was supported by the US Department of Energy, Office of Nuclear Energy Fuel Cycle Technology Program. NR 16 TC 0 Z9 0 U1 3 U2 10 PU ACADEMIC PRESS LTD- ELSEVIER SCIENCE LTD PI LONDON PA 24-28 OVAL RD, LONDON NW1 7DX, ENGLAND SN 0021-9614 EI 1096-3626 J9 J CHEM THERMODYN JI J. Chem. Thermodyn. PD APR PY 2016 VL 95 BP 72 EP 76 DI 10.1016/j.jct.2015.11.026 PG 5 WC Thermodynamics; Chemistry, Physical SC Thermodynamics; Chemistry GA DB8JI UT WOS:000368762600009 ER PT J AU Spencer, S Chung, J Thompson, M Piedra, PA Jewell, A Avadhanula, V Mei, MH Jackson, ML Meece, J Sundaram, M Belongia, EA Cross, R Johnson, E Bullotta, A Rinaldo, C Gaglani, M Murthy, K Clipper, L Berman, L Flannery, B AF Spencer, Sarah Chung, Jessie Thompson, Mark Piedra, Pedro A. Jewell, Alan Avadhanula, Vasanthi Mei, Minghua Jackson, Michael L. Meece, Jennifer Sundaram, Maria Belongia, Edward A. Cross, Rachel Johnson, Emileigh Bullotta, Arlene Rinaldo, Charles Gaglani, Manjusha Murthy, Kempapura Clipper, Lydia Berman, LaShondra Flannery, Brendan TI Factors associated with real-time RT-PCR cycle threshold values among medically attended influenza episodes SO JOURNAL OF MEDICAL VIROLOGY LA English DT Article DE Influenza; RT-PCR; cycle threshold value ID REVERSE TRANSCRIPTION-PCR; VACCINE EFFECTIVENESS; SEASONAL INFLUENZA; VIRUS DETECTION; ADULT PATIENTS; UNITED-STATES; VIRAL LOADS; QUANTIFICATION; INFECTION; DIAGNOSIS AB We evaluated the cycle threshold (CT) values of 1,160 influenza A positive and 806 influenza B positive specimens from two seasons of the US Flu VE Network to identify factors associated with CT values. Low CT values (high genomic load) were associated with shorter intervals between illness onset and specimen collection, young age (ages 3-8 years old), and self-rated illness severity for both influenza A and B. Low CT values were also associated with reported fever/feverishness and age 65 years for influenza A. J. Med. Virol. 88:719-723, 2016. (c) 2015 Wiley Periodicals, Inc. C1 [Spencer, Sarah; Chung, Jessie; Thompson, Mark; Berman, LaShondra; Flannery, Brendan] Ctr Dis Control & Prevent, Influenza Div, Atlanta, GA 30329 USA. [Spencer, Sarah; Chung, Jessie] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Piedra, Pedro A.; Jewell, Alan; Avadhanula, Vasanthi; Mei, Minghua] Baylor Coll Med, Dept Mol Virol & Microbiol, Houston, TX 77030 USA. [Piedra, Pedro A.] Baylor Coll Med, Dept Pediat, Houston, TX 77030 USA. [Jackson, Michael L.] Grp Hlth Res Inst, Seattle, WA USA. [Meece, Jennifer; Sundaram, Maria; Belongia, Edward A.] Marshfield Clin Res Fdn, Marshfield, WI USA. [Cross, Rachel; Johnson, Emileigh] Univ Michigan, Sch Publ Hlth, Dept Epidemiol, Ann Arbor, MI 48109 USA. [Bullotta, Arlene; Rinaldo, Charles] Univ Pittsburgh, Dept Pathol, Pittsburgh, PA USA. [Gaglani, Manjusha; Murthy, Kempapura; Clipper, Lydia] Scott & White Healthcare, Temple, TX USA. RP Spencer, S (reprint author), Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA.; Spencer, S (reprint author), Ctr Dis Control & Prevent, 1600 Clifton RD MS A32, Atlanta, GA 30329 USA. EM vmf5@cdc.gov FU Centers for Disease Control and Prevention; Group Health Research Institute [U01 IP000474]; Marshfield Clinic Research Foundation [U01 IP000466]; University of Pittsburgh [U01 IP000471]; Scott and White Healthcare [U01 IP000467]; University of Michigan [U01 IP000473] FX Grant sponsor: Centers for Disease Control and Prevention; Group Health Research Institute; Grant number: U01 IP000474; Grant sponsor: Marshfield Clinic Research Foundation; Grant number: U01 IP000466; Grant sponsor: University of Pittsburgh; Grant number: U01 IP000471; Grant sponsor: Scott and White Healthcare; Grant number: U01 IP000467; Grant sponsor: University of Michigan; Grant number: U01 IP000473. NR 25 TC 1 Z9 1 U1 1 U2 13 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0146-6615 EI 1096-9071 J9 J MED VIROL JI J. Med. Virol. PD APR PY 2016 VL 88 IS 4 BP 719 EP 723 DI 10.1002/jmv.24373 PG 5 WC Virology SC Virology GA DC4IL UT WOS:000369184300020 PM 26334765 ER PT J AU Mudiyanselage, K Luo, S Kim, HY Yang, XF Baber, AE Hoffmann, FM Senanayake, S Rodriguez, JA Chen, JGG Liu, P Stacchiola, DJ AF Mudiyanselage, Kumudu Luo, Si Kim, Hyun You Yang, Xiaofang Baber, Ashleigh E. Hoffmann, Friedrich M. Senanayake, Sanjaya Rodriguez, Jose A. Chen, Jingguang G. Liu, Ping Stacchiola, Dario J. TI How to stabilize highly active Cu+ cations in a mixed-oxide catalyst SO CATALYSIS TODAY LA English DT Article DE IRRAS; Mixed -metal oxides; CO; Copper; Titanium; Catalysis ID WATER-GAS SHIFT; IN-SITU; CARBON-MONOXIDE; METAL-OXIDE; ADSORPTION; CU(111); SURFACE; COPPER; CO; NANOPARTICLES AB Mixed-metal oxides exhibit novel properties that are not present in their isolated constituent metal oxides and play a significant role in heterogeneous catalysis. In this study, a titanium-copper mixed-oxide (TiCuOx) film has been synthesized on Cu(1 1 1) and characterized by complementary experimental and theoretical methods. At sub-monolayer coverages of titanium, a Cu2O-like phase coexists with TiCuOx and TiOx domains. When the mixed-oxide surface is exposed at elevated temperatures (600-650 K) to oxygen, the formation of a well-ordered TiCuOx film occurs. Stepwise oxidation of TiCuOx shows that the formation of the mixed -oxide is faster than that of pure Cu2O. As the Ti coverage increases, Ti-rich islands (TiOx) form. The adsorption of CO has been used to probe the exposed surface sites on the TiOx-CuO, system, indicating the existence of a new Cu+ adsorption site that is not present on Cu2O/Cu(1 1 1). Adsorption of CO on Cu+ sites of TiCuO, is thermally more stable than on Cu(1 1 1), Cu2O/Cu(1 1 1) or TiO2(1 1 0). The Cu+ sites in TiCuOx domains are stable under both reducing and oxidizing conditions whereas the Cu2O domains present on sub-monolayer loads of Ti can be reduced or oxidized under mild conditions. The results presented here demonstrate novel properties of TiCuOx films, which are not present on Cu(1 1 1), Cu2O/Cu(1 1 1), or Ti02(1 10), and highlight the importance of the preparation and characterization of well-defined mixed-metal oxides in order to understand fundamental processes that could guide the design of new materials. (C) 2015 Elsevier B.V. All rights reserved. C1 [Mudiyanselage, Kumudu; Yang, Xiaofang; Senanayake, Sanjaya; Rodriguez, Jose A.; Liu, Ping; Stacchiola, Dario J.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Luo, Si] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Kim, Hyun You] Chungnam Natl Univ, Dept Mat Sci & Engn, Taejon 305764, South Korea. [Baber, Ashleigh E.] James Madison Univ, Dept Chem & Biochem, Harrisonburg, VA 22807 USA. [Hoffmann, Friedrich M.] BMCC CUNY, Dept Sci, New York, NY 10007 USA. [Chen, Jingguang G.] Columbia Univ, Dept Chem Engn, New York, NY 10027 USA. RP Stacchiola, DJ (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM djs@bnl.gov RI Stacchiola, Dario/B-1918-2009; Mudiyanselage, Kumudu/B-2277-2013 OI Stacchiola, Dario/0000-0001-5494-3205; Mudiyanselage, Kumudu/0000-0002-3539-632X FU U.S. Department of Energy, Office of Basic Energy Science [DE-SC0012704] FX This manuscript has been authored by employees of Brookhaven Science Associates, LLC under Contract No. DE-SC0012704 with the U.S. Department of Energy, Office of Basic Energy Science. The publisher by accepting the manuscript for publication acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. NR 30 TC 1 Z9 1 U1 18 U2 83 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD APR 1 PY 2016 VL 263 SI SI BP 4 EP 10 DI 10.1016/j.cattod.2015.08.025 PG 7 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA DB5XS UT WOS:000368587700002 ER PT J AU Kraemer, S Rondinone, AJ Tsai, YT Schwartz, V Overbury, SH Idrobo, JC Wu, ZL AF Kraemer, Shannon Rondinone, Adam J. Tsai, Yu-Tong Schwartz, Viviane Overbury, Steven H. Idrobo, Juan-Carlos Wu, Zili TI Oxidative dehydrogenation of isobutane over vanadia catalysts supported by titania nanoshapes SO CATALYSIS TODAY LA English DT Article DE Titania; Vanadia; Support effect; Nanoshapes; Surface facets; Surface structure; Oxygen vacancy formation energy; Isobutane oxidative dehydrogenation; Raman spectroscopy ID SITU RAMAN-SPECTROSCOPY; OXIDE CATALYSTS; MOLECULAR-STRUCTURES; V2O5/TIO2 CATALYSTS; VOX/CEO2 CATALYSTS; PROPANE; CERIA; TIO2; REACTIVITY; KINETICS AB Support plays a complex role in catalysis by supported metal oxides and the exact support effect still remains elusive. One of the approaches to gain fundamental insights into the support effect is to utilize model support systems. In this paper, we employed for the first time titania nanoshapes as the model supports and investigated how the variation of surface structure of the support (titania, TiO2) impacts the catalysis of supported oxide (vanadia, VOx). TiO2 truncated rhombi, spheres and rods were synthesized via hydrothermal method and characterized with XRD and TEM. These TiO2 nanoshapes represent different mixtures of surface facets including [101], [010] and [001] and were used to support vanadia. The structure of supported VOx species was characterized in detail with in situ Raman spectroscopy as a function of loading on the three TiO2 nanoshapes. Oxidative dehydrogenation (ODH) of isobutane to isobutene was used as a model reaction to test how the support shape influences the activity, selectivity and activation energy of the surface VOx species. It was shown that the shape of TiO2 support does not pose evident effect on either the structure of surface VOx species or the catalytic performance of surface VOx species in isobutane ODH reaction. This insignificant support shape effect was ascribed to the small difference in the surface oxygen vacancy formation energy among the different TiO2 surfaces and the multi-faceting nature of the TiO2 nanoshapes. Published by Elsevier B.V. C1 [Kraemer, Shannon; Rondinone, Adam J.; Tsai, Yu-Tong; Schwartz, Viviane; Overbury, Steven H.; Idrobo, Juan-Carlos; Wu, Zili] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Wu, ZL (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM wuz1@ornl.gov RI Overbury, Steven/C-5108-2016; Rondinone, Adam/F-6489-2013 OI Overbury, Steven/0000-0002-5137-3961; Rondinone, Adam/0000-0003-0020-4612 FU Center for Understanding & Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME), an Energy Frontier Research Center - DOE, Office of Science, Basic Energy Sciences FX This work was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. Z. Wu was partly supported by the Center for Understanding & Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME), an Energy Frontier Research Center funded by DOE, Office of Science, Basic Energy Sciences. NR 42 TC 1 Z9 1 U1 12 U2 81 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD APR 1 PY 2016 VL 263 SI SI BP 84 EP 90 DI 10.1016/j.cattod.2015.09.049 PG 7 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA DB5XS UT WOS:000368587700012 ER PT J AU Schuck, PJ Bao, W Borys, NJ AF Schuck, P. James Bao, Wei Borys, Nicholas J. TI A polarizing situation: Taking an in-plane perspective for next-generation near-field studies SO FRONTIERS OF PHYSICS LA English DT Review DE near-field optical microscopy; nano-optics; TERS; plasmonics; optical antenna; 2D materials ID ENHANCED RAMAN-SPECTROSCOPY; SCANNING OPTICAL MICROSCOPY; SINGLE-LAYER MOS2; VAN-DER-WAALS; TRANSITION-METAL DICHALCOGENIDES; CARBON NANOTUBES; PLASMONIC NANOANTENNAS; 2-DIMENSIONAL MATERIALS; GRAPHENE PLASMONS; MAGNETIC DOMAINS AB By enabling the probing of light-matter interactions at the functionally relevant length scales of most materials, near-field optical imaging and spectroscopy accesses information that is unobtainable with other methods. The advent of apertureless techniques, which exploit the ultralocalized and enhanced near-fields created by sharp metallic tips or plasmonic nanoparticles, has resulted in rapid adoption of near-field approaches for studying novel materials and phenomena, with spatial resolution approaching sub-molecular levels. However, these approaches are generally limited by the dominant out-of-plane polarization response of apertureless tips, restricting the exploration and discovery of many material properties. This has led to recent design and fabrication breakthroughs in near-field tips engineered specifically for enhancing in-plane interactions with near-field light components. This mini-review provides a perspective on recent progress and emerging directions aimed at utilizing and controlling in-plane optical polarization, highlighting key application spaces where in-plane near-field tip responses have enabled recent advancements in the understanding and development of new nanostructured materials and devices. C1 [Schuck, P. James; Bao, Wei; Borys, Nicholas J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Bao, Wei] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Schuck, PJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. EM pjschuck@lbl.gov FU Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of U.S. Department of Energy [DE-AC02-05CH11231] FX The authors thank our colleagues at the Molecular Foundry for stimulating discussion and assistance. Work at the Molecular Foundry was supported by the Director, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 263 TC 1 Z9 1 U1 17 U2 145 PU HIGHER EDUCATION PRESS PI BEIJING PA NO 4 DEWAI DAJIE, BEIJING 100120, PEOPLES R CHINA SN 2095-0462 J9 FRONT PHYS-BEIJING JI Front. Phys. PD APR PY 2016 VL 11 IS 2 AR 117804 DI 10.1007/s11467-015-0526-5 PG 17 WC Physics, Multidisciplinary SC Physics GA DB1UE UT WOS:000368293700003 ER PT J AU van Baren, MJ Bachy, C Reistetter, EN Purvine, SO Grimwood, J Sudek, S Yu, H Poirier, C Deerinck, TJ Kuo, A Grigoriev, IV Wong, CH Smith, RD Callister, SJ Wei, CL Schmutz, J Worden, AZ AF van Baren, Marijke J. Bachy, Charles Reistetter, Emily Nahas Purvine, Samuel O. Grimwood, Jane Sudek, Sebastian Yu, Hang Poirier, Camille Deerinck, Thomas J. Kuo, Alan Grigoriev, Igor V. Wong, Chee-Hong Smith, Richard D. Callister, Stephen J. Wei, Chia-Lin Schmutz, Jeremy Worden, Alexandra Z. TI Evidence-based green algal genomics reveals marine diversity and ancestral characteristics of land plants SO BMC GENOMICS LA English DT Article DE GreenCut; Archaeplastida evolution; Viridiplantae; Introner Elements; RNA sequencing; Proteomics; Evidence-based gene models; Peptidoglycan; PPASP ID PEPTIDOGLYCAN SYNTHESIS PATHWAY; TANDEM MASS-SPECTRA; RNA-SEQ DATA; CHLOROPLAST DIVISION; EUKARYOTIC LINEAGES; MICROMONAS-PUSILLA; CELL WALL; PROTEINS; PRASINOPHYCEAE; BIOSYNTHESIS AB Background: Prasinophytes are widespread marine green algae that are related to plants. Cellular abundance of the prasinophyte Micromonas has reportedly increased in the Arctic due to climate-induced changes. Thus, studies of these unicellular eukaryotes are important for marine ecology and for understanding Viridiplantae evolution and diversification. Results: We generated evidence-based Micromonas gene models using proteomics and RNA-Seq to improve prasinophyte genomic resources. First, sequences of four chromosomes in the 22 Mb Micromonas pusilla (CCMP1545) genome were finished. Comparison with the finished 21 Mb genome of Micromonas commoda (RCC299; named herein) shows they share <= 8,141 of similar to 10,000 protein-encoding genes, depending on the analysis method. Unlike RCC299 and other sequenced eukaryotes, CCMP1545 has two abundant repetitive intron types and a high percent (26 %) GC splice donors. Micromonas has more genus-specific protein families (19 %) than other genome sequenced prasinophytes (11 %). Comparative analyses using predicted proteomes from other prasinophytes reveal proteins likely related to scale formation and ancestral photosynthesis. Our studies also indicate that peptidoglycan (PG) biosynthesis enzymes have been lost in multiple independent events in select prasinophytes and plants. However, CCMP1545, polar Micromonas CCMP2099 and prasinophytes from other classes retain the entire PG pathway, like moss and glaucophyte algae. Surprisingly, multiple vascular plants also have the PG pathway, except the Penicillin-Binding Protein, and share a unique bi-domain protein potentially associated with the pathway. Alongside Micromonas experiments using antibiotics that halt bacterial PG biosynthesis, the findings highlight unrecognized phylogenetic complexity in PG-pathway retention and implicate a role in chloroplast structure or division in several extant Viridiplantae lineages. Conclusions: Extensive differences in gene loss and architecture between related prasinophytes underscore their divergence. PG biosynthesis genes from the cyanobacterial endosymbiont that became the plastid, have been selectively retained in multiple plants and algae, implying a biological function. Our studies provide robust genomic resources for emerging model algae, advancing knowledge of marine phytoplankton and plant evolution. C1 [van Baren, Marijke J.; Bachy, Charles; Reistetter, Emily Nahas; Sudek, Sebastian; Yu, Hang; Poirier, Camille; Worden, Alexandra Z.] Monterey Bay Aquarium Res Inst, 7700 Sandholdt Rd, Moss Landing, CA 95039 USA. [Purvine, Samuel O.; Smith, Richard D.; Callister, Stephen J.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Grimwood, Jane; Kuo, Alan; Grigoriev, Igor V.; Wong, Chee-Hong; Wei, Chia-Lin; Schmutz, Jeremy] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Grimwood, Jane; Schmutz, Jeremy] Hudson Alpha, 601 Genome Way, Huntsville, AL 35806 USA. [Worden, Alexandra Z.] Canadian Inst Adv Res, Integrated Microbial Biodivers Program, Toronto, ON M5G 1Z8, Canada. [Yu, Hang] CALTECH, Ronald & Maxine Linde Ctr Global Environm Sci, Pasadena, CA 91125 USA. [Deerinck, Thomas J.] Univ Calif San Diego, Ctr Res Biol Syst, La Jolla, CA 92093 USA. [Deerinck, Thomas J.] Univ Calif San Diego, Natl Ctr Microscopy & Imaging Res, La Jolla, CA 92093 USA. RP Worden, AZ (reprint author), Monterey Bay Aquarium Res Inst, 7700 Sandholdt Rd, Moss Landing, CA 95039 USA.; Worden, AZ (reprint author), Canadian Inst Adv Res, Integrated Microbial Biodivers Program, Toronto, ON M5G 1Z8, Canada. EM azworden@mbari.org RI Smith, Richard/J-3664-2012 OI Smith, Richard/0000-0002-2381-2349 FU National Institute of General Medical Sciences [GM103412]; DOE by Battelle [DE-AC05-76RLO1830]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; JGI Technology Development Grant; David and Lucile Packard Foundation; Gordon and Betty Moore Foundation [GBMF3788]; NSF [IOS0843119]; [DOE-DE-SC0004765] FX We thank D McRose, S Yan and M Cuvelier for assistance with growing algae. We thank N Turland for guidance on the International Code of Nomenclature (http://www.iapt-taxon.org/nomen/main.php) protocol for species naming and N Simon for proof reading it. We are deeply grateful to V Jimenez for leading manual annotation efforts and J-H Lee, C-J Choi, J Guo, M Gutowska, C Poirier and S Wilken for contributions. We also thank the anonymous reviewers for comments on the manuscript. Electron microscopic imaging was supported by an award from the National Institute of General Medical Sciences (GM103412) to MH Ellisman. Proteomics were performed in the EMSL, a DOE/BER national scientific user facility located at PNNL and operated for the DOE by Battelle under Contract DE-AC05-76RLO1830. Additional support was provided by BER as part of the Pan-omics Program. Portal construction for release of Wlab models was supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 to the U.S. Department of Energy Joint Genome Institute. Major support also came from a JGI Technology Development Grant, the David and Lucile Packard Foundation, the Gordon and Betty Moore Foundation (GBMF3788) and NSF (IOS0843119) grants to AZW. Primary funding was by DOE-DE-SC0004765 (to AZW, SJC and RDS). NR 110 TC 4 Z9 4 U1 8 U2 16 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1471-2164 J9 BMC GENOMICS JI BMC Genomics PD MAR 31 PY 2016 VL 17 AR 267 DI 10.1186/s12864-016-2585-6 PG 22 WC Biotechnology & Applied Microbiology; Genetics & Heredity SC Biotechnology & Applied Microbiology; Genetics & Heredity GA DI5RV UT WOS:000373557900001 PM 27029936 ER PT J AU Head, AR Tsyshevsky, R Trotochaud, L Eichhorn, B Kuklja, MM Bluhm, H AF Head, Ashley R. Tsyshevsky, Roman Trotochaud, Lena Eichhorn, Bryan Kuklja, Maija M. Bluhm, Hendrik TI Electron Spectroscopy and Computational Studies of Dimethyl Methylphosphonate SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID X-RAY PHOTOELECTRON; DENSITY-FUNCTIONAL CALCULATIONS; SELF-ASSEMBLED MONOLAYERS; GAUSSIAN-BASIS SETS; ABSORPTION-SPECTRA; DMMP ADSORPTION; AB-INITIO; ATOMS LI; ENERGY; APPROXIMATION AB Dimethyl methylphosphonate (DMMP) is one of the most widely used molecules to simulate chemical warfare agents in adsorption experiments. However, the details of the electronic structure of the isolated molecule have not yet been reported. We have directly probed the occupied valence and core levels, using gas phase photoelectron spectroscopy and the unoccupied states using near-edge X-ray absorption fine structure (NEXAFS) spectroscopy. Density functional theory (DFT) calculations were used to study the electronic structure, assign the spectral features, and visualize the molecular orbitals. Comparison with parent molecules shows that valence and core-level binding energies of DMMP follow trends of functional group substitution on the P center. The photoelectron and NEXAFS spectra of the isolated molecule will serve as a reference in studies of DMMP adsorbed on surfaces. C1 [Head, Ashley R.; Trotochaud, Lena; Bluhm, Hendrik] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Tsyshevsky, Roman; Kuklja, Maija M.] Univ Maryland, Mat Sci & Engn Dept, College Pk, MD 20742 USA. [Eichhorn, Bryan] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA. RP Bluhm, H (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.; Kuklja, MM (reprint author), Univ Maryland, Mat Sci & Engn Dept, College Pk, MD 20742 USA. EM mkukla@umd.edu; hbluhm@lbl.gov FU Department of Defense [HDTRA11510005]; NSF XSEDE resources [DMR-130077]; DOE NERSC resources [DE-AC02-05CH11231]; Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of the Director of National Science Foundation under the Independent Research and Development program FX This work was funded by the Department of Defense (Grant HDTRA11510005). R.T. and M.M.K. acknowledge support from NSF XSEDE resources (Grant DMR-130077) and DOE NERSC resources (Contract DE-AC02-05CH11231). Osman Karslioglu and Matthias Hard are thanked for their assistance with data collection. M.M.K. is grateful to the Office of the Director of National Science Foundation for support under the Independent Research and Development program. Any appearance of findings, conclusions, or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of NSF. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 42 TC 2 Z9 2 U1 9 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAR 31 PY 2016 VL 120 IS 12 BP 1985 EP 1991 DI 10.1021/acs.jpca.6b01098 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DI3RQ UT WOS:000373416600005 PM 26977778 ER PT J AU Houk, AL Givens, RS Elles, CG AF Houk, Amanda L. Givens, Richard S. Elles, Christopher G. TI Two-Photon Activation of p-Hydroxyphenacyl Phototriggers: Toward Spatially Controlled Release of Diethyl Phosphate and ATP SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID PHOTOREMOVABLE PROTECTING GROUPS; TRANSFORM INFRARED-SPECTROSCOPY; PHOTO-FAVORSKII REARRANGEMENT; SCATTERING CROSS-SECTIONS; WHITE-LIGHT CONTINUUM; EXCITED-STATE; RAMAN-SCATTERING; LIQUID 1-CHLORONAPHTHALENE; TRANSIENT ABSORPTION; CONDENSED MEDIA AB Two-photon activation of the p-hydroxyphenacyl (pHP) photoactivated protecting group is demonstrated for the first time using visible light at 550 nm from a pulsed laser. Broadband two-photon absorption measurements reveal a strong two-photon transition (>10 GM) near 4.5 eV that closely resembles the lowest-energy band at the same total excitation energy in the one-photon absorption spectrum of the pHP chromophore. The polarization dependence of the two-photon absorption band is consistent with excitation to the same S-3 ((1)pi pi*) excited state for both one- and two-photon activation. Monitoring the progress of the uncaging reaction under nonresonant excitation at 550 nm confirms a quadratic intensity dependence and that two-photon activation of the uncaging reaction is possible using visible light in the range 500-620 nm. Deprotonation of the pHP chromophore under mildly basic conditions shifts the absorption band to lower energy (3.8 eV) in both the one- and two-photon absorption spectra, suggesting that two-photon activation of the pHP chromophore may be possible using light in the range 550-720 nm. The results of these measurements open the possibility of spatially and temporally selective release of biologically active compounds from the pHP protecting group using visible light from a pulsed laser. C1 [Houk, Amanda L.; Givens, Richard S.; Elles, Christopher G.] Univ Kansas, Dept Chem, Lawrence, KS 66045 USA. [Houk, Amanda L.] Savannah River Natl Lab, Aiken, SC 29808 USA. RP Givens, RS; Elles, CG (reprint author), Univ Kansas, Dept Chem, Lawrence, KS 66045 USA. EM givensr@ku.edu; elles@ku.edu RI Houk, Amanda/M-1760-2013 OI Houk, Amanda/0000-0002-5099-2285 FU National Science Foundation [CHE-1151555] FX This work was supported by the National Science Foundation through Career Award CHE-1151555. The authors are grateful to Dr. Sanjeewa Senadheera (Dept. of Pharmaceutical Chemistry, KU) and Dr. Sabine Amslinger (currently at Institute of Org. Chem., Regensburg Univ.) for synthesizing the compounds used in this study. NR 65 TC 1 Z9 1 U1 13 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 31 PY 2016 VL 120 IS 12 BP 3178 EP 3186 DI 10.1021/acs.jpcb.5b12150 PG 9 WC Chemistry, Physical SC Chemistry GA DI3RR UT WOS:000373416700019 PM 26962676 ER PT J AU Mamontov, E Sharma, VK Borreguero, JM Tyagi, M AF Mamontov, E. Sharma, V. K. Borreguero, J. M. Tyagi, M. TI Protein-Style Dynamical Transition in a Non-Biological Polymer and a Non-Aqueous Solvent SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID ELASTIC NEUTRON-SCATTERING; AMORPHOUS POLYSTYRENE; HYDRATION WATER; FLUCTUATIONS; MOTIONS AB Temperature-dependent onset of apparent anharmonicity in the microscopic dynamics of hydrated proteins and other biomolecules has been known as protein dynamical transition for the last quarter of a century. Using neutron scattering and molecular dynamics simulation, techniques most often associated with protein dynamical transition studies, we have investigated the microscopic dynamics of one of the most common polymers, polystyrene, which was exposed to toluene vapor, mimicking the process of protein hydration from water vapor. Polystyrene with adsorbed toluene is an example of a solvent-solute system, which, unlike biopolymers, is anhydrous and lacks hydrogen bonding. Nevertheless, it exhibits the essential traits of the dynamical transition in biomolecules, such as a specific dependence of the microscopic dynamics of both solvent and host on the temperature and the amount of solvent adsorbed. We conclude that the protein dynamical transition is a manifestation of a universal solvent-solute dynamical relationship, which is not specific to either biomolecules as solute, or aqueous media as solvent, or even a particular type of interactions between solvent and solute. C1 [Mamontov, E.] Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Sharma, V. K.] Oak Ridge Natl Lab, Neutron Sci Directorate, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Sharma, V. K.] Bhabha Atom Res Ctr, Div Solid State Phys, Bombay 400085, Maharashtra, India. [Borreguero, J. M.] Oak Ridge Natl Lab, Neutron Sci Directorate, Neutron Data Anal & Visualizat Div, Oak Ridge, TN 37831 USA. [Tyagi, M.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Tyagi, M.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. RP Mamontov, E (reprint author), Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. EM mamontove@ornl.gov RI Mamontov, Eugene/Q-1003-2015 OI Mamontov, Eugene/0000-0002-5684-2675 FU National Science Foundation [DMR-1508249]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Center for Accelerating Materials Modeling (CAMM) - U.S. Department of Energy, Basic Energy Sciences, Material Sciences and Engineering Division [FWP-3ERKCSNL]; U.S. Department of Energy [DE-AC05-00OR22725] FX The neutron scattering experiments on HFBS at NCNR were supported in part by the National Science Foundation under Agreement No. DMR-1508249. The neutron scattering experiments on BASIS at SNS were supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. J.M.B. is supported by the Center for Accelerating Materials Modeling (CAMM) funded by the U.S. Department of Energy, Basic Energy Sciences, Material Sciences and Engineering Division under FWP-3ERKCSNL. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). Certain commercial material suppliers are identified in this paper to foster understanding. Such identification does not imply recommendation or endorsement by the National Institute of Standards and Technology, nor does it imply that the materials or equipment identified are necessarily the best available for the purpose. The authors declare no competing financial interests. NR 36 TC 3 Z9 3 U1 0 U2 4 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 31 PY 2016 VL 120 IS 12 BP 3232 EP 3239 DI 10.1021/acs.jpcb.6b00866 PG 8 WC Chemistry, Physical SC Chemistry GA DI3RR UT WOS:000373416700025 PM 26977709 ER PT J AU Leung, K Soto, F Hankins, K Balbuena, PB Harrison, KL AF Leung, Kevin Soto, Fernando Hankins, Kie Balbuena, Perla B. Harrison, Katharine L. TI Stability of Solid Electrolyte Interphase Components on Lithium Metal and Reactive Anode Material Surfaces SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LI-ION BATTERIES; 1ST PRINCIPLES; PHOTOELECTRON-SPECTROSCOPY; FLUOROETHYLENE CARBONATE; MOLECULAR-DYNAMICS; SEI FORMATION; ELECTROCHEMICAL PERFORMANCE; 1ST-PRINCIPLES CALCULATIONS; RECHARGEABLE BATTERIES; SECONDARY BATTERIES AB Lithium ion batteries (LIB) can feature reactive anodes that operate at low potentials, such as lithium metal or silicon, passivated by solid electrolyte interphase (SEI) films. SEI is known to evolve over time as cycling proceeds. In this modeling work, we focus on the stability of two main SEI components, lithium carbonate (Li2CO3) and lithium ethylene dicarbonate (LEDC). Both components are electrochemically stable but thermodynamically unstable near the equilibrium Li-4/Li(s) potential. Interfacial reactions represent one way to trigger the intrinsic thermodynamic instability. Both Li2CO3 and LEDC are predicted to exhibit exothermic reactions on lithium metal surfaces, and the barriers are sufficiently low to permit reactions on battery operation time scales. LEDC also readily decomposes on high Li-content LixSi surfaces. Our studies suggest that the innermost SEI layer on lithium metal surfaces should be a thin layer of Li2O, the only thermodynamically and kinetically stable component (in the absence of a fluoride source). This work should also be relevant to inadvertent lithium plating during battery cycling and SEI evolution on LixSi surfaces. C1 [Leung, Kevin; Harrison, Katharine L.] Sandia Natl Labs, MS 1415, Albuquerque, NM 87185 USA. [Soto, Fernando; Hankins, Kie; Balbuena, Perla B.] Texas A&M Univ, Dept Chem Engn, College Stn, TX 77843 USA. RP Leung, K (reprint author), Sandia Natl Labs, MS 1415, Albuquerque, NM 87185 USA. EM kleung@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy [DE-AC02-05CH11231, 7060634] FX We thank Oleg Borodin, Byron Konstantinos Antonopoulos, Wentao Song, and Janice Reutt-Robey for discussions and input. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This work was supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, Subcontract No. 7060634 under the Advanced Batteries Materials Research (BMR) Program. NR 97 TC 8 Z9 8 U1 44 U2 122 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 31 PY 2016 VL 120 IS 12 BP 6302 EP 6313 DI 10.1021/acs.jpcc.5b11719 PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DI3RP UT WOS:000373416500002 ER PT J AU Sachsenhauser, M Sharp, ID Stutzmann, M Garrido, JA AF Sachsenhauser, Matthias Sharp, Ian D. Stutzmann, Martin Garrido, Jose A. TI Surface State Mediated Electron Transfer Across the N-Type SiC/Electrolyte Interface SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SEMICONDUCTOR ELECTRODES; SILICON-CARBIDE; PHOTOELECTROCHEMICAL CHARACTERIZATION; ELECTROCHEMICAL PROPERTIES; GAAS ELECTRODES; CHARGE-TRANSFER; IMPEDANCE; HYDROGEN; WATER; PHOSPHIDE AB Understanding the mechanisms of charge transfer across the semiconductor/electrolyte interface is a basic prerequisite for a variety of practical applications. In particular, electrically active surface states located in the semiconductor band gap are expected to play an important role, but direct experimental evidence of surface states has proven to be challenging, and further experimental studies are required to verify their influence on the exchange of charge carriers between semiconductor and electrolyte. Due to its wide band gap, chemical stability, and controllable surface termination, silicon carbide (SiC) provides an excellent model system for this purpose. In this report, we provide a fundamental electrochemical study of n-type 6H-SiC and 4H-SiC electrodes in aqueous electrolytes containing the ferricyanide/ferrocyanide redox couple. Cyclic voltammetry and impedance spectroscopy measurements are performed over a wide range of potentials to determine the energetic positions of the SiC band edges and to investigate the electron-transfer kinetics between SiC and the ferricyanide molecules. For both polytypes, a broad distribution of surface states with energy levels close to the conduction band is found to mediate electron transfer, resulting in deviations of the observed charge transport characteristics from the predictions of well-established models. Moreover, a detailed evaluation of the impedance data allows for explicit correlation of the charge transfer resistance associated with the ferricyanide reduction reaction with the potential-dependent distribution of surface states. In addition to the relevance of our studies for advancing the implementation of SiC in biosensing, electrocatalytic, and photocatalytic applications, the presented methodology can also be adopted for fundamental electrochemical investigations of other semiconductor electrodes. C1 [Sachsenhauser, Matthias; Stutzmann, Martin] Tech Univ Munich, Walter Schottky Inst, Coulombwall 4, D-85748 Garching, Germany. [Sachsenhauser, Matthias; Stutzmann, Martin] Tech Univ Munich, Dept Phys, Coulombwall 4, D-85748 Garching, Germany. [Sharp, Ian D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynthesis, Berkeley, CA 94720 USA. [Sharp, Ian D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Garrido, Jose A.] CSIC, Catalan Inst Nanosci & Nanotechnol ICN2, Campus UAB, Barcelona 08193, Spain. [Garrido, Jose A.] Barcelona Inst Sci & Technol, Campus UAB, Barcelona 08193, Spain. [Garrido, Jose A.] ICREA, Barcelona 08070, Spain. RP Garrido, JA (reprint author), CSIC, Catalan Inst Nanosci & Nanotechnol ICN2, Campus UAB, Barcelona 08193, Spain.; Garrido, JA (reprint author), Barcelona Inst Sci & Technol, Campus UAB, Barcelona 08193, Spain.; Garrido, JA (reprint author), ICREA, Barcelona 08070, Spain. EM joseantonio.garrido@icn.cat RI Garrido, Jose A./K-7491-2015; Stutzmann, Martin/B-1480-2012 OI Garrido, Jose A./0000-0001-5621-1067; FU IGSSE; Technische Universitat Munchen-Institute for Advanced Study - German Excellence Initiative; Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub through Office of Science of the U.S. Department of Energy [DE-SC0004993] FX M.S. acknowledges support of the IGSSE and of the Technische Universitat Munchen-Institute for Advanced Study, funded by the German Excellence Initiative. I.D.S. was supported by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under award no. DE-SC0004993. NR 42 TC 2 Z9 2 U1 15 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 31 PY 2016 VL 120 IS 12 BP 6524 EP 6533 DI 10.1021/acs.jpcc.5b11569 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DI3RP UT WOS:000373416500027 ER PT J AU Yuan, FL Liu, B Zhang, YW Weber, WJ AF Yuan, Fenglin Liu, Bin Zhang, Yanwen Weber, William J. TI Segregation and Migration of the Oxygen Vacancies in the Sigma 3 (111) Tilt Grain Boundaries of Ceria SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; GAS-SHIFT REACTION; OXIDE FUEL-CELLS; CEO2 NANOPARTICLES; DOPED CERIA; THIN-FILMS; BASIS-SET; SIZE AB In nanocrystalline materials, defect grain boundary (GB) interactions play a key role in determining structural stability, as well as size-dependent ionic, electronic, magnetic, and chemical properties. In this study, using density functional theory, we systematically investigated the segregation and migration of oxygen vacancies at the Sigma 3 [1 (1) over bar0]/(111) grain boundary of ceria. Three oxygen layers near the GB are predicted to be segregation sites for oxygen vacancies. Moreover, the presence of oxygen vacancies stabilizes this tilt GB at a low Fermi level and/or under oxygen-poor conditions. An atomic strain model is proposed to rationalize the layer dependency of the relaxation energy for a 2+-charged oxygen vacancy. The structural origin of the large relaxation energies at layers 1 and 2 was determined to be free-volume space, which induces ion relaxation toward the GB. Our results not only pave the way for improving oxygen transport near GBs in ceria, but also provide important insights into the engineering of the GB structure of nanocrystalline ceria for better ionic, magnetic, and chemical properties. C1 [Yuan, Fenglin; Liu, Bin; Zhang, Yanwen; Weber, William J.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Zhang, Yanwen; Weber, William J.] Oak Ridge Natl Lab, Div Mat Sci & Technol, POB 2008, Oak Ridge, TN 37831 USA. RP Yuan, FL; Weber, WJ (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA.; Weber, WJ (reprint author), Oak Ridge Natl Lab, Div Mat Sci & Technol, POB 2008, Oak Ridge, TN 37831 USA. EM fyuan5@utk.edu; wjweber@utk.edu RI Weber, William/A-4177-2008; Liu, Bin/N-9955-2014 OI Weber, William/0000-0002-9017-7365; FU DOE Office of Nuclear Energy's Nuclear Energy University Programs FX This research was supported by the DOE Office of Nuclear Energy's Nuclear Energy University Programs. The simulations were performed at the National Energy Research Scientific Computing Center (NERSC). NR 64 TC 0 Z9 0 U1 4 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 31 PY 2016 VL 120 IS 12 BP 6625 EP 6632 DI 10.1021/acs.jpcc.6b00325 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DI3RP UT WOS:000373416500038 ER PT J AU Cherukara, MJ Germann, TC Kober, EM Strachan, A AF Cherukara, Mathew J. Germann, Timothy C. Kober, Edward M. Strachan, Alejandro TI Shock Loading of Granular Ni/Al Composites. Part 2: Shock-Induced Chemistry SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID MOLECULAR-DYNAMICS; SIMULATIONS; MODEL AB We use molecular dynamics simulations to characterize the chemical processes resulting from the shock compaction of a loosely packed granular reactive composite of Ni and Al. For all of the impact strengths studied (with piston velocities up in the range 0.5-2.5 km/s), we find that reactions initiate in the vicinity of the collapsed pores. For the lowest impact velocities (u(p) <= 0.75 km/s), the reactions that initiate at the collapsed pores subsequently slow down as thermal transport dissipates the initial temperature excursion and outpaces the exothermic energy release rate. At intermediate impact velocities (u(p) approximate to 1.0 km/s), the localization of thermal kinetic energy is sufficient to establish a reaction rate that is self-sustaining in exothermic energy release, and the sample reacts within a few nanoseconds. At the highest impact velocities (u(p) >= 1.5 km/s), the localization of translational kinetic energy as well as thermal energy following pore collapse drives the rapid propagation of the reaction from the collapsed pores. C1 [Cherukara, Mathew J.; Strachan, Alejandro] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Cherukara, Mathew J.; Strachan, Alejandro] Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. [Cherukara, Mathew J.; Germann, Timothy C.; Kober, Edward M.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Cherukara, Mathew J.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Strachan, A (reprint author), Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA.; Strachan, A (reprint author), Purdue Univ, Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. EM strachan@purdue.edu OI Germann, Timothy/0000-0002-6813-238X FU U.S. Defense Threat Reduction Agency [HDTRA1-10-1-0119]; U.S. Department of Energy National Nuclear Security Administration [DE-AC52-06NA25396]; Institute for Materials Science (LANL); ExMatEx project; Argonne [LDRD 2015-149-R1] FX This work was supported by the U.S. Defense Threat Reduction Agency, HDTRA1-10-1-0119 (Program Manager Suhithi Peiris) and used resources provided by the Los Alamos National Laboratory Institutional Computing Program, which is supported by the U.S. Department of Energy National Nuclear Security Administration under Contract No. DE-AC52-06NA25396. E.M.K acknowledges support from the Institute for Materials Science (LANL) and T.C.G. acknowledges support from the ExMatEx project. M.J.C. also acknowledges support from Argonne LDRD 2015-149-R1 (Integrated Imaging, Modeling, and Analysis of Ultrafast Energy Transport in Nanomaterials) while preparing the manuscript. We also wish thank the reviewers for several helpful suggestions with regards to the preparation of this manuscript. NR 38 TC 1 Z9 1 U1 5 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 31 PY 2016 VL 120 IS 12 BP 6804 EP 6813 DI 10.1021/acs.jpcc.5b11528 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DI3RP UT WOS:000373416500059 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahn, SU Aimo, I Aiola, S Ajaz, M Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Almaraz, JRM Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Armesto, N Arnaldi, R Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Bach, M Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Baldisseri, A Pedrosa, FBD Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F Martinez, HB Bellwied, R Belmont, R Belmont-Moreno, E Belyaev, V Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bertens, RA Berzano, D Betev, L Bhasin, A Bhat, IR Bhati, AK Bhattacharjee, B Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Biswas, R Biswas, S Bjelogrlic, S Blair, JT Blanco, F Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Borri, M Bossu, F Botta, E Bottger, S Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brucken, EJ Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Butt, JB Buxton, JT Caffarri, D Cai, X Caines, H Diaz, LC Caliva, A Villar, EC Camerini, P Carena, F Carena, W Carnesecchi, F Castellanos, JC Castro, AJ Casula, EAR Cavicchioli, C Sanchez, CC Cepila, J Cerello, P Cerkala, J Chang, B Chapeland, S Chartier, M Charvet, JL Chattopadhyay, S Chattopadhyay, S Chelnokov, V Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Chochula, P Choi, K Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Chunhui, Z Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Colocci, M Balbastre, GC del Valle, ZC Connors, ME Contreras, JG Cormier, TM Morales, YC Maldonado, IC Cortese, P Cosentino, MR Costa, F Crochet, P Albino, RC Cuautle, E Cunqueiro, L Dahms, T Dainese, A Danu, A Das, D Das, I Das, S Dash, A Dash, S De, S De Caro, A de Cataldo, G de Cuveland, J De Falco, A De Gruttola, D De Marco, N De Pasquale, S Deisting, A Deloff, A Denes, E D'Erasmo, G Di Bari, D Di Mauro, A Di Nezza, P Corchero, MAD Dietel, T Dillenseger, P Divia, R Djuvsland, O Dobrin, A Dobrowolski, T Gimenez, DD Donigus, B Dordic, O Drozhzhova, T Dubey, AK Dubla, A Ducroux, L Dupieux, P Ehlers, RJ Elia, D Engel, H Erazmus, B Erdemir, I Erhardt, F Eschweiler, D Espagnon, B Estienne, M Esumi, S Eum, J Evans, D Evdokimov, S Eyyubova, G Fabbietti, L Fabris, D Faivre, J Fantoni, A Fasel, M Feldkamp, L Felea, D Feliciello, A Feofilov, G Ferencei, J Tellez, AF Ferreiro, EG Ferretti, A Festanti, A Feuillard, VJG Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Fleck, MG Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fuchs, U Furget, C Furs, A Girard, MF Gaardhoje, JJ Gagliardi, M Gago, AM Gallio, M Gangadharan, DR Ganoti, P Gao, C Garabatos, C Garcia-Solis, E Gargiulo, C Gasik, P Germain, M Gheata, A Gheata, M Ghosh, P Ghosh, SK Gianotti, P Giubellino, P Giubilato, P Gladysz-Dziadus, E Glassel, P Coral, DMG Ramirez, AG Gonzalez-Zamora, P Gorbunov, S Gorlich, L Gotovac, S Grabski, V Graczykowski, LK Graham, KL Grelli, A Grigoras, A Grigoras, C Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Grosse-Oetringhaus, JF Grossiord, JY Grosso, R 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CA ALICE Collaboration TI Event-shape engineering for inclusive spectra and elliptic flow in Pb-Pb collisions at root(NN)-N-S=2.76 TeV SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION COLLISIONS; ROOT-S(NN)=5.02 TEV; NUCLEAR COLLISIONS; DEPENDENCE; HADRONS; PARTON AB We report on results obtained with the event-shape engineering technique applied to Pb-Pb collisions at root s(NN) = 2.76 TeV. By selecting events in the same centrality interval, but with very different average flow, different initial-state conditions can be studied. We find the effect of the event-shape selection on the elliptic flow coefficient v(2) to be almost independent of transverse momentum p(T), which is as expected if this effect is attributable to fluctuations in the initial geometry of the system. Charged-hadron, -pion, -kaon, and -proton transverse momentum distributions are found to be harder in events with higher-than-average elliptic flow, indicating an interplay between radial and elliptic flow. 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J.; Ullaland, K.; Velure, A.; Wagner, B.; Zhang, H.; Zhou, Z.; Zhu, H.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Azmi, M. D.; Hussain, T.; Irfan, M.; Khan, M. Mohisin; Tariq, M.] Aligarh Muslim Univ, Dept Phys, Aligarh 202002, Uttar Pradesh, India. [Buxton, J. T.; Humanic, T. J.; Kubera, A. M.; Lisa, M. A.; Salzwedel, J.; Steinpreis, M.] Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. [Hwang, D. S.; Kim, S.] Sejong Univ, Dept Phys, Seoul, South Korea. [Arsene, I. C.; Batzing, P. C.; Dordic, O.; Lindal, S.; Mahmood, S. M.; Milosevic, J.; Qvigstad, H.; Richter, M.; Roed, K.; Skaali, T. B.; Tveter, T. S.; Wikne, J.; Zhao, C.] Univ Oslo, Dept Phys, Oslo, Norway. [Minervini, L. M.] Politecn Bari, Dipartimento Elettrotecn & Elettron, Bari, Italy. [Meddi, F.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Meddi, F.] Sezione Ist Nazl Fis Nucl, Rome, Italy. [Casula, E. A. R.; Collu, A.; De Falco, A.; Fionda, F. M.; Puddu, G.; Terrevoli, C.; Usai, G. L.] Univ Cagliari, Dipartimento Fis, Cagliari, Italy. [Casula, E. A. R.; Collu, A.; De Falco, A.; Fionda, F. M.; Puddu, G.; Terrevoli, C.; Usai, G. L.] Sezione Ist Nazl Fis Nucl, Cagliari, Italy. [Camerini, P.; Lea, R.; Luparello, G.; Margagliotti, G. V.; Rui, R.] Univ Trieste, Dipartimento Fis, Trieste, Italy. [Camerini, P.; Lea, R.; Luparello, G.; Margagliotti, G. V.; Rui, R.] Sezione Ist Nazl Fis Nucl, Trieste, Italy. [Beole, S.; Berzano, D.; Botta, E.; Bufalino, S.; Corrales Morales, Y.; Ferretti, A.; Gagliardi, M.; Gallio, M.; Lattuca, A.; Leoncino, M.; Marchisone, M.; Masera, M.; Russo, R.; Shtejer, K.; Vallero, S.; Vercellin, E.] Univ Turin, Dipartimento Fis, Turin, Italy. [Beole, S.; Berzano, D.; Botta, E.; Bufalino, S.; Corrales Morales, Y.; Ferretti, A.; Gagliardi, M.; Gallio, M.; Lattuca, A.; Leoncino, M.; Marchisone, M.; Masera, M.; Russo, R.; Shtejer, K.; Vallero, S.; Vercellin, E.] Sezione Ist Nazl Fis Nucl, Turin, Italy. [Arcelli, S.; Basile, M.; Bellini, F.; Carnesecchi, F.; Cifarelli, L.; Colocci, M.; Guerzoni, B.; Scioli, G.; Zichichi, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arcelli, S.; Basile, M.; Bellini, F.; Carnesecchi, F.; Cifarelli, L.; Colocci, M.; Guerzoni, B.; Scioli, G.; Zichichi, A.] Sezione Ist Nazl Fis Nucl, Bologna, Italy. [Barbera, R.; La Rocca, P.; Petta, C.; Riggi, F.] Univ Catania, Dipartimento Fis & Astron, Catania, Italy. [Barbera, R.; La Rocca, P.; Petta, C.; Riggi, F.] Sezione Ist Nazl Fis Nucl, Catania, Italy. [Festanti, A.; Francescon, A.; Giubilato, P.; Jena, C.; Lunardon, M.; Morando, M.; Moretto, S.; Rossi, A.; Scarlassara, F.; Soramel, F.; Terrevoli, C.; Viesti, G.] Univ Padua, Dipartimento Fis & Astron, Padua, Italy. [Festanti, A.; Francescon, A.; Giubilato, P.; Jena, C.; Lunardon, M.; Morando, M.; Moretto, S.; Rossi, A.; Scarlassara, F.; Soramel, F.; Terrevoli, C.; Viesti, G.] Sezione Ist Nazl Fis Nucl, Padua, Italy. [De Caro, A.; De Gruttola, D.; De Pasquale, S.; Fusco Girard, M.; Meninno, E.; Pagano, P.; Virgili, T.] Univ Salerno, Dipartimento Fis ER Caianiello, I-84100 Salerno, Italy. [De Caro, A.; De Gruttola, D.; De Pasquale, S.; Fusco Girard, M.; Meninno, E.; Pagano, P.; Virgili, T.] Grp Collegato INFN, Salerno, Italy. [Cortese, P.; Ramello, L.; Sitta, M.] Univ Piemonte Orientale, Dipartimento Sci & Innovaz Tecnol, Alessandria, Italy. [Cortese, P.; Ramello, L.; Sitta, M.] Grp Collegato INFN, Alessandria, Italy. [Barile, F.; Bruno, G. E.; Colamaria, F.; Colella, D.; D'Erasmo, G.; Di Bari, D.; Fiore, E. M.; Mastroserio, A.; Tangaro, M. A.] Dipartimento Interateneo Fis M Merlin, Bari, Italy. [Barile, F.; Bruno, G. E.; Colamaria, F.; Colella, D.; D'Erasmo, G.; Di Bari, D.; Fiore, E. M.; Mastroserio, A.; Tangaro, M. A.] Sezione Ist Nazl Fis Nucl, Bari, Italy. [Christiansen, P.; Ljunggren, H. M.; Oskarsson, A.; Richert, T.; Silvermyr, D.; Sogaard, C.; Stenlund, E.; Vislavicius, V.] Lund Univ, Div Expt High Energy Phys, Lund, Sweden. [Hess, B. A.; Schmidt, H. R.; Wiechula, J.] Univ Tubingen, Tubingen, Germany. [Rinella, G. Aglieri; Augustinus, A.; Baltasar Dos Santos Pedrosa, F.; Barth, K.; Berzano, D.; Betev, L.; Buncic, P.; Caffarri, D.; Carena, F.; Carena, W.; Cavicchioli, C.; Chapeland, S.; Chibante Barroso, V.; Chochula, P.; Colella, D.; Costa, F.; Cunqueiro, L.; Di Mauro, A.; Divia, R.; Erazmus, B.; Floris, M.; Francescon, A.; Fuchs, U.; Gargiulo, C.; Gheata, A.; Gheata, M.; Giubellino, P.; Grigoras, A.; Grigoras, C.; Grosse-Oetringhaus, J. F.; Grosso, R.; Hillemanns, H.; Hristov, P.; Kalweit, A.; Keil, M.; Klein, J.; Kluge, A.; Kofarago, M.; Kouzinopoulos, C.; Kryshen, E.; Kugathasan, T.; Lakomov, I.; Laudi, E.; Legrand, I.; Mager, M.; Manzari, V.; Martinengo, P.; Martinez Pedreira, M.; Milano, L.; Morsch, A.; Musa, L.; Niculescu, M.; Niedziela, J.; Ohlson, A.; Pinazza, O.; Preghenella, R.; Reidt, F.; Riedler, P.; Riegler, W.; Rossi, A.; Sararik, K.; Schukraft, J.; Schutz, Y.; Shahoyan, R.; Sielewicz, K. M.; Simonetti, G.; Szczepankiewicz, A.; Tauro, A.; Telesca, A.; Van Hoorne, J. W.; Vande Vyvre, P.; Verweij, M.; Volpe, G.; von Haller, B.; Vranic, D.; Weber, M.; Zimmermann, M. B.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Dahms, T.; Fabbietti, L.; Gasik, P.; Vorobyev, I.] Tech Univ Munich, Excellence Cluster Universe, D-80290 Munich, Germany. [Alme, J.; Helstrup, H.; Hetland, K. F.; Kileng, B.] Bergen Univ Coll, Fac Engn, Bergen, Norway. [Meres, M.; Pikna, M.; Sitar, B.; Strmen, P.; Szabo, A.; Szarka, I.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Adam, J.; Bielcik, J.; Broz, M.; Cepila, J.; Contreras, J. G.; Eyyubova, G.; Petracek, V.; Schulc, M.; Spacek, M.] Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic. [Bombara, M.; Kravcakova, A.; Vrlakova, J.] Safarik Univ, Fac Sci, Kosice, Slovakia. [Langoy, R.; Lien, J.] Buskerud & Vestfold Univ Coll, Fac Technol, Vestfold, Norway. [Alt, T.; Bach, M.; de Cuveland, J.; Eschweiler, D.; Gorbunov, S.; Hartmann, H.; Hutter, D.; Kirsch, S.; Kisel, I.; Kollegger, T.; Kretz, M.; Krzewicki, M.; Lindenstruth, V.; Rettig, F.; Rohr, D.; Zyzak, M.] Goethe Univ Frankfurt, Frankfurt Inst Adv Studies, D-60054 Frankfurt, Germany. [Baek, Y. W.; Jung, H.; Kim, D. W.; Kim, J. S.; Kim, M.] Gangneung Wonju Natl Univ, Kangnung, South Korea. [Bhattacharjee, B.; Hussain, N.] Gauhati Univ, Dept Phys, Gauhati, India. [Brucken, E. J.; Hilden, T. E.; Mieskolainen, M. M.; Orava, R.; Rasanen, S. S.] HIP, Helsinki, Finland. [Okubo, T.; Sekihata, D.; Shigaki, K.; Sugitate, T.; Yano, S.] Hiroshima Univ, Hiroshima, Japan. [Agrawal, N.; Behera, N. K.; Dash, S.; Meethaleveedu, G. Koyithatta; Kumar, J.; Nandi, B. K.; Pandey, A. K.; Pant, D.; Varma, R.] Indian Inst Technol, Mumbai, Maharashtra, India. [Behera, N. K.; Mishra, A. N.; Pareek, P.; Roy, A.; Sahoo, P.; Sahoo, R.] Indian Inst Technol Indore, Indore, India. [Kweon, M. J.] Inha Univ, Inchon, South Korea. [Conesa del Valle, Z.; Das, I.; Espagnon, B.; Hadjidakis, C.; Suire, C.; Takaki, J. D. Tapia; Tarhini, M.] Univ Paris 11, CNRS, IN2P3, IPNO, F-91405 Orsay, France. [Boettger, S.; Breitner, T.; Engel, H.; Gomez Ramirez, A.; Kebschull, U.; Lara, C.] Goethe Univ Frankfurt, Inst Informat, D-60054 Frankfurt, Germany. [Appelshaeuser, H.; Arslandok, M.; Bailhache, R.; Bartsch, E.; Beck, H.; Blume, C.; Book, J.; Broker, T. A.; Buesching, H.; Dillenseger, P.; Doenigus, B.; Drozhzhova, T.; Erdemir, I.; Heckel, S. T.; Kamin, J.; Klein, C.; Luettig, P.; Marquard, M.; Ozdemir, M.; Perez Lezama, E.; Peskov, V.; Rascanu, B. T.; Reichelt, P.; Renfordt, R.; Sahlmuller, B.; Schuchmann, S.; Peloni, A. Tarantola; Toia, A.] Goethe Univ Frankfurt, Inst Kernphys, Frankfurt, Germany. [Anielski, J.; Bathen, B.; Feldkamp, L.; Haake, R.; Heide, M.; Klein-Boesing, C.; De Godoy, D. A. Moreira; Muehlheim, D.; Passfeld, A.; Wessels, J. P.; Westerhoff, U.; Wilde, M.; Zimmermann, M. B.] Univ Munster, Inst Kernphys, Wilhelm Klemm Str 9, D-48149 Munster, Germany. [Belikov, I.; Hippolyte, B.; Kuhn, C.; Maire, A.; Molnar, L.; Rami, F.; Roy, C.; Castro, X. Sanchez] Univ Strasbourg, CNRS, IN2P3, IPHC, Strasbourg, France. [Finogeev, D.; Furs, A.; Guber, F.; Karavichev, O.; Karavicheva, T.; Karpechev, E.; Konevskikh, A.; Kurepin, A.; Kurepin, A. B.; Maevskaya, A.; Pshenichnov, I.; Reshetin, A.; Shabanov, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Bertens, R. A.; Bianchin, C.; Bjelogrlic, S.; Caliva, A.; Chunhui, Z.; Dobrin, A.; Dubla, A.; Grelli, A.; Keijdener, D. L. D.; Leogrande, E.; Lodato, D. F.; Margutti, J.; Mischke, A.; Mohammadi, N.; Nooren, G.; Peitzmann, T.; Rocco, E.; Snellings, R. J. M.; Van der Maarel, J.; van Leeuwen, M.; Veen, A. M.; Veldhoen, M.; Wang, H.; Yang, H.; Zhou, Y.] Univ Utrecht, Inst Subat Phys, Utrecht, Netherlands. [Akindinov, A.; Kiselev, S.; Mal'Kevich, D.; Mikhaylov, K.; Nedosekin, A.; Sultanov, R.; Voloshin, K.; Zhigareva, N.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Colella, D.; Kalinak, P.; Kralik, I.; Krivda, M.; Musinsky, J.; Sandor, L.; Vala, M.] Slovak Acad Sci, Inst Expt Phys, Kosice 04353, Slovakia. [Mares, J.; Zavada, P.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Baral, R. C.; Sahoo, S.; Sahu, P. K.; Sharma, N.] Inst Phys, Bhubaneswar 751007, Orissa, India. [Danu, A.; Felea, D.; Gheata, M.; Haiduc, M.; Mitu, C. M.; Niculescu, M.; Ristea, C.; Sevcenco, A.; Stan, I.; Zgura, I. S.] ISS, Bucharest, Romania. [Cuautle, E.; Maldonado Cervantes, I.; Nellen, L.; Ortiz Velasquez, A.; Paic, G.] Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City 04510, DF, Mexico. [Molina, R. Alfaro; Belmont-Moreno, E.; Gomez Coral, D. M.; Grabski, V.; Menchaca-Rocha, A.; Sandoval, A.; Serradilla, E.] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City, DF, Mexico. [Bossu, F.; Buthelezi, Z.; Foertsch, S.; Murray, S.; Senosi, K.; Steyn, G.] Natl Res Fdn, iThemba LABS, Somerset West, South Africa. [Batyunya, B.; Grigoryan, S.; Malinina, L.; Mikhaylov, K.; Nomokonov, P.; Rogochaya, E.; Vodopyanov, A.; Zaporozhets, S.] Joint Inst Nucl Res, Dubna, Russia. [Oh, S. K.; Seo, J.] Konkuk Univ, Seoul, South Korea. [Ahn, S. U.; Jang, H. J.; Kim, D. W.] Korea Inst Sci & Technol Informat, Daejeon, South Korea. [Uysal, A. Karasu; Okatan, A.] KTO Karatay Univ, Konya, Turkey. [Barret, V.; Bastid, N.; Camejo, A. Batista; Crochet, P.; Dupieux, P.; Feuillard, V. J. G.; Li, S.; Lopez, X.; Manso, F.; Porteboeuf-Houssais, S.; Rosnet, P.; Palomo, L. Valencia; Vulpescu, B.] Univ Clermont Ferrand, Clermont Univ, LPC, CNRS,IN2P3, Clermont Ferrand, France. [Conesa Balbastre, G.; Faivre, J.; Furget, C.; Guernane, R.; Real, J. S.; Silvestre, C.; Vauthier, A.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [Bianchi, N.; Calero Diaz, L.; Di Nezza, P.; Fantoni, A.; Gianotti, P.; Muccifora, V.; Reolon, A. R.; Ronchetti, F.; Sakai, S.; Spiriti, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Ricci, R. A.; Venaruzzo, M.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Bock, F.; Fasel, M.; Gangadharan, D. R.; Jacobs, P. M.; Loizides, C.; Ploskon, M.; Porter, J.; Symons, T. J. 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S.; Zaccolo, V.; Zhou, Y.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Christakoglou, P.; Dobrin, A.; Kuijer, P. G.; Lehas, F.; Perez Lara, C. E.; Rodriguez Manso, A.] Natl Inst Subatomaire Fys, Nikhef, Amsterdam, Netherlands. [Borri, M.; Lemmon, R. C.] STFC Daresbury Lab, Nucl Phys Grp, Daresbury, England. [Adamova, D.; Bielcikova, J.; Ferencei, J.; Krizek, F.; Kucera, V.; Kushpil, S.; Pospisil, J.; Sumbera, M.; Vajzer, M.; Vanat, T.] Acad Sci Czech Republic, Inst Nucl Phys, CZ-25068 Rez, Czech Republic. [Cormier, T. M.; Poghosyan, M. G.; Silvermyr, D.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Berdnikov, Y.; Ivanov, V.; Khanzadeev, A.; Malaev, M.; Nikulin, V.; Riabov, V.; Ryabov, Y.; Samsonov, V.; Zhalov, M.] Petersburg Nucl Phys Inst, Gatchina, Russia. [Cherney, M.; Poghosyan, M. G.; Seger, J. E.] Creighton Univ, Dept Phys, Omaha, NE 68178 USA. [Aggarwal, M. M.; Bhati, A. K.; Kumar, L.; Parmar, S.; Rathee, D.] Panjab Univ, Dept Phys, Chandigarh 160014, India. [Ganoti, P.; Roukoutakis, F.; Spyropoulou-Stassinaki, M.; Vasileiou, M.] Univ Athens, Dept Phys, Athens, Greece. [Cleymans, J.; Dietel, T.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Bala, R.; Bhasin, A.; Bhat, I. R.; Gupta, A.; Gupta, R.; Kour, M.; Kumar, A.; Mahajan, S.; Rajput, S.; Sambyal, S.; Sharma, A.; Sharma, M.] Univ Jammu, Dept Phys, Jammu 180004, India. [Raniwala, R.; Raniwala, S.] Univ Rajasthan, Dept Phys, Jaipur 302004, Rajasthan, India. [Dahms, T.; Fabbietti, L.; Gasik, P.; Vorobyev, I.] Tech Univ Munich, Dept Phys, D-80290 Munich, Germany. [Anguelov, V.; Bock, F.; Busch, O.; Deisting, A.; Fleck, M. G.; Glaessel, P.; Karayan, L.; Klein, J.; Knichel, M. L.; Leardini, L.; Mercado Perez, J.; Oeschler, H.; Oyama, K.; Pachmayer, Y.; Reidt, F.; Reygers, K.; Schicker, R.; Stachel, J.; Stiller, J. H.; Voelkl, M. A.; Wang, Y.; Wilkinson, J.; Windelband, B.; Winn, M.; Zimmermann, A.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Aimo, I.] Politecn Torino, Turin, Italy. [Browning, T. A.; Scharenberg, R. P.; Srivastava, B. K.] Purdue Univ, W Lafayette, IN 47907 USA. [Borissov, A.; Choi, K.; Chung, S. U.; Eum, J.; Seo, J.; Song, J.; Yoo, I. -K.] Pusan Natl Univ, Pusan 609735, South Korea. [Andronic, A.; Averbeck, R.; Braun-Munzinger, P.; Deisting, A.; Foka, P.; Frankenfeld, U.; Garabatos, C.; Ivanov, M.; Jimenez Bustamante, R. T.; Karayan, L.; Kollegger, T.; Lippmann, C.; Malzacher, P.; Marin, A.; Martin, N. A.; Masciocchi, S.; Miskowiec, D.; Nicassio, M.; Onderwaater, J.; Park, W. J.; Schmidt, C.; Schwarz, K.; Schweda, K.; Selyuzhenkov, I.; Thaeder, J.; Vranic, D.; Wagner, J.; Weber, S. G.] GSI Helmholtzzentrum Schwerionenforsch, Div Res, Darmstadt, Germany. [Andronic, A.; Averbeck, R.; Braun-Munzinger, P.; Deisting, A.; Foka, P.; Frankenfeld, U.; Garabatos, C.; Ivanov, M.; Jimenez Bustamante, R. T.; Karayan, L.; Kollegger, T.; Lippmann, C.; Malzacher, P.; Marin, A.; Martin, N. A.; Masciocchi, S.; Miskowiec, D.; Nicassio, M.; Onderwaater, J.; Park, W. J.; Schmidt, C.; Schwarz, K.; Schweda, K.; Selyuzhenkov, I.; Thaeder, J.; Vranic, D.; Wagner, J.; Weber, S. G.] GSI Helmholtzzentrum Schwerionenforsch, ExtreMe Matter Inst EMMI, Darmstadt, Germany. [Anticic, T.] Rudjer Boskovic Inst, Zagreb, Croatia. [Budnikov, D.; Filchagin, S.; Ilkaev, R.; Kuryakin, A.; Mamonov, A.; Nazarenko, S.; Punin, V.; Tumkin, A.; Vinogradov, Y.; Vyushin, A.; Zaviyalov, N.] Russian Fed Nucl Ctr VNIIEF, Sarov, Russia. [Aleksandrov, D.; Blau, D.; Fokin, S.; Ippolitov, M.; Manko, V.; Nikolaev, S.; Nikulin, S.; Nyanin, A.; Peresunko, D.; Ryabinkin, E.; Sibiriak, Y.; Vasiliev, A.; Vinogradov, A.; Yushmanov, I.] Kurchatov Inst, Russian Res Ctr, Moscow, Russia. [Chattopadhyay, S.; Das, D.; Das, I.; Khan, P.; Paul, B.; Roy, P.; Sinha, T.] Saha Inst Nucl Phys, Kolkata, India. [Alexandre, D.; Barnby, L. S.; Evans, D.; Graham, K. L.; Jones, P. G.; Jusko, A.; Krivda, M.; Lee, G. R.; Lietava, R.; Baillie, O. Villalobos; Zardoshti, N.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Calvo Villar, E.; Gago, A. M.] Pontificia Univ Catolica Peru, Dept Ciencias, Secc Fis, Lima, Peru. [de Cataldo, G.; Elia, D.; Lenti, V.; Manzari, V.; Minervini, L. M.; Nappi, E.; Paticchio, V.] Sezione Ist Nazl Fis Nucl, Bari, Italy. [Alici, A.; Antonioli, P.; Cindolo, F.; Hatzifotiadou, D.; Margotti, A.; Nania, R.; Noferini, F.; Pinazza, O.; Preghenella, R.; Scapparone, E.; Williams, M. C. S.; Zampolli, C.] Sezione Ist Nazl Fis Nucl, Bologna, Italy. [Cicalo, C.; Masoni, A.; Siddhanta, S.] Sezione Ist Nazl Fis Nucl, Cagliari, Italy. [Badala, A.; Pappalardo, G. S.] Sezione Ist Nazl Fis Nucl, Catania, Italy. [Antinori, F.; Dainese, A.; Fabris, D.; Turrisi, R.] Sezione Ist Nazl Fis Nucl, Padua, Italy. [Mazzoni, M. A.] Sezione Ist Nazl Fis Nucl, Rome, Italy. [Fragiacomo, E.; Grion, N.; Piano, S.; Rachevski, A.] Sezione Ist Nazl Fis Nucl, Trieste, Italy. [Agnello, M.; Aimo, I.; Akindinov, A.; Alessandro, B.; Arnaldi, R.; Bagnasco, S.; Barbano, A. M.; Bedda, C.; Bogdanov, A.; Borissov, A.; Bruna, E.; Bufalino, S.; Cerello, P.; De Marco, N.; Feliciello, A.; La Pointe, S. L.; Oppedisano, C.; Prino, F.; Puccio, M.; Rivetti, A.; Scomparin, E.; Trogolo, S.] Sezione Ist Nazl Fis Nucl, Turin, Italy. [Evdokimov, S.; Izucheev, V.; Kharlov, Y.; Kondratyuk, E.; Petrov, V.; Polichtchouk, B.; Sadovsky, S.; Shangaraev, A.] NRC Kurchatov Inst, SSC IHEP, Protvino, Russia. [Akindinov, A.; Aphecetche, L.; Audurier, B.; Batigne, G.; Erazmus, B.; Estienne, M.; Germain, M.; Martin Blanco, J.; Martinez Garcia, G.; Massacrier, L.; De Godoy, D. A. Moreira; Morreale, A.; Pillot, P.; Ronflette, L.; Schutz, Y.; Shabetai, A.; Stocco, D.; Wang, M.; Zhu, J.] Univ Nantes, Ecole Mines Nantes, SUBATECH, CNRS,IN2P3, Nantes, France. [Kobdaj, C.; Poonsawat, W.] Suranaree Univ Technol, Nakhon Ratchasima, Thailand. [Cerkala, J.; Jadlovska, S.; Kopcik, M.; Papcun, P.] Tech Univ Kosice, Kosice, Slovakia. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ Split FESB, Split, Croatia. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Goerlich, L.; Kowalski, M.; Matyja, A.; Mayer, C.; Otwinowski, J.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Blair, J. T.; Knospe, A. G.; Markert, C.; Thomas, D.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Almaraz, J. R. M.; Leon Monzon, I.; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Alves Garcia Prado, C.; Bregant, M.; Cosentino, M. R.; De, S.; Gimenez, D. Domenicis; Figueredo, M. A. S.; Jahnke, C.; Lagana Fernandes, C.; Luz, P. H. F. N. D.; Mas, A.; Munhoz, M. G.; Oliveira Da Silva, A. C.; Pereira De Oliveira Filho, E.; Suaide, A. A. P.; de Toledo, A. Szanto; Zanoli, H. J. C.] Univ Sao Paulo, BR-09500900 Sao Paulo, Brazil. [Chinellato, D. D.; Dash, A.; Takahashi, J.] Univ Estadual Campinas, UNICAMP, Campinas, SP, Brazil. [Akindinov, A.; Bianchi, L.; Mcdonald, D.; Ng, F.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.] Univ Houston, Houston, TX USA. [Chang, B.; Kim, D. J.; Kral, J.; Rak, J.; Slupecki, M.; Snellman, T. W.; Trzaska, W. H.; Vargyas, M.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Chartier, M.; Figueredo, M. A. S.; Norman, J.; Romita, R.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Castro, A. J.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.; Sorensen, S.] Univ Tennessee, Knoxville, TN USA. [Vilakazi, Z.] Univ Witwatersrand, Johannesburg 2050, South Africa. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Sekiguchi, Y.; Terasaki, K.; Tsuji, T.; Watanabe, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Busch, O.; Chujo, T.; Esumi, S.; Hosokawa, R.; Inaba, M.; Kobayashi, T.; Masui, H.; Miake, Y.; Sano, M.; Tanaka, N.; Watanabe, D.; Yokoyama, H.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Erhardt, F.; Planinic, M.; Poljak, N.; Simatovic, G.; Utrobicic, A.] Univ Zagreb, Zagreb 41000, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Teyssier, B.; Tieulent, R.; Uras, A.] Univ Lyon 1, CNRS, IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Ahammed, Z.; Alam, S. N.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mitra, J.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Patra, R. N.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata, India. [Graczykowski, L. K.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pluta, J.; Szymanski, M.; Zaborowska, A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Belmont, R.; Bianchin, C.; Pan, J.; Pruneau, C. A.; Pujahari, P.; Putschke, J.; Reed, R. J.; Saleh, M. A.; Verweij, M.; Voloshin, S. A.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Barnafoeldi, G. G.; Bencedi, G.; Berenyi, D.; Boldizsar, L.; Denes, E.; Hamar, G.; Kiss, G.; Levai, P.; Lowe, A.; Olah, L.; Pochybova, S.; Varga, D.; Volpe, G.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Aiola, S.; Caines, H.; Connors, M. E.; Ehlers, R. J.; Harris, J. W.; Majka, R. D.; Mulligan, J. D.; Oh, S.; Oliver, M. H.; Schuster, T.; Smirnov, N.] Yale Univ, New Haven, CT USA. [Kang, J. H.; Kim, B.; Kim, H.; Kim, M.; Kim, T.; Kwon, Y.; Lee, S.; Song, M.] Yonsei Univ, Seoul 120749, South Korea. [Keidel, R.] Fachhsch Worms, ZTT, Worms, Germany. RP Adam, J (reprint author), Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic. RI Armesto, Nestor/C-4341-2017; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Kovalenko, Vladimir/C-5709-2013; Altsybeev, Igor/K-6687-2013; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Cosentino, Mauro/L-2418-2014; Suaide, Alexandre/L-6239-2016; Barnby, Lee/G-2135-2010; Peitzmann, Thomas/K-2206-2012; Kondratiev, Valery/J-8574-2013; Vinogradov, Leonid/K-3047-2013; Castillo Castellanos, Javier/G-8915-2013; Ferreiro, Elena/C-3797-2017; Chinellato, David/D-3092-2012; Pshenichnov, Igor/A-4063-2008; Felea, Daniel/C-1885-2012; Bregant, Marco/I-7663-2012; Sevcenco, Adrian/C-1832-2012; De Pasquale, Salvatore/B-9165-2008; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Vechernin, Vladimir/J-5832-2013; Akindinov, Alexander/J-2674-2016; Takahashi, Jun/B-2946-2012 OI Armesto, Nestor/0000-0003-0940-0783; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Kovalenko, Vladimir/0000-0001-6012-6615; Altsybeev, Igor/0000-0002-8079-7026; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Riggi, Francesco/0000-0002-0030-8377; Scarlassara, Fernando/0000-0002-4663-8216; Melikyan, Yury/0000-0002-4165-505X; Giubilato, Piero/0000-0003-4358-5355; Fernandez Tellez, Arturo/0000-0001-5092-9748; Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Cosentino, Mauro/0000-0002-7880-8611; Suaide, Alexandre/0000-0003-2847-6556; Barnby, Lee/0000-0001-7357-9904; Peitzmann, Thomas/0000-0002-7116-899X; Kondratiev, Valery/0000-0002-0031-0741; Vinogradov, Leonid/0000-0001-9247-6230; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; Chinellato, David/0000-0002-9982-9577; Pshenichnov, Igor/0000-0003-1752-4524; Felea, Daniel/0000-0002-3734-9439; Sevcenco, Adrian/0000-0002-4151-1056; De Pasquale, Salvatore/0000-0001-9236-0748; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Vechernin, Vladimir/0000-0003-1458-8055; Akindinov, Alexander/0000-0002-7388-3022; Takahashi, Jun/0000-0002-4091-1779 FU Worldwide LHC Computing Grid (WLCG) collaboration; State Committee of Science, Armenia; World Federation of Scientists (WFS), Armenia; Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics; "Region Pays de Loire", France; "Region Alsace", France; "Region Auvergne", France; CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA); National Office for Research and Technology (NKTH); Department of Atomic Energy of the Government of India; Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN), Italy; Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; Joint Institute for Nuclear Research, Dubna, Russia; National Research Foundation of Korea (NRF); Amerique Latine Formation academique-European Commission (ALFA-EC); EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM), Netherlands; Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics, Romania; National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); E-Infrastructure shared between Europe and Latin America (EELA); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN); Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; Ministry of Science, Education and Sports of Croatia, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Unity through Knowledge Fund, Croatia; United States National Science Foundation; State of Texas; State of Ohio; Academy of Finland; French CNRS-IN2P3, France; MEXT, Japan; Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico (DGAPA), Mexico FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centers and the Worldwide LHC Computing Grid (WLCG) collaboration.; The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the "Region Pays de Loire," "Region Alsace," "Region Auvergne," and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA) and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna, Russia; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico (DGAPA), Mexico; Amerique Latine Formation academique-European Commission (ALFA-EC) and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India. NR 52 TC 3 Z9 3 U1 4 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 31 PY 2016 VL 93 IS 3 AR 034916 DI 10.1103/PhysRevC.93.034916 PG 22 WC Physics, Nuclear SC Physics GA DH9HA UT WOS:000373105800005 ER PT J AU Thiaville, JJ Frelin, O Garcia-Salinas, C Harrison, K Hasnain, G Horenstein, NA de la Garza, RID Henry, CS Hanson, AD de Crecy-Lagard, V AF Thiaville, Jennifer J. Frelin, Oceane Garcia-Salinas, Carolina Harrison, Katherine Hasnain, Ghulam Horenstein, Nicole A. de la Garza, Rocio I. Diaz Henry, Christopher S. Hanson, Andrew D. de Crecy-Lagard, Valerie TI Experimental and Metabolic Modeling Evidence for a Folate-Cleaving Side-Activity of Ketopantoate Hydroxymethyltransferase (PanB) SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE metabolite repair; side-reaction; Acinetobacter baylyi; paralogs; folate biosynthesis ID MULTIPLE SEQUENCE ALIGNMENT; ONE-CARBON METABOLISM; ESCHERICHIA-COLI; DIHYDROPTEROATE SYNTHASE; ABSOLUTE-CONFIGURATION; PLANTS; ENZYME; BIOSYNTHESIS; ACID; EXPRESSION AB Tetrahydrofolate (THF) and its one-carbon derivatives, collectively termed folates, are essential cofactors, but are inherently unstable. While it is clear that chemical oxidation can cleave folates or damage their pterin precursors, very little is known about enzymatic damage to these molecules or about whether the folate biosynthesis pathway responds adaptively to damage to its end-products. The presence of a duplication of the gene encoding the folate biosynthesis enzyme 6-hydroxymethyl-7,8-dihydropterin pyrophosphokinase (FolK) in many sequenced bacterial genomes combined with a strong chromosomal clustering of the folK gene with panB, encoding the 5,10-methylene-THF-dependent enzyme ketopantoate hydroxymethyltransferase, led us to infer that PanB has a side activity that cleaves 5,10-methylene-THF, yielding a pterin product that is recycled by FolK. Genetic and metabolic analyses of Escherichia poll strains showed that overexpression of PanB leads to accumulation of the likely folate cleavage product 6-hydroxymethylpterin and other pterins in cells and medium, and unexpectedly to a 46% increase in total folate content. In silico modeling of the folate biosynthesis pathway showed that these observations are consistent with the in vivo cleavage of 5,10-methylene-THF by a side-activity of PanB, with FolK-mediated recycling of the pterin cleavage product, and with regulation of folate biosynthesis by folates or their damage products. C1 [Thiaville, Jennifer J.; Harrison, Katherine; de Crecy-Lagard, Valerie] Univ Florida, Dept Microbiol & Cell Sci, Gainesville, FL 32611 USA. [Frelin, Oceane; Hasnain, Ghulam; Hanson, Andrew D.] Univ Florida, Dept Hort Sci, Gainesville, FL 32611 USA. [Garcia-Salinas, Carolina; de la Garza, Rocio I. Diaz] Tecnol Monterrey, Campus Monterrey, Monterrey, Mexico. [Horenstein, Nicole A.] Univ Florida, Dept Chem, Gainesville, FL 32611 USA. [Henry, Christopher S.] Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Henry, Christopher S.] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [de Crecy-Lagard, Valerie] Univ Florida, Genet Inst, Gainesville, FL USA. RP de Crecy-Lagard, V (reprint author), Univ Florida, Dept Microbiol & Cell Sci, Gainesville, FL 32611 USA.; Hanson, AD (reprint author), Univ Florida, Dept Hort Sci, Gainesville, FL 32611 USA.; de Crecy-Lagard, V (reprint author), Univ Florida, Genet Inst, Gainesville, FL USA. EM adha@ufl.edu; vcrecy@ufl.edu FU US National Science Foundation (NSF) [MCB-1153413] FX This work was funded by US National Science Foundation (NSF) grants MCB-1153413. NR 83 TC 1 Z9 1 U1 3 U2 6 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD MAR 31 PY 2016 VL 7 AR 431 DI 10.3389/fmicb.2016.00431 PG 14 WC Microbiology SC Microbiology GA DI1SY UT WOS:000373277300001 PM 27065985 ER PT J AU Petousis, I Chen, W Hautier, G Graf, T Schladt, TD Persson, KA Prinz, FB AF Petousis, Ioannis Chen, Wei Hautier, Geoffroy Graf, Tanja Schladt, Thomas D. Persson, Kristin A. Prinz, Fritz B. TI Benchmarking density functional perturbation theory to enable high-throughput screening of materials for dielectric constant and refractive index SO PHYSICAL REVIEW B LA English DT Article ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; LINEAR-RESPONSE; BASIS-SET; CRYSTALS; EXCHANGE; BEHAVIOR; APPROXIMATIONS; DEPENDENCE AB We demonstrate a high-throughput density functional perturbation theory (DFPT) methodology capable of screening compounds for their dielectric properties. The electronic and ionic dielectric tensors are calculated for 88 compounds, where the eigenvalues of the total dielectric tensors are compared with single crystal and polycrystalline experimental values reported in the literature. We find that GGA/PBE has a smaller mean average deviation from experiments (MARD = 16.2%) when compared to LDA. The prediction accuracy of DFPT is lowest for compounds that exhibit complex structural relaxation effects (e.g., octahedra rotation in perovskites) and/or strong anharmonicity. Despite some discrepancies between DFPT results and reported experimental values, the high-throughput methodology is found to be useful in identifying interesting compounds by ranking. This is demonstrated by the high Spearman correlation factor (rho = 0.92). Finally, we demonstrate that DFPT provides a good estimate for the refractive index of a compound without calculating the frequency dependence of the dielectric matrix (MARD = 5.7%). C1 [Petousis, Ioannis; Prinz, Fritz B.] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. [Chen, Wei] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Technol Area, Berkeley, CA 94720 USA. [Chen, Wei] IIT, Dept Mech Mat & Aerosp Engn, Chicago, IL 60616 USA. [Hautier, Geoffroy] Catholic Univ Louvain, Inst Condensed Matter & Nanosci, B-1348 Louvain La Neuve, Belgium. [Graf, Tanja; Schladt, Thomas D.] Volkswagen Grp Res, Berliner Ring 2, D-38840 Wolfsburg, Germany. [Persson, Kristin A.] Dept Mat Sci & Engn, Hearst Min Mem Bldg, Berkeley, CA 94720 USA. [Prinz, Fritz B.] Stanford Univ, Dept Mech Engn, Stanford, CA 94305 USA. RP Petousis, I (reprint author), Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. EM ioannis.petousis@gmail.com RI Chen, Wei/B-3045-2012 OI Chen, Wei/0000-0002-1135-7721 FU Volkswagen group; Materials Project Center, under the Department of Energy (USA), Basic Energy Sciences (USA) [EDCBEE]; Office of Basic Energy Sciences (USA) of the U.S. Department of Energy (USA) [DE-AC02-05CH11231] FX This work was supported financially by the Volkswagen group. Kristin Persson and Wei Chen gratefully acknowledge support from the Materials Project Center, under the Department of Energy (USA), Basic Energy Sciences (USA), Grant No. EDCBEE. The calculations were performed using the computational resources of the National Energy Research Scientific Computing Center, which is supported under the Office of Basic Energy Sciences (USA) of the U.S. Department of Energy (USA) under Contract No. DE-AC02-05CH11231. NR 56 TC 2 Z9 2 U1 5 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 31 PY 2016 VL 93 IS 11 AR 115151 DI 10.1103/PhysRevB.93.115151 PG 8 WC Physics, Condensed Matter SC Physics GA DH9GM UT WOS:000373104400004 ER PT J AU Huang, PS Joglekar, A Li, B Wagner, CEM AF Huang, Peisi Joglekar, Aniket Li, Bing Wagner, Carlos E. M. TI Probing the electroweak phase transition at the LHC SO PHYSICAL REVIEW D LA English DT Article ID BOSON PAIR PRODUCTION; HIGGS-BOSON; BARYON ASYMMETRY; STANDARD MODEL; SUPERSYMMETRIC MODEL; CP-INVARIANCE; GLUON FUSION; BARYOGENESIS; MASS; VIOLATION AB We study the correlation between the value of the triple Higgs coupling and the nature of the electroweak phase transition. We use an effective potential approach, including higher order, nonrenormalizable terms coming from integrating out new physics. We show that if only the dimension six operators are considered, large positive deviations of the triple Higgs coupling from its standard model (SM) value are predicted in the regions of parameter space consistent with a strong first order electroweak phase transition. We also show that at higher orders sizable and negative deviations of the triple Higgs coupling may be obtained, and the sign of the corrections tends to be correlated with the order of the phase transition. We also consider a singlet extension of the SM, which allows us to establish the connection with the effective field theory approach and analyze the limits of its validity. Furthermore, we study how to probe the triple Higgs coupling from the double Higgs production at the LHC. We show that selective cuts in the invariant mass of the two Higgs bosons should be used, to maximize the sensitivity for values of the triple Higgs coupling significantly different from the standard model one. C1 [Huang, Peisi; Joglekar, Aniket; Li, Bing; Wagner, Carlos E. M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Wagner, Carlos E. M.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Huang, Peisi; Wagner, Carlos E. M.] Argonne Natl Lab, HEP Div, 9700 Cass Ave, Argonne, IL 60439 USA. RP Huang, PS (reprint author), Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA.; Huang, PS (reprint author), Argonne Natl Lab, HEP Div, 9700 Cass Ave, Argonne, IL 60439 USA. FU U.S. Department of Energy [DE-FG02-13ER41958, DE-AC02-06CH11357, DE-FG02-04ER41286] FX We thank V. Barger, L. Everett, J. Gao, H. Haber, A. Ismail, I. Lewis, M. Peskin and L. T. Wang for useful discussions. Work is supported by the U.S. Department of Energy under Award No. DE-FG02-13ER41958. Work at ANL is supported in part by the U.S. Department of Energy under Award No. DE-AC02-06CH11357. P. H. is partially supported by U.S. Department of Energy Award No. DE-FG02-04ER41286. NR 111 TC 7 Z9 7 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 31 PY 2016 VL 93 IS 5 AR 055049 DI 10.1103/PhysRevD.93.055049 PG 21 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH9HJ UT WOS:000373106700007 ER PT J AU Sun, Y Zhang, F Ye, Z Zhang, Y Fang, XW Ding, ZJ Wang, CZ Mendelev, MI Ott, RT Kramer, MJ Ho, KM AF Sun, Yang Zhang, Feng Ye, Zhuo Zhang, Yue Fang, Xiaowei Ding, Zejun Wang, Cai-Zhuang Mendelev, Mikhail I. Ott, Ryan T. Kramer, Matthew J. Ho, Kai-Ming TI 'Crystal Genes' in Metallic Liquids and Glasses SO SCIENTIFIC REPORTS LA English DT Article ID MECHANICAL-PROPERTIES; STRUCTURAL MODEL; CU-ZR; AL; ORDER; ALLOYS; PHASE; STABILITY AB We analyze the underlying structural order that transcends liquid, glass and crystalline states in metallic systems. A genetic algorithm is applied to search for the most common energetically favorable packing motifs in crystalline structures. These motifs are in turn compared to the observed packing motifs in the actual liquid or glass structures using a cluster-alignment method. Using this method, we have revealed the nature of the short-range order in Cu64Zr36 glasses. More importantly, we identified a novel structural order in the Al90Sm10 system. In addition, our approach brings new insight into understanding the origin of vitrification and describing mesoscopic order-disorder transitions in condensed matter systems. C1 [Sun, Yang; Fang, Xiaowei; Ding, Zejun; Ho, Kai-Ming] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [Sun, Yang; Fang, Xiaowei; Ding, Zejun; Ho, Kai-Ming] Univ Sci & Technol China, Dept Phys, Hefei 230026, Anhui, Peoples R China. [Sun, Yang; Zhang, Feng; Ye, Zhuo; Zhang, Yue; Fang, Xiaowei; Wang, Cai-Zhuang; Mendelev, Mikhail I.; Ott, Ryan T.; Kramer, Matthew J.; Ho, Kai-Ming] US DOE, Ames Lab, Ames, IA 50011 USA. [Wang, Cai-Zhuang; Ho, Kai-Ming] Iowa State Univ, Dept Phys, Ames, IA 50011 USA. [Ho, Kai-Ming] Univ Sci & Technol China, Int Ctr Quantum Design Funct Mat ICQD, Hefei 230026, Anhui, Peoples R China. [Ho, Kai-Ming] Univ Sci & Technol China, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China. RP Ho, KM (reprint author), Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China.; Ho, KM (reprint author), Univ Sci & Technol China, Dept Phys, Hefei 230026, Anhui, Peoples R China.; Zhang, F; Ho, KM (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA.; Ho, KM (reprint author), Iowa State Univ, Dept Phys, Ames, IA 50011 USA.; Ho, KM (reprint author), Univ Sci & Technol China, Int Ctr Quantum Design Funct Mat ICQD, Hefei 230026, Anhui, Peoples R China.; Ho, KM (reprint author), Univ Sci & Technol China, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China. EM fzhang@ameslab.gov; kmh@ameslab.gov OI Sun, Yang/0000-0002-4344-2920 FU US Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division [DE-AC02-07CH11358]; Advanced Photon Source, Argonne National Laboratory [DE-AC02-06CH11357]; China Scholarship Council [201406340015]; National Natural Science Foundation of China [11274288, 11574289]; National Basic Research Program of China [2012CB933702]; USTC Qian-Ren B (1000-Talents Program B) fund; National Energy Research Supercomputing Center (NERSC) in Berkeley, CA FX Work at Ames Laboratory was supported by the US Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division, under Contract No. DE-AC02-07CH11358, including a grant of computer time at the National Energy Research Supercomputing Center (NERSC) in Berkeley, CA. The high-energy X-ray experiments were performed at the Advanced Photon Source, Argonne National Laboratory, under Grant No. DE-AC02-06CH11357. Y.S. acknowledges support from China Scholarship Council (File No. 201406340015). Z.D. acknowledges support from the National Natural Science Foundation of China (No. 11274288 and No. 11574289) and the National Basic Research Program of China (No. 2012CB933702). K.-M.H. acknowledges support from USTC Qian-Ren B (1000-Talents Program B) fund. NR 56 TC 3 Z9 3 U1 10 U2 38 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 31 PY 2016 VL 6 AR 23734 DI 10.1038/srep23734 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH9BO UT WOS:000373091000001 PM 27030071 ER PT J AU Chen, L Xie, WY Wang, GC Bhat, I Zhang, SB Goyal, A Lu, TM AF Chen, Liang Xie, Weiyu Wang, Gwo-Ching Bhat, Ishwara Zhang, Shengbai Goyal, Amit Lu, Toh-Ming TI Heteroepitaxy of large grain Ge film on cube-textured Ni(001) foils through CaF2 buffer layer SO THIN SOLID FILMS LA English DT Article DE Heteroepitaxy; Biaxial film; Nickel foils; Buffer layer; Germanium; X-ray diffraction; Large grain size ID BEAM-ASSISTED DEPOSITION; INCLINED-SUBSTRATE DEPOSITION; THIN-FILMS; CRYSTAL SILICON; BIAXIAL ALIGNMENT; CARRIER MOBILITY; GROWTH; NI; OXIDE; GLASS AB Cube-textured Ni(001) foils have been considered as a viable alternative substrate to grow high quality functional films for large area optoelectronic devices. In this work, we report the heteroepitaxial growth of CaF2(001) films on cube-textured Ni(001) foils at 350-600 degrees C with in-plane orientation of CaF2[110]//Ni[100] and CaF2[(1) over bar 10]//Ni[010] with 45 degrees rotation respect to the Ni(001) substrate. Unlike CaF2(111)/Ni(001) films where there exist four independent rotational domains with rotational domain boundaries, CaF2(001)/Ni(001) contains no rotational domains or rotational domain boundaries. This makes CaF2(001)/Ni(001) films better candidates as templates for the growth of high quality functional semiconductors. We also demonstrate that Ge(001) film with no rotational domains and with a grain size of similar to 50 mu m similar to that of the Ni substrate can be grown on the CaF2(001) buffered Ni substrate. (C) 2016 Elsevier B.V. All rights reserved. C1 [Chen, Liang; Xie, Weiyu; Wang, Gwo-Ching; Zhang, Shengbai; Lu, Toh-Ming] Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA. [Bhat, Ishwara] Rensselaer Polytech Inst, Dept Elect Comp & Syst Engn, Troy, NY 12180 USA. [Goyal, Amit] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Chen, L (reprint author), Rensselaer Polytech Inst, Dept Phys Appl Phys & Astron, Troy, NY 12180 USA. EM talentcl1987@gmail.com RI chen, liang/L-9868-2013 OI chen, liang/0000-0002-1680-2628 FU NSF [DMR 1305293] FX This work was supported by the NSF DMR 1305293. The authors thank Dr. Zhonghuan Lu in assisting the EBSD data acquisition. The authors also thank Aaron Littlejohn in English editing of the original manuscript. NR 41 TC 1 Z9 1 U1 4 U2 6 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0040-6090 J9 THIN SOLID FILMS JI Thin Solid Films PD MAR 31 PY 2016 VL 603 BP 428 EP 434 DI 10.1016/j.tsf.2016.03.007 PG 7 WC Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Materials Science; Physics GA DH4ZQ UT WOS:000372794900071 ER PT J AU Louder, RK He, Y Lopez-Blance, JR Fang, J Chacon, P Nogales, E AF Louder, Robert K. He, Yuan Ramon Lopez-Blance, Jose Fang, Jie Chacon, Pablo Nogales, Eva TI Structure of promoter-bound TFIID and model of human pre-initiation complex assembly SO NATURE LA English DT Article ID RNA-POLYMERASE-II; TATA-BINDING PROTEIN; CORE PROMOTER; TRANSCRIPTION INITIATION; ELECTRON-MICROSCOPY; CRYSTAL-STRUCTURE; HUMAN GENOME; CRYO-EM; TAFS; ARCHITECTURE AB The general transcription factor IID (TFIID) plays a central role in the initiation of RNA polymerase II (Pol II)-dependent transcription by nucleating pre-initiation complex (PIC) assembly at the core promoter. TFIID comprises the TATA-binding protein (TBP) and 13 TBP-associated factors (TAF1-13), which specifically interact with a variety of core promoter DNA sequences. Here we present the structure of human TFIID in complex with TFIIA and core promoter DNA, determined by single-particle cryo-electron microscopy at sub-nanometre resolution. All core promoter elements are contacted by subunits of TFIID, with TAF1 and TAF2 mediating major interactions with the downstream promoter. TFIIA bridges the TBP-TATA complex with lobe B of TFIID. We also present the cryo-electron microscopy reconstruction of a fully assembled human TAF-less PIC. Superposition of common elements between the two structures provides novel insights into the general role of TFIID in promoter recognition, PIC assembly, and transcription initiation. C1 [Louder, Robert K.] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [He, Yuan; Nogales, Eva] Univ Calif Berkeley, Dept Mol & Cell Biol, Inst QB3, Berkeley, CA 94720 USA. [He, Yuan; Chacon, Pablo; Nogales, Eva] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrat Bioimaging Div, Berkeley, CA 94720 USA. [Ramon Lopez-Blance, Jose] CSIC, Dept Biol Phys Chem, Rocasolano Phys Chem Inst, Serrano 119, Madrid 28006, Spain. [Fang, Jie; Nogales, Eva] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [He, Yuan] Northwestern Univ, Interdisciplinary Biol Sci Program, Evanston, IL 60208 USA. RP Nogales, E (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, Inst QB3, Berkeley, CA 94720 USA.; Nogales, E (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrat Bioimaging Div, Berkeley, CA 94720 USA.; Nogales, E (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. EM ENogales@lbl.gov RI Chacon, Pablo/B-4211-2014 OI Chacon, Pablo/0000-0002-3168-4826 FU National Energy Research Scientific Computing Center [DE-AC02-05CH11231]; NIGMS [GM63072]; Spanish Ministry of Economy and Competitiveness [BFU2013-44306P]; NIGMS Molecular Biophysics Training Grant [GM008295] FX We thank P. Grob, S. Howes, and R. Zhang for electron microscopy support; T. Houweling for computer support; S. Scheres for technical advice on image processing; A. Patel for discussion; C. Inouye for providing us with recombinant TFIIF; S. Zheng for providing TAF4 mAb; and D. King for providing peptides. We are thankful to R. Tjian and J. Kadonaga for their comments on the manuscript. Computational resources were provided in part by the National Energy Research Scientific Computing Center (DE-AC02-05CH11231). This work was funded by NIGMS (GM63072 to E.N.) and Spanish Ministry of Economy and Competitiveness (BFU2013-44306P to P.C.). R.K.L. was supported by the NIGMS Molecular Biophysics Training Grant (GM008295). E.N. is a Howard Hughes Medical Institute Investigator. NR 73 TC 17 Z9 17 U1 9 U2 28 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAR 31 PY 2016 VL 531 IS 7596 BP 604 EP + DI 10.1038/nature17394 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH8EX UT WOS:000373027400031 PM 27007846 ER PT J AU Brady, NF Appavoo, K Seo, M Nag, J Prasankumar, RP Haglund, RF Hilton, DJ AF Brady, Nathaniel F. Appavoo, Kannatassen Seo, Minah Nag, Joyeeta Prasankumar, Rohit P. Haglund, Richard F., Jr. Hilton, David J. TI Heterogeneous nucleation and growth dynamics in the light-induced phase transition in vanadium dioxide SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE insulator-to-metal phase transitions; heterogeneous phase transitions; light-induced phase transitions ID METAL-INSULATOR-TRANSITION; ELECTRON-DIFFRACTION; VO2; SPECTROSCOPY; KINETICS AB We report on ultrafast optical investigations of the light-induced insulator-to-metal phase transition in vanadium dioxide with controlled disorder generated by substrate mismatch. These results reveal common dynamics of this optically-induced phase transition that are independent of this disorder. Above the fluence threshold for completing the transition to the rutile crystalline phase, we find a common time scale, independent of sample morphology, of 40.5 +/- 2 ps that is consistent with nucleation and growth dynamics of the R phase from the parent M1 ground state. C1 [Brady, Nathaniel F.; Hilton, David J.] Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. [Appavoo, Kannatassen; Nag, Joyeeta; Haglund, Richard F., Jr.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Seo, Minah] Korea Inst Sci & Technol, Seoul 136791, South Korea. [Seo, Minah; Prasankumar, Rohit P.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Hilton, DJ (reprint author), Univ Alabama Birmingham, Dept Phys, Birmingham, AL 35294 USA. EM dhilton@uab.edu FU U.S. Dept. Education GAANN Fellowship [P200A090143]; National Science Foundation [ECS-0801985]; US Department of Energy [DE-FG02-01ER4591]; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX NFB acknowledges support from the U.S. Dept. Education GAANN Fellowship (P200A090143). JN was supported by the National Science Foundation under contract ECS-0801985 for synthesis and characterization of the thin films, and KA was supported by the US Department of Energy under contract DE-FG02-01ER4591 for the ultrafast experiments. This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Los Alamos National Laboratory, an affirmative action equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under contract DE-AC52-06NA25396. NR 36 TC 1 Z9 1 U1 10 U2 31 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAR 31 PY 2016 VL 28 IS 12 AR 125603 DI 10.1088/0953-8984/28/12/125603 PG 7 WC Physics, Condensed Matter SC Physics GA DG2OJ UT WOS:000371906600010 PM 26932975 ER PT J AU Lesseux, GG Garitezi, TM Rosa, PFS Jesus, CBR Oseroff, SB Sarrao, JL Fisk, Z Urbano, RR Pagliuso, PG Rettori, C AF Lesseux, G. G. Garitezi, T. M. Rosa, P. F. S. Jesus, C. B. R. Oseroff, S. B. Sarrao, J. L. Fisk, Z. Urbano, R. R. Pagliuso, P. G. Rettori, C. TI Unusual diffusive effects on the ESR of Nd3+ ions in the tunable topologically nontrivial semimetal YBiPt SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE topological materials; electron spin resonance; half-Heusler compound ID ELECTRON-SPIN-RESONANCE; HGTE QUANTUM-WELLS; SINGLE DIRAC CONE; CRYSTALLINE INSULATORS; MAGNETIC IONS; SURFACE; METALS; STATE; SMB6; ABSORPTION AB Electron spin resonance (ESR) of diluted Nd3+ ions in the topologically nontrivial semimetallic (TNSM) YBiPt compound is reported. The cubic YBiPt compound is a non-centrosymmetric half Heusler material which crystallizes in the F43m space group. The low temperature Nd3+ ESR spectra showed a g-value of 2.66(4) corresponding to a Gamma(6) cubic crystal field Kramers' doublet ground state. Remarkably, the observed metallic and diffusive (Dysonian) Nd3+ lineshape presented an unusual dependence with grain size, microwave power, Nd3+ concentration and temperature. Moreover, the spin dynamic of the localized Nd3+ ions in YBiPt was found to be characteristic of a phonon-bottleneck regime. It is claimed that, in this regime for YBiPt, phonons are responsible for mediating the diffusion of the microwave energy absorbed at resonance by the Nd3+ ions to the thermal bath throughout the skin depth (delta similar or equal to 15 mu m). We argue that this is only possible because of the existence of highly mobile conduction electrons inside the skin depth of YBiPt that are strongly coupled to the phonons by spin-orbit coupling. Therefore, our unexpected ESR results point to a coexistence of metallic and insulating behaviors within the skin depth of YBiPt. This scenario is discussed in the light of the TNSM properties of this compound. C1 [Lesseux, G. G.; Garitezi, T. M.; Rosa, P. F. S.; Jesus, C. B. R.; Urbano, R. R.; Pagliuso, P. G.; Rettori, C.] Univ Estadual Campinas, Inst Fis Gleb Wataghin, BR-13083859 Campinas, SP, Brazil. [Rosa, P. F. S.; Fisk, Z.] Univ Calif Irvine, Irvine, CA 92697 USA. [Oseroff, S. B.] San Diego State Univ, San Diego, CA 92182 USA. [Sarrao, J. L.; Rettori, C.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. Univ Fed ABC UFABC, CCNH, BR-09210580 Santo Andre, SP, Brazil. RP Lesseux, GG (reprint author), Univ Estadual Campinas, Inst Fis Gleb Wataghin, BR-13083859 Campinas, SP, Brazil. EM lesseuxgg@gmail.com RI Jesus, C/J-5829-2013 OI Jesus, C/0000-0003-3177-0385 FU FAPESP [2006/60440-0, 2007/50986-0, 2011/01564-0, 2012/05903-6]; CNPq (Brazil); FINEP (Brazil); CAPES (Brazil); NSF (USA) [DMR-0801253] FX We are thankful to Y Kopelevich for enlightening discussions. This work was conducted under the auspices of FAPESP (Grant Nos. 2006/60440-0, 2007/50986-0, 2011/01564-0, 2012/05903-6), CNPq, FINEP and CAPES (Brazil), and NSF (DMR-0801253) (USA). NR 59 TC 0 Z9 0 U1 11 U2 20 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAR 31 PY 2016 VL 28 IS 12 AR 125601 DI 10.1088/0953-8984/28/12/125601 PG 9 WC Physics, Condensed Matter SC Physics GA DG2OJ UT WOS:000371906600008 PM 26912417 ER PT J AU Ai, G Wang, ZH Zhao, H Mao, WF Fu, YB Yi, R Gao, Y Battaglia, V Wang, DH Lopatin, S Liu, G AF Ai, Guo Wang, Zhihui Zhao, Hui Mao, Wenfeng Fu, Yanbao Yi, Ran Gao, Yue Battaglia, Vincent Wang, Donghai Lopatin, Sergey Liu, Gao TI Scalable process for application of stabilized lithium metal powder in Li-ion batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Stabilized lithium metal powder (SLMP (R)); Prelithiation; SiO; Full cell ID FUNCTIONAL CONDUCTIVE POLYMER; ANODE MATERIALS; RATIONAL DESIGN; GRAPHITE ANODE; HIGH-CAPACITY; PERFORMANCE; CATHODE; CARBON; CELLS; SLMP AB A simple solution processing method is developed to achieve a uniform and scalable stabilized lithium metal powder (SLMP) coating on a Li-ion negative electrode. A solvent and binder system for the SLMP coating is developed, including the selection of solvent, polymer binder, and optimization of polymer concentration. The optimized binder solution is a 1% concentration of polymer binder in xylene; a mixture of polystyrene-co-butadiene) rubber (SBR) and polystyrene (PS) is chosen as the polymer binder. Results show that long-sustained, uniformly dispersed SLMP suspension can be achieved with the optimized binder solution. The uniform SLMP coating can be achieved using a simple "doctor blade" coating method, and the resulting SLMP coating can be firmly glued on the anode surface. By using SLMP to prelithiate the negative electrode, improvements in electrochemical performances are demonstrated in both graphite/NMC and SiO/NMC full cells. (C) Published by Elsevier B.V. C1 [Ai, Guo; Wang, Zhihui; Zhao, Hui; Mao, Wenfeng; Fu, Yanbao; Battaglia, Vincent; Liu, Gao] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Energy Technol Area, Berkeley, CA 94720 USA. [Ai, Guo] Minist Ind & Informat Technol, Sci & Technol Reliabil Phys & Applicat Elect Comp, Elect Res Inst 5, Guangzhou 510610, Guangdong, Peoples R China. [Yi, Ran; Gao, Yue; Wang, Donghai] Penn State Univ, Dept Mech & Nucl Engn, University Pk, PA 16802 USA. [Lopatin, Sergey] Appl Mat Inc, Santa Clara, CA 95054 USA. RP Liu, G (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Storage & Distributed Resources Div, Energy Technol Area, Berkeley, CA 94720 USA. EM gliu@lbl.gov FU Assistant Secretary for Energy Efficiency, Office of Vehicle Technologies of the U.S. Department of Energy (U.S. DOE) under the Advanced Battery Materials Research (BMR) program; Advanced Light Source at the Lawrence Berkeley National Laboratory - U.S. Department of Energy [DE-AC02-05CH11231]; Distinguished Young Scientist Program of Guangdong Province [2015A030306002]; China Scholarship Council; National Center for Electron Microscopy of the Molecular Foundry FX This work is funded by the Assistant Secretary for Energy Efficiency, Office of Vehicle Technologies of the U.S. Department of Energy (U.S. DOE) under the Advanced Battery Materials Research (BMR) program, along with the National Center for Electron Microscopy of the Molecular Foundry and the Advanced Light Source at the Lawrence Berkeley National Laboratory, which are supported by the U.S. Department of Energy under Contract # DE-AC02-05CH11231. Guo Ai is supported by the funding from the Distinguished Young Scientist Program of Guangdong Province (2015A030306002) and the China Scholarship Council. Ziyan Zheng (University of California, Berkeley) provided comments and modifications to the manuscript. NR 41 TC 2 Z9 2 U1 29 U2 109 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD MAR 31 PY 2016 VL 309 BP 33 EP 41 DI 10.1016/j.jpowsour.2016.01.061 PG 9 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DF7PD UT WOS:000371549100005 ER PT J AU Ahluwalia, RK Wang, X Steinbach, AJ AF Ahluwalia, R. K. Wang, X. Steinbach, A. J. TI Performance of advanced automotive fuel cell systems with heat rejection constraint SO JOURNAL OF POWER SOURCES LA English DT Article DE Polymer electrolyte fuel cells; Automotive application; Heat rejection; Kinetic and mass transfer losses; Mass transfer in cathode catalysts; Oxygen reduction reaction kinetics; Stability and durability ID PLATINUM ALLOY CATALYST; KINETICS; DURABILITY AB Although maintaining polymer electrolyte fuel cells (PEFC) at temperatures below 80 degrees C is desirable for extended durability and enhanced performance, the automotive application also requires the PEFC stacks to operate at elevated temperatures and meet the heat rejection constraint, stated as Q/Delta T < 1.45 kW/degrees C, where Q is the stack heat load for an 80-kW(e) net power PEFC system and Delta T is the difference between the stack coolant temperature and 40 degrees C ambient temperature. We have developed a method to determine the optimum design and operating conditions for an automotive stack subject to this Q/Delta T constraint, and illustrate it by applying it to a state-of-the-art stack with nano-structured thin film ternary catalysts in the membrane electrode assemblies. In the illustrative example, stack coolant temperatures >90 degrees C, stack inlet pressures >2 atm, and cathode stoichiometries <2 are needed to satisfy the Q/Delta T constraint in a cost effective manner. The reference PEFC stack with 0.1 mg/cm(2) Pt loading in the cathode achieves 753 mW cm(-2) power density at the optimum conditions for heat rejection, compared to 964 mW cm(-2) in the laboratory cell at the same cell voltage (663 mV) and pressure (2.5 atm) but lower temperature (85 degrees C), higher cathode stoichiometry (2), and 100% relative humidity. (C) 2016 Elsevier B.V. All rights reserved. C1 [Ahluwalia, R. K.; Wang, X.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Steinbach, A. J.] 3M Fuel Cell Components Program, St Paul, MN USA. RP Ahluwalia, RK (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM walia@anl.gov FU Fuel Cell Technologies Office of the U.S. Department of Energy's (DOE) Office of Energy Efficiency and Renewable Energy; DOE, Office of Science Laboratory [DE-AC02-06CH11357] FX This work was supported by the Fuel Cell Technologies Office of the U.S. Department of Energy's (DOE) Office of Energy Efficiency and Renewable Energy. Dr. Nancy Garland is the DOE Technology Development Manager for this work. Argonne is a DOE, Office of Science Laboratory operated under Contract No. DE-AC02-06CH11357 by the UChicago Argonne, LLC. NR 15 TC 0 Z9 0 U1 3 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD MAR 31 PY 2016 VL 309 BP 178 EP 191 DI 10.1016/j.jpowsour.2016.01.060 PG 14 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DF7PD UT WOS:000371549100021 ER PT J AU Lin, YX Liu, Z Leung, K Chen, LQ Lu, P Qi, Y AF Lin, Yu-Xiao Liu, Zhe Leung, Kevin Chen, Long-Qing Lu, Peng Qi, Yue TI Connecting the irreversible capacity loss in Li-ion batteries with the electronic insulating properties of solid electrolyte interphase (SEI) components SO JOURNAL OF POWER SOURCES LA English DT Article DE Electron tunneling model; Density function theory; Solid electrolyte interphase; Lithium ion battery; Irreversible capacity loss; Stress and strain ID METAL WORK FUNCTION; MECHANICAL-PROPERTIES; GRAPHITE-ELECTRODES; NEGATIVE ELECTRODE; 1ST-PRINCIPLES CALCULATIONS; SURFACE-PROPERTIES; LITHIUM BATTERIES; SILICON ANODES; BAND-STRUCTURE; FILM FORMATION AB The formation and continuous growth of a solid electrolyte interphase (SEI) layer are responsible for the irreversible capacity loss of batteries in the initial and subsequent cycles, respectively. In this article, the electron tunneling barriers from Li metal through three insulating SEI components, namely Li2CO3, LiF and Li3PO4, are computed by density function theory (DFT) approaches. Based on electron tunneling theory, it is estimated that sufficient to block electron tunneling. It is also found that the band gap decreases under tension while the work function remains the same, and thus the tunneling barrier decreases under tension and increases under compression. A new parameter, eta, characterizing the average distances between anions, is proposed to unify the variation of band gap with strain under different loading conditions into a single linear function of eta. An analytical model based on the tunneling results is developed to connect the irreversible capacity loss, due to the Li ions consumed in forming these SEI component layers on the surface of negative electrodes. The agreement between the model predictions and experimental results suggests that only the initial irreversible capacity loss is due to the self-limiting electron tunneling property of the SEI. (C) 2016 Elsevier B.V. All rights reserved. C1 [Lin, Yu-Xiao; Qi, Yue] Michigan State Univ, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA. [Liu, Zhe; Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. [Leung, Kevin] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Lu, Peng] Gen Motors Res & Dev Ctr, Warren, MI 48090 USA. RP Qi, Y (reprint author), Michigan State Univ, Dept Chem Engn & Mat Sci, E Lansing, MI 48824 USA. EM yueqi@egr.msu.edu RI Qi, Yue/B-9869-2008; OI Qi, Yue/0000-0001-5331-1193 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences [DESC0001160]; NSF GOALI [CMMI-1235092]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX YXL, KL, and YQ acknowledge the support for degradation mechanism modeling as part of Nanostructures for Electrical Energy Storage (NEES), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award number DESC0001160. ZL, LQC, PL, and YQ are grateful for the financial support by NSF GOALI under CMMI-1235092. The computer simulations were carried out at MSU High Performance Computer Center (HPCC). Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 86 TC 3 Z9 3 U1 27 U2 114 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD MAR 31 PY 2016 VL 309 BP 221 EP 230 DI 10.1016/j.jpowsour.2016.01.078 PG 10 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DF7PD UT WOS:000371549100025 ER PT J AU Leu, BM Sage, JT AF Leu, Bogdan M. Sage, J. Timothy TI Stiffness, resilience, compressibility Atomic scale force spectroscopy of biomolecules SO HYPERFINE INTERACTIONS LA English DT Proceedings Paper CT International Conference on the Applications of the Mossbauer Effect (ICAME) CY SEP 13-18, 2015 CL Hamburg, GERMANY DE Nuclear resonance vibrational spectroscopy; Heme proteins; Flexibility ID RESONANCE VIBRATIONAL SPECTROSCOPY; NUCLEAR INELASTIC-SCATTERING; X-RAY-SCATTERING; CYTOCHROME-C; ACTIVE-SITE; MOSSBAUER-SPECTROSCOPY; NEUTRON-SCATTERING; GLOBULAR-PROTEINS; IRON; DYNAMICS AB The flexibility of a protein is an important component of its functionality. We use nuclear resonance vibrational spectroscopy (NRVS) to quantify the flexibility of the heme iron environment in the electron-carrying protein cytochrome c by measuring the stiffness and the resilience. These quantities are sensitive to structural differences between the active sites of different proteins, as illustrated by a comparative analysis with myoglobin. The elasticity of the entire protein, on the other hand, can be probed quantitatively from NRVS and high energy-resolution inelastic X-ray scattering (IXS) measurements, an approach that we used to extract the bulk modulus of cytochrome c. C1 [Leu, Bogdan M.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Sage, J. Timothy] Northeastern Univ, Dept Phys, Boston, MA 02115 USA. [Sage, J. Timothy] Northeastern Univ, Ctr Interdisciplinary Res Complex Syst, Boston, MA 02115 USA. RP Sage, JT (reprint author), Northeastern Univ, Dept Phys, Boston, MA 02115 USA.; Sage, JT (reprint author), Northeastern Univ, Ctr Interdisciplinary Res Complex Syst, Boston, MA 02115 USA. EM jtsage@neu.edu NR 57 TC 0 Z9 0 U1 0 U2 0 PU SPRINGER PI DORDRECHT PA VAN GODEWIJCKSTRAAT 30, 3311 GZ DORDRECHT, NETHERLANDS SN 0304-3843 J9 HYPERFINE INTERACT JI Hyperfine Interact. PD MAR 30 PY 2016 VL 237 AR 87 DI 10.1007/s10751-016-1275-8 PG 12 WC Physics, Atomic, Molecular & Chemical; Physics, Condensed Matter; Physics, Nuclear SC Physics GA DQ2GT UT WOS:000379021400001 ER PT J AU Jones, CG Stavila, V Conroy, MA Feng, P Slaughter, BV Ashley, CE Allendorf, MD AF Jones, Christopher G. Stavila, Vitalie Conroy, Marissa A. Feng, Patrick Slaughter, Brandon V. Ashley, Carlee E. Allendorf, Mark D. TI Versatile Synthesis and Fluorescent Labeling of ZIF-90 Nanoparticles for Biomedical Applications SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE ZIP-90; nanoparticle; surface functionalization; cellular uptake; bioimaging ID METAL-ORGANIC FRAMEWORKS; ZEOLITIC IMIDAZOLATE FRAMEWORKS; DRUG-DELIVERY; CELLULAR UPTAKE; CANCER; PLATFORM; FUNCTIONALIZATION; NANOMEDICINE; CYTOTOXICITY; NANOCRYSTALS AB We describe a versatile method for the synthesis and fluorescent labeling of ZIF-90 nanoparticles (NPs). Gram-scale quantities of NPs can be produced under mild conditions, circumventing the need for high temperatures and extended reaction periods required by existing procedures. Monitoring the reaction in situ using UV-vis spectroscopy reveals that ZIF-90 NP nucleation in solution starts within seconds. In addition to reporting a method to reproducibly form sub-100 nm ZIF-90 particles, we show that particles of various sizes can be produced, ranging from 30 to 1000 nm, by altering amine chemistry or reaction temperature. The presence of linker aldehyde groups on the NP surface allows for postsynthetic labeling with amine-functionalized fluorescent dyes, providing utility for imaging within biological systems. In vitro cell studies show that ZIF-90 NPs have a high rate of cellular internalization; provide finite degradation periods of the order of several weeks, and are biocompatible with six different cell lines (>90% viable when incubated with NPs for up to 7 days). These features highlight the potential for use of ZIF-90 nanostructures in bioimaging and targeted drug delivery applications. C1 [Stavila, Vitalie; Allendorf, Mark D.] Sandia Natl Labs, Livermore, CA 94551 USA. Sandia Natl Labs, Albuquerque, NM 87123 USA. RP Stavila, V; Allendorf, MD (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM vnstavi@sandia.gov; mdallen@sandia.gov FU Sandia Laboratory Directed Research and Development Program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Sandia Laboratory Directed Research and Development Program. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. The authors thank Dr. Christopher A. Lino for helpful discussions. NR 42 TC 3 Z9 3 U1 26 U2 72 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAR 30 PY 2016 VL 8 IS 12 BP 7623 EP 7630 DI 10.1021/acsami.5b11760 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DI5DQ UT WOS:000373519500003 PM 26950894 ER PT J AU Samant, SP Grabowski, CA Kisslinger, K Yager, KG Yuan, GC Satija, SK Durstock, MF Raghavan, D Karim, A AF Samant, Saumil P. Grabowski, Christopher A. Kisslinger, Kim Yager, Kevin G. Yuan, Guangcui Satija, Sushil K. Durstock, Michael F. Raghavan, Dharmaraj Karim, Alamgir TI Directed Self-Assembly of Block Copolymers for High Breakdown Strength Polymer Film Capacitors SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE block copolymer; directed self-assembly; cold zone annealing soft-shear; lamellae; breakdown strength; barrier effect; dielectric; capacitor ID THIN-FILMS; DIELECTRIC-BREAKDOWN; SOLID DIELECTRICS; ELECTRIC-FIELD; ENERGY; NANOCOMPOSITES; ORIENTATION; ALIGNMENT; NANOPARTICLES; PERFORMANCE AB Emerging needs for fast charge/discharge yet high-power, lightweight, and flexible electronics requires the use of polymer-film-based solid-state capacitors with high energy densities. Fast charge/discharge rates of film capacitors on the order of microseconds are not achievable with slower charging conventional batteries, supercapacitors and related hybrid technologies. However, the current energy densities of polymer film capacitors fall short of rising demand, and could be significantly enhanced by increasing the breakdown strength (E-BD) and dielectric permittivity (epsilon(r)) of the polymer films. Co-extruded two-homopolymer component multilayered films have demonstrated much promise in this regard showing higher E-BD over that of component polymers. Multilayered films can also help incorporate functional features besides energy storage, such as enhanced optical, mechanical, thermal and barrier properties. In this work, we report accomplishing multilayer, multicomponent block copolymer dielectric films (BCDF) with soft-shear driven highly oriented self-assembled lamellar diblock copolymers (BCP) as a novel application of this important class of self-assembling materials. Results of a model PS-b-PMMA system show similar to 50% enhancement in E-BD of self-assembled multilayer lamellar BCP films compared to unordered as-cast films, indicating that the breakdown is highly sensitive to the nanostructure of the BCP. The enhancement in E-BD is attributed to the "barrier effect", where the multiple interfaces between the lamellae block components act as barriers to the dielectric breakdown through the film. The increase in E-BD corresponds to more than doubling the energy storage capacity using a straightforward directed self-assembly strategy. This approach opens a new nanomaterial paradigm for designing high energy density dielectric materials. C1 [Samant, Saumil P.; Karim, Alamgir] Univ Akron, Dept Polymer Engn, Akron, OH 44325 USA. [Grabowski, Christopher A.; Durstock, Michael F.] Wright Patterson Air Force Base, Air Force Res Lab, Dayton, OH 45433 USA. [Kisslinger, Kim; Yager, Kevin G.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Yuan, Guangcui; Satija, Sushil K.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Raghavan, Dharmaraj] Howard Univ, Dept Chem, Washington, DC 20059 USA. RP Karim, A (reprint author), Univ Akron, Dept Polymer Engn, Akron, OH 44325 USA. EM alamgir@uakron.edu FU Air Force Office of Scientific Research (AFOSR) [FA9550-12-1-0306]; National Science Foundation (NSF) [DMR-1006421] FX This work was supported by Air Force Office of Scientific Research (AFOSR) under contract No. FA9550-12-1-0306 and the National Science Foundation (NSF) via Grant DMR-1006421. NR 43 TC 7 Z9 7 U1 19 U2 59 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAR 30 PY 2016 VL 8 IS 12 BP 7966 EP 7976 DI 10.1021/acsami.5b11851 PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DI5DQ UT WOS:000373519500043 PM 26942835 ER PT J AU Ng, RTL Maravelias, CT AF Ng, Rex T. L. Maravelias, Christos T. TI Design of Cellulosic Ethanol Supply Chains with Regional Depots SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID LIQUID TRANSPORTATION FUELS; EXPANSION AFEX PRETREATMENT; BIOMASS PROCESSING DEPOTS; LIGNOCELLULOSIC BIOMASS; CORN STOVER; TECHNOECONOMIC ANALYSIS; ENZYMATIC-HYDROLYSIS; INTEGRATED BIOMASS; MULTIOBJECTIVE OPTIMIZATION; PEROXIDE PRETREATMENT AB The conversion of lignocellulosic biomass to fuels has the potential to reduce our dependence on fossil fuels. To ensure biomass supply meets biofuel demand, it is necessary to have an effective biomass supply network. Toward this end, the concept of regional biomass processing depot, where biomass is pretreated and/or densified to a higher density intermediate, has been introduced to improve the performance of supply network in terms of costs and emissions. In this article, we develop a mixed-integer nonlinear programming model for the capacity and inventory planning problem of biofuels supply chain including depots. Importantly, the proposed model accounts for variable locations of depots, which is a subject that has not been studied in the literature. In addition, our models account for biomass selection and allocation, technology selection and capacity planning at depots and biorefineries, and biomass seasonality. C1 [Ng, Rex T. L.; Maravelias, Christos T.] Univ Wisconsin Madison, Dept Chem & Biol Engn, 1415 Engn Dr, Madison, WI 53706 USA. [Ng, Rex T. L.; Maravelias, Christos T.] Univ Wisconsin Madison, DOE Great Lakes Bioenergy Res Ctr, 1415 Engn Dr, Madison, WI 53706 USA. RP Maravelias, CT (reprint author), Univ Wisconsin Madison, Dept Chem & Biol Engn, 1415 Engn Dr, Madison, WI 53706 USA.; Maravelias, CT (reprint author), Univ Wisconsin Madison, DOE Great Lakes Bioenergy Res Ctr, 1415 Engn Dr, Madison, WI 53706 USA. EM christos.maravelias@wisc.edu RI Maravelias, Christos/B-1376-2009 OI Maravelias, Christos/0000-0002-4929-1748 FU DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science) [DE-FC02-07ER64494] FX This work was funded by the DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science DE-FC02-07ER64494). NR 104 TC 3 Z9 3 U1 5 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD MAR 30 PY 2016 VL 55 IS 12 BP 3420 EP 3432 DI 10.1021/acs.iecr.5b03677 PG 13 WC Engineering, Chemical SC Engineering GA DI5DO UT WOS:000373519300019 ER PT J AU Yao, Y Graziano, DJ Riddle, M Cresko, J Masanet, E AF Yao, Yuan Graziano, Diane J. Riddle, Matthew Cresko, Joe Masanet, Eric TI Prospective Energy Analysis of Emerging Technology Options for the United States Ethylene Industry SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID STRUCTURED PACKINGS; STEAM CRACKING; HOLLOW FIBERS; OLEFINS AB In this study, a bottom-up technology assessment model is constructed and applied to evaluate potential changes in the cradle-to-gate primary energy consumption and greenhouse gas (GHG) emissions of U.S. ethylene production in the future. Three chemical pathways are modeled: conventional natural gas to ethylene, shale gas to ethylene, and crude-oil-based naphtha to ethylene. State-of-the-art technology and five emerging technologies for the production of ethylene from natural gas are evaluated at the process and national levels. The results quantify the primary energy and GHG emissions reductions achievable with state-Of-the-art and emerging technologies, highlight the key parameters influencing their reduction potentials, and shed light on the implications of possible feedstock and technology shifts for U.S. ethylene production over the next several decades. The generalized and flexible modeling framework presented can be further used by energy, policy, and environmental analysts for assessing the savings potential of different technologies, making decisions in research and development investment, and strategic planning for meeting energy and emissions reduction goals. C1 [Yao, Yuan; Masanet, Eric] Northwestern Univ, Dept Chem & Biol Engn, 2145 Sheridan Rd, Evanston, IL 60201 USA. [Graziano, Diane J.] Argonne Natl Lab, Global Secur Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Riddle, Matthew] Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. [Cresko, Joe] US DOE, Adv Mfg Off, 1000 Independence Ave SW, Washington, DC 20585 USA. [Masanet, Eric] Northwestern Univ, Dept Mech Engn, 2145 Sheridan Rd, Evanston, IL 60201 USA. RP Yao, Y; Masanet, E (reprint author), Northwestern Univ, Dept Chem & Biol Engn, 2145 Sheridan Rd, Evanston, IL 60201 USA.; Masanet, E (reprint author), Northwestern Univ, Dept Mech Engn, 2145 Sheridan Rd, Evanston, IL 60201 USA. EM yuanyao2011@u.northwestern.edu; eric.masanet@northwestem.edu RI Masanet, Eric /I-5649-2012; Yao, Yuan/A-9150-2017 OI Yao, Yuan/0000-0001-9359-2030 FU Argonne, a U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX The submitted paper has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 52 TC 2 Z9 2 U1 1 U2 3 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD MAR 30 PY 2016 VL 55 IS 12 BP 3493 EP 3505 DI 10.1021/acs.iecr.5b03413 PG 13 WC Engineering, Chemical SC Engineering GA DI5DO UT WOS:000373519300024 ER PT J AU Blennow, M Coloma, P Fernandez-Martinez, E AF Blennow, Mattias Coloma, Pilar Fernandez-Martinez, Enrique TI The MOMENT to search for CP violation SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE CP violation; Neutrino Physics ID NEUTRINO OSCILLATION EXPERIMENTS; LINE-EXPERIMENT-SIMULATOR; BARYON ASYMMETRY; ELEMENTARY-PARTICLES; UNIFIED MODEL; PHYSICS AB In this letter, we analyze for the first time the physics reach in terms of sensitivity to leptonic CP violation of the proposed MuOn-decay MEdium baseline NeuTrino beam (MOMENT) experiment, a novel neutrino oscillation facility that would operate with neutrinos from muon decay. Apart from obtaining a sufficiently intense flux, the bottlenecks to the physics reach of this experiment will be achieving a high enough suppression of the atmospheric background and, particularly, attaining a sufficient level of charge identification. We thus present our results as a function of these two factors. As for the detector, we consider a very massive Gd-doped Water Cherenkov detector. We find that MOMENT will be competitive with other currently planned future oscillation experiments if a charge identification of at least 80 % can be achieved at the same time that the atmospheric background can be suppressed by at least a factor of ten. We also find a large synergy of MOMENT with the current generation of neutrino oscillation experiments, T2K and NOvA, which significantly enhances its final sensitivity. C1 [Blennow, Mattias] KTH Royal Inst Technol, Albanova Univ Ctr, Sch Engn Sci, Dept Theoret Phys, S-10691 Stockholm, Sweden. [Coloma, Pilar] Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA. [Fernandez-Martinez, Enrique] Univ Autonoma Madrid, Dept Fis Teor, E-28049 Madrid, Spain. [Fernandez-Martinez, Enrique] Inst Fis Teor UAM CSIC, Calle Nicolas Cabrera 13-15, E-28049 Madrid, Spain. RP Blennow, M (reprint author), KTH Royal Inst Technol, Albanova Univ Ctr, Sch Engn Sci, Dept Theoret Phys, S-10691 Stockholm, Sweden.; Coloma, P (reprint author), Fermilab Natl Accelerator Lab, Dept Theoret Phys, POB 500, Batavia, IL 60510 USA.; Fernandez-Martinez, E (reprint author), Univ Autonoma Madrid, Dept Fis Teor, E-28049 Madrid, Spain.; Fernandez-Martinez, E (reprint author), Inst Fis Teor UAM CSIC, Calle Nicolas Cabrera 13-15, E-28049 Madrid, Spain. EM emb@kth.se; pcoloma@fnal.gov; enrique.fernandez-martinez@uam.es FU Goran Gustafsson Foundation; European Union through the ITN INVISIBLES (Marie Curie Actions) [PITN-GA-2011-289442-INVISIBLES]; EU through the FP7 Marie Curie Actions CIG NeuProbes [PCIG11-GA-2012-321582]; Spanish MINECO through the "Ramon y Cajal" programme [RYC2011-07710, FPA2009-09017]; Spanish MINECO through the Centro de excelencia Severo Ochoa Program [SEV-2012-0249]; Mainz Institute for Theoretical Physics; United States Department of Energy [DE-AC02-07CH11359] FX The work of MB was supported by the Goran Gustafsson Foundation. PC and EFM acknowledge financial support from the European Union through the ITN INVISIBLES (Marie Curie Actions, PITN-GA-2011-289442-INVISIBLES). EFM also acknowledges support from the EU through the FP7 Marie Curie Actions CIG NeuProbes (PCIG11-GA-2012-321582) and the Spanish MINECO through the "Ramon y Cajal" programme (RYC2011-07710) and the project FPA2009-09017. MB and EFM were also supported by the Spanish MINECO through the Centro de excelencia Severo Ochoa Program under grant SEV-2012-0249. MB would also like to thank the Instituto de Fisica Teorica, Madrid, for warm hospitality during the time when this work was initiated. PC would like to thank the Mainz Institute for Theoretical Physics for hospitality and partial support during completion of this work. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. NR 45 TC 5 Z9 5 U1 1 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 30 PY 2016 IS 3 AR 197 DI 10.1007/JHEP03(2016)197 PG 11 WC Physics, Particles & Fields SC Physics GA DI3II UT WOS:000373391900006 ER PT J AU Platero-Prats, AE Mavrandonakis, A Gallington, LC Liu, YY Hupp, JT Farha, OK Cramer, CJ Chapmant, KW AF Platero-Prats, Ana E. Mavrandonakis, Andreas Gallington, Leighanne C. Liu, Yangyang Hupp, Joseph T. Farha, Omar K. Cramer, Christopher J. Chapman, Karena W. TI Structural Transitions of the Metal -Oxide Nodes within Metal- Organic Frameworks: On the Local Structures of NU-1000 and UiO-66 SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID ATOMIC LAYER DEPOSITION; PHASE-TRANSITIONS; FUTURE-TRENDS; CATALYST; ZIRCONIA; STABILITY; COMPLEXES; TRANSFORMATION; DESTRUCTION; DIFFRACTION AB In situ pair distribution function (PDF) analyses and density functional theory (DFT) computations are used to probe local structural transitions of M6O8 nodes found in two metal organic frameworks (MOFs), NU-1000 and UiO-66, for M = Zr, Hf. Such transitions are found to occur without change to the global framework symmetry at temperatures within a range relevant to many potential MOF applications. For the particular M-6(O)(8) nodes studied here, the observed distortions can be mapped to polymorphic forms known for bulk ZrO2. In the MOF framework, however, node distortions are found to occur at substantially lower temperature than analogous distortions in bulk ZrO2 owing to the nanoscale nature of the former. C1 [Platero-Prats, Ana E.; Gallington, Leighanne C.; Chapman, Karena W.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mavrandonakis, Andreas; Cramer, Christopher J.] Univ Minnesota, Dept Chem, Chem Theory Ctr, Minneapolis, MN 55455 USA. [Mavrandonakis, Andreas; Cramer, Christopher J.] Univ Minnesota, Supercomp Inst, Minneapolis, MN 55455 USA. [Liu, Yangyang; Hupp, Joseph T.; Farha, Omar K.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Farha, Omar K.] King Abdulaziz Univ, Fac Sci, Dept Chem, Jeddah 21589, Saudi Arabia. RP Chapmant, KW (reprint author), Argonne Natl Lab, Adv Photon Source, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM chapmank@aps.anl.gov RI Mavrantonakis, Andreas/J-6274-2014; Gallington, Leighanne/G-9341-2011; Cramer, Christopher/B-6179-2011; Platero-Prats, Ana Eva/B-2870-2017; Faculty of, Sciences, KAU/E-7305-2017 OI Mavrantonakis, Andreas/0000-0002-5053-8154; Gallington, Leighanne/0000-0002-0383-7522; Cramer, Christopher/0000-0001-5048-1859; Platero-Prats, Ana Eva/0000-0002-2248-2739; FU Inorganometallic Catalysis Design Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0012702]; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357]; Ministry of Economy and Knowledge from the Catalan Government [BP-DGR 2014] FX This work was supported as part of the Inorganometallic Catalysis Design Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award No. DE-SC0012702. Work done at Argonne was performed using the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. We thank Mr. Joshua Borycz for technical assistance with some of the periodic calculations reported herein and also the Minnesota Supercomputing Institute (MSI) at the University of Minnesota for providing resources that contributed to the research results reported within this paper. A.E.P.P. acknowledges a Beatriu de Pinos fellowship (BP-DGR 2014) from the Ministry of Economy and Knowledge from the Catalan Government. NR 50 TC 9 Z9 9 U1 54 U2 141 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 30 PY 2016 VL 138 IS 12 BP 4178 EP 4185 DI 10.1021/jacs.6b00069 PG 8 WC Chemistry, Multidisciplinary SC Chemistry GA DI5DJ UT WOS:000373518800037 PM 26926342 ER PT J AU Xu, Y Yu, JR Cao, YJ Lu, XN Yu, JQ AF Xu, Yong Yu, Jingrong Cao, Yijia Lu, Xiaonan Yu, Jiaqi TI Double resonant output filter to eliminating the tradeoff between bandwidth and switching ripple in shunt active power filters SO IET POWER ELECTRONICS LA English DT Article ID VOLTAGE-SOURCE INVERTER; DESIGN AB Since shunt active power filters (SAPFs) are designed to inject harmonic current, its bandwidth should be much wider compared to regular inverters. LCL filters are commonly employed in regular inverters. However, it cannot completely meet the requirements of SAPF due to its filtering performance and the impact on system stability. This study proposes a novel double resonant LCL (DR-LCL) filter for SAPFs. Derived from the conventional LCL filters, one RC damping circuit and two LC resonant circuits are employed in the proposed filter. Meanwhile, a resistor is connected in parallel with the grid-side inductor. The mutual impact among different components of the filter is discussed, and the stability of SAPF with DR-LCL filter is studied. This DR-LCL filter can not only inherit the advantages of LCL filters, but also eliminate the tradeoff between bandwidth and switching ripple in SAPFs. Finally, the design principle of the proposed output filter is presented and the parameters of the filter are applied to a 66 kW three-phase three-wire SAPF prototype. Simulation and experimental results verify the feasibility of DR-LCL filter. C1 [Xu, Yong; Cao, Yijia; Yu, Jiaqi] Hunan Univ, Coll Elect & Informat Engn, Changsha 410082, Hunan, Peoples R China. [Yu, Jingrong] Cent S Univ, Sch Informat Sci & Engn, Changsha, Hunan, Peoples R China. [Lu, Xiaonan] Argonne Natl Lab, Div Energy Syst, Lemont, IL USA. RP Yu, JR (reprint author), Cent S Univ, Sch Informat Sci & Engn, Changsha, Hunan, Peoples R China. EM jingrong_yu@126.com FU National Science and Technology Support Program of China [2013BAA01B01]; Key Program of the National Natural Science Foundation of China [61233008] FX This work was supported by the National Science and Technology Support Program of China under Grant 2013BAA01B01 and by the Key Program of the National Natural Science Foundation of China (61233008). NR 19 TC 0 Z9 0 U1 0 U2 1 PU INST ENGINEERING TECHNOLOGY-IET PI HERTFORD PA MICHAEL FARADAY HOUSE SIX HILLS WAY STEVENAGE, HERTFORD SG1 2AY, ENGLAND SN 1755-4535 EI 1755-4543 J9 IET POWER ELECTRON JI IET Power Electron. PD MAR 30 PY 2016 VL 9 IS 4 BP 846 EP 854 DI 10.1049/iet-pel.2015.0005 PG 9 WC Engineering, Electrical & Electronic SC Engineering GA DH5RF UT WOS:000372848800025 ER PT J AU Adamson, P Anghel, I Aurisano, A Barr, G Bishai, M Blake, A Bock, GJ Bogert, D Cao, SV Carroll, TJ Castromonte, CM Chen, R Childress, S Coelho, JAB Corwin, L Cronin-Hennessy, D de Jong, JK De Rijck, S Devan, AV Devenish, NE Diwan, MV Escobar, CO Evans, JJ Falk, E Feldman, GJ Flanagan, W Frohne, MV Gabrielyan, M Gallagher, HR Germani, S Gomes, RA Goodman, MC Gouffon, P Graf, N Gran, R Grzelak, K Habig, A Hahn, SR Hartnell, J Hatcher, R Holin, A Huang, J Hylen, J Irwin, GM Isvan, Z James, C Jensen, D Kafka, T Kasahara, SMS Koizumi, G Kordosky, M Kreymer, A Lang, K Ling, J Litchfield, PJ Lucas, P Mann, WA Marshak, ML Mayer, N McGivern, C Medeiros, MM Mehdiyev, R Meier, JR Messier, MD Miller, WH Mishra, SR Sher, SM Moore, CD Mualem, L Musser, J Naples, D Nelson, JK Newman, HB Nichol, RJ Nowak, JA O'Connor, J Orchanian, M Pahlka, RB Paley, J Patterson, RB Pawloski, G Perch, A Pfutzner, MM Phan, DD Phan-Budd, S Plunkett, RK Poonthottathil, N Qiu, X Radovic, A Rebel, B Rosenfeld, C Rubin, HA Sail, P Sanchez, MC Schneps, J Schreckenberger, A Schreiner, P Sharma, R Sousa, A Tagg, N Talaga, RL Thomas, J Thomson, MA Tian, X Timmons, A Todd, J Tognini, SC Toner, R Torretta, D Tzanakos, G Urheim, J Vahle, P Viren, B Weber, A Webb, RC White, C Whitehead, L Whitehead, LH Wojcicki, SG Zwaska, R AF Adamson, P. Anghel, I. Aurisano, A. Barr, G. Bishai, M. Blake, A. Bock, G. J. Bogert, D. Cao, S. V. Carroll, T. J. Castromonte, C. M. Chen, R. Childress, S. Coelho, J. A. B. Corwin, L. Cronin-Hennessy, D. de Jong, J. K. De Rijck, S. Devan, A. V. Devenish, N. E. Diwan, M. V. Escobar, C. O. Evans, J. J. Falk, E. Feldman, G. J. Flanagan, W. Frohne, M. V. Gabrielyan, M. Gallagher, H. R. Germani, S. Gomes, R. A. Goodman, M. C. Gouffon, P. Graf, N. Gran, R. Grzelak, K. Habig, A. Hahn, S. R. Hartnell, J. Hatcher, R. Holin, A. Huang, J. Hylen, J. Irwin, G. M. Isvan, Z. James, C. Jensen, D. Kafka, T. Kasahara, S. M. S. Koizumi, G. Kordosky, M. Kreymer, A. Lang, K. Ling, J. Litchfield, P. J. Lucas, P. Mann, W. A. Marshak, M. L. Mayer, N. McGivern, C. Medeiros, M. M. Mehdiyev, R. Meier, J. R. Messier, M. D. Miller, W. H. Mishra, S. R. Sher, S. Moed Moore, C. D. Mualem, L. Musser, J. Naples, D. Nelson, J. K. Newman, H. B. Nichol, R. J. Nowak, J. A. O'Connor, J. Orchanian, M. Pahlka, R. B. Paley, J. Patterson, R. B. Pawloski, G. Perch, A. Pfuetzner, M. M. Phan, D. D. Phan-Budd, S. Plunkett, R. K. Poonthottathil, N. Qiu, X. Radovic, A. Rebel, B. Rosenfeld, C. Rubin, H. A. Sail, P. Sanchez, M. C. Schneps, J. Schreckenberger, A. Schreiner, P. Sharma, R. Sousa, A. Tagg, N. Talaga, R. L. Thomas, J. Thomson, M. A. Tian, X. Timmons, A. Todd, J. Tognini, S. C. Toner, R. Torretta, D. Tzanakos, G. Urheim, J. Vahle, P. Viren, B. Weber, A. Webb, R. C. White, C. Whitehead, L. Whitehead, L. H. Wojcicki, S. G. Zwaska, R. CA MINOS Collaboration TI Measurement of the multiple-muon charge ratio in the MINOS Far Detector SO PHYSICAL REVIEW D LA English DT Article ID TEV; SPECTRUM AB The charge ratio, R-mu = N mu+/N mu-, for cosmogenic multiple-muon events observed at an underground depth of 2070 mwe has been measured using the magnetized MINOS Far Detector. The multiple-muon events, recorded nearly continuously from August 2003 until April 2012, comprise two independent data sets imaged with opposite magnetic field polarities, the comparison of which allows the systematic uncertainties of the measurement to be minimized. The multiple-muon charge ratio is determined to be R mu = 1.104 +/- 0.006(stat)(-0.010)(+0.009) (syst). This measurement complements previous determinations of single-muon and multiple-muon charge ratios at underground sites and serves to constrain models of cosmic-ray interactions at TeV energies. C1 [Anghel, I.; Goodman, M. C.; Paley, J.; Phan-Budd, S.; Sanchez, M. C.; Schreiner, P.; Talaga, R. L.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Bishai, M.; Diwan, M. V.; Isvan, Z.; Ling, J.; Viren, B.; Whitehead, L.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Mualem, L.; Newman, H. B.; Orchanian, M.; Patterson, R. B.] CALTECH, Lauritsen Lab, Pasadena, CA 91125 USA. [Blake, A.; Thomson, M. A.; Toner, R.] Univ Cambridge, Cavendish Lab, Madingley Rd, Cambridge CB3 0HE, England. [Escobar, C. O.] Univ Estadual Campinas, IFGW UNICAMP, CP 6165, BR-13083970 Campinas, SP, Brazil. [Aurisano, A.; Sousa, A.; Todd, J.] Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. [Adamson, P.; Bock, G. J.; Bogert, D.; Childress, S.; Hahn, S. R.; Hatcher, R.; Hylen, J.; James, C.; Jensen, D.; Koizumi, G.; Kreymer, A.; Lucas, P.; Sher, S. Moed; Moore, C. D.; Pahlka, R. B.; Plunkett, R. K.; Poonthottathil, N.; Rebel, B.; Sharma, R.; Torretta, D.; Zwaska, R.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Castromonte, C. M.; Gomes, R. A.; Medeiros, M. M.; Tognini, S. C.] Univ Fed Goias, Inst Fis, BR-74690900 Goiania, Go, Brazil. [Feldman, G. J.; Sousa, A.; Toner, R.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Frohne, M. V.] Coll Holy Cross, Notre Dame, IN 46556 USA. [Whitehead, L.] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Graf, N.; Rubin, H. A.; White, C.] Illinois Inst Technol, Dept Phys, Chicago, IL 60616 USA. [Corwin, L.; Mayer, N.; Messier, M. D.; Musser, J.; Urheim, J.] Indiana Univ, Bloomington, IN 47405 USA. [Anghel, I.; Sanchez, M. C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Germani, S.; Holin, A.; Nichol, R. J.; O'Connor, J.; Perch, A.; Pfuetzner, M. M.; Thomas, J.; Whitehead, L. H.] UCL, Dept Phys & Astron, Mortimer St, London WC1E 6BT, England. [Chen, R.; Evans, J. J.; Timmons, A.] Univ Manchester, Sch Phys & Astron, Oxford Rd, Manchester M13 9PL, Lancs, England. [Cronin-Hennessy, D.; Gabrielyan, M.; Kasahara, S. M. S.; Litchfield, P. J.; Marshak, M. L.; Meier, J. R.; Miller, W. H.; Nowak, J. A.; Pawloski, G.; Schreckenberger, A.] Univ Minnesota, Minneapolis, MN 55455 USA. [Gran, R.; Habig, A.] Univ Minnesota Duluth, Dept Phys, Duluth, MN 55812 USA. [Tagg, N.] Otterbein Coll, Westerville, OH 43081 USA. [Barr, G.; de Jong, J. K.; Weber, A.] Univ Oxford, Subdept Particle Phys, Oxford OX1 3RH, England. [Graf, N.; Isvan, Z.; McGivern, C.; Naples, D.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Litchfield, P. J.; Weber, A.] Rutherford Appleton Lab, Sci & Technol Facil Council, Didcot OX11 0QX, Oxon, England. [Gouffon, P.] Univ Sao Paulo, Inst Fis, CP 66318, BR-05315970 Sao Paulo, SP, Brazil. [Mishra, S. R.; Rosenfeld, C.; Tian, X.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Irwin, G. M.; Pawloski, G.; Qiu, X.; Wojcicki, S. G.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Devenish, N. E.; Falk, E.; Hartnell, J.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. [Webb, R. C.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Cao, S. V.; Carroll, T. J.; De Rijck, S.; Flanagan, W.; Huang, J.; Lang, K.; Mehdiyev, R.; Phan, D. D.; Sail, P.; Schreckenberger, A.] Univ Texas Austin, Dept Phys, 1 Univ Stn C1600, Austin, TX 78712 USA. [Coelho, J. A. B.; Gallagher, H. R.; Kafka, T.; Mann, W. A.; Mayer, N.; Schneps, J.] Tufts Univ, Dept Phys, Medford, MA 02155 USA. [Grzelak, K.] Univ Warsaw, Dept Phys, Pasteura 5, PL-02093 Warsaw, Poland. [Devan, A. V.; Kordosky, M.; Nelson, J. K.; Radovic, A.; Vahle, P.] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Tzanakos, G.] Univ Athens, Dept Phys, GR-15771 Athens, Greece. [Corwin, L.] Univ Lancaster, Lancaster LA1 4YB, England. [Frohne, M. V.; Tzanakos, G.] South Dakota Sch Mines & Technol, Rapid City, SD 57701 USA. RP Adamson, P (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RI Gomes, Ricardo/B-6899-2008; Gouffon, Philippe/I-4549-2012; Nowak, Jaroslaw/P-2502-2016; Ling, Jiajie/I-9173-2014; OI Weber, Alfons/0000-0002-8222-6681; Gomes, Ricardo/0000-0003-0278-4876; Gouffon, Philippe/0000-0001-7511-4115; Nowak, Jaroslaw/0000-0001-8637-5433; Ling, Jiajie/0000-0003-2982-0670; Corwin, Luke/0000-0001-7143-3821; Hartnell, Jeffrey/0000-0002-1744-7955; Castromonte Flores, Cesar Manuel/0000-0002-9559-3704 FU U.S. DOE; U.K. STFC; U.S. NSF; State and University of Minnesota; University of Athens, Greece; Brazil FAPESP; Brazil CAPES; Brazil CNPq FX This work was supported by the U.S. DOE, the U.K. STFC, the U.S. NSF, the State and University of Minnesota, the University of Athens, Greece, and Brazil's FAPESP, CAPES and CNPq. We are grateful to the Texas Advanced Computer Center, the Minnesota Department of Natural Resources, the crew of Soudan Underground Laboratory, and the Fermilab personnel for their contributions to this effort. NR 25 TC 1 Z9 1 U1 6 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 30 PY 2016 VL 93 IS 5 AR 052017 DI 10.1103/PhysRevD.93.052017 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH9HH UT WOS:000373106500001 ER PT J AU Sedlacek, JA Kim, E Rittenhouse, ST Weck, PF Sadeghpour, HR Shaffer, JP AF Sedlacek, J. A. Kim, E. Rittenhouse, S. T. Weck, P. F. Sadeghpour, H. R. Shaffer, J. P. TI Electric Field Cancellation on Quartz by Rb Adsorbate-Induced Negative Electron Affinity SO PHYSICAL REVIEW LETTERS LA English DT Article ID SILICON DIOXIDE; SURFACE-STATES; LIQUID-HELIUM; RYDBERG ATOMS; ALPHA-QUARTZ; VAPOR; DIAMOND; SYSTEMS; CESIUM; LAYERS AB We investigate the (0001) surface of single crystal quartz with a submonolayer of Rb adsorbates. Using Rydberg atom electromagnetically induced transparency, we investigate the electric fields resulting from Rb adsorbed on the quartz surface, and measure the activation energy of the Rb adsorbates. We show that the adsorbed Rb induces negative electron affinity (NEA) on the quartz surface. The NEA surface allows low energy electrons to bind to the surface and cancel the electric field from the Rb adsorbates. Our results will be important for integrating Rydberg atoms into hybrid quantum systems, as fundamental probes of atom-surface interactions, and for studies of 2D electron gases bound to surfaces. C1 [Sedlacek, J. A.; Shaffer, J. P.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Kim, E.] Univ Nevada, Dept Phys & Astron, Las Vegas, NV 89154 USA. [Rittenhouse, S. T.] Western Washington Univ, Dept Phys & Astron, Bellingham, WA 98225 USA. [Rittenhouse, S. T.] US Naval Acad, Dept Phys, Annapolis, MD 21402 USA. [Weck, P. F.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Sadeghpour, H. R.] Harvard Smithsonian Ctr Astrophys, Inst Theoret Atom & Mol Phys, Cambridge, MA 02138 USA. RP Shaffer, JP (reprint author), Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. EM shaffer@nhn.ou.edu FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; DARPA Quasar program by a grant through ARO [60181-PH-DRP]; AFOSR [FA9550-12-1-0282]; NSF [PHY-1104424, NSF PHY-1516421]; NSF grant through ITAMP at the Harvard-Smithsonian Center for Astrophysics FX Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. This work was supported by the DARPA Quasar program by a grant through ARO (Grant No. 60181-PH-DRP), AFOSR (Grant No. FA9550-12-1-0282), NSF (Grants No. PHY-1104424) and No. NSF PHY-1516421) and an NSF grant through ITAMP at the Harvard-Smithsonian Center for Astrophysics. The authors thank Tilman Pfau for useful discussions. NR 67 TC 6 Z9 6 U1 4 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 30 PY 2016 VL 116 IS 13 AR 133201 DI 10.1103/PhysRevLett.116.133201 PG 7 WC Physics, Multidisciplinary SC Physics GA DH9EP UT WOS:000373099500006 PM 27081976 ER PT J AU Chen, XF Liu, GQ Wong, YLE Deng, LL Wang, Z Li, W Chan, TWD AF Chen, Xiangfeng Liu, Guoqiang Wong, Y. L. Elaine Deng, Liulin Wang, Ze Li, Wan Chan, T. -W. Dominic TI Dissociation of trivalent metal ion (Al3+, Ga3+, In3+ and Rh3+)-peptide complexes under electron capture dissociation conditions SO RAPID COMMUNICATIONS IN MASS SPECTROMETRY LA English DT Article ID CHARGED PROTEIN CATIONS; MASS-SPECTROMETRY; PEPTIDE COMPLEXES; GAS-PHASE; RADICALS; BEHAVIOR; STATES AB RationaleThe electron capture dissociation (ECD) of proteins/peptides is affected by the nature of charge carrier. It has been reported that transition metal ions could tune the ECD pathway of peptides. To further explore the charge carrier effect of metal ions, ECD of peptides adducted with trivalent transition metal ions, including group IIIB (Al3+, Ga3+, and In3+) and Rh3+, were investigated and compared with that of the lanthanide ion (Ln(3+)). MethodsBradykinin-derived peptides were used as model peptides to probe the dissociation pathways. The ECD experiments were performed on a Bruker APEX III 4.7T Fourier transform ion cyclotron resonance (FTICR) mass spectrometer. ResultsTypical c-/z-ions with and without metal ions were observed in the ECD of peptides adducted with Group IIIB metal ions as charge carriers. Connection of non-metalated c-ions and metalated z-ions at the position of the serine residue indicated that serine is one of the binding sites of the metal ion on the model peptides. Typical slow heating ions, including metalated a-/b-ions and non-metalated y-ions, were generated in ECD of Rh3+-adducted peptides. ConclusionsBased on the experimental results, it is proposed that (i) for Group IIIB metal ion-peptide complexes, the incoming electron is captured by the proton in the salt-bridge structures of precursor ions; (ii) for Rh3+-peptide complexes, the incoming electron is captured by the metal ion due to the formation of charge-solvated precursor ions formed through arginine residue-metal coordination. Our results indicate that the heterogeneity of precursor ions plays an important role for the ECD of metalated peptides. Copyright (c) 2016 John Wiley & Sons, Ltd. C1 [Chen, Xiangfeng; Liu, Guoqiang; Wong, Y. L. Elaine; Deng, Liulin; Wang, Ze; Li, Wan; Chan, T. -W. Dominic] Chinese Univ Hong Kong, Dept Chem, Shatin, Hong Kong, Peoples R China. [Chen, Xiangfeng] Shandong Acad Sci, Jinan, Shandong, Peoples R China. [Deng, Liulin] Pacific NW Natl Lab, Div Biol Sci, Washington, DC USA. [Deng, Liulin] Pacific NW Natl Lab, Environm Mol Sci Lab, Washington, DC USA. RP Chen, XF; Chan, TWD (reprint author), Chinese Univ Hong Kong, Dept Chem, Shatin, Hong Kong, Peoples R China.; Chen, XF (reprint author), Shandong Acad Sci, Jinan, Shandong, Peoples R China. EM xiangfchensdas@163.com; twdchan@cuhk.edu.hk OI Chen, Xiangfeng/0000-0001-9266-7707 FU National Natural Science Foundation of China [NSFC 21205071]; Research Grant Council of the Hong Kong Special Administrative Region [2060351]; Natural Science Foundation of Shandong Province [ZR2012BQ009]; Funds for Fostering Distinguished Young Scholar of Shandong Academy of Sciences FX The authors would like to acknowledge the financial support from National Natural Science Foundation of China (NSFC 21205071), Research Grant Council of the Hong Kong Special Administrative Region (Research Grant Direct Allocation, Ref. 2060351), Natural Science Foundation of Shandong Province (ZR2012BQ009), and Funds for Fostering Distinguished Young Scholar of Shandong Academy of Sciences. NR 30 TC 2 Z9 2 U1 5 U2 22 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0951-4198 EI 1097-0231 J9 RAPID COMMUN MASS SP JI Rapid Commun. Mass Spectrom. PD MAR 30 PY 2016 VL 30 IS 6 BP 705 EP 710 DI 10.1002/rcm.7502 PG 6 WC Biochemical Research Methods; Chemistry, Analytical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA DD8MT UT WOS:000370181700006 PM 26864523 ER PT J AU Ho, ME Quek, SI True, LD Seiler, R Fleischmann, A Bagryanova, L Kim, SR Chia, D Goodglick, L Shimizu, Y Rosser, CJ Gao, YQ Liu, AY AF Ho, Melissa E. Quek, Sue-Ing True, Lawrence D. Seiler, Roland Fleischmann, Achim Bagryanova, Lora Kim, Sara R. Chia, David Goodglick, Lee Shimizu, Yoshiko Rosser, Charles J. Gao, Yuqian Liu, Alvin Y. TI Bladder cancer cells secrete while normal bladder cells express but do not secrete AGR2 SO ONCOTARGET LA English DT Article DE secreted AGR2; bladder cancer; subcellular localization; urine biomarker ID PROSTATE-CANCER; CD10 EXPRESSION; GENE-EXPRESSION; UROTHELIAL CARCINOMA; PANCREATIC-CANCER; BIOMARKER; PROTEINS; SURFACE; URINE; TRANSCRIPTOMES AB Anterior gradient 2 (AGR2) is a cancer-associated secreted protein found predominantly in adenocarcinomas. Given its ubiquity in solid tumors, cancer-secreted AGR2 could be a useful biomarker in urine or blood for early detection. However, normal organs express and might also secrete AGR2, which would impact its utility as a cancer biomarker. Uniform AGR2 expression is found in the normal bladder urothelium. Little AGR2 is secreted by the urothelial cells as no measurable amounts could be detected in urine. The urinary proteomes of healthy people contain no listing for AGR2. Likewise, the blood proteomes of healthy people also contain no significant peptide counts for AGR2 suggesting little urothelial secretion into capillaries of the lamina propria. Expression of AGR2 is lost in urothelial carcinoma, with only 25% of primary tumors observed to retain AGR2 expression in a cohort of lymph node-positive cases. AGR2 is secreted by the urothelial carcinoma cells as urinary AGR2 was measured in the voided urine of 25% of the cases analyzed in a cohort of cancer vs. non-cancer patients. The fraction of AGR2-positive urine samples was consistent with the fraction of urothelial carcinoma that stained positive for AGR2. Since cancer cells secrete AGR2 while normal cells do not, its measurement in body fluids could be used to indicate tumor presence. Furthermore, AGR2 has also been found on the cell surface of cancer cells. Taken together, secretion and cell surface localization of AGR2 are characteristic of cancer, while expression of AGR2 by itself is not. C1 [Ho, Melissa E.; Quek, Sue-Ing; Liu, Alvin Y.] Univ Washington, Dept Urol, Inst Stem Cell & Regenerat Med, Seattle, WA 98195 USA. [True, Lawrence D.] Univ Washington, Dept Pathol, Seattle, WA 98195 USA. [Seiler, Roland] Univ Hosp Bern, Dept Urol, CH-3010 Bern, Switzerland. [Fleischmann, Achim] Univ Hosp Bern, Inst Pathol, CH-3010 Bern, Switzerland. [Bagryanova, Lora; Kim, Sara R.; Chia, David; Goodglick, Lee] Univ Calif Los Angeles, David Geffen Sch Med, Dept Pathol & Lab Med, Los Angeles, CA 90095 USA. [Kim, Sara R.; Chia, David; Goodglick, Lee] Univ Calif Los Angeles, David Geffen Sch Med, Jonsson Comprehens Canc Ctr, Los Angeles, CA 90095 USA. [Shimizu, Yoshiko; Rosser, Charles J.] Univ Hawaii, Ctr Canc, Honolulu, HI 96822 USA. [Gao, Yuqian] Pacific NW Natl Lab, Biol Sci Div, Richland, WA 99352 USA. [Ho, Melissa E.] Univ Calif San Francisco, Med Ctr, San Francisco, CA USA. [Quek, Sue-Ing] Singapore Polytech, Ctr Biomed & Life Sci, Singapore, Singapore. RP Liu, AY (reprint author), Univ Washington, Dept Urol, Inst Stem Cell & Regenerat Med, Seattle, WA 98195 USA. EM aliu@uw.edu FU NCI-EDRN [CA86366, CA111244] FX This work was supported in part by NCI-EDRN grants CA86366 (DC, LG) and CA111244 (AL). NR 35 TC 1 Z9 1 U1 1 U2 1 PU IMPACT JOURNALS LLC PI ALBANY PA 6211 TIPTON HOUSE, STE 6, ALBANY, NY 12203 USA SN 1949-2553 J9 ONCOTARGET JI Oncotarget PD MAR 29 PY 2016 VL 7 IS 13 BP 15747 EP 15756 PG 10 WC Oncology; Cell Biology SC Oncology; Cell Biology GA DL5QW UT WOS:000375692900036 PM 26894971 ER PT J AU Sullivan, RJ Kim, J Hoyt, C Silks, LA Schlaf, M AF Sullivan, Ryan J. Kim, Jin Hoyt, Caroline Silks, Louis A. (Pete), III Schlaf, Marcel TI Ruthenium-8-quinolinethiolate-phenylterpyridine versus ruthenium-bipyridine-phenyl-terpyridine complexes as homogeneous water and high temperature stable hydrogenation catalysts for biomass-derived substrates SO POLYHEDRON LA English DT Article DE Homogeneous catalysis; Hydrodeoxygenation; Biomass; Ruthenium complexes; Aqueous media ID MOLECULAR-ORBITAL METHODS; POLARIZABLE CONTINUUM MODEL; BASIS-SETS; TRANSITION-ELEMENTS; HYDRIDE ION; DIHYDROGEN; 2,5-DIMETHYLFURAN; MECHANISM; HOMOLOGS; KINETICS AB [(4'-Ph-terpy)(bipy)Ru(L)](OTf)(n) and [(4'-Ph-terpy)(quS)Ru(L)](OTf)(n) (n = 0 or 1 depending on the charge of L, L = labile ligand, e.g., H2O, CH3CN or OTf, bipy = 2,2'-bipyridine, quS = quinoline-8-thiolate) have been evaluated as catalysts for the hydrogenation of the biomass-derivable C6-substrates 2,5-dimethylfuran (obtainable from 5-hydroxymethylfurfural) and 2,5-hexanedione (the hydrolysis product of 2,5-dimethylfuran). Operating in aqueous acidic medium at T = 175-225 degrees C the bipy complex is only marginally active, while the quinoline-8-thiolate complex realizes yields of hydrogenated products up to 97% starting from 2,5-hexanedione and up to 66% starting from 2,5-dimethylfuran. The catalyst can also convert the 5-HMF derived acetone 4-(5-methyl-2-furanyl)-3-buten-2-one into 2,5,8-nonatriol, a potentially valuable cross-linker for polymer formulations. On the basis of DFT calculations, the higher activity of the quinoline-8-thiolate complex is proposed to be rooted in a metal-ligand bifunctional mechanism for the heterolytic activation and transfer of dihydrogen to the carbonyl substrate with the hydride-thiol complex [(4'-Ph-terpy)(quSH)Ru(H)r as the active catalyst. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Sullivan, Ryan J.; Schlaf, Marcel] Univ Guelph, Dept Chem, Guelph Waterloo Ctr Grad Work Chem GWC2, 50 Stone Rd East, Guelph, ON N1G 2W1, Canada. [Kim, Jin; Hoyt, Caroline; Silks, Louis A. (Pete), III] Los Alamos Natl Lab, Biosci Div, Grp B11,MS E529,POB 1663, Los Alamos, NM 87545 USA. RP Schlaf, M (reprint author), Univ Guelph, Dept Chem, Guelph Waterloo Ctr Grad Work Chem GWC2, 50 Stone Rd East, Guelph, ON N1G 2W1, Canada. EM mschlaf@uoguelph.ca OI Sullivan, Ryan/0000-0001-5540-6962; Silks, Pete/0000-0002-2993-5630 FU Natural Science and Engineering Council (NSERC) Canada; Bioeconomy Program of the Ontario Ministry for Agriculture, Food and Rural Affairs (OMAFRA); Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) program FX The authors thank the Natural Science and Engineering Council (NSERC) Canada, the Bioeconomy Program of the Ontario Ministry for Agriculture, Food and Rural Affairs (OMAFRA) and the Los Alamos National Laboratory (LANL) Laboratory Directed Research and Development (LDRD) program for supporting this research. NR 37 TC 1 Z9 1 U1 10 U2 20 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-5387 J9 POLYHEDRON JI Polyhedron PD MAR 29 PY 2016 VL 108 BP 104 EP 114 DI 10.1016/j.poly.2015.10.049 PG 11 WC Chemistry, Inorganic & Nuclear; Crystallography SC Chemistry; Crystallography GA DL3ED UT WOS:000375516100017 ER PT J AU Alexandropoulos, DI Moushi, EE Papatriantafyllopoulou, C Beavers, CM Teat, SJ Tasiopoulos, AJ Christou, G Stamatatos, TC AF Alexandropoulos, Dimitris I. Moushi, Eleni E. Papatriantafyllopoulou, Constantina Beavers, Christine M. Teat, Simon J. Tasiopoulos, Anastasios J. Christou, George Stamatatos, Theocharis C. TI Cyanate groups in higher oxidation state metal cluster chemistry: Mixed-valence (II/III) Mn-16 and Mn-18 clusters SO POLYHEDRON LA English DT Article DE Manganese; Cyanates; 2-(Hydroxymethyl)pyridine; Crystal structures; Magnetism ID SINGLE-MOLECULE MAGNETS; MANGANESE CARBOXYLATE CLUSTER; HIGH-SPIN MOLECULES; HIGH-NUCLEARITY; HIGH-SYMMETRY; NI-II; COMPLEXES; LIGAND; CAGE; TRIETHANOLAMINE AB The employment of cyanato (OCN-) group in high oxidation state manganese cluster chemistry, in conjunction with carboxylate ions and the organic chelating/bridging ligand 2-(hydroxymethyl)pyridine (hmpH), is reported. The syntheses, crystal structures, and magnetochemical characterization are described for [Mn16O8(OR)(4)(OCN)(4)(O2CMe)(12)(hmp)(6)(ROH)(2)] (R = Me (1), Et (2)) and [Mn18O14(O2CR)(18) (hmp)(4)(hmpH)(2)(H2O)(2)] (R = Me (3), Et (4)). The 2:1:1:1 reactions of Mn(O2CMe)(2)center dot 4H(2)O, hmpH, NaOCN and NEt3 in solvent MeOH or EtOH afford the isostructural complexes [Mn16O8(OR)(4)(OCN)(4) (O2CMe)(12)(hmp)(6)(ROH)(2)] (R = Me (1), Et (2)). The [Mn-16(mu(4)-O-4(mu 3-OMe)(4)(mu-OR)(6)(mu-OR)(6)](10+) core of representative complex 1 comprises a (Mn4Mn4III)-Mn-II double-cubane subunit attached on either side to two symmetry-related (MnMn3III)-Mn-II defective dicubanes. A similar reaction of Mn(O2CR)(2)center dot 4H(2)O, hmpH, NaOCN and NEt3, but in solvent MeCN, led instead to the formation of [Mn18O14(O2CR)(18)(hmp)(4)(hmpH)(2)(H2O)(2)](R = Me (3), Et (4)). Compounds 3 and 4 are very similar to each other and can be described as a central [Mn-4(III)(mu-O)(6)] rodlike subunit attached on either side to two symmetry-related [Mn(7)O9] subunits. Variable-temperature, solid-state dc and ac magnetic susceptibility studies revealed the presence of predominant antiferromagnetic exchange interactions in all compounds, and possible S = 2 or 1 (for 1 and 2) and S = 0 (for 3 and 4) ground state spin values. The combined results demonstrate the ability of cyanato groups to facilitate the formation of new polynuclear Mn complexes with structures different than these obtained from the use of the related azides. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Alexandropoulos, Dimitris I.; Stamatatos, Theocharis C.] Brock Univ, Dept Chem, St Catharines, ON L2S 3A1, Canada. [Moushi, Eleni E.; Papatriantafyllopoulou, Constantina; Tasiopoulos, Anastasios J.] Univ Cyprus, Dept Chem, CY-1678 Nicosia, Cyprus. [Papatriantafyllopoulou, Constantina; Christou, George] Univ Florida, Dept Chem, Gainesville, FL 32611 USA. [Beavers, Christine M.; Teat, Simon J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Stamatatos, TC (reprint author), Brock Univ, Dept Chem, St Catharines, ON L2S 3A1, Canada. EM tstamatatos@brocku.ca RI Beavers, Christine/C-3539-2009; Christou, George /A-3072-2014 OI Beavers, Christine/0000-0001-8653-5513; FU Brock University; NSERC-DG; ERA; Ontario Trillium Foundation; National Science Foundation [DMR-1213030]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by Brock University, NSERC-DG and ERA (to Th.C.S), the Ontario Trillium Foundation (graduate scholarship to D.I.A), and the National Science Foundation (DMR-1213030 to G.C). The Advance Light Source is supported by The Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. NR 74 TC 0 Z9 0 U1 10 U2 22 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0277-5387 J9 POLYHEDRON JI Polyhedron PD MAR 29 PY 2016 VL 108 BP 131 EP 142 DI 10.1016/j.poly.2015.11.031 PG 12 WC Chemistry, Inorganic & Nuclear; Crystallography SC Chemistry; Crystallography GA DL3ED UT WOS:000375516100020 ER PT J AU Eng, CH Yuzawa, S Wang, G Baidoo, EEK Katz, L Keasling, JD AF Eng, Clara H. Yuzawa, Satoshi Wang, George Baidoo, Edward E. K. Katz, Leonard Keasling, Jay D. TI Alteration of Polyketide Stereochemistry from anti to syn by a Ketoreductase Domain Exchange in a Type I Modular Polyketide Synthase Subunit SO BIOCHEMISTRY LA English DT Article ID EQUILIBRIUM ISOTOPE-EXCHANGE; MOLECULAR-BASIS; BETA-LIPOMYCIN; CELMERS RULES; CATALYSIS; STEREOSPECIFICITY; BIOSYNTHESIS; ELUCIDATION; MUTAGENESIS AB Polyketide natural products have broad applications in medicine. Exploiting the modular nature of polyketide synthases to alter stereospecificity is an attractive strategy for obtaining natural product analogues with altered pharmaceutical properties. We demonstrate that by retaining a dimerization element present in LipPks1+TE, we are able to use a ketoreductase domain exchange to alter alpha-methyl group stereochemistry with unprecedented retention of activity and simultaneously achieve a novel alteration of polyketide product stereochemistry from anti to syn. The substrate promiscuity of LipPks1+TE further provided a unique opportunity to investigate the substrate dependence of ketoreductase activity in a polyketide synthase module context. C1 [Eng, Clara H.; Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94270 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94270 USA. [Yuzawa, Satoshi; Katz, Leonard; Keasling, Jay D.] Univ Calif Berkeley, Inst QB3, Berkeley, CA 94270 USA. [Eng, Clara H.; Katz, Leonard; Keasling, Jay D.] Synthet Biol Engn Res Ctr, 5885 Hollis St, Emeryville, CA 94608 USA. [Wang, George; Baidoo, Edward E. K.; Keasling, Jay D.] Joint BioEnergy Inst, 5885 Hollis St, Emeryville, CA 94608 USA. [Wang, George; Baidoo, Edward E. K.; Keasling, Jay D.] Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94270 USA. RP Keasling, JD (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94270 USA.; Keasling, JD (reprint author), Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94270 USA.; Keasling, JD (reprint author), Univ Calif Berkeley, Inst QB3, Berkeley, CA 94270 USA.; Keasling, JD (reprint author), Synthet Biol Engn Res Ctr, 5885 Hollis St, Emeryville, CA 94608 USA.; Keasling, JD (reprint author), Joint BioEnergy Inst, 5885 Hollis St, Emeryville, CA 94608 USA.; Keasling, JD (reprint author), Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94270 USA. EM keasling@berkeley.edu FU Joint BioEnergy Institute; Office of Science, Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [EEC-0540879, MCB-1341894]; National Science Foundation Graduate Research Fellowship Program [DGE 1106400] FX This work was supported by the Joint BioEnergy Institute, which is funded by the Office of Science, Office of Biological and Environmental Research, of the U.S. Department of Energy (Contract DE-AC02-05CH11231), by the National Science Foundation (Grants EEC-0540879 and MCB-1341894), and by the National Science Foundation Graduate Research Fellowship Program (Grant DGE 1106400 to C.H.E.). NR 28 TC 4 Z9 4 U1 1 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAR 29 PY 2016 VL 55 IS 12 BP 1677 EP 1680 DI 10.1021/acs.biochem.6b00129 PG 4 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DI1HQ UT WOS:000373247600002 PM 26976746 ER PT J AU Shams, H Golji, J Garakani, K Mofrad, MRK AF Shams, Hengameh Golji, Javad Garakani, Kiavash Mofrad, Mohammad R. K. TI Dynamic Regulation of alpha-Actinin's Calponin Homology Domains on F-Actin SO BIOPHYSICAL JOURNAL LA English DT Article ID MOLECULAR-DYNAMICS; EXTRACELLULAR-MATRIX; FORCE TRANSMISSION; FOCAL ADHESIONS; STRESS FIBERS; BINDING; PROTEINS; VINCULIN; MECHANOTRANSDUCTION; CYTOSKELETON AB alpha-Actinin is an essential actin cross-linker involved in cytoskeletal organization and dynamics. The molecular conformation of alpha-actinin's actin-binding domain (ABD) regulates its association with actin and thus mutations in this domain can lead to severe pathogenic conditions. A point mutation at lysine 255 in human alpha-actinin-4 to glutamate increases the binding affinity resulting in stiffer cytoskeletal structures. The role of different ABD conformations and the effect of K255E mutation on ABD conformations remain elusive. To evaluate the impact of K255E mutation on ABD binding to actin we use all-atom molecular dynamics and free energy calculation methods and study the molecular mechanism of actin association in both wild-type a-actinin and in the K225E mutant. Our models illustrate that the strength of actin association is indeed sensitive to the ABD conformation, predict the effect of K255E mutation-based on simulations with the K237E mutant chicken alpha-actinin-and evaluate the mechanism of alpha-actinin binding to actin. Furthermore, our simulations showed that the calmodulin domain binding to the linker region was important for regulating the distance between actin and ABD. Our results provide valuable insights into the molecular details of this critical cellular phenomenon and further contribute to an understanding of cytoskeletal dynamics in health and disease. C1 [Shams, Hengameh; Golji, Javad; Garakani, Kiavash; Mofrad, Mohammad R. K.] Univ Calif Berkeley, Dept Bioengn, Mol Cell Biomech Lab, Berkeley, CA 94720 USA. [Shams, Hengameh; Golji, Javad; Garakani, Kiavash; Mofrad, Mohammad R. K.] Univ Calif Berkeley, Dept Mech Engn, Mol Cell Biomech Lab, Berkeley, CA 94720 USA. [Mofrad, Mohammad R. K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrat Bioimaging Div, Berkeley, CA 94720 USA. RP Mofrad, MRK (reprint author), Univ Calif Berkeley, Dept Bioengn, Mol Cell Biomech Lab, Berkeley, CA 94720 USA.; Mofrad, MRK (reprint author), Univ Calif Berkeley, Dept Mech Engn, Mol Cell Biomech Lab, Berkeley, CA 94720 USA.; Mofrad, MRK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrat Bioimaging Div, Berkeley, CA 94720 USA. EM mofrad@berkeley.edu FU National Science Foundation CAREER Award [CBET-0955291]; National Science Foundation [ACI-1053575] FX This work was supported by the National Science Foundation CAREER Award CBET-0955291 to M.R.K.M. In addition, this research used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation grant No. ACI-1053575. NR 51 TC 0 Z9 0 U1 1 U2 2 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0006-3495 EI 1542-0086 J9 BIOPHYS J JI Biophys. J. PD MAR 29 PY 2016 VL 110 IS 6 BP 1444 EP 1455 DI 10.1016/j.bpj.2016.02.024 PG 12 WC Biophysics SC Biophysics GA DI4RO UT WOS:000373487200025 PM 27028653 ER PT J AU Gupta, S Mamontov, E Jalarvo, N Stingaciu, L Ohl, M AF Gupta, S. Mamontov, E. Jalarvo, N. Stingaciu, L. Ohl, M. TI Characteristic length scales of the secondary relaxations in glass-forming glycerol SO EUROPEAN PHYSICAL JOURNAL E LA English DT Article ID NEUTRON SPIN-ECHO; GOLDSTEIN BETA-RELAXATION; MODE-COUPLING-THEORY; LIGHT-SCATTERING; SUPERCOOLED LIQUIDS; DIELECTRIC-SPECTROSCOPY; PROPYLENE CARBONATE; ALPHA-RELAXATION; MOLECULAR GLASS; IONIC CONDUCTORS AB We investigate the secondary relaxations and their link to the main structural relaxation in glass-forming liquids using glycerol as a model system. We analyze the incoherent neutron scattering signal dependence on the scattering momentum transfer, Q, in order to obtain the characteristic length scale for different secondary relaxations. Such a capability of neutron scattering makes it somewhat unique and highly complementary to the traditional techniques of glass physics, such as light scattering and broadband dielectric spectroscopy, which provide information on the time scale, but not the length scales, of relaxation processes. The choice of suitable neutron scattering techniques depends on the time scale of the relaxation of interest. We use neutron backscattering to identify the characteristic length scale of 0.7 angstrom for the faster secondary relaxation described in the framework of the mode-coupling theory (MCT). Neutron spin-echo is employed to probe the slower secondary relaxation of the excess wing type at a low temperature (similar to 1.13T(g)). The characteristic length scale for this excess wing dynamics is approximately 4.7 angstrom. Besides the Q-dependence, the direct coupling of neutron scattering signal to density fluctuation makes this technique indispensable for measuring the length scale of the microscopic relaxation dynamics. C1 [Gupta, S.; Jalarvo, N.; Stingaciu, L.; Ohl, M.] Oak Ridge Natl Lab, Neutron Sci Directorate, Biol & Soft Matter Div, JCNS SNS, POB 2008 MS6473,Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Mamontov, E.; Jalarvo, N.] Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, POB 2008 MS6473, Oak Ridge, TN 37831 USA. RP Gupta, S (reprint author), Oak Ridge Natl Lab, Neutron Sci Directorate, Biol & Soft Matter Div, JCNS SNS, POB 2008 MS6473,Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM s.gupta@fz-juelich.de RI Mamontov, Eugene/Q-1003-2015; Jalarvo, Niina/Q-1320-2015 OI Mamontov, Eugene/0000-0002-5684-2675; Jalarvo, Niina/0000-0003-0644-6866 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy FX We thank Antti Soininen for support in data analysis and Malcolm Cochran for critical reading of the manuscript. Research conducted at ORNL's Spallation Neutron Source, was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. NR 72 TC 1 Z9 1 U1 6 U2 18 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1292-8941 EI 1292-895X J9 EUR PHYS J E JI Eur. Phys. J. E PD MAR 29 PY 2016 VL 39 IS 3 AR 40 DI 10.1140/epje/i2016-16040-7 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary; Physics, Applied; Polymer Science SC Chemistry; Materials Science; Physics; Polymer Science GA DI0FX UT WOS:000373171800003 PM 27021657 ER PT J AU Rivers, AR Burns, AS Chan, LK Moran, MA AF Rivers, Adam R. Burns, Andrew S. Chan, Leong-Keat Moran, Mary Ann TI Experimental Identification of Small Non-Coding RNAs in the Model Marine Bacterium Ruegeria pomeroyi DSS-3 SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE small RNA; Ruegeria; Roseobacter; ncRNA; sRNA ID ESCHERICHIA-COLI; VIBRIO-CHOLERAE; ORGANIC-MATTER; VIRULENCE; SYNECHOCOCCUS; TRANSCRIPTION; EXPRESSION; SEQUENCE; OPERON; CARBON AB In oligotrophic ocean waters where bacteria are often subjected to chronic nutrient limitation, community transcriptome sequencing has pointed to the presence of highly abundant small RNAs (sRNAs). The role of sRNAs in regulating response to nutrient stress was investigated in a model heterotrophic marine bacterium Ruegeria pomeroyi grown in continuous culture under carbon (C) and nitrogen (N) limitation. RNAseq analysis identified 99 putative sRNAs. Sixty-nine were cis-encoded and located antisense to a presumed target gene. Thirty were trans encoded and initial target prediction was performed computationally. The most prevalent functional roles of genes anti-sense to the cis-sRNAs were transport, cell-cell interactions, signal transduction, and transcriptional regulation. Most sRNAs were transcribed equally under both C and N limitation, and may be involved in a general stress response. However, 14 were regulated differentially between the C and N treatments and may respond to specific nutrient limitations. A network analysis of the predicted target genes of the R. pomeroyi cis-sRNAs indicated that they average fewer connections than typical protein encoding genes, and appear to be more important in peripheral or niche-defining functions encoded in the pan genome. C1 [Rivers, Adam R.] United States Dept Energy, Joint Genome Inst, Walnut Creek, CA USA. [Burns, Andrew S.; Moran, Mary Ann] Univ Georgia, Dept Marine Sci, Athens, GA 30602 USA. [Chan, Leong-Keat] WaferGen Biosyst Inc, Fremont, CA USA. [Burns, Andrew S.] Georgia Inst Technol, Dept Biol, Atlanta, GA 30332 USA. RP Moran, MA (reprint author), Univ Georgia, Dept Marine Sci, Athens, GA 30602 USA. EM mmoran@uga.edu OI Moran, Mary Ann/0000-0002-0702-8167 FU NSF [OCE1342694, OCE1356010]; Gordon and Betty Moore Foundation [GBMF538.01] FX This research was supported by NSF grants OCE1342694 and OCE1356010 and Gordon and Betty Moore Foundation grant GBMF538.01. NR 48 TC 3 Z9 3 U1 5 U2 11 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD MAR 29 PY 2016 VL 7 AR 380 DI 10.3389/fmicb.2016.00380 PG 15 WC Microbiology SC Microbiology GA DH6HZ UT WOS:000372892900001 PM 27065955 ER PT J AU Zeitlin, C La Tessa, C AF Zeitlin, Cary La Tessa, Chiara TI The Role of Nuclear Fragmentation in Particle Therapy and Space Radiation Protection SO FRONTIERS IN ONCOLOGY LA English DT Review DE galactic cosmic rays; nuclear fragmentation models; nuclear interactions; Bragg curve; space radiation; space radiation shielding; heavy-ion therapy ID CROSS-SECTIONS; MODELS AB The transport of the so-called HZE particles (those having high charge, Z, and energy, E) through matter is crucially important both in space radiation protection and in the clinical setting where heavy ions are used for cancer treatment. HZE particles are usually considered those having Z > 1, though sometimes Z > 2 is meant. Transport physics is governed by two types of interactions, electromagnetic (ionization energy loss) and nuclear. Models of transport, such as those used in treatment planning and space mission planning must account for both effects in detail. The theory of electromagnetic interactions is well developed, but nucleus-nucleus collisions are so complex that no fundamental physical theory currently describes them. Instead, interaction models are generally anchored to experimental data, which in some areas are far from complete. The lack of fundamental physics knowledge introduces uncertainties in the calculations of exposures and their associated risks. These uncertainties are greatly compounded by the much larger uncertainties in biological response to HZE particles. In this article, we discuss the role of nucleus-nucleus interactions in heavy charged particle therapy and in deep space, where astronauts will receive a chronic low dose from galactic cosmic rays (GCRs) and potentially higher short-term doses from sporadic, unpredictable solar energetic particles (SEPs). GCRs include HZE particles; SEPs typically do not and we, therefore, exclude them from consideration in this article. Nucleus-nucleus collisions can result in the breakup of heavy ions into lighter ions. In space, this is generally beneficial because dose and dose equivalent are, on the whole, reduced in the process. The GCRs can be considered a radiation field with a significant high-LET component; when they pass through matter, the high-LET component is attenuated, at the cost of a slight increase in the low-LET component. Not only are the standard measures of risk reduced by fragmentation, but it can be argued that fragmentation also reduces the uncertainties in risk calculations by shifting the LET distribution toward one that is more concentrated at low LET, where biological effects are better understood. We review previous work in this area, including measurements made by the Radiation Assessment Detector during its journey to Mars and while on the surface of Mars aboard the Curiosity rover. Transport of HZE is also critically important in heavy-ion therapy, as it is necessary to know the details of the radiation field at the treatment site. This field is substantially modified compared to the incident pure (or nearly pure) ion beam by the same mechanisms of energy loss and nuclear fragmentation that pertain to the transport of space radiation. C1 [Zeitlin, Cary] Lockheed Martin Informat Serv & Global Solut, Houston, TX USA. [La Tessa, Chiara] Brookhaven Natl Lab, Collider Accelerator Dept, Upton, NY 11973 USA. RP Zeitlin, C (reprint author), Lockheed Martin Informat Serv & Global Solut, Houston, TX USA. EM cary.j.zeitlin@nasa.gov NR 45 TC 0 Z9 0 U1 5 U2 6 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 2234-943X J9 FRONT ONCOL JI Front. Oncol. PD MAR 29 PY 2016 VL 6 AR 65 DI 10.3389/fonc.2016.00065 PG 13 WC Oncology SC Oncology GA DI0PI UT WOS:000373198900002 PM 27065350 ER PT J AU Sumino, Y Yamada, NL Nagao, M Honda, T Kitahata, H Melnichenko, YB Seto, H AF Sumino, Yutaka Yamada, Norifumi L. Nagao, Michihiro Honda, Takuya Kitahata, Hiroyuki Melnichenko, Yuri B. Seto, Hideki TI Mechanism of Spontaneous Blebbing Motion of an Oil-Water Interface: Elastic Stress Generated by a Lamellar-Lamellar Transition SO LANGMUIR LA English DT Article ID ALCOHOL; SURFACTANT; CHLORIDE; SYSTEM AB A quaternary system composed of surfactant, cosurfactant, oil, and water showing spontaneous motion of the oil-water interface-under far-from-equilibrium condition is studied in order to understand nanometer-scale structures and their roles in spontaneous motion. The interfacial motion is characterized by the repetitive. extension and retraction of spherical protrusions at the interface, i.e, blebbing motion. During, the, blebbing motion, elastic aggregates are accumulated, which were characterized as surfactant lamellar structures with mean repeat distances d of 25 to 40 nm. Still unclear is the relationship between the structure formation and, the dynamics of the interfacial motion. In the present study, we find that a new lamellar structure with d larger than. 80 run is formed at. the blebbing oil-water interface,. while the resultant elastic aggregates, which are the one reported before, have a lamellar structure with smaller d (25 to 40 nm). Such transition of lamellar structures from the larger d to smaller d is induced by a penetration of surfactants from an aqueous phase into the aggregates. We propose a model in which elastic stress generated by the transition-drives the blebbing motion at the interface. The present results explain the link between nanometer-scale transition of lamellar structure and millimeter-scale dynamics at an oil water interface. C1 [Sumino, Yutaka] Tokyo Univ Sci, Fac Sci, Dept Appl Phys, Tokyo 1258585, Japan. [Yamada, Norifumi L.; Seto, Hideki] High Energy Accelerator Res Org, Inst Mat Struct Sci, KENS&CMRC, Tokai, Ibaraki 3190016, Japan. [Nagao, Michihiro] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Nagao, Michihiro] Indiana Univ, Ctr Explorat Energy & Matter, Bloomington, IN 47408 USA. [Honda, Takuya] Aichi Univ Educ, Dept Educ, Kariya, Aichi 4488542, Japan. [Kitahata, Hiroyuki] Chiba Univ, Grad Sch Sci, Dept Phys, Chiba, Chiba 2638522, Japan. [Melnichenko, Yuri B.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. RP Sumino, Y (reprint author), Tokyo Univ Sci, Fac Sci, Dept Appl Phys, Tokyo 1258585, Japan. EM ysumino@rs.tus.ac.jp RI Kitahata, Hiroyuki/E-8635-2015; OI Kitahata, Hiroyuki/0000-0003-3453-9883; Seto, Hideki/0000-0002-1658-3576 FU JSPS [24740287]; U.S.-Japan Cooperative Program on Neutron Scattering; NIST, U.S. Department of Commerce [70NANB10H255]; Scientific User Facilities Division, office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported in part by a Grant-in-Aid for Young Scientists B by JSPS to Y.S. (No. 24740287) and by the U.S.-Japan Cooperative Program on Neutron Scattering, and also performed under the Cooperative Research Program of "Network Joint Research Center for Materials and Devices." M.N. acknowledges the funding support of cooperative agreement 70NANB10H255 from NIST, U.S. Department of Commerce. The authors wish to thank M. Hishida (University of Tsukuba) for helpful discussions. The SAXS analyses were performed under the approval of the Photon Factory Program Advisory Committee (Proposal Nos. 2013G530 and 2013G525). The authors also extend special thanks to N. Igarashi and N. Shimizu (Photon Factory, KEK) for their invaluable assistance in obtaining data from beamline BL6A. The SANS analyses were performed under the approval of the HFIR (Cycle 445 CG-2; IPTS-7094). The research at Oak Ridge National Laboratory's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, office of Basic Energy Sciences, U.S. Department of Energy. NR 22 TC 0 Z9 0 U1 4 U2 9 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAR 29 PY 2016 VL 32 IS 12 BP 2891 EP 2899 DI 10.1021/acs.langmuir.6b00107 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DI1HO UT WOS:000373247400006 PM 26938640 ER PT J AU Shi, HL Ming, WM Du, MH AF Shi, Hongliang Ming, Wenmei Du, Mao-Hua TI Bismuth chalcohalides and oxyhalides as optoelectronic materials SO PHYSICAL REVIEW B LA English DT Article ID AUGMENTED-WAVE METHOD; HALIDE PEROVSKITES; THIN-FILMS AB Several Tl and Pb based halides and chalcohalides have recently been discovered as promising optoelectronic materials [i.e., photovoltaic (PV) and gamma-ray detectionmaterials]. Efficient carrier transport in these materials is attributed partly to the special chemistry of ns(2) ions (e.g., Tl+, Pb2+, and Bi3+). However, the toxicity of Tl and Pb is challenging to the development and the wide use of Tl and Pb based materials. In this paper, we investigate materials that contain Bi3+, which is also an ns(2) ion. By combining Bi halides with Bi chalcogenides or oxides, the resulting ternary compounds exhibit a wide range of band gaps, offering opportunities in various optoelectronic applications. Density functional calculations of electronic structure, dielectric properties, optical properties, and defect properties are performed on selected Bi3+ based chalcohalides and oxyhalides, i.e., BiSeBr, BiSI, BiSeI, and BiOBr. We propose different applications for these Bi compounds based on calculated properties, i.e., n-BiSeBr, p-BiSI, and p-BiSeI as PV materials, BiSeBr and BiSI as room-temperature radiation detection materials, and BiOBr as a p-type transparent conducting material. BiSeBr, BiSI, and BiSeBr have chain structures while BiOBr has a layered structure. However, in BiSI, BiSeI, and BiOBr, significant valence-band dispersion is found in the directions perpendicular to the atomic chain or layer because the valence-band edge states are dominated by the halogen states that have strong interchain or interlayer coupling. We find significantly enhanced Born effective charges and anomalously large static dielectric constants of the Bi compounds, which should reduce carrier scattering and trapping and promote efficient carrier transport in these materials. The strong screening and the small anion coordination numbers in Bi chalcohalides should lead to weak potentials for electron localization at anion vacancies. Defect calculations indeed show that the anion vacancies (Se and Br vacancies) in BiSeBr are shallow, which is beneficial to efficient electron transport. C1 [Shi, Hongliang; Ming, Wenmei; Du, Mao-Hua] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Shi, Hongliang; Ming, Wenmei; Du, Mao-Hua] Oak Ridge Natl Lab, Ctr Radiat Detect Mat & Syst, Oak Ridge, TN 37831 USA. [Shi, Hongliang] Beihang Univ, Sch Phys & Nucl Energy Engn, Key Lab Micronano Measurement Manipulat & Phys, Minist Educ, Beijing 100191, Peoples R China. RP Shi, HL (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.; Shi, HL (reprint author), Oak Ridge Natl Lab, Ctr Radiat Detect Mat & Syst, Oak Ridge, TN 37831 USA. RI Shi, Hongliang/A-7568-2010; Du, Mao-Hua/B-2108-2010 OI Shi, Hongliang/0000-0003-0713-4688; Du, Mao-Hua/0000-0001-8796-167X FU Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; U.S. Department of Energy [DE-AC05-00OR22725]; Department of Energy; DOE FX We are grateful for the helpful discussions with David J. Singh. This work was supported by the Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 45 TC 9 Z9 9 U1 10 U2 34 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 29 PY 2016 VL 93 IS 10 AR 104108 DI 10.1103/PhysRevB.93.104108 PG 7 WC Physics, Condensed Matter SC Physics GA DH9FR UT WOS:000373102300001 ER PT J AU Arrington, J AF Arrington, J. TI Comment on "Nonidentical protons" SO PHYSICAL REVIEW C LA English DT Letter C1 [Arrington, J.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Arrington, J (reprint author), Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. NR 9 TC 1 Z9 1 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 29 PY 2016 VL 93 IS 3 AR 039801 DI 10.1103/PhysRevC.93.039801 PG 1 WC Physics, Nuclear SC Physics GA DH9GW UT WOS:000373105400003 ER PT J AU Bhardwaj, V Miyabayashi, K Panzenboeck, E Trabelsi, K Frey, A Abdesselam, A Adachi, I Aihara, H Al Said, S Arinstein, K Asner, DM Atmacan, H Aulchenko, V Aushev, T Ayad, R Babu, V Badhrees, I Bahinipati, S Bakich, AM Bala, A Bansal, V Barberio, E Bhuyan, B Biswal, J Bobrov, A Bondar, A Bozek, A Bracko, M Browder, TE Cervenkov, D Chekelian, V Chen, A Cheon, BG Chilikin, K Chistov, R Cho, K Chobanova, V Choi, SK Choi, Y Cinabro, D Dalseno, J Danilov, M Dolezal, Z Dutta, D Eidelman, S Farhat, H Fast, JE Ferber, T Frost, O Fulsom, BG Gaur, V Gabyshev, N Ganguly, S Garmash, A Gillard, R Glattauer, R Goh, YM Goldenzweig, P Golob, B Greenwald, D Haba, J Hamer, P Hayasaka, K Hayashii, H He, XH Hou, WS Iijima, T Inami, K Ishikawa, A Itoh, R Iwasaki, Y Jaegle, I Joffe, D Joo, KK Julius, T Kato, E Katrenko, P Kawasaki, T Kiesling, C Kim, DY Kim, JB Kim, KT Kim, MJ Kim, SH Kim, YJ Kinoshita, K Ko, BR Kobayashi, N Kodys, P Korpar, S Krizan, P Krokovny, P Kuhr, T Kumar, R Kumita, T Kuzmin, A Kwon, YJ Lee, IS Li, C Li, Y Gioi, LL Libby, J Liventsev, D Loos, A Lukin, P Masuda, M Matvienko, D Miyata, H Mizuk, R Mohanty, GB Mohanty, S Moll, A Moon, HK Mussa, R Nakano, E Nakao, M Nanut, T Natkaniec, Z Nayak, M Nisar, NK Nishida, S Ogawa, S Okuno, S Pakhlova, G Pal, B Park, CW Park, H Pedlar, TK Pestotnik, R Petric, M Piilonen, LE Pulvermacher, C Purohit, MV Rauch, J Ribezl, E Ritter, M Rostomyan, A Sahoo, H Sakai, Y Sandilya, S Santelj, L Sanuki, T Sato, Y Savinov, V Schneider, O Schnell, G Schwanda, C Seino, Y Semmler, D Senyo, K Seon, O Sevior, ME Shebalin, V Shen, CP Shibata, TA Shiu, JG Shwartz, B Simon, F Singh, JB Sohn, YS Sokolov, A Solovieva, E Staric, M Stypula, J Sumihama, M Sumiyoshi, T Tamponi, U Tanida, K Teramoto, Y Uchida, M Uehara, S Uglov, T Unno, Y Uno, S Urquijo, P Usov, Y Van Hulse, C Vanhoefer, P Varner, G Vinokurova, A Vorobyev, V Wang, CH Wang, MZ Wang, P Wang, XL Watanabe, M Watanabe, Y Wehle, S Won, E Yamaoka, J Yashchenko, S Ye, H Yook, Y Yuan, CZ Yusa, Y Zhang, ZP Zhilich, V Zhulanov, V Zupanc, A AF Bhardwaj, V. Miyabayashi, K. Panzenboeck, E. Trabelsi, K. Frey, A. Abdesselam, A. Adachi, I. Aihara, H. Al Said, S. Arinstein, K. Asner, D. M. Atmacan, H. Aulchenko, V. Aushev, T. Ayad, R. Babu, V. Badhrees, I. Bahinipati, S. Bakich, A. M. Bala, A. Bansal, V. Barberio, E. Bhuyan, B. Biswal, J. Bobrov, A. Bondar, A. Bozek, A. Bracko, M. Browder, T. E. Cervenkov, D. Chekelian, V. Chen, A. Cheon, B. G. Chilikin, K. Chistov, R. Cho, K. Chobanova, V. Choi, S-K. Choi, Y. Cinabro, D. Dalseno, J. Danilov, M. Dolezal, Z. Dutta, D. Eidelman, S. Farhat, H. Fast, J. E. Ferber, T. Frost, O. Fulsom, B. G. Gaur, V. Gabyshev, N. Ganguly, S. Garmash, A. Gillard, R. Glattauer, R. Goh, Y. M. Goldenzweig, P. Golob, B. Greenwald, D. Haba, J. Hamer, P. Hayasaka, K. Hayashii, H. He, X. H. Hou, W-S. Iijima, T. Inami, K. Ishikawa, A. Itoh, R. Iwasaki, Y. Jaegle, I. Joffe, D. Joo, K. K. Julius, T. Kato, E. Katrenko, P. Kawasaki, T. Kiesling, C. Kim, D. Y. Kim, J. B. Kim, K. T. Kim, M. J. Kim, S. H. Kim, Y. J. Kinoshita, K. Ko, B. R. Kobayashi, N. Kodys, P. Korpar, S. Krizan, P. Krokovny, P. Kuhr, T. Kumar, R. Kumita, T. Kuzmin, A. Kwon, Y-J. Lee, I. S. Li, C. Li, Y. Gioi, L. Li Libby, J. Liventsev, D. Loos, A. Lukin, P. Masuda, M. Matvienko, D. Miyata, H. Mizuk, R. Mohanty, G. B. Mohanty, S. Moll, A. Moon, H. K. Mussa, R. Nakano, E. Nakao, M. Nanut, T. Natkaniec, Z. Nayak, M. Nisar, N. K. Nishida, S. Ogawa, S. Okuno, S. Pakhlova, G. Pal, B. Park, C. W. Park, H. Pedlar, T. K. Pestotnik, R. Petric, M. Piilonen, L. E. Pulvermacher, C. Purohit, M. V. Rauch, J. Ribezl, E. Ritter, M. Rostomyan, A. Sahoo, H. Sakai, Y. Sandilya, S. Santelj, L. Sanuki, T. Sato, Y. Savinov, V. Schneider, O. Schnell, G. Schwanda, C. Seino, Y. Semmler, D. Senyo, K. Seon, O. Sevior, M. E. Shebalin, V. Shen, C. P. Shibata, T-A. Shiu, J-G. Shwartz, B. Simon, F. Singh, J. B. Sohn, Y-S. Sokolov, A. Solovieva, E. Staric, M. Stypula, J. Sumihama, M. Sumiyoshi, T. Tamponi, U. Tanida, K. Teramoto, Y. Uchida, M. Uehara, S. Uglov, T. Unno, Y. Uno, S. Urquijo, P. Usov, Y. Van Hulse, C. Vanhoefer, P. Varner, G. Vinokurova, A. Vorobyev, V. Wang, C. H. Wang, M-Z. Wang, P. Wang, X. L. Watanabe, M. Watanabe, Y. Wehle, S. Won, E. Yamaoka, J. Yashchenko, S. Ye, H. Yook, Y. Yuan, C. Z. Yusa, Y. Zhang, Z. P. Zhilich, V. Zhulanov, V. Zupanc, A. CA Belle Collaboration TI Inclusive and exclusive measurements of B decays to chi(c1) and chi(c2) at Belle SO PHYSICAL REVIEW D LA English DT Article ID CHARMONIUM PRODUCTION; DETECTOR AB We report inclusive and exclusive measurements for chi(c1) and chi(c2) production in B decays. We measure B(B -> chi X-c1) = (3.03 +/- 0.05 (stat) +/- 0.24(syst)) x 10(-3) and B(B -> chi X-c2) = (0.70 +/- 0.06 (stat) +/- 0.10(syst)) x 10(-3). For the first time, chi(c2) production in exclusive B decays in the modes B-0 -> chi(c2) pi K--(+) and B-0 -> chi(c2) pi(-)pi K-+(+) has been observed, along with first evidence for the B-0 -> chi(c2) pi K--(s)0 decay mode. For chi c1 production, we report the first observation in the B+ -> chi(c1) pi(-)pi K-+(+), B-0 -> chi(c1) pi(-)pi K-+(s)0 and B-0 -> chi(c1) pi(-)pi K-+(+) decay modes. Using these decay modes, we observe a difference in the production mechanism of chi(c2) in comparison to chi(c1) in B decays. In addition, we report searches for X(3872) and chi(c1) (2P) in the B+ -> (chi(c1) pi(+)pi(-))K+ decay mode. The reported results use 772 x 10(6) B (B) over bar events collected at the Upsilon(4S) resonance with the Belle detector at the KEKB asymmetric-energy e(+)e(-) collider. C1 [Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Bilbao 48080, Spain. [Shen, C. P.] Beihang Univ, Beijing 100191, Peoples R China. [Arinstein, K.; Aulchenko, V.; Bobrov, A.; Bondar, A.; Eidelman, S.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Budker Inst Nucl Phys SB RAS, Novosibirsk 630090, Russia. [Cervenkov, D.; Dolezal, Z.; Kodys, P.] Charles Univ Prague, Fac Math & Phys, CR-12116 Prague, Czech Republic. [Joo, K. K.] Chonnam Natl Univ, Kwangju 660701, South Korea. [Kinoshita, K.; Pal, B.] Univ Cincinnati, Cincinnati, OH 45221 USA. [Ferber, T.; Frost, O.; Rostomyan, A.; Wehle, S.; Yashchenko, S.; Ye, H.] DESY, D-22607 Hamburg, Germany. [Semmler, D.] Univ Giessen, D-35392 Giessen, Germany. [Sumihama, M.] Gifu Univ, Gifu 5011193, Japan. [Panzenboeck, E.; Frey, A.; Hamer, P.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Trabelsi, K.; Adachi, I.; Haba, J.; Itoh, R.; Nakao, M.; Nishida, S.; Sakai, Y.; Uehara, S.; Uno, S.] SOKENDAI, Hayama 2400193, Japan. [Choi, S-K.] Gyeongsang Natl Univ, Chinju 660701, South Korea. [Cheon, B. G.; Goh, Y. M.; Kim, S. H.; Lee, I. S.; Unno, Y.] Hanyang Univ, Seoul 133791, South Korea. [Browder, T. E.; Jaegle, I.; Sahoo, H.; Varner, G.] Univ Hawaii, Honolulu, HI 96822 USA. [Trabelsi, K.; Adachi, I.; Haba, J.; Itoh, R.; Iwasaki, Y.; Liventsev, D.; Nakao, M.; Nishida, S.; Sakai, Y.; Santelj, L.; Uehara, S.; Uno, S.] High Energy Accelerator Res Org KEK, Tsukuba, Ibaraki 3050801, Japan. [Schnell, G.] Basque Fdn Sci, IKERBASQUE, Bilbao 48013, Spain. [Bahinipati, S.] Indian Inst Technol Bhubaneswar, Satya Nagar 751007, India. [Bhuyan, B.] Indian Inst Technol Guwahati, Gauhati 781039, Assam, India. [Libby, J.; Nayak, M.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Wang, P.; Yuan, C. Z.] Chinese Acad Sci, Inst High Energy Phys, Beijing 100049, Peoples R China. [Glattauer, R.; Schwanda, C.] Inst High Energy Phys, A-1050 Vienna, Austria. [Sokolov, A.] Inst High Energy Phys, Protvino 142281, Russia. [Mussa, R.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Biswal, J.; Bracko, M.; Golob, B.; Korpar, S.; Krizan, P.; Nanut, T.; Pestotnik, R.; Petric, M.; Ribezl, E.; Staric, M.; Zupanc, A.] Jozef Stefan Inst, Ljubljana 1000, Slovenia. [Okuno, S.; Watanabe, Y.] Kanagawa Univ, Yokohama, Kanagawa 2218686, Japan. [Goldenzweig, P.; Pulvermacher, C.] Karlsruhe Inst Technol, Inst Expt Kernphys, D-76131 Karlsruhe, Germany. [Joffe, D.] Kennesaw State Univ, Kennesaw, GA 30144 USA. [Badhrees, I.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. [Al Said, S.] King Abdulaziz Univ, Dept Phys, Fac Sci, Jeddah 21589, Saudi Arabia. [Cho, K.; Kim, Y. J.] Korea Inst Sci & Technol Informat, Daejeon 305806, South Korea. [Kim, J. B.; Kim, K. T.; Ko, B. R.; Moon, H. K.; Won, E.] Korea Univ, Seoul 136713, South Korea. [Kim, M. J.; Park, H.] Kyungpook Natl Univ, Daegu 702701, South Korea. [Schneider, O.] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Golob, B.; Krizan, P.] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. [Kuhr, T.] Univ Munich, Marchioninistr 15, D-80539 Munich, Germany. [Pedlar, T. K.] Luther Coll, Decorah, IA 52101 USA. [Bracko, M.; Korpar, S.] Univ Maribor, SLO-2000 Maribor, Slovenia. [Chekelian, V.; Chobanova, V.; Dalseno, J.; Kiesling, C.; Gioi, L. Li; Moll, A.; Ritter, M.; Simon, F.; Vanhoefer, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Barberio, E.; Julius, T.; Li, C.; Sevior, M. E.; Urquijo, P.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Atmacan, H.] Middle E Tech Univ, TR-06531 Ankara, Turkey. [Chilikin, K.; Chistov, R.; Danilov, M.; Mizuk, R.] Moscow Phys Engn Inst, Moscow 115409, Russia. [Aushev, T.; Katrenko, P.; Mizuk, R.; Pakhlova, G.; Solovieva, E.; Uglov, T.] Moscow Inst Phys & Technol, Moscow 141700, Moscow Region, Russia. [Iijima, T.; Inami, K.; Sato, Y.; Seon, O.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648602, Japan. [Hayasaka, K.; Iijima, T.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Miyabayashi, K.; Panzenboeck, E.; Hayashii, H.] Nara Womens Univ, Nara 6308506, Japan. [Chen, A.] Natl Cent Univ, Chungli 32054, Taiwan. [Wang, C. H.] Natl United Univ, Miaoli 36003, Taiwan. [Hou, W-S.; Shiu, J-G.; Wang, M-Z.] Natl Taiwan Univ, Dept Phys, Taipei 10617, Taiwan. [Bozek, A.; Natkaniec, Z.; Stypula, J.] H Niewodniczanski Inst Nucl Phys, PL-31342 Krakow, Poland. [Kawasaki, T.; Miyata, H.; Seino, Y.; Watanabe, M.; Yusa, Y.] Niigata Univ, Niigata 9502181, Japan. [Arinstein, K.; Aulchenko, V.; Bobrov, A.; Bondar, A.; Eidelman, S.; Gabyshev, N.; Garmash, A.; Krokovny, P.; Kuzmin, A.; Lukin, P.; Matvienko, D.; Shebalin, V.; Shwartz, B.; Usov, Y.; Vinokurova, A.; Vorobyev, V.; Zhilich, V.; Zhulanov, V.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Nakano, E.; Teramoto, Y.] Osaka City Univ, Osaka 5588585, Japan. [Asner, D. M.; Bansal, V.; Fast, J. E.; Fulsom, B. G.; Yamaoka, J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Bala, A.; Singh, J. B.] Panjab Univ, Chandigarh 160014, India. [He, X. H.] Peking Univ, Beijing 100871, Peoples R China. [Savinov, V.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Kumar, R.] Punjab Agr Univ, Ludhiana 141004, Punjab, India. [Zhang, Z. P.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Tanida, K.] Seoul Natl Univ, Seoul 151742, South Korea. [Kim, D. Y.] Soongsil Univ, Seoul 156743, South Korea. [Bhardwaj, V.; Loos, A.; Purohit, M. V.] Univ S Carolina, Columbia, SC 29208 USA. [Choi, Y.; Park, C. W.] Sungkyunkwan Univ, Suwon 440746, South Korea. [Bakich, A. M.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdesselam, A.; Al Said, S.; Ayad, R.; Badhrees, I.] Univ Tabuk, Dept Phys, Fac Sci, Tabuk 71451, Saudi Arabia. [Babu, V.; Dutta, D.; Gaur, V.; Mohanty, G. B.; Mohanty, S.; Nisar, N. K.; Sandilya, S.] Tata Inst Fundamental Res, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Dalseno, J.; Moll, A.; Simon, F.] Tech Univ Munich, Excellence Cluster Universe, D-85748 Garching, Germany. [Greenwald, D.; Rauch, J.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany. [Ogawa, S.] Toho Univ, Funabashi, Chiba 2748510, Japan. [Ishikawa, A.; Kato, E.; Sanuki, T.] Tohoku Univ, Sendai, Miyagi 9808578, Japan. [Masuda, M.] Univ Tokyo, Earthquake Res Inst, Tokyo 1130032, Japan. [Aihara, H.] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Kobayashi, N.; Shibata, T-A.; Uchida, M.] Tokyo Inst Technol, Tokyo 1528550, Japan. [Kumita, T.; Sumiyoshi, T.] Tokyo Metropolitan Univ, Tokyo 1920397, Japan. [Tamponi, U.] Univ Turin, I-10124 Turin, Italy. [Mohanty, S.] Utkal Univ, Bhubaneswar 751004, Orissa, India. [Li, Y.; Liventsev, D.; Piilonen, L. E.; Wang, X. L.] Virginia Polytech Inst & State Univ, CNP, Blacksburg, VA 24061 USA. [Cinabro, D.; Farhat, H.; Ganguly, S.; Gillard, R.] Wayne State Univ, Detroit, MI 48202 USA. [Senyo, K.] Yamagata Univ, Yamagata 9908560, Japan. [Kwon, Y-J.; Sohn, Y-S.; Yook, Y.] Yonsei Univ, Seoul 120749, South Korea. [Bhardwaj, V.] Indian Inst Sci Educ & Res Mohali, Sas Nagar 140306, India. RP Bhardwaj, V (reprint author), Univ S Carolina, Columbia, SC 29208 USA.; Bhardwaj, V (reprint author), Indian Inst Sci Educ & Res Mohali, Sas Nagar 140306, India. RI Solovieva, Elena/B-2449-2014; Aihara, Hiroaki/F-3854-2010; Katrenko, Petr/D-1229-2016; Danilov, Mikhail/C-5380-2014; Uglov, Timofey/B-2406-2014; Chilikin, Kirill/B-4402-2014; Chistov, Ruslan/B-4893-2014; Mizuk, Roman/B-3751-2014; Pakhlova, Galina/C-5378-2014; Cervenkov, Daniel/D-2884-2017 OI Solovieva, Elena/0000-0002-5735-4059; Aihara, Hiroaki/0000-0002-1907-5964; Bhardwaj, Vishal/0000-0001-8857-8621; Katrenko, Petr/0000-0002-8808-1786; Danilov, Mikhail/0000-0001-9227-5164; Uglov, Timofey/0000-0002-4944-1830; Chilikin, Kirill/0000-0001-7620-2053; Chistov, Ruslan/0000-0003-1439-8390; Pakhlova, Galina/0000-0001-7518-3022; Cervenkov, Daniel/0000-0002-1865-741X FU Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan; Japan Society for the Promotion of Science (JSPS); Tau-Lepton Physics Research Center of Nagoya University; Australian Research Council; Austrian Science Fund [P 22742-N16, P 26794-N20]; National Natural Science Foundation of China [10575109, 10775142, 10875115, 11175187, 11475187]; Chinese Academy of Science Center for Excellence in Particle Physics; Ministry of Education, Youth and Sports of the Czech Republic [LG14034]; Carl Zeiss Foundation; Deutsche Forschungsgemeinschaft; VolkswagenStiftung; Department of Science and Technology of India; Istituto Nazionale di Fisica Nucleare of Italy; National Research Foundation (NRF) of Korea [2011-0029457, 2012-0008143, 2012R1A1A2008330, 2013R1A1A3007772, 2014R1A2A2A01005286, 2014R1A2A2A01002734, 2015R1A2A2A01003280, 2015H1A2A1033649]; Basic Research Lab program under NRF [KRF-2011-0020333]; Center for Korean J-PARC Users [NRF-2013K1A3A7A06056592]; Brain Korea 21-Plus program; Radiation Science Research Institute; Polish Ministry of Science and Higher Education; National Science Center; Ministry of Education and Science of the Russian Federation; Russian Foundation for Basic Research; Slovenian Research Agency; Basque Foundation for Science (IKERBASQUE) (Spain); Euskal Herriko Unibertsitatea (UPV/EHU) (Spain) [UFI 11/55]; Swiss National Science Foundation; National Science Council; Ministry of Education of Taiwan; U.S. Department of Energy; National Science Foundation; MEXT; JSPS; WCU program of the Ministry of Education FX We thank the KEKB group for the excellent operation of the accelerator; the KEK cryogenics group for the efficient operation of the solenoid; and the KEK computer group, the National Institute of Informatics, and the PNNL/EMSL computing group for valuable computing and SINET4 network support. We acknowledge support from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) of Japan, the Japan Society for the Promotion of Science (JSPS), and the Tau-Lepton Physics Research Center of Nagoya University; the Australian Research Council; Austrian Science Fund under Grants No. P 22742-N16 and No. P 26794-N20; the National Natural Science Foundation of China under Contracts No. 10575109, No. 10775142, No. 10875115, No. 11175187, and No. 11475187; the Chinese Academy of Science Center for Excellence in Particle Physics; the Ministry of Education, Youth and Sports of the Czech Republic under Contract No. LG14034; the Carl Zeiss Foundation, the Deutsche Forschungsgemeinschaft and the VolkswagenStiftung; the Department of Science and Technology of India; the Istituto Nazionale di Fisica Nucleare of Italy; the WCU program of the Ministry of Education, National Research Foundation (NRF) of Korea Grants No. 2011-0029457, No. 2012-0008143, No. 2012R1A1A2008330, No. 2013R1A1A3007772, No. 2014R1A2A2A01005286, No. 2014R1A2A2A01002734, No. 2015R1A2A2A01003280, and No. 2015H1A2A1033649; the Basic Research Lab program under NRF Grant No. KRF-2011-0020333, Center for Korean J-PARC Users, Grant No. NRF-2013K1A3A7A06056592; the Brain Korea 21-Plus program and Radiation Science Research Institute; the Polish Ministry of Science and Higher Education and the National Science Center; the Ministry of Education and Science of the Russian Federation and the Russian Foundation for Basic Research; the Slovenian Research Agency; the Basque Foundation for Science (IKERBASQUE) and the Euskal Herriko Unibertsitatea (UPV/EHU) under program Grant No. UFI 11/55 (Spain); the Swiss National Science Foundation; the National Science Council and the Ministry of Education of Taiwan; and the U.S. Department of Energy and the National Science Foundation. This work is supported by a Grant-in-Aid from MEXT for Science Research in a Priority Area ("New Development of Flavor Physics"), for Scientific Research on Innovative Areas ("Elucidation of New Hadrons with a Variety of Flavors"), and from JSPS for Creative Scientific Research ("Evolution of Tau-lepton Physics"). NR 33 TC 1 Z9 1 U1 3 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 29 PY 2016 VL 93 IS 5 AR 052016 DI 10.1103/PhysRevD.93.052016 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH9HE UT WOS:000373106200002 ER PT J AU Sanchez, PD Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyakov, SI Skovpen, YI Solodov, EP Todyshev, KY Lankford, AJ Gary, JW Long, O Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Vazquez, WP Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Kim, J Miyashita, TS Ongmongkolkul, P Porter, FC Rohrken, M Andreassen, R Huard, Z Meadows, BT Pushpawela, BG Sokoloff, MD Sun, L Ford, WT Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Santoro, V Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Zallo, A Contri, R Monge, MR Passaggio, S Patrignani, C Bhuyan, B Prasad, V Adametz, A Uwer, U Lacker, HM Mallik, U Chen, C Cochran, J Prell, S Ahmed, H Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Schubert, KR Barlow, RJ Lafferty, GD Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Cheaib, R Patel, PM Robertson, SH Dey, B Neri, N Palombo, F Cremaldi, L Godang, R Summers, DJ Simard, M Taras, P De Nardo, G Onorato, G Sciacca, C Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Biasini, M Manoni, E Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Chrzaszcz, M Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Rama, M Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Anulli, F Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Pilloni, A Piredda, G Bunger, C Dittrich, S Grunberg, O Hess, M Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S Vasseur, G Aston, D Bard, DJ Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Graham, MT Hast, C Innes, WR Kim, P Leith, DWGS Luitz, S Luth, V MacFarlane, DB Muller, DR Neal, H Pulliam, T Ratcliff, BN Roodman, A Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wisniewski, WJ Wulsin, HW Purohit, MV Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Schwitters, RF Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Albert, J Banerjee, S Beaulieu, A Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Sanchez, P. del Amo Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyakov, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Lankford, A. J. Gary, J. W. Long, O. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Vazquez, W. Panduro Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Kim, J. Miyashita, T. S. Ongmongkolkul, P. Porter, F. C. Roehrken, M. Andreassen, R. Huard, Z. Meadows, B. T. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Ford, W. T. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Santoro, V. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Zallo, A. Contri, R. Monge, M. R. Passaggio, S. Patrignani, C. Bhuyan, B. Prasad, V. Adametz, A. Uwer, U. Lacker, H. M. Mallik, U. Chen, C. Cochran, J. Prell, S. Ahmed, H. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Cheaib, R. Patel, P. M. Robertson, S. H. Dey, B. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Onorato, G. Sciacca, C. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Biasini, M. Manoni, E. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Chrzaszcz, M. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Rama, M. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Anulli, F. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Pilloni, A. Piredda, G. Buenger, C. Dittrich, S. Gruenberg, O. Hess, M. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. Vasseur, G. Aston, D. Bard, D. J. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Leith, D. W. G. S. Luitz, S. Luth, V. MacFarlane, D. B. Muller, D. R. Neal, H. Pulliam, T. Ratcliff, B. N. Roodman, A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wisniewski, W. J. Wulsin, H. W. Purohit, M. V. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Schwitters, R. F. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Albert, J. Banerjee, Sw. Beaulieu, A. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BaBaR Collaboration TI Time-dependent analysis of B-0 -> K-S(0)pi(-)pi(+)gamma decays and studies of the K+pi(-)pi(+) system in B+ -> K+pi(-)pi(+)gamma decays SO PHYSICAL REVIEW D LA English DT Article ID BABAR DETECTOR; STANDARD MODEL; MESONS AB We measure the time-dependent CP asymmetry in the radiative-penguin decay B-0 -> K-S(0)pi(-)pi(+)gamma, using a sample of 471 x 10(6) Upsilon(4S) -> B (B) over bar events recorded with the BABAR detector at the PEP-II e(+)(e) over tilde (-) storage ring at SLAC. Using events with m(K pi pi) < 1.8 GeV/c(2), we measure the branching fractions of B+ -> K+pi(-)pi(+)gamma and B-0 -> K-S(0)pi(-)pi(+)gamma, the branching fractions of the kaonic resonances decaying to K+pi(-)pi(+)gamma, as well as the overall branching fractions of the B+ -> rho K-0(+.)gamma, B+ -> K*(0)pi(+)gamma. and S-wave B+ -> (K pi)(0)(*0) pi(+)gamma components. For events from the rho mass band, we measure the CP-violating parameters SKS0 pi+pi-gamma = 0.14 +/- 0.25 +/- 0.03 and CKS0 pi+pi-gamma = -0.39 +/- 0.20(-0.02)(+0.003), where the first uncertainties are statistical and the second are systematic. We extract from this measurement the time-dependent CP asymmetry related to the CP eigenstate rho K-0(S)0 and obtain S-KS(0) = -0.18 +/- 0.32(-0.05)(+0.06), which provides information on the photon polarization in the underlying b -> s gamma transition. C1 [Sanchez, P. del Amo; Lees, J. P.; Poireau, V.; Tisserand, V.] Univ Savoie, CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules LAPP, F-74941 Annecy Le Vieux, France. [Grauges, E.; Bozzi, C.] Univ Barcelona, Fac Fis, Dept ECM, E-08028 Barcelona, Spain. [Palano, A.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Palano, A.] Univ Bari, Dipartimento Fis, I-70126 Bari, Italy. [Eigen, G.; Stugu, B.] Univ Bergen, Inst Phys, N-5007 Bergen, Norway. [Brown, D. N.; Kerth, L. T.; Kolomensky, Yu. 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[Palombo, F.] Univ Milan, Dipartimento Fis, Via Celoria 16, I-20133 Milan, Italy. [Cremaldi, L.; Godang, R.; Summers, D. J.] Univ Mississippi, University, MS 38677 USA. [Simard, M.; Taras, P.] Univ Montreal, Phys Particules, Montreal, PQ H3C 3J7, Canada. [De Nardo, G.; Onorato, G.; Sciacca, C.] Ist Nazl Fis Nucl, Sez Napoli, I-80126 Naples, Italy. [De Nardo, G.; Onorato, G.; Sciacca, C.] Univ Naples Federico II, Dipartimento Sci Fis, I-80126 Naples, Italy. [Raven, G.] Natl Inst Nucl Phys & High Energy Phys, NIKHEF, NL-1009 DB Amsterdam, Netherlands. [Jessop, C. P.; LoSecco, J. M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Honscheid, K.; Kass, R.] Ohio State Univ, Columbus, OH 43210 USA. [Margoni, M.; Morandin, M.; Posocco, M.; Rotondo, M.; Simi, G.; Simonetto, F.; Stroili, R.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Margoni, M.; Simi, G.; Simonetto, F.; Stroili, R.] Univ Padua, Dipartimento Fis, I-35131 Padua, Italy. [Akar, S.; Ben-Haim, E.; Bomben, M.; Bonneaud, G. R.; Briand, H.; Calderini, G.; Chauveau, J.; Leruste, Ph.; Marchiori, G.; Ocariz, J.] Univ Paris 07, CNRS, IN2P3, Univ Paris 06,Lab Phys Nucl & Hautes Energies, F-75252 Paris, France. [Biasini, M.; Manoni, E.; Rossi, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Biasini, M.] Univ Perugia, Dipartimento Fis, I-06123 Perugia, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Chrzaszcz, M.; Forti, F.; Giorgi, M. A.; Lusiani, A.; Oberhof, B.; Paoloni, E.; Rama, M.; Rizzo, G.; Walsh, J. J.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Forti, F.; Giorgi, M. A.; Oberhof, B.; Paoloni, E.; Rizzo, G.] Univ Pisa, Dipartimento Fis, I-56127 Pisa, Italy. [Lusiani, A.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Pegna, D. Lopes; Olsen, J.; Smith, A. J. S.] Princeton Univ, Princeton, NJ 08544 USA. [Anulli, F.; Faccini, R.; Ferrarotto, F.; Ferroni, F.; Gaspero, M.; Pilloni, A.; Piredda, G.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Faccini, R.; Ferroni, F.; Gaspero, M.; Pilloni, A.] Univ Rome, Dipartimento Fis, I-00185 Rome, Italy. [Buenger, C.; Dittrich, S.; Gruenberg, O.; Hess, M.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; Vasseur, G.] CEA, Irfu, SPP, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Aston, D.; Bard, D. J.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Leith, D. W. G. S.; Luitz, S.; Luth, V.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wisniewski, W. J.; Wulsin, H. W.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Purohit, M. V.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.; Spanier, S. M.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Schwitters, R. F.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.] Univ Turin, Dipartimento Fis, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Albert, J.; Banerjee, Sw.; Beaulieu, A.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Ayad, R.] Univ Tabuk, Tabuk 71491, Saudi Arabia. [Malaescu, B.] CNRS, IN2P3, Lab Phys Nucl & Hautes Energies, F-75252 Paris, France. [Barlow, R. J.] Univ Huddersfield, Huddersfield HD1 3DH, W Yorkshire, England. [Godang, R.] Univ S Alabama, Mobile, AL 36688 USA. [Carpinelli, M.] Univ Sassari, I-07100 Sassari, Italy. RP Sanchez, PD (reprint author), Univ Savoie, CNRS, IN2P3, Lab Annecy Le Vieux Phys Particules LAPP, F-74941 Annecy Le Vieux, France. RI Patrignani, Claudia/C-5223-2009; Kravchenko, Evgeniy/F-5457-2015; Di Lodovico, Francesca/L-9109-2016; bettarini, stefano/M-2502-2016; Calcaterra, Alessandro/P-5260-2015; OI Patrignani, Claudia/0000-0002-5882-1747; Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Bettarini, Stefano/0000-0001-7742-2998 FU U.S. Department of Energy (Canada); National Science Foundation (Canada); Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique (France); Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung (Germany); Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (Netherlands); Research Council of Norway; Ministry of Education and Science of the Russian Federation; Ministerio de Ciencia e Innovacion (Spain); Science and Technology Facilities Council (United Kingdom); Marie-Curie IEF program (European Union); A. P. Sloan Foundation (USA); Binational Science Foundation (USA-Israel) FX We thank E. Kou for help throughout the analysis, especially with the computation of the dilution factor, and A. Le Yaouanc for valuable discussions. We are grateful for the extraordinary contributions of our PEP-II2 colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the U.S. Department of Energy and National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Ciencia e Innovacion (Spain), and the Science and Technology Facilities Council (United Kingdom). Individuals have received support from the Marie-Curie IEF program (European Union), the A. P. Sloan Foundation (USA) and the Binational Science Foundation (USA-Israel). NR 40 TC 2 Z9 2 U1 4 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 29 PY 2016 VL 93 IS 5 AR 052013 DI 10.1103/PhysRevD.93.052013 PG 29 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH9HE UT WOS:000373106200001 ER PT J AU van der Plas, F Manning, P Soliveres, S Allan, E Scherer-Lorenzen, M Verheyen, K Wirth, C Zavala, MA Ampoorter, E Baeten, L Barbaro, L Bauhus, J Benavides, R Benneter, A Bonal, D Bouriaud, O Bruelheide, H Bussotti, F Carnol, M Castagneyroli, B Charbonnier, Y Coomes, DA Coppi, A Bestias, CC Dawud, SM De Wandeler, H Domisch, T Finer, L Gessler, A Granier, A Grossiord, C Guyot, V Hattenschwiler, S Jactel, H Jaroszewicz, B Joly, FX Jucker, T Koricheva, J Milligan, H Mueller, S Muys, B Nguyen, D Pollastrini, M Ratcliffe, S Raulund-Rasmussen, K Selvi, F Stenlid, J Valladares, F Vesterdal, L Zielinski, D Fischer, M AF van der Plas, Fons Manning, Pete Soliveres, Santiago Allan, Eric Scherer-Lorenzen, Michael Verheyen, Kris Wirth, Christian Zavala, Miguel A. Ampoorter, Evy Baeten, Lander Barbaro, Luc Bauhus, Juergen Benavides, Raquel Benneter, Adam Bonal, Damien Bouriaud, Olivier Bruelheide, Helge Bussotti, Filippo Carnol, Monique Castagneyroli, Bastien Charbonnier, Yohan Coomes, David Anthony Coppi, Andrea Bestias, Cristina C. Dawud, Seid Muhie De Wandeler, Hans Domisch, Timo Finer, Leena Gessler, Arthur Granier, Andre Grossiord, Charlotte Guyot, Virginie Haettenschwiler, Stephan Jactel, Herve Jaroszewicz, Bogdan Joly, Franois-Xavier Jucker, Tommaso Koricheva, Julia Milligan, Harriet Mueller, Sandra Muys, Bart Nguyen, Diem Pollastrini, Martina Ratcliffe, Sophia Raulund-Rasmussen, Karsten Selvi, Federico Stenlid, Jan Valladares, Fernando Vesterdal, Lars Zielinski, Dawid Fischer, Markus TI Biotic homogenization can decrease landscape-scale forest multifunctionality SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE beta-diversity; biodiversity; ecosystem functioning; FunDivEUROPE; spatial scale ID MULTIPLE ECOSYSTEM SERVICES; LAND-USE; SPECIES RICHNESS; BIODIVERSITY; DIVERSITY; INTENSIFICATION; PERSPECTIVES; METAANALYSIS; STABILITY; TRAITS AB Many experiments have shown that local biodiversity loss impairs the ability of ecosystems to maintain multiple ecosystem functions at high levels (multifunctionality). In contrast, the role of biodiversity in driving ecosystem multifunctionality at landscape scales remains unresolved. We used a comprehensive pan-European dataset, including 16 ecosystem functions measured in 209 forest plots across six European countries, and performed simulations to investigate how local plot-scale richness of tree species (alpha-diversity) and their turnover between plots (beta-diversity) are related to landscape-scale multifunctionality. After accounting for variation in environmental conditions, we found that relationships between alpha-diversity and landscape-scale multifunctionality varied from positive to negative depending on the multifunctionality metric used. In contrast, when significant, relationships between beta-diversity and landscape-scale multifunctionality were always positive, because a high spatial turnover in species composition was closely related to a high spatial turnover in functions that were supported at high levels. Our findings have major implications for forest management and indicate that biotic homogenization can have previously unrecognized and negative consequences for large-scale ecosystem multifunctionality. C1 [van der Plas, Fons; Manning, Pete; Soliveres, Santiago; Allan, Eric; Fischer, Markus] Univ Bern, Inst Plant Sci, Plant Ecol Grp, CH-3013 Bern, Switzerland. [van der Plas, Fons; Manning, Pete; Fischer, Markus] Senckenberg Gesellsch Nat Forsch, Biodivers & Climate Res Ctr, D-60325 Frankfurt, Germany. [Scherer-Lorenzen, Michael; Benavides, Raquel; Mueller, Sandra] Univ Freiburg, Fac Biol Geobot, D-79104 Freiburg, Germany. [Verheyen, Kris; Ampoorter, Evy; Baeten, Lander] Univ Ghent, Dept Forest & Water Management, Forest & Nat Lab, B-9000 Ghent, Belgium. [Wirth, Christian; Ratcliffe, Sophia] Univ Leipzig, Systemat Bot & Funct Biodivers Study Grp, D-04103 Leipzig, Germany. [Wirth, Christian] German Ctr Integrat Biodivers Res iDiv, D-04103 Leipzig, Germany. [Zavala, Miguel A.] Univ Alcala de Henares, Dept Life Sci, Forest Ecol & Restorat Grp, Madrid 28805, Spain. [Baeten, Lander] Univ Ghent, Dept Biol, Terr Ecol Unit, B-9000 Ghent, Belgium. [Barbaro, Luc; Castagneyroli, Bastien; Charbonnier, Yohan; Guyot, Virginie; Jactel, Herve] INRA, Biodivers Genes & Communautes BIOGECO, F-33610 Cestas, France. [Barbaro, Luc; Castagneyroli, Bastien; Charbonnier, Yohan; Guyot, Virginie; Jactel, Herve] Univ Bordeaux, Biodivers Genes & Communautes, UMR 1202, F-33600 Pessac, France. [Bauhus, Juergen; Benneter, Adam] Univ Freiburg, Fac Environm & Nat Resources, D-79085 Freiburg, Germany. [Bonal, Damien; Granier, Andre] INRA, UMR Ecol & Ecophysiol Forestieres, F-54280 Champenoux, France. [Bouriaud, Olivier] Stefan cel Mare Univ Suceava, Fac Forestry, Suceava 720229, Romania. [Bruelheide, Helge] Univ Halle Wittenberg, Inst Biol, Geobot & Bot Garden, D-06108 Halle, Germany. [Bussotti, Filippo; Coppi, Andrea; Pollastrini, Martina; Selvi, Federico] Univ Florence, Dept Agrifood Prod & Environm Sci, Lab Appl & Environm Bot, I-50144 Florence, Italy. [Carnol, Monique] Univ Liege, Dept Biol Ecol Evolut, Lab Plant & Microbial Ecol, B-4000 Cointe Ougree, Belgium. [Coomes, David Anthony] Univ Cambridge, Dept Plant Sci, Forest Ecol & Conservat, Cambridge CB2 3EA, England. [Bestias, Cristina C.; Valladares, Fernando] CSIC, Natl Museum Nat Sci MNCN, Dept Biogeog & Global Change, Plaza Murillo 2, E-28006 Madrid, Spain. [Dawud, Seid Muhie; Vesterdal, Lars] Univ Copenhagen, Dept Geosci & Nat Resource Management, DK-1958 Frederiksberg C, Denmark. [De Wandeler, Hans; Muys, Bart] Katholieke Univ Leuven, Dept Earth & Environm Sci, Div Forest Nat & Landscape, KU Leuven, BE-3001 Leuven, Belgium. [Domisch, Timo; Finer, Leena] Nat Resources Inst Finland, FI-80101 Joensuu, Finland. [Gessler, Arthur] Swiss Fed Inst Forest Snow & Landscape Res, CH-8903 Birmensdorf, Switzerland. [Grossiord, Charlotte] Los Alamos Natl Lab, Earth & Environm Sci Div, POB 1663, Los Alamos, NM 87545 USA. [Guyot, Virginie] INRA, UMR 1201, Dynam & Ecol Forest Landscapes, F-31326 Castanet Tolosan, France. [Haettenschwiler, Stephan; Joly, Franois-Xavier] Univ Montpellier, Univ Paul Valery Montpellier, Ecole Prat Hautes Etud, Ctr Evolutionary & Funct Ecol UMR 5175, F-34293 Montpellier 5, France. [Jaroszewicz, Bogdan; Zielinski, Dawid] Univ Warsaw, Fac Biol, Bialowieza Geobot Stn, PL-17230 Bialowieza, Poland. [Koricheva, Julia; Milligan, Harriet] Univ London, Sch Biol Sci, Ecol Evolut & Behav, Egham TW20 0EX, Surrey, England. [Nguyen, Diem; Stenlid, Jan] Swedish Univ Agr Sci, Dept Forest Mycol & Plant Pathol, SE-75007 Uppsala, Sweden. [Valladares, Fernando] Univ Rey Juan Carlos, Escuela Super Ciencias Expt & Tecnol, Dept Biol & Geol, Mostoles 28933, Spain. [Fischer, Markus] Univ Bern, Oeschger Ctr Climate Change Res, CH-3012 Bern, Switzerland. [Bussotti, Filippo] Univ Florence, Dept Biol, I-50121 Florence, Italy. RP van der Plas, F (reprint author), Univ Bern, Inst Plant Sci, Plant Ecol Grp, CH-3013 Bern, Switzerland.; van der Plas, F (reprint author), Senckenberg Gesellsch Nat Forsch, Biodivers & Climate Res Ctr, D-60325 Frankfurt, Germany. EM fonsvanderplas@gmail.com RI Coppi, Andrea/D-2886-2016; Fischer, Markus/C-6411-2008; Gessler, Arthur/C-7121-2008; Bouriaud, Olivier/C-4700-2011; Raulund-Rasmussen, Karsten/E-8424-2015; Manning, Peter/I-6523-2012; Suceava, USV/E-8611-2011; Zavala, Miguel/H-3603-2015; Bauhus, Jurgen/G-4449-2013; Vesterdal, Lars/D-5227-2011; Pollastrini, Martina/N-7989-2014; Bastias, Cristina C. /C-3657-2017 OI Baeten, Lander/0000-0003-4262-9221; Castagneyrol, Bastien/0000-0001-8795-7806; DAWUD, SEID MUHIE/0000-0002-5587-945X; Coppi, Andrea/0000-0003-4760-8403; Benavides, Raquel/0000-0003-2328-5371; Soliveres Codina, Santiago/0000-0001-9661-7192; Nguyen, Diem/0000-0002-9680-5772; Jucker, Tommaso/0000-0002-0751-6312; Fischer, Markus/0000-0002-5589-5900; Gessler, Arthur/0000-0002-1910-9589; Bouriaud, Olivier/0000-0002-8046-466X; Raulund-Rasmussen, Karsten/0000-0003-1573-1167; Manning, Peter/0000-0002-7940-2023; Zavala, Miguel/0000-0003-1456-0132; Bauhus, Jurgen/0000-0002-9673-4986; Vesterdal, Lars/0000-0003-0309-3735; Pollastrini, Martina/0000-0003-0959-9489; Bastias, Cristina C. /0000-0002-2479-2001 FU European Union [265171] FX We thank the Hainich National Park administration as well as Felix Berthold and Carsten Beinhoff for support of this study and Gerald Kaendler and the Johann Heinrich von Thunen-Institut for providing access to the German National Forest Inventory data. The research leading to these results received funding from the European Union Seventh Framework Programme (FP7/2007-2013) under Grant Agreement 265171. NR 52 TC 8 Z9 8 U1 34 U2 71 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 29 PY 2016 VL 113 IS 13 BP 3557 EP 3562 DI 10.1073/pnas.1517903113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH6BQ UT WOS:000372876400054 PM 26979952 ER PT J AU Stingaciu, LR Ivanova, O Ohl, M Biehl, R Richter, D AF Stingaciu, Laura R. Ivanova, Oxana Ohl, Michael Biehl, Ralf Richter, Dieter TI Fast antibody fragment motion: flexible linkers act as entropic spring SO SCIENTIFIC REPORTS LA English DT Article ID X-RAY-SCATTERING; IMMUNOGLOBULIN-G ANTIBODY; SEGMENTAL FLEXIBILITY; NEUTRON-SCATTERING; CRYSTALLOGRAPHIC REFINEMENT; HYDRODYNAMIC INTERACTIONS; CONCENTRATED SUSPENSION; MONOCLONAL-ANTIBODIES; ROTATIONAL DIFFUSION; LIGHT-SCATTERING AB A flexible linker region between three fragments allows antibodies to adjust their binding sites to an antigen or receptor. Using Neutron Spin Echo Spectroscopy we observed fragment motion on a timescale of 7 ns with motional amplitudes of about 1 nm relative to each other. The mechanistic complexity of the linker region can be described by a spring model with Brownian motion of the fragments in a harmonic potential. Displacements, timescale, friction and force constant of the underlying dynamics are accessed. The force constant exhibits a similar strength to an entropic spring, with friction of the fragment matching the unbound state. The observed fast motions are fluctuations in pre-existing equilibrium configurations. The Brownian motion of domains in a harmonic potential is the appropriate model to examine functional hinge motions dependent on the structural topology and highlights the role of internal forces and friction to function. C1 [Stingaciu, Laura R.; Ohl, Michael] Oak Ridge Natl Lab, Forschungszentrum Julich, JCNS, Outstn SNS, Oak Ridge, TN 37831 USA. [Ivanova, Oxana] Forschungszentrum Julich, JCNS, Outstn MLZ, D-85747 Garching, Germany. [Biehl, Ralf; Richter, Dieter] Forschungszentrum Julich, JCNS, JCNS 1, D-52425 Julich, Germany. [Biehl, Ralf; Richter, Dieter] Forschungszentrum Julich, ICS 1, D-52425 Julich, Germany. RP Biehl, R (reprint author), Forschungszentrum Julich, JCNS, JCNS 1, D-52425 Julich, Germany.; Biehl, R (reprint author), Forschungszentrum Julich, ICS 1, D-52425 Julich, Germany. EM ra.biehl@fz-juelich.de RI Ivanova, Oxana/B-5939-2016; OI Ivanova, Oxana/0000-0003-4888-942X; Stingaciu, Laura/0000-0003-2696-5233 NR 61 TC 2 Z9 2 U1 5 U2 14 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 29 PY 2016 VL 6 AR 22148 DI 10.1038/srep22148 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH6PZ UT WOS:000372914800001 PM 27020739 ER PT J AU Zhu, WH Shi, MR Yu, D Liu, CX Huang, TL Wu, FC AF Zhu, Weihuang Shi, Mengran Yu, Dan Liu, Chongxuan Huang, Tinglin Wu, Fengchang TI Characteristics and Kinetic Analysis of AQS Transformation and Microbial Goethite Reduction: Insight into "Redox mediator-Microbe-Iron oxide" Interaction Process SO SCIENTIFIC REPORTS LA English DT Article ID ELECTRON-TRANSFER; HUMIC SUBSTANCES; SHEWANELLA-PUTREFACIENS; ANAEROBIC RESPIRATION; FE(III) REDUCTION; GAMMA-FEOOH; FERRIHYDRITE; HEMATITE; AQDS; ANTHRAQUINONE-2,6-DISULFONATE AB The characteristics and kinetics of redox transformation of a redox mediator, anthraquinone-2-sulfonate (AQS), during microbial goethite reduction by Shewanella decolorationis S12, a dissimilatory iron reduction bacterium (DIRB), were investigated to provide insights into "redox mediator-iron oxide" interaction in the presence of DIRB. Two pre-incubation reaction systems of the "strain S12-goethite" and the "strain S12-AQS" were used to investigate the dynamics of goethite reduction and AQS redox transformation. Results show that the concentrations of goethite and redox mediator, and the inoculation cell density all affect the characteristics of microbial goethite reduction, kinetic transformation between oxidized and reduced species of the redox mediator. Both abiotic and biotic reactions and their coupling regulate the kinetic process for "Quinone-Iron" interaction in the presence of DIRB. Our results provide some new insights into the characteristics and mechanisms of interaction among "quinone-DIRB-goethite" under biotic/abiotic driven. C1 [Zhu, Weihuang; Shi, Mengran; Yu, Dan; Huang, Tinglin] Xian Univ Architecture & Technol, Minist Educ, Key Lab Northwest Water Resources, Xian 710055, Peoples R China. [Liu, Chongxuan] Pacific NW Natl Lab, Richland, WA 99352 USA. [Wu, Fengchang] Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China. RP Zhu, WH (reprint author), Xian Univ Architecture & Technol, Minist Educ, Key Lab Northwest Water Resources, Xian 710055, Peoples R China. EM zhuweihuang@gmail.com RI Liu, Chongxuan/C-5580-2009 FU Chinese National Natural Science Foundation [41373093, 41173095, 40903042]; Natural Science Foundation of Shaanxi province [2015JM5169] FX This research was supported by the Chinese National Natural Science Foundation (No. 41373093, 41173095, 40903042) and the Natural Science Foundation of Shaanxi province (No. 2015JM5169). NR 32 TC 0 Z9 0 U1 11 U2 30 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 29 PY 2016 VL 6 AR 23718 DI 10.1038/srep23718 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH6SM UT WOS:000372921800002 PM 27020166 ER PT J AU Yoshida, M Ishii, K Naka, M Ishihara, S Jarrige, I Ikeuchi, K Murakami, Y Kudo, K Koike, Y Nagata, T Fukada, Y Ikeda, N Mizuki, J AF Yoshida, M. Ishii, K. Naka, M. Ishihara, S. Jarrige, I. Ikeuchi, K. Murakami, Y. Kudo, K. Koike, Y. Nagata, T. Fukada, Y. Ikeda, N. Mizuki, J. TI Observation of momentum-resolved charge fluctuations proximate to the charge-order phase using resonant inelastic x-ray scattering SO SCIENTIFIC REPORTS LA English DT Article ID LADDER; SR14-XCAXCU24O41; SR14CU24O41; TRANSPORT; CA; SR(14-X)A(X)CU(24)O(41) AB In strongly correlated electron systems, enhanced fluctuations in the proximity of the ordered states of electronic degrees of freedom often induce anomalous electronic properties such as unconventional superconductivity. While spin fluctuations in the energy-momentum space have been studied widely using inelastic neutron scattering, other degrees of freedom, i.e., charge and orbital, have hardly been explored thus far. Here, we use resonant inelastic x-ray scattering to observe charge fluctuations proximate to the charge-order phase in transition metal oxides. In the two-leg ladder of Sr14-xCaxCu24O41, charge fluctuations are enhanced at the propagation vector of the charge order (q(CO)) when the order is melted by raising temperature or by doping holes. In contrast, charge fluctuations are observed not only at q(CO) but also at other momenta in a geometrically frustrated triangular bilayer lattice of LuFe2O4. The observed charge fluctuations have a high energy (similar to 1 eV), suggesting that the Coulomb repulsion between electrons plays an important role in the formation of the charge order. C1 [Yoshida, M.; Ishii, K.; Jarrige, I.; Ikeuchi, K.; Mizuki, J.] Japan Atom Energy Agcy, SPring 8, Sayo, Hyogo 6795148, Japan. [Yoshida, M.; Ishihara, S.] Tohoku Univ, Grad Sch Sci, Dept Phys, Sendai, Miyagi 9808578, Japan. [Naka, M.] RIKEN, CEMS, Wako, Saitama 3510198, Japan. [Ishihara, S.] JST, CREST, Chiyoda Ku, Tokyo 1020076, Japan. [Ikeuchi, K.] CROSS, Res Ctr Neutron Sci & Technol, Tokai, Ibaraki 3191106, Japan. [Murakami, Y.] High Energy Accelerator Res Org, Inst Mat Struct Sci, Tsukuba, Ibaraki 3050801, Japan. [Kudo, K.; Nagata, T.; Fukada, Y.; Ikeda, N.] Okayama Univ, Dept Phys, Okayama 7008530, Japan. [Koike, Y.] Tohoku Univ, Grad Sch Engn, Dept Appl Phys, Sendai, Miyagi 9808579, Japan. [Mizuki, J.] Kwansei Gakuin Univ, Sch Sci & Technol, Sanda, Hyogo 6691337, Japan. [Jarrige, I.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. RP Ishii, K (reprint author), Japan Atom Energy Agcy, SPring 8, Sayo, Hyogo 6795148, Japan. EM kenji@spring8.or.jp RI KUDO, Kazutaka/B-1468-2011 FU JSPS KAKENHI [25400333, 25400372, 15H01047] FX The authors thank K. Iwasa, H. Seo, K. Tsutsui, K. Yoshii, and T. Tohyama for their valuable discussions. The RIXS experiments at BL11XU of SPring-8 were performed with the approval of the Japan Synchrotron Radiation Research Institute (JASRI). This work was financially supported by JSPS KAKENHI Grant Number 25400333, 25400372, and 15H01047. NR 42 TC 0 Z9 0 U1 4 U2 16 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 29 PY 2016 VL 6 AR 23611 DI 10.1038/srep23611 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH6RE UT WOS:000372918100001 PM 27021464 ER PT J AU Scullard, CR Jacobsen, JL AF Scullard, Christian R. Jacobsen, Jesper Lykke TI Potts-model critical manifolds revisited SO JOURNAL OF PHYSICS A-MATHEMATICAL AND THEORETICAL LA English DT Article DE Potts model; percolation; critical polynomials; critical thresholds ID PERCOLATION THRESHOLDS; 2 DIMENSIONS; LATTICES; PHASE AB We compute critical polynomials for the q-state Potts model on the Archimedean lattices, using a parallel implementation of the algorithm of Jacobsen (2014 J. Phys. A: Math. Theor 47 135001) that gives us access to larger sizes than previously possible. The exact polynomials are computed for bases of size 6 x 6 unit cells, and the root in the temperature variable v = e(K) - 1 is determined numerically at q = 1 for bases of size 8 x 8. This leads to improved results for bond percolation thresholds, and for the Potts-model critical manifolds in the real (q, v) plane. In the two most favourable cases, we find now the kagome-lattice threshold to eleven digits and that of the (3, 12(2)) lattice to thirteen. Our critical manifolds reveal many interesting features in the antiferromagnetic region of the Potts model, and determine accurately the extent of the Berker-Kadanoff phase for the lattices studied. C1 [Scullard, Christian R.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Jacobsen, Jesper Lykke] PSL Res Univ, Ecole Normale Super, LPTENS, 24 Rue Lhomond, F-75231 Paris 05, France. [Jacobsen, Jesper Lykke] Univ Paris 06, Sorbonne Univ, CNRS, UMR 8549, F-75005 Paris, France. [Jacobsen, Jesper Lykke] CEA Saclay, Inst Phys Theor, F-91191 Gif Sur Yvette, France. RP Scullard, CR (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM scullard1@llnl.gov; jesper.jacobsen@ens.fr FU U S Department of Energy at the Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Agence Nationale de la Recherche [ANR-10-BLAN-0414]; European Research Council (advanced grant NuCFT); Institut Universitaire de France FX CRS acknowledges the helpful advice of Jim Glosli at LLNL in programming the parallel implementation. This work was partially performed under the auspices of the U S Department of Energy at the Lawrence Livermore National Laboratory under Contract No DE-AC52-07NA27344. The research of JLJ is supported by the Agence Nationale de la Recherche (grant ANR-10-BLAN-0414: DIME), the European Research Council (advanced grant NuCFT), and the Institut Universitaire de France. NR 28 TC 1 Z9 1 U1 1 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1751-8113 EI 1751-8121 J9 J PHYS A-MATH THEOR JI J. Phys. A-Math. Theor. PD MAR 29 PY 2016 VL 49 IS 12 AR 125003 DI 10.1088/1751-8113/49/12/125003 PG 17 WC Physics, Multidisciplinary; Physics, Mathematical SC Physics GA DD9WW UT WOS:000370277400005 ER PT J AU Iberi, V Ievlev, AV Vlassiouk, I Jesse, S Kalinin, SV Joy, DC Rondinone, AJ Belianinov, A Ovchinnikova, OS AF Iberi, Vighter Ievlev, Anton V. Vlassiouk, Ivan Jesse, Stephen Kalinin, Sergei V. Joy, David C. Rondinone, Adam J. Belianinov, Alex Ovchinnikova, Olga S. TI Graphene engineering by neon ion beams SO NANOTECHNOLOGY LA English DT Article DE graphene; helium ion microscopy; direct-write lithography; Kelvin probe force microscopy; band excitation force modulation microscopy; Raman; scanning probe microscopy ID CHEMICAL-VAPOR-DEPOSITION; RAMAN-SPECTROSCOPY; FORCE MICROSCOPY; EXCITATION; DEFECTS AB Achieving the ultimate limits of lithographic resolution and material performance necessitates engineering of matter with atomic, molecular, and mesoscale fidelity. With the advent of scanning helium ion microscopy, maskless He+ and Ne+ beam lithography of 2D materials, such as graphene-based nanoelectronics, is coming to the forefront as a tool for fabrication and surface manipulation. However, the effects of using a Ne focused-ion-beam on the fidelity of structures created out of 2D materials have yet to be explored. Here, we will discuss the use of energetic Ne ions in engineering graphene nanostructures and explore their mechanical, electromechanical and chemical properties using scanning probe microscopy (SPM). By using SPM-based techniques such as band excitation (BE) force modulation microscopy, Kelvin probe force microscopy (KPFM) and Raman spectroscopy, we are able to ascertain changes in the mechanical, electrical and optical properties of Ne+ beam milled graphene nanostructures and surrounding regions. Additionally, we are able to link localized defects around the milled graphene to ion milling parameters such as dwell time and number of beam passes in order to characterize the induced changes in mechanical and electromechanical properties of the graphene surface. C1 [Iberi, Vighter; Ievlev, Anton V.; Jesse, Stephen; Kalinin, Sergei V.; Joy, David C.; Rondinone, Adam J.; Belianinov, Alex; Ovchinnikova, Olga S.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Iberi, Vighter; Joy, David C.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Vlassiouk, Ivan] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Ievlev, Anton V.; Jesse, Stephen; Kalinin, Sergei V.; Belianinov, Alex; Ovchinnikova, Olga S.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Ievlev, Anton V.; Jesse, Stephen; Kalinin, Sergei V.; Belianinov, Alex; Ovchinnikova, Olga S.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Iberi, V; Ovchinnikova, OS (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.; Iberi, V (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA.; Ovchinnikova, OS (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM iberivo@ornl.gov; ovchinnikovo@ornl.gov RI Vlassiouk, Ivan/F-9587-2010; Rondinone, Adam/F-6489-2013; Ievlev, Anton/H-3678-2012; OI Vlassiouk, Ivan/0000-0002-5494-0386; Rondinone, Adam/0000-0003-0020-4612; Ievlev, Anton/0000-0003-3645-0508; Belianinov, Alex/0000-0002-3975-4112 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory FX This research was conducted at the Center for Nanophase Materials Sciences, which is a Department of Energy (DOE) Office of Science User Facility. Partial support given by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the US Department of Energy (A B). NR 37 TC 4 Z9 4 U1 11 U2 36 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD MAR 29 PY 2016 VL 27 IS 12 AR 125302 DI 10.1088/0957-4484/27/12/125302 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DE2FT UT WOS:000370442900010 PM 26890062 ER PT J AU Huang, YJ Bharill, S Karandur, D Peterson, SM Marita, M Shi, XJ Kaliszewski, MJ Smith, AW Isacoff, EY Kuriyan, J AF Huang, Yongjian Bharill, Shashank Karandur, Deepti Peterson, Sean M. Marita, Morgan Shi, Xiaojun Kaliszewski, Megan J. Smith, Adam W. Isacoff, Ehud Y. Kuriyan, John TI Molecular basis for multimerization in the activation of the epidermal growth factor receptor SO ELIFE LA English DT Article ID EGF RECEPTOR; ERBB RECEPTORS; KINASE DOMAIN; CELL-SURFACE; LIVING CELLS; LUNG-CANCER; NEGATIVE COOPERATIVITY; ALLOSTERIC ACTIVATION; EXTRACELLULAR DOMAINS; STRUCTURAL-ANALYSIS AB The epidermal growth factor receptor (EGFR) is activated by dimerization, but activation also generates higher-order multimers, whose nature and function are poorly understood. We have characterized ligand-induced dimerization and multimerization of EGFR using single-molecule analysis, and show that multimerization can be blocked by mutations in a specific region of Domain IV of the extracellular module. These mutations reduce autophosphorylation of the C-terminal tail of EGFR and attenuate phosphorylation of phosphatidyl inositol 3-kinase, which is recruited by EGFR. The catalytic activity of EGFR is switched on through allosteric activation of one kinase domain by another, and we show that if this is restricted to dimers, then sites in the tail that are proximal to the kinase domain are phosphorylated in only one subunit. We propose a structural model for EGFR multimerization through self-association of ligand-bound dimers, in which the majority of kinase domains are activated cooperatively, thereby boosting tail phosphorylation. C1 [Huang, Yongjian; Bharill, Shashank; Karandur, Deepti; Peterson, Sean M.; Isacoff, Ehud Y.; Kuriyan, John] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [Huang, Yongjian; Karandur, Deepti; Peterson, Sean M.; Isacoff, Ehud Y.; Kuriyan, John] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Huang, Yongjian; Karandur, Deepti; Peterson, Sean M.; Kuriyan, John] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Huang, Yongjian; Isacoff, Ehud Y.; Kuriyan, John] Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA. [Marita, Morgan; Shi, Xiaojun; Kaliszewski, Megan J.; Smith, Adam W.] Univ Akron, Dept Chem, Akron, OH 44325 USA. [Isacoff, Ehud Y.; Kuriyan, John] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Isacoff, Ehud Y.] Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA. [Kuriyan, John] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Isacoff, EY; Kuriyan, J (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA.; Isacoff, EY; Kuriyan, J (reprint author), Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA.; Kuriyan, J (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA.; Isacoff, EY; Kuriyan, J (reprint author), Univ Calif Berkeley, Biophys Grad Grp, Berkeley, CA 94720 USA.; Smith, AW (reprint author), Univ Akron, Dept Chem, Akron, OH 44325 USA.; Isacoff, EY; Kuriyan, J (reprint author), Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.; Isacoff, EY (reprint author), Univ Calif Berkeley, Helen Wills Neurosci Inst, Berkeley, CA 94720 USA.; Kuriyan, J (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM asmith5@uakron.edu; ehud@berkeley.edu; kuriyan@berkeley.edu FU National Cancer Institute [2RO1CA09650406]; National Institutes of Health [R15EY024451, 1R01GM117051] FX National Cancer Institute 2RO1CA09650406 John Kuriyan; National Institutes of Health R15EY024451 Adam W Smith; National Institutes of Health 1R01GM117051 Ehud Y Isacoff; The funders had no role in study design, data collection and interpretation, or the decision to submit the work for publication. NR 81 TC 5 Z9 5 U1 0 U2 0 PU ELIFE SCIENCES PUBLICATIONS LTD PI CAMBRIDGE PA SHERATON HOUSE, CASTLE PARK, CAMBRIDGE, CB3 0AX, ENGLAND SN 2050-084X J9 ELIFE JI eLife PD MAR 28 PY 2016 VL 5 AR e14107 DI 10.7554/eLife.14107 PG 27 WC Biology SC Life Sciences & Biomedicine - Other Topics GA EB5XC UT WOS:000387453000001 ER PT J AU Oki, NO Edwards, SW AF Oki, Noffisat O. Edwards, Stephen W. TI An integrative data mining approach to identifying adverse outcome pathway signatures SO TOXICOLOGY LA English DT Article DE Adverse outcome pathway (AOP); cpAOP; Steatosis; Glaucoma ID ARYL-HYDROCARBON RECEPTOR; FATTY LIVER-DISEASE; PRIMARY CONGENITAL GLAUCOMA; HUMAN CYP1B1 GENE; HEPATIC STEATOSIS; PEROXISOME PROLIFERATORS; CELL-DIFFERENTIATION; TRUNCATING MUTATIONS; CYTOCHROME P4501B1; LIPID-METABOLISM AB The Adverse Outcome Pathway (AOP) framework is a tool for making biological connections and summarizing key information across different levels of biological organization to connect biological perturbations at the molecular level to adverse outcomes for an individual or population. Computational approaches to explore and determine these connections can accelerate the assembly of AOPs. By leveraging the wealth of publicly available data covering chemical effects on biological systems, computationally-predicted AOPs (cpAOPs) were assembled via data mining of high-throughput screening (HTS) in vitro data, in vivo data and other disease phenotype information. Frequent Itemset Mining (FIM) was used to find associations between the gene targets of ToxCast HTS assays and disease data from Comparative Toxicogenomics Database (CTD) by using the chemicals as the common aggregators between datasets. The method was also used to map gene expression data to disease data from CTD. A cpAOP network was defined by considering genes and diseases as nodes and FIM associations as edges. This network contained 18,283 gene to disease associations for the ToxCast data and 110,253 for CTD gene expression. Two case studies show the value of the cpAOP network by extracting subnetworks focused either on fatty liver disease or the Aryl Hydrocarbon Receptor (AHR). The subnetwork surrounding fatty liver disease included many genes known to play a role in this disease. When querying the cpAOP network with the AHR gene, an interesting subnetwork including glaucoma was identified. While substantial literature exists to support the potential for AHR ligands to elicit glaucoma, it was not explicitly captured in the public annotation information in CTD. The subnetwork from this analysis suggests a cpAOP that includes changes in CYP1B1 expression, which has been previously established in the literature as a primary cause of glaucoma. These case studies highlight the value in integrating multiple data sources when defining cpAOPs for HTS data. (C) 2016 Published by Elsevier Ireland Ltd. C1 [Oki, Noffisat O.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Edwards, Stephen W.] US EPA, Integrated Syst Toxicol Div, Natl Hlth & Environm Effects Res Lab, Off Res & Dev, Res Triangle Pk, NC 27711 USA. RP Edwards, SW (reprint author), 109 TW Alexander Dr,Mail Code B305 01, Res Triangle Pk, NC 27709 USA. EM oki.noffisat@epa.gov; edwards.stephen@epa.gov FU U. S. Environmental Protection Agency FX The authors thank Carolyn Mattingly and the CTD team for invaluable assistance in working with their data. Shannon Bell originally adapted the FIM method for defining cpAOP networks from toxicogenomics data and was extremely helpful in further adapting that workflow for this study. Finally, we thank Rong-Lin Wang and Brian Chorley for constructive comments on the manuscript and Mark Nelms and Christopher Grant for reviewing the supplemental files. The information in this document has been funded wholly (or in part) by the U. S. Environmental Protection Agency. It has been subjected to review by the National Health and Environmental Effects Research Laboratory and approved for publication. Approval does not signify that the contents reflect the views of the Agency, nor does mention of trade names or commercial products constitute endorsement or recommendation for use. NR 57 TC 0 Z9 0 U1 4 U2 10 PU ELSEVIER IRELAND LTD PI CLARE PA ELSEVIER HOUSE, BROOKVALE PLAZA, EAST PARK SHANNON, CO, CLARE, 00000, IRELAND SN 0300-483X J9 TOXICOLOGY JI Toxicology PD MAR 28 PY 2016 VL 350 BP 49 EP 61 DI 10.1016/j.tox.2016.04.004 PG 13 WC Pharmacology & Pharmacy; Toxicology SC Pharmacology & Pharmacy; Toxicology GA DO4GJ UT WOS:000377739500006 PM 27108252 ER PT J AU Bennett, T Nirooman, H Pamu, R Ivanov, I Mukherjee, D Khomami, B AF Bennett, Tyler Nirooman, Hanieh Pamu, Ravi Ivanov, Ilia Mukherjee, Dibyendu Khomami, Bamin TI Elucidating the role of methyl viologen as a scavenger of photoactivated electrons from photosystem I under aerobic and anaerobic conditions SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID SELF-ASSEMBLED MONOLAYERS; PHOTOCURRENT GENERATION; ENERGY-CONVERSION; CARBON NANOTUBES; ELECTROCHEMISTRY; PROTEIN; FILMS; FABRICATION; COMPLEXES; SURFACES AB We present detailed electrochemical investigations into the role of dissolved O-2 in electrolyte solutions in scavenging photoactivated electrons from a uniform photosystem I (PS I) monolayer assembled on alkanethiolate SAM (self-assembled monolayer)/Au surfaces while using methyl viologen (MV2+) as the redox mediator. To this end, we report results for direct measurements of light induced photocurrent from uniform monolayer assemblies of PS I on C9 alkanethiolate SAM/Au surfaces. These measurements, apart from demonstrating the ability of dissolved O-2 in the electrolyte medium to act as an electron scavenger, also reveal its essential role in driving the solution-phase methyl viologen to initiate light-induced directional electron transfer from an electron donor surface (Au) via surface assembled PS I trimers. Specifically, our systematic electrochemical measurements have revealed that the dissolved O-2 in aqueous electrolyte solutions form a complex intermediate species with MV that plays the essential role in mediating redox pathways for unidirectional electron transfer processes. This critical insight into the redox-mediated electron transfer pathways allows for rational design of electron scavengers through systematic tuning of mediator combinations that promote such intermediate formation. Our current findings facilitate the incorporation of PS I-based bio-hybrid constructs as photo-anodes in future photoelectrochemical cells and bio-electronic devices. C1 [Bennett, Tyler; Nirooman, Hanieh; Mukherjee, Dibyendu; Khomami, Bamin] Univ Tennessee, Dept Chem & Biomol Engn, MRAIL, Knoxville, TN 37996 USA. [Bennett, Tyler; Nirooman, Hanieh; Mukherjee, Dibyendu; Khomami, Bamin] Univ Tennessee, SEERC, Knoxville, TN 37996 USA. [Pamu, Ravi; Mukherjee, Dibyendu; Khomami, Bamin] Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA. [Ivanov, Ilia] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Mukherjee, D; Khomami, B (reprint author), Univ Tennessee, Dept Chem & Biomol Engn, MRAIL, Knoxville, TN 37996 USA.; Mukherjee, D; Khomami, B (reprint author), Univ Tennessee, SEERC, Knoxville, TN 37996 USA.; Mukherjee, D; Khomami, B (reprint author), Univ Tennessee, Dept Mech Aerosp & Biomed Engn, Knoxville, TN 37996 USA. EM dmukherj@utk.edu; bkhomami@utk.edu RI ivanov, ilia/D-3402-2015; Mukherjee, Dibyendu/A-9787-2010 OI ivanov, ilia/0000-0002-6726-2502; Mukherjee, Dibyendu/0000-0002-9232-6774 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX B. K. would like to acknowledge the National Science Foundation (EPS-1004083) and the Gibson Family Foundation. A portion of this research was conducted at the Center for Nanophase Materials Sciences (CNMS), which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 35 TC 1 Z9 1 U1 5 U2 13 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAR 28 PY 2016 VL 18 IS 12 BP 8512 EP 8521 DI 10.1039/c6cp00049e PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG7FB UT WOS:000372249100021 PM 26941212 ER PT J AU Krechkivska, O Wilcox, CM Troy, TP Nauta, K Chan, B Jaco, R Reid, SA Radom, L Schmidt, TW Kable, SH AF Krechkivska, Olha Wilcox, Callan M. Troy, Tyler P. Nauta, Klaas Chan, Bun Jaco, Rebecca Reid, Scott A. Radom, Leo Schmidt, Timothy W. Kable, Scott H. TI Hydrogen-atom attack on phenol and toluene is ortho-directed SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID POLYCYCLIC AROMATIC-HYDROCARBONS; ELECTRONIC-ABSORPTION-SPECTRA; GAS-PHASE BASICITIES; PROTONATED NAPHTHALENE; EXCITATION SPECTRUM; REACTION-MECHANISM; INTERNAL-ROTATION; P-FLUOROTOLUENE; RADICALS; CYCLOHEXADIENYL AB The reaction of H + phenoL and H/D + toluene has been studied in a supersonic expansion after electric discharge. The (1 + 1') resonance-enhanced muLtiphoton ionization (REMPI) spectra of the reaction products, at m/z = parent + 1, or parent + 2 amu, were measured by scanning the first (resonance) Laser. The resulting spectra are highly structured. Ionization energies were measured by scanning the second (ionization) Laser, while the first Laser was tuned to a specific transition. Theoretical calculations, benchmarked to the well studied H + benzene -> cyclohexadienyl radical reaction, were performed. The spectrum arising from the reaction of H + phenoL is attributed solely to the ortho-hydroxy-cycLohexadienyL radical, which was found in two conformers (syn and anti). Similarly, the reaction of H/D + toluene formed solely the ortho isomer. The preference for the ortho isomer at 100-200 K in the molecular beam is attributed to kinetic, not thermodynamic effects, caused by an entrance channel barrier that is-5 kJ moL-1 Lower for ortho than for other isomers. Based on these results, we predict that the reaction of H + phenoL and H + toluene should still favour the ortho isomer under elevated temperature conditions in the early stages of combustion (200-400 degrees C). C1 [Krechkivska, Olha; Wilcox, Callan M.; Nauta, Klaas; Schmidt, Timothy W.; Kable, Scott H.] Univ New S Wales, Sch Chem, Kensington, NSW 2052, Australia. [Troy, Tyler P.; Chan, Bun; Jaco, Rebecca; Radom, Leo] Univ Sydney, Sch Chem, Sydney, NSW 2006, Australia. [Reid, Scott A.] Marquette Univ, Dept Chem, Milwaukee, WI 53201 USA. [Troy, Tyler P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, MS 6R-2100, Berkeley, CA 94720 USA. RP Kable, SH (reprint author), Univ New S Wales, Sch Chem, Kensington, NSW 2052, Australia. EM s.kable@unsw.edu.au RI Reid, Scott/J-6491-2016 OI Reid, Scott/0000-0001-9916-7414 FU Australian Research Council [DP120102559] FX This work was supported by the Australian Research Council (grant DP120102559). CMW acknowledges an Australian Postgraduate Award scholarship. We gratefully acknowledge generous allocations of supercomputer time from the National Computational Infrastructure (NCI) National Facility and Intersect Australia Ltd. NR 64 TC 2 Z9 2 U1 7 U2 28 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAR 28 PY 2016 VL 18 IS 12 BP 8625 EP 8636 DI 10.1039/c5cp07619f PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG7FB UT WOS:000372249100033 PM 26948897 ER PT J AU Hesse, M Liu, YH Chen, LJ Bessho, N Kuznetsova, M Birn, J Burch, JL AF Hesse, Michael Liu, Yi-Hsin Chen, Li-Jen Bessho, Naoki Kuznetsova, Masha Birn, Joachim Burch, James L. TI On the electron diffusion region in asymmetric reconnection with a guide magnetic field SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE magnetic reconnection; magnetopause; magnetospheric multiscale; kinetic physics; distribution function; plasma physics AB Particle-in-cell simulations in a 2.5-D geometry and analytical theory are employed to study the electron diffusion region in asymmetric reconnection with a guide magnetic field. The analysis presented here demonstrates that similar to the case without guide field, in-plane flow stagnation and null of the in-plane magnetic field are well separated. In addition, it is shown that the electric field at the local magnetic X point is again dominated by inertial effects, whereas it remains dominated by nongyrotropic pressure effects at the in-plane flow stagnation point. A comparison between local electron Larmor radii and the magnetic gradient scale lengths predicts that distribution should become nongyrotropic in a region enveloping both field reversal and flow stagnation points. This prediction is verified by an analysis of modeled electron distributions, which show clear evidence of mixing in the critical region. C1 [Hesse, Michael; Liu, Yi-Hsin; Chen, Li-Jen; Bessho, Naoki; Kuznetsova, Masha] NASA, Goddard Space Flight Ctr, Heliophys Sci Div, Greenbelt, MD USA. [Birn, Joachim] Space Sci Inst, Boulder, CO USA. [Birn, Joachim] Los Alamos Natl Lab, Los Alamos, NM USA. [Burch, James L.] SW Res Inst, San Antonio, TX USA. RP Hesse, M (reprint author), NASA, Goddard Space Flight Ctr, Heliophys Sci Div, Greenbelt, MD USA. EM michael.hesse@nasa.gov RI NASA MMS, Science Team/J-5393-2013 OI NASA MMS, Science Team/0000-0002-9504-5214 FU NASA's Magnetospheric Multiscale mission; NSF [AGS-1543598, AGS-1552142] FX This work was supported by NASA's Magnetospheric Multiscale mission and NSF grants AGS-1543598 and AGS-1552142. Access to simulation data can be provided upon request. NR 15 TC 5 Z9 5 U1 2 U2 6 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAR 28 PY 2016 VL 43 IS 6 BP 2359 EP 2364 DI 10.1002/2016GL068373 PG 6 WC Geosciences, Multidisciplinary SC Geology GA DK1TM UT WOS:000374697200003 ER PT J AU Chen, LJ Hesse, M Wang, S Bessho, N Daughton, W AF Chen, Li-Jen Hesse, Michael Wang, Shan Bessho, Naoki Daughton, William TI Electron energization and structure of the diffusion region during asymmetric reconnection SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE magnetic reconnection; electron diffusion region; electron acceleration; electron heating; collisionless resistivity; collisionless dissipation ID MAGNETIC RECONNECTION; X-LINE; PHYSICS AB Results from particle-in-cell simulations of reconnection with asymmetric upstream conditions are reported to elucidate electron energization and structure of the electron diffusion region (EDR). Acceleration of unmagnetized electrons results in discrete structures in the distribution functions and supports the intense current and perpendicular heating in the EDR. The accelerated electrons are cyclotron turned by the reconnected magnetic field to produce the outflow jets, and as such, the acceleration by the reconnection electric field is limited, leading to resistivity without particle-particle or particle-wave collisions. A map of electron distributions is constructed, and its spatial evolution is compared with quantities previously proposed to be EDR identifiers to enable effective identifications of the EDR in terrestrial magnetopause reconnection. C1 [Chen, Li-Jen; Hesse, Michael; Wang, Shan; Bessho, Naoki] NASA, Goddard Space Flight Ctr, Greenbelt, MD USA. [Chen, Li-Jen; Wang, Shan; Bessho, Naoki] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Daughton, William] Los Alamos Natl Lab, Los Alamos, NM USA. RP Chen, LJ (reprint author), NASA, Goddard Space Flight Ctr, Greenbelt, MD USA.; Chen, LJ (reprint author), Univ Maryland, Dept Astron, College Pk, MD 20742 USA. EM li-jen.chen@nasa.gov RI Daughton, William/L-9661-2013; NASA MMS, Science Team/J-5393-2013 OI NASA MMS, Science Team/0000-0002-9504-5214 FU NSF [AGS-1202537, AGS-1543598, AGS-1552142]; Theory and Modeling Program; Fast Plasma Investigation of the Magnetospheric Multiscale mission; NASA Heliophysics Theory Program FX The research was supported in part by NSF grants AGS-1202537, AGS-1543598, and AGS-1552142 and at NASA GSFC by the Theory and Modeling Program and the Fast Plasma Investigation of the Magnetospheric Multiscale mission. Contribution from W.D. was supported by NASA Heliophysics Theory Program. The simulation runs were performed on Pleiades under the NASA HEC Program and on Titan at the National Center for Computational Sciences at ORNL. L.J.C. acknowledges the contributions of J. Shuster and M. Argall to the PIC data plotting software. The data are available upon request to the authors. NR 28 TC 15 Z9 15 U1 4 U2 6 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAR 28 PY 2016 VL 43 IS 6 BP 2405 EP 2412 DI 10.1002/2016GL068243 PG 8 WC Geosciences, Multidisciplinary SC Geology GA DK1TM UT WOS:000374697200009 ER PT J AU Le, CF Lehrter, JC Hu, C Obenour, DR AF Le, Chengfeng Lehrter, John C. Hu, Chuanmin Obenour, Daniel R. TI Satellite-based empirical models linking river plume dynamics with hypoxic area and volume SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article ID GULF-OF-MEXICO; CONTINENTAL-SHELF; RETROSPECTIVE ANALYSIS; ORGANIC-CARBON; VARIABILITY; DISTRIBUTIONS AB Satellite-based empirical models explaining hypoxic area and volume variation were developed for the seasonally hypoxic (O-2 < 2 mg L-1) northern Gulf of Mexico adjacent to the Mississippi River. Annual variations in midsummer hypoxic area and volume were related to Moderate Resolution Imaging Spectroradiometer-derived monthly estimates of river plume area (km(2)) and average, inner shelf chlorophyll a concentration (Chl a, mg m(-3)). River plume area in June was negatively related with midsummer hypoxic area (km(2)) and volume (km(3)), while July inner shelf Chl a was positively related to hypoxic area and volume. Multiple regression models using river plume area and Chl a as independent variables accounted for most of the variability in hypoxic area (R-2=0.92) or volume (R-2=0.89). These models explain more variation in hypoxic area than models using Mississippi River nutrient loads as independent variables. The results here also support a hypothesis that confinement of the river plume to the inner shelf is an important mechanism controlling hypoxia area and volume in this region. C1 [Le, Chengfeng] Zhejiang Univ, Ocean Coll, Hangzhou 310003, Zhejiang, Peoples R China. [Le, Chengfeng] US EPA, ORISE, Gulf Ecol Div, Gulf Breeze, FL USA. [Lehrter, John C.] US EPA, Gulf Ecol Div, Gulf Breeze, FL USA. [Hu, Chuanmin] Univ S Florida, Coll Marine Sci, St Petersburg, FL 33701 USA. [Obenour, Daniel R.] N Carolina State Univ, Dept Civil Construct & Environm Engn, Raleigh, NC 27695 USA. RP Le, CF (reprint author), Zhejiang Univ, Ocean Coll, Hangzhou 310003, Zhejiang, Peoples R China.; Le, CF (reprint author), US EPA, ORISE, Gulf Ecol Div, Gulf Breeze, FL USA. EM chengfengle@zju.edu.cn FU U.S. EPA Office of Research and Development, an Oak Ridge institute for the Science and Education (ORISE) appointment for Chengfeng Le to the EPA Research Participation Program FX This work was partly supported by the U.S. EPA Office of Research and Development, by an Oak Ridge institute for the Science and Education (ORISE) appointment for Chengfeng Le to the EPA Research Participation Program. We thank Rochelle Labiosa for a helpful review of an earlier draft of this manuscript and the two anonymous reviewers for their suggestions to improve this manuscript. NR 24 TC 1 Z9 1 U1 9 U2 12 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAR 28 PY 2016 VL 43 IS 6 BP 2693 EP 2699 DI 10.1002/2015GL067521 PG 7 WC Geosciences, Multidisciplinary SC Geology GA DK1TM UT WOS:000374697200044 ER PT J AU Nouicer, R AF Nouicer, R. TI New state of nuclear matter: Nearly perfect fluid of quarks and gluons in heavy-ion collisions at RHIC energies SO EUROPEAN PHYSICAL JOURNAL PLUS LA English DT Review ID PLUS AU COLLISIONS; JET CROSS-SECTION; SQUARE-ROOT-S; TRANSVERSE-MOMENTUM SPECTRA; PROTON-ANTIPROTON COLLIDER; ELLIPTIC FLOW; HADRON-PRODUCTION; PBARP COLLISIONS; PB COLLISIONS; QCD AB This article reviews several important results from RHIC experiments and discusses their implications. They were obtained in a unique environment for studying QCD matter at temperatures and densities that exceed the limits wherein hadrons can exist as individual entities and raises to prominence the quark-gluon degrees of freedom. These findings are supported by major experimental observations via measuring of the bulk properties of particle production, particle ratios and chemical freeze-out conditions, and elliptic flow; followed by hard probe measurements: high-pT hadron suppression, dijet fragment azimuthal correlations, and heavy-flavor probes. These measurements are presented for particles of different species as a function of system sizes, collision centrality, and energy carried out in RHIC experiments. The results reveal that a dense, strongly interacting medium is created in central Au + Au collisions at root(NN)-N-S = 200 GeV at RHIC. This revelation of a new state of nuclear matter has also been observed in measurements at the LHC. Further, the IP-Glasma model coupled with viscous hydrodynamic models, which assumes the formation of a QGP, reproduces well the experimental flow results from Au + Au at root(NN)-N-S = 200 GeV. This implies that the fluctuations in the initial geometry state are important and the created medium behaves as a nearly perfect liquid of nuclear matter because it has an extraordinarily low ratio of shear viscosity to entropy density, eta/s approximate to 0.12. However, these discoveries are far from being fully understood. Furthermore, recent experimental results from RHIC and LHC in small p + A, d + Au and He-3 + Au collision systems provide brand new insight into the role of initial and final state effects. These have proven to be interesting and more surprising than originally anticipated; and could conceivably shed new light in our understanding of collective behavior in heavy-ion physics. Accordingly, the focus of the experiments at both facilities RHIC and the LHC is on detailed exploration of the properties of this new state of nuclear matter, the QGP. C1 [Nouicer, R.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Nouicer, R (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM rachid.nouicer@bnl.gov FU US Department of Energy [DE-AC02-98CH10886] FX The author thanks F. Karsch, B. Schenke, P. Stankus, C. Beck, D. Morrison, M. McCumber and L. McLerran for their stimulating discussions. P. Tribedy, R. Venugopalan and A. Andronic are warmly thanked for useful suggestions and for providing model calculations plotted on figs. 5 and 9. C. Roy and Institut Pluridisciplinaire Hubert Curien (IPHC) as well as A. Nourreddine and Universite de Strasbourg are fully acknowledge for their supports for HDR ("Habilitation a Diriger des Recherches") where parts of the present review paper were presented in the HDR written document available at https://tel.archives-ouvertes.fr/tel-00925262. The author's research was supported by US Department of Energy, DE-AC02-98CH10886. NR 140 TC 2 Z9 2 U1 5 U2 9 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 2190-5444 J9 EUR PHYS J PLUS JI Eur. Phys. J. Plus PD MAR 28 PY 2016 VL 131 IS 3 AR 70 DI 10.1140/epjp/i2016-16070-2 PG 26 WC Physics, Multidisciplinary SC Physics GA DL0FF UT WOS:000375307100006 ER PT J AU Zhang, Y Tayebjee, MJY Smyth, S Dvorak, M Wen, ZM Xia, HZ Heilmann, M Liao, YX Zhang, ZW Williamson, T Williams, J Bremner, S Shrestha, S Huang, SJ Schmidt, TW Conibeer, GJ AF Zhang, Yi Tayebjee, Murad J. Y. Smyth, Suntrana Dvorak, Miroslav Xiaoming Wen Hongze Xia Heilmann, Martin Yuanxun Liao Zewen Zhang Williamson, Todd Williams, Joshua Bremner, Stephen Shrestha, Santosh Shujuan Huang Schmidt, Timothy W. Conibeer, Gavin J. TI Extended hot carrier lifetimes observed in bulk In0.265 +/- 0.02Ga0.735N under high-density photoexcitation SO APPLIED PHYSICS LETTERS LA English DT Article ID JUNCTION SOLAR-CELLS; QUANTUM-WELLS; RELAXATION-TIME; INGAN EPILAYERS; EFFICIENCY; DYNAMICS; FILMS; GAAS; SEMICONDUCTORS; ALLOYS AB We have investigated the ultrafast carrier dynamics in a 1 mu m bulk In0.265Ga0.735N thin film grown using energetic neutral atom-beam lithography/epitaxy molecular beam epitaxy. Cathodoluminescence and X-ray diffraction experiments are used to observe the existence of indium-rich domains in the sample. These domains give rise to a second carrier population and biexponential carrier cooling is observed with characteristic lifetimes of 1.6 and 14 ps at a carrier density of 1.3 x 10 16 cm(-3). A combination of band-filling, screening, and hot-phonon effects gives rise to a two-fold enhanced mono-exponential cooling rate of 28 ps at a carrier density of 8.4 x 10(18) cm(-3). This is the longest carrier thermalization time observed in bulk InGaN alloys to date. (C) 2016 AIP Publishing LLC. C1 [Zhang, Yi; Tayebjee, Murad J. Y.; Smyth, Suntrana; Xiaoming Wen; Hongze Xia; Yuanxun Liao; Zewen Zhang; Bremner, Stephen; Shrestha, Santosh; Shujuan Huang; Conibeer, Gavin J.] Univ New S Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia. [Dvorak, Miroslav] Univ Sydney, Sch Chem, Sydney, NSW 2006, Australia. [Heilmann, Martin] Max Planck Inst Sci Light, Gunther Scharowsky Str 1, D-91058 Erlangen, Germany. [Williamson, Todd; Williams, Joshua] Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. [Schmidt, Timothy W.] UNSW, Sch Chem, Sydney, NSW 2052, Australia. RP Zhang, Y (reprint author), Univ New S Wales, Sch Photovolta & Renewable Energy Engn, Sydney, NSW 2052, Australia. FU Australian Government through the Australian Renewable Energy Agency (ARENA); Australian Research Council [FT130100177]; [DP130104231] FX This project has been supported by the Australian Government through the Australian Renewable Energy Agency (ARENA). Responsibility for the views, information, or advice expressed herein is not accepted by the Australian Government. T.W.S. acknowledges the Australian Research Council for a Future Fellowships (FT130100177). This work was partially funded through DP130104231. NR 39 TC 1 Z9 1 U1 6 U2 20 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 28 PY 2016 VL 108 IS 13 AR 131904 DI 10.1063/1.4945594 PG 5 WC Physics, Applied SC Physics GA DI6IC UT WOS:000373601400016 ER PT J AU Bondi, RJ Fox, BP Marinella, MJ AF Bondi, Robert J. Fox, Brian P. Marinella, Matthew J. TI Role of atomistic structure in the stochastic nature of conductivity in substoichiometric tantalum pentoxide SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; OXYGEN VACANCY; 1ST PRINCIPLES; DENSITY; METALS; MEMRISTOR; DEFECTS AB First-principles calculations of electrical conductivity (sigma(o)) are revisited to determine the atomistic origin of its stochasticity in a distribution generated from sampling 14 ab-initio molecular dynamics configurations from 10 independently quenched models (n = 140) of substoichiometric amorphous Ta2O5, where each structure contains a neutral O monovacancy (V-O(0)). Structural analysis revealed a distinct minimum Ta-Ta separation (dimer/trimer) corresponding to each V-O(0) location. Bader charge decomposition using a commonality analysis approach based on the sigma(o) distribution extremes revealed nanostructural signatures indicating that both the magnitude and distribution of cationic charge on the Ta subnetwork have a profound influence on sigma(o). Furthermore, visualization of local defect structures and their electron densities reinforces these conclusions and suggests sigma(o) in the amorphous oxide is best suppressed by a highly charged, compact Ta cation shell that effectively screens and minimizes localized V-O(0) interaction with the a-Ta2O5 network; conversely, delocalization of V-O(0) corresponds to metallic character and high sigma(o). The random network of a-Ta2O5 provides countless variations of an ionic configuration scaffold in which small perturbations affect the electronic charge distribution and result in a fixed-stoichiometry distribution of sigma(o); consequently, precisely controlled and highly repeatable oxide fabrication processes are likely paramount for advancement of resistive memory technologies. (C) 2016 AIP Publishing LLC. C1 [Bondi, Robert J.; Fox, Brian P.; Marinella, Matthew J.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Bondi, RJ (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM rjbondi@sandia.gov FU Laboratory Directed Research and Development Program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was partially supported by the Laboratory Directed Research and Development Program at Sandia National Laboratories. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. We also thank Mike Desjarlais, Aidan Thompson, Peter Schultz, Mike Brumbach, and Gaddi Haase for helpful discussions. NR 51 TC 0 Z9 0 U1 1 U2 14 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 28 PY 2016 VL 119 IS 12 AR 124101 DI 10.1063/1.4943163 PG 14 WC Physics, Applied SC Physics GA DI6II UT WOS:000373602000013 ER PT J AU Burcklen, C Soufli, R Dennetiere, D Polack, F Capitanio, B Gullikson, E Meltchakov, E Thomasset, M Jerome, A de Rossi, S Delmotte, F AF Burcklen, C. Soufli, R. Dennetiere, D. Polack, F. Capitanio, B. Gullikson, E. Meltchakov, E. Thomasset, M. Jerome, A. de Rossi, S. Delmotte, F. TI Cr/B4C multilayer mirrors: Study of interfaces and X-ray reflectance SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID EXTREME-ULTRAVIOLET; LIGHT-SOURCE; RANGE; FILMS; FABRICATION; REGION; PHOTOABSORPTION; BEAMLINE; DESIGN; OPTICS AB We present an experimental study of the effect of layer interfaces on the x-ray reflectance in Cr/B4C multilayer interference coatings with layer thicknesses ranging from 0.7 nm to 5.4 nm. The multi-layers were deposited by magnetron sputtering and by ion beam sputtering. Grazing incidence x-ray reflectometry, soft x-ray reflectometry, and transmission electron microscopy reveal asymmetric multilayer structures with a larger B4C-on-Cr interface, which we modeled with a 1-1.5 nm thick interfacial layer. Reflectance measurements in the vicinity of the Cr L-2,L-3 absorption edge demonstrate fine structure that is not predicted by simulations using the currently tabulated refractive index (optical constants) values for Cr. (C) 2016 AIP Publishing LLC. C1 [Burcklen, C.; Soufli, R.; Meltchakov, E.; Jerome, A.; de Rossi, S.; Delmotte, F.] Univ Paris Saclay, CNRS, Grad Sch, Inst Opt,Lab Charles Fabry, F-91127 Palaiseau, France. [Soufli, R.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. [Dennetiere, D.; Polack, F.; Capitanio, B.; Thomasset, M.] LOrme Merisiers, Synchrotron SOLEIL, BP 48, F-91192 Gif Sur Yvette, France. [Gullikson, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Xray Opt, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Burcklen, C (reprint author), Univ Paris Saclay, CNRS, Grad Sch, Inst Opt,Lab Charles Fabry, F-91127 Palaiseau, France. FU French Research Agency [ANR-11-EQPX-0029, ANR-10-LABX-0039]; U.S. Department of Energy by Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344]; University of California Lawrence Berkeley National Laboratory [DE-AC03-76F00098]; LLNL's Professional Research and Teaching Leave Program FX The authors would like to thank Santhosh Chenna and Lancy Chung (EAG Labs) for assistance with the TEM image acquisition. MS samples have been deposited as part of CEMOX (Centrale d'Elaboration et de Metrologie d'Optique X), a platform of LUMAT federation (CNRS FR2764). This work was partly supported by the French Research Agency under Contract Nos. ANR-11-EQPX-0029 and ANR-10-LABX-0039. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory (LLNL) under Contract No. DE-AC52-07NA27344 and by the University of California Lawrence Berkeley National Laboratory under Contract No. DE-AC03-76F00098. Funding was provided in part by LLNL's Professional Research and Teaching Leave Program. NR 33 TC 1 Z9 1 U1 4 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 28 PY 2016 VL 119 IS 12 AR 125307 DI 10.1063/1.4944723 PG 9 WC Physics, Applied SC Physics GA DI6II UT WOS:000373602000062 ER PT J AU Roslyak, O Piryatinski, A AF Roslyak, Oleksiy Piryatinski, Andrei TI Thermoelectric properties of semiconductor nanowire networks SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID BISMUTH TELLURIDE; GROWTH; ARRAYS; HEAT AB To examine the thermoelectric (TE) properties of a semiconductor nanowire (NW) network, we propose a theoretical approach mapping the TE network on a two-port network. In contrast to a conventional single-port (i.e., resistor) network model, our model allows for large scale calculations showing convergence of TE figure of merit, ZT, with an increasing number of junctions. Using this model, numerical simulations are performed for the Bi2Te3 branched nanowire (BNW) and Cayley tree NW (CTNW) network. We find that the phonon scattering at the network junctions plays a dominant role in enhancing the network ZT. Specifically, disordered BNW and CTNW demonstrate an order of magnitude higher ZT enhancement compared to their ordered counterparts. Formation of preferential TE pathways in CTNW makes the network effectively behave as its BNW counterpart. We provide formalism for simulating large scale nanowire networks hinged upon experimentally measurable TE parameters of a single T-junction. (C) 2016 AIP Publishing LLC. C1 [Roslyak, Oleksiy] Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, Div Theoret, Los Alamos, NM 87545 USA. [Roslyak, Oleksiy] Fordham Univ, Dept Phys & Engn Phys, Bronx, NY 10458 USA. [Piryatinski, Andrei] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Roslyak, O (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol CINT, Div Theoret, Los Alamos, NM 87545 USA.; Roslyak, O (reprint author), Fordham Univ, Dept Phys & Engn Phys, Bronx, NY 10458 USA.; Piryatinski, A (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM oroslyak@fordham.edu; apiryat@lanl.gov RI Piryatinski, Andrei/B-5543-2009 FU Center for Integrated Nanotechnologies (CINT), a U.S. Department of Energy, Office of Basic Energy Sciences (OBES) user facility; Los Alamos National Laboratory Directed Research and Development (LDRD) Funds FX O.R. acknowledges the support provided by the Center for Integrated Nanotechnologies (CINT), a U.S. Department of Energy, Office of Basic Energy Sciences (OBES) user facility. A.P. acknowledges the support provided by Los Alamos National Laboratory Directed Research and Development (LDRD) Funds. We thank Jennifer Hollingsworth for stimulating discussions. NR 40 TC 1 Z9 1 U1 6 U2 22 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 28 PY 2016 VL 119 IS 12 AR 125107 DI 10.1063/1.4944715 PG 9 WC Physics, Applied SC Physics GA DI6II UT WOS:000373602000052 ER PT J AU Singh, A Schefer, J Sura, R Conder, K Sibille, RF Ceretti, M Frontzek, M Paulus, W AF Singh, Anar Schefer, Juerg Sura, Ravi Conder, Kazimierz Sibille, Romain F. Ceretti, Monica Frontzek, Matthias Paulus, Werner TI Evidence for monoclinic distortion in the ground state phase of underdoped La1.95Sr0.05CuO4: A single crystal neutron diffraction study SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID MAGNETIC FLUCTUATIONS; SUPERCONDUCTIVITY; EXCITATIONS; LA2CUO4; LA2-XSR(X)CUO4; LA2-XBAXCUO4; LA2-XSRXCUO4; PURE AB The existing controversy about the symmetry of the crystal structure of the ground state of the critical doped La1.95Sr0.05CuO4 has been resolved by analyzing the single crystal neutron diffraction data collected between 5 and 730 K. We observed small but significant intensities for "forbidden" reflections given by extinction rules of the orthorhombic Bmab space group at low temperatures. A careful investigation of neutron diffraction data reveals that the crystal structure of La1.95Sr0.05CuO4 at 5 K is monoclinic with B2/m (2/m 1 1) space group. The monoclinic structure emerges from the orthorhombic structure in a continuous way; however, the structure is stable below similar to 120K which agrees with other observed phenomena. Our results on symmetry changes are crucial for the interpretation of physical properties also in other high temperature superconductors with similar structures. (C) 2016 AIP Publishing LLC. C1 [Singh, Anar; Schefer, Juerg; Sura, Ravi; Frontzek, Matthias] Paul Scherrer Inst, Lab Neutron Scattering & Imaging LNS, CH-5232 Villigen, Switzerland. [Sura, Ravi] Univ Rennes 1, Sci Chim Rennes, UMR 6226, Campus Beaulieu, F-35042 Rennes, France. [Conder, Kazimierz; Sibille, Romain F.] Paul Scherrer Inst, Lab Sci Dev & Novel Mat LDM, CH-5232 Villigen, Switzerland. [Ceretti, Monica; Paulus, Werner] Univ Montpellier, CNRS, Inst Charles Gerhardt, UMR 5253, F-34095 Montpellier, France. [Singh, Anar] Inst Chem Technol, Dept Phys, Mumbai 400019, Maharashtra, India. [Frontzek, Matthias] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Singh, A (reprint author), Paul Scherrer Inst, Lab Neutron Scattering & Imaging LNS, CH-5232 Villigen, Switzerland.; Singh, A (reprint author), Inst Chem Technol, Dept Phys, Mumbai 400019, Maharashtra, India. EM singhanar@gmail.com RI Frontzek, Matthias/C-5146-2012; sibille, romain/B-2104-2012 OI Frontzek, Matthias/0000-0001-8704-8928; sibille, romain/0000-0001-6360-7262 FU project SECTOR [ANR-14-CE36-0006-01/SNF 200021L_157131/1]; Centre National de la Recherche Scientific (CNRS)/France; Paul Scherrer Institute (PSI)/Switzerland; Department of Science and Technology (DST), India FX This work was fully based on experiments performed on the single crystal neutron diffraction instrument TriCS at the Swiss spallation neutron source SINQ and at the Laboratory for Scientific Developments and Novel Materials (LDM), both at Paul Scherrer Institute (PSI), Switzerland. This work was funded with the project SECTOR (ANR-14-CE36-0006-01/SNF 200021L_157131/1). R.S. has been supported by the grants of Centre National de la Recherche Scientific (CNRS)/France and by Paul Scherrer Institute (PSI)/Switzerland. A.S. acknowledges support from Department of Science and Technology (DST), India under INSPIRE faculty scheme. NR 45 TC 0 Z9 0 U1 5 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 28 PY 2016 VL 119 IS 12 AR 123902 DI 10.1063/1.4944797 PG 8 WC Physics, Applied SC Physics GA DI6II UT WOS:000373602000008 ER PT J AU Bhattacherjee, A Attar, AR Leone, SR AF Bhattacherjee, Aditi Attar, Andrew R. Leone, Stephen R. TI Transition state region in the A-Band photodissociation of allyl iodide-A femtosecond extreme ultraviolet transient absorption study SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID RESOLVED PHOTOELECTRON-SPECTROSCOPY; MAGNETIC CIRCULAR-DICHROISM; POTENTIAL-ENERGY SURFACES; REAL-TIME OBSERVATION; METHYL-IODIDE; CHEMICAL-REACTIONS; EXCITED-STATES; DYNAMICS; SPECTRA; RADICALS AB Femtosecond extreme ultraviolet (XUV) transient absorption spectroscopy based on a high-harmonic generation source is used to study the 266 nm induced A-band photodissociation dynamics of allyl iodide (CH2=CHCH2I). The photolysis of the C-I bond at this wavelength produces iodine atoms both in the ground (P-2(3/2), I) and spin-orbit excited (P-2(1/2), I*) states, with the latter as the predominant channel. Using XUV absorption at the iodine N-4/5 edge (45-60 eV), the experiments constitute a direct probe of not only the long-lived atomic iodine reaction products but also the fleeting transition state region of the repulsive n(I)sigma*(C-I) excited states. Specifically, three distinct features are identified in the XUV transient absorption spectrum at 45.3 eV, 47.4 eV, and 48.4 eV (denoted transients A, B, and C, respectively), which arise from the repulsive valence-excited n sigma* states and project onto the high-lying core-excited states of the dissociating molecule via excitation of 4d(I) core electrons. Transients A and B originate from 4d(I) -> n(I) core-to-valence transitions, whereas transient C is best assigned to a 4d(I) -> sigma*(C-I) transition. The measured differential absorbance of these new features along with the I/I* branching ratios known from the literature is used to suggest a more definitive assignment, albeit provisional, of the transients to specific dissociative states within the A-band manifold. The transients are found to peak around 55 fs-65 fs and decay completely by 145 fs-185 fs, demonstrating the ability of XUV spectroscopy to map the evolution of reactants into products in real time. The similarity in the energies of transients A and B with analogous features observed in methyl iodide [Attar et al. J. Phys. Chem. Lett. 6, 5072, (2015)] together with the new observation of transient C in the present work provides a more complete picture of the valence electronic structure in the transition state region. The results provide a benchmark for theoretical calculations on the nature of core-excited states in halogenated hydrocarbons, especially in the transition state region along the C-I reaction coordinate. (C) 2016 AIP Publishing LLC. C1 [Bhattacherjee, Aditi; Attar, Andrew R.; Leone, Stephen R.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Bhattacherjee, Aditi; Attar, Andrew R.; Leone, Stephen R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Leone, Stephen R.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Leone, SR (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Leone, SR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.; Leone, SR (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM abhattacherjee@berkeley.edu; andrewattar@berkeley.edu; srl@berkeley.edu FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-05CH11231]; Chemical Sciences Division of Lawrence Berkeley National Laboratory; NSF ERC, EUV Science and Technology [EEC-0310717] FX This research work, A.B. and A.R.A. were supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (Contract No. DE-AC02-05CH11231), the gas phase chemical physics program through the Chemical Sciences Division of Lawrence Berkeley National Laboratory. The apparatus was partially funded by a NSF ERC, EUV Science and Technology, under a previously completed grant (No. EEC-0310717). NR 74 TC 1 Z9 1 U1 10 U2 19 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 28 PY 2016 VL 144 IS 12 AR 124311 DI 10.1063/1.4944930 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DI6XV UT WOS:000373644400035 PM 27036452 ER PT J AU Calero, C Knorowski, C Travesset, A AF Calero, C. Knorowski, C. Travesset, A. TI Determination of anharmonic free energy contributions: Low temperature phases of the Lennard-Jones system SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID INVERSE-POWER POTENTIALS; SOLID-FLUID COEXISTENCE; COMPUTER-SIMULATION; DIAGRAM; DYNAMICS; MODEL; TRANSITION; ENTROPY; FCC AB We investigate a general method to calculate the free energy of crystalline solids by considering the harmonic approximation and quasistatically switching the anharmonic contribution. The advantage of this method is that the harmonic approximation provides an already very accurate estimate of the free energy, and therefore the anharmonic term is numerically very small and can be determined to high accuracy. We further show that the anharmonic contribution to the free energy satisfies a number of exact inequalities that place constraints on its magnitude and allows approximate but fast and accurate estimates. The method is implemented into a readily available general software by combining the code HOODLT (Highly Optimized Object Oriented Dynamic Lattice Theory) for the harmonic part and the molecular dynamics (MD) simulation package HOOMD-blue for the anharmonic part. We use the method to calculate the low temperature phase diagram for Lennard-Jones particles. We demonstrate that hcp is the equilibrium phase at low temperature and pressure and obtain the coexistence curve with the fcc phase, which exhibits reentrant behavior. Several implications of the method are discussed. (C) 2016 AIP Publishing LLC. C1 [Calero, C.] Boston Univ, Ctr Polymer Studies, 590 Commonwealth Ave, Boston, MA 02215 USA. [Calero, C.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Calero, C.] Univ Barcelona, Dept Fis Fonamental, Marti & Franques 1, E-08028 Barcelona, Spain. [Knorowski, C.; Travesset, A.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Knorowski, C.; Travesset, A.] Iowa State Univ, Ames Lab, Ames, IA 50011 USA. RP Calero, C (reprint author), Boston Univ, Ctr Polymer Studies, 590 Commonwealth Ave, Boston, MA 02215 USA.; Calero, C (reprint author), Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA.; Calero, C (reprint author), Univ Barcelona, Dept Fis Fonamental, Marti & Franques 1, E-08028 Barcelona, Spain.; Travesset, A (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA.; Travesset, A (reprint author), Iowa State Univ, Ames Lab, Ames, IA 50011 USA. EM ccalero@bu.edu; trvsst@ameslab.gov RI Calero, Carles/B-4178-2017 OI Calero, Carles/0000-0002-1977-1724 FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials, Materials Science and Engineering Division; Beatriu de Pinos program [BP-DGR 2011]; US DOE by Iowa State University [DE-AC02-07CH11358] FX This work is supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, which is operated for the US DOE by Iowa State University under Contract No. DE-AC02-07CH11358. C.C. acknowledges the support from the Beatriu de Pinos program (No. BP-DGR 2011). NR 39 TC 2 Z9 2 U1 2 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 28 PY 2016 VL 144 IS 12 AR 124102 DI 10.1063/1.4944069 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DI6XV UT WOS:000373644400005 PM 27036422 ER PT J AU Weichman, ML Song, XW Fagiani, MR Debnath, S Gewinner, S Schollkopf, W Neumark, DM Asmis, KR AF Weichman, Marissa L. Song, Xiaowei Fagiani, Matias R. Debnath, Sreekanta Gewinner, Sandy Schoellkopf, Wieland Neumark, Daniel M. Asmis, Knut R. TI Gas phase vibrational spectroscopy of cold (TiO2)(n)(-) (n=3-8) clusters SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID METAL-OXIDE CLUSTERS; SENSITIZED SOLAR-CELLS; LASER-ABLATED TITANIUM; TIO2 NANOTUBE ARRAYS; ELECTRONIC-STRUCTURE; PHOTODISSOCIATION SPECTROSCOPY; INFRARED-SPECTROSCOPY; MOLECULAR-STRUCTURES; OPTICAL-PROPERTIES; SURFACE SCIENCE AB We report infrared photodissociation (IRPD) spectra for the D-2-tagged titanium oxide cluster anions (TiO2)(n)(-) with n = 3-8 in the spectral region from 450 to 1200 cm(-1). The IRPD spectra are interpreted with the aid of harmonic spectra from BP86/6-311+G* density functional theory calculations of energetically low-lying isomers. We conclusively assign the IRPD spectra of the n = 3 and n = 6 clusters to global minimum energy structures with C-s and C-2 symmetry, respectively. The vibrational spectra of the n = 4 and n = 7 clusters can be attributed to contributions of at most two low-lying structures. While our calculations indicate that the n = 5 and n = 8 clusters have many more low-lying isomers than the other clusters, the dominant contributions to their spectra can be assigned to the lowest energy structures. Through comparison between the calculated and experimental spectra, we can draw conclusions about the size-dependent evolution of the properties of (TiO2)(n)(-) clusters, and on their potential utility as model systems for catalysis on a bulk TiO2 surface. (C) 2016 AIP Publishing LLC. C1 [Weichman, Marissa L.; Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Song, Xiaowei; Fagiani, Matias R.; Debnath, Sreekanta; Gewinner, Sandy; Schoellkopf, Wieland] Max Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, Germany. [Fagiani, Matias R.; Debnath, Sreekanta; Asmis, Knut R.] Univ Leipzig, Wilhelm Ostwald Inst Phys & Theoret Chem, Linnestr 2, D-04103 Leipzig, Germany. [Neumark, Daniel M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Asmis, KR (reprint author), Univ Leipzig, Wilhelm Ostwald Inst Phys & Theoret Chem, Linnestr 2, D-04103 Leipzig, Germany.; Neumark, DM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu; knut.asmis@uni-leipzig.de RI Asmis, Knut/N-5408-2014; Neumark, Daniel/B-9551-2009; OI Asmis, Knut/0000-0001-6297-5856; Neumark, Daniel/0000-0002-3762-9473; Weichman, Marissa/0000-0002-2551-9146; Schollkopf, Wieland/0000-0003-0564-203X FU Air Force Office of Scientific Research [FA9550-12-1-0160]; German Research Foundation (DFG) within Collaborative Research Center [1109]; National Science Foundation; Alexander von Humboldt foundation FX This research is funded by the Air Force Office of Scientific Research under Grant No. FA9550-12-1-0160 and by the German Research Foundation (DFG) within the Collaborative Research Center 1109. M.L.W. thanks the National Science Foundation for a graduate research fellowship. X.S. thanks the Alexander von Humboldt foundation for a postdoctoral fellowship. NR 80 TC 0 Z9 0 U1 11 U2 28 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 28 PY 2016 VL 144 IS 12 AR 124308 DI 10.1063/1.4942194 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DI6XV UT WOS:000373644400032 PM 27036449 ER PT J AU Nemeth, B Young, DL Page, MR LaSalvia, V Johnston, S Reedy, R Stradins, P AF Nemeth, Bill Young, David L. Page, Matthew R. LaSalvia, Vincenzo Johnston, Steve Reedy, Robert Stradins, Paul TI Polycrystalline silicon passivated tunneling contacts for high efficiency silicon solar cells SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID BORON-DIFFUSION; HYDROGEN PASSIVATION; BIPOLAR-TRANSISTORS; SI; LAYERS; DEPOSITION; GROWTH; OXIDE AB We apply n- and p-type polycrystalline silicon (poly-Si) films on tunneling SiOx to form passivated contacts to n-type Si wafers. The resulting induced emitter and n+/n back surface field junctions of high carrier selectivity and low contact resistivity enable high efficiency Si solar cells. This work addresses the materials science of their performance governed by the properties of the individual layers (poly-Si, tunneling oxide) and more importantly, by the process history of the cell as a whole. Tunneling SiOx layers (<2 nm) are grown thermally or chemically, followed by a plasma enhanced chemical vapor deposition growth of p+ or n+ doped a-Si: H. The latter is thermally crystallized into poly-Si, resulting in grain nucleation and growth as well as dopant diffusion within the poly-Si and penetration through the tunneling oxide into the Si base wafer. The cell process is designed to improve the passivation of both oxide interfaces and tunneling transport through the oxide. A novel passivation technique involves coating of the passivated contact and whole cell with atomic layer deposited Al2O3 and activating them at 400 degrees C. The resulting excellent passivation persists after subsequent chemical removal of the Al2O3. The preceding cell process steps must be carefully tailored to avoid structural and morphological defects, as well as to maintain or improve passivation, and carrier selective transport. Furthermore, passivated contact metallization presents significant challenges, often resulting in passivation loss. Suggested remedies include improved Si cell wafer surface morphology (without micropyramids) and postdeposited a-Si:H capping layers over the poly-Si. C1 [Nemeth, Bill; Young, David L.; Page, Matthew R.; LaSalvia, Vincenzo; Johnston, Steve; Reedy, Robert; Stradins, Paul] Natl Renewable Energy Lab, Golden, CO 80401 USA. RP Nemeth, B (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM William.Nemeth@nrel.gov FU U.S. Department of Energy EERE SETP [DOE DE-EE00025783, DE-EE0006336] FX We would like to thank the silicon group at Fraunhofer ISE for providing n-FZ B-emitter samples, Ajeet Rohatgi at Georgia Tech for discussions, Adam Payne at Suniva for providing wafer random pyramid texturing, and Clay DeHart for aluminum e-beam deposition on samples. This work was supported by the U.S. Department of Energy EERE SETP under contracts DOE DE-EE00025783 and DE-EE0006336. NR 33 TC 4 Z9 4 U1 12 U2 29 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD MAR 28 PY 2016 VL 31 IS 6 BP 671 EP 681 DI 10.1557/jmr.2016.77 PG 11 WC Materials Science, Multidisciplinary SC Materials Science GA DI4KV UT WOS:000373469700001 ER PT J AU Furnish, TA Boyce, BL Sharon, JA O'Brien, CJ Clark, BG Arrington, CL Pillars, JR AF Furnish, Timothy A. Boyce, Brad L. Sharon, John A. O'Brien, Christopher J. Clark, Blythe G. Arrington, Christian L. Pillars, Jamin R. TI Fatigue stress concentration and notch sensitivity in nanocrystalline metals SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID MECHANICAL-PROPERTIES; GRAIN-GROWTH; BEHAVIOR; FRACTURE; SIZE; ALLOYS; NICKEL; STRENGTH; COPPER; FILMS AB Recent studies have shown the potential for nanocrystalline metals to possess excellent fatigue resistance compared to their coarse-grained counterparts. Although the mechanical properties of nanocrystalline metals are believed to be particularly susceptible to material defects, a systematic study of the effects of geometric discontinuities on their fatigue performance has not yet been performed. In the present work, nanocrystalline Ni-40 wt% Fe containing both intrinsic and extrinsic defects were tested in tension-tension fatigue. The defects were found to dramatically reduce the fatigue resistance, which was attributed to the relatively high notch sensitivity in the nanocrystalline material. Microstructural analysis within the crack-initiation zones underneath the defects revealed cyclically-induced abnormal grain growth (AGG) as a predominant deformation and crack initiation mechanism during high-cycle fatigue. The onset of AGG and the ensuing fracture is likely accelerated by the stress concentrations, resulting in the reduced fatigue resistance compared to the relatively defect-free counterparts. C1 [Furnish, Timothy A.; Boyce, Brad L.; Sharon, John A.; O'Brien, Christopher J.; Clark, Blythe G.] Sandia Natl Labs, Mat Sci & Engn, POB 5800, Albuquerque, NM 87185 USA. [Sharon, John A.] United Technol Res Ctr, Hartford, CT 06118 USA. [Arrington, Christian L.; Pillars, Jamin R.] Sandia Natl Labs, Microsyst Sci Technol & Components, POB 5800, Albuquerque, NM 87185 USA. RP Boyce, BL (reprint author), Sandia Natl Labs, Mat Sci & Engn, POB 5800, Albuquerque, NM 87185 USA. EM blboyce@sandia.gov OI O'Brien, Christopher/0000-0001-7210-9257 FU United States Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors thank Michael Rye for FIB notch preparation and microscopy support and Dr. Bill Mook and Amy Allen for additional microscopy support. The authors also thank Dr. Khalid Hattar and Dr. Stephen Foiles for careful internal review of this manuscript. This work was performed, in part, at the Center for Integrated Nanotechnologies, a United States Department of Energy, Office of Basic Energy Sciences user facility. This work was funded by the United States Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 54 TC 1 Z9 1 U1 7 U2 9 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD MAR 28 PY 2016 VL 31 IS 6 BP 740 EP 752 DI 10.1557/jmr.2016.66 PG 13 WC Materials Science, Multidisciplinary SC Materials Science GA DI4KV UT WOS:000373469700008 ER PT J AU Timokhina, IB Miller, MK Beladi, H Hodgson, PD AF Timokhina, Ilana B. Miller, Michael K. Beladi, Hossein Hodgson, Peter D. TI The influence of fine ferrite formation on the gamma/alpha interface, fine bainite and retained austenite in a thermomechanically-processed transformation induced plasticity steel SO JOURNAL OF MATERIALS RESEARCH LA English DT Article ID FE-C-MN; ATOM-PROBE TOMOGRAPHY; DUAL-PHASE STEELS; TRANSMISSION ELECTRON-MICROSCOPY; HIGH-STRENGTH STEELS; TRIP STEELS; MECHANICAL-PROPERTIES; CARBON-STEELS; ULTRAFINE FERRITE; GROWTH-KINETICS AB An Fe-0.26C-1.96Si-2Mn with 0.31Mo (wt%) steel was subjected to a novel thermomechanical processing route to produce fine ferrite with different volume fractions, bainite, and retained austenite. Two types of fine ferrites were found to be: (i) formed along prior austenite grain boundaries, and (ii) formed intragranularly in the interior of austenite grains. An increase in the volume fraction of fine ferrite led to the preferential formation of blocky retained austenite with low stability, and to a decrease in the volume fraction of bainite with stable layers of retained austenite. The difference in the morphology of the bainitic ferrite and the retained austenite after different isothermal ferrite times was found to be responsible for the deterioration of the mechanical properties. The segregation of Mn, Mo, and C at distances of 2-2.5 nm from the ferrite and retained austenite/martensite interface on the retained austenite/martensite site was observed after 2700 s of isothermal hold. It was suggested that the segregation occurred during the austenite-to-ferrite transformation, and that this would decrease the interface mobility, which affects the austenite-to-ferrite transformation and ferrite grain size. C1 [Timokhina, Ilana B.; Beladi, Hossein; Hodgson, Peter D.] Deakin Univ, Inst Frontier Mat, Geelong, Vic 3217, Australia. [Miller, Michael K.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Timokhina, IB (reprint author), Deakin Univ, Inst Frontier Mat, Geelong, Vic 3217, Australia. EM ilana.timokhina@deakin.edu.au FU ARC Laureate Fellowship scheme; ORNL's Center for Nanophase Materials Sciences (CNMS); Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX The authors would like to acknowledge the technical and scientific support of the Center for Electron Microscopy at Monash University. One of the authors (I.T.) acknowledges the support of Outside Study Program from Deakin University. One of the authors (P.D.H.) also acknowledges the support of the ARC Laureate Fellowship scheme. Atom probe tomography (M.K.M.) was supported through a user project supported by ORNL's Center for Nanophase Materials Sciences (CNMS), which is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 62 TC 0 Z9 0 U1 6 U2 10 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD MAR 28 PY 2016 VL 31 IS 6 BP 806 EP 818 DI 10.1557/jmr.2016.73 PG 13 WC Materials Science, Multidisciplinary SC Materials Science GA DI4KV UT WOS:000373469700014 ER PT J AU Saquet, N Holland, DMP Pratt, ST Cubaynes, D Tang, X Garcia, GA Nahon, L Reid, KL AF Saquet, N. Holland, D. M. P. Pratt, S. T. Cubaynes, D. Tang, X. Garcia, G. A. Nahon, L. Reid, K. L. TI Effect of electronic angular momentum exchange on photoelectron anisotropy following the two-color ionization of krypton atoms SO PHYSICAL REVIEW A LA English DT Article ID SYNCHROTRON-RADIATION; VARIABLE-POLARIZATION; DISTRIBUTIONS; SPECTROSCOPY; DYNAMICS; PHOTOIONIZATION; DICHROISM; MOLECULES; LASER AB We present photoelectron energy and angular distributions for resonant two-photon ionization via several low-lying Rydberg states of atomic Kr. The experiments were performed by using synchrotron radiation to pump the Rydberg states and a continuous-wave laser to probe them. Photoelectron images, recorded with both linear and circular polarized pump and probe light, were obtained in coincidence with mass-analyzed Kr ions. The photoelectron angular distributions and branching ratios for direct ionization into the Kr+ P-2(3/2) and P-2(1/2) spin-orbit continua show considerable dependence on the intermediate level, as well as on the polarizations of the pump and probe light. Photoelectron images were also recorded with several polarization combinations following two-color excitation of the (P-2(1/2))5f[5/2](2) autoionizing resonance. These results are compared with the results of recent work on the corresponding autoionizing resonance in atomic Xe [E. V. Gryzlova et al., New J. Phys. 17, 043054 (2015)]. C1 [Saquet, N.; Reid, K. L.] Univ Nottingham, Sch Chem, Nottingham NG7 2RD, England. [Holland, D. M. P.] STFC, Daresbury Lab, Warrington WA4 4AD, Cheshire, England. [Pratt, S. T.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Cubaynes, D.] Univ Paris 11, CNRS UMR 8214, ISMO, F-91405 Orsay, France. [Cubaynes, D.; Tang, X.; Garcia, G. A.; Nahon, L.] Synchrotron Soleil, LOrme Merisiers, St Aubin BP 48, F-91192 Gif Sur Yvette, France. [Tang, X.] Chinese Acad Sci, Lab Atmospher Phys Chem, Anhui Inst Opt & Fine Mech, Hefei 230031, Anhui, Peoples R China. RP Reid, KL (reprint author), Univ Nottingham, Sch Chem, Nottingham NG7 2RD, England. EM Katharine.Reid@nottingham.ac.uk OI Garcia, Gustavo/0000-0003-2915-2553 FU Leverhulme Trust [RPG-2013-032]; Science and Technology Facilities Council, UK; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357] FX We are grateful to the SOLEIL general staff for the smooth running of the facility under proposal 20140882. In particular, we wish to thank J.-F. Gil for his technical help with the SAPHIRS setup and Catherine Le Bris for her assistance in setting up the dye laser. N.S. thanks the Leverhulme Trust for a research fellowship under Grant No. RPG-2013-032, which also provided travel support to N.S. and K.L.R.; D.M.P.H. was supported by the Science and Technology Facilities Council, UK. S.T.P. was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences, under Contract No. DE-AC02-06CH11357. NR 33 TC 0 Z9 0 U1 8 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD MAR 28 PY 2016 VL 93 IS 3 AR 033419 DI 10.1103/PhysRevA.93.033419 PG 11 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DH5AQ UT WOS:000372797700008 ER PT J AU Kaluarachchi, US Lin, QS Xie, WW Taufour, V Bud'ko, SL Miller, GJ Canfield, PC AF Kaluarachchi, Udhara S. Lin, Qisheng Xie, Weiwei Taufour, Valentin Bud'ko, Sergey L. Miller, Gordon J. Canfield, Paul C. TI Superconducting properties of Rh9In4S4 single crystals SO PHYSICAL REVIEW B LA English DT Article ID CHARGE-DENSITY-WAVE; HIGH MAGNETIC-FIELDS; ELECTRICAL-PROPERTIES; HARD SUPERCONDUCTORS; II SUPERCONDUCTORS; SOLUTION GROWTH; TRANSITION; TEMPERATURE; DEPENDENCE; PARKERITE AB The synthesis and crystallographic, thermodynamic, and transport properties of single crystalline Rh9In4S4 were studied. The resistivity, magnetization, and specific heat measurements all clearly indicate bulk superconductivity with a critical temperature, T-c similar to 2.25 K. The Sommerfeld coefficient gamma and the Debye temperature(Theta(D)) were found to be 34 mJ mol(-1) K-2 and 217 K, respectively. The observed specific heat jump, Delta C/gamma T-c = 1.66, is larger than the expected BCS weak coupling value of 1.43. Ginzburg-Landau (GL) is large: kappa similar to 60. Furthermore, we observed a peak effect in the resistivity measurement as a function ratio of the low-temperature GL-penetration depth, lambda(GL) approximate to 5750 angstrom, to the GL-coherence length, xi(GL) approximate to 94 angstrom, of both temperature and magnetic field. C1 [Kaluarachchi, Udhara S.; Lin, Qisheng; Xie, Weiwei; Taufour, Valentin; Bud'ko, Sergey L.; Miller, Gordon J.; Canfield, Paul C.] Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA. [Kaluarachchi, Udhara S.; Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Xie, Weiwei; Miller, Gordon J.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Xie, Weiwei] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. RP Kaluarachchi, US (reprint author), Iowa State Univ, Ames Lab, US DOE, Ames, IA 50011 USA.; Kaluarachchi, US (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; U.S. DOE [DE-AC02-07CH11358]; Critical Material Institute, an Energy Innovation Hub - U.S. DOE, Office of Energy Efficiency and Renewal Energy, Advanced Manufacturing Office FX We thank W. Straszheim, Z. Lin, and K. Sun for experimental assistance and A. Kreyssig, R. Prozorov, V. G. Kogan, T. Kong, M. Kramer, and R. J. Cava (Princeton University) for useful discussions. This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Materials Science and Engineering Division. The research was performed at the Ames Laboratory, which is operated for the U.S. DOE by Iowa State University under Contract No. DE-AC02-07CH11358. V.T. is partially supported by Critical Material Institute, an Energy Innovation Hub funded by U.S. DOE, Office of Energy Efficiency and Renewal Energy, Advanced Manufacturing Office. NR 66 TC 0 Z9 0 U1 6 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 28 PY 2016 VL 93 IS 9 AR 094524 DI 10.1103/PhysRevB.93.094524 PG 7 WC Physics, Condensed Matter SC Physics GA DH5BA UT WOS:000372798800005 ER PT J AU Kuhn, SJ Kawano-Furukawa, H Jellyman, E Riyat, R Forgan, EM Ono, M Kihou, K Lee, CH Hardy, F Adelmann, P Wolf, T Meingast, C Gavilano, J Eskildsen, MR AF Kuhn, S. J. Kawano-Furukawa, H. Jellyman, E. Riyat, R. Forgan, E. M. Ono, M. Kihou, K. Lee, C. H. Hardy, F. Adelmann, P. Wolf, Th. Meingast, C. Gavilano, J. Eskildsen, M. R. TI Simultaneous evidence for Pauli paramagnetic effects and multiband superconductivity in KFe2As2 by small-angle neutron scattering studies of the vortex lattice SO PHYSICAL REVIEW B LA English DT Article ID FLUX-LINE-LATTICE; HIGH-TEMPERATURE SUPERCONDUCTIVITY; UNIAXIAL SUPERCONDUCTORS; II SUPERCONDUCTORS; DIFFRACTION; FIELD; SYMMETRY; NIOBIUM; STATE AB We study the intrinsic anisotropy of the superconducting state in KFe2As2 by using small-angle neutron scattering to image the vortex lattice as the applied magnetic field is rotated towards the FeAs crystalline planes. The anisotropy is found to be strongly field dependent, indicating multiband superconductivity. Furthermore, the high-field anisotropy significantly exceeds that of the upper critical field, providing further support for Pauli limiting in KFe2As2 for fields applied in the basal plane. The effect of Pauli paramagnetism on the unpaired quasiparticles in the vortex cores is directly evident from the ratio of scattered intensities due to the longitudinal and transverse vortex lattice field modulation. C1 [Kuhn, S. J.; Eskildsen, M. R.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Kawano-Furukawa, H.] Ochanomizu Univ, Grad Sch Humanities & Sci, Div Nat Appl Sci, Bunkyo Ku, Tokyo 1128610, Japan. [Jellyman, E.; Riyat, R.; Forgan, E. M.] Univ Birmingham, Sch Phys & Astron, Birmingham B15 2TT, W Midlands, England. [Ono, M.] Ochanomizu Univ, Dept Phys, Bunkyo Ku, Tokyo 1128610, Japan. [Kihou, K.; Lee, C. H.] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058568, Japan. [Hardy, F.; Adelmann, P.; Wolf, Th.; Meingast, C.] Karlsruhe Inst Technol, Inst Solid State Phys IFP, D-76021 Karlsruhe, Germany. [Gavilano, J.] Paul Scherrer Inst, Neutron Scattering Lab, CH-5232 Villigen, Switzerland. [Kuhn, S. J.] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Eskildsen, MR (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. EM eskildsen@nd.edu RI Kawano-Furukawa, Hazuki/M-7646-2016; Kawano-Furukawa, Hazuki/M-7695-2016 OI Kawano-Furukawa, Hazuki/0000-0003-4713-3727; Kawano-Furukawa, Hazuki/0000-0003-4713-3727 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-FG02-10ER46783]; Institute for Solid State Physics, University of Tokyo [14573]; European Commission [283883]; UK EPSRC [EP/J016977]; Japan Society for the Promotion of Science [24340090] FX We acknowledge valuable discussions with K. Machida. This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Award No. DE-FG02-10ER46783 (SJK, MRE); the Institute for Solid State Physics, University of Tokyo and originally approved (Proposal No. 14573) for JRR-3, Japan Atomic Energy Agency (HKF); the European Commission under the 7th Framework Programme through the "Research Infrastructures" action of the "Capacities" Programme, NMI3-II Grant No 283883 and the UK EPSRC under Grant No. EP/J016977 (EJ, RR, and EMF); the Japan Society for the Promotion of Science, under Grant-in-Aid for Scientific Research B No. 24340090. This work is based on experiments performed at the Swiss Spallation Neutron Source SINQ, Paul Scherrer Institute, Villigen, Switzerland. NR 53 TC 0 Z9 0 U1 5 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 28 PY 2016 VL 93 IS 10 AR 104527 DI 10.1103/PhysRevB.93.104527 PG 8 WC Physics, Condensed Matter SC Physics GA DH5AX UT WOS:000372798400005 ER PT J AU Li, LJ Wang, KF Graf, D Wang, LM Wang, AF Petrovic, C AF Li, Lijun Wang, Kefeng Graf, D. Wang, Limin Wang, Aifeng Petrovic, C. TI Electron-hole asymmetry, Dirac fermions, and quantum magnetoresistance in BaMnBi2 SO PHYSICAL REVIEW B LA English DT Article ID TOPOLOGICAL INSULATORS; GRAPHENE; SUPERCONDUCTORS; OSCILLATIONS; SRMNBI2 AB We report two-dimensional quantum transport and Dirac fermions in BaMnBi2 single crystals. BaMnBi2 is a layered bad metal with highly anisotropic conductivity and magnetic order below 290 K. Magnetotransport properties, nonzero Berry phase, small cyclotronmass, and the first-principles band structure calculations indicate the presence of Dirac fermions in Bi square nets. Quantum oscillations in the Hall channel suggest the presence of both electron and hole pockets, whereas Dirac and parabolic states coexist at the Fermi level. C1 [Li, Lijun; Wang, Kefeng; Wang, Limin; Wang, Aifeng; Petrovic, C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Graf, D.] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32306 USA. [Li, Lijun] Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Peoples R China. [Wang, Kefeng; Wang, Limin] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. RP Li, LJ (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA.; Li, LJ (reprint author), Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Peoples R China. FU U.S. DOE [DE-SC0012704]; NSF [DMR-0654118]; state of Florida FX Work at Brookhaven is supported by the U.S. DOE under Contract No. DE-SC0012704. Work at the National High Magnetic Field Laboratory is supported by the NSF Cooperative Agreement No. DMR-0654118, and by the state of Florida. NR 40 TC 5 Z9 5 U1 15 U2 37 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 28 PY 2016 VL 93 IS 11 AR 115141 DI 10.1103/PhysRevB.93.115141 PG 5 WC Physics, Condensed Matter SC Physics GA DH5BD UT WOS:000372799100001 ER PT J AU Nazarov, R Shulenburger, L Morales, M Hood, RQ AF Nazarov, R. Shulenburger, L. Morales, M. Hood, Randolph Q. TI Benchmarking the pseudopotential and fixed-node approximations in diffusion Monte Carlo calculations of molecules and solids SO PHYSICAL REVIEW B LA English DT Article ID EFFECTIVE CORE POTENTIALS; HARTREE-FOCK PSEUDOPOTENTIALS; MANY-BODY SIMULATIONS; DISSOCIATION-ENERGY; GROUND-STATE; DIATOMIC-MOLECULES; STOCHASTIC METHOD; ARGON MATRICES; WAVE-FUNCTIONS; ELECTRON-GAS AB We performed diffusion Monte Carlo (DMC) calculations of the spectroscopic properties of a large set of molecules, assessing the effect of different approximations. In systems containing elements with large atomic numbers, we show that the errors associated with the use of nonlocal mean-field-based pseudopotentials in DMC calculations can be significant and may surpass the fixed-node error. We suggest practical guidelines for reducing these pseudopotential errors, which allow us to obtain DMC-computed spectroscopic parameters of molecules and equation of state properties of solids in excellent agreement with experiment. C1 [Nazarov, R.; Morales, M.; Hood, Randolph Q.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Shulenburger, L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. RP Nazarov, R (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; LDRD [13-ERD-067]; Predictive Theory and Modeling for Materials and Chemical Science program by the U.S. Department of Energy Office of Science, Basic Energy Sciences (BES); U.S. Department of Energy [DE-AC04-94AL85000] FX Work by R.N., R.Q.H., and M.M. was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. This paper has been supported by LDRD 13-ERD-067. L.S. was supported through the Predictive Theory and Modeling for Materials and Chemical Science program by the U.S. Department of Energy Office of Science, Basic Energy Sciences (BES). Sandia National Laboratories is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 100 TC 5 Z9 5 U1 4 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 28 PY 2016 VL 93 IS 9 AR 094111 DI 10.1103/PhysRevB.93.094111 PG 15 WC Physics, Condensed Matter SC Physics GA DH5BA UT WOS:000372798800001 ER PT J AU Aad, G Abbott, B Abdallah, J Khalek, SA Abdinov, O Aben, R Abi, B Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Agatonovic-Jovin, T Aguilar-Saavedra, JA Agustoni, M Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aring;kesson, TPA Akimoto, G Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexandre, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Allbrooke, BMM Allison, LJ Allport, PP Almond, J Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Alviggi, MG Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anderson, KJ Andreazza, A Andrei, V Anduaga, XS Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonaki, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Apolle, R Arabidze, G Aracena, I Arai, Y Araque, JP Arce, ATH Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Aring;sman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Azuelos, G Azuma, Y Baak, MA Baas, AE Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Mayes, JB Badescu, E Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Balek, P Balli, F Banas, E Banerjee, S Bannoura, AAE Bansal, V Bansil, HS Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bartsch, V Bassalat, A Basye, A Bates, RL Batley, JR Battaglia, M Battistin, M Bauer, F Bawa, HS Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bedikian, S Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, PJ Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Benslama, K Bentvelsen, S Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernat, P Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Bieniek, SP Bierwagen, K Biesiada, J Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Black, CW Black, JE 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Buckingham, RM Buckley, AG Buda, SI Budagov, IA Buehrer, F Bugge, L Bugge, MK Bulekov, O Bundock, AC Burckhart, H Burdin, S Burghgrave, B Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Buszello, CP Butler, B Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Byszewski, M Urban, SC Caforio, D Cakir, O Calafiura, P Calandri, A Calderini, G Calfayan, P Calkins, R Caloba, LP Calvet, D Calvet, S Toro, RC Camarda, S Cameron, D Caminada, LM Armadans, RC Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrill, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Cardarelli, R Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catastini, P Catinaccio, A Catmore, JR Cattai, A Cattani, G Caudron, J Caughron, S Cavaliere, V Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Cerio, BC Cerny, K Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chang, P Chapleau, B Chapman, JD Charfeddine, D Charlton, DG Chau, CC Barajas, CAC Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, L Chen, S Chen, X Chen, Y Chen, Y Cheng, HC Cheng, Y Cheplakov, A El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiefari, G Childers, JT Chilingarov, A Chiodini, G Chisholm, AS Chislett, RT Chitan, A Chizhov, MV Chouridou, S Chow, BKB Chromek-Burckhart, D Chu, ML Chudoba, J Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Ciftci, R Cinca, D Cindro, V Ciocio, A Cirkovic, P Citron, ZH Ciubancan, M Clark, A Clark, PJ Clarke, RN Cleland, W Clemens, JC Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Cogan, JG Coggeshall, J Cole, B Cole, S Colijn, AP Collot, J Colombo, T Colon, G Compostella, G Muino, PC Coniavitis, E Conidi, MC Connell, SH Connelly, IA Consonni, SM Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cooper-Smith, NJ Copic, K Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cote, D Cottin, G Cowan, G Cox, BE Cranmer, K Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Cuciuc, CM Donszelmann, TC Cummings, J Curatolo, M Cuthbert, C Czirr, H Czodrowski, P Czyczula, Z D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dafinca, A Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Daniells, AC Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, E Davies, M Davignon, O Davison, AR Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Nooij, L De Pedis, D De Salvo, A De Sanctis, U De 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G Ducu, OA Duda, D Dudarev, A Dudziak, F Duflot, L Duguid, L Duhrssen, M Dunford, M Yildiz, HD Duren, M Durglishvili, A Dwuznik, M Dyndal, M Ebke, J Edson, W Edwards, NC Ehrenfeld, W Eifert, T Eigen, G Einsweiler, K Ekelof, T El Kacimi, M Ellert, M Elles, S Ellinghaus, F Ellis, N Elmsheuser, J Elsing, M Emeliyanov, D Enari, Y Endner, OC Endo, M Erdmann, J Ereditato, A Eriksson, D Ernis, G Ernst, J Ernst, M Ernwein, J Errede, D Errede, S Ertel, E Escalier, M Esch, H Escobar, C Esposito, B Etienvre, AI Etzion, E Evans, H Ezhilov, A Fabbri, L Facini, G Fakhrutdinov, RM Falciano, S Falla, RJ Faltova, J Fang, Y Fanti, M Farbin, A Farilla, A Farooque, T Farrell, S Farrington, SM Farthouat, P Fassi, F Fassnacht, P Fassouliotis, D Favareto, A Fayard, L Federic, P Fedin, OL Fedorko, W Fehling-Kaschek, M Feigl, S Feligioni, L Feng, C Feng, EJ Feng, H Fenyuk, AB Perez, SF Ferrag, S Ferrando, J Ferrari, A Ferrari, P Ferrari, R de Lima, DEF Ferrer, A Ferrere, D Ferretti, C Parodi, AF Fiascaris, M 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TI Centrality, rapidity, and transverse momentum dependence of isolated prompt photon production in lead-lead collisions at root S-NN=2.76 TeV measured with the ATLAS detector SO PHYSICAL REVIEW C LA English DT Article ID CROSS-SECTION; P(P)OVER-BAR COLLISIONS; NUCLEAR COLLISIONS; PP COLLISIONS; PROTON; COLLIDER; QUARK; FLOW AB Prompt photon production in root S-NN = 2.76-TeV Pb + Pb collisions has been measured by the ATLAS experiment at the Large Hadron Collider using data collected in 2011 with an integrated luminosity of 0.14 nb(-1). Inclusive photon yields, scaled by the mean nuclear thickness function, are presented as a function of collision centrality and transverse momentum in two pseudorapidity intervals, vertical bar eta vertical bar < 1.37 and 1.52 <= vertical bar eta vertical bar < 2.37. The scaled yields in the two pseudorapidity intervals, as well as the ratios of the forward yields to those at midrapidity, are compared to the expectations from next-to-leading-order perturbative QCD (pQCD) calculations. The measured cross sections agree well with the predictions for proton-proton collisions within statistical and systematic uncertainties. Both the yields and the ratios are also compared to two other pQCD calculations, one which uses the isospin content appropriate to colliding lead nuclei and another which includes nuclear modifications to the nucleon parton distribution functions. C1 [Jackson, P.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Gingrich, D. M.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Sbrizzi, A.; Vaque, F. 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[Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Latour, B. Martin Dit; Rosendahl, P. L.; Sandaker, H.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Barnett, R. M.; Beringer, J.; Biesiada, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Kravchenko, A.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Barnett, R. M.; Beringer, J.; Biesiada, J.; Brandt, G.; Brosamer, J.; Calafiura, P.; Caminada, L. M.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Copic, K.; Dube, S.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Holmes, T. R.; Hurwitz, M.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quarrie, D. R.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Tsulaia, V.; Virzi, J.; Wang, H.; Yao, W-M.; Yu, D. R.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Herrberg-Schubert, R.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Stamm, S.; Wendland, D.; zur Nedden, M.] Humboldt Univ, Dept Phys, D-10099 Berlin, Germany. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Meloni, F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Agustoni, M.; Beck, H. P.; Cervelli, A.; Ereditato, A.; Gallo, V.; Haug, S.; Kruker, T.; Marti, L. F.; Meloni, F.; Schneider, B.; Sciacca, F. G.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allbrooke, B. M. M.; Bella, L. Aperio; Bansil, H. S.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Daniells, A. C.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Palmer, J. D.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istin, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Alberghi, G. L.; Bellagamba, L.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Caforio, D.; Corradi, M.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Semprini-Cesari, N.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Caforio, D.; De Castro, S.; Di Sipio, R.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Semprini-Cesari, N.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Brock, I.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Haefner, P.; Hageboeck, S.; Hellmich, D.; Hillert, S.; Huegging, F.; Janssen, J.; Khoriauli, G.; Koevesarki, P.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lapoire, C.; Lehmacher, M.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Mueller, K.; Nanava, G.; Nattermann, T.; Obermann, T.; Pohl, D.; Sarrazin, B.; Schaepe, S.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Stillings, J. A.; Tannoury, N.; Therhaag, J.; Uchida, K.; Uhlenbrock, M.; Velz, T.; Vogel, A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Zimmermann, R.; Zimmermann, S.] Univ Bonn, Inst Phys, Nussallee 12, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Fitzgerald, E. A.; Gozpinar, S.; Sciolla, G.; Venturini, A.; Zambito, S.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes De Andrade Filho, L.] Fed Univ Juiz de Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Klimentov, A.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Okawa, H.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Schovancova, J.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Badescu, E.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Cuciuc, C. -M.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Buttinger, W.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Frost, J. A.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Sandoval, T.; Thomson, M.; Ward, C. P.; Williams, S.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; Marchand, J. F.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.; Whalen, K.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Abreu, R.; Aleksa, M.; Andari, N.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Battistin, M.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Franchino, S.; Francis, D.; Froidevaux, D.; Garonne, V.; Gianotti, F.; Gillberg, D.; Glatzer, J.; Godlewski, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hauschild, M.; Hawkings, R. J.; Heller, M.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Hubacek, Z.; Huhtinen, M.; Jaekel, M. R.; Jakobsen, S.; Jansen, H.; Jenni, P.; Jungst, R. M.; Kaneda, M.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Martin, B.; Marzin, A.; Messina, A.; Meyer, J.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Negri, G.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Rodrigues, L.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Savu, D. O.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van der Ster, D.; van Eldik, N.; van Woerden, M. C.; Vandelli, W.; Vigne, R.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Boveia, A.; Cheng, Y.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Li, H. L.; Meehan, S.; Melachrinos, C.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Shochet, M. J.; Tompkins, L.; Vukotic, I.; Webster, J. S.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Liu, B.; Ouyang, Q.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Yao, L.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guan, L.; Han, L.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, K.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, Y.; Wang, C.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Clermont Ferrand 2, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Ghodbane, N.; Gilles, G.; Gris, Ph.; Guicheney, C.; Liao, H.; Pallin, D.; Hernandez, D. Paredes; Podlyski, F.; Santoni, C.; Theveneaux-Pelzer, T.; Valery, L.; Vazeille, F.] Univ Blaise Pascal, Clermont Ferrand, France. [Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Chen, Y.; Cole, B.; Guo, J.; Hu, D.; Hughes, E. W.; Mohapatra, S.; Nikiforou, N.; Parsons, A.; Reale, V. Perez; Scherzer, M. I.; Thompson, E. N.; Tian, F.; Tuts, P. M.; Urbaniec, D.; Wulf, E.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Petersen, T. C.; Pingel, A.; Simonyan, M.; Thomsen, L. A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Collegato Cosenza, Frascati, Italy. [Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dwuznik, M.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hoffman, J.; Kama, S.; Kehoe, R.; Randle-Conde, A. S.; Sekula, S. J.; Stroynowski, R.; Wang, H.; Ye, J.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Lou, X.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Camarda, S.; Dassoulas, J.; Deterre, C.; Dietrich, J.; Filipuzzi, M.; Friedrich, C.; Glazov, A.; Fajardo, L. S. Gomez; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Belenguer, M. Jimenez; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lisovyi, M.; Lobodzinska, E.; Lohwasser, K.; Medinnis, M.; Moenig, K.; Naumann, T.; Peschke, R.; Petit, E.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Wildt, M. A.; Yatsenko, E.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Esch, H.; Goessling, C.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Wittig, T.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Kobel, M.; Leonhardt, K.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Pollard, C. S.; Wang, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Garay Walls, F. M.; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Selbach, K. E.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Annovi, A.; Antonelli, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Prokofiev, K.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Consorti, V.; Dao, V.; Di Simone, A.; Fehling-Kaschek, M.; Flechl, M.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Lai, S.; Landgraf, U.; Madar, R.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Rave, T. C.; Ronzani, M.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Anh, T. Vu; Warsinsky, M.; Weiser, C.; Werner, M.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Alexandre, G.; Ancu, L. S.; Barone, G.; Bell, P. J.; Bell, W. H.; De Mendizabal, J. Bilbao; Bucci, F.; Toro, R. Camacho; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Doglioni, C.; Ferrere, D.; Gadomski, S.; Gonzalez-Sevilla, S.; Goulette, M. P.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; La Rosa, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nektarijevic, S.; Nessi, M.; Nikolics, K.; Picazio, A.; Pohl, M.; Rosbach, K.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Guido, E.; Osculati, B.; Parodi, F.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doherty, T.; Doyle, A. T.; Ferrag, S.; Ferrando, J.; de Lima, D. E. Ferreira; Gemmell, A.; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Moraes, A.; O'Shea, V.; Barrera, C. Oropeza; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Saxon, D. H.; Smith, K. M.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.; Wright, M.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Bierwagen, K.; Bindi, M.; Blumenschein, U.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Hensel, C.; Kawamura, G.; Kroeninger, K.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Moreno Llacer, M.; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Serkin, L.; Shabalina, E.; Stolte, P.; Schroeder, T. Vazquez; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Dechenaux, B.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Butler, B.; Catastini, P.; Conti, G.; Franklin, M.; Huth, J.; Ippolito, V.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Yen, A. L.; della Porta, G. Zevi] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Dietzsch, T. A.; Djuvsland, J. I.; Dunford, M.; Hanke, P.; Jongmanns, J.; Khomich, A.; Kluge, E. -E.; Laier, H.; Lang, V. S.; Meier, K.; Mueller, F.; Poddar, S.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kasieczka, G.; Narayan, R.; Schaetzel, S.; Schmitt, S.; Schoening, A.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Brunet, S.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Poveda, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Franz, S.; Jussel, P.; Kneringer, E.; Lukas, W.; Nagai, K.; Ritsch, E.; Usanova, A.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Gandrajula, R. P.; Mallik, U.; Mandrysch, R.; Morange, N.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Dudziak, F.; Krumnack, N.; Prell, S.; Shrestha, S.; Yamamoto, K.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Glonti, G. L.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Kazarinov, M. Y.; Khramov, E.; Kotov, V. M.; Krumshteyn, Z. V.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Olchevski, A. G.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Topilin, N. D.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Kruchonak, U.; Makida, Y.; Mitsui, S.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Sasaki, O.; Suzuki, Y.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki 305, Japan. [Chen, Y.; Hasegawa, M.; Inamaru, Y.; Kishimoto, T.; Kurashige, H.; Kurumida, R.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Anduaga, X. S.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Allison, L. J.; Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Chilingarov, A.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Smizanska, M.; Walder, J.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Orlando, N.; Perrino, R.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Orlando, N.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Allport, P. P.; Bundock, A. C.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Mahmoud, S.; Maxfield, S. J.; Mehta, A.; Migas, S.; Price, J.; Readioff, N. P.; Schnellbach, Y. J.; Sellers, G.; Vossebeld, J. H.; Waller, P.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bona, M.; Bret, M. Cano; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cooper-Smith, N. J.; Cowan, G.; Duguid, L.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Rose, M.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bernat, P.; Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Cooper, B. D.; Davison, A. R.; Davison, P.; Falla, R. J.; Gregersen, K.; Gutschow, C.; Hesketh, G. G.; Jansen, E.; Konstantinidis, N.; Korn, A.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Pilkington, A. D.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.; Wijeratne, P. A.] UCL, Dept Phys & Astron, London, England. [Bernius, C.; Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Sircar, A.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; Davignon, O.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Liu, K.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Meirose, B.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Ellinghaus, F.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Goeringer, C.; Heck, T.; Hohlfeld, M.; Hsu, P. J.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koenig, S.; Koepke, L.; Lin, T. H.; Lungwitz, M.; Masetti, L.; Mattmann, J.; Meyer, C.; Moreno, D.; Moritz, S.; Mueller, T.; Poettgen, R.; Sander, H. G.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Wollstadt, S. J.; Zimmermann, C.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Almond, J.; Borri, M.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Klinger, J. A.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Owen, M.; Pater, J. R.; Peters, R. F. Y.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.; Yang, U. K.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Bertella, C.; Chen, L.; Clemens, J. C.; Coadou, Y.; Diglio, S.; Djama, F.; Feligioni, L.; Gao, J.; Hoffmann, D.; Hubaut, F.; Knoops, E. B. F. G.; Le Guirriec, E.; Li, B.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Ughetto, M.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Brau, B.; Colon, G.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Meade, A.; Moyse, E. J. 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M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Gonzalez, B. Alvarez; Arabidze, G.; Brock, R.; Bromberg, C.; Caughron, S.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Koll, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.; Zhang, H.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Simoniello, R.; Turra, R.; Perez, M. 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Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Grishkevich, Y. V.; Kramarenko, V. A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Ebke, J.; Elmsheuser, J.; Fanti, M.; Heller, C.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Schieck, J.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Will, J. Z.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Moser, H. G.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Pahl, C.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Sforza, F.; Spettel, F.; Stern, S.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Weigell, P.; Wildauer, A.; Zanzi, D.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Chiefari, G.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Giordano, R.; Iengo, P.; Izzo, V.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Chiefari, G.; Di Donato, C.; Giordano, R.; Merola, L.; Patricelli, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.; Wang, R.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Besjes, G. J.; Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Klok, P. F.; Konig, A. C.; Salvucci, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Boterenbrood, H.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Deviveiros, P. O.; Dhaliwal, S.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Lee, H.; Linde, F.; Mahlstedt, J.; Mechnich, J.; Oussoren, K. P.; Pani, P.; Salek, D.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Milosavljevic, M. Vranjes; Vreeswijk, M.; Weits, H.] Univ Amsterdam, Amsterdam, Netherlands. [Burghgrave, B.; Calkins, R.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.; Zutshi, V.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Kazanin, V. F.; Korol, A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Skovpen, K. Yu.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Lewis, G. H.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Merritt, H.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Tannenwald, B. B.; Yang, Y.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Bertsche, C.; Bertsche, D.; Gutierrez, P.; Hasib, A.; Norberg, S.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Abi, B.; Bousson, N.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kagan, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Brau, J. E.; Brost, E.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] Univ Paris 11, LAL, Orsay, France. [Khalek, S. Abdel; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; Charfeddine, D.; De Regie, J. B. De Vivie; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Tran, H. L.; Zerwas, D.; Zhang, Z.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Lee, J. S. H.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Gjelsten, B. K.; Gramstad, E.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Read, A. L.; Rohne, O.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Apolle, R.; Barr, A. J.; Behr, J. K.; Boddy, C. R.; Buckingham, R. M.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; King, R. S. B.; Kogan, L. A.; Lewis, A.; Livermore, S. S. A.; Nickerson, R. B.; Pachal, K.; Pinder, A.; Ryder, N. C.; Sawyer, C.; Short, D.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Wildt, M. A.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Via Palestro 3, I-27100 Pavia, Italy. [Brendlinger, K.; Heim, S.; Hines, E.; Hong, T. M.; Jackson, B.; Kroll, J.; Kunkle, J.; Lester, C. M.; Lipeles, E.; Meyer, C.; Ospanov, R.; Saxon, J.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Grebenyuk, O. G.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Kittelmann, T.; Mueller, J.; Prieur, D.; Sapp, K.; Su, J.; Yoosoofmiya, R.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Anjos, N.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Machado Miguens, J.; Maio, A.; Maneira, J.; Marques, C. N.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Stanescu, C.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, P-1000 Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Do Valle Wemans, A.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Silva, J.; Tavares Delgado, A.; Veloso, F.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC Fac Ciencias & Tecnol, Caparica, Portugal. [Bohm, J.; Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Gallus, P.; Guenther, J.; Jakubek, J.; Kohout, Z.; Kral, V.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Leitner, R.; Pleskot, V.; Reznicek, P.; Rybar, M.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Denisov, S. P.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Korotkov, V. A.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] State Res Ctr Inst High Energy Phys, Protvino, Russia. [Adye, T.; Apolle, R.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Scott, W. G.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Benslama, K.] Univ Regina, Dept Phys, Regina, SK S4S 0A2, Canada. [Tanaka, S.] Ritsumeikan Univ, Kusatsu, Shiga, Japan. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Dionisi, C.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Mirabelli, G.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Sidoti, A.; Vanadia, M.; Vari, R.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Dionisi, C.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Piazzale Aldo Moro 5, I-00185 Rome, Italy. [Aielli, G.; Cardarelli, R.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Paolozzi, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Cattani, G.; Di Ciaccio, A.; Grossi, G. C.; Iuppa, R.; Mazzaferro, L.; Paolozzi, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Passeri, A.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Bortolotto, V.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Taccini, C.; Trovatelli, M.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Gouighri, M.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Boutouil, S.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Ernwein, J.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Grabas, H. M. X.; Guyot, C.; Hanna, R.; Hassani, S.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mal, P.; Mansoulie, B.; Martinez, H.; Meric, N.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Tsionou, D.; Vranjes, N.; Xiao, M.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, Inst Rech Lois Fondamentles Univers, DSM IRFU, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Kuhl, A.; Law, A. T.; Liang, Z.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Fakhrutdinov, R. M.; Goussiou, A. G.; Harris, O. M.; Hsu, S. -C.; Litke, A. M.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; De Bruin, P. H. Sales; Solodkov, A. A.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Korolkova, E. V.; Paredes, B. Lopez; Miyagawa, P. S.; Paganis, E.; Suruliz, K.; Tovey, D. R.] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Sipica, V.; Stelzer, B.; Walkowiak, W.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Dawe, E.; Godfrey, J.; O'Neil, D. C.; Tanasijczuk, A. J.; Torres, H.; Trottier-McDonald, M.; Van Nieuwkoop, J.; Vetterli, M. C.; Ziolkowski, M.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Aracena, I.; Mayes, J. Backus; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Eifert, T.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Kocian, M.; Koi, T.; Lowe, A. J.; Malone, C.; Mount, R.; Nef, P. D.; Nelson, T. K.; Piacquadio, G.; Salnikov, A.; Schwartzman, A.; Silverstein, D.; Strauss, E.; Su, D.; Swiatlowski, M.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aloisio, A.; Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Yacoob, S.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Carrillo-Montoya, G. D.; Chen, X.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.; Vickey, T.; Boeriu, O. E. Vickey] Univ Witwatersrand, Sch Phys, Johannesburg 2050, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Eriksson, D.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Johansson, K. E.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Petridis, A.; Plucinski, P.; Rossetti, V.; Strandberg, S.; Tylmad, M.] Oskar Klein Ctr, Stockholm, Sweden. [Jovicevic, J.; Kuwertz, E. S.; Lund-Jensen, B.; Morley, A. K.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Bee, C. P.; Noccioli, E. Benhar; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bee, C. P.; Noccioli, E. Benhar; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Bartsch, V.; Cerri, A.; Barajas, C. A. Chavez; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Santoyo Castillo, I.; Shehu, C. Y.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Chu, M. L.; Hou, S.; Jamin, D. O.; Lee, C. A.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Ren, Z. L.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Weng, Z.; Zhang, L.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Di Mattia, A.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Guttman, N.; Munwes, Y.; Oren, Y.; Sadeh, I.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kordas, K.; Kouskoura, V.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.; Sidiropoulou, O.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Akimoto, G.; Asai, S.; Azuma, Y.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kessoku, K.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Nakamura, T.; Ninomiya, Y.; Okuyama, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamaguchi, H.; Yamamoto, S.; Yamamura, T.; Yamanaka, T.; Yoshihara, K.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. 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RI Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Mindur, Bartosz/A-2253-2017; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Moraes, Arthur/F-6478-2010; Solodkov, Alexander/B-8623-2017; Carli, Ina/C-2189-2017; Kantserov, Vadim/M-9761-2015; Mitsou, Vasiliki/D-1967-2009; Villa, Mauro/C-9883-2009; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; KHODINOV, ALEKSANDR/D-6269-2015; Conde Muino, Patricia/F-7696-2011; Boyko, Igor/J-3659-2013; SULIN, VLADIMIR/N-2793-2015; Warburton, Andreas/N-8028-2013; Snesarev, Andrey/H-5090-2013; 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Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Mindur, Bartosz/0000-0002-5511-2611; Fabbri, Laura/0000-0002-4002-8353; Moraes, Arthur/0000-0002-5157-5686; Solodkov, Alexander/0000-0002-2737-8674; Carli, Ina/0000-0002-0411-1141; Kantserov, Vadim/0000-0001-8255-416X; Mitsou, Vasiliki/0000-0002-1533-8886; Villa, Mauro/0000-0002-9181-8048; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; KHODINOV, ALEKSANDR/0000-0003-3551-5808; Conde Muino, Patricia/0000-0002-9187-7478; Boyko, Igor/0000-0002-3355-4662; SULIN, VLADIMIR/0000-0003-3943-2495; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Mashinistov, Ruslan/0000-0001-7925-4676; Vykydal, Zdenek/0000-0003-2329-0672; Olshevskiy, Alexander/0000-0002-8902-1793; Guo, Jun/0000-0001-8125-9433; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Wemans, Andre/0000-0002-9669-9500; Carvalho, Joao/0000-0002-3015-7821; Perrino, Roberto/0000-0002-5764-7337; Livan, Michele/0000-0002-5877-0062; Tikhomirov, Vladimir/0000-0002-9634-0581; White, Ryan/0000-0003-3589-5900; Doyle, Anthony/0000-0001-6322-6195; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Gladilin, Leonid/0000-0001-9422-8636 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon, European Union; Marie Skodowska-Curie Actions, European Union; Investissement d'Avenir Labex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos program; Thales program; Aristeia program - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; Investissement d'Avenir Idex, France FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST, and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR, and VSC CR, Czech Republic; DNRF, DNSRC, and Lundbeck Foundation, Denmark; IN2P3-CNRS and CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE, and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF, Cantons of Bern, and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020, and Marie Skodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; BSF, GIF, and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (U.K.), and BNL (USA) and in the Tier-2 facilities worldwide. NR 52 TC 1 Z9 1 U1 23 U2 60 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 28 PY 2016 VL 93 IS 3 AR 034914 DI 10.1103/PhysRevC.93.034914 PG 28 WC Physics, Nuclear SC Physics GA DH5BM UT WOS:000372800000003 ER PT J AU Amole, C Ardid, M Asner, DM Baxter, D Behnke, E Bhattacharjee, P Borsodi, H Bou-Cabo, M Brice, SJ Broemmelsiek, D Clark, K Collar, JI Cooper, PS Crisler, M Dahl, CE Daley, S Das, M Debris, F Dhungana, N Fallows, S Farine, J Felis, I Filgas, R Girard, F Giroux, G Grandison, A Hai, M Hall, J Harris, O Jin, M Krauss, CB Lafreniere, M Laurin, M Lawson, I Levine, I Lippincott, WH Mann, E Maurya, D Mitra, P Neilson, R Noble, AJ Plante, A Podviianiuk, RB Priya, S Ramberg, E Robinson, AE Rucinski, R Ruschman, M Scallon, O Seth, S Simon, P Sonnenschein, A Stekl, I Vazquez-Jauregui, E Wells, J Wichoski, U Zacek, V Zhang, J Shkrob, IA AF Amole, C. Ardid, M. Asner, D. M. Baxter, D. Behnke, E. Bhattacharjee, P. Borsodi, H. Bou-Cabo, M. Brice, S. J. Broemmelsiek, D. Clark, K. Collar, J. I. Cooper, P. S. Crisler, M. Dahl, C. E. Daley, S. Das, M. Debris, F. Dhungana, N. Fallows, S. Farine, J. Felis, I. Filgas, R. Girard, F. Giroux, G. Grandison, A. Hai, M. Hall, J. Harris, O. Jin, M. Krauss, C. B. Lafreniere, M. Laurin, M. Lawson, I. Levine, I. Lippincott, W. H. Mann, E. Maurya, D. Mitra, P. Neilson, R. Noble, A. J. Plante, A. Podviianiuk, R. B. Priya, S. Ramberg, E. Robinson, A. E. Rucinski, R. Ruschman, M. Scallon, O. Seth, S. Simon, P. Sonnenschein, A. Stekl, I. Vazquez-Jauregui, E. Wells, J. Wichoski, U. Zacek, V. Zhang, J. Shkrob, I. A. CA PICO Collaboration TI Dark matter search results from the PICO-60 CF3I bubble chamber SO PHYSICAL REVIEW D LA English DT Article ID CANDIDATES; CONSTRAINTS AB New data are reported from the operation of the PICO-60 dark matter detector, a bubble chamber filled with 36.8 kg of CF3I and located in the SNOLAB underground laboratory. PICO-60 is the largest bubble chamber to search for dark matter to date. With an analyzed exposure of 92.8 livedays, PICO-60 exhibits the same excellent background rejection observed in smaller bubble chambers. Alpha decays in PICO-60 exhibit frequency-dependent acoustic calorimetry, similar but not identical to that reported recently in a C3F8 bubble chamber. PICO-60 also observes a large population of unknown background events, exhibiting acoustic, spatial, and timing behaviors inconsistent with those expected from a dark matter signal. These behaviors allow for analysis cuts to remove all background events while retaining 48.2% of the exposure. Stringent limits on weakly interacting massive particles interacting via spin-dependent proton and spin-independent processes are set, and most interpretations of the DAMA/LIBRA modulation signal as dark matter interacting with iodine nuclei are ruled out. C1 [Amole, C.; Daley, S.; Giroux, G.; Noble, A. J.] Queens Univ, Dept Phys, Kingston, ON K7L 3N6, Canada. [Ardid, M.; Bou-Cabo, M.; Felis, I.] Univ Politecn Valencia, IGIC, Gandia 46730, Spain. [Asner, D. M.; Hall, J.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Baxter, D.; Dahl, C. E.; Jin, M.; Zhang, J.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Behnke, E.; Borsodi, H.; Grandison, A.; Harris, O.; Levine, I.; Mann, E.; Wells, J.] Indiana Univ South Bend, Dept Phys & Astron, South Bend, IN 46634 USA. [Bhattacharjee, P.; Das, M.; Seth, S.] Saha Inst Nucl Phys, Astroparticle Phys & Cosmol Div, Kolkata 700064, India. [Brice, S. J.; Broemmelsiek, D.; Cooper, P. S.; Crisler, M.; Dahl, C. E.; Lippincott, W. H.; Ramberg, E.; Rucinski, R.; Ruschman, M.; Simon, P.; Sonnenschein, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Clark, K.] Univ Toronto, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada. [Collar, J. I.; Hai, M.; Neilson, R.; Robinson, A. E.] Univ Chicago, KICP, Enrico Fermi Inst, Chicago, IL 60637 USA. [Collar, J. I.; Hai, M.; Neilson, R.; Robinson, A. E.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Debris, F.; Girard, F.; Lafreniere, M.; Laurin, M.; Plante, A.; Scallon, O.; Zacek, V.] Univ Montreal, Dept Phys, Montreal, PQ H3C 3J7, Canada. [Dhungana, N.; Farine, J.; Girard, F.; Lawson, I.; Podviianiuk, R. B.; Scallon, O.; Vazquez-Jauregui, E.; Wichoski, U.] Laurentian Univ, Dept Phys, Sudbury, ON P3E 2C6, Canada. [Filgas, R.] Czech Tech Univ, Inst Expt & Appl Phys, Prague 12800, Czech Republic. [Fallows, S.; Krauss, C. B.; Mitra, P.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2G7, Canada. [Lawson, I.; Vazquez-Jauregui, E.] SNOLAB, Lively, ON P3Y 1N2, Canada. [Maurya, D.; Priya, S.] Virginia Tech, CEHMS, Blacksburg, VA 24061 USA. [Neilson, R.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Vazquez-Jauregui, E.] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City 01000, DF, Mexico. [Shkrob, I. A.] Argonne Natl Lab, Div Chem, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Harris, O (reprint author), Indiana Univ South Bend, Dept Phys & Astron, South Bend, IN 46634 USA.; Lippincott, WH (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM harriso@iusb.edu; hugh@fnal.gov FU U.S. Department of Energy, Office of Science, Office of High Energy Physics [DE-SC-0012161]; National Science Foundation [PHY-1242637, PHY-0919526, PHY-1205987]; National Sciences and Engineering Research Council of Canada (NSERC); Canada Foundation for Innovation (CFI); Spanish Ministerio de Economia y Competitividad [Consolider MultiDark CSD2009-00064]; Czech Ministry of Education, Youth and Sports [LM2011027]; [De-AC02-07CH11359] FX The PICO Collaboration would like to thank SNOLAB and its staff for providing an exceptional underground laboratory space and invaluable technical support. We acknowledge technical assistance from Fermilab's Computing, Particle Physics, and Accelerator Divisions and from A. Behnke at IUSB. We thank V. Gluscevic and S. McDermott for useful conversations and their assistance with the DMDD code package. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of High Energy Physics under Award No. DE-SC-0012161. Fermi National Accelerator Laboratory is operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359. Part of the research described in this paper was conducted under the Ultra Sensitive Nuclear Measurements Initiative at Pacific Northwest National Laboratory, a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy. We acknowledge the National Science Foundation for their support including Grants No. PHY-1242637, No. PHY-0919526, and No. PHY-1205987. We acknowledge the support of the National Sciences and Engineering Research Council of Canada (NSERC) and the Canada Foundation for Innovation (CFI). We thank the Kavli Institute for Cosmological Physics at the University of Chicago. We were also supported by the Spanish Ministerio de Economia y Competitividad, Consolider MultiDark CSD2009-00064 Grant. We thank the Department of Atomic Energy (DAE), Government of India, under the project CAPP-II at SINP, Kolkata. We acknowledge the Czech Ministry of Education, Youth and Sports, Grant No. LM2011027. NR 68 TC 25 Z9 25 U1 2 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 28 PY 2016 VL 93 IS 5 AR 052014 DI 10.1103/PhysRevD.93.052014 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH5BS UT WOS:000372800700002 ER PT J AU Lees, JP Poireau, V Tisserand, V Grauges, E Palano, A Eigen, G Stugu, B Brown, DN Kerth, LT Kolomensky, YG Lee, MJ Lynch, G Koch, H Schroeder, T Hearty, C Mattison, TS McKenna, JA So, RY Khan, A Blinov, VE Buzykaev, AR Druzhinin, VP Golubev, VB Kravchenko, EA Onuchin, AP Serednyako, SI Skovpen, YI Solodov, EP Todyshev, KY Lankford, AJ Dey, B Gary, JW Long, O Sevilla, MF Hong, TM Kovalskyi, D Richman, JD West, CA Eisner, AM Lockman, WS Vazquez, WP Schumm, BA Seiden, A Chao, DS Cheng, CH Echenard, B Flood, KT Hitlin, DG Miyashita, TS Ongmongkolkul, P Porter, FC Rohrken, M Andreassen, R Huard, Z Meadows, BT Pushpawela, BG Sokoloff, MD Sun, L Bloom, PC Ford, WT Gaz, A Smith, JG Wagner, SR Ayad, R Toki, WH Spaan, B Bernard, D Verderi, M Playfer, S Bettoni, D Bozzi, C Calabrese, R Cibinetto, G Fioravanti, E Garzia, I Luppi, E Piemontese, L Santoro, V Calcaterra, A de Sangro, R Finocchiaro, G Martellotti, S Patteri, P Peruzzi, IM Piccolo, M Zallo, A Contri, R Monge, MR Passaggio, S Patrignani, C Bhuyan, B Prasad, V Adametz, A Uwer, U Lacker, HM Mallik, U Chen, C Cochran, J Prell, S Ahmed, H Gritsan, AV Arnaud, N Davier, M Derkach, D Grosdidier, G Le Diberder, F Lutz, AM Malaescu, B Roudeau, P Stocchi, A Wormser, G Lange, DJ Wright, DM Coleman, JP Fry, JR Gabathuler, E Hutchcroft, DE Payne, DJ Touramanis, C Bevan, AJ Di Lodovico, F Sacco, R Cowan, G Brown, DN Davis, CL Denig, AG Fritsch, M Gradl, W Griessinger, K Hafner, A Schubert, KR Barlow, RJ Lafferty, GD Cenci, R Hamilton, B Jawahery, A Roberts, DA Cowan, R Cheaib, R Patel, PM Robertson, SH Neri, N Palombo, F Cremaldi, L Godang, R Summers, DJ Simard, M Taras, P De Nardo, G Onorato, G Sciacca, C Raven, G Jessop, CP LoSecco, JM Honscheid, K Kass, R Margoni, M Morandin, M Posocco, M Rotondo, M Simi, G Simonetto, F Stroili, R Akar, S Ben-Haim, E Bomben, M Bonneaud, GR Briand, H Calderini, G Chauveau, J Leruste, P Marchiori, G Ocariz, J Biasini, M Manoni, E Rossi, A Angelini, C Batignani, G Bettarini, S Carpinelli, M Casarosa, G Chrzaszcz, M Forti, F Giorgi, MA Lusiani, A Oberhof, B Paoloni, E Rama, M Rizzo, G Walsh, JJ Pegna, DL Olsen, J Smith, AJS Anulli, F Faccini, R Ferrarotto, F Ferroni, F Gaspero, M Pilloni, A Piredda, G Bunger, C Dittrich, S Grunberg, O Hess, M Leddig, T Voss, C Waldi, R Adye, T Olaiya, EO Wilson, FF Emery, S Vasseur, G Aston, D Bard, DJ Cartaro, C Convery, MR Dorfan, J Dubois-Felsmann, GP Dunwoodie, W Ebert, M Field, RC Fulsom, BG Graham, MT Hast, C Innes, WR Kim, P Leith, DWGS Luitz, S Luth, V MacFarlane, DB Muller, DR Neal, H Pulliam, T Ratcliff, BN Roodman, A Schindler, RH Snyder, A Su, D Sullivan, MK Va'vra, J Wisniewski, WJ Wulsin, HW Purohit, MV Wilson, JR Randle-Conde, A Sekula, SJ Bellis, M Burchat, PR Puccio, EMT Alam, MS Ernst, JA Gorodeisky, R Guttman, N Peimer, DR Soffer, A Spanier, SM Ritchie, JL Schwitters, RF Izen, JM Lou, XC Bianchi, F De Mori, F Filippi, A Gamba, D Lanceri, L Vitale, L Martinez-Vidal, F Oyanguren, A Albert, J Banerjee, S Beaulieu, A Bernlochner, FU Choi, HHF King, GJ Kowalewski, R Lewczuk, MJ Lueck, T Nugent, IM Roney, JM Sobie, RJ Tasneem, N Gershon, TJ Harrison, PF Latham, TE Band, HR Dasu, S Pan, Y Prepost, R Wu, SL AF Lees, J. P. Poireau, V. Tisserand, V. Grauges, E. Palano, A. Eigen, G. Stugu, B. Brown, D. N. Kerth, L. T. Kolomensky, Yu. G. Lee, M. J. Lynch, G. Koch, H. Schroeder, T. Hearty, C. Mattison, T. S. McKenna, J. A. So, R. Y. Khan, A. Blinov, V. E. Buzykaev, A. R. Druzhinin, V. P. Golubev, V. B. Kravchenko, E. A. Onuchin, A. P. Serednyako, S. I. Skovpen, Yu. I. Solodov, E. P. Todyshev, K. Yu. Lankford, A. J. Dey, B. Gary, J. W. Long, O. Sevilla, M. Franco Hong, T. M. Kovalskyi, D. Richman, J. D. West, C. A. Eisner, A. M. Lockman, W. S. Vazquez, W. Panduro Schumm, B. A. Seiden, A. Chao, D. S. Cheng, C. H. Echenard, B. Flood, K. T. Hitlin, D. G. Miyashita, T. S. Ongmongkolkul, P. Porter, F. C. Roehrken, M. Andreassen, R. Huard, Z. Meadows, B. T. Pushpawela, B. G. Sokoloff, M. D. Sun, L. Bloom, P. C. Ford, W. T. Gaz, A. Smith, J. G. Wagner, S. R. Ayad, R. Toki, W. H. Spaan, B. Bernard, D. Verderi, M. Playfer, S. Bettoni, D. Bozzi, C. Calabrese, R. Cibinetto, G. Fioravanti, E. Garzia, I. Luppi, E. Piemontese, L. Santoro, V. Calcaterra, A. de Sangro, R. Finocchiaro, G. Martellotti, S. Patteri, P. Peruzzi, I. M. Piccolo, M. Zallo, A. Contri, R. Monge, M. R. Passaggio, S. Patrignani, C. Bhuyan, B. Prasad, V. Adametz, A. Uwer, U. Lacker, H. M. Mallik, U. Chen, C. Cochran, J. Prell, S. Ahmed, H. Gritsan, A. V. Arnaud, N. Davier, M. Derkach, D. Grosdidier, G. Le Diberder, F. Lutz, A. M. Malaescu, B. Roudeau, P. Stocchi, A. Wormser, G. Lange, D. J. Wright, D. M. Coleman, J. P. Fry, J. R. Gabathuler, E. Hutchcroft, D. E. Payne, D. J. Touramanis, C. Bevan, A. J. Di Lodovico, F. Sacco, R. Cowan, G. Brown, D. N. Davis, C. L. Denig, A. G. Fritsch, M. Gradl, W. Griessinger, K. Hafner, A. Schubert, K. R. Barlow, R. J. Lafferty, G. D. Cenci, R. Hamilton, B. Jawahery, A. Roberts, D. A. Cowan, R. Cheaib, R. Patel, P. M. Robertson, S. H. Neri, N. Palombo, F. Cremaldi, L. Godang, R. Summers, D. J. Simard, M. Taras, P. De Nardo, G. Onorato, G. Sciacca, C. Raven, G. Jessop, C. P. LoSecco, J. M. Honscheid, K. Kass, R. Margoni, M. Morandin, M. Posocco, M. Rotondo, M. Simi, G. Simonetto, F. Stroili, R. Akar, S. Ben-Haim, E. Bomben, M. Bonneaud, G. R. Briand, H. Calderini, G. Chauveau, J. Leruste, Ph. Marchiori, G. Ocariz, J. Biasini, M. Manoni, E. Rossi, A. Angelini, C. Batignani, G. Bettarini, S. Carpinelli, M. Casarosa, G. Chrzaszcz, M. Forti, F. Giorgi, M. A. Lusiani, A. Oberhof, B. Paoloni, E. Rama, M. Rizzo, G. Walsh, J. J. Pegna, D. Lopes Olsen, J. Smith, A. J. S. Anulli, F. Faccini, R. Ferrarotto, F. Ferroni, F. Gaspero, M. Pilloni, A. Piredda, G. Bunger, C. Dittrich, S. Gruenberg, O. Hess, M. Leddig, T. Voss, C. Waldi, R. Adye, T. Olaiya, E. O. Wilson, F. F. Emery, S. Vasseur, G. Aston, D. Bard, D. J. Cartaro, C. Convery, M. R. Dorfan, J. Dubois-Felsmann, G. P. Dunwoodie, W. Ebert, M. Field, R. C. Fulsom, B. G. Graham, M. T. Hast, C. Innes, W. R. Kim, P. Leith, D. W. G. S. Luitz, S. Luth, V. MacFarlane, D. B. Muller, D. R. Neal, H. Pulliam, T. Ratcliff, B. N. Roodman, A. Schindler, R. H. Snyder, A. Su, D. Sullivan, M. K. Va'vra, J. Wisniewski, W. J. Wulsin, H. W. Purohit, M. V. Wilson, J. R. Randle-Conde, A. Sekula, S. J. Bellis, M. Burchat, P. R. Puccio, E. M. T. Alam, M. S. Ernst, J. A. Gorodeisky, R. Guttman, N. Peimer, D. R. Soffer, A. Spanier, S. M. Ritchie, J. L. Schwitters, R. F. Izen, J. M. Lou, X. C. Bianchi, F. De Mori, F. Filippi, A. Gamba, D. Lanceri, L. Vitale, L. Martinez-Vidal, F. Oyanguren, A. Albert, J. Banerjee, Sw. Beaulieu, A. Bernlochner, F. U. Choi, H. H. F. King, G. J. Kowalewski, R. Lewczuk, M. J. Lueck, T. Nugent, I. M. Roney, J. M. Sobie, R. J. Tasneem, N. Gershon, T. J. Harrison, P. F. Latham, T. E. Band, H. R. Dasu, S. Pan, Y. Prepost, R. Wu, S. L. CA BABAR Collaboration TI Measurement of angular asymmetries in the decays B -> K*l(+) l(+) SO PHYSICAL REVIEW D LA English DT Article ID SEMILEPTONIC RARE DECAYS; BABAR DETECTOR AB We study the lepton forward-backward asymmetry AFB and the longitudinal K* polarization F-L, as well as an observable P-2 derived from them, in the rare decays B -> K*l(+)l(-), where l(+)l(-) is either e(+)e(-) or mu(+)mu(-), using the full sample of 471 million B (B) over bar events collected at the Upsilon(4S) resonance with the BABAR, detector at the PEP-II e(+)e(-) collider. We separately fit and report results for the K*(0)(892)l(+)l(-) and K*(+)(892) l(+)l(-) final states, as well as their combination K*l(+)l(-), in five disjoint dilepton mass-squared bins. An angular analysis of B+ -> K*(+)l(+)l(-) decays is presented here for the first time. C1 [Lees, J. 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P.; Golubev, V. B.; Kravchenko, E. A.; Onuchin, A. P.; Serednyako, S. I.; Skovpen, Yu. I.; Solodov, E. P.; Todyshev, K. Yu.] RAS, SB, Budker Inst Nucl Phys, Novosibirsk 630090, Russia. [Blinov, V. E.; Druzhinin, V. P.; Golubev, V. B.; Kravchenko, E. A.; Onuchin, A. P.; Serednyako, S. I.; Skovpen, Yu. I.; Solodov, E. P.; Todyshev, K. Yu.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Blinov, V. E.; Onuchin, A. P.] Novosibirsk State Tech Univ, Novosibirsk 630092, Russia. [Lankford, A. J.] Univ Calif Irvine, Irvine, CA 92697 USA. [Dey, B.; Gary, J. W.; Long, O.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sevilla, M. Franco; Hong, T. M.; Kovalskyi, D.; Richman, J. D.; West, C. A.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Eisner, A. M.; Lockman, W. S.; Vazquez, W. Panduro; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Inst Particle Phys, Santa Cruz, CA 95064 USA. [Chao, D. S.; Cheng, C. H.; Echenard, B.; Flood, K. T.; Hitlin, D. G.; Miyashita, T. 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M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Honscheid, K.; Kass, R.] Ohio State Univ, Columbus, OH 43210 USA. [Margoni, M.; Morandin, M.; Posocco, M.; Rotondo, M.; Simi, G.; Simonetto, F.; Stroili, R.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Margoni, M.; Simi, G.; Simonetto, F.; Stroili, R.] Univ Padua, Dipartimento Fis, I-35131 Padua, Italy. [Akar, S.; Ben-Haim, E.; Bomben, M.; Bonneaud, G. R.; Briand, H.; Calderini, G.; Chauveau, J.; Leruste, Ph.; Marchiori, G.; Ocariz, J.] Univ Paris 07, Univ Paris 06, CNRS IN2P3, Lab Phys Nucl & Hautes Energies, F-75252 Paris, France. [Biasini, M.; Manoni, E.; Rossi, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06123 Perugia, Italy. [Biasini, M.] Univ Perugia, Dipartimento Fis, I-06123 Perugia, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Chrzaszcz, M.; Forti, F.; Giorgi, M. A.; Lusiani, A.; Oberhof, B.; Paoloni, E.; Rama, M.; Rizzo, G.; Walsh, J. J.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Angelini, C.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Forti, F.; Giorgi, M. A.; Lusiani, A.; Oberhof, B.; Paoloni, E.; Rizzo, G.] Univ Pisa, Dipartimento Fis, I-56127 Pisa, Italy. Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Pegna, D. Lopes; Olsen, J.; Smith, A. J. S.] Princeton Univ, Princeton, NJ 08544 USA. [Anulli, F.; Faccini, R.; Ferrarotto, F.; Ferroni, F.; Gaspero, M.; Pilloni, A.; Piredda, G.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Faccini, R.; Ferroni, F.; Gaspero, M.; Pilloni, A.] Univ Roma La Sapienza, Dipartimento Fis, I-00185 Rome, Italy. [Bunger, C.; Dittrich, S.; Gruenberg, O.; Hess, M.; Leddig, T.; Voss, C.; Waldi, R.] Univ Rostock, D-18051 Rostock, Germany. [Adye, T.; Olaiya, E. O.; Wilson, F. F.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Emery, S.; Vasseur, G.] CEA, Irfu, SPP, Ctr Saclay, F-91191 Gif Sur Yvette, France. [Aston, D.; Bard, D. J.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dubois-Felsmann, G. P.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Leith, D. W. G. S.; Luitz, S.; Luth, V.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Pulliam, T.; Ratcliff, B. N.; Roodman, A.; Schindler, R. H.; Snyder, A.; Su, D.; Sullivan, M. K.; Va'vra, J.; Wisniewski, W. J.; Wulsin, H. W.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Purohit, M. V.; Wilson, J. R.] Univ S Carolina, Columbia, SC 29208 USA. [Randle-Conde, A.; Sekula, S. J.] So Methodist Univ, Dallas, TX 75275 USA. [Bellis, M.; Burchat, P. R.; Puccio, E. M. T.] Stanford Univ, Stanford, CA 94305 USA. [Alam, M. S.; Ernst, J. A.] SUNY Albany, Albany, NY 12222 USA. [Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Spanier, S. M.] Univ Tennessee, Knoxville, TN 37996 USA. [Ritchie, J. L.; Schwitters, R. F.] Univ Texas Austin, Austin, TX 78712 USA. [Izen, J. M.; Lou, X. C.] Univ Texas Dallas, Richardson, TX 75083 USA. [Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Bianchi, F.; De Mori, F.; Gamba, D.] Univ Turin, Dipartimento Fis, I-10125 Turin, Italy. [Lanceri, L.; Vitale, L.] Ist Nazl Fis Nucl, Sez Trieste, I-34127 Trieste, Italy. [Lanceri, L.; Vitale, L.] Univ Trieste, Dipartimento Fis, I-34127 Trieste, Italy. [Martinez-Vidal, F.; Oyanguren, A.] Univ Valencia, CSIC, IFIC, E-46071 Valencia, Spain. [Albert, J.; Banerjee, Sw.; Beaulieu, A.; Bernlochner, F. U.; Choi, H. H. F.; King, G. J.; Kowalewski, R.; Lewczuk, M. J.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Sobie, R. J.; Tasneem, N.] Univ Victoria, Victoria, BC V8W 3P6, Canada. [Gershon, T. J.; Harrison, P. F.; Latham, T. E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Band, H. R.; Dasu, S.; Pan, Y.; Prepost, R.; Wu, S. L.] Univ Wisconsin, Madison, WI 53706 USA. [Ayad, R.] Univ Tabuk, Tabuk 71491, Saudi Arabia. [Malaescu, B.] IN2P3 CNRS, Lab Phys Nucl & Hautes Energies, F-75252 Paris, France. [Barlow, R. J.] Univ Huddersfield, Huddersfield HD1 3DH, W Yorkshire, England. [Godang, R.] Univ S Alabama, Mobile, AL 36688 USA. [Carpinelli, M.] Univ Sassari, I-07100 Sassari, Italy. RP Lees, JP (reprint author), Univ Savoie, CNRS IN2P3, Lab Annecy le Vieux Phys Particules LAPP, F-74941 Annecy Le Vieux, France. RI Kravchenko, Evgeniy/F-5457-2015; Di Lodovico, Francesca/L-9109-2016; Calcaterra, Alessandro/P-5260-2015; Patrignani, Claudia/C-5223-2009 OI Di Lodovico, Francesca/0000-0003-3952-2175; Calcaterra, Alessandro/0000-0003-2670-4826; Patrignani, Claudia/0000-0002-5882-1747 FU U.S. Department of Energy (Canada); National Science Foundation (Canada); Natural Sciences and Engineering Research Council (Canada); Commissariat a l'Energie Atomique (France); Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung (Germany); Deutsche Forschungsgemeinschaft (Germany); Istituto Nazionale di Fisica Nucleare (Italy); Foundation for Fundamental Research on Matter (The Netherlands); Research Council of Norway (Spain); Ministry of Education and Science of the Russian Federation; Ministerio de Economia y Competitividad (Spain); Science and Technology Facilities Council (United Kingdom); Binational Science Foundation (U.S.-Israel); Marie-Curie IEF program (European Union); A. P. Sloan Foundation (USA) FX We would like to express our gratitude to Joaquim Matias for discussions regarding the observable P2. We are grateful for the extraordinary contributions of our PEP-II colleagues in achieving the excellent luminosity and machine conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the computing organizations that support BABAR. The collaborating institutions wish to thank SLAC for its support and the kind hospitality extended to them. This work is supported by the U.S. Department of Energy and the National Science Foundation, the Natural Sciences and Engineering Research Council (Canada), the Commissariat a l'Energie Atomique and Institut National de Physique Nucleaire et de Physique des Particules (France), the Bundesministerium fur Bildung und Forschung and Deutsche Forschungsgemeinschaft (Germany), the Istituto Nazionale di Fisica Nucleare (Italy), the Foundation for Fundamental Research on Matter (The Netherlands), the Research Council of Norway, the Ministry of Education and Science of the Russian Federation, Ministerio de Economia y Competitividad (Spain), the Science and Technology Facilities Council (United Kingdom), and the Binational Science Foundation (U.S.-Israel). Individuals have received support from the Marie-Curie IEF program (European Union) and the A. P. Sloan Foundation (USA). NR 54 TC 2 Z9 2 U1 3 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 28 PY 2016 VL 93 IS 5 AR 052015 DI 10.1103/PhysRevD.93.052015 PG 16 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH5BS UT WOS:000372800700003 ER PT J AU Manzotti, A Dodelson, S Park, Y AF Manzotti, Alessandro Dodelson, Scott Park, Youngsoo TI External priors for the next generation of CMB experiments SO PHYSICAL REVIEW D LA English DT Article ID BARYON ACOUSTIC-OSCILLATIONS; LARGE-SCALE STRUCTURE; SOUTH-POLE TELESCOPE; POWER SPECTRUM; COSMOLOGICAL PARAMETERS; MICROWAVE; CONSTRAINTS; MISSION AB Planned cosmic microwave background (CMB) experiments will improve what we know about neutrino physics, inflation, and dark energy. The low level of noise, together with improved angular resolution, will increase the signal-to-noise ratio of the CMB polarized data as well as the reconstructed lensing potential of large scale structure. Projected constraints on cosmological parameters are tight, but these can be improved even further with information from external experiments. Here, we examine quantitatively the extent to which external priors can lead to improvement in projected constraints from a CMB-Stage IV (S4) experiment on neutrino and dark energy properties. We find that CMB S4 constraints on neutrino mass could be strongly enhanced by external constraints on the cold dark matter density Omega(c)h(2) and the Hubble constant H-0. If polarization on the largest scales (l < 50) will not be measured, an external prior on the primordial amplitude A(s) or the optical depth tau will also be important. A CMB constraint on the number of relativistic degrees of freedom, N-eff, will benefit from an external prior on the spectral index n(s) and the baryon energy density Omega(b)h(2). Finally, an external prior on H-0 will help constrain the dark energy equation of state (w). C1 [Manzotti, Alessandro; Dodelson, Scott] Univ Chicago, Dept Astron & Astrophys, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Manzotti, Alessandro; Dodelson, Scott] Univ Chicago, Enrico Fermi Inst, Kavli Inst Cosmol Phys, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Dodelson, Scott] Fermilab Natl Accelerator Lab, Fermilab Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. [Park, Youngsoo] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. RP Manzotti, A (reprint author), Univ Chicago, Dept Astron & Astrophys, 5640 S Ellis Ave, Chicago, IL 60637 USA.; Manzotti, A (reprint author), Univ Chicago, Enrico Fermi Inst, Kavli Inst Cosmol Phys, 5640 S Ellis Ave, Chicago, IL 60637 USA. EM manzotti.alessandro@gmail.com FU Kavli Institute for Cosmological Physics at the University of Chicago [NSF PHY-1125897]; U.S. Department of Energy [DE-FG02-95ER40896] FX We thank Wayne Hu for useful discussions. A. M. wants to thank Zhen Pan who allowed a careful cross-check of our results. This work was partially supported by the Kavli Institute for Cosmological Physics at the University of Chicago through Grant No. NSF PHY-1125897 and an endowment from the Kavli Foundation and its founder Fred Kavli. The work of S. D. is supported by the U.S. Department of Energy, including Grant No. DE-FG02-95ER40896. NR 35 TC 2 Z9 2 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 28 PY 2016 VL 93 IS 6 AR 063009 DI 10.1103/PhysRevD.93.063009 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH5BZ UT WOS:000372801500002 ER PT J AU Bouchard, KE Conant, DF Anumanchipalli, GK Dichter, B Chaisanguanthum, KS Johnson, K Chang, EF AF Bouchard, Kristofer E. Conant, David F. Anumanchipalli, Gopala K. Dichter, Benjamin Chaisanguanthum, Kris S. Johnson, Keith Chang, Edward F. TI High-Resolution, Non-Invasive Imaging of Upper Vocal Tract Articulators Compatible with Human Brain Recordings SO PLOS ONE LA English DT Article ID NONNEGATIVE MATRIX FACTORIZATION; OROFACIAL SENSORIMOTOR CORTEX; MOVEMENTS; VOWELS; LIP; VARIABILITY; CONSONANTS; ACOUSTICS; ALGORITHM; DYNAMICS AB A complete neurobiological understanding of speech motor control requires determination of the relationship between simultaneously recorded neural activity and the kinematics of the lips, jaw, tongue, and larynx. Many speech articulators are internal to the vocal tract, and therefore simultaneously tracking the kinematics of all articulators is nontrivial-especially in the context of human electrophysiology recordings. Here, we describe a noninvasive, multi-modal imaging system to monitor vocal tract kinematics, demonstrate this system in six speakers during production of nine American English vowels, and provide new analysis of such data. Classification and regression analysis revealed considerable variability in the articulator-to-acoustic relationship across speakers. Non-negative matrix factorization extracted basis sets capturing vocal tract shapes allowing for higher vowel classification accuracy than traditional methods. Statistical speech synthesis generated speech from vocal tract measurements, and we demonstrate perceptual identification. We demonstrate the capacity to predict lip kinematics from ventral sensorimotor cortical activity. These results demonstrate a multi-modal system to non-invasively monitor articulator kinematics during speech production, describe novel analytic methods for relating kinematic data to speech acoustics, and provide the first decoding of speech kinematics from electrocorticography. These advances will be critical for understanding the cortical basis of speech production and the creation of vocal prosthetics. C1 [Bouchard, Kristofer E.] Lawrence Berkeley Natl Labs, Biol Syst & Engn Div, Berkeley, CA USA. [Bouchard, Kristofer E.] Lawrence Berkeley Natl Labs, Computat Res Div, Berkeley, CA USA. [Bouchard, Kristofer E.; Conant, David F.; Anumanchipalli, Gopala K.; Dichter, Benjamin; Chaisanguanthum, Kris S.; Chang, Edward F.] Univ Calif San Francisco, Dept Neurol Surg, San Francisco, CA USA. [Conant, David F.; Anumanchipalli, Gopala K.; Dichter, Benjamin; Chaisanguanthum, Kris S.; Chang, Edward F.] UCSF, Ctr Integrat Neurosci, San Francisco, CA USA. [Johnson, Keith] Univ Calif Berkeley, Dept Linguist, Berkeley, CA 94720 USA. RP Chang, EF (reprint author), Univ Calif San Francisco, Dept Neurol Surg, San Francisco, CA USA.; Chang, EF (reprint author), UCSF, Ctr Integrat Neurosci, San Francisco, CA USA. EM changed@neurosurg.ucsf.edu FU National Institutes of Health [DP2-OD00862, R01-DC012379]; DARPA SUBNETS; Bowes Foundation; Curci Foundation; McKnight Foundation; New York Stem Cell Foundation; Laboratory Directed Research and Development (LDRD) from Berkeley Lab; U.S. Department of Energy [DE-AC02-05CH11231] FX E.F.C. was supported by National Institutes of Health grants DP2-OD00862 and R01-DC012379, DARPA SUBNETS, Bowes Foundation, Curci Foundation, and McKnight Foundation. Edward Chang is a New York Stem Cell Foundation-Robertson Investigator. This research was supported by The New York Stem Cell Foundation. KEB was supported by a Laboratory Directed Research and Development (LDRD) funding from Berkeley Lab, provided by the Director, Office of Science, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The author(s) received no specific funding for this work. NR 61 TC 1 Z9 1 U1 1 U2 3 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 28 PY 2016 VL 11 IS 3 AR e0151327 DI 10.1371/journal.pone.0151327 PG 30 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH5EH UT WOS:000372807800010 PM 27019106 ER PT J AU McLaughlin, BM Ballance, CP Schippers, S Hellhund, J Kilcoyne, ALD Phaneuf, RA Muller, A AF McLaughlin, B. M. Ballance, C. P. Schippers, S. Hellhund, J. Kilcoyne, A. L. D. Phaneuf, R. A. Mueller, A. TI Photoionization of tungsten ions: experiment and theory for W2+ and W3+ SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE photoionization cross sections; tungsten ions; large scale ID R-MATRIX METHOD; ELECTRON-SCATTERING; CROSS-SECTION; IONIZATION; EXCITATION AB Experimental and theoretical results are reported for single-photon single ionization of W2+ and W3+ tungsten ions. Experiments were performed at the photon-ion merged-beam setup of the Advanced Light Source in Berkeley. Absolute cross sections and detailed energy scans were measured over an energy range 20-90 eV at a bandwidth of 100 meV. Broad peak features with widths typically around 5 eV have been observed with almost no narrow resonances present in the investigated energy range. Theoretical results were obtained from a Dirac-Coulomb R-matrix approach. The calculations were carried out for the lowest-energy terms of the investigated tungsten ions with levels 5s(2)5p(6)5d(4) D-5(J) = 0, 1, 2, 3, 4 for W2+ and 5s(2)5p(6)5d(3) F-4(J') J' = 3 2, 5 2, 7 2, 9 2 for W3+. Assuming a statistically weighted distribution of ions in the initial ground-term levels there is good agreement of theory and experiment for W3+ ions. However, for W2+ ions at higher energies there is a factor of approximately two difference between experimental and theoretical cross sections. C1 [McLaughlin, B. M.; Ballance, C. P.] Queens Univ Belfast, CTAMOP, Sch Math & Phys, David Bates Bldg,7 Coll Pk, Belfast BT7 1NN, Antrim, North Ireland. [McLaughlin, B. M.] Harvard Smithsonian Ctr Astrophys, Inst Theoret Atom & Mol Phys, MS-14, Cambridge, MA 02138 USA. [Schippers, S.; Hellhund, J.; Mueller, A.] Univ Giessen, Inst Atom & Mol Phys, D-35392 Giessen, Germany. [Schippers, S.] Univ Giessen, Inst Phys 1, D-35392 Giessen, Germany. [Kilcoyne, A. L. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Hellhund, J.; Phaneuf, R. A.] Univ Nevada, Dept Phys, Reno, NV 89557 USA. RP McLaughlin, BM (reprint author), Queens Univ Belfast, CTAMOP, Sch Math & Phys, David Bates Bldg,7 Coll Pk, Belfast BT7 1NN, Antrim, North Ireland.; McLaughlin, BM (reprint author), Harvard Smithsonian Ctr Astrophys, Inst Theoret Atom & Mol Phys, MS-14, Cambridge, MA 02138 USA.; Muller, A (reprint author), Univ Giessen, Inst Atom & Mol Phys, D-35392 Giessen, Germany. EM bmclaughlin899@btinternet.com; Alfred.Mueller@iamp.physik.uni-giessen.de RI Muller, Alfred/A-3548-2009; Kilcoyne, David/I-1465-2013; Schippers, Stefan/A-7786-2008 OI Muller, Alfred/0000-0002-0030-6929; Schippers, Stefan/0000-0002-6166-7138 FU Deutsche Forschungsgemeinschaft (DFG) [Mu 1068/20]; NASA; NSF grants through Auburn University; US National Science Foundation; Office of Science of the US Department of Energy [DE-AC05-00OR22725]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX The Giessen group acknowledges support by Deutsche Forschungsgemeinschaft (DFG) under project number Mu 1068/20. C P Ballance was supported by NASA and NSF grants through Auburn University. B M McLaughlin acknowledges support by the US National Science Foundation through a grant to ITAMP at the Harvard-Smithsonian Center for Astrophysics, under the visitors program, Queen's University Belfast for the award of a visiting research fellowship (VRF). The computational work was carried out at the National Energy Research Scientific Computing Center in Oakland, CA, USA and at the High Performance Computing Center Stuttgart (HLRS) of the University of Stuttgart, Stuttgart, Germany. This research also used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC05-00OR22725. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 41 TC 1 Z9 1 U1 4 U2 10 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD MAR 28 PY 2016 VL 49 IS 6 AR 065201 DI 10.1088/0953-4075/49/6/065201 PG 9 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DG0UW UT WOS:000371782200028 ER PT J AU Chen, YY Sanchez, C Yue, Y de Almeida, M Gonzalez, JM Parkinson, DY Liang, H AF Chen, Yunyun Sanchez, Carlos Yue, Yuan de Almeida, Mauricio Gonzalez, Jorge M. Parkinson, Dilworth Y. Liang, Hong TI Observation of yttrium oxide nanoparticles in cabbage (Brassica oleracea) through dual energy K-edge subtraction imaging SO JOURNAL OF NANOBIOTECHNOLOGY LA English DT Article DE Synchrotron X-ray micro-tomography; K-edge subtraction imaging; Yttria nanoparticles; Cabbage; Accumulation ID QUANTUM-DOT NANOPARTICLES; SILVER NANOPARTICLES; CERIUM OXIDE; FOOD-CHAIN; PLANTS; ACCUMULATION; TRANSLOCATION; NANOMATERIALS; ARABIDOPSIS; NANOTUBES AB Background: The potential transfer of engineered nanoparticles (ENPs) from plants into the food chain has raised widespread concerns. In order to investigate the effects of ENPs on plants, young cabbage plants (Brassica oleracea) were exposed to a hydroponic system containing yttrium oxide (yttria) ENPs. The objective of this study was to reveal the impacts of NPs on plants by using K-edge subtraction imaging technique. Results: Using synchrotron dual-energy X-ray micro-tomography with K-edge subtraction technique, we studied the uptake, accumulation, distribution and concentration mapping of yttria ENPs in cabbage plants. It was found that yttria ENPs were uptaken by the cabbage roots but did not effectively transferred and mobilized through the cabbage stem and leaves. This could be due to the accumulation of yttria ENPs blocked at primary-lateral-root junction. Instead, non-yttria minerals were found in the xylem vessels of roots and stem. Conclusions: Synchrotron dual-energy X-ray micro-tomography is an effective method to observe yttria NPs inside the cabbage plants in both whole body and microscale level. Furthermore, the blockage of a plant's roots by nanoparticles is likely the first and potentially fatal environmental effect of such type of nanoparticles. C1 [Chen, Yunyun; Yue, Yuan; Liang, Hong] Texas A&M Univ, Mat Sci & Engn, College Stn, TX 77843 USA. [Sanchez, Carlos; Liang, Hong] Texas A&M Univ, Mech Engn, College Stn, TX 77843 USA. [de Almeida, Mauricio; Gonzalez, Jorge M.] Calif State Univ Fresno, Dept Plant Sci, Fresno, CA 93740 USA. [Parkinson, Dilworth Y.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Liang, H (reprint author), Texas A&M Univ, Mat Sci & Engn, College Stn, TX 77843 USA. EM hliang@tamu.edu RI Yue, Yuan/F-2177-2017 FU ALS fellowship; Provost's Assigned Time for Research; California State University Fresno, Research, Scholarship and Creative proposal Award; CSUF Provost's undergraduate Research Grant; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX YYC was partially sponsored by the ALS fellowship. JMG and MA were supported by the Provost's Assigned Time for Research (Summer 2015), California State University Fresno, Research, Scholarship and Creative proposal Awarded (2014-2015) and the CSUF Provost's undergraduate Research Grant (2014-2015). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 38 TC 5 Z9 5 U1 5 U2 16 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1477-3155 J9 J NANOBIOTECHNOL JI J. Nanobiotechnol. PD MAR 25 PY 2016 VL 14 AR 23 DI 10.1186/s12951-016-0175-z PG 10 WC Biotechnology & Applied Microbiology; Nanoscience & Nanotechnology SC Biotechnology & Applied Microbiology; Science & Technology - Other Topics GA DI1QH UT WOS:000373270100001 PM 27015946 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahn, SU Aimo, I Aiola, S Ajaz, M Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Almaraz, JRM Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Armesto, N Arnaldi, R Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Bach, M Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Baldisseri, A Pedrosa, FBD Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F Martinez, HB Bellwied, R Belmont, R Belmont-Moreno, E Belyaev, V Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bertens, RA Berzano, D Betev, L Bhasin, A Bhat, IR Bhati, AK Bhattacharjee, B Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Biswas, R Biswas, S Bjelogrlic, S Blair, JT Blanco, F Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Borri, M Bossu, F Botta, E Bottger, S Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brucken, EJ Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Butt, JB Buxton, JT Caffarri, D Cai, X Caines, H Diaz, LC Caliva, A Villar, EC Camerini, P Carena, F Carena, W Carnesecchi, F Castellanos, JC Castro, AJ Casula, EAR Cavicchioli, C Sanchez, CC Cepila, J Cerello, P Cerkala, J Chang, B Chapeland, S Chartier, M Charvet, JL Chattopadhyay, S Chattopadhyay, S Chelnokov, V Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Chochula, P Choi, K Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Chunhui, Z Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Colocci, M Balbastre, GC del Valle, ZC Connors, ME Contreras, JG Cormier, TM Morales, YC Maldonado, IC Cortese, P Cosentino, MR Costa, F Crochet, P Albino, RC Cuautle, E Cunqueiro, L Dahms, T Dainese, A Danu, A Das, D Das, I Das, S Dash, A Dash, S De, S De Caro, A de Cataldo, G de Cuveland, J De Falco, A De Gruttola, D De Marco, N De Pasquale, S Deisting, A Deloff, A Denes, E D'Erasmo, G Di Bari, D Di Mauro, A Di Nezza, P Corchero, MAD Dietel, T Dillenseger, P Divia, R Djuvsland, O Dobrin, A Dobrowolski, T Gimenez, DD Donigus, B Dordic, O Drozhzhova, T Dubey, AK Dubla, A Ducroux, L Dupieux, P Ehlers, RJ Elia, D Engel, H Erazmus, B Erdemir, I Erhardt, F Eschweiler, D Espagnon, B Estienne, M Esumi, S Eum, J Evans, D Evdokimov, S Eyyubova, G Fabbietti, L Fabris, D Faivre, J Fantoni, A Fasel, M Feldkamp, L Felea, D Feliciello, A Feofilov, G Ferencei, J Tellez, AF Ferreiro, EG Ferretti, A Festanti, A Feuillard, VJG Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fiore, EM Fleck, MG Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fuchs, U Furget, C Furs, A Girard, MF Gaardhoje, JJ Gagliardi, M Gago, AM Gallio, M Gangadharan, DR Ganoti, P Gao, C Garabatos, C Garcia-Solis, E Gargiulo, C Gasik, P Germain, M Gheata, A Gheata, M Ghosh, P Ghosh, SK Gianotti, P Giubellino, P Giubilato, P Gladysz-Dziadus, E Glassel, P Coral, DMG Ramirez, AG Gonzalez-Zamora, P Gorbunov, S Gorlich, L Gotovac, S Grabski, V Graczykowski, LK Graham, KL Grelli, A Grigoras, A Grigoras, C Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Grosse-Oetringhaus, JF Grossiord, JY Grosso, R Guber, F Guernane, R Guerzoni, B Gulbrandsen, K Gulkanyan, H Gunji, T Gupta, A Gupta, R Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H Hamar, G Hansen, A Harris, JW Hartmann, H Harton, A Hatzifotiadou, D Hayashi, S Heckel, ST Heide, M Helstrup, H Herghelegiu, A Corral, GH Hess, BA Hetland, KF Hilden, TE Hillemanns, H Hippolyte, B Hosokawa, R Hristov, P Huang, M Humanic, TJ Hussain, N Hussain, T Hutter, D Hwang, DS Ilkaev, R Ilkiv, I Inaba, M Ippolitov, M Irfan, M Ivanov, M Ivanov, V Izucheev, V Jacobs, PM Jadlovska, S Jahnke, C Jang, HJ Janik, MA Jayarathna, PHSY Jena, C Jena, S Bustamante, RTJ Jones, PG Jung, H Jusko, A Kalinak, P Kalweit, A Kamin, J Kang, JH Kaplin, V Kar, S Uysal, AK Karavichev, O Karavicheva, T Karayan, L Karpechev, E Kebschull, U Keidel, R Keijdener, DLD Keil, M Khan, KH Khan, MM Khan, P Khan, SA Khanzadeev, A Kharlov, Y Kileng, B Kim, B Kim, DW Kim, DJ Kim, H Kim, JS Kim, M Kim, M Kim, S Kim, T Kirsch, S Kisel, I Kiselev, S Kisiel, A Kiss, G Klay, JL Klein, C Klein, J Klein-Bosing, C Kluge, A Knichel, ML Knospe, AG Kobayashi, T Kobdaj, C Kofarago, M Kollegger, T Kolojvari, A Kondratiev, V Kondratyeva, N Kondratyuk, E Konevskikh, A Kopcik, M Kour, M Kouzinopoulos, C Kovalenko, O Kovalenko, V Kowalski, M Meethaleveedu, GK Kral, J Kralik, I Kravcakova, A Krelina, M Kretz, M Krivda, M Krizek, F Kryshen, E Krzewicki, M Kubera, AM Kucera, V Kugathasan, T Kuhn, C Kuijer, PG Kulakov, I Kumar, A Kumar, J Kumar, L Kurashvili, P Kurepin, A Kurepin, AB Kuryakin, A Kushpil, S Kweon, MJ Kwon, Y La Pointe, SL La Rocca, P Fernandes, CL Lakomov, I Langoy, R Lara, C Lardeux, A Lattuca, A Laudi, E Lea, R Leardini, L Lee, GR Lee, S Legrand, I Lehas, F Lemmon, RC Lenti, V Leogrande, E Monzon, IL Leoncino, M Levai, P Li, S Li, X Lien, J Lietava, R Lindal, S Lindenstruth, V Lippmann, C Lisa, MA Ljunggren, HM Lodato, DF Loenne, PI Loginov, V Loizides, C Lopez, X Torres, EL Lowe, A Luettig, P Lunardon, M Luparello, G Luz, PHFND Maevskaya, A Mager, M Mahajan, S Mahmood, SM Maire, A Majka, RD Malaev, M Cervantes, IM Malinina, L Mal'Kevich, D Malzacher, P Mamonov, A Manko, V Manso, F Manzari, V Marchisone, M Mares, J Margagliotti, GV Margotti, A Margutti, J Marin, A Markert, C Marquard, M Martin, NA Blanco, JM Martinengo, P Martinez, MI Garcia, GM Pedreira, MM Martynov, Y Mas, A Masciocchi, S Masera, M Masoni, A Massacrier, L Mastroserio, A Masui, H Matyja, A Mayer, C Mazer, J Mazzoni, MA Mcdonald, D Meddi, F Melikyan, Y Menchaca-Rocha, A Meninno, E Perez, JM Meres, M Miake, Y Mieskolainen, MM Mikhaylov, K Milano, L Milosevic, J Minervini, LM Mischke, A Mishra, AN Miskowiec, D Mitra, J Mitu, CM Mohammadi, N Mohanty, B Molnar, L Zetina, LM Montes, E Morando, M De Godoy, DAM Moretto, S Morreale, A Morsch, A Muccifora, V Mudnic, E Muhlheim, D Muhuri, S Mukherjee, M Mulligan, JD Munhoz, MG Murray, S Musa, L Musinsky, J Nandi, BK Nania, R Nappi, E Naru, MU Nattrass, C Nayak, K Nayak, TK Nazarenko, S Nedosekin, A Nellen, L Ng, F Nicassio, M Niculescu, M Niedziela, J Nielsen, BS Nikolaev, S Nikulin, S Nikulin, V Noferini, F Nomokonov, P Nooren, G Noris, JCC Norman, J Nyanin, A Nystrand, J Oeschler, H Oh, S Oh, SK Ohlson, A Okatan, A Okubo, T Olah, L Oleniacz, J Da Silva, ACO Oliver, MH Onderwaater, J Oppedisano, C Orava, R Velasquez, AO Oskarsson, A Otwinowski, J Oyama, K Ozdemir, M Pachmayer, Y Pagano, P Paic, G Pajares, C Pal, SK Pan, J Pandey, AK Pant, D Papcun, P Papikyan, V Pappalardo, GS Pareek, P Park, WJ Parmar, S Passfeld, A Paticchio, V Patra, RN Paul, B Peitzmann, T Da Costa, HP De Oliveira, EP Peresunko, D Lara, CEP Lezama, EP Peskov, V Pestov, Y Petracek, V Petrov, V Petrovici, M Petta, C Piano, S Pikna, M Pillot, P Pinazza, O Pinsky, L Piyarathna, DB Ploskon, M Planinic, M Pluta, J Pochybova, S Podesta-Lerma, PLM Poghosyan, MG Polichtchouk, B Poljak, N Poonsawat, W Pop, A Porteboeuf-Houssais, S Porter, J Pospisil, J Prasad, SK Preghenella, R Prino, F Pruneau, CA Pshenichnov, I Puccio, M Puddu, G Pujahari, P Punin, V Putschke, J Qvigstad, H 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JE Sekiguchi, Y Sekihata, D Selyuzhenkov, I Senosi, K Seo, J Serradilla, E Sevcenco, A Shabanov, A Shabetai, A Shadura, O Shahoyan, R Shangaraev, A Sharma, A Sharma, M Sharma, M Sharma, N Shigaki, K Shtejer, K Sibiriak, Y Siddhanta, S Sielewicz, KM Siemiarczuk, T Silvermyr, D Silvestre, C Simatovic, G Simonetti, G Singaraju, R Singh, R Singha, S Singhal, V Sinha, BC Sinha, T Sitar, B Sitta, M Skaali, TB Slupecki, M Smirnov, N Snellings, RJM Snellman, TW Sogaard, C Soltz, R Song, J Song, M Song, Z Soramel, F Sorensen, S Spacek, M Spiriti, E Sputowska, I Spyropoulou-Stassinaki, M Srivastava, BK Stachel, J Stan, I Stefanek, G Steinpreis, M Stenlund, E Steyn, G Stiller, JH Stocco, D Strmen, P Suaide, AAP Sugitate, T Suire, C Suleymanov, M Sultanov, R Sumbera, MO Symons, TJM Szabo, A de Toledo, AS Szarka, I Szczepankiewicz, A Szymanski, M Takahashi, J Tambave, GJ Tanaka, N Tangaro, MA Takaki, JDT Peloni, AT Tarhini, M Tariq, M Tarzila, MG Tauro, A Munoz, GT Telesca, A Terasaki, K Terrevoli, C Teyssier, B Thader, J Thomas, D Tieulent, R Timmins, AR Toia, A Trogolo, S Trubnikov, V Trzaska, WH Tsuji, T Tumkin, A Turrisi, R Tveter, TS Ullaland, K Uras, A Usai, GL Utrobicic, A Vajzer, M Vala, M Palomo, LV Vallero, S Van der Maarel, J Van Hoorne, JW van Leeuwen, M Vanat, T Vyvre, PV Varga, D Vargas, A Vargyas, M Varma, R Vasileiou, M Vasiliev, A Vauthier, A Vechernin, V Veen, AM Veldhoen, M Velure, A Venaruzzo, M Vercellin, E Limon, SV Vernet, R Verweij, M Vickovic, L Viesti, G Viinikainen, J Vilakazi, Z Baillie, OV Vinogradov, A Vinogradov, L Vinogradov, Y Virgili, T Vislavicius, V Viyogi, YP Vodopyanov, A Volkl, MA Voloshin, K Voloshin, SA Volpe, G von Haller, B Vorobyev, I Vranic, D Vrlakova, J Vulpescu, B Vyushin, A Wagner, B Wagner, J Wang, H Wang, M Wang, Y Watanabe, D Watanabe, Y Weber, M Weber, SG Wessels, JP Westerhoff, U Wiechula, J Wikne, J Wilde, M Wilk, G Wilkinson, J Williams, MCS Windelband, B Winn, M Yaldo, CG Yang, H Yang, P Yano, S Yin, Z Yokoyama, H Yoo, IK Yurchenko, V Yushmanov, I Zaborowska, A Zaccolo, V Zaman, A Zampolli, C Zanoli, HJC Zaporozhets, S Zardoshti, N Zarochentsev, A Zavada, P Zaviyalov, N Zbroszczyk, H Zgura, IS Zhalov, M Zhang, H Zhang, X Zhang, Y Zhao, C Zhigareva, N Zhou, D Zhou, Y Zhou, Z Zhu, H Zhu, J Zhu, X Zichichi, A Zimmermann, A Zimmermann, MB Zinovjev, G Zyzak, M AF Adam, J. 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CA ALICE Collaboration TI Centrality dependence of the nuclear modification factor of charged pions, kaons, and protons in Pb-Pb collisions at root s(NN)=2.76 TeV SO PHYSICAL REVIEW C LA English DT Article ID LARGE TRANSVERSE-MOMENTUM; QUARK-GLUON PLASMA; PARTICLE PRODUCTION; AA-COLLISIONS; PP COLLISIONS; MATTER; COLLABORATION; PERSPECTIVE; SUPPRESSION; SPECTRA AB Transverse momentum (p(T)) spectra of pions, kaons, and protons up to p(T) = 20 GeV/c have been measured in Pb-Pb collisions at root s(NN) = 2.76 TeV using the ALICE detector for six different centrality classes covering 0%-80%. The proton-to-pion and the kaon-to-pion ratios both show a distinct peak at p(T) approximate to 3 GeV/c in central Pb-Pb collisions that decreases for more peripheral collisions. For p(T) > 10 GeV/c, the nuclear modification factor is found to be the same for all three particle species in each centrality interval within systematic uncertainties of 10%-20%. 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Moreira; Morreale, A.; Pillot, P.; Ronflette, L.; Schutz, Y.; Shabetai, A.; Stocco, D.; Wang, M.; Zhu, J.] Univ Nantes, CNRS IN2P3, Ecole Mines Nantes, SUBATECH, Nantes, France. [Kobdaj, C.; Poonsawat, W.] Suranaree Univ Technol, Nakhon Ratchasima, Thailand. [Cerkala, J.; Jadlovska, S.; Kopcik, M.; Papcun, P.] Tech Univ Kosice, Kosice, Slovakia. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ Split FESB, Split, Croatia. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Goerlich, L.; Kowalski, M.; Matyja, A.; Mayer, C.; Otwinowski, J.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Blair, J. T.; Knospe, A. G.; Markert, C.; Thomas, D.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Almaraz, J. R. M.; Leon Monzon, I.; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Alves Garcia Prado, C.; Bregant, M.; Cosentino, M. R.; De, S.; Domenicis Gimenez, D.; Figueredo, M. A. S.; Jahnke, C.; Lagana Fernandes, C.; Luz, P. 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H.; Kim, B.; Kim, H.; Kim, M.; Kim, T.; Kwon, Y.; Lee, S.; Song, M.] Yonsei Univ, Seoul 120749, South Korea. [Keidel, R.] Fachhsch Worms, ZTT, Worms, Germany. [Malinina, L.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl, Moscow, Russia. [Takaki, J. D. Tapia] Univ Kansas, Lawrence, KS 66045 USA. RP Adam, J (reprint author), Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-16635 Prague, Czech Republic. RI Ferreiro, Elena/C-3797-2017; Armesto, Nestor/C-4341-2017; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Kovalenko, Vladimir/C-5709-2013; Altsybeev, Igor/K-6687-2013; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; Chinellato, David/D-3092-2012; Jena, Satyajit/P-2409-2015; Pshenichnov, Igor/A-4063-2008; Vechernin, Vladimir/J-5832-2013; Akindinov, Alexander/J-2674-2016; Felea, Daniel/C-1885-2012; Bregant, Marco/I-7663-2012; Sevcenco, Adrian/C-1832-2012; De Pasquale, Salvatore/B-9165-2008; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Takahashi, Jun/B-2946-2012; Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Cosentino, Mauro/L-2418-2014; Suaide, Alexandre/L-6239-2016; Barnby, Lee/G-2135-2010; Peitzmann, Thomas/K-2206-2012; Kondratiev, Valery/J-8574-2013; Vinogradov, Leonid/K-3047-2013; Martynov, Yevgen/L-3009-2015; Castillo Castellanos, Javier/G-8915-2013 OI Giubilato, Piero/0000-0003-4358-5355; Fernandez Tellez, Arturo/0000-0001-5092-9748; Ferreiro, Elena/0000-0002-4449-2356; Armesto, Nestor/0000-0003-0940-0783; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Kovalenko, Vladimir/0000-0001-6012-6615; Altsybeev, Igor/0000-0002-8079-7026; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Riggi, Francesco/0000-0002-0030-8377; Scarlassara, Fernando/0000-0002-4663-8216; Melikyan, Yury/0000-0002-4165-505X; Chinellato, David/0000-0002-9982-9577; Jena, Satyajit/0000-0002-6220-6982; Pshenichnov, Igor/0000-0003-1752-4524; Vechernin, Vladimir/0000-0003-1458-8055; Akindinov, Alexander/0000-0002-7388-3022; Felea, Daniel/0000-0002-3734-9439; Sevcenco, Adrian/0000-0002-4151-1056; De Pasquale, Salvatore/0000-0001-9236-0748; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Takahashi, Jun/0000-0002-4091-1779; Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Cosentino, Mauro/0000-0002-7880-8611; Suaide, Alexandre/0000-0003-2847-6556; Barnby, Lee/0000-0001-7357-9904; Peitzmann, Thomas/0000-0002-7116-899X; Kondratiev, Valery/0000-0002-0031-0741; Vinogradov, Leonid/0000-0001-9247-6230; Martynov, Yevgen/0000-0003-0753-2205; Castillo Castellanos, Javier/0000-0002-5187-2779 FU Grid centres; Worldwide LHC Computing Grid (WLCG); State Committee of Science, Armenia; World Federation of Scientists (WFS), Armenia; Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3, France; Region Pays de Loire, France; Region Alsace, France; Region Auvergne, France; CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Greece; Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA); National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN), Italy; Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Mexico; Direccion General de Asuntos del Personal Academico(DGAPA), Mexico; Amerique Latine Formation academique-European Commission (ALFA-EC); EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM), Netherlands; Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics, Romania; National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), Cuba; Xunta de Galicia (Conselleria de Educacion), Cuba; Centro de Aplicaciones Tecnolgicas y Desarrollo Nuclear (CEADEN), Cuba; Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia, Croatia; Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; E-Infrastructure shared between Europe and Latin America (EELA), Cuba; Ministerio de Economia y Competitividad (MINECO) of Spain, Cuba FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) collaboration.; The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the "Region Pays de Loire," "Region Alsace," "Region Auvergne," and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA) and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi-Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi," Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico(DGAPA), Mexico, Amerique Latine Formation academique-European Commission (ALFA-EC) and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), Centro de Aplicaciones Tecnolgicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India. NR 72 TC 6 Z9 6 U1 7 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 25 PY 2016 VL 93 IS 3 AR 034913 DI 10.1103/PhysRevC.93.034913 PG 31 WC Physics, Nuclear SC Physics GA DH3XL UT WOS:000372720000004 ER PT J AU Adamson, P Ader, C Andrews, M Anfimov, N Anghel, I Arms, K Arrieta-Diaz, E Aurisano, A Ayres, DS Backhouse, C Baird, M Bambah, BA Bays, K Bernstein, R Betancourt, M Bhatnagar, V Bhuyan, B Bian, J Biery, K Blackburn, T Bocean, V Bogert, D Bolshakova, A Bowden, M Bower, C Broemmelsiek, D Bromberg, C Brunetti, G Bu, X Butkevich, A Capista, D Catano-Mur, E Chase, TR Childress, S Choudhary, BC Chowdhury, B Coan, TE Coelho, JAB Colo, M Cooper, J Corwin, L Cronin-Hennessy, D Cunningham, A Davies, GS Davies, JP Del Tutto, M Derwent, PF Deepthi, KN Demuth, D Desai, S Deuerling, G Devan, A Dey, J Dharmapalan, R Ding, P Dixon, S Djurcic, Z Dukes, EC Duyang, H Ehrlich, R Feldman, GJ Felt, N Fenyves, EJ Flumerfelt, E Foulkes, S Frank, MJ Freeman, W Gabrielyan, M Gallagher, HR Gebhard, M Ghosh, T Gilbert, W Giri, A Goadhouse, S Gomes, RA Goodenough, L Goodman, MC Grichine, V Grossman, N Group, R Grudzinski, J Guarino, V Guo, B Habig, A Handler, T Hartnell, J Hatcher, R Hatzikoutelis, A Heller, K Howcroft, C Huang, J Huang, X Hylen, J Ishitsuka, M Jediny, F Jensen, C Jensen, D Johnson, C Jostlein, H Kafka, GK Kamyshkov, Y Kasahara, SMS Kasetti, S Kephart, K Koizumi, G Kotelnikov, S Kourbanis, I Krahn, Z Kravtsov, V Kreymer, A Kulenberg, C Kumar, A Kutnink, T Kwarciancy, R Kwong, J Lang, K Lee, A Lee, WM Lee, K Lein, S Liu, J Lokajicek, M Lozier, J Lu, Q Lucas, P Luchuk, S Lukens, P Lukhanin, G Magill, S Maan, K Mann, WA Marshak, ML Martens, M Martincik, J Mason, P Matera, K Mathis, M Matveev, V Mayer, N McCluskey, E Mehdiyev, R Merritt, H Messier, MD Meyer, H Miao, T Michael, D Mikheyev, SP Miller, WH Mishra, SR Mohanta, R Moren, A Mualem, L Muether, M Mufson, S Musser, J Newman, HB Nelson, JK Niner, E Norman, A Nowak, J Oksuzian, Y Olshevskiy, A Oliver, J Olson, T Paley, J Pandey, P Para, A Patterson, RB Pawloski, G Pearson, N Perevalov, D Pershey, D Peterson, E Petti, R Phan-Budd, S Piccoli, L Pla-Dalmau, A Plunkett, RK Poling, R Potukuchi, B Psihas, F Pushka, D Qiu, X Raddatz, N Radovic, A Rameika, RA Ray, R Rebel, B Rechenmacher, R Reed, B Reilly, R Rocco, D Rodkin, D Ruddick, K Rusack, R Ryabov, V Sachdev, K Sahijpal, S Sahoo, H Samoylov, O Sanchez, MC Saoulidou, N Schlabach, P Schneps, J Schroeter, R Sepulveda-Quiroz, J Shanahan, P Sherwood, B Sheshukov, A Singh, J Singh, V Smith, A Smith, D Smolik, J Solomey, N Sotnikov, A Sousa, A Soustruznik, K Stenkin, Y Strait, M Suter, L Talaga, RL Tamsett, MC Tariq, S Tas, P Tesarek, RJ Thayyullathil, RB Thomsen, K Tian, X Tognini, SC Toner, R Trevor, J Tzanakos, G Urheim, J Vahle, P Valerio, L Vinton, L Vrba, T Waldron, AV Wang, B Wang, Z Weber, A Wehmann, A Whittington, D Wilcer, N Wildberger, R Wildman, D Williams, K Wojcicki, SG Wood, K Xiao, M Xin, T Yadav, N Yang, S Zadorozhnyy, S Zalesak, J Zamorano, B Zhao, A Zirnstein, J Zwaska, R AF Adamson, P. Ader, C. Andrews, M. Anfimov, N. Anghel, I. Arms, K. Arrieta-Diaz, E. Aurisano, A. Ayres, D. S. Backhouse, C. Baird, M. Bambah, B. A. Bays, K. Bernstein, R. Betancourt, M. Bhatnagar, V. Bhuyan, B. Bian, J. Biery, K. Blackburn, T. Bocean, V. Bogert, D. Bolshakova, A. Bowden, M. Bower, C. Broemmelsiek, D. Bromberg, C. Brunetti, G. Bu, X. Butkevich, A. Capista, D. Catano-Mur, E. Chase, T. R. Childress, S. Choudhary, B. C. Chowdhury, B. Coan, T. E. Coelho, J. A. B. Colo, M. Cooper, J. Corwin, L. Cronin-Hennessy, D. Cunningham, A. Davies, G. S. Davies, J. P. Del Tutto, M. Derwent, P. F. Deepthi, K. N. Demuth, D. Desai, S. Deuerling, G. Devan, A. Dey, J. Dharmapalan, R. Ding, P. Dixon, S. Djurcic, Z. Dukes, E. C. Duyang, H. Ehrlich, R. Feldman, G. J. Felt, N. Fenyves, E. J. Flumerfelt, E. Foulkes, S. Frank, M. J. Freeman, W. Gabrielyan, M. Gallagher, H. R. Gebhard, M. Ghosh, T. Gilbert, W. Giri, A. Goadhouse, S. Gomes, R. A. Goodenough, L. Goodman, M. C. Grichine, V. Grossman, N. Group, R. Grudzinski, J. Guarino, V. Guo, B. Habig, A. Handler, T. Hartnell, J. Hatcher, R. Hatzikoutelis, A. Heller, K. Howcroft, C. Huang, J. Huang, X. Hylen, J. Ishitsuka, M. Jediny, F. Jensen, C. Jensen, D. Johnson, C. Jostlein, H. Kafka, G. K. Kamyshkov, Y. Kasahara, S. M. S. Kasetti, S. Kephart, K. Koizumi, G. Kotelnikov, S. Kourbanis, I. Krahn, Z. Kravtsov, V. Kreymer, A. Kulenberg, Ch. Kumar, A. Kutnink, T. Kwarciancy, R. Kwong, J. Lang, K. Lee, A. Lee, W. M. Lee, K. Lein, S. Liu, J. Lokajicek, M. Lozier, J. Lu, Q. Lucas, P. Luchuk, S. Lukens, P. Lukhanin, G. Magill, S. Maan, K. Mann, W. A. Marshak, M. L. Martens, M. Martincik, J. Mason, P. Matera, K. Mathis, M. Matveev, V. Mayer, N. McCluskey, E. Mehdiyev, R. Merritt, H. Messier, M. D. Meyer, H. Miao, T. Michael, D. Mikheyev, S. P. Miller, W. H. Mishra, S. R. Mohanta, R. Moren, A. Mualem, L. Muether, M. Mufson, S. Musser, J. Newman, H. B. Nelson, J. K. Niner, E. Norman, A. Nowak, J. Oksuzian, Y. Olshevskiy, A. Oliver, J. Olson, T. Paley, J. Pandey, P. Para, A. Patterson, R. B. Pawloski, G. Pearson, N. Perevalov, D. Pershey, D. Peterson, E. Petti, R. Phan-Budd, S. Piccoli, L. Pla-Dalmau, A. Plunkett, R. K. Poling, R. Potukuchi, B. Psihas, F. Pushka, D. Qiu, X. Raddatz, N. Radovic, A. Rameika, R. A. Ray, R. Rebel, B. Rechenmacher, R. Reed, B. Reilly, R. Rocco, D. Rodkin, D. Ruddick, K. Rusack, R. Ryabov, V. Sachdev, K. Sahijpal, S. Sahoo, H. Samoylov, O. Sanchez, M. C. Saoulidou, N. Schlabach, P. Schneps, J. Schroeter, R. Sepulveda-Quiroz, J. Shanahan, P. Sherwood, B. Sheshukov, A. Singh, J. Singh, V. Smith, A. Smith, D. Smolik, J. Solomey, N. Sotnikov, A. Sousa, A. Soustruznik, K. Stenkin, Y. Strait, M. Suter, L. Talaga, R. L. Tamsett, M. C. Tariq, S. Tas, P. Tesarek, R. J. Thayyullathil, R. B. Thomsen, K. Tian, X. Tognini, S. C. Toner, R. Trevor, J. Tzanakos, G. Urheim, J. Vahle, P. Valerio, L. Vinton, L. Vrba, T. Waldron, A. V. Wang, B. Wang, Z. Weber, A. Wehmann, A. Whittington, D. Wilcer, N. Wildberger, R. Wildman, D. Williams, K. Wojcicki, S. G. Wood, K. Xiao, M. Xin, T. Yadav, N. Yang, S. Zadorozhnyy, S. Zalesak, J. Zamorano, B. Zhao, A. Zirnstein, J. Zwaska, R. CA NOvA Collaboration TI First measurement of muon-neutrino disappearance in NOvA SO PHYSICAL REVIEW D LA English DT Article ID LEPTON CHARGE; BEAM AB This paper reports the first measurement using the NOvA detectors of nu(mu) disappearance in a nu(mu) beam. The analysis uses a 14 kton-equivalent exposure of 2.74 x 10(20) protons-on-target from the Fermilab NuMI beam. Assuming the normal neutrino mass hierarchy, we measure Delta m(32)(2) = (2.52(-0.18)(+0.20)) x 10(-3) eV(2) and sin(2) theta(23) in the range 0.38-0.65, both at the 68% confidence level, with two statistically degenerate best-fit points at sin(2) theta(23) = 0.43 and 0.60. Results for the inverted mass hierarchy are also presented. C1 [Anghel, I.; Ayres, D. S.; Dharmapalan, R.; Djurcic, Z.; Goodenough, L.; Goodman, M. C.; Grudzinski, J.; Guarino, V.; Huang, X.; Magill, S.; Sahoo, H.; Sanchez, M. C.; Sepulveda-Quiroz, J.; Suter, L.; Talaga, R. L.; Wood, K.; Zhao, A.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Lokajicek, M.; Zalesak, J.] Acad Sci Czech Republic, Inst Phys, Prague 18221, Czech Republic. [Tzanakos, G.] Univ Athens, Dept Phys, GR-15771 Athens, Greece. [Singh, V.] Banaras Hindu Univ, Dept Phys, Varanasi 221005, Uttar Pradesh, India. [Lee, K.] Univ Calif Los Angeles, Dept Phys & Astron, Box 951547, Los Angeles, CA 90095 USA. [Backhouse, C.; Bays, K.; Howcroft, C.; Lozier, J.; Michael, D.; Mualem, L.; Newman, H. B.; Patterson, R. B.; Pershey, D.; Trevor, J.] CALTECH, Pasadena, CA 91125 USA. [Soustruznik, K.; Tas, P.] Charles Univ Prague, Fac Math & Phys, Inst Particle & Nucl Phys, Prague 11636 1, Czech Republic. [Aurisano, A.; Sousa, A.; Yang, S.] Univ Cincinnati, Dept Phys, Cincinnati, OH 45221 USA. [Thayyullathil, R. B.] Cochin Univ Sci & Technol, Dept Phys, Cochin 682022, Kerala, India. [Jediny, F.; Martincik, J.; Smolik, J.; Vrba, T.] Czech Tech Univ, Brehova 7, Prague 11519 1, Czech Republic. [Choudhary, B. C.; Pandey, P.] Univ Delhi, Dept Phys & Astrophys, Delhi 110007, India. [Adamson, P.; Ader, C.; Andrews, M.; Bernstein, R.; Biery, K.; Bocean, V.; Bogert, D.; Bowden, M.; Broemmelsiek, D.; Brunetti, G.; Bu, X.; Capista, D.; Childress, S.; Cooper, J.; Del Tutto, M.; Derwent, P. F.; Deuerling, G.; Dey, J.; Ding, P.; Dixon, S.; Foulkes, S.; Freeman, W.; Grossman, N.; Hatcher, R.; Hylen, J.; Jensen, C.; Jensen, D.; Jostlein, H.; Kephart, K.; Koizumi, G.; Kourbanis, I.; Kreymer, A.; Kwarciancy, R.; Lee, A.; Lee, W. M.; Lu, Q.; Lucas, P.; Lukens, P.; Lukhanin, G.; Martens, M.; Matera, K.; McCluskey, E.; Miao, T.; Norman, A.; Paley, J.; Para, A.; Perevalov, D.; Piccoli, L.; Pla-Dalmau, A.; Plunkett, R. K.; Pushka, D.; Rameika, R. A.; Ray, R.; Rebel, B.; Rechenmacher, R.; Reilly, R.; Saoulidou, N.; Schlabach, P.; Shanahan, P.; Tariq, S.; Tesarek, R. J.; Valerio, L.; Wehmann, A.; Wilcer, N.; Wildman, D.; Williams, K.; Xiao, M.; Zwaska, R.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Ghosh, T.; Gomes, R. A.; Tognini, S. C.] Univ Fed Goias, Inst Fis, BR-74690900 Goiania, Go, Brazil. [Bhuyan, B.; Yadav, N.] IIT Guwahati, Dept Phys, Gauhati 781039, India. [Feldman, G. J.; Felt, N.; Kafka, G. K.; Oliver, J.; Schroeter, R.; Toner, R.] Harvard Univ, Dept Phys, Cambridge, MA 02138 USA. [Bambah, B. A.; Deepthi, K. N.; Kasetti, S.; Mohanta, R.] Univ Hyderabad, Sch Phys, Hyderabad 500046, Andhra Pradesh, India. [Giri, A.] IIT Hyderabad, Dept Phys, Hyderabad 502205, Andhra Pradesh, India. [Baird, M.; Bower, C.; Davies, G. S.; Gebhard, M.; Ishitsuka, M.; Johnson, C.; Merritt, H.; Messier, M. D.; Mufson, S.; Musser, J.; Niner, E.; Psihas, F.; Urheim, J.; Whittington, D.] Indiana Univ, Bloomington, IN 47405 USA. [Butkevich, A.; Luchuk, S.; Matveev, V.; Mikheyev, S. P.; Rodkin, D.; Stenkin, Y.; Zadorozhnyy, S.] Acad Sci 7A, October Anniversary prospect 60, Institute Nucl Res Russian, Moscow 117312, Russia. [Anghel, I.; Catano-Mur, E.; Kutnink, T.; Sanchez, M. C.; Sepulveda-Quiroz, J.; Xin, T.] Iowa State Univ Sci & Technol, Dept Phys & Astron, Ames, IA 50011 USA. [Potukuchi, B.] Univ Jammu, Dept Phys & Elect, Jammu 180006, Jammu & Kashmir, India. [Anfimov, N.; Bolshakova, A.; Kulenberg, Ch.; Olshevskiy, A.; Samoylov, O.; Sheshukov, A.; Sotnikov, A.] Joint Inst Nucl Res Joliot Curie, Dubna 141980, Moscow Region, Russia. [Grichine, V.; Kotelnikov, S.; Ryabov, V.] Lebedev Phys Inst, Nucl Phys Dept, Leninsky Prospect 53, Moscow 119991, Russia. [Bromberg, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Demuth, D.] Univ Minnesota Crookston, Math Sci & Technol Dept, Crookston, MN 56716 USA. [Habig, A.; Moren, A.; Thomsen, K.] Univ Minnesota, Dept Phys & Astron, Duluth, MN 55812 USA. [Arms, K.; Betancourt, M.; Bian, J.; Chase, T. R.; Cronin-Hennessy, D.; Desai, S.; Gabrielyan, M.; Gilbert, W.; Heller, K.; Kasahara, S. M. S.; Krahn, Z.; Kwong, J.; Lein, S.; Marshak, M. L.; Miller, W. H.; Nowak, J.; Pawloski, G.; Pearson, N.; Peterson, E.; Poling, R.; Raddatz, N.; Rocco, D.; Ruddick, K.; Rusack, R.; Sachdev, K.; Sherwood, B.; Smith, A.; Strait, M.; Wildberger, R.; Zirnstein, J.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Weber, A.] Univ Oxford, Subdept Particle Phys, Oxford OX1 3RH, England. [Bhatnagar, V.; Kumar, A.; Maan, K.; Sahijpal, S.; Singh, J.] Panjab Univ, Dept Phys, Chandigarh 106014, India. [Weber, A.] Rutherford Appleton Lab, Sci & Technol Facil Council, Didcot OX11 0QX, Oxon, England. [Chowdhury, B.; Duyang, H.; Guo, B.; Mishra, S. R.; Petti, R.; Tian, X.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Corwin, L.; Reed, B.; Smith, D.] South Dakota Sch Mines & Technol, Rapid City, SD 57701 USA. [Arrieta-Diaz, E.; Coan, T. E.; Kravtsov, V.; Wang, B.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Qiu, X.; Wojcicki, S. G.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Blackburn, T.; Davies, J. P.; Hartnell, J.; Tamsett, M. C.; Vinton, L.; Waldron, A. V.; Zamorano, B.] Univ Sussex, Dept Phys & Astron, Brighton BN1 9QH, E Sussex, England. [Flumerfelt, E.; Handler, T.; Hatzikoutelis, A.; Kamyshkov, Y.; Mason, P.] Univ Tennessee, Dept Phys & Astron, 1408 Circle Dr, Knoxville, TN 37996 USA. [Huang, J.; Lang, K.; Mehdiyev, R.] Univ Texas Austin, Dept Phys, 1 Univ Stn C1600, Austin, TX 78712 USA. [Cunningham, A.; Fenyves, E. J.] Univ Texas Dallas, Dept Phys, 800 W Campbell Rd, Richardson, TX 75083 USA. [Coelho, J. A. B.; Gallagher, H. R.; Mann, W. A.; Mayer, N.; Olson, T.; Schneps, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Dukes, E. C.; Ehrlich, R.; Frank, M. J.; Goadhouse, S.; Group, R.; Oksuzian, Y.; Wang, Z.] Univ Virginia, Dept Phys, Charlottesville, VA 22904 USA. [Meyer, H.; Muether, M.; Solomey, N.] Wichita State Univ, Div Phys, 1845 Fairmout St, Wichita, KS 67220 USA. [Colo, M.; Devan, A.; Liu, J.; Mathis, M.; Nelson, J. K.; Radovic, A.; Vahle, P.] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Phan-Budd, S.] Winona State Univ, Dept Phys, POB 5838, Winona, MN 55987 USA. RP Adamson, P (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RI Kotelnikov, Sergey/A-9711-2014; Gomes, Ricardo/B-6899-2008; Sheshukov, Andrey/I-1193-2016; Ryabov, Vladimir/E-1281-2014; Anfimov, Nikolay/I-1322-2016; Olshevskiy, Alexander/I-1580-2016; Samoylov, Oleg/L-7271-2013; Kamyshkov, Yuri/J-7999-2016; Nowak, Jaroslaw/P-2502-2016; Martincik, Jiri/H-3566-2014; Stenkin, Yuri/M-5796-2014; OI Corwin, Luke/0000-0001-7143-3821; Hartnell, Jeffrey/0000-0002-1744-7955; Bernstein, Robert/0000-0002-7610-950X; Weber, Alfons/0000-0002-8222-6681; Kotelnikov, Sergey/0000-0002-8027-4612; Gomes, Ricardo/0000-0003-0278-4876; Anfimov, Nikolay/0000-0002-9099-7574; Olshevskiy, Alexander/0000-0002-8902-1793; Samoylov, Oleg/0000-0003-2141-8230; Kamyshkov, Yuri/0000-0002-3789-7152; Nowak, Jaroslaw/0000-0001-8637-5433; Martincik, Jiri/0000-0002-5379-441X; Group, Robert/0000-0002-4097-5254 FU U.S. Department of Energy (DOE); U.S. National Science Foundation; Department of Science and Technology, India; European Research Council; MSMT CR, Czech Republic; RAS, Russia; CNPq, Brazil; State and University of Minnesota; U.S. DOE [De-AC02-07CH11359]; RMES, Russia; RFBR, Russia; FAPEG, Brazil FX This work was supported by the U.S. Department of Energy (DOE); the U.S. National Science Foundation; the Department of Science and Technology, India; the European Research Council; the MSMT CR, Czech Republic; the RAS, RMES, and RFBR, Russia; CNPq and FAPEG, Brazil; and the State and University of Minnesota. We are grateful for the contributions of the staffs of the University of Minnesota module assembly facility and NOvA FD Laboratory, Argonne National Laboratory, and Fermilab. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. De-AC02-07CH11359 with the U.S. DOE. NR 34 TC 18 Z9 18 U1 7 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 25 PY 2016 VL 93 IS 5 AR 051104 DI 10.1103/PhysRevD.93.051104 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH3XV UT WOS:000372721000001 ER PT J AU Chen, WQ Wang, LF Van Berkel, GJ Kertesz, V Gan, JP AF Chen, Weiqi Wang, Lifei Van Berkel, Gary J. Kertesz, Vilmos Gan, Jinping TI Quantitation of repaglinide and metabolites in mouse whole-body thin tissue sections using droplet-based liquid microjunction surface sampling-high-performance liquid chromatography-electrospray ionization tandem mass spectrometry SO JOURNAL OF CHROMATOGRAPHY A LA English DT Article DE Liquid microjunction; Droplet-based liquid extraction; Quantitation; Autosampler; Spatial distribution; Repaglinide ID SPATIALLY-RESOLVED ANALYSIS; RAT-BRAIN TISSUE; TRYPTIC DIGESTION; DRUG DISTRIBUTION; LESA-MS; PROTEINS; MS/MS; AUTORADIOGRAPHY; TERFENADINE; DISCOVERY AB Herein, quantitation aspects of a fully automated autosampler/HPLC-MS/MS system applied for unattended droplet-based surface sampling of repaglinide dosed thin tissue sections with subsequent HPLC separation and mass spectrometric analysis of parent drug and various drug metabolites were studied. Major organs (brain, lung, liver, kidney and muscle) from whole-body thin tissue sections and corresponding organ homogenates prepared from repaglinide dosed mice were sampled by surface sampling and by bulk extraction, respectively, and analyzed by HPLC-MS/MS. A semi-quantitative agreement between data obtained by surface sampling and that by employing organ homogenate extraction was observed. Drug concentrations obtained by the two methods followed the same patterns for post-dose time points (0.25, 0.5, 1 and 2h). Drug amounts determined in the specific tissues was typically higher when analyzing extracts from the organ homogenates. In addition, relative comparison of the levels of individual metabolites between the two analytical methods also revealed good semi-quantitative agreement. (C) 2015 Elsevier B.V. All rights reserved. C1 [Chen, Weiqi; Wang, Lifei; Gan, Jinping] Bristol Myers Squibb Res & Dev, Pharmaceut Candidate Optimizat, Princeton, NJ 08543 USA. [Van Berkel, Gary J.; Kertesz, Vilmos] Oak Ridge Natl Lab, Div Chem Sci, Organ & Biol Mass Spectrometry Grp, Oak Ridge, TN 37831 USA. RP Gan, JP (reprint author), Bristol Myers Squibb Res & Dev, Pharmaceut Candidate Optimizat, Princeton, NJ 08543 USA.; Kertesz, V (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Organ & Biol Mass Spectrometry Grp, Oak Ridge, TN 37831 USA. EM kerteszv@ornl.gov; jinping.gan@bms.com RI Kertesz, Vilmos/M-8357-2016; OI Kertesz, Vilmos/0000-0003-0186-5797; Gan, Jinping/0000-0002-7072-7614 FU Cooperative Research and Development Agreement with Sciex (CRADA) [NFE-10-02966]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division FX W.C., L.W. and J.G. would like to thank Mr. Markus Fancher and the Technical Support Unit at Bristol-Myers Squibb for assistance in animal handling and dosing. Support for V.K. and G.J.V.B. was provided through a Cooperative Research and Development Agreement with Sciex (CRADA NFE-10-02966). The software package LMJ Points Plus (c) V2.98 was previously developed with support from the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. NR 28 TC 2 Z9 2 U1 1 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0021-9673 EI 1873-3778 J9 J CHROMATOGR A JI J. Chromatogr. A PD MAR 25 PY 2016 VL 1439 BP 137 EP 143 DI 10.1016/j.chroma.2015.10.093 PG 7 WC Biochemical Research Methods; Chemistry, Analytical SC Biochemistry & Molecular Biology; Chemistry GA DH3GS UT WOS:000372676100013 PM 26589943 ER PT J AU Goddard, PA Singleton, J Franke, I Moller, JS Lancaster, T Steele, AJ Topping, CV Blundell, SJ Pratt, FL Baines, C Bendix, J McDonald, RD Brambleby, J Lees, MR Lapidus, SH Stephens, PW Twamley, BW Conner, MM Funk, K Corbey, JF Tran, HE Schlueter, JA Manson, JL AF Goddard, Paul A. Singleton, John Franke, Isabel Moeller, Johannes S. Lancaster, Tom Steele, Andrew J. Topping, Craig V. Blundell, Stephen J. Pratt, Francis L. Baines, C. Bendix, Jesper McDonald, Ross D. Brambleby, Jamie Lees, Martin R. Lapidus, Saul H. Stephens, Peter W. Twamley, Brendan W. Conner, Marianne M. Funk, Kylee Corbey, Jordan F. Tran, Hope E. Schlueter, J. A. Manson, Jamie L. TI Control of the third dimension in copper-based square-lattice antiferromagnets SO PHYSICAL REVIEW B LA English DT Article ID HEISENBERG-ANTIFERROMAGNET; MAGNETIC-PROPERTIES; LOW-TEMPERATURES; EXCHANGE; PYRAZINE; STATE; SUPEREXCHANGE; PERCHLORATE; BEHAVIOR; IONS AB Using a mixed-ligand synthetic scheme, we create a family of quasi-two-dimensional antiferromagnets, namely, [Cu(HF2)(pyz)(2)]ClO4 [pyz = pyrazine], [CuL2(pyz)(2)](ClO4)(2) [L = pyO = pyridine-N-oxide and 4-phpy-O = 4-phenylpyridine-N-oxide. These materials are shown to possess equivalent two-dimensional [Cu(pyz)(2)](2+) nearly square layers, but exhibit interlayer spacings that vary from 6.5713 to 16.777 angstrom, as dictated by the axial ligands. We present the structural and magnetic properties of this family as determined via x-ray diffraction, electron-spin resonance, pulsed-and quasistatic-field magnetometry and muon-spin rotation, and compare them to those of the prototypical two-dimensional magnetic polymer Cu(pyz)(2)(ClO4)(2). We find that, within the limits of the experimental error, the two-dimensional, intralayer exchange coupling in our family of materials remains largely unaffected by the axial ligand substitution, while the observed magnetic ordering temperature (1.91 K for the material with the HF2 axial ligand, 1.70 K for the pyO and 1.63 K for the 4-phpy-O) decreases slowly with increasing layer separation. Despite the structural motifs common to this family and Cu(pyz)(2)(ClO4)(2), the latter has significantly stronger two-dimensional exchange interactions and hence a higher ordering temperature. We discuss these results, as well as the mechanisms that might drive the long-range order in these materials, in terms of departures from the ideal S = 1/2 two-dimensional square-lattice Heisenberg antiferromagnet. In particular, we find that both spin-exchange anisotropy in the intralayer interaction and interlayer couplings (exchange, dipolar, or both) are needed to account for the observed ordering temperatures, with the intralayer anisotropy becoming more important as the layers are pulled further apart. C1 [Goddard, Paul A.; Brambleby, Jamie; Lees, Martin R.] Univ Warwick, Dept Phys, Gibbet Hill Rd, Coventry CV4 7AL, W Midlands, England. [Singleton, John; McDonald, Ross D.] Los Alamos Natl Lab, Natl High Magnet Field Lab, MS-E536, Los Alamos, NM 87545 USA. [Singleton, John; Franke, Isabel; Moeller, Johannes S.; Steele, Andrew J.; Topping, Craig V.; Blundell, Stephen J.] Univ Oxford, Dept Phys, Clarendon Lab, Parks Rd, Oxford OX1 3PU, England. [Lancaster, Tom] Univ Durham, Dept Phys, South Rd, Durham DH1 3LE, England. [Pratt, Francis L.] STFC Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Baines, C.] Paul Scherrer Inst, Lab Muon Spin Spect, CH-5232 Villigen, Switzerland. [Bendix, Jesper] Univ Copenhagen, Dept Chem, DK-2100 Copenhagen, Denmark. [Lapidus, Saul H.; Stephens, Peter W.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Lapidus, Saul H.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Lemont, IL 60439 USA. [Twamley, Brendan W.] Univ Idaho, Univ Res Off, Moscow, ID 83844 USA. [Conner, Marianne M.; Corbey, Jordan F.; Tran, Hope E.; Manson, Jamie L.] Eastern Washington Univ, Dept Chem & Biochem, Cheney, WA 99004 USA. [Funk, Kylee; Schlueter, J. A.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Franke, Isabel] Helios, 29 Hercules Way,Aerosp Blvd,Aero Pk, Farnborough GU14 6UU, Hants, England. [Moeller, Johannes S.] ETH, Solid State Phys Lab, Neutron Scattering & Magnetism, CH-8093 Zurich, Switzerland. RP Goddard, PA (reprint author), Univ Warwick, Dept Phys, Gibbet Hill Rd, Coventry CV4 7AL, W Midlands, England.; Manson, JL (reprint author), Eastern Washington Univ, Dept Chem & Biochem, Cheney, WA 99004 USA. EM p.goddard@warwick.ac.uk; jmanson@ewu.edu RI Lees, Martin/D-9584-2013; Goddard, Paul/A-8638-2015 OI Lees, Martin/0000-0002-2270-2295; Goddard, Paul/0000-0002-0666-5236 FU Engineering and Physical Sciences Research Council (EPSRC); National Science Foundation [DMR-1306158, DMR-1157490]; State of Florida; US Department of Energy (DoE) through the DoE Basic Energy Science Field Work Proposal "Science in 100 T" FX Work done in the UK is supported by the Engineering and Physical Sciences Research Council (EPSRC). Data presented in this paper resulting from the UK effort will be made available at http://wrap.warwick.ac.uk/77684. The work at EWU was supported by the National Science Foundation under grant no. DMR-1306158. A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by National Science Foundation Cooperative Agreement No. DMR-1157490, the State of Florida, and the US Department of Energy (DoE) and through the DoE Basic Energy Science Field Work Proposal "Science in 100 T". Part of this work was carried out at the STFC ISIS Facility, Rutheford Appleton Laboratory (UK) and at the Swiss Muon Source, Paul Scherrer Institut (Switzerland); we are very grateful for the provision of beamtime. JS thanks the University of Oxford for provision of a visiting professorship, which was vital to the completion of this manuscript. NR 70 TC 2 Z9 2 U1 5 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 25 PY 2016 VL 93 IS 9 AR 094430 DI 10.1103/PhysRevB.93.094430 PG 15 WC Physics, Condensed Matter SC Physics GA DH3UK UT WOS:000372712100002 ER PT J AU Bramante, J Desai, N Fox, P Martin, A Ostdiek, B Plehn, T AF Bramante, Joseph Desai, Nishita Fox, Patrick Martin, Adam Ostdiek, Bryan Plehn, Tilman TI Towards the final word on neutralino dark matter SO PHYSICAL REVIEW D LA English DT Article ID LIGHTEST SUPERSYMMETRIC PARTICLE; LHC RUN 1; STAU COANNIHILATION; SPLIT SUPERSYMMETRY; HADRON COLLIDERS; MEASURING MASSES; RELIC DENSITY; 2 PHOTONS; ANNIHILATION; CHARGINOS AB We present a complete phenomenological prospectus for thermal relic neutralinos. Including Sommerfeld enhancements to relic abundance and halo annihilation calculations, we obtain direct, indirect, and collider discovery prospects for all neutralinos with mass parameters M-1, M-2, vertical bar mu vertical bar < 4 TeV, which freeze out to the observed dark matter abundance, with scalar superpartners decoupled. Much of the relic neutralino sector will be uncovered by the direct detection experiments Xenon1T and LZ, as well as indirect detection with Cerenkov Telescope Array. We emphasize that thermal relic Higgsinos will be found by next-generation direct detection experiments, so long as M-1,M-2 < 4 TeV. Charged tracks at a 100 TeV hadron collider complement indirect searches for relic winos. Thermal relic bino-winos still evade all planned experiments, including disappearing charged-track searches. However, they can be discovered by compressed electroweakino searches at a 100 TeV collider, completing the full coverage of the relic neutralino surface. C1 [Bramante, Joseph; Martin, Adam; Ostdiek, Bryan] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Desai, Nishita; Plehn, Tilman] Heidelberg Univ, Inst Theoret Phys, D-69120 Heidelberg, Germany. [Fox, Patrick] Fermilab Natl Accelerator Lab, Dept Theoret Phys, Batavia, IL 60510 USA. [Ostdiek, Bryan] Univ Oregon, Dept Phys, Eugene, OR 97403 USA. RP Bramante, J (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. FU CETUP; National Science Foundation [PHY-1066293, PHY-1417118]; Alexander von Humboldt Foundation; U.S. Department of Energy [DE-SC0011640]; Aspen Center for Physics FX We thank Andrzsej Hryczuk for useful correspondence and the use of DARKSE. We would also like to thank Zhenyu Han and Graham Kribs for useful discussions. J. B. thanks CETUP for hospitality and support, as well as the Aspen Center for Physics, which is supported by National Science Foundation Grant No. PHY-1066293. N. D. was partially supported by the Alexander von Humboldt Foundation. B. O. was partially supported by the U.S. Department of Energy under Grant No. DE-SC0011640. The work of A. M. was partially supported by the National Science Foundation under Grant No. PHY-1417118. We specifically acknowledge the assistance of the Notre Dame Center for Research Computing for computing resources. NR 200 TC 7 Z9 7 U1 0 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 25 PY 2016 VL 93 IS 6 AR 063525 DI 10.1103/PhysRevD.93.063525 PG 15 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH3YS UT WOS:000372723300002 ER PT J AU Bulgac, A Magierski, P Roche, KJ Stetcu, I AF Bulgac, Aurel Magierski, Piotr Roche, Kenneth J. Stetcu, Ionel TI Induced Fission of Pu-240 within a Real-Time Microscopic Framework SO PHYSICAL REVIEW LETTERS LA English DT Article ID DENSITY-FUNCTIONAL THEORY; ONE-BODY DISSIPATION; NUCLEAR-FISSION; DYNAMICS; MOTION; SUPERCONDUCTIVITY; DISINTEGRATION; SUPERFLUID; SCISSION; LIBRARY AB We describe the fissioning dynamics of Pu-240 from a configuration in the proximity of the outer fission barrier to full scission and the formation of the fragments within an implementation of density functional theory extended to superfluid systems and real-time dynamics. The fission fragments emerge with properties similar to those determined experimentally, while the fission dynamics appears to be quite complex, with many excited shape and pairing modes. The evolution is found to be much slower than previously expected, and the ultimate role of the collective inertia is found to be negligible in this fully nonadiabatic treatment of nuclear dynamics, where all collective degrees of freedom (CDOF) are included (unlike adiabatic treatments with a small number of CDOF). C1 [Bulgac, Aurel; Magierski, Piotr; Roche, Kenneth J.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Magierski, Piotr] Warsaw Univ Technol, Fac Phys, Ulica Koszykowa 75, PL-00662 Warsaw, Poland. [Roche, Kenneth J.] Pacific NW Natl Lab, Richland, WA 99352 USA. [Stetcu, Ionel] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Bulgac, A (reprint author), Univ Washington, Dept Phys, Seattle, WA 98195 USA. FU U.S. Department of Energy (DOE) [DE-FG02-97ER41014]; Polish National Science Center (NCN) [UMO-2013/08/A/ST3/00708, UMO-2012/07/B/ST2/03907]; U.S. Department of Energy through an Early Career Award of the LANL/LDRD Program; DOE Office of Science [DE-AC05-00OR22725]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX We have greatly benefited from numerous discussions with G. F. Bertsch and, over the years, from interactions with A. B. Migdal, P. Moller, J. Randrup, A. Sierk, W. J. Swiatecki, and P. Talou. We thank J. Wells for his continuous support. We thank G. F. Bertsch, A. Sierk, and P. Talou for their careful reading of the manuscript and suggestions as well as the referees for their very thoughtful suggestions. This work was supported in part by U.S. Department of Energy (DOE) Grant No. DE-FG02-97ER41014 and the Polish National Science Center (NCN) under Contracts No. UMO-2013/08/A/ST3/00708 and No. UMO-2012/07/B/ST2/03907. I. S. gratefully acknowledges the partial support of the U.S. Department of Energy through an Early Career Award of the LANL/LDRD Program. Calculations have been performed at the OLCF Titan [70] and at NERSC Edison. This research used resources of the Oak Ridge Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract No. DE-AC05-00OR22725, and the research also used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 102 TC 11 Z9 11 U1 6 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 25 PY 2016 VL 116 IS 12 AR 122504 DI 10.1103/PhysRevLett.116.122504 PG 7 WC Physics, Multidisciplinary SC Physics GA DH4BF UT WOS:000372729800003 PM 27058076 ER PT J AU Coleman, MA Cappuccio, JA Blanchette, CD Gao, TJ Arroyo, ES Hinz, AK Bourguet, FA Segelke, B Hoeprich, PD Huser, T Laurence, TA Motin, VL Chromy, BA AF Coleman, Matthew A. Cappuccio, Jenny A. Blanchette, Craig D. Gao, Tingjuan Arroyo, Erin S. Hinz, Angela K. Bourguet, Feliza A. Segelke, Brent Hoeprich, Paul D. Huser, Thomas Laurence, Ted A. Motin, Vladimir L. Chromy, Brett A. TI Expression and Association of the Yersinia pestis Translocon Proteins, YopB and YopD, Are Facilitated by Nanolipoprotein Particles SO PLOS ONE LA English DT Article ID CELL-FREE EXPRESSION; MEMBRANE-PROTEIN; OUTER PROTEINS; V-ANTIGEN; SECRETION; PSEUDOTUBERCULOSIS; INFECTION; SYSTEM; PLAGUE; LCRV AB Yersinia pestis enters host cells and evades host defenses, in part, through interactions between Yersinia pestis proteins and host membranes. One such interaction is through the type III secretion system, which uses a highly conserved and ordered complex for Yersinia pestis outer membrane effector protein translocation called the injectisome. The portion of the injectisome that interacts directly with host cell membranes is referred to as the translocon. The translocon is believed to form a pore allowing effector molecules to enter host cells. To facilitate mechanistic studies of the translocon, we have developed a cell-free approach for expressing translocon pore proteins as a complex supported in a bilayer membrane mimetic nano-scaffold known as a nanolipoprotein particle (NLP) Initial results show cell-free expression of Yersinia pestis outer membrane proteins YopB and YopD was enhanced in the presence of liposomes. However, these complexes tended to aggregate and precipitate. With the addition of co-expressed (NLP) forming components, the YopB and/or YopD complex was rendered soluble, increasing the yield of protein for biophysical studies. Biophysical methods such as Atomic Force Microscopy and Fluorescence Correlation Spectroscopy were used to confirm that the soluble YopB/D complex was associated with NLPs. An interaction between the YopB/D complex and NLP was validated by immunoprecipitation. The YopB/D translocon complex embedded in a NLP provides a platform for protein interaction studies between pathogen and host proteins. These studies will help elucidate the poorly understood mechanism which enables this pathogen to inject effector proteins into host cells, thus evading host defenses. C1 [Coleman, Matthew A.; Blanchette, Craig D.; Arroyo, Erin S.; Hinz, Angela K.; Bourguet, Feliza A.; Segelke, Brent; Hoeprich, Paul D.; Laurence, Ted A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Coleman, Matthew A.; Gao, Tingjuan; Huser, Thomas; Chromy, Brett A.] Univ Calif Davis, NSF, Ctr Biophoton, Sacramento, CA 95817 USA. [Cappuccio, Jenny A.] Humboldt State Univ, Dept Chem, Arcata, CA 95521 USA. [Motin, Vladimir L.] Univ Texas Med Branch, Galveston, TX 77555 USA. RP Coleman, MA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.; Coleman, MA; Chromy, BA (reprint author), Univ Calif Davis, NSF, Ctr Biophoton, Sacramento, CA 95817 USA. EM coleman16@llnl.gov; bachromy@ucdavis.edu RI Motin, Vladimir/O-1535-2013; OI Coleman, Matthew/0000-0003-1389-4018 FU Laboratory Directed Research and Development Office [06-SI-003, 01-ERD-045]; National Science Foundation through the Center for Biophotonics Science and Technology Center [PHY 0120999]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Laboratory Directed Research; NSF [PHY 0120999] FX Laboratory Directed Research and Development Office Grants 06-SI-003 and 01-ERD-045. National Science Foundation through the Center for Biophotonics Science and Technology Center, managed by the University of California Davis under Cooperative Agreement No. PHY 0120999.; This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and support from the Laboratory Directed Research. Part of the work was also performed at the NSF Center for Biophotonics, an NSF Science and Technology Center, which is managed by the University of California, Davis, under cooperative agreement no. PHY 0120999 with the NSF. The authors are grateful to Dr. Gregory Plano for his generous donation of the YopD antibodies. NR 35 TC 0 Z9 0 U1 1 U2 8 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 25 PY 2016 VL 11 IS 3 AR e0150166 DI 10.1371/journal.pone.0150166 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH3TE UT WOS:000372708900020 PM 27015536 ER PT J AU Kim, JW Brawley, SH Prochnik, S Chovatia, M Grimwood, J Jenkins, J LaButti, K Mavromatis, K Nolan, M Zane, M Schmutz, J Stiller, JW Grossman, AR AF Kim, Jay W. Brawley, Susan H. Prochnik, Simon Chovatia, Mansi Grimwood, Jane Jenkins, Jerry LaButti, Kurt Mavromatis, Konstantinos Nolan, Matt Zane, Matthew Schmutz, Jeremy Stiller, John W. Grossman, Arthur R. TI Genome Analysis of Planctomycetes Inhabiting Blades of the Red Alga Porphyra umbilicalis SO PLOS ONE LA English DT Article ID BACTERIUM ZOBELLIA-GALACTANIVORANS; MARINE BACTERIUM; AUREOCOCCUS-ANOPHAGEFFERENS; GLYCOSIDE HYDROLASES; ESCHERICHIA-COLI; OXIDATIVE STRESS; BETA-AGARASES; CELL-WALLS; SP-NOV; EVOLUTION AB Porphyra is a macrophytic red alga of the Bangiales that is important ecologically and economically. We describe the genomes of three bacteria in the phylum Planctomycetes (designated P1, P2 and P3) that were isolated from blades of Porphyra umbilicalis (P. um. 1). These three Operational Taxonomic Units (OTUs) belong to distinct genera; P2 belongs to the genus Rhodopirellula, while P1 and P3 represent undescribed genera within the Planctomycetes. Comparative analyses of the P1, P2 and P3 genomes show large expansions of distinct gene families, which can be widespread throughout the Planctomycetes (e.g., protein kinases, sensors/response regulators) and may relate to specific habitat (e.g., sulfatase gene expansions in marine Planctomycetes) or phylogenetic position. Notably, there are major differences among the Planctomycetes in the numbers and sub-functional diversity of enzymes (e.g., sulfatases, glycoside hydrolases, polysaccharide lyases) that allow these bacteria to access a range of sulfated polysaccharides in macroalgal cell walls. These differences suggest that the microbes have varied capacities for feeding on fixed carbon in the cell walls of P. um. 1 and other macrophytic algae, although the activities among the various bacteria might be functionally complementary in situ. Additionally, phylogenetic analyses indicate augmentation of gene functions through expansions arising from gene duplications and horizontal gene transfers; examples include genes involved in cell wall degradation (e.g., kappa-carrageenase, alginate lyase, fucosidase) and stress responses (e.g., efflux pump, amino acid transporter). Finally P1 and P2 contain various genes encoding selenoproteins, many of which are enzymes that ameliorate the impact of environmental stresses that occur in the intertidal habitat. C1 [Kim, Jay W.] Univ Calif Santa Cruz, Dept Biomol Engn, Santa Cruz, CA 95064 USA. [Brawley, Susan H.] Univ Maine, Sch Marine Sci, Orono, ME USA. [Prochnik, Simon; Chovatia, Mansi; Grimwood, Jane; Jenkins, Jerry; LaButti, Kurt; Mavromatis, Konstantinos; Nolan, Matt; Zane, Matthew; Schmutz, Jeremy] Joint Genome Inst, Dept Energy, Walnut Creek, CA USA. [Grimwood, Jane; Jenkins, Jerry; Schmutz, Jeremy] HudsonAlpha Inst Biotechnol, Huntsville, AL USA. [Stiller, John W.] E Carolina Univ, Dept Biol, Greenville, NC USA. [Grossman, Arthur R.] Carnegie Inst Sci, Dept Plant Biol, 290 Panama St, Stanford, CA 94305 USA. RP Kim, JW (reprint author), Univ Calif Santa Cruz, Dept Biomol Engn, Santa Cruz, CA 95064 USA. EM jay.wj.kim@gmail.com FU NSF Porphyra Research Collaboration Network grant [NSF IOS 074097]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX The study design, data collection and analysis for this work was supported by an NSF Porphyra Research Collaboration Network grant (NSF IOS 074097 to S. H. Brawley, E. Gantt, A. R. Grossman, J. Stiller). The work conducted by the Joint Genome Institute (Dept. of Energy), consisting of sequencing and assembly, was through a Community Science Program award from the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 (to SHB, EG, ARG, JS). NR 75 TC 1 Z9 1 U1 14 U2 21 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 25 PY 2016 VL 11 IS 3 AR e0151883 DI 10.1371/journal.pone.0151883 PG 22 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH3TE UT WOS:000372708900033 PM 27015628 ER PT J AU Cate, JHD AF Cate, Jamie H. D. TI STRUCTURE A Big Bang in spliceosome structural biology SO SCIENCE LA English DT Editorial Material ID U4/U6.U5 TRI-SNRNP; CRYO-EM; RESOLUTION C1 [Cate, Jamie H. D.] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [Cate, Jamie H. D.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Cate, Jamie H. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging, Berkeley, CA 94720 USA. RP Cate, JHD (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA.; Cate, JHD (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Cate, JHD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging, Berkeley, CA 94720 USA. EM jcate@lbl.gov NR 12 TC 1 Z9 1 U1 1 U2 7 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAR 25 PY 2016 VL 351 IS 6280 BP 1390 EP 1392 DI 10.1126/science.aaf3061 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH4KZ UT WOS:000372756200018 PM 27013712 ER PT J AU Ruehl, CR Davies, JF Wilson, KR AF Ruehl, Christopher R. Davies, James F. Wilson, Kevin R. TI An interfacial mechanism for cloud droplet formation on organic aerosols SO SCIENCE LA English DT Article ID CONDENSATION NUCLEI CCN; SURFACE-TENSION; HYGROSCOPIC GROWTH; SOLUBLE ORGANICS; ACTIVATION; PARTICLES; SITE AB Accurate predictions of aerosol/cloud interactions require simple, physically accurate parameterizations of the cloud condensation nuclei (CCN) activity of aerosols. Current models assume that organic aerosol species contribute to CCN activity by lowering water activity. We measured droplet diameters at the point of CCN activation for particles composed of dicarboxylic acids or secondary organic aerosol and ammonium sulfate. Droplet activation diameters were 40 to 60% larger than predicted if the organic was assumed to be dissolved within the bulk droplet, suggesting that a new mechanism is needed to explain cloud droplet formation. A compressed film model explains how surface tension depression by interfacial organic molecules can alter the relationship between water vapor supersaturation and droplet size (i.e., the Kohler curve), leading to the larger diameters observed at activation. C1 [Ruehl, Christopher R.; Davies, James F.; Wilson, Kevin R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Ruehl, Christopher R.] Calif Air Resources Board, Sacramento, CA USA. RP Ruehl, CR; Wilson, KR (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.; Ruehl, CR (reprint author), Calif Air Resources Board, Sacramento, CA USA. EM chris.ruehl@arb.ca.gov; krwilson@lbl.gov RI Davies, James/G-1113-2015 OI Davies, James/0000-0002-7415-3638 FU Office of Science Early Career Research Program, through the Office of Energy Research, Office of Basic Energy Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work is supported by the Office of Science Early Career Research Program, through the Office of Energy Research, Office of Basic Energy Science of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. The continuous-flow streamwise thermal gradient chamber was originally developed by Patrick Chuang and Anthanasios Nenes with support from NASA's Atmospheric Radiation Measurement program. NR 29 TC 15 Z9 15 U1 31 U2 82 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAR 25 PY 2016 VL 351 IS 6280 BP 1447 EP 1450 DI 10.1126/science.aad4889 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH4KZ UT WOS:000372756200048 PM 27013731 ER PT J AU Lejaeghere, K Bihlmayer, G Bjorkman, T Blaha, P Blugel, S Blum, V Caliste, D Castelli, IE Clark, SJ Dal Corso, A de Gironcoli, S Deutsch, T Dewhurst, JK Di Marco, I Draxl, C Dulak, M Eriksson, O Flores-Livas, JA Garrity, KF Genovese, L Giannozzi, P Giantomassi, M Goedecker, S Gonze, X Granas, O Gross, EKU Gulans, A Gygi, F Hamann, DR Hasnip, PJ Holzwarth, NAW Iusan, D Jochym, DB Jollet, F Jones, D Kresse, G Koepernik, K Kucukbenli, E Kvashnin, YO Locht, ILM Lubeck, S Marsman, M Marzari, N Nitzsche, U Nordstrom, L Ozaki, T Paulatto, L Pickard, CJ Poelmans, W Probert, MIJ Refson, K Richter, M Rignanese, GM Saha, S Scheffler, M Schlipf, M Schwarz, K Sharma, S Tavazza, F Thunstrom, P Tkatchenko, A Torrent, M Vanderbilt, D van Setten, MJ Van Speybroeck, V Wills, JM Yates, JR Zhang, GX Cottenier, S AF Lejaeghere, Kurt Bihlmayer, Gustav Bjoerkman, Torbjoern Blaha, Peter Bluegel, Stefan Blum, Volker Caliste, Damien Castelli, Ivano E. Clark, Stewart J. Dal Corso, Andrea de Gironcoli, Stefano Deutsch, Thierry Dewhurst, John Kay Di Marco, Igor Draxl, Claudia Dulak, Marcin Eriksson, Olle Flores-Livas, Jose A. Garrity, Kevin F. Genovese, Luigi Giannozzi, Paolo Giantomassi, Matteo Goedecker, Stefan Gonze, Xavier Granaes, Oscar Gross, E. K. U. Gulans, Andris Gygi, Francois Hamann, D. R. Hasnip, Phil J. Holzwarth, N. A. W. Iusan, Diana Jochym, Dominik B. Jollet, Francois Jones, Daniel Kresse, Georg Koepernik, Klaus Kuecuekbenli, Emine Kvashnin, Yaroslav O. Locht, Inka L. M. Lubeck, Sven Marsman, Martijn Marzari, Nicola Nitzsche, Ulrike Nordstrom, Lars Ozaki, Taisuke Paulatto, Lorenzo Pickard, Chris J. Poelmans, Ward Probert, Matt I. J. Refson, Keith Richter, Manuel Rignanese, Gian-Marco Saha, Santanu Scheffler, Matthias Schlipf, Martin Schwarz, Karlheinz Sharma, Sangeeta Tavazza, Francesca Thunstroem, Patrik Tkatchenko, Alexandre Torrent, Marc Vanderbilt, David van Setten, Michiel J. Van Speybroeck, Veronique Wills, John M. Yates, Jonathan R. Zhang, Guo-Xu Cottenier, Stefaan TI Reproducibility in density functional theory calculations of solids SO SCIENCE LA English DT Article ID GENERALIZED-GRADIENT APPROXIMATION; AUGMENTED-WAVE METHOD; REGULAR APPROXIMATIONS; PSEUDOPOTENTIALS; SILICON; STATE; 1ST-PRINCIPLES; CRYSTALS; SCIENCE; ENERGY AB The widespread popularity of density functional theory has given rise to an extensive range of dedicated codes for predicting molecular and crystalline properties. However, each code implements the formalism in a different way, raising questions about the reproducibility of such predictions. We report the results of a community-wide effort that compared 15 solid-state codes, using 40 different potentials or basis set types, to assess the quality of the Perdew-Burke-Ernzerhof equations of state for 71 elemental crystals. We conclude that predictions from recent codes and pseudopotentials agree very well, with pairwise differences that are comparable to those between different high-precision experiments. Older methods, however, have less precise agreement. Our benchmark provides a framework for users and developers to document the precision of new applications and methodological improvements. C1 [Lejaeghere, Kurt; Poelmans, Ward; Van Speybroeck, Veronique; Cottenier, Stefaan] Univ Ghent, Ctr Mol Modeling, Technol Pk 903, BE-9052 Zwijnaarde, Belgium. [Bihlmayer, Gustav; Bluegel, Stefan] Forschungszentrum Julich, Peter Grunberg Inst, D-52425 Julich, Germany. [Bihlmayer, Gustav; Bluegel, Stefan] Forschungszentrum Julich, Inst Adv Simulat, D-52425 Julich, Germany. [Bjoerkman, Torbjoern] Abo Akad Univ, Dept Phys, FI-20500 Turku, Finland. [Bjoerkman, Torbjoern] Aalto Univ, Sch Sci, Ctr Excellence Computat Nanosci, POB 11100, FI-00076 Aalto, Finland. [Bjoerkman, Torbjoern] Aalto Univ, Sch Sci, Dept Appl Phys, POB 11100, FI-00076 Aalto, Finland. [Blaha, Peter; Schwarz, Karlheinz] Vienna Univ Technol, Inst Mat Chem, Getreidemarkt 9-165-TC, A-1060 Vienna, Austria. [Blum, Volker] Duke Univ, Dept Mech Engn & Mat Sci, Durham, NC 27708 USA. [Caliste, Damien; Deutsch, Thierry; Genovese, Luigi] Univ Grenoble Alpes, Inst Nanosci, F-38042 Grenoble, France. [Caliste, Damien; Deutsch, Thierry; Genovese, Luigi] Cryogenie Modeling & Mat Explorat Dept INAC MEM, L Sim, F-38042 Grenoble, France. [Caliste, Damien; Deutsch, Thierry; Genovese, Luigi] CEA, L Sim, INAC MEM, F-38054 Grenoble, France. [Castelli, Ivano E.; Kuecuekbenli, Emine; Marzari, Nicola] Ecole Polytech Fed Lausanne, Theory & Simulat Mat THEOS, CH-1015 Lausanne, Switzerland. [Castelli, Ivano E.; Kuecuekbenli, Emine; Marzari, Nicola] Ecole Polytech Fed Lausanne, Natl Ctr Computat Design & Discovery Novel Mat MA, CH-1015 Lausanne, Switzerland. [Clark, Stewart J.] Univ Durham, Dept Phys, South Rd, Durham DH1 3LE, England. [Dal Corso, Andrea; de Gironcoli, Stefano; Kuecuekbenli, Emine] SISSA, Via Bonomea 265, I-34136 Trieste, Italy. [Dewhurst, John Kay; Flores-Livas, Jose A.; Gross, E. K. U.; Sharma, Sangeeta] Max Planck Inst Mikrostrukturphys, Weinberg 2, D-06120 Halle, Germany. [Di Marco, Igor; Eriksson, Olle; Iusan, Diana; Kvashnin, Yaroslav O.; Locht, Inka L. M.; Nordstrom, Lars] Uppsala Univ, Div Mat Theory, Dept Phys & Astron, POB 516, SE-75120 Uppsala, Sweden. [Draxl, Claudia; Gulans, Andris; Lubeck, Sven] Humboldt Univ, Inst Phys, Windkanal 6, D-12489 Berlin, Germany. [Draxl, Claudia; Gulans, Andris; Lubeck, Sven] Humboldt Univ, IRIS, Windkanal 6, D-12489 Berlin, Germany. [Draxl, Claudia; Gulans, Andris; Scheffler, Matthias; Tkatchenko, Alexandre] Max Planck Gesell, Fritz Haber Inst, Faradayweg 4-6, D-14195 Berlin, Germany. [Dulak, Marcin] Tech Univ Denmark, Dept Phys, Ctr Atom Scale Mat Design, DK-2800 Lyngby, Denmark. [Garrity, Kevin F.; Tavazza, Francesca] NIST, Mat Measurement Lab, 100 Bur Dr,Stop 8553, Gaithersburg, MD 20899 USA. [Giannozzi, Paolo; Granaes, Oscar] Univ Udine, Dept Math Comp Sci & Phys, Via Sci 206, I-33100 Udine, Italy. [Giantomassi, Matteo; Gonze, Xavier; Rignanese, Gian-Marco; van Setten, Michiel J.] Catholic Univ Louvain, Inst Condensed Matter & Nanosci Nanoscop, Chemin Etoiles 8, BE-1348 Louvain, Belgium. [Goedecker, Stefan; Saha, Santanu] Univ Basel, Inst Phys, Klingelbergstr 82, CH-4056 Basel, Switzerland. [Granaes, Oscar] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Gygi, Francois; Schlipf, Martin] Univ Calif Davis, Dept Comp Sci, Davis, CA 95616 USA. [Hamann, D. R.; Vanderbilt, David] Rutgers State Univ, Dept Phys, Piscataway, NJ 08854 USA. [Hamann, D. R.] Mat Sim Res, POB 742, Murray Hill, NJ 07974 USA. [Hasnip, Phil J.; Probert, Matt I. J.] Univ York, Dept Phys, York YO10 5DD, N Yorkshire, England. [Holzwarth, N. A. W.] Wake Forest Univ, Dept Phys, Winston Salem, NC 27109 USA. [Jochym, Dominik B.] Rutherford Appleton Lab, Sci & Technol Facil Council, Sci Comp Dept, Didcot OX11 0QX, Oxon, England. [Jollet, Francois; Torrent, Marc] DIF, DAM, CEA, F-91297 Arpajon, France. [Jones, Daniel; Yates, Jonathan R.] Univ Oxford, Dept Mat, 16 Parks Rd, Oxford OX1 3PH, England. [Kresse, Georg; Marsman, Martijn] Univ Vienna, Fac Phys, Sensengasse 8-12, A-1090 Vienna, Austria. [Kresse, Georg; Marsman, Martijn] Univ Vienna, Ctr Computat Mat Sci, Sensengasse 8-12, A-1090 Vienna, Austria. [Koepernik, Klaus; Nitzsche, Ulrike; Richter, Manuel] Leibniz Inst Festkorper & Werkstoffforsch IFW Dre, POB 270 116, D-01171 Dresden, Germany. [Koepernik, Klaus; Richter, Manuel] Tech Univ Dresden, Dresden Ctr Computat Mat Sci DCMS, D-01069 Dresden, Germany. [Locht, Inka L. M.] Radboud Univ Nijmegen, Inst Mol & Mat, Heyendaalseweg 135, NL-6525 AJ Nijmegen, Netherlands. [Ozaki, Taisuke] Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan. [Paulatto, Lorenzo] Univ Paris 06, IMPMC, CNRS, UMR 7590,Museum Natl Hist Nat,IRD,Unite Rech 206, 4 Pl Jussieu, F-75005 Paris, France. [Pickard, Chris J.] Univ Cambridge, Dept Mat Sci & Met, 27 Charles Babbage Rd, Cambridge CB3 0FS, England. [Poelmans, Ward] Univ Ghent, High Performance Comp Unit, Krijgslaan 281 S9, BE-9000 Ghent, Belgium. [Refson, Keith] Univ London, Royal Holloway & Bedford New Coll, Dept Phys, Egham TW20 0EX, Surrey, England. [Refson, Keith] Rutherford Appleton Lab, Sci & Technol Facil Council, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Scheffler, Matthias] Univ Calif Santa Barbara, Dept Chem & Biochem, Santa Barbara, CA 93106 USA. [Scheffler, Matthias] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. [Thunstroem, Patrik] Vienna Univ Technol, Inst Solid State Phys, A-1040 Vienna, Austria. [Tkatchenko, Alexandre] Univ Luxembourg, Phys & Mat Sci Res Unit, L-1511 Luxembourg, Luxembourg. [Wills, John M.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Zhang, Guo-Xu] Harbin Inst Technol, Sch Chem & Chem Engn, Inst Theoret & Simulat Chem, Harbin 150001, Peoples R China. [Cottenier, Stefaan] Univ Ghent, Dept Mat Sci & Engn, Technol Pk 903, BE-9052 Zwijnaarde, Belgium. RP Lejaeghere, K; Cottenier, S (reprint author), Univ Ghent, Ctr Mol Modeling, Technol Pk 903, BE-9052 Zwijnaarde, Belgium.; Cottenier, S (reprint author), Univ Ghent, Dept Mat Sci & Engn, Technol Pk 903, BE-9052 Zwijnaarde, Belgium. EM kurt.lejaeghere@ugent.be; stefaan.cottenier@ugent.be RI Paulatto, Lorenzo/E-3974-2016; Draxl, Claudia/O-6189-2016; TU Dresden, DCMS/B-7669-2015; Rignanese, Gian-Marco/A-7435-2008; Blaha, Peter/F-2847-2010; Deutsch, Thierry/A-6077-2009; Di Marco, Igor/O-5190-2014; van Setten, Michiel/B-2766-2008; Scheffler, Matthias/O-4649-2016; Bihlmayer, Gustav/G-5279-2013; Richter, Manuel/F-2485-2016; Genovese, Luigi/C-5937-2011; Dal Corso, Andrea/A-5745-2008; Blum, Volker/J-6591-2012; Iusan, Diana/C-2356-2011; Castelli, Ivano/N-1627-2015; Bjorkman, Torbjorn/B-9844-2012; OI Draxl, Claudia/0000-0003-3523-6657; TU Dresden, DCMS/0000-0003-1370-3074; Rignanese, Gian-Marco/0000-0002-1422-1205; Hasnip, Philip/0000-0002-4314-4093; Lejaeghere, Kurt/0000-0002-4462-8209; Caliste, Damien/0000-0002-4967-9275; Deutsch, Thierry/0000-0001-7503-3390; Di Marco, Igor/0000-0003-1714-0942; van Setten, Michiel/0000-0003-0557-5260; Bihlmayer, Gustav/0000-0002-6615-1122; Richter, Manuel/0000-0002-9999-8290; Genovese, Luigi/0000-0003-1747-0247; Blum, Volker/0000-0001-8660-7230; Iusan, Diana/0000-0001-7467-9317; Castelli, Ivano/0000-0001-5880-5045; Bjorkman, Torbjorn/0000-0002-1154-9846; Poelmans, Ward/0000-0002-0399-3613 FU Research Board of Ghent University; Fond de la Recherche Scientifique de Belgique (FRS-FNRS) through Projet de Recherches (PDR) [T.0238.13-AIXPHO, T.1031.14-HiT4FiT]; Communaute Francaise de Belgique through BATTAB project [ARC 14/19-057]; U.S. NSF [DMR-14-08838, DMR-1105485]; Swedish Research Council; Knut and Alice Wallenberg Foundation [2013.0020, 2012.0031]; Fund for Scientific Research-Flanders (FWO) [G0E0116N]; U.S. Department of Energy [DOE-BES DE-SC0008938]; European Union [329386, 676580]; eSSENCE; Academy of Finland [263416]; COMP Centre of Excellence; Deutsche Forschungsgemeinschaft (DFG); Einstein Foundation, Berlin; Novel Materials Discovery (NOMAD) Laboratory, a European Center of Excellence; Italian Ministry of Education, Universities, and Research (MIUR) through PRIN [20105ZZTSE_005]; Engineering and Physical Sciences Research Council (EPSRC) under UK Car-Parrinello (UKCP) grant [EP/K013564/1]; Collaborative Computational Project for NMR Crystallography under EPSRC grant [EP/J010510/1]; FWO; EPSRC [EP/J017639/1]; Swiss National Science Foundation (SNSF); FRS-FNRS; SNSF's National Centre of Competence in Research MARVEL; Austrian Science Fund [SFB-F41]; OCAS NV by an OCAS-endowed chair at Ghent University; Ghent University; Flemish Government (Economy, Science, and Innovation Department); Walloon Region [1117545]; FRS-FNRS [2.5020.11]; CASTEP by Biovia FX This research benefited from financial support from the Research Board of Ghent University; the Fond de la Recherche Scientifique de Belgique (FRS-FNRS), through Projet de Recherches (PDR) grants T.0238.13-AIXPHO and T.1031.14-HiT4FiT; the Communaute Francaise de Belgique, through the BATTAB project (grant ARC 14/19-057); the U.S. NSF (grant DMR-14-08838); the Swedish Research Council; the Knut and Alice Wallenberg Foundation (grants 2013.0020 and 2012.0031); the Fund for Scientific Research-Flanders (FWO) (project no. G0E0116N); and the U.S. Department of Energy (grant DOE-BES DE-SC0008938). N.A.W.H. was supported by U.S. NSF grant DMR-1105485. J.A.F.-L. acknowledges financial support from the European Union's 7th Framework Marie-Curie Scholarship Program within the ExMaMa Project (project no. 329386). I.D.M., O.E., O.G., D.I., Y.O.K., I.L.M.L., and L.N. acknowledge support from eSSENCE. T.B. was supported by the Academy of Finland (grant 263416) and the COMP Centre of Excellence. C.D., A.G., and S.L. acknowledge support from the Deutsche Forschungsgemeinschaft (DFG) and the Einstein Foundation, Berlin. M.Sche. and C.D. received funding from the European Union's Horizon 2020 research and innovation program under grant agreement no. 676580 with The Novel Materials Discovery (NOMAD) Laboratory, a European Center of Excellence. A.D.C., S.d.G., and E.K. acknowledge support from the Italian Ministry of Education, Universities, and Research (MIUR) through PRIN (Projects of National Interest) 2010-2011 (registration no. 20105ZZTSE_005). P.J.H., D.B.J., and M.I.J.P. are grateful for financial support by the Engineering and Physical Sciences Research Council (EPSRC) under UK Car-Parrinello (UKCP) grant EP/K013564/1. C.J.P. and J.R.Y. acknowledge support from the Collaborative Computational Project for NMR Crystallography under EPSRC grant EP/J010510/1. W.P. acknowledges funding by FWO. D.J. is grateful for financial support by EPSRC under grant EP/J017639/1. S.Sa. acknowledges support from the Swiss National Science Foundation (SNSF). G.-M.R. is thankful for personal financial support from FRS-FNRS. The work by I.E.C. and N.M. was supported by the SNSF's National Centre of Competence in Research MARVEL. G.K. and P.B. acknowledge support by the Austrian Science Fund, project SFB-F41 (ViCoM). S.C. acknowledges financial support from OCAS NV by an OCAS-endowed chair at Ghent University. Computational resources were as follows: The Ghent University contributors used the Stevin Supercomputer Infrastructure at Ghent University, which is funded by Ghent University, FWO, and the Flemish Government (Economy, Science, and Innovation Department). The Universite Catholique de Louvain contributors used the Tier-1 supercomputer of the Federation Wallonie-Bruxelles (funded by the Walloon Region under grant agreement no. 1117545), the Centre de Calcul Intensif et de Stockage de Masse-Universite Catholique de Louvain supercomputing facilities, and the Consortium des Equipements de Calcul Intensif en Federation Wallonie-Bruxelles (CECI) (funded by the FRS-FNRS under convention 2.5020.11). The Science and Technology Facilities Council, Scientific Computing Department's SCARF (Scientific Computing Application Resource for Facilities) cluster was used for the CASTEP calculations. The Basel University and Ecole Polytechnique Federale de Lausanne contributors used the Swiss National Supercomputing Center in Lugano. Finland's IT Centre for Science was used for the RSPt calculations. K.L. and F.T. thank C.; Becker for instructive discussions on the comparison of atomic-scale simulations. K.L. and S.C. thank W. Dewitte for drafting the summary figure. S.J.C., P.J.H., C.J.P., M.I.J.P., K.R., and J.R.Y. declare the receipt of income from commercial sales of CASTEP by Biovia. N.M. and M.Sche. are members of the Board of Trustees of the Psi-k Electronic Structure Network. P.G. is director of the Quantum ESPRESSO Foundation, and N.M. is a representative member. X.G., D.R.H., M.T., D.C., F.J., and G.-M.R. are members of the Advisory Board of ABINIT, an organization that develops and publishes open-source software related to this article. Commercial software is identified to specify procedures. Such identification does not imply recommendation by the National Institute of Standards and Technology. Atomic Simulation Environment scripts (46) for several of the codes are available online (48). All data are listed in tables S3 to S42. NR 61 TC 69 Z9 70 U1 69 U2 177 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAR 25 PY 2016 VL 351 IS 6280 AR aad3000 DI 10.1126/science.aad3000 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH4KZ UT WOS:000372756200038 ER PT J AU Simmhan, Y Ramakrishnan, L Antoniu, G Goble, C AF Simmhan, Yogesh Ramakrishnan, Lavanya Antoniu, Gabriel Goble, Carole TI Cloud computing for data-driven science and engineering SO CONCURRENCY AND COMPUTATION-PRACTICE & EXPERIENCE LA English DT Editorial Material C1 [Simmhan, Yogesh] Indian Inst Sci, Bangalore 560012, Karnataka, India. [Ramakrishnan, Lavanya] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Antoniu, Gabriel] Inria, Rennes, France. [Goble, Carole] Univ Manchester, Manchester, Lancs, England. RP Simmhan, Y (reprint author), Indian Inst Sci, Bangalore 560012, Karnataka, India. EM simmhan@serc.iisc.in OI Simmhan, Yogesh/0000-0003-4140-7774 NR 6 TC 0 Z9 0 U1 0 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1532-0626 EI 1532-0634 J9 CONCURR COMP-PRACT E JI Concurr. Comput.-Pract. Exp. PD MAR 25 PY 2016 VL 28 IS 4 SI SI BP 947 EP 949 DI 10.1002/cpe.3668 PG 3 WC Computer Science, Software Engineering; Computer Science, Theory & Methods SC Computer Science GA DE5BR UT WOS:000370646300001 ER PT J AU Beland, LK Samolyuk, GD Stoller, RE AF Beland, Laurent Karim Samolyuk, German D. Stoller, Roger E. TI Differences in the accumulation of ion-beam damage in Ni and NiFe explained by atomistic simulations SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Atomistic modelling; Radiation damage; Concentrated alloy; Nickel; Iron ID ACTIVATION-RELAXATION TECHNIQUE; MOLECULAR-DYNAMICS; ALGORITHMS; ENERGY AB Following low-dose irradiation with a 3 MeV beam of Au ions, i.e. less than one displacement per atom, a lower number of defects were experimentally observed in NiFe than in pure Ni. At higher doses, more damage is observed in NiFe than in pure Ni. Also, at these high doses, defect structures are observed deep in the material, far from the region where ions are implanted, more so in Ni than in NiFe. In this study, these experimental results are explained using atomistic modeling. Sequences of overlapping displacement cascades with intervening defect aging are simulated. Evidence is provided that nanosecond aging at 900 K can be used as a surrogate for long-time, room-temperature aging. Then, using this procedure, it is shown that the low defect diffusivity of NiFe leads to less aggregation and recombination events between each displacement cascade in a given volume than in Ni. Variations in the local defect chemistry in NiFe produces a broad spectrum of defect formation energy, leading to the trapping of defects at energetically favorable sites: this explains the low defect diffusivity. Also, this low diffusivity explains why, at high dose, defects in NiFe do not propagate as deeply in the material than in pure Ni. (C) 2015 Elsevier B.V. All rights reserved. C1 [Beland, Laurent Karim; Samolyuk, German D.; Stoller, Roger E.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Beland, LK (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM belandlk@ornl.gov FU Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences; Fonds Quebecois de recherche Nature et Technologies FX This work was supported as part of the Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. LKB acknowledges additional support from a fellowship awarded by the Fonds Quebecois de recherche Nature et Technologies. We thank Alexandre Barachev, Ke Jin, and Raina Olsen for insightful discussions. NR 31 TC 7 Z9 7 U1 3 U2 23 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD MAR 25 PY 2016 VL 662 BP 415 EP 420 DI 10.1016/j.jallcom.2015.11.185 PG 6 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA DB2KF UT WOS:000368336200057 ER PT J AU Patil, RS Banerjee, D Zhang, C Thallapally, PK Atwood, JL AF Patil, Rahul S. Banerjee, Debasis Zhang, Chen Thallapally, Praveen K. Atwood, Jerry L. TI Selective CO2 Adsorption in a Supramolecular Organic Framework SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE CO2; gas sorption; hydrogen bonding; supramolecular organic frameworks; pyrogallol[4]arene ID CARBON-DIOXIDE CAPTURE; SEPARATION; CAPSULES; STORAGE; GAS; BIPYRIDINE; POROSITY; ZEOLITE; CRYSTAL; BINDING AB Considering the rapidly rising CO2 level, there is a constant need for versatile materials which can selectively adsorb CO2 at low cost. The quest for efficient sorptive materials is still on since the practical applications of conventional porous materials possess certain limitations. In that context, we designed, synthesized, and characterized two novel supramolecular organic frameworks based on C-pentylpyrogallol[4]arene (PgC(5)) with spacer molecules, such as 4,4-bipyridine (bpy). Highly optimized and symmetric intermolecular hydrogen-bonding interactions between the main building blocks and comparatively weak van der Waals interactions between solvent molecules and PgC(5) leads to the formation of robust extended frameworks, which withstand solvent evacuation from the crystal lattice. The evacuated framework shows excellent affinity for carbon dioxide over nitrogen and adsorbs ca. 3wt % of CO2 at ambient temperature and pressure. C1 [Patil, Rahul S.; Zhang, Chen; Atwood, Jerry L.] Univ Missouri, Dept Chem, 601 S Coll Ave, Columbia, MO 65211 USA. [Banerjee, Debasis; Thallapally, Praveen K.] Pacific NW Natl Lab, Fundamental & Comp Sci Directorate, Richland, WA 99352 USA. RP Atwood, JL (reprint author), Univ Missouri, Dept Chem, 601 S Coll Ave, Columbia, MO 65211 USA. EM AtwoodJ@missouri.edu OI Zhang, Chen/0000-0001-5552-1960 NR 35 TC 6 Z9 7 U1 24 U2 70 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAR 24 PY 2016 VL 55 IS 14 BP 4523 EP 4526 DI 10.1002/anie.201600658 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DH9RI UT WOS:000373133000019 PM 26934637 ER PT J AU Dunning, TH Xu, LT Takeshita, TY Lindquist, BA AF Dunning, Thom H., Jr. Xu, Lu T. Takeshita, Tyler Y. Lindquist, Beth A. TI Insights into the Electronic Structure of Molecules from Generalized Valence Bond Theory SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID IMPROVED QUANTUM-THEORY; D-ORBITAL PARTICIPATION; AB-INITIO CALCULATIONS; CASSCF WAVE-FUNCTIONS; GAUSSIAN-BASIS SETS; POINT-OF-VIEW; COUPLED-CLUSTER; CHEMICAL-BOND; POLYATOMIC-MOLECULES; INVERSION BARRIERS AB In this article we describe the unique insights into the electronic structure of molecules provided by generalized valence bond (GVB) theory. We consider selected prototypical hydrocarbons as well as a number of hypervalent molecules and a set of first- and second-row valence isoelectronic species. The GVB wave function is obtained by variationally optimizing the orbitals and spin coupling in the valence bond wave function. The GVB wave function is a generalization of the Hartree-Fock (HF) wave function, lifting the double occupancy restriction on a subset of the HF orbitals as well as the associated orthogonality and spin coupling constraints. The GVB wave function includes a major fraction (if not all) of the nondynamical correlation energy of a molecule. Because of this, GVB theory properly describes bond formation and can answer one of the most compelling questions in chemistry: How are atoms changed by molecular formation? We show that GVB theory provides a unified description of the nature of the bonding in all of the above molecular species as well as contributing new insights into the well-known, but poorly understood, first-row anomaly. C1 [Dunning, Thom H., Jr.; Xu, Lu T.; Takeshita, Tyler Y.; Lindquist, Beth A.] Univ Illinois, Dept Chem, 600 S Mathews Ave, Urbana, IL 61801 USA. [Dunning, Thom H., Jr.] Univ Washington, Northwest Inst Adv Comp, Pacific NW Natl Lab, 127 Sieg Hall, Seattle, WA 98195 USA. [Dunning, Thom H., Jr.] Univ Washington, Dept Chem, Seattle, WA 98195 USA. [Takeshita, Tyler Y.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Lindquist, Beth A.] Univ Texas Austin, Dept Chem Engn, Austin, TX 78712 USA. RP Dunning, TH (reprint author), Univ Illinois, Dept Chem, 600 S Mathews Ave, Urbana, IL 61801 USA.; Dunning, TH (reprint author), Univ Washington, Northwest Inst Adv Comp, Pacific NW Natl Lab, 127 Sieg Hall, Seattle, WA 98195 USA.; Dunning, TH (reprint author), Univ Washington, Dept Chem, Seattle, WA 98195 USA. EM thdjr@illinois.edu FU Distinguished Chair for Research Excellence in Chemistry; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign FX This work was supported by funding from the Distinguished Chair for Research Excellence in Chemistry and the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign. NR 163 TC 7 Z9 7 U1 10 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAR 24 PY 2016 VL 120 IS 11 BP 1763 EP 1778 DI 10.1021/acs.jpca.5b12335 PG 16 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DH7BL UT WOS:000372946100001 PM 26909685 ER PT J AU Markus, IM Jones, G Garcia, JM AF Markus, Isaac M. Jones, Gavin Garcia, Jeannette M. TI Investigation of Electrolyte Concentration Effects on the Performance of Lithium-Oxygen Batteries SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID LI-AIR BATTERIES; NONAQUEOUS LI-O-2 BATTERIES; KINETIC OVERPOTENTIALS; BASIS-SETS; LIMITATIONS; STABILITY; PEROXIDE; CATHODE; ENERGY; LI2O2 AB A combined experimental and computational study has been performed in order to elucidate the effect of electrolyte salt concentration on the performance of Li-O-2 batteries. Four electrolyte solutions with varying lithium triflimide (LiTFSI) content in 1;2-dimethoxyethane (DME) were studied to identify principal failure Mechanisms in Li-O-2 batteries for dilute and concentrated electrolytes (0.1 M to saturation) in cells cycled with high overpotentials and/or deep discharge. Quantitative F-19 NMR was employed to determine that in 0.1 M electrolyte solutions salt decomposition can contribute to limitations in cell recycling arising from low ionic conductivity due to a decrease in available soluble Li+ over multiple cycles. In contrast, increased salt decomposition in high-concentration electrolytes can result in cathode passivation by insoluble Li salts that impact capacity by hindering Li2O2 production and further inhibiting electronic conductivity. By employing first-principles calculations, we modeled different pathways for the decomposition of the TFSI anion and found that it was particularly susceptible to decomposition in its neutral state, for example, if H+ is present and bound to the TFSI anion. The cumulative results suggest that employing low-concentration electrolytes with more stable lithium salts are ideal for better cell performance. C1 [Markus, Isaac M.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Markus, Isaac M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA. [Jones, Gavin; Garcia, Jeannette M.] IBM Corp, Almaden Res Ctr, San Jose, CA 95120 USA. RP Markus, IM (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Markus, IM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA 94720 USA.; Garcia, JM (reprint author), IBM Corp, Almaden Res Ctr, San Jose, CA 95120 USA. EM isaac.markus@berkeley.edu; jmgarcia@us.ibm.com FU IBM; NSF FX I.M.M. acknowledges the Leading to Africa program sponsored by IBM for providing financial resources to conduct a summer research internship. In addition, I.M.M. thanks Dr. Don Bethune for help with DEMS, Ms. Leslie Thompson for SEM/EDS analysis, Dr. Jed Pitera for helpful scientific discussions, and Simona Dalmasso for assistance with cell assembly and testing. I.M.M acknowledges the support of the NSF graduate research fellowship program. NR 35 TC 5 Z9 5 U1 20 U2 48 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 24 PY 2016 VL 120 IS 11 BP 5949 EP 5957 DI 10.1021/acs.jpcc.6b01474 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH7BN UT WOS:000372946300012 ER PT J AU Dass, A Jones, T Rambukwella, M Crasto, D Gagnon, KJ Sementa, L De Vetta, M Baseggio, O Apra, E Stener, M Fortunelli, A AF Dass, Amala Jones, Tanya Rambukwella, Milan Crasto, David Gagnon, Kevin J. Sementa, Luca De Vetta, Martina Baseggio, Oscar Apra, Edoardo Stener, Mauro Fortunelli, Alessandro TI Crystal Structure and Theoretical Analysis of Green Gold Au-30(S-tBu)(18) Nanomolecules and Their Relation to Au30S(S-tBu)(18) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CLUSTER; EXCHANGE; AU-144(SCH2CH2PH)(60); PSEUDOPOTENTIALS; APPROXIMATION; NANOPARTICLE; MOLECULES; THIOLATE AB We report the complete X-ray crystallographic structure as determined through single-crystal X-ray diffraction and a thorough theoretical analysis of the green gold Au-30(S-tBu)(18). While the structure of Au30S(S-tBu)(18) with 19 sulfur atoms has been reported, the crystal structure of Au-30(S-tBu)(18) without the mu(3)-sulfur has remained elusive until now, though matrix-assisted laser desorption ionization mass spectrometry (MALDI-MS) and electrospray ionization mass spectrometry (ESI-MS) data unequivocally show its presence in abundance. The Au-30(S-tBu)(18) nanomolecule not only is distinct in its crystal structure but also has unique temperature-dependent optical properties. Structure determination allows a rigorous comparison and an excellent agreement with theoretical predictions of structure, stability, and optical response. C1 [Dass, Amala; Jones, Tanya; Rambukwella, Milan; Crasto, David] Univ Mississippi, Dept Chem & Biochem, Oxford, MS 38677 USA. [Gagnon, Kevin J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Sementa, Luca; Fortunelli, Alessandro] CNR, CNR ICCOM, I-56124 Pisa, Italy. [De Vetta, Martina; Baseggio, Oscar; Stener, Mauro] Univ Trieste, Dipartmento Sci Chim & Farmaceut, I-34127 Trieste, Italy. [Apra, Edoardo] Pacific NW Natl Lab, Environm Mol Sci Lab, POB 999,K8-91, Richland, WA 99352 USA. RP Dass, A (reprint author), Univ Mississippi, Dept Chem & Biochem, Oxford, MS 38677 USA. EM amal@olemiss.edu RI Apra, Edoardo/F-2135-2010; Stener, Mauro/B-7987-2014 OI Apra, Edoardo/0000-0001-5955-0734; Stener, Mauro/0000-0003-3700-7903 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Biological and Environmental Research; PNNL Institutional Computing at Pacific Northwest National Laboratory; [NSF-CHE-1255519] FX We gratefully acknowledge the funding for experimental research from NSF-CHE-1255519. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Computational research was performed in part using EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, and PNNL Institutional Computing at Pacific Northwest National Laboratory. NR 33 TC 7 Z9 7 U1 6 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 24 PY 2016 VL 120 IS 11 BP 6256 EP 6261 DI 10.1021/acs.jpcc.6b00062 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH7BN UT WOS:000372946300045 ER PT J AU Mamo, KA Yee, HU AF Mamo, Kiminad A. Yee, Ho-Ung TI Spin polarized photons from an axially charged plasma at weak coupling: Complete leading order SO PHYSICAL REVIEW D LA English DT Article ID HEAVY-ION COLLISIONS; QUARK-GLUON PLASMA; ODD BUBBLES; DYNAMICS AB In the presence of (approximately conserved) axial charge in the QCD plasma at finite temperature, the emitted photons are spin aligned, which is a unique P- and CP-odd signature of axial charge in the photon emission observables. We compute this "P-odd photon emission rate" in a weak coupling regime at a high temperature limit to complete leading order in the QCD coupling constant: the leading log as well as the constant under the log. As in the P-even total emission rate in the literature, the computation of the P-odd emission rate at leading order consists of three parts: (1) Compton and pair annihilation processes with hard momentum exchange, (2) soft t- and u-channel contributions with hard thermal loop resummation, (3) Landau-Pomeranchuk-Migdal resummation of collinear bremsstrahlung and pair annihilation. We present analytical and numerical evaluations of these contributions to our P-odd photon emission rate observable. C1 [Mamo, Kiminad A.; Yee, Ho-Ung] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Yee, Ho-Ung] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. RP Mamo, KA; Yee, HU (reprint author), Univ Illinois, Dept Phys, Chicago, IL 60607 USA.; Yee, HU (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. EM kabebe2@uic.edu; hyee@uic.edu NR 24 TC 1 Z9 1 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 24 PY 2016 VL 93 IS 6 AR 065053 DI 10.1103/PhysRevD.93.065053 PG 23 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH3YN UT WOS:000372722800007 ER PT J AU Petri, A Haiman, Z May, M AF Petri, Andrea Haiman, Zoltan May, Morgan TI Sample variance in weak lensing: How many simulations are required? SO PHYSICAL REVIEW D LA English DT Article ID SYNOPTIC SURVEY TELESCOPE; MATTER POWER SPECTRUM; SHEAR-PEAK STATISTICS; COVARIANCE-MATRIX; COSMIC SHEAR; COSMOLOGY; BARYONS; COUNTS; CONSTRAINTS; PREDICTIONS AB Constraining cosmology using weak gravitational lensing consists of comparing a measured feature vector of dimension N-b with its simulated counterpart. An accurate estimate of the N-b x N-b feature covariance matrix C is essential to obtain accurate parameter confidence intervals. When C is measured from a set of simulations, an important question is how large this set should be. To answer this question, we construct different ensembles of N-r realizations of the shear field, using a common randomization procedure that recycles the outputs from a smaller number N-s <= N-r of independent ray-tracing N-body simulations. We study parameter confidence intervals as a function of (N-s, N-r) in the range 1 <= N-s <= 200 and 1 <= N-r <= 10(5). Previous work [S. Dodelson and M. D. Schneider, Phys. Rev. D 88, 063537 (2013)] has shown that Gaussian noise in the feature vectors (from which the covariance is estimated) lead, at quadratic order, to an O (1/N-r) degradation of the parameter confidence intervals. Using a variety of lensing features measured in our simulations, including shear-shear power spectra and peak counts, we show that cubic and quartic covariance fluctuations lead to additional O (1/N-r(2)) error degradation that is not negligible when N-r is only a factor of few larger than N-b. We study the large Nr limit, and find that a single, 240 Mpc/h sized 512(3)-particle N-body simulation (N-s = 1) can be repeatedly recycled to produce as many as N-r = few x 10(4) shear maps whose power spectra and high-significance peak counts can be treated as statistically independent. As a result, a small number of simulations (N-s = 1 or 2) is sufficient to forecast parameter confidence intervals at percent accuracy. C1 [Petri, Andrea] Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. [Petri, Andrea; May, Morgan] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Haiman, Zoltan] Columbia Univ, Dept Astron, New York, NY 10027 USA. RP Petri, A (reprint author), Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA.; Petri, A (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM apetri@phys.columbia.edu FU State of New York; U.S. Department of Energy [DE-AC02-98CH10886, DE-SC0012704]; NSF [AST-1210877]; Research Opportunities and Approaches to Data Science (ROADS) program at the Institute for Data Sciences and Engineering at Columbia University; [ACI-1053575] FX We thank Lam Hui for useful discussions. The simulations in this work were performed at the NSF XSEDE facility, supported by Grant No. ACI-1053575, and at the New York Center for Computational Sciences, a cooperative effort between Brookhaven National Laboratory and Stony Brook University, supported in part by the State of New York. This work was supported in part by the U.S. Department of Energy under Contracts No. DE-AC02-98CH10886 and NO. DE-SC0012704, and by the NSF Grant No. AST-1210877 (to Z.H.) and by the Research Opportunities and Approaches to Data Science (ROADS) program at the Institute for Data Sciences and Engineering at Columbia University (to Z.H.). NR 42 TC 5 Z9 5 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 24 PY 2016 VL 93 IS 6 AR 063524 DI 10.1103/PhysRevD.93.063524 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH3YN UT WOS:000372722800002 ER PT J AU Adare, A Aidala, C Ajitanand, NN Akiba, Y Al-Bataineh, H Alexander, J Alfred, M Angerami, A Aoki, K Apadula, N Aramaki, Y Asano, H Atomssa, ET Averbeck, R Awes, TC Azmoun, B Babintsev, V Bai, M Baksay, G Baksay, L Bandara, NS Bannier, B Barish, KN Bassalleck, B Basye, AT Bathe, S Baublis, V Baumann, C Bazilevsky, A Beaumier, M Beckman, S Belikov, S Belmont, R Bennett, R Berdnikov, A Berdnikov, Y Bhom, JH Blau, DS Bok, JS Boyle, K Brooks, ML Bryslawskyj, J Buesching, H Bumazhnov, V Bunce, G Butsyk, S Campbell, S Caringi, A Chen, CH Chi, CY Chiu, M Choi, IJ Choi, JB Choudhury, RK Christiansen, P Chujo, T Chung, P Chvala, O Cianciolo, V Citron, Z Cole, BA del Valle, ZC Connors, M Csanad, M Csorgo, T Dahms, T Dairaku, S Danchev, I Danley, TW Das, K Datta, A Daugherity, MS David, G Dayananda, MK DeBlasio, K Dehmelt, K Denisov, A Deshpande, A Desmond, EJ Dharmawardane, KV Dietzsch, O Dion, A Diss, PB Do, JH Donadelli, M D'Orazio, L Drapier, O Drees, A Drees, KA Durham, JM Durum, A Dutta, D Edwards, S Efremenko, YV Ellinghaus, F Engelmore, T Enokizono, A En'yo, H Esumi, S Fadem, B Feege, N Fields, DE Finger, M Finger, M Fleuret, F Fokin, SL Fraenkel, Z Frantz, JE Franz, A Frawley, AD Fujiwara, K Fukao, Y Fusayasu, T Gal, C Gallus, P Garg, P Garishvili, I Ge, H Giordano, F Glenn, A Gong, H Gonin, M Goto, Y de Cassagnac, RG Grau, N Greene, SV Grim, G Perdekamp, MG Gunji, T Gustafsson, HA Hachiya, T Haggerty, JS Hahn, KI Hamagaki, H Hamblen, J Hamilton, HF Han, R Han, SY Hanks, J Hasegawa, S Haseler, TOS Hashimoto, K Haslum, E Hayano, R He, X Heffner, M Hemmick, TK Hester, T Hill, JC Hohlmann, M Hollis, RS Holzmann, W Homma, K Hong, B Horaguchi, T Hornback, D Hoshino, T Hotvedt, N Huang, J Huang, S Ichihara, T Ichimiya, R Ikeda, Y Imai, K Inaba, M Iordanova, A Isenhower, D Ishihara, M Issah, M Ivanishchev, D Iwanaga, Y Jacak, BV Jezghani, M Jia, J Jiang, X Jin, J Johnson, BM Jones, T Joo, KS Jouan, D Jumper, DS Kajihara, F Kamin, J Kanda, S Kang, JH Kapustinsky, J Karatsu, K Kasai, M Kawall, D Kawashima, M Kazantsev, AV Kempel, T Key, JA Khachatryan, V Khanzadeev, A Kijima, KM Kikuchi, J Kim, A Kim, BI Kim, C Kim, DJ Kim, EJ Kim, GW Kim, M Kim, YJ Kimelman, B Kinney, E Kiss, A Kistenev, E Kitamura, R Klatsky, J Kleinjan, D Kline, P Koblesky, T Kochenda, L Komkov, B Konno, M Koster, J Kotov, D Kral, A Kravitz, A Kunde, GJ Kurita, K Kurosawa, M Kwon, Y Kyle, GS Lacey, R Lai, YS Lajoie, JG Lebedev, A Lee, DM Lee, J Lee, KB Lee, KS Lee, S Lee, SH Leitch, MJ Leite, MAL Li, X Lichtenwalner, P Liebing, P Lim, SH Levy, LAL Liska, T Liu, H Liu, MX Love, B Lynch, D Maguire, CF Makdisi, YI Makek, M Malik, MD Manion, A Manko, VI Mannel, E Mao, Y Masui, H Matathias, F McCumber, M McGaughey, PL McGlinchey, D McKinney, C Means, N Meles, A Mendoza, M Meredith, B Miake, Y Mibe, T Mignerey, AC Miki, K Milov, A Mishra, DK Mitchell, JT Miyasaka, S Mizuno, S Mohanty, AK Montuenga, P Moon, HJ Moon, T Morino, Y Morreale, A Morrison, DP Moukhanova, TV Murakami, T Murata, J Mwai, A Nagamiya, S Nagashima, K Nagle, JL Naglis, M Nagy, MI Nakagawa, I Nakagomi, H Nakamiya, Y Nakamura, KR Nakamura, T Nakano, K Nam, S Nattrass, C Netrakanti, PK Newby, J Nguyen, M Nihashi, M Niida, T Nishimura, S Nouicer, R Novak, T Novitzky, N Nyanin, AS Oakley, C O'Brien, E Oda, SX Ogilvie, CA Oka, M Okada, K Onuki, Y Koop, JDO Osborn, JD Oskarsson, A Ouchida, M Ozawa, K Pak, R Pantuev, V Papavassiliou, V Park, IH Park, JS Park, S Park, SK Park, WJ Pate, SF Patel, M Pei, H Peng, JC Pereira, H Perepelitsa, DV Perera, GDN Peressounko, DY Perry, J Petti, R Pinkenburg, C Pinson, R Pisani, RP Proissl, M Purschke, ML Qu, H Rak, J Ramson, BJ Ravinovich, I Read, KF Rembeczki, S Reygers, K Reynolds, D Riabov, V Riabov, Y Richardson, E Rinn, T Roach, D Roche, G Rolnick, SD 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CA PHENIX Collaboration TI Centrality-Dependent Modification of Jet-Production Rates in Deuteron-Gold Collisions at root s(NN)=200 GeV SO PHYSICAL REVIEW LETTERS LA English DT Article ID CROSS-SECTIONS; PPB COLLISIONS; P PLUS; ANGULAR-CORRELATIONS; PARTICLE-PRODUCTION; NUCLEAR COLLISIONS; CGC PREDICTIONS; LONG-RANGE; LHC; TEV AB Jet production rates are measured in p + p and d + Au collisions at root s(NN) = 200 GeV recorded in 2008 with the PHENIX detector at the Relativistic Heavy Ion Collider. Jets are reconstructed using the R = 0.3 anti-k(t) algorithm from energy deposits in the electromagnetic calorimeter and charged tracks in multiwire proportional chambers, and the jet transverse momentum (p(T)) spectra are corrected for the detector response. Spectra are reported for jets with 12 < p(T) < 50 GeV/c, within a pseudorapidity acceptance of vertical bar eta vertical bar < 0.3. The nuclear-modification factor (R-dAu) values for 0%-100% d + Au events are found to be consistent with unity, constraining the role of initial state effects on jet production. However, the centrality-selected RdAu values and central-to-peripheral ratios (R-CP) show large, p(T)-dependent deviations from unity, challenging the conventional models that relate hard-process rates and soft-particle production in collisions involving nuclei. C1 [Basye, A. T.; Daugherity, M. S.; Hamilton, H. F.; Isenhower, D.; Jones, T.; Jumper, D. S.; Pinson, R.; Thomas, D.; Towell, C. L.; Towell, R.; Towell, R. S.; Wright, R. M.] Abilene Christian Univ, Abilene, TX 79699 USA. [Grau, N.] Augustana Univ, Dept Phys, Sioux Falls, SD 57197 USA. [Garg, P.; Singh, B. K.; Singh, C. P.; Singh, V.; Tarafdar, S.] Banaras Hindu Univ, Dept Phys, Varanasi 221005, Uttar Pradesh, India. [Choudhury, R. K.; Dutta, D.; Mishra, D. K.; Mohanty, A. K.; Netrakanti, P. 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[Garishvili, I.; Glenn, A.; Heffner, M.; Newby, J.; Soltz, R. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Brooks, M. L.; Butsyk, S.; Durham, J. M.; Grim, G.; Jiang, X.; Kapustinsky, J.; Kunde, G. J.; Lee, D. M.; Leitch, M. J.; Liu, H.; Liu, M. X.; McCumber, M.; McGaughey, P. L.; Silva, C. L.; Snowball, M.; Sondheim, W. E.; van Hecke, H. W.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Roche, G.] Univ Clermont Ferrand, LPC, IN2P3, IN2P3,Clermont Fd, F-63177 Aubiere, France. [Christiansen, P.; Gustafsson, H. -A.; Haslum, E.; Oskarsson, A.; Rosendahl, S. S. E.; Silvermyr, D.; Stenlund, E.] Lund Univ, Dept Phys, Box 118, SE-22100 Lund, Sweden. [Diss, P. B.; D'Orazio, L.; Mignerey, A. C.; Richardson, E.; Sexton, A.] Univ Maryland, College Pk, MD 20742 USA. [Aidala, C.; Bandara, N. S.; Datta, A.; Kawall, D.; Stepanov, M.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Aidala, C.; Belmont, R.; Osborn, J. D.; Ramson, B. J.; Rubin, J. G.; White, A. S.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Baumann, C.; Reygers, K.; Sahlmueller, B.; Wessels, J.] Univ Munster, Inst Kernphys, Wilhelm Klemm Str 9, D-48149 Munster, Germany. [Caringi, A.; Fadem, B.; Kimelman, B.; Lichtenwalner, P.] Muhlenberg Coll, Allentown, PA 18104 USA. [Joo, K. S.; Moon, H. J.] Myongji Univ, Yongin 449728, Kyonggido, South Korea. [Fusayasu, T.; Tanaka, Y.] Nagasaki Inst Appl Sci, Nagasaki 8510193, Japan. [Shimomura, M.] Nara Womens Univ, Kita Uoya Nishi Machi, Nara 6308506, Japan. [Riabov, V.; Samsonov, V.; Taranenko, A.] Natl Res Nucl Univ, MEPhI, Moscow Engn Phys Inst, Moscow 115409, Russia. [Bassalleck, B.; Datta, A.; DeBlasio, K.; Fields, D. E.; Key, J. A.; Malik, M. D.; Thomas, T. L.; Younus, I.] Univ New Mexico, Albuquerque, NM 87131 USA. [Al-Bataineh, H.; Bok, J. S.; Dharmawardane, K. V.; Kyle, G. S.; Meles, A.; Papavassiliou, V.; Pate, S. F.; Perera, G. D. N.; Stepanov, M.; Wang, X. R.; Wei, F.] New Mexico State Univ, Las Cruces, NM 88003 USA. [Danley, T. W.; Frantz, J. E.; Xia, B.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Awes, T. C.; Cianciolo, V.; Efremenko, Y. V.; Enokizono, A.; Read, K. F.; Silvermyr, D.; Stankus, P. W.; Wysocki, M.; Young, G. R.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Jouan, D.] Univ Paris Saclay, Univ Paris Sud, IPN Orsay, CNRS,IN2P3, BP1, F-91406 Orsay, France. [Han, R.; Mao, Y.; You, Z.; Yu, H.] Peking Univ, Beijing 100871, Peoples R China. [Baublis, V.; Ivanishchev, D.; Khanzadeev, A.; Kochenda, L.; Komkov, B.; Kotov, D.; Riabov, V.; Riabov, Y.; Samsonov, V.; Vznuzdaev, E.] Petersburg Nucl Phys Inst, Gatchina 188300, Leningrad Regio, Russia. [Akiba, Y.; Aoki, K.; Aramaki, Y.; Asano, H.; Dairaku, S.; Enokizono, A.; En'yo, H.; Fujiwara, K.; Fukao, Y.; Goto, Y.; Hachiya, T.; Hashimoto, K.; Ichihara, T.; Ichimiya, R.; Imai, K.; Ishihara, M.; Karatsu, K.; Kasai, M.; Kawashima, M.; Kurita, K.; Kurosawa, M.; Mao, Y.; Miki, K.; Miyasaka, S.; Mizuno, S.; Murakami, T.; Murata, J.; Nagamiya, S.; Nakagawa, I.; Nakagomi, H.; Nakamura, K. R.; Nakamura, T.; Nakano, K.; Onuki, Y.; Ouchida, M.; Sakashita, K.; Seidl, R.; Shibata, T. -A.; Shoji, K.; Sumita, T.; Taketani, A.; Tanida, K.; Todoroki, T.; Watanabe, Y.; Yamaguchi, Y. L.; Yokkaichi, S.] RIKEN, Nishina Ctr Accelerator Based Sci, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. [Akiba, Y.; Bathe, S.; Boyle, K.; Bunce, G.; Chen, C. -H.; Deshpande, A.; En'yo, H.; Goto, Y.; Ichihara, T.; Kawall, D.; Kurosawa, M.; Liebing, P.; Nakagawa, I.; Nouicer, R.; Okada, K.; Seidl, R.; Taketani, A.; Tanida, K.; Togawa, M.; Wang, X. R.; Watanabe, Y.; Yokkaichi, S.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Enokizono, A.; Hashimoto, K.; Kasai, M.; Kawashima, M.; Kurita, K.; Murata, J.] Rikkyo Univ, Dept Phys, Toshima Ku, 3-34-1 Nishi Ikebukuro, Tokyo 1718501, Japan. [Berdnikov, A.; Berdnikov, Y.; Kotov, D.; Riabov, Y.] St Petersburg State Polytech Univ, St Petersburg 195251, Russia. [Dietzsch, O.; Donadelli, M.; Leite, M. A. L.; Takagui, E. M.] Univ Sao Paulo, Inst Fis, Caixa Postal 66318, BR-05315970 Sao Paulo, Brazil. [Kim, M.; Park, J. S.; Park, S.; Tanida, K.; Yoon, I.] Seoul Natl Univ, Dept Phys & Astron, Seoul 151742, South Korea. [Ajitanand, N. N.; Alexander, J.; Chung, P.; Jia, J.; Lacey, R.; Mwai, A.; Reynolds, D.; Taranenko, A.; Wei, R.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Apadula, N.; Averbeck, R.; Bannier, B.; Bennett, R.; Boyle, K.; Campbell, S.; Chen, C. -H.; Citron, Z.; Connors, M.; Dahms, T.; Dehmelt, K.; Deshpande, A.; Dion, A.; Drees, A.; Durham, J. M.; Feege, N.; Frantz, J. E.; Gal, C.; Ge, H.; Gong, H.; Hanks, J.; Hemmick, T. K.; Jacak, B. V.; Kamin, J.; Khachatryan, V.; Kline, P.; Lee, S. H.; Manion, A.; McCumber, M.; Means, N.; Nguyen, M.; Novitzky, N.; Pantuev, V.; Petti, R.; Proissl, M.; Sahlmueller, B.; Sharma, D.; Sun, J.; Taneja, S.; Themann, H.; Toia, A.; Yalcin, S.; Yamaguchi, Y. L.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Garishvili, I.; Hamblen, J.; Hornback, D.; Nattrass, C.; Read, K. F.; Schmoll, B. K.; Sen, A.; Sorensen, S. P.] Univ Tennessee, Knoxville, TN 37996 USA. [Miyasaka, S.; Nakano, K.; Sakashita, K.; Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Chujo, T.; Esumi, S.; Ikeda, Y.; Inaba, M.; Konno, M.; Masui, H.; Miake, Y.; Miki, K.; Mizuno, S.; Nakagomi, H.; Niida, T.; Oka, M.; Sato, T.; Shimomura, M.; Tanabe, R.; Todoroki, T.; Watanabe, K.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki 305, Japan. [Belmont, R.; Danchev, I.; Greene, S. V.; Huang, S.; Issah, M.; Love, B.; Maguire, C. F.; Roach, D.; Schaefer, B.; Valle, H.; Velkovska, J.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Kikuchi, J.; Sano, S.] Waseda Univ, Adv Res Inst Sci & Engn, Shinjuku Ku, 17 Kikui Cho, Tokyo 1620044, Japan. [Citron, Z.; Fraenkel, Z.; Milov, A.; Naglis, M.; Ravinovich, I.; Sharma, D.; Tarafdar, S.; Tserruya, I.] Weizmann Inst Sci, IL-76100 Rehovot, Israel. [Csorgo, T.; Nagy, M. I.; Novak, T.; Sziklai, J.; Vertesi, R.] Hungarian Acad Sci, Inst Particle & Nucl Phys, Wigner Res Ctr Phys, Wigner RCP,RMKI, POB 49, H-1525 Budapest 114, Hungary. [Bhom, J. H.; Bok, J. S.; Choi, I. J.; Do, J. H.; Kang, J. H.; Kwon, Y.; Lee, S.; Lim, S. H.; Moon, T.] Yonsei Univ, IPAP, Seoul 120749, South Korea. [Makek, M.] Univ Zagreb, Fac Sci, Dept Phys, Bijenicka 32, HR-10002 Zagreb, Croatia. RP Morrison, DP (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.; Nagle, JL (reprint author), Univ Colorado, Boulder, CO 80309 USA. EM morrison@bnl.gov; jamie.nagle@colorado.edu RI Durum, Artur/C-3027-2014; Sen, Abhisek/J-1157-2016; Nattrass, Christine/J-6752-2016; Sorensen, Soren /K-1195-2016; Hayano, Ryugo/F-7889-2012; Jung, David/Q-4068-2016; Yokkaichi, Satoshi/C-6215-2017; Taketani, Atsushi/E-1803-2017; OI Garg, Prakhar/0000-0001-5143-4384; Sen, Abhisek/0000-0003-1192-3938; Nattrass, Christine/0000-0002-8768-6468; Sorensen, Soren /0000-0002-5595-5643; Hayano, Ryugo/0000-0002-1214-7806; Jung, David/0000-0001-8631-610X; Taketani, Atsushi/0000-0002-4776-2315; Chvala, Ondrej/0000-0003-4614-6649 FU Office of Nuclear Physics in the Office of Science of the Department of Energy (U.S.A); National Science Foundation (U.S.A); Abilene Christian University Research Council (U.S.A); Research Foundation of SUNY (U.S.A); Ministry of Education, Culture, Sports, Science, and Technology (Japan); Japan Society for the Promotion of Science (Japan); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (Brazil); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil); Natural Science Foundation of China (People's Republic of China); Croatian Science Foundation (Croatia); Ministry of Science, Education, and Sports (Croatia); Ministry of Education, Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique (France); Commissariat a l'Energie Atomique (France); Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung (Germany); Deutscher Akademischer Austausch Dienst (Germany); Alexander von Humboldt Stiftung (Germany); National Science Fund (Hungary); OTKA (Hungary); Karoly Robert University College (Hungary); Ch. Simonyi Fund (Hungary); Department of Atomic Energy (India); Israel Science Foundation (Israel); Basic Science Research Program through NRF of the Ministry of Education (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science (Russia); Federal Agency of Atomic Energy (Russia); VR (Sweden); Wallenberg Foundation (Sweden); U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union; Hungarian American Enterprise Scholarship Fund; US-Israel Binational Science Foundation; Department of Science and Technology (India); Russian Academy of Sciences (Russia) FX We thank the staff of the Collider-Accelerator and Physics Departments at Brookhaven National Laboratory and the staff of the other PHENIX participating institutions for their vital contributions. We acknowledge support from the Office of Nuclear Physics in the Office of Science of the Department of Energy, the National Science Foundation, Abilene Christian University Research Council, Research Foundation of SUNY, and Dean of the College of Arts and Sciences, Vanderbilt University (U.S.A), Ministry of Education, Culture, Sports, Science, and Technology and the Japan Society for the Promotion of Science (Japan), Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil), Natural Science Foundation of China (People's Republic of China), Croatian Science Foundation and Ministry of Science, Education, and Sports (Croatia), Ministry of Education, Youth and Sports (Czech Republic), Centre National de la Recherche Scientifique, Commissariat a l'Energie Atomique, and Institut National de Physique Nucleaire et de Physique des Particules (France), Bundesministerium fur Bildung und Forschung, Deutscher Akademischer Austausch Dienst, and Alexander von Humboldt Stiftung (Germany), National Science Fund, OTKA, Karoly Robert University College, and the Ch. Simonyi Fund (Hungary), Department of Atomic Energy and Department of Science and Technology (India), Israel Science Foundation (Israel), Basic Science Research Program through NRF of the Ministry of Education (Korea), Physics Department, Lahore University of Management Sciences (Pakistan), Ministry of Education and Science, Russian Academy of Sciences, Federal Agency of Atomic Energy (Russia), VR and Wallenberg Foundation (Sweden), the U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union, the Hungarian American Enterprise Scholarship Fund, and the US-Israel Binational Science Foundation. NR 54 TC 5 Z9 5 U1 8 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 24 PY 2016 VL 116 IS 12 AR 122301 DI 10.1103/PhysRevLett.116.122301 PG 9 WC Physics, Multidisciplinary SC Physics GA DH4AZ UT WOS:000372729200005 PM 27058071 ER PT J AU Stephanov, MA Yee, HU AF Stephanov, Mikhail A. Yee, Ho-Ung TI No-Drag Frame for Anomalous Chiral Fluid SO PHYSICAL REVIEW LETTERS LA English DT Article AB We show that for an anomalous fluid carrying dissipationless chiral magnetic and/or vortical currents there is a frame in which a stationary obstacle experiences no drag, but energy and charge currents do not vanish, resembling superfluidity. However, unlike ordinary superfluid flow, the anomalous chiral currents can transport entropy in this frame. We show that the second law of thermodynamics completely determines the amounts of these anomalous nondissipative currents in the "no-drag frame" as polynomials in temperature and chemical potential with known anomaly coefficients. These general results are illustrated and confirmed by a calculation in the chiral kinetic theory and in the quark-gluon plasma at high temperature. C1 [Stephanov, Mikhail A.; Yee, Ho-Ung] Univ Illinois, Dept Phys, Chicago, IL 60607 USA. [Yee, Ho-Ung] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. RP Stephanov, MA (reprint author), Univ Illinois, Dept Phys, Chicago, IL 60607 USA. FU U.S. DOE [DE-FG0201ER41195] FX We thank R. Pisarski, K. Rajagopal, A. Sadofyev, and Y. Yin for discussions. This work is supported by U.S. DOE Grant No. DE-FG0201ER41195. NR 24 TC 7 Z9 7 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 24 PY 2016 VL 116 IS 12 AR 122302 DI 10.1103/PhysRevLett.116.122302 PG 5 WC Physics, Multidisciplinary SC Physics GA DH4AZ UT WOS:000372729200006 PM 27058072 ER PT J AU Kim, MG Heitmann, TW Mulcahy, SR Bourret-Courchesne, ED Birgeneau, RJ AF Kim, M. G. Heitmann, T. W. Mulcahy, S. R. Bourret-Courchesne, E. D. Birgeneau, R. J. TI Structural and antiferromagnetic properties of Ba(Fe1-x-yCoxRhy)(2)As-2 compounds SO PHYSICAL REVIEW B LA English DT Article ID SUPERCONDUCTIVITY AB We present a systematic investigation of the electrical, structural, and antiferromagnetic properties for the series of Ba(Fe1-x-yCoxRhy)(2)As-2 compounds with fixed x approximate to 0.027 and 0 <= y <= 0.035. We compare our results for the Co-Rh doped Ba(Fe1-x-yCoxRhy)(2)As-2 compounds with the Co doped Ba(Fe1-xCox)(2)As-2 compounds. We demonstrate that the electrical, structural, antiferromagnetic, and superconducting properties of the Co-Rh doped compounds are similar to the properties of the Co doped compounds. We find that the overall behaviors of Ba(Fe1-x-yCoxRhy)(2)As-2 and Ba(Fe1-xCox)(2)As-2 compounds are very similar when the total number of extra electrons per Fe/TM (TM = transition metal) site is considered, which is consistent with the rigid band model. Despite the similarity, we find that the details of the transitions, for example, the temperature difference between the structural and antiferromagnetic transition temperatures and the incommensurability of the antiferromangetic peaks, are different between Ba(Fe1-x-yCoxRhy)(2)As-2 and Ba(Fe1-xCox)(2)As-2 compounds. C1 [Kim, M. G.; Bourret-Courchesne, E. D.; Birgeneau, R. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Heitmann, T. W.] Univ Missouri, Missouri Res Reactor, Columbia, MO 65211 USA. [Mulcahy, S. R.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94720 USA. [Birgeneau, R. J.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Birgeneau, R. J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Mulcahy, S. R.] Western Washington Univ, Dept Geol, Bellingham, WA 98225 USA. RP Kim, MG (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM mgkim@lbl.gov; sean.mulcahy@wwu.edu RI Kim, Min Gyu/B-8637-2012 OI Kim, Min Gyu/0000-0001-7676-454X FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-05CH11231] FX We are grateful to M. Wang and Z. Xu for valuable discussions. The work at the Lawrence Berkeley National Laboratory was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract No. DE-AC02-05CH11231. NR 32 TC 1 Z9 1 U1 3 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 24 PY 2016 VL 93 IS 9 AR 094520 DI 10.1103/PhysRevB.93.094520 PG 7 WC Physics, Condensed Matter SC Physics GA DH3UJ UT WOS:000372712000004 ER PT J AU Li, G Rangel, T Liu, ZF Cooper, VR Neaton, JB AF Li, Guo Rangel, Tonatiuh Liu, Zhen-Fei Cooper, Valentino R. Neaton, Jeffrey B. TI Energy level alignment of self-assembled linear chains of benzenediamine on Au(111) from first principles SO PHYSICAL REVIEW B LA English DT Article ID SINGLE-MOLECULE JUNCTIONS; AUGMENTED-WAVE METHOD; BASIS-SET; CONDUCTANCE; METALS; APPROXIMATION; ELECTRONICS; TRANSPORT; CIRCUITS; DYNAMICS AB Using density functional theory (DFT) with a van der Waals density functional, we calculate the adsorption energetics and geometry of benzenediamine (BDA) molecules on Au(111) surfaces. Our results demonstrate that the reported self-assembled linear chain structure of BDA, stabilized via hydrogen bonds between amine groups, is energetically favored over previously studied monomeric phases. Moreover, using a model, which includes nonlocal polarization effects from the substrate and the neighboring molecules and incorporates many-body perturbation theory calculations within the GW approximation, we obtain approximate self-energy corrections to the DFT highest occupied molecular orbital (HOMO) energy associated with BDA adsorbate phases. We find that, independent of coverage, the HOMO energy of the linear chain phase is lower relative to the Fermi energy than that of the monomer phase, and in good agreement with values measured with ultraviolet photoelectron spectroscopy and x-ray photoelectron spectroscopy. C1 [Li, Guo] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Li, Guo; Rangel, Tonatiuh; Liu, Zhen-Fei; Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Li, Guo; Rangel, Tonatiuh; Liu, Zhen-Fei; Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Cooper, Valentino R.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Neaton, Jeffrey B.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. RP Li, G (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA.; Li, G; Neaton, JB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.; Li, G; Neaton, JB (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Neaton, JB (reprint author), Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. EM guoli@lbl.gov; jbneaton@lbl.gov RI Cooper, Valentino /A-2070-2012; Liu, Zhenfei/D-8980-2017 OI Cooper, Valentino /0000-0001-6714-4410; FU Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05-CH11231]; Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy [DE-AC02-05CH11231]; U.S. DOE, Office of Science, Basic Energy Sciences, Materials Sciences and Energy Division FX We thank Isaac Tamblyn and Kyuho Lee for the beneficial discussions. This work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05-CH11231. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences and by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Work by V.R.C. was supported by the U.S. DOE, Office of Science, Basic Energy Sciences, Materials Sciences and Energy Division. All calculations were carried out at NERSC. NR 50 TC 3 Z9 3 U1 4 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 24 PY 2016 VL 93 IS 12 AR 125429 DI 10.1103/PhysRevB.93.125429 PG 5 WC Physics, Condensed Matter SC Physics GA DH3WE UT WOS:000372716700004 ER PT J AU Plugge, S Zazunov, A Eriksson, E Tsvelik, AM Egger, R AF Plugge, S. Zazunov, A. Eriksson, E. Tsvelik, A. M. Egger, R. TI Kondo physics from quasiparticle poisoning in Majorana devices SO PHYSICAL REVIEW B LA English DT Article ID SEMICONDUCTOR-SUPERCONDUCTOR NANOWIRES; FERMIONS; STATES AB We present a theoretical analysis of quasiparticle poisoning in Coulomb-blockaded Majorana fermion systems tunnel-coupled to normal-conducting leads. Taking into account finite-energy quasiparticles, we derive the effective low-energy theory and present a renormalization group analysis. We find qualitatively new effects when a quasiparticle state with very low energy is localized near a tunnel contact. For M = 2 attached leads, such "dangerous" quasiparticle poisoning processes cause a spin S = 1/2 single-channel Kondo effect, which can be detected through a characteristic zero-bias anomaly conductance peak in all Coulomb blockade valleys. For more than two attached leads, the topological Kondo effect of the unpoisoned system becomes unstable. A strong-coupling bosonization analysis indicates that at low energy the poisoned lead is effectively decoupled and hence, forM > 3, the topological Kondo fixed point re-emerges, though now it involves only M - 1 leads. As a consequence, for M = 3, the low-energy fixed point becomes trivial corresponding to decoupled leads. C1 [Plugge, S.; Zazunov, A.; Eriksson, E.; Egger, R.] Univ Dusseldorf, Inst Theoret Phys, D-40225 Dusseldorf, Germany. [Eriksson, E.] Univ Grenoble Alpes, INAC SPSMS, F-38000 Grenoble, France. [Eriksson, E.] CEA Grenoble, INAC SPSMS, F-38000 Grenoble, France. [Tsvelik, A. M.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Plugge, S (reprint author), Univ Dusseldorf, Inst Theoret Phys, D-40225 Dusseldorf, Germany. RI Egger, Reinhold/A-9163-2010 OI Egger, Reinhold/0000-0001-5451-1883 FU Humboldt Prize of the Alexander-von-Humboldt foundation [SPP 1666]; Humboldt Prize of the Alexander-von-Humboldt foundation FX We thank A. Altland, B. Beri, K. Flensberg, C. M. Marcus, E. Sela, and A. Levy Yeyati for useful discussions. This work has been supported by the Deutsche Forschungsgemeinschaft within network SPP 1666 (R.E.) and by a Humboldt Prize of the Alexander-von-Humboldt foundation, enabling an extended stay of A.M.T. in Dusseldorf. NR 46 TC 5 Z9 5 U1 3 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 24 PY 2016 VL 93 IS 10 AR 104524 DI 10.1103/PhysRevB.93.104524 PG 13 WC Physics, Condensed Matter SC Physics GA DH3VH UT WOS:000372714400003 ER PT J AU Rusz, J Idrobo, JC AF Rusz, Jan Idrobo, Juan Carlos TI Aberrated electron probes for magnetic spectroscopy with atomic resolution: Theory and practical aspects SO PHYSICAL REVIEW B LA English DT Article ID ORBITAL ANGULAR-MOMENTUM; VORTEX BEAMS; CHIRAL DICHROISM; MICROSCOPE AB It was recently proposed that electron magnetic circular dichroism can be measured in scanning transmission electron microscopy with atomic resolution by tuning the phase distribution of an electron beam. Here, we describe the theoretical and practical aspects for the detection of out-of-plane and in-plane magnetization utilizing atomic size electron probes. We present the calculated optimized astigmatic probes and discuss how to achieve them experimentally. C1 [Rusz, Jan] Uppsala Univ, Dept Phys & Astron, POB 516, S-75120 Uppsala, Sweden. [Idrobo, Juan Carlos] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Rusz, J (reprint author), Uppsala Univ, Dept Phys & Astron, POB 516, S-75120 Uppsala, Sweden. RI Rusz, Jan/A-3324-2008 OI Rusz, Jan/0000-0002-0074-1349 FU ORNL's Center for Nanophase Materials Sciences (CNMS), U.S. Department of Energy, Office of Science User Facility FX J.R. acknowledges Swedish Research Council, STINT and Goran Gustafsson's Foundation. J.-C.I. acknowledges support by ORNL's Center for Nanophase Materials Sciences (CNMS), which is a U.S. Department of Energy, Office of Science User Facility. NR 42 TC 3 Z9 3 U1 8 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 24 PY 2016 VL 93 IS 10 AR 104420 DI 10.1103/PhysRevB.93.104420 PG 15 WC Physics, Condensed Matter SC Physics GA DH3VH UT WOS:000372714400002 ER PT J AU Xu, B Dai, YM Zhao, LX Wang, K Yang, R Zhang, W Liu, JY Xiao, H Chen, GF Taylor, AJ Yarotski, DA Prasankumar, RP Qiu, XG AF Xu, B. Dai, Y. M. Zhao, L. X. Wang, K. Yang, R. Zhang, W. Liu, J. Y. Xiao, H. Chen, G. F. Taylor, A. J. Yarotski, D. A. Prasankumar, R. P. Qiu, X. G. TI Optical spectroscopy of the Weyl semimetal TaAs SO PHYSICAL REVIEW B LA English DT Article ID FERMI ARCS; DISCOVERY; ELECTRON; PHASE; NODES AB We present a systematic study of both the temperature and frequency dependence of the optical response in TaAs, a material that has recently been realized to host the Weyl semimetal state. Our study reveals that the optical conductivity of TaAs features a narrow Drude response alongside a conspicuous linear dependence on frequency. The weight of the Drude peak decreases upon cooling, following a T-2 temperature dependence, in good agreement with theoretical predictions. Two linear components with distinct slopes dominate the low-temperature optical conductivity. A comparison between our experimental results and theoretical calculations suggests that the linear conductivity below similar to 230 cm(-1) arises purely from interband transitions near the Weyl points, providing rich information about the Weyl semimetal state in TaAs. C1 [Xu, B.; Zhao, L. X.; Wang, K.; Yang, R.; Zhang, W.; Liu, J. Y.; Xiao, H.; Chen, G. F.; Qiu, X. G.] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, POB 603, Beijing 100190, Peoples R China. [Dai, Y. M.; Yarotski, D. A.; Prasankumar, R. P.] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA. [Chen, G. F.; Qiu, X. G.] Collaborat Innovat Ctr Quantum Matter, Beijing 100190, Peoples R China. [Taylor, A. J.] Los Alamos Natl Lab, Associate Directorate Chem Life & Earth Sci, POB 1663, Los Alamos, NM 87545 USA. RP Qiu, XG (reprint author), Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, POB 603, Beijing 100190, Peoples R China.; Prasankumar, RP (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, POB 1663, Los Alamos, NM 87545 USA.; Qiu, XG (reprint author), Collaborat Innovat Ctr Quantum Matter, Beijing 100190, Peoples R China. EM rpprasan@lanl.gov; xgqiu@iphy.ac.cn RI Dai, Yaomin/E-4259-2016 OI Dai, Yaomin/0000-0002-2464-3161 FU MOST (973 Projects) [2015CB921303, 2015CB921102, 2012CB921302, 2012CB821403]; NSFC [91121004, 91421304, 11374345]; LANL LDRD program; UC Office of the President under the UC Lab Fees Research Program [237789]; NSAF [U1530402] FX We acknowledge very illuminating discussions with Simin Nie, Hongming Weng, Yongkang Luo, Hu Miao, John Bowlan, Pamela Bowlan, Brian McFarland, and Ricardo Lobo. Work at IOP CAS was supported by MOST (973 Projects No. 2015CB921303, No. 2015CB921102, No. 2012CB921302, and No. 2012CB821403), and NSFC (Grants No. 91121004, No. 91421304, and No. 11374345). Work at LANL was performed at the Center for Integrated Nanotechnologies, a US Department of Energy, Office of Basic Energy Sciences user facility, and funded by the LANL LDRD program and by the UC Office of the President under the UC Lab Fees Research Program, Grant ID No. 237789. H. Xiao is supported by NSAF, Grant No. U1530402. NR 41 TC 12 Z9 12 U1 14 U2 32 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 24 PY 2016 VL 93 IS 12 AR 121110 DI 10.1103/PhysRevB.93.121110 PG 5 WC Physics, Condensed Matter SC Physics GA DH3WE UT WOS:000372716700001 ER PT J AU Carneiro, KMM Zhai, HL Zhu, L Horst, JA Sitlin, M Nguyen, M Wagner, M Simpliciano, C Milder, M Chen, CL Ashby, P Bonde, J Li, W Habelitz, S AF Carneiro, Karina M. M. Zhai, Halei Zhu, Li Horst, Jeremy A. Sitlin, Melody Nguyen, Mychi Wagner, Martin Simpliciano, Cheryl Milder, Melissa Chen, Chun-Long Ashby, Paul Bonde, Johan Li, Wu Habelitz, Stefan TI Amyloid-like ribbons of amelogenins in enamel mineralization SO SCIENTIFIC REPORTS LA English DT Article ID DEVELOPING DENTAL ENAMEL; SECRETORY-STAGE; PROTEINS; MATRIX; FIBRILS; ORGANIZATION; PEPTIDE; HYDROXYAPATITE; CONFORMATION; NANORIBBONS AB Enamel, the outermost layer of teeth, is an acellular mineralized tissue that cannot regenerate; the mature tissue is composed of high aspect ratio apatite nanocrystals organized into rods and inter-rod regions. Amelogenin constitutes 90% of the protein matrix in developing enamel and plays a central role in guiding the hierarchical organization of apatite crystals observed in mature enamel. To date, a convincing link between amelogenin supramolecular structures and mature enamel has yet to be described, in part because the protein matrix is degraded during tissue maturation. Here we show compelling evidence that amelogenin self-assembles into an amyloid-like structure in vitro and in vivo. We show that enamel matrices stain positive for amyloids and we identify a specific region within amelogenin that self-assembles into beta-sheets. We propose that amelogenin nanoribbons template the growth of apatite mineral in human enamel. This is a paradigm shift from the current model of enamel development. C1 [Carneiro, Karina M. M.; Sitlin, Melody; Nguyen, Mychi; Simpliciano, Cheryl; Milder, Melissa; Habelitz, Stefan] Univ Calif San Francisco, Sch Dent, Dept Prevent & Restorat Dent Sci, San Francisco, CA 94143 USA. [Zhai, Halei; Zhu, Li; Horst, Jeremy A.; Li, Wu] Univ Calif San Francisco, Sch Dent, Dept Orofacial Sci, San Francisco, CA 94143 USA. [Horst, Jeremy A.] Univ Calif San Francisco, Sch Med, Dept Biochem & Biophys, San Francisco, CA 94158 USA. [Wagner, Martin] Bruker Nano Surfaces Div, 112 Robin Hill Rd, Santa Barbara, CA 93117 USA. [Chen, Chun-Long] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, One Cyclotron Rd,Bldg 67, Berkeley, CA 94720 USA. [Ashby, Paul] Pacific NW Natl Lab, POB 999,MSIN K4-18, Richland, WA 99352 USA. [Bonde, Johan] Lund Univ, Div Pure & Appl Biochem, Ctr Appl Life Sci, POB 124, SE-22100 Lund, Sweden. RP Habelitz, S (reprint author), Univ Calif San Francisco, Sch Dent, Dept Prevent & Restorat Dent Sci, San Francisco, CA 94143 USA.; Li, W (reprint author), Univ Calif San Francisco, Sch Dent, Dept Orofacial Sci, San Francisco, CA 94143 USA. EM wu.li@ucsf.edu; stefan.habelitz@ucsf.edu FU National Institute of Health (NIH/NIDCR) [DE023422, 5R01DE015821]; Swedish Foundation "O.E. och Edla Johanssons vetenskapliga stiftelse"; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Natural Sciences and Engineering Research Council of Canada (NSERC); Department of Energy [DE-AC05-76RL01830] FX The authors acknowledge the National Institute of Health (NIH/NIDCR DE023422 to SH and 5R01DE015821 to WL) and The Swedish Foundation "O.E. och Edla Johanssons vetenskapliga stiftelse" for funding and the Lawrence Berkeley National Laboratory for facility access (proposal numbers 3465 and 3330). Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. K.M.M.C. thanks the Natural Sciences and Engineering Research Council of Canada (NSERC) for a postdoctoral fellowship. The authors acknowledge the laboratory of James Simmer (Michigan) for providing murine tissue samples and Jan Stohr (UCSF) for help with the ThT assay. Pacific Northwest National Laboratory (PNNL) is multi-program national laboratory operated for Department of Energy by Battelle under Contracts No. DE-AC05-76RL01830. NR 52 TC 1 Z9 1 U1 6 U2 18 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 24 PY 2016 VL 6 AR 23105 DI 10.1038/srep23105 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH3NZ UT WOS:000372695000001 PM 27009419 ER PT J AU Salman, V Berben, T Bowers, RM Woyke, T Teske, A Angert, ER AF Salman, Verena Berben, Tom Bowers, Robert M. Woyke, Tanja Teske, Andreas Angert, Esther R. TI Insights into the single cell draft genome of "Candidatus Achromatium palustre" SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE "Candidatus Achromatium palustre"; Large sulfide-oxidizing bacteria; Thiotrichaceae; Calcium carbonate; Sippewissett Salt Marsh ID SULFUR BACTERIA; UNCULTURED BACTERIA; NATURAL COMMUNITIES; GENUS ACHROMATIUM; MICROBIAL GENOMES; ANALYSIS SYSTEM; SEQUENCE DATA; OXALIFERUM; MICROAUTORADIOGRAPHY; SPP. AB "Candidatus Achromatium palustre" was recently described as the first marine representative of the Achromatium spp. in the Thiotrichaceae - a sister lineage to the Chromatiaceae in the Gammaproteobacteria. Achromatium spp. belong to the group of large sulfur bacteria as they can grow to nearly 100 mu m in size and store elemental sulfur (S-0) intracellularly. As a unique feature, Achromatium spp. can accumulate colloidal calcite (CaCO3) inclusions in great amounts. Currently, both process and function of calcite accumulation in bacteria is unknown, and all Achromatium spp. are uncultured. Recently, three single-cell draft genomes of Achromatium spp. from a brackish mineral spring were published, and here we present the first draft genome of a single "Candidatus Achromatium palustre" cell collected in the sediments of the Sippewissett Salt Marsh, Cape Cod, MA. Our draft dataset consists of 3.6 Mbp, has a G + C content of 38.1 % and is nearly complete (83 %). The next closest relative to the Achromatium spp. genomes is Thiorhodovibrio sp. 907 of the family Chromatiaceae, containing phototrophic sulfide-oxidizing bacteria. C1 [Salman, Verena; Angert, Esther R.] Cornell Univ, Ithaca, NY USA. [Berben, Tom] Univ Amsterdam, Amsterdam, Netherlands. [Bowers, Robert M.; Woyke, Tanja] DOE Joint Genome Inst, Walnut Creek, CA USA. [Teske, Andreas] Univ N Carolina, Chapel Hill, NC USA. RP Salman, V (reprint author), Cornell Univ, Ithaca, NY USA. EM vcarvalh@mpi-bremen.de OI Carvalho, Verena/0000-0001-7760-8995 FU Marine Biological Laboratories; Horace W Stunkard Scholarship Fund; NSF [MCB 124437, IOS 1354911]; Deutsche Forschungsgemeinschaft [Sa 2505/1-1]; ERC advanced Grant PARASOL [322551]; U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility [DE-AC02-05CH11231] FX Cell collection was financially assisted by the Marine Biological Laboratories and the Horace W Stunkard Scholarship Fund. Sequencing was funded by the NSF MCB 1244378. VS was supported by the Deutsche Forschungsgemeinschaft (Sa 2505/1-1) and NSF IOS 1354911. TB was supported by the ERC advanced Grant PARASOL (No. 322551). The work conducted by the U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, is supported under Contract No. DE-AC02-05CH11231. NR 48 TC 0 Z9 0 U1 2 U2 2 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD MAR 23 PY 2016 VL 11 AR 28 DI 10.1186/s40793-016-0146-x PG 8 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DO7HA UT WOS:000377952000001 PM 27014417 ER PT J AU Cunsolo, A Suvorov, A Cai, YQ AF Cunsolo, Alessandro Suvorov, Alexey Cai, Yong Q. TI The onset of shear modes in the high frequency spectrum of simple disordered systems: current knowledge and perspectives SO PHILOSOPHICAL MAGAZINE LA English DT Article DE non-hydrodynamic modes; disordered systems; inelastic X ray scattering ID X-RAY-SCATTERING; WAVELENGTH COLLECTIVE EXCITATIONS; INELASTIC NEUTRON-SCATTERING; LIQUID WATER; ENERGY RESOLUTION; HEAVY-WATER; DYNAMICAL PROPERTIES; TRANSVERSE DYNAMICS; VITREOUS SILICA; BOSON PEAK AB Nearly two decades of thorough inelastic X-ray scattering (IXS) studies of transverse-like excitation in the spectrum of simple amorphous materials are reviewed. Particular attention is given to the case of liquid water and other prototypical samples, through discussion of both solved and still open issues. The perspectives opened up by the development of next generation IXS instruments with unprecedented contrast and resolution bandwidth are briefly illustrated. C1 [Cunsolo, Alessandro; Suvorov, Alexey; Cai, Yong Q.] Brookhaven Natl Lab, Photon Sci Directorate, POB 5000, Upton, NY 11973 USA. RP Cunsolo, A (reprint author), Brookhaven Natl Lab, Photon Sci Directorate, POB 5000, Upton, NY 11973 USA. EM acunsolo@bnl.gov FU US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0012704] FX Work performed at the National Synchrotron Light Source II, Brookhaven National Laboratory, was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. NR 63 TC 2 Z9 2 U1 3 U2 7 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1478-6435 EI 1478-6443 J9 PHILOS MAG JI Philos. Mag. PD MAR 23 PY 2016 VL 96 IS 7-9 SI SI BP 732 EP 742 DI 10.1080/14786435.2015.1096975 PG 11 WC Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering; Physics, Applied; Physics, Condensed Matter SC Materials Science; Metallurgy & Metallurgical Engineering; Physics GA DI1DK UT WOS:000373236000005 ER PT J AU Nandwana, V Ryoo, SR Kanthala, S De, M Chou, SS Prasad, PV Dravid, VP AF Nandwana, Vikas Ryoo, Soo-Ryoon Kanthala, Shanthi De, Mrinmoy Chou, Stanley S. Prasad, Pottumarthi V. Dravid, Vinayak P. TI Engineered Theranostic Magnetic Nanostructures: Role of Composition and Surface Coating on Magnetic Resonance Imaging Contrast and Thermal Activation SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE magnetic nanostructures; theranostics; thermal activation; magnetic resonance imaging contrast; magnetic nanoparticles; biomedical applications; hyperthermia; nanomedicine ID IRON-OXIDE NANOPARTICLES; MRI CONTRAST; NANOCRYSTALS; HYPERTHERMIA; AGENTS; CELLS; FIELD; RELAXIVITY; PEGYLATION; SPINEL AB Magnetic nanostructures (MNS) have emerged as promising functional probes for simultaneous diagnostics and therapeutics (theranostic) applications due to their ability to enhance localized contrast in magnetic resonance imaging (MRI) and heat under external radio frequency (RF) field, respectively. We show that the "theranostic" potential of the MNS can be significantly enhanced by tuning their core composition and architecture of surface coating. Metal ferrite (e.g., MFe2O4) nanoparticles of similar to 8 nm size and nitrodopamine conjugated polyethylene glycol (NDOPA-PEG) were used as the core and surface coating of the MNS, respectively. The composition was controlled by tuning the stoichiometry of MFe2O4 nanoparticles (M = Fe, MO, Zn, ZnxMn1-x) while the architecture of surface coating was tuned by changing the molecular weight of PEG, such that larger weight is expected to result in longer length extended away from the MNS surface. Our results suggest that both core as well as surface coating are important factors to take into consideration during the design of MNS as theranostic agents which is illustrated by relativity and thermal activation plots of MNS with different core composition and surface coating thickness. After optimization of these parameters;. the r(2) relativity and specific absorption rate (SAR) up to 552 mM(-1) s(-1) and 385 W/g were obtained, respectively, which are among the highest values reported for MNS with core magnetic nanoparticles of size below 10 nm. In addition, NDOPA-PEG coated MFe2O4 nanostructures showed enhanced biocompatibility (up to [Fe] = 200 mu g/mL) and reduced nonspecific uptake in macrophage cells in comparison to other well established FDA approved Fe based MR contrast agents. C1 [Nandwana, Vikas; Ryoo, Soo-Ryoon; Kanthala, Shanthi; Dravid, Vinayak P.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [De, Mrinmoy] Indian Inst Sci, Dept Organ Chem, Bengaluru, India. [Chou, Stanley S.] Sandia Natl Labs, Dept Elect Opt & Nano Mat, Albuquerque, NM 87185 USA. [Prasad, Pottumarthi V.] Northshore Univ Healthcare, Dept Radiol, Evanston, IL 60201 USA. RP Dravid, VP (reprint author), Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. EM v-dravid@northwestern.edu RI Dravid, Vinayak/B-6688-2009; OI Prasad, Pottumarthi/0000-0002-4214-5465 FU Center of Cancer Nanotechnology Excellence (CCNE) initiative of the National Institutes of Health (NIH) [U54 CA151880]; NTU-NU Institute for NanoMedicine at the International Institute for Nanotechnology, Northwestern University, USA; Nanyang Technological University, Singapore; MRSEC program at the Materials Research Center [NSF DMR-1121262] FX The authors would like to thank Prof. M. Aslam (IIT Bombay, India) for the intellectual discussion. This research was supported by the Center of Cancer Nanotechnology Excellence (CCNE) initiative of the National Institutes of Health (NIH) under Award number U54 CA151880. Any opinions, findings, conclusions, or recommendations expressed in this material are those of the authors and do not necessarily reflect those of the NIH. V.N., S.K., S.R, and V.P.D. gratefully acknowledges support from the NTU-NU Institute for NanoMedicine located at the International Institute for Nanotechnology, Northwestern University, USA and the Nanyang Technological University, Singapore. This work made use of the (EPIC, Keck-II, and/or SPID) facility(ies) of the NUANCE Center at Northwestern University, which has received support from the Soft and Hybrid Nanotechnology Experimental (SHyNE) Resource (NSF NNCI-1542205); the MRSEC program (NSF DMR-1121262) at the Materials Research Center; the International Institute for Nanotechnology (IIN); the Keck Foundation; and the State of Illinois, through the IIN. NR 40 TC 0 Z9 0 U1 12 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAR 23 PY 2016 VL 8 IS 11 BP 6953 EP 6961 DI 10.1021/acsami.6b01377 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DH7BQ UT WOS:000372946600021 PM 26936392 ER PT J AU Belianinov, A Iberi, V Tselev, A Susner, MA McGuire, MA Joy, D Jesse, S Rondinone, AJ Kalinin, SV Ovchinnikova, OS AF Belianinov, Alex Iberi, Vighter Tselev, Alexander Susner, Michael A. McGuire, Michael A. Joy, David Jesse, Stephen Rondinone, Adam J. Kalinin, Sergei V. Ovchinnikova, Olga S. TI Polarization Control via He-Ion Beam Induced Nanofabrication in Layered Ferroelectric Semiconductors SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE helium ion microscopy; atomic force microscopy; layered materials; ferroelectricity; 2D crystals ID RAMAN-SPECTROSCOPY; BAND EXCITATION; MICROSCOPY; LITHOGRAPHY; CUINP2S6; PHASE; TRANSITION; GRAPHENE; CRYSTALS; CARBON AB Rapid advances in nanoscience rely on continuous improvements of material manipulation at near atomic scales. Currently, the workhorse of nanofabrication is resist-based lithography and its various derivatives. However, the use of local electron, ion, and physical probe methods is expanding, driven largely by the need for fabrication without the multistep preparation processes that can result in contamination from resists and solvents. Furthermore, probe based methods extend beyond nanofabrication to nano manipulation and to imaging which are all vital for a rapid transition to the prototyping and testing of devices. In this work we study helium ion interactions with the surface of bulk copper indium thiophosphate (CuMP2X6)-P-III (M = Cr, In; X = S, Se), a novel layered 2D material, with a Helium Ion Microscope (HIM). Using this technique, we are able to control ferrielectric domains and, grow conical nanostructures with enhanced conductivity whose material volumes scale with the beam dosage. Compared to the copper indium thiophosphate (CITP) from which they grow, the nanostructures are oxygen rich, sulfur poor, and with virtually unchanged copper concentration as confirmed by energy-dispersive X-ray spectroscopy (EDX). Scanning electron microscopy (SEM) imaging contrast as well as scanning microwave microscopy (SMM) measurements suggest enhanced conductivity in the formed particles, whereas atomic force microscopy (AFM) measurements indicate that the produced structures have lower dissipation and are softer as compared to the CITP. C1 [Belianinov, Alex; Tselev, Alexander; Jesse, Stephen; Kalinin, Sergei V.; Ovchinnikova, Olga S.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Belianinov, Alex; Iberi, Vighter; Tselev, Alexander; Joy, David; Jesse, Stephen; Rondinone, Adam J.; Kalinin, Sergei V.; Ovchinnikova, Olga S.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Susner, Michael A.; McGuire, Michael A.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. [Tselev, Alexander] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Joy, David] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Belianinov, A; Ovchinnikova, OS (reprint author), Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA.; Belianinov, A; Ovchinnikova, OS (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM belianinova@ornl.gov; ovchinnikovo@ornl.gov RI McGuire, Michael/B-5453-2009; Susner, Michael/B-1666-2013; Rondinone, Adam/F-6489-2013 OI McGuire, Michael/0000-0003-1762-9406; Susner, Michael/0000-0002-1211-8749; Rondinone, Adam/0000-0003-0020-4612 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; U.S. Government [DE-AC05-00OR22725] FX Research was supported (V.I., A.T., D.J., S.V.K, S.J., A.J.R., O.S.O.) and partially conducted (AFM, Data Analysis) at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Research was partially sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy (Helium Ion Microscopy, A.B.; crystal growth, M.A.S. and M.A.M.). This manuscript has been authored by a contractor of the U.S. Government under contract DE-AC05-00OR22725. NR 40 TC 1 Z9 1 U1 19 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAR 23 PY 2016 VL 8 IS 11 BP 7349 EP 7355 DI 10.1021/acsami.5b12056 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DH7BQ UT WOS:000372946600067 PM 26918591 ER PT J AU Feier, HM Reid, OG Pace, NA Park, J Bergkamp, JJ Sellinger, A Gust, D Rumbles, G AF Feier, Hilary M. Reid, Obadiah G. Pace, Natalie A. Park, Jaehong Bergkamp, Jesse J. Sellinger, Alan Gust, Devens Rumbles, Garry TI Local Intermolecular Order Controls Photoinduced Charge Separation at Donor/Acceptor Interfaces in Organic Semiconductors SO ADVANCED ENERGY MATERIALS LA English DT Article DE charge photogeneration; organic photovoltaics; transient absorption; free charge generation; organic semiconductors ID FREE-CARRIER GENERATION; SOLAR-CELLS; BULK HETEROJUNCTIONS; CONJUGATED POLYMERS; FULLERENE HETEROJUNCTIONS; RECOMBINATION DYNAMICS; PHOTOGENERATED CHARGE; TRANSIENT ABSORPTION; EXCITON DISSOCIATION; POLY(3-HEXYLTHIOPHENE) AB How free charge is generated at organic donor-acceptor interfaces is an important question, as the binding energy of the lowest energy (localized) charge transfer states should be too high for the electron and hole to escape each other. Recently, it has been proposed that delocalization of the electronic states participating in charge transfer is crucial, and aggregated or otherwise locally ordered structures of the donor or the acceptor are the precondition for this electronic characteristic. The effect of intermolecular aggregation of both the polymer donor and fullerene acceptor on charge separation is studied. In the first case, the dilute electron acceptor triethylsilylhydroxy-1,4,8,11,15,18,22,25-octabutoxyphthalocyaninatosilicon(IV) (SiPc) is used to eliminate the influence of acceptor aggregation, and control polymer order through side-chain regioregularity, comparing charge generation in 96% regioregular (RR-) poly(3-hexylthiophene) (P3HT) with its regiorandom (RRa-) counterpart. In the second case, ordered phases in the polymer are eliminated by using RRa-P3HT, and phenyl-C-61-butyric acid methyl ester (PC61BM) is used as the acceptor, varying its concentration to control aggregation. Time-resolved microwave conductivity, time-resolved photoluminescence, and transient absorption spectroscopy measurements show that while ultrafast charge transfer occurs in all samples, long-lived charge carriers are only produced in films with intermolecular aggregates of either RR-P3HT or PC61BM, and that polymer aggregates are just as effective in this regard as those of fullerenes. C1 [Feier, Hilary M.; Reid, Obadiah G.; Pace, Natalie A.; Park, Jaehong; Rumbles, Garry] Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. [Feier, Hilary M.] Univ Colorado, Dept Chem & Biol Engn, Boulder, CO 80309 USA. [Reid, Obadiah G.; Rumbles, Garry] Univ Colorado, Renewable & Sustainable Energy Inst, Boulder, CO 80309 USA. [Pace, Natalie A.; Rumbles, Garry] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Bergkamp, Jesse J.; Gust, Devens] Arizona State Univ, Dept Chem & Biochem, Tempe, AZ 85287 USA. [Sellinger, Alan] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA. RP Rumbles, G (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM garry.rumbles@nrel.gov RI Sellinger, Alan/C-6250-2015; OI Sellinger, Alan/0000-0001-6705-1548; Park, Jaehong/0000-0002-0509-3934; Rumbles, Garry/0000-0003-0776-1462; Bergkamp, Jesse/0000-0003-3443-0255 FU Solar Photochemistry Program, Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC36-08-GO28308]; National Renewable Energy Laboratory; Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Energy Biosciences, Department of Energy [DE-FG02-03ER15393] FX This work was supported by the Solar Photochemistry Program, Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy under contract number DE-AC36-08-GO28308 with the National Renewable Energy Laboratory. The experimental development for controlling polymer crystalline domain size was supported by the Laboratory Directed Research and Development (LDRD) Program at the National Renewable Energy Laboratory under task number 06RF1201. Synthesis of the silicon phthalocyanine was supported by the Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Energy Biosciences, Department of Energy under Contract No. DE-FG02-03ER15393. The authors acknowledge Martin Heeney and George Barnes for the synthesis of the poly(2,2':5',2 ''-3,3 ''-dihexyl-terthiophene) (PTTT) used in Section 4 in the Supporting Information. NR 56 TC 5 Z9 5 U1 8 U2 76 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD MAR 23 PY 2016 VL 6 IS 6 AR 1502176 DI 10.1002/aenm.201502176 PG 9 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA DH9XQ UT WOS:000373149700015 ER PT J AU Heo, TW Tang, M Chen, LQ Wood, BC AF Heo, Tae Wook Tang, Ming Chen, Long-Qing Wood, Brandon C. TI Defects, Entropy, and the Stabilization of Alternative Phase Boundary Orientations in Battery Electrode Particles SO ADVANCED ENERGY MATERIALS LA English DT Article DE interfacial defects; electrode particles; microelasticity theory; phase boundary orientations; phase-field models ID LITHIUM-ION BATTERIES; MICROSTRUCTURE EVOLUTION; LIFEPO4 NANOPARTICLES; TRANSITION PATHWAYS; FIELD MODELS; SEPARATION; OLIVINES; DISLOCATION; DEPENDENCE; DYNAMICS AB Using a novel statistical approach that efficiently explores the space of possible defect configurations, the present study investigates the chemomechanical coupling between interfacial structural defects and phase boundary alignments within phase-separating electrode particles. Applied to the battery cathode material LiXFePO4 as an example, the theoretical analysis reveals that small, defect-induced deviations from an ideal interface can lead to dramatic shifts in the orientations of phase boundaries between Li-rich and Li-lean phases, stabilizing otherwise unfavorable orientations. Significantly, this stabilization arises predominantly from configurational entropic factors associated with the presence of the interfacial defects rather than from absolute energetic considerations. The specific entropic factors pertain to the diversity of defect configurations and their contributions to rotational/orientational rigidity of phase boundaries. Comparison of the predictions with experimental observations indicates that the additional entropy contributions indeed play a dominant role under actual cycling conditions, leading to the conclusion that interfacial defects must be considered when analyzing the stability and evolution kinetics of the internal phase microstructure of strongly phase-separating systems. Possible implications for tuning the kinetics of (de)lithiation based on selective defect incorporation are discussed. This understanding can be generalized to the chemomechanics of other defective solid phase boundaries. C1 [Heo, Tae Wook; Wood, Brandon C.] Lawrence Livermore Natl Lab, Div Mat Sci, Livermore, CA 94550 USA. [Tang, Ming] Rice Univ, Dept Mat Sci & NanoEngn, Houston, TX 77024 USA. [Chen, Long-Qing] Penn State Univ, Dept Mat Sci & Engn, University Pk, PA 16802 USA. RP Heo, TW; Wood, BC (reprint author), Lawrence Livermore Natl Lab, Div Mat Sci, Livermore, CA 94550 USA. EM heo1@llnl.gov; wood37@llnl.gov FU U.S. Department of Energy by Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344]; Laboratory Directed Research and Development Program at LLNL [12-ERD-053, 15-ERD-022]; DOE [DE-SC0002626]; NSF [CMMI-1235092]; [LLNL-SR-648484] FX The work of T.W.H. and B.C.W. was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory (LLNL) under Contract DE-AC52-07NA27344. This work was funded by the Laboratory Directed Research and Development Program at LLNL under project tracking codes 12-ERD-053 and 15-ERD-022. M.T. acknowledges the support from DOE project number DE-SC0002626. The work of L.-Q.C. was supported by Subcontract LLNL-SR-648484 and partially by NSF under Grant Number CMMI-1235092. Helpful discussions with Y.M. Wang, J. Ye, J. Lee, and Y. An (LLNL) are acknowledged. NR 34 TC 0 Z9 0 U1 14 U2 51 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1614-6832 EI 1614-6840 J9 ADV ENERGY MATER JI Adv. Energy Mater. PD MAR 23 PY 2016 VL 6 IS 6 AR 1501759 DI 10.1002/aenm.201501759 PG 10 WC Chemistry, Physical; Energy & Fuels; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Energy & Fuels; Materials Science; Physics GA DH9XQ UT WOS:000373149700002 ER PT J AU Airapetian, A Akopov, N Akopov, Z Augustyniak, W Avetissian, A Blok, HP Borissov, A Bryzgalov, V Capiluppi, M Capitani, GP Cisbani, E Ciullo, G Contalbrigo, M Dalpiaz, PF Deconinck, W De Leo, R De Sanctis, E Diefenthaler, M Di Nezza, P Duren, M Ehrenfried, M Elbakian, G Ellinghaus, F Etzelmuller, E Fabbri, R Felawka, L Frullani, S Gabbert, D Gapienko, G Gapienko, V Garibaldi, F Gavrilov, G Gharibyan, V Hartig, M Hasch, D Holler, Y Hristova, I Ivanilov, A Jackson, HE Joosten, S Kaiser, R Karyan, G Keri, T Kinney, E Kisselev, A Korotkov, V Kozlov, V Kravchenko, P Krivokhijine, VG Lagamba, L Lapikas, L Lehmann, I Lenisa, P Lorenzon, W Ma, BQ Mahon, D Manaenkov, SI Mao, Y Marianski, B Marukyan, H Movsisyan, A Murray, M Naryshkin, Y Nass, A Nowak, WD Pappalardo, LL Perez-Benito, R Petrosyan, A Reimer, PE Reolon, AR Riedl, C Rith, K Rostomyan, A Ryckbosch, D Schafer, A Schnell, G Schuler, KP Seitz, B Shibata, TA Stahl, M Stancari, M Statera, M Steffens, E Steijger, JJM Taroian, S Terkulov, A Truty, R Trzcinski, A Tytgat, M Van Haarlem, Y Van Hulse, C Vikhrov, V Vilardi, I Wang, S Yaschenko, S Yen, S Zeiler, D Zihlmann, B Zupranski, P AF Airapetian, A. Akopov, N. Akopov, Z. Augustyniak, W. Avetissian, A. Blok, H. P. Borissov, A. Bryzgalov, V. Capiluppi, M. Capitani, G. P. Cisbani, E. Ciullo, G. Contalbrigo, M. Dalpiaz, P. F. Deconinck, W. De Leo, R. De Sanctis, E. Diefenthaler, M. Di Nezza, P. Dueren, M. Ehrenfried, M. Elbakian, G. Ellinghaus, F. Etzelmueller, E. Fabbri, R. Felawka, L. Frullani, S. Gabbert, D. Gapienko, G. Gapienko, V. Garibaldi, F. Gavrilov, G. Gharibyan, V. Hartig, M. Hasch, D. Holler, Y. Hristova, I. Ivanilov, A. Jackson, H. E. Joosten, S. Kaiser, R. Karyan, G. Keri, T. Kinney, E. Kisselev, A. Korotkov, V. Kozlov, V. Kravchenko, P. Krivokhijine, V. G. Lagamba, L. Lapikas, L. Lehmann, I. Lenisa, P. Lorenzon, W. Ma, B. -Q. Mahon, D. Manaenkov, S. I. Mao, Y. Marianski, B. Marukyan, H. Movsisyan, A. Murray, M. Naryshkin, Y. Nass, A. Nowak, W. -D. Pappalardo, L. L. Perez-Benito, R. Petrosyan, A. Reimer, P. E. Reolon, A. R. Riedl, C. Rith, K. Rostomyan, A. Ryckbosch, D. Schaefer, A. Schnell, G. Schueler, K. P. Seitz, B. Shibata, T. -A. Stahl, M. Stancari, M. Statera, M. Steffens, E. Steijger, J. J. M. Taroian, S. Terkulov, A. Truty, R. Trzcinski, A. Tytgat, M. Van Haarlem, Y. Van Hulse, C. Vikhrov, V. Vilardi, I. Wang, S. Yaschenko, S. Yen, S. Zeiler, D. Zihlmann, B. Zupranski, P. CA HERMES Collaboration TI Spin density matrix elements in exclusive omega electroproduction on H-1 and H-2 targets at 27.5 GeV beam energy (vol 74, 3110, 2014) SO EUROPEAN PHYSICAL JOURNAL C LA English DT Correction ID MINIMAL FLAVOR VIOLATION; HIGGS-BOSON; STANDARD MODEL; PHYSICS; DECAYS; LHC; COUPLINGS; SYMMETRY; PARTICLE; SEARCH C1 [Jackson, H. E.; Reimer, P. E.] Argonne Natl Lab, Div Phys, 9700 S Cass Ave, Argonne, IL 60439 USA. [De Leo, R.; Lagamba, L.; Vilardi, I.] Ist Nazl Fis Nucl, Sez Bari, I-70124 Bari, Italy. [Ma, B. -Q.; Mao, Y.; Wang, S.] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Schnell, G.; Van Hulse, C.] Univ Basque Country UPV EHU, Dept Theoret Phys, Bilbao 48080, Spain. [Schnell, G.] Basque Fdn Sci, Ikerbasque, Bilbao 48013, Spain. [Ellinghaus, F.; Kinney, E.] Univ Colorado, Nucl Phys Lab, Boulder, CO 80309 USA. [Akopov, Z.; Borissov, A.; Deconinck, W.; Gavrilov, G.; Hartig, M.; Holler, Y.; Rostomyan, A.; Schueler, K. P.; Yaschenko, S.; Zihlmann, B.] DESY, D-22603 Hamburg, Germany. [Fabbri, R.; Gabbert, D.; Hristova, I.; Nowak, W. -D.; Riedl, C.] DESY, D-15738 Zeuthen, Germany. [Krivokhijine, V. G.] Joint Inst Nucl Res, Dubna 141980, Russia. [Diefenthaler, M.; Nass, A.; Rith, K.; Steffens, E.; Yaschenko, S.; Zeiler, D.] Univ Erlangen Nurnberg, Inst Phys, D-91058 Erlangen, Germany. [Capiluppi, M.; Ciullo, G.; Contalbrigo, M.; Dalpiaz, P. F.; Lenisa, P.; Movsisyan, A.; Pappalardo, L. L.; Stancari, M.; Statera, M.] Ist Nazl Fis Nucl, Sez Ferrara, I-44122 Ferrara, Italy. [Capiluppi, M.; Ciullo, G.; Dalpiaz, P. F.; Lenisa, P.; Pappalardo, L. L.; Stancari, M.; Statera, M.] Univ Ferrara, Dipartimento Fis & Sci Terra, I-44122 Ferrara, Italy. [Capitani, G. P.; De Sanctis, E.; Di Nezza, P.; Hasch, D.; Reolon, A. R.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Joosten, S.; Ryckbosch, D.; Schnell, G.; Tytgat, M.; Van Haarlem, Y.; Van Hulse, C.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Airapetian, A.; Dueren, M.; Ehrenfried, M.; Etzelmueller, E.; Keri, T.; Perez-Benito, R.; Stahl, M.] Univ Giessen, Inst Phys 2, D-35392 Giessen, Germany. [Kaiser, R.; Lehmann, I.; Mahon, D.; Murray, M.; Seitz, B.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow G12 8QQ, Lanark, Scotland. [Diefenthaler, M.; Joosten, S.; Riedl, C.; Truty, R.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Airapetian, A.; Lorenzon, W.] Univ Michigan, Randall Lab Phys, Ann Arbor, MI 48109 USA. [Kozlov, V.; Terkulov, A.] PN Lebedev Phys Inst, Moscow 117924, Russia. [Blok, H. P.; Lapikas, L.; Steijger, J. J. M.] Natl Inst Subat Phys Nikhef, NL-1009 DB Amsterdam, Netherlands. [Gavrilov, G.; Kisselev, A.; Kravchenko, P.; Manaenkov, S. I.; Naryshkin, Y.; Vikhrov, V.] BP Konstantinov Petersburg Nucl Phys Inst, Gatchina 188300, Leningrad Regio, Russia. [Bryzgalov, V.; Gapienko, G.; Gapienko, V.; Ivanilov, A.; Korotkov, V.] Inst High Energy Phys, Protvino 142281, Moscow Region, Russia. [Schaefer, A.] Univ Regensburg, Inst Theoret Phys, D-93040 Regensburg, Germany. [Cisbani, E.; Frullani, S.; Garibaldi, F.] Ist Nazl Fis Nucl, Grp Coll Sanita, Sez Roma, I-00161 Rome, Italy. [Cisbani, E.; Frullani, S.; Garibaldi, F.] Ist Super Sanita, Viale Regina Elena 299, I-00161 Rome, Italy. [Felawka, L.; Gavrilov, G.; Yen, S.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [Blok, H. P.] Vrije Univ Amsterdam, Dept Phys & Astron, NL-1081 HV Amsterdam, Netherlands. [Augustyniak, W.; Marianski, B.; Trzcinski, A.; Zupranski, P.] Natl Ctr Nucl Res, PL-00689 Warsaw, Poland. [Avetissian, A.; Elbakian, G.; Gharibyan, V.; Karyan, G.; Marukyan, H.; Movsisyan, A.; Petrosyan, A.; Taroian, S.] Yerevan Phys Inst, Yerevan 375036, Armenia. RP Schnell, G (reprint author), Univ Basque Country UPV EHU, Dept Theoret Phys, Bilbao 48080, Spain.; Schnell, G (reprint author), Basque Fdn Sci, Ikerbasque, Bilbao 48013, Spain.; Schnell, G (reprint author), Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. EM gunar.schnell@desy.de RI Kozlov, Valentin/M-8000-2015; Terkulov, Adel/M-8581-2015 NR 80 TC 1 Z9 1 U1 5 U2 10 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAR 23 PY 2016 VL 76 IS 3 AR 162 DI 10.1140/epjc/s10052-016-3996-x PG 17 WC Physics, Particles & Fields SC Physics GA DH9UX UT WOS:000373142600001 ER PT J AU Lopez, CDC Wozny, G Flores-Tlacuahuac, A Vasquez-Medrano, R Zavala, VM AF Lopez, Diana C. C. Wozny, Guenter Flores-Tlacuahuac, Antonio Vasquez-Medrano, Ruben Zavala, Victor M. TI A Computational Framework for Identifiability and III-Conditioning Analysis of Lithium-Ion Battery Models SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID FULLER-NEWMAN MODEL; PARAMETER-ESTIMATION; RIDGE REGRESSION; INSERTION CELL; SIMULATION; SYSTEMS; IDENTIFICATION; SELECTION; SUBSETS; DESIGN AB The lack of informative experimental data and the complexity of first-principles battery models make the recovery of kinetic, transport, and thermodynamic parameters complicated. We present a computational framework that combines sensitivity, singular value, and Monte Carlo analysis to explore how different sources of experimental data affect parameter structural ill conditioning and identifiability. Our study is conducted on a modified version of the Doyle-Fuller-Newman model. We demonstrate that the use of voltage discharge curves only enables the identification of a small parameter subset, regardless of the number of experiments considered. Furthermore, we show that the inclusion of a single electrolyte concentration measurement significantly aids identifiability and mitigates ill-conditioning. C1 [Lopez, Diana C. C.; Wozny, Guenter] Tech Univ Berlin, Chair Proc Dynam & Operat, Sekr KWT 9,Str 17,Juni 135, D-10623 Berlin, Germany. [Flores-Tlacuahuac, Antonio] Tecnol Monterrey, Escuela Ingn Ciencias, Campus Monterrey,Ave Eugenio Garza Sada 2501, Monterrey 64849, NL, Mexico. [Vasquez-Medrano, Ruben] Univ Iberoamer, Dept Ingn & Ciencias Quim, Prolongac Paseo de la Reforma 880, Mexico City 01210, DF, Mexico. [Zavala, Victor M.] Argonne Natl Lab, Math & Comp Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Zavala, Victor M.] Univ Wisconsin, Chem & Biol Engn, 1415 Engn Dr, Madison, WI 53706 USA. RP Lopez, CDC (reprint author), Tech Univ Berlin, Chair Proc Dynam & Operat, Sekr KWT 9,Str 17,Juni 135, D-10623 Berlin, Germany. EM diana.lopez@mailbox.tu-berlin.de FU U.S. Department of Energy [DE-ACO2-06CH11357]; Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) [TRR 63]; German Academic Interchange Service (DAAD) FX This work was supported by the U.S. Department of Energy, under Contract No. DE-ACO2-06CH11357 and is part of the Collaborative Research Center/. Transregio 63 "Integrated Chemical Processes in Liquid Multiphase Systems" (subproject C4). Financial support by the Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) is gratefully acknowledged (TRR 63). Diana C. Lopez C. gratefully acknowledges the financial support from the German Academic Interchange Service (DAAD) for a doctoral stipend. NR 54 TC 0 Z9 0 U1 2 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD MAR 23 PY 2016 VL 55 IS 11 BP 3026 EP 3042 DI 10.1021/acs.iecr.5b03910 PG 17 WC Engineering, Chemical SC Engineering GA DH5TK UT WOS:000372854600012 ER PT J AU Conley, MP Lapadula, G Sanders, K Gajan, D Lesage, A del Rosa, I Maron, L Lukens, WW Coperet, C Andersen, RA AF Conley, Matthew P. Lapadula, Giuseppe Sanders, Kevin Gajan, David Lesage, Anne del Rosa, Iker Maron, Laurent Lukens, Wayne W. Coperet, Christophe Andersen, Richard A. TI The Nature of Secondary Interactions at Electrophilic Metal Sites of Molecular and Silica-Supported Organolutetium Complexes from Solid-State NMR Spectroscopy SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID OPENING METATHESIS POLYMERIZATION; RAY CRYSTAL-STRUCTURE; GENERALIZED GRADIENT APPROXIMATION; SURFACE ORGANOMETALLIC CHEMISTRY; DEFINED HETEROGENEOUS CATALYSTS; CONSISTENT PERTURBATION-THEORY; IMIDO ALKYLIDENE COMPLEXES; AGOSTIC INTERACTIONS; C-H; STRUCTURAL-CHARACTERIZATION AB Lu[CH(SiMe3)(2)](3) reacts with [SiO2-700] to give [(equivalent to SiO)Lu[CH(SiMe3)(2)](2)] and CH2(SiMe3)(2). [(equivalent to SiO)Lu[CH(SiMe3)(2)](2)] is characterized by solid-state NMR and EXAFS spectroscopy, which show that secondary Lu center dot center dot center dot C and Lu center dot center dot center dot O interactions, involving a gamma-CH3 and a siloxane bridge, are present. From X-ray crystallographic analysis, the molecular analogues Lu[CH(SiMe3)(2)](3),[O-2,6-tBu-C6H3](x) (x = 0-2) also have secondary Lu center dot center dot center dot C interactions. The H-1 NMR spectrum of Lu[CH(SiMe3)(2)](3) shows that the -SiMe3 groups are equivalent to -125 degrees C and inequivalent below that temperature, Delta G((Te = 148 K))(double dagger) = 7.1 kcal mol(-1). Both -SiMe3 groups in Lu[CH(SiMe3)(2)](3) have (1)J(CH) = 117 +/- 1 Hz at -140 degrees C. The solid-state C-13 CPMAS NMR spectrum at 20 degrees C shows three chemically inequivalent resonances in the area ratio of 4:1:1 (12:3:3); the J-resolved spectra for each resonance give (1)J(CH) = 117 +/- 2 Hz. The Si-29 CPMAS NMR spectrum shows two chemically inequivalent resonances with different values of chemical shift anisotropy. Similar observations are obtained for Lu[CH(SiMe3)(2)](3),[O-2,6-tBu-C6H3](x) (x = 1 and 2). The spectroscopic data point to short Lu center dot center dot center dot C gamma contacts corresponding to 3c-2e Lu center dot center dot center dot C gamma-Si beta interactions, which are supported by DFT calculations. Calculated natural bond orbital (NBO) charges show that C gamma carries a negative charge, while Lu, H gamma, and Si beta carry positive charges; as the number of O-based ligands increases so does the positive charge at Lu, which in turns shortens the Lu center dot center dot center dot C gamma distance. The change in NBO charges and the resulting changes in the spectroscopic and crystallographic properties show how ligands and surface-support sites rearrange to accommodate these changes, consistent with Pauling's electroneutrality concept. C1 [Conley, Matthew P.; Lapadula, Giuseppe; Coperet, Christophe] ETH, Dept Chem & Appl Biosci, Vladimir Prelog Weg 1-5, CH-8093 Zurich, Switzerland. [Sanders, Kevin; Gajan, David; Lesage, Anne] Univ Lyon 1, Ctr RMN Tres Hauts Champs, CRNS, ENS Lyon, 5 Rue Doua, F-69100 Villeurbanne, France. [del Rosa, Iker; Maron, Laurent] Univ Toulouse, 135 Ave Rangueil, F-31077 Toulouse 4, France. [del Rosa, Iker; Maron, Laurent] CNRS, LPCNO, INSA, UPS, 135 Ave Rangueil, F-31077 Toulouse 4, France. [Lukens, Wayne W.] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Andersen, Richard A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Coperet, C (reprint author), ETH, Dept Chem & Appl Biosci, Vladimir Prelog Weg 1-5, CH-8093 Zurich, Switzerland.; Andersen, RA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM ccoperet@ethz.ch; raandersen@lbl.gov FU Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Biosciences, and Geosciences Division (CSGB) [DE-AC02-05CH11231]; HPCs CALcul en Midi-Pyrennes (CALIMP-EOS) [P0833]; TGIR-RMN-THC, CNRS [Fr3050] FX C.C. thanks the Miller Institute for a Visiting Professor position at UC Berkeley, during which this manuscript was finalized. Portions of this work were performed at Lawrence Berkeley National Laboratory under contract no. DE-AC02-05CH11231 and at the Stanford Synchrotron Radiation Lightsource (SSRL). Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under contract no. DE-AC02-76SF00515. Portions of this work were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Biosciences, and Geosciences Division (CSGB), Heavy Element Chemistry Program and were performed at Lawrence Berkeley National Laboratory under contract no. DE-AC02-05CH11231. We also thank the HPCs CALcul en Midi-Pyrennes (CALIMP-EOS, grant P0833) for the generous allocation of computer time. Financial support from the TGIR-RMN-THC Fr3050 CNRS for conducting the research is gratefully acknowledged. NR 96 TC 2 Z9 2 U1 13 U2 35 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 23 PY 2016 VL 138 IS 11 BP 3831 EP 3843 DI 10.1021/jacs.6b00071 PG 13 WC Chemistry, Multidisciplinary SC Chemistry GA DH5TG UT WOS:000372854200032 PM 26887899 ER PT J AU Neel, AJ Milo, A Sigman, MS Toste, FD AF Neel, Andrew J. Milo, Anat Sigman, Matthew S. Toste, F. Dean TI Enantiodivergent Fluorination of Allylic Alcohols: Data Set Design Reveals Structural Interplay between Achiral Directing Group and Chiral Anion SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID PHASE-TRANSFER CATALYSIS; FREE-ENERGY RELATIONSHIPS; NONLINEAR HAMMETT RELATIONSHIPS; WAGNER-MEERWEIN REARRANGEMENT; SEMI-PINACOL REARRANGEMENT; DOT-PI INTERACTIONS; ASYMMETRIC CATALYSIS; LONE-PAIR; ENANTIOSELECTIVE FLUORINATION; AROMATIC INTERACTIONS AB Enantioselectivity values represent relative rate measurements that are sensitive to the structural features of the substrates and catalysts interacting to produce them. Therefore, well-designed enantioselectivity data sets are information rich and can provide key insights regarding specific molecular interactions. However, if the mechanism for enantioselection varies throughout a data set, these values cannot be easily compared. This premise, which is the crux of free energy relationships, exposes a challenging issue of identifying mechanistic breaks within multivariate correlations. Herein, we describe an approach to addressing this problem in the context of a chiral phosphoric acid catalyzed fluorination of allylic alcohols using aryl boronic acids as transient directing groups. By designing a data set in which both the phosphoric and boronic acid structures were systematically varied, key enantioselectivity outliers were identified and analyzed. A mechanistic study was executed to reveal the structural origins of these outliers, which was consistent with the presence of several mechanistic regimes within the data set. While 2- and 4-substituted aryl boronic acids favored the (R)-enantiomer with most of the studied catalysts, meta-alkoxy substituted aryl boronic acids resulted in the (S)-enantiomer when used in combination with certain (R)-phosphoric acids. We propose that this selectivity reversal is the result of a lone pair-pi interaction between the substrate ligated boronic acid and the phosphate. On the basis of this proposal, a catalyst system was identified, capable of producing either enantiomer in high enantioselectivity (77% (R)-2 to 92% (S)-2) using the same chiral catalyst by subtly changing the structure of the achiral boronic acid. C1 [Neel, Andrew J.; Toste, F. Dean] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Neel, Andrew J.; Toste, F. Dean] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Milo, Anat; Sigman, Matthew S.] Univ Utah, Dept Chem, 315 South 1400 East, Salt Lake City, UT 84112 USA. [Milo, Anat] Ben Gurion Univ Negev, Dept Chem, IL-84105 Beer Sheva, Israel. RP Toste, FD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.; Toste, FD (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Sigman, MS (reprint author), Univ Utah, Dept Chem, 315 South 1400 East, Salt Lake City, UT 84112 USA. EM sigman@chem.utah.edu; fdtoste@berkeley.edu FU NSF [CHE-0749506, CHE-1361296]; National Institute of General Medical Sciences [R01 GM104534]; Center for High Performance Computing at the University of Utah FX We thank the NSF (CHE-0749506 and CHE-1361296) and the National Institute of General Medical Sciences (R01 GM104534) for partial support of this work. The support and resources from the Center for High Performance Computing at the University of Utah are gratefully acknowledged. Eiji Yamamoto, Matt Larsen, Weiwei Zi, and Willie Wolf are acknowledged for helpful discussions. NR 123 TC 10 Z9 10 U1 21 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 23 PY 2016 VL 138 IS 11 BP 3863 EP 3875 DI 10.1021/jacs.6b00356 PG 13 WC Chemistry, Multidisciplinary SC Chemistry GA DH5TG UT WOS:000372854200035 PM 26967114 ER PT J AU Adare, A Aidala, C Ajitanand, NN Akiba, Y Akimoto, R Alexander, J Alfred, M Aoki, K Apadula, N Aramaki, Y Asano, H Aschenauer, EC Atomssa, ET Awes, TC Azmoun, B Babintsev, V Bai, M Bai, X Bandara, NS Bannier, B Barish, KN Bassalleck, B Bathe, S Baublis, V Baumann, C Baumgart, S Bazilevsky, A Beaumier, M Beckman, S Belmont, R Berdnikov, A Berdnikov, Y Black, D Blau, DS Bok, JS Boyle, K Brooks, ML Bryslawskyj, J Buesching, H Bumazhnov, V Butsyk, S Campbell, S Chen, CH Chi, CY Chiu, M Choi, IJ Choi, JB Choi, S Choudhury, RK Christiansen, P Chujo, T Chvala, O Cianciolo, V Citron, Z Cole, BA Connors, M Cronin, N Crossette, N Csanad, M Csorgo, T Dairaku, S Danley, TW Datta, A Daugherity, MS David, G DeBlasio, K Dehmelt, K Denisov, A Deshpande, A Desmond, EJ Dietzsch, O Ding, L Dion, A Diss, PB Do, JH Donadelli, M D'Orazio, L Drapier, O Drees, A Drees, KA Durham, JM Durum, A Edwards, S Efremenko, YV Engelmore, T Enokizono, A En'yo, H Esumi, S Eyser, KO Fadem, B Feege, N Fields, DE Finger, M Finger, M Fleuret, F Fokin, SL Frantz, JE Franz, A Frawley, AD Fukao, Y Fusayasu, T Gainey, K Gal, C Gallus, P Garg, P Garishvili, A Garishvili, I Ge, H Giordano, F Glenn, A Gong, X Gonin, M Goto, Y de Cassagnac, RG Grau, N Greene, SV Perdekamp, MG Gu, Y Gunji, T Guragain, H Hachiya, T Haggerty, JS Hahn, KI Hamagaki, H Hamilton, HF Han, SY Hanks, J Hasegawa, S Haseler, TOS Hashimoto, K Hayano, R Hayashi, S He, X Hemmick, TK Hester, T Hill, JC Hollis, RS Homma, K Hong, B Horaguchi, T Hoshino, T Hotvedt, N Huang, J Huang, S Ichihara, T Iinuma, H Ikeda, Y Imai, K Imazu, Y Imrek, J Inaba, M Iordanova, A Isenhower, D Isinhue, A Ivanishchev, D Jacak, BV Javani, M Jeon, SJ Jezghani, M Jia, J Jiang, X Johnson, BM Joo, E Joo, KS Jouan, D Jumper, DS Kamin, J Kanda, S Kang, BH Kang, JH Kang, JS Kapustinsky, J Karatsu, K Kawall, D Kazantsev, AV Kempel, T Key, JA Khachatryan, V Khandai, PK Khanzadeev, A Kihara, K Kijima, KM Kim, BI Kim, C Kim, DH Kim, DJ Kim, EJ Kim, GW Kim, HJ Kim, M Kim, YJ Kim, YK Kimelman, B Kinney, E Kistenev, E Kitamura, R Klatsky, J Kleinjan, D Kline, P Koblesky, T Kofarago, M Komkov, B Koster, J Kotchetkov, D Kotov, D Krizek, F Kurita, K Kurosawa, M Kwon, Y Kyle, GS Lacey, R Lai, YS Lajoie, JG Lebedev, A Lee, DM Lee, GH Lee, J Lee, KB Lee, KS Lee, S Lee, SH Lee, SR Leitch, MJ Leite, MAL Leitgab, M Lewis, B Li, X Lim, SH Levy, LAL Liu, MX Lynch, D Maguire, CF Makdisi, YI Makek, M Manion, A Manko, VI Mannel, E Maruyama, T McCumber, M McGaughey, PL McGlinchey, D McKinney, C Meles, A Mendoza, M Meredith, B Miake, Y Mibe, T Midori, J Mignerey, AC Miller, AJ Milov, A Mishra, DK Mitchell, JT Miyasaka, S Mizuno, S Mohanty, AK Mohapatra, S Montuenga, P Moon, HJ Moon, T Morrison, DP Moskowitz, M Moukhanova, TV Murakami, T Murata, J Mwai, A Nagae, T Nagamiya, S Nagashima, K Nagle, JL Nagy, MI Nakagawa, I Nakagomi, H Nakamiya, Y Nakamura, KR Nakamura, T Nakano, K Nattrass, C Netrakanti, PK Nihashi, M Niida, T Nishimura, S Nouicer, R Novak, T Novitzky, N Nukariya, A Nyanin, AS Obayashi, H O'Brien, E Ogilvie, CA Oide, H Okada, K Koop, JDO Osborn, JD Oskarsson, A Ozaki, H Ozawa, K Pak, R Pantuev, V Papavassiliou, V Park, IH Park, JS Park, S Park, SK Pate, SF Patel, L Patel, M Pei, H Peng, JC Perepelitsa, DV Perera, GDN Peressounko, DY Perry, J Petti, R Pinkenburg, C Pinson, R Pisani, RP Purschke, ML Qu, H Rak, J Ramson, BJ Ravinovich, I Read, KF Reynolds, D Riabov, V Riabov, Y Richardson, E Rinn, T Riveli, N Roach, D Roche, G Rolnick, SD Rosati, M Rowan, Z Rubin, JG Ryu, MS Sahlmueller, B Saito, N Sakaguchi, T Sako, H Samsonov, V Sarsour, M Sato, S Sawada, S Schaefer, B Schmoll, BK Sedgwick, K Seele, J Seidl, R Sekiguchi, Y Sen, A Seto, R Sett, P Sexton, A Sharma, D Shaver, A Shein, I Shibata, TA Shigaki, K Shimomura, M Shoji, K Shukla, P Sickles, A Silva, CL Silvermyr, D Sim, KS Singh, BK Singh, CP Singh, V Skolnik, M Slunecka, M Snowball, M Solano, S Soltz, RA Sondheim, WE Sorensen, SP Sourikova, IV Stankus, PW Steinberg, P Stenlund, E Stepanov, M Ster, A Stoll, SP Stone, MR Sugitate, T Sukhanov, A Sumita, T Sun, J Sziklai, J Takagui, EM Takahara, A Taketani, A Tanaka, Y Taneja, S Tanida, K Tannenbaum, MJ Tarafdar, S Taranenko, A Tennant, E Tieulent, R Timilsina, A Todoroki, T Tomasek, M Torii, H Towell, CL Towell, M Towell, R Towell, RS Tserruya, I Tsuchimoto, Y Vale, C van Hecke, HW Vargyas, M Vazquez-Zambrano, E Veicht, A Velkovska, J Vertesi, R Virius, M Voas, B Vrba, V Vznuzdaev, E Wang, XR Watanabe, D Watanabe, K Watanabe, Y Watanabe, YS Wei, F Whitaker, S White, AS White, SN Winter, D Wolin, S Woody, CL Wysocki, M Xia, B Xue, L Yalcin, S Yamaguchi, YL Yanovich, A Ying, J Yokkaichi, S Yoo, JH Yoon, I You, Z Younus, I Yu, H Yushmanov, IE Zajc, WA Zelenski, A Zhou, S Zou, L AF Adare, A. 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CA PHENIX Collaboration TI Measurement of parity-violating spin asymmetries in W-+/- production at midrapidity in longitudinally polarized p plus p collisions SO PHYSICAL REVIEW D LA English DT Article ID MUON-PROTON; SCATTERING; DISTRIBUTIONS; PHYSICS; G1 AB We present midrapidity measurements from the PHENIX experiment of large parity-violating single-spin asymmetries of high transverse momentum electrons and positrons from W-+/-/Z decays, produced in longitudinally polarized p + p collisions at center of mass energies of root s = 500 and 510 GeV. These asymmetries allow direct access to the antiquark polarized parton distribution functions due to the parity-violating nature of the W-boson coupling to quarks and antiquarks. The results presented are based on data collected in 2011, 2012, and 2013 with an integrated luminosity of 240 pb(-1), which exceeds previous PHENIX published results by a factor of more than 27. 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[Shimomura, M.] Nara Womens Univ, Kita Uoya Nishi Machi, Nara 6308506, Japan. [Riabov, V.; Samsonov, V.; Taranenko, A.] Natl Res Nucl Univ, MEPhI, Moscow Engn Phys Inst, Moscow 115409, Russia. [Bassalleck, B.; Bok, J. S.; Butsyk, S.; Datta, A.; DeBlasio, K.; Fields, D. E.; Key, J. A.; Younus, I.] Univ New Mexico, Albuquerque, NM 87131 USA. [Bok, J. S.; Kyle, G. S.; Meles, A.; Papavassiliou, V.; Pate, S. F.; Perera, G. D. N.; Tennant, E.; Wang, X. R.; Wei, F.] New Mexico State Univ, Las Cruces, NM 88003 USA. [Danley, T. W.; Frantz, J. E.; Kotchetkov, D.; Riveli, N.; Xia, B.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Awes, T. C.; Cianciolo, V.; Efremenko, Y. V.; Enokizono, A.; Read, K. F.; Silvermyr, D.; Stankus, P. W.; Wysocki, M.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Jouan, D.] Univ Paris Saclay, Univ Paris Sud, IPN Orsay, CNRS,IN2P3, BP1, F-91406 Orsay, France. [Yu, H.] Peking Univ, Beijing 100871, Peoples R China. [Baublis, V.; Ivanishchev, D.; Khanzadeev, A.; Komkov, B.; Kotov, D.; Riabov, V.; Riabov, Y.; Samsonov, V.; Vznuzdaev, E.] Petersburg Nucl Phys Inst, Gatchina 188300, Leningrad Regio, Russia. [Akiba, Y.; Aoki, K.; Aramaki, Y.; Asano, H.; Baumgart, S.; Dairaku, S.; Enokizono, A.; En'yo, H.; Fukao, Y.; Goto, Y.; Hachiya, T.; Hashimoto, K.; Ichihara, T.; Ikeda, Y.; Imazu, Y.; Kanda, S.; Karatsu, K.; Kurita, K.; Kurosawa, M.; Miyasaka, S.; Mizuno, S.; Murakami, T.; Murata, J.; Nagamiya, S.; Nakagawa, I.; Nakagomi, H.; Nakamura, K. R.; Nakamura, T.; Nakano, K.; Nihashi, M.; Seidl, R.; Shibata, T. -A.; Shoji, K.; Sumita, T.; Taketani, A.; Todoroki, T.; Watanabe, K.; Watanabe, Y.; Yokkaichi, S.] RIKEN, Nishina Ctr Accelerator Based Sci, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. 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N.; Alexander, J.; Gong, X.; Gu, Y.; Jia, J.; Lacey, R.; Mohapatra, S.; Mwai, A.; Reynolds, D.; Taranenko, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Apadula, N.; Atomssa, E. T.; Bannier, B.; Chen, C. -H.; Citron, Z.; Connors, M.; Cronin, N.; Dehmelt, K.; Deshpande, A.; Dion, A.; Drees, A.; Durham, J. M.; Feege, N.; Gal, C.; Ge, H.; Hanks, J.; Hemmick, T. K.; Jacak, B. V.; Kamin, J.; Khachatryan, V.; Kline, P.; Lee, S. H.; Lewis, B.; Manion, A.; Novitzky, N.; Petti, R.; Sahlmueller, B.; Sharma, D.; Sun, J.; Taneja, S.; Yalcin, S.; Yamaguchi, Y. L.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Garishvili, A.; Nattrass, C.; Read, K. F.; Schmoll, B. K.; Sen, A.; Sorensen, S. P.] Univ Tennessee, Knoxville, TN 37996 USA. [Miyasaka, S.; Nakano, K.; Shibata, T. -A.] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Chujo, T.; Esumi, S.; Horaguchi, T.; Ikeda, Y.; Inaba, M.; Kihara, K.; Miake, Y.; Mizuno, S.; Nakagomi, H.; Niida, T.; Ozaki, H.; Shimomura, M.; Todoroki, T.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki 305, Japan. [Belmont, R.; Greene, S. V.; Huang, S.; Maguire, C. F.; Roach, D.; Schaefer, B.; Velkovska, J.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Citron, Z.; Makek, M.; Milov, A.; Ravinovich, I.; Sharma, D.; Tarafdar, S.; Tserruya, I.] Weizmann Inst Sci, IL-76100 Rehovot, Israel. [Csorgo, T.; Nagy, M. I.; Novak, T.; Ster, A.; Sziklai, J.; Vargyas, M.; Vertesi, R.] Hungarian Acad Sci, Wigner Res Ctr Phys, Inst Particle & Nucl Phys, RMKI, POB 49, H-1525 Budapest 114, Hungary. [Do, J. H.; Kang, J. H.; Kim, H. -J.; Kwon, Y.; Lee, S.; Lim, S. H.; Moon, T.] Yonsei Univ, IPAP, Seoul 120749, South Korea. [Makek, M.] Univ Zagreb, Fac Sci, Dept Phys, Bijenicka 32, HR-10002 Zagreb, Croatia. RP Morrison, DP (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.; Nagle, JL (reprint author), Univ Colorado, Boulder, CO 80309 USA. EM morrison@bnl.gov; jamie.nagle@colorado.edu RI Durum, Artur/C-3027-2014; Sen, Abhisek/J-1157-2016; Nattrass, Christine/J-6752-2016; Sorensen, Soren /K-1195-2016; Hayano, Ryugo/F-7889-2012; Yokkaichi, Satoshi/C-6215-2017; Taketani, Atsushi/E-1803-2017 OI Sen, Abhisek/0000-0003-1192-3938; Nattrass, Christine/0000-0002-8768-6468; Sorensen, Soren /0000-0002-5595-5643; Hayano, Ryugo/0000-0002-1214-7806; Taketani, Atsushi/0000-0002-4776-2315 FU Office of Nuclear Physics in the Office of Science of the Department of Energy (U.S.); National Science Foundation (U.S.); Abilene Christian University Research Council (U.S.); Research Foundation of SUNY (U.S.); Dean of the College of Arts and Sciences, Vanderbilt University (U.S.); Japan Society for the Promotion of Science (Japan); Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (Brazil); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil); Natural Science Foundation of China (People's Republic of China); Croatian Science Foundation (Croatia); Ministry of Science, Education, and Sports (Croatia); Ministry of Education, Youth and Sports (Czech Republic); Centre National de la Recherche Scientifique (France); Commissariat a l'Energie Atomique (France); Institut National de Physique Nucleaire et de Physique des Particules (France); Bundesministerium fur Bildung und Forschung (Germany); Deutscher Akademischer Austausch Dienst (Germany); Alexander von Humboldt Stiftung (Germany); National Science Fund (Hungary); OTKA (Hungary); Karoly Robert University College (Hungary); Ch. Simonyi Fund (Hungary); Department of Atomic Energy (India); Department of Science and Technology (India); Israel Science Foundation (Israel); Basic Science Research Program through NRF of the Ministry of Education (Korea); Physics Department, Lahore University of Management Sciences (Pakistan); Ministry of Education and Science, Russian Academy of Sciences, Federal Agency of Atomic Energy (Russia); VR (Sweden); Wallenberg Foundation (Sweden); U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union; Hungarian American Enterprise Scholarship Fund; US-Israel Binational Science Foundation; Ministry of Education, Culture, Sports, Science, and Technology (Japan) FX We thank the staff of the Collider-Accelerator and Physics Departments at Brookhaven National Laboratory and the staff of the other PHENIX participating institutions for their vital contributions. We acknowledge support from the Office of Nuclear Physics in the Office of Science of the Department of Energy, the National Science Foundation, Abilene Christian University Research Council, Research Foundation of SUNY, and Dean of the College of Arts and Sciences, Vanderbilt University (U.S.), Ministry of Education, Culture, Sports, Science, and Technology and the Japan Society for the Promotion of Science (Japan), Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (Brazil), Natural Science Foundation of China (People's Republic of China), Croatian Science Foundation and Ministry of Science, Education, and Sports (Croatia), Ministry of Education, Youth and Sports (Czech Republic), Centre National de la Recherche Scientifique, Commissariat a l'Energie Atomique, and Institut National de Physique Nucleaire et de Physique des Particules (France), Bundesministerium fur Bildung und Forschung, Deutscher Akademischer Austausch Dienst, and Alexander von Humboldt Stiftung (Germany), National Science Fund, OTKA, Karoly Robert University College, and the Ch. Simonyi Fund (Hungary), Department of Atomic Energy and Department of Science and Technology (India), Israel Science Foundation (Israel), Basic Science Research Program through NRF of the Ministry of Education (Korea), Physics Department, Lahore University of Management Sciences (Pakistan), Ministry of Education and Science, Russian Academy of Sciences, Federal Agency of Atomic Energy (Russia), VR and Wallenberg Foundation (Sweden), the U.S. Civilian Research and Development Foundation for the Independent States of the Former Soviet Union, the Hungarian American Enterprise Scholarship Fund, and the US-Israel Binational Science Foundation. NR 32 TC 4 Z9 4 U1 8 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 23 PY 2016 VL 93 IS 5 AR 051103 DI 10.1103/PhysRevD.93.051103 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH3XR UT WOS:000372720600001 ER PT J AU Ling, X Lin, YX Ma, Q Wang, ZQ Song, Y Yu, LL Huang, SX Fang, WJ Zhang, X Hsu, AL Bie, YQ Lee, YH Zhu, YM Wu, LJ Li, J Jarillo-Herrero, P Dresselhaus, M Palacios, T Kong, J AF Ling, Xi Lin, Yuxuan Ma, Qiong Wang, Ziqiang Song, Yi Yu, Lili Huang, Shengxi Fang, Wenjing Zhang, Xu Hsu, Allen L. Bie, Yaqing Lee, Yi-Hsien Zhu, Yimei Wu, Lijun Li, Ju Jarillo-Herrero, Pablo Dresselhaus, Mildred Palacios, Tomas Kong, Jing TI Parallel Stitching of 2D Materials SO ADVANCED MATERIALS LA English DT Article ID HEXAGONAL BORON-NITRIDE; LATERAL HETEROSTRUCTURES; INPLANE HETEROSTRUCTURES; MOLYBDENUM-DISULFIDE; EPITAXIAL-GROWTH; GRAPHENE; ELECTRONICS; FILMS; HETEROJUNCTIONS; LAYERS AB Diverse parallel stitched 2D heterostructures, including metal-semiconductor, semiconductor-semiconductor, and insulator-semiconductor, are synthesized directly through selective "sowing" of aromatic molecules as the seeds in the chemical vapor deposition (CVD) method. The methodology enables the large-scale fabrication of lateral hetero structures, which offers tremendous potential for its application in integrated circuits. C1 [Ling, Xi; Lin, Yuxuan; Song, Yi; Yu, Lili; Huang, Shengxi; Fang, Wenjing; Zhang, Xu; Hsu, Allen L.; Dresselhaus, Mildred; Palacios, Tomas; Kong, Jing] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA. [Ma, Qiong; Bie, Yaqing; Jarillo-Herrero, Pablo; Dresselhaus, Mildred] MIT, Dept Phys, Cambridge, MA 02139 USA. [Wang, Ziqiang; Li, Ju] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA. [Lee, Yi-Hsien] Natl Tsing Hua Univ, Mat Sci & Engn, Hsinchu 20013, Taiwan. [Zhu, Yimei; Wu, Lijun] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Li, Ju] MIT, Dept Nucl Sci & Engn, 77 Massachusetts Ave, Cambridge, MA 02139 USA. RP Palacios, T; Kong, J (reprint author), MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA. EM tpalacios@mit.edu; jingkong@mit.edu RI Li, Ju/A-2993-2008 OI Li, Ju/0000-0002-7841-8058 FU U.S. Army Research Office through the MIT Institute for Soldier Nanotechnologies [023674]; National Science Foundation (NSF) [NSF/DMR 1004147]; Department of Energy (DOE) [DE-SC0001299]; Office of Naval Research (ONR) Presidential Early Career Awards for Scientists and Engineers (PECASE) program [021302-001]; DOE-Basic Energy Sciences (BES)/Materials Science and Engineering (MSE) division [DE-AC02-98CH10886]; Ministry of Science and Technology of the Republic of China [MOST 103-2112-M-007-001-MY3]; National Science Foundation under NSF [ECS-0335765] FX X.L. and Y.L. contributed equally to this work. This work was supported by the U.S. Army Research Office through the MIT Institute for Soldier Nanotechnologies, under Award No. 023674. X.L., Y.L., and M.D. acknowledge partial support from the National Science Foundation (NSF) under Award No. NSF/DMR 1004147. X.L. and M.D. acknowledge partial support from the Department of Energy (DOE) under Award No. DE-SC0001299. Y.L. and T.P. acknowledge the support from the Office of Naval Research (ONR) Presidential Early Career Awards for Scientists and Engineers (PECASE) program under Award No. 021302-001. Y.Z. and L.W. acknowledge the support from DOE-Basic Energy Sciences (BES)/Materials Science and Engineering (MSE) division under Contract No. DE-AC02-98CH10886. Y.-H.L. acknowledges partial support from the Ministry of Science and Technology of the Republic of China (MOST 103-2112-M-007-001-MY3). This work was performed in part at the Center for Nanoscale Systems (CNS), a member of the National Nanotechnology Infrastructure Network (NNIN), which is supported by the National Science Foundation under NSF Award No. ECS-0335765. CNS is part of Harvard University. Device fabrications were made in MIT Microsystems Technology Laboratories (MTL). TEM characterization was carried out at Brookhaven National Laboratory and at MIT Center for Material Science and Engineering (CMSE). The authors thank Xiang Zhou, Xiaoting Jia, Albert D. Liao, Xiang Ji, and Edbert J. Sie for their help and advice. NR 27 TC 14 Z9 14 U1 42 U2 118 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD MAR 23 PY 2016 VL 28 IS 12 BP 2322 EP 2329 DI 10.1002/adma.201505070 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DH0GB UT WOS:000372459600004 PM 26813882 ER PT J AU Goff, J Sulaiman, S Arkles, B Lewicki, JP AF Goff, Jonathan Sulaiman, Santy Arkles, Barry Lewicki, James P. TI Soft Materials with Recoverable Shape Factors from Extreme Distortion States SO ADVANCED MATERIALS LA English DT Article ID POLYMERS; RELAXATION; MELT AB Elastomeric polysiloxane nanocomposites with elongations of >5000% (more than 3x greater than any previously reported material) with excellent shape recovery are presented. Highly deformable materials are desirable for the fabrication of stretchable implants and microfluidic devices. No crosslinking or domain formation is observed by a variety of analytical techniques, suggesting that their elastomeric behavior is caused by polymer chain entanglements. C1 [Goff, Jonathan; Sulaiman, Santy; Arkles, Barry] Gelest Inc, 11 East Steel Rd, Morrisville, PA 19067 USA. [Lewicki, James P.] Lawrence Livermore Natl Lab, 700 East Ave, Livermore, CA 94550 USA. RP Goff, J; Arkles, B (reprint author), Gelest Inc, 11 East Steel Rd, Morrisville, PA 19067 USA. EM jgoff@gelest.com OI Arkles, Barry/0000-0003-4580-2579 FU Department of Energy [DE-AC52-07NA27344] FX Portions of this work were performed at Lawrence Livermore National Laboratory under the auspices of the Department of Energy under Contract No. DE-AC52-07NA27344. NR 39 TC 3 Z9 3 U1 6 U2 38 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD MAR 23 PY 2016 VL 28 IS 12 BP 2393 EP 2398 DI 10.1002/adma.201503320 PG 6 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DH0GB UT WOS:000372459600013 PM 26786598 ER PT J AU Crawford, HL Fallon, P Macchiavelli, AO Poves, A Bader, VM Bazin, D Bowry, M Campbell, CM Carpenter, MP Clark, RM Cromaz, M Gade, A Ideguchi, E Iwasaki, H Langer, C Lee, IY Loelius, C Lunderberg, E Morse, C Richard, AL Rissanen, J Smalley, D Stroberg, SR Weisshaar, D Whitmore, K Wiens, A Williams, SJ Wimmer, K Yamamato, T AF Crawford, H. L. Fallon, P. Macchiavelli, A. O. Poves, A. Bader, V. M. Bazin, D. Bowry, M. Campbell, C. M. Carpenter, M. P. Clark, R. M. Cromaz, M. Gade, A. Ideguchi, E. Iwasaki, H. Langer, C. Lee, I. Y. Loelius, C. Lunderberg, E. Morse, C. Richard, A. L. Rissanen, J. Smalley, D. Stroberg, S. R. Weisshaar, D. Whitmore, K. Wiens, A. Williams, S. J. Wimmer, K. Yamamato, T. TI Rotational band structure in Mg-32 SO PHYSICAL REVIEW C LA English DT Article ID SHELL CLOSURE; BETA-DECAY; NUCLEI; DEFORMATION; MG-30,MG-32; TRANSITION; STABILITY; FEATURES; MODEL AB There is significant evidence supporting the existence of deformed ground states within the neutron-rich N approximate to 20 neon, sodium, and magnesium isotopes that make up what is commonly called the "island of inversion." However, the rotational band structures, which are a characteristic fingerprint of a rigid nonspherical shape, have yet to be observed. In this work, we report on a measurement and analysis of the yrast (lowest lying) rotational band in Mg-32 up to spin I = 6(+) produced in a two-step projectile fragmentation reaction and observed using the state-of-the-art gamma-ray tracking detector array, GRETINA (gamma-ray energy tracking in-beam nuclear array). Large-scale shell-model calculations using the SDPF-U-MIX effective interaction show excellent agreement with the new data. Moreover, a theoretical analysis of the spectrum of rotational states as a function of the pairing gap, together with cranked-shell-model calculations, provides intriguing evidence for a reduction in pairing correlations with increased angular momentum, also in line with the shell-model results. C1 [Crawford, H. L.; Fallon, P.; Macchiavelli, A. O.; Campbell, C. M.; Clark, R. M.; Cromaz, M.; Lee, I. Y.; Rissanen, J.; Wiens, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Crawford, H. L.; Richard, A. L.] Ohio Univ, Inst Nucl & Particle Phys, Athens, OH 45701 USA. [Crawford, H. L.; Richard, A. L.] Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. [Poves, A.] Univ Autonoma Madrid, Dept Fis Teor, E-28049 Madrid, Spain. [Poves, A.] Univ Autonoma Madrid, CSIC, IFT UAM, E-28049 Madrid, Spain. [Bader, V. M.; Bazin, D.; Bowry, M.; Gade, A.; Iwasaki, H.; Langer, C.; Loelius, C.; Lunderberg, E.; Morse, C.; Smalley, D.; Stroberg, S. R.; Weisshaar, D.; Whitmore, K.; Williams, S. J.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Bader, V. M.; Gade, A.; Iwasaki, H.; Loelius, C.; Lunderberg, E.; Morse, C.; Stroberg, S. R.; Whitmore, K.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Carpenter, M. P.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. [Ideguchi, E.; Yamamato, T.] Osaka Univ, RCNP, Osaka 5670047, Japan. [Wimmer, K.] Univ Tokyo, Dept Phys, Bunkyo Ku, Tokyo 1130033, Japan. RP Crawford, HL (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Crawford, HL (reprint author), Ohio Univ, Inst Nucl & Particle Phys, Athens, OH 45701 USA.; Crawford, HL (reprint author), Ohio Univ, Dept Phys & Astron, Athens, OH 45701 USA. EM hlcrawford@lbl.gov RI Gade, Alexandra/A-6850-2008; Poves, Alfredo/L-2594-2013; Langer, Christoph/L-3422-2016 OI Gade, Alexandra/0000-0001-8825-0976; Poves, Alfredo/0000-0001-7539-388X; FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-05CH11231, DE-AC02-06CH11357]; Department of Energy National Nuclear Security Administration [DE-NA0000979]; National Science Foundation (NSF) [PHY-1102511]; U.S. DOE Office of Science; NSF under Cooperative Agreement [PHY11-02511]; DOE [DE-AC02-05CH11231]; MINECO (Spain) Grant [FPA2014-57196]; Programme "Centros de Excelencia Severo Ochoa" [SEV-2012-0249] FX The authors would like to thank S. Frauendorf for fruitful discussions. We also would like to thank the operations team at NSCL for their work in beam delivery during the experiment. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under Contracts No. DE-AC02-05CH11231 (LBNL) and No. DE-AC02-06CH11357 (ANL), by the Department of Energy National Nuclear Security Administration under Award No. DE-NA0000979 and the National Science Foundation (NSF) under PHY-1102511. GRETINA was funded by the U.S. DOE Office of Science. Operation of the array at NSCL is supported by NSF under Cooperative Agreement PHY11-02511 (NSCL) and DOE under Grant No. DE-AC02-05CH11231 (LBNL). A.P. is partly supported by MINECO (Spain) Grant FPA2014-57196 and Programme "Centros de Excelencia Severo Ochoa" SEV-2012-0249. NR 31 TC 3 Z9 3 U1 3 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 23 PY 2016 VL 93 IS 3 AR 031303 DI 10.1103/PhysRevC.93.031303 PG 5 WC Physics, Nuclear SC Physics GA DH3XI UT WOS:000372719700001 ER PT J AU Alraddadi, S Hines, W Yilmaz, T Gu, GD Sinkovic, B AF Alraddadi, S. Hines, W. Yilmaz, T. Gu, G. D. Sinkovic, B. TI Structural phase diagram for ultra-thin epitaxial Fe3O4/MgO(001) films: thickness and oxygen pressure dependence SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE Fe3O4; epitaxial growth; Verwey transition; thin film; iron oxide ID IRON-OXIDE FILMS; MOLECULAR-BEAM EPITAXY; VERWEY TRANSITION; MAGNETITE; GROWTH; ALPHA-FE2O3; FE3O4; ALPHA-AL2O3(0001); AG(111) AB A systematic investigation of the thickness and oxygen pressure dependence for the structural properties of ultra-thin epitaxial magnetite (Fe3O4) films has been carried out; for such films, the structural properties generally differ from those for the bulk when the thickness <= 10 nm. Iron oxide ultra-thin films with thicknesses varying from 3 nm to 20 nm were grown on MgO (0 0 1) substrates using molecular beam epitaxy under different oxygen pressures ranging from 1 x 10(-7) torr to 1 x 10(-5) torr. The crystallographic and electronic structures of the films were characterized using low energy electron diffraction (LEED) and x-ray photoemission spectroscopy (XPS), respectively. The quality of the epitaxial Fe3O4 ultra-thin films was judged by magnetic measurements of the Verwey transition, along with complementary XPS spectra. It was observed that under the same growth conditions the stoichiometry of ultra-thin films under 10 nm transforms from the Fe3O4 phase to the FeO phase. In this work, a phase diagram based on thickness and oxygen pressure has been constructed to explain the structural phase transformation. It was found that high-quality magnetite films with thicknesses <= 20 nm formed within a narrow range of oxygen pressure. An optimal and controlled growth process is a crucial requirement for the accurate study of the magnetic and electronic properties for ultra-thin Fe3O4 films. Furthermore, these results are significant because they may indicate a general trend in the growth of other oxide films, which has not been previously observed or considered. C1 [Alraddadi, S.; Hines, W.; Yilmaz, T.; Sinkovic, B.] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. [Gu, G. D.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Alraddadi, S (reprint author), Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. EM alraddadi@phys.uconn.edu FU Physics Department at UCONN; Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, U.S. Department of Energy [DE-SC00112704] FX The authors would like to acknowledge the support of the Physics Department at UCONN. The work at Brookhaven was supported by the Office of Basic Energy Sciences, Division of Materials Sciences and Engineering, U.S. Department of Energy under Contract No. DE-SC00112704. We also like to thank Prof Joseph I Budnick for many helpful discussions. NR 29 TC 2 Z9 2 U1 14 U2 59 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAR 23 PY 2016 VL 28 IS 11 AR 115402 DI 10.1088/0953-8984/28/11/115402 PG 8 WC Physics, Condensed Matter SC Physics GA DE6HA UT WOS:000370733400011 PM 26894934 ER PT J AU Forrest, TR Valdivia, PN Rotundu, CR Bourret-Courchesne, E Birgeneau, RJ AF Forrest, T. R. Valdivia, P. N. Rotundu, C. R. Bourret-Courchesne, E. Birgeneau, R. J. TI The effects of post-growth annealing on the structural and magnetic properties of BaFe2As2 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE iron-pnicitide superconductors; structural phase transition; annealing AB We investigate the effects of post-growth annealing on the structural and magnetic properties of BaFe2As2. Magnetic susceptibility measurements, which exhibit a signal corresponding to the magnetic phase transition, and high-resolution x-ray diffraction measurements, which directly probe the structural order parameter, show that annealing causes the ordering temperatures of both the phase transitions to increase, sharpen and converge. In the as grown sample, our measurements show two distinct transitions corresponding to structural and magnetic ordering, which are separated in temperature by approximately 1 K. After 46 days (d) of annealing at 700 degrees C, the two become concurrent in temperature. These measurements demonstrate that the structural phase transition is second-order like when the magnetic and structural phase transitions are separated in temperature, and first-order like when the two phase transition temperatures coincide. This observation indicates that annealing causes the system to cross a hitherto undiscovered tricritical point. In addition, x-ray diffraction measurements show that the c-axis lattice parameter increases with annealing up to 30 d, but remains constant for longer annealing times. Comparisons of BaFe2As2 to SrFe2As2 are made when possible. C1 [Forrest, T. R.; Birgeneau, R. J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Valdivia, P. N.; Birgeneau, R. J.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Rotundu, C. R.; Birgeneau, R. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Bourret-Courchesne, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Forrest, T. R.] European Synchrotron Radiat Facil, BP 220, F-38043 Grenoble, France. [Rotundu, C. R.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. RP Forrest, TR (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Forrest, TR (reprint author), European Synchrotron Radiat Facil, BP 220, F-38043 Grenoble, France. EM forrest@esrf.fr FU US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-05CH11231] FX We thank S Mulcahy, J Heron, R Marks and V Borzenets for their assistance. This work was supported by the US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract No. DE-AC02-05CH11231. Portions of this research were carried out at the Stanford Synchrotron Radiation Lightsource, a Directorate of SLAC National Accelerator Laboratory and an Office of Science User Facility operated for the US Department of Energy Office of Science by Stanford University. NR 31 TC 0 Z9 0 U1 6 U2 14 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAR 23 PY 2016 VL 28 IS 11 AR 115702 DI 10.1088/0953-8984/28/11/115702 PG 8 WC Physics, Condensed Matter SC Physics GA DE6HA UT WOS:000370733400016 PM 26895292 ER PT J AU Zhang, W Lu, WC Zhang, HX Ho, KM Wang, CZ AF Zhang, Wei Lu, Wen-Cai Zhang, Hong-Xing Ho, K. M. Wang, C. Z. TI Tight-binding calculation studies of vacancy and adatom defects in graphene SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE tight-binding calculation; defects in graphene; structure optimization; formation energy ID FILMS; OXIDE AB Computational studies of complex defects in graphene usually need to deal with a larger number of atoms than the current first-principles methods can handle. Here, we show that a recently developed three-center tight-binding potential for carbon is very efficient for large scale atomistic simulations and can accurately describe the structures and energies of various defects in graphene. Using the three-center tight-binding potential, we have systematically studied the stable structures and formation energies of vacancy and embedded-atom defects of various sizes up to four vacancies and four embedded atoms in graphene. Our calculations reveal low-energy defect structures and provide a more comprehensive understanding of the structures and stability of defects in graphene. C1 [Zhang, Wei; Lu, Wen-Cai; Zhang, Hong-Xing] Jilin Univ, Int Joint Res Lab Nanomicro Architecture Chem, Changchun 130023, Jilin, Peoples R China. [Zhang, Wei; Lu, Wen-Cai; Zhang, Hong-Xing] Jilin Univ, Inst Theoret Chem, Changchun 130023, Jilin, Peoples R China. [Zhang, Wei; Ho, K. M.; Wang, C. Z.] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Zhang, Wei; Ho, K. M.; Wang, C. Z.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Lu, Wen-Cai] Qingdao Univ, Dept Phys, Qingdao 266071, Shandong, Peoples R China. [Lu, Wen-Cai] Qingdao Univ, State Key Lab Cultivat Base Adv Fibers & Text Mat, Qingdao 266071, Shandong, Peoples R China. RP Zhang, W (reprint author), Jilin Univ, Int Joint Res Lab Nanomicro Architecture Chem, Changchun 130023, Jilin, Peoples R China.; Zhang, W (reprint author), Jilin Univ, Inst Theoret Chem, Changchun 130023, Jilin, Peoples R China.; Zhang, W; Wang, CZ (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA.; Zhang, W; Wang, CZ (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM zhangw_bxx@jlu.edu.cn; wangcz@ameslab.gov FU China Scholarship Council [201406175053]; National Natural Science Foundation of China [21173096]; State Key Development Program for Basic Research of China [2013CB834801]; US Department of Energy, Basic Energy Sciences, Division of materials Science and Engineering [DE-AC02-07CH11358]; National Energy Research Scientific Computing Centre (NERSC) in Berkeley, CA [DE-AC02-07CH11358] FX W Zhang acknowledges the support from China Scholarship Council (File NO.201406175053) to work as a visiting scientist at Ames Laboratory where most of the work for this paper was carried out. W Zhang and H X Zhang were also supported by the National Natural Science Foundation of China (Grant No.21173096) and the State Key Development Program for Basic Research of China (Grant No.2013CB834801). Work at Ames Laboratory was supported by the US Department of Energy, Basic Energy Sciences, Division of materials Science and Engineering, including a grant of computer time at the National Energy Research Scientific Computing Centre (NERSC) in Berkeley, CA under Contract No. DE-AC02-07CH11358. NR 28 TC 1 Z9 1 U1 7 U2 22 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAR 23 PY 2016 VL 28 IS 11 AR 115001 DI 10.1088/0953-8984/28/11/115001 PG 10 WC Physics, Condensed Matter SC Physics GA DE6HA UT WOS:000370733400007 PM 26902952 ER PT J AU Fowler, MJ Howard, M Luttman, A Mitchell, SE Webb, TJ AF Fowler, Michael J. Howard, Marylesa Luttman, Aaron Mitchell, Stephen E. Webb, Timothy J. TI A stochastic approach to quantifying the blur with uncertainty estimation for high-energy X-ray imaging systems SO INVERSE PROBLEMS IN SCIENCE AND ENGINEERING LA English DT Article DE inverse problems; pulsed power; X-ray radiography; Markov chain Monte Carlo; uncertainty quantification; bound constrained optimization; 15A29; 65C60; 65F22; 94A08 ID QUANTIFICATION; MCMC; DIFFERENTIATION; RECONSTRUCTION; IMAGES; DIODE; NOISE AB One of the primary causes of blur in a high-energy X-ray imaging system is the shape and extent of the radiation source, or spot'. It is important to be able to quantify the size of the spot as it provides a lower bound on the recoverable resolution for a radiograph, and penumbral imaging methods - which involve the analysis of blur caused by a structured aperture - can be used to obtain the spot's spatial profile. We present a Bayesian approach for estimating the spot shape that, unlike variational methods, is robust to the initial choice of parameters. The posterior is obtained from a normal likelihood, which was constructed from a weighted least squares approximation to a Poisson noise model, and prior assumptions that enforce both smoothness and non-negativity constraints. A Markov chain Monte Carlo algorithm is used to obtain samples from the target posterior, and the reconstruction and uncertainty estimates are the computed mean and variance of the samples, respectively. Synthetic data-sets are used to demonstrate accurate reconstruction, while real data taken with high-energy X-ray imaging systems are used to demonstrate applicability and feasibility. C1 [Fowler, Michael J.; Howard, Marylesa; Luttman, Aaron; Mitchell, Stephen E.] Natl Secur Technol LLC, Nevada Operat, Las Vegas, NV 89030 USA. [Webb, Timothy J.] Sandia Natl Labs, Adv Radiog Technol Dept, Albuquerque, NM 87185 USA. RP Fowler, MJ (reprint author), Natl Secur Technol LLC, Nevada Operat, Las Vegas, NV 89030 USA. EM fowlermj@clarkson.edu FU US Department of Energy [DE-AC52-06NA25946]; Site-Directed Research and Development Program FX The authors would like to thank the US Department of Energy Nevada Radiography Working Group and the RITS research group at Sandia National Laboratories for providing the Cygnus and RITS-6 data, respectively. We also thank Dr Johnathan Bardsley for helpful comments and suggestions on the sampling schemes and the manuscript. This work was done by National Security Technologies, LLC, under Contract No. DE-AC52-06NA25946 with the US Department of Energy and supported by the Site-Directed Research and Development Program. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable and worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. DOE/NV/25946-2015. NR 37 TC 0 Z9 0 U1 0 U2 1 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 1741-5977 EI 1741-5985 J9 INVERSE PROBL SCI EN JI Inverse Probl. Sci. Eng. PD MAR 23 PY 2016 VL 24 IS 3 BP 353 EP 371 DI 10.1080/17415977.2015.1046859 PG 19 WC Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications SC Engineering; Mathematics GA DA6LP UT WOS:000367916500001 ER PT J AU Xu, C Reece, CE Kelley, MJ AF Xu, Chen Reece, Charles E. Kelley, Michael J. TI Simulation of nonlinear superconducting rf losses derived from characteristic topography of etched and electropolished niobium surfaces SO PHYSICAL REVIEW ACCELERATORS AND BEAMS LA English DT Article AB A simplified numerical model has been developed to simulate nonlinear superconducting radiofrequency (SRF) losses on Nb surfaces. This study focuses exclusively on excessive surface resistance (R-s) losses due to the microscopic topographical magnetic field enhancements. When the enhanced local surface magnetic field exceeds the superconducting critical transition magnetic field H-c, small volumes of surface material may become normal conducting and increase the effective surface resistance without inducing a quench. We seek to build an improved quantitative characterization of this qualitative model. Using topographic data from typical buffered chemical polish (BCP)- and electropolish (EP)-treated fine grain niobium, we have estimated the resulting field-dependent losses and extrapolated this model to the implications for cavity performance. The model predictions correspond well to the characteristic BCP versus EP high field Q(0) performance differences for fine grain niobium. We describe the algorithm of the model, its limitations, and the effects of this nonlinear loss contribution on SRF cavity performance. C1 [Xu, Chen; Reece, Charles E.; Kelley, Michael J.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Xu, Chen; Kelley, Michael J.] Coll William & Mary, Dept Appl Sci, Williamsburg, VA 23185 USA. RP Xu, C (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA.; Xu, C (reprint author), Coll William & Mary, Dept Appl Sci, Williamsburg, VA 23185 USA. FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC05-06OR23177] FX This material is based on work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under Contract No. DE-AC05-06OR23177. C. X. is grateful for discussions with Alexander Gurevich in Old Dominion University, Haipeng Wang, Hui Tian and Olga Trofimova at Jefferson Lab, John Delos at College of William and Mary and Toby Driscoll at University of Delaware. NR 34 TC 1 Z9 1 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9888 J9 PHYS REV ACCEL BEAMS JI Phys. Rev. Accel. Beams PD MAR 22 PY 2016 VL 19 IS 3 AR 033501 DI 10.1103/PhysRevAccelBeams.19.033501 PG 13 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DQ6VJ UT WOS:000379343300003 ER PT J AU Batth, I Yun, HY Hussain, S Meng, P Osumulski, P Huang, THM Bedolla, R Profit, A Reddick, R Kumar, A AF Batth, Izhar Yun, Huiyoung Hussain, Suleman Meng, Peng Osumulski, Powel Huang, Tim Hui-Ming Bedolla, Roble Profit, Amanda Reddick, Robert Kumar, Addanki TI Crosstalk between RON and androgen receptor signaling in the development of castration resistant prostate cancer SO ONCOTARGET LA English DT Article DE castrate resistant prostate cancer; apoptosis; FLIP; RON; MSTIR ID EPITHELIAL-MESENCHYMAL TRANSITION; TYROSINE KINASE; PANCREATIC-CANCER; DEPRIVATION THERAPY; ALTERED EXPRESSION; TUMOR PROGRESSION; BREAST-CANCER; C-MET; CELLS; GROWTH AB Castrate-resistant prostate cancer (CRPC) is the fatal form of prostate cancer. Although reactivation of androgen receptor (AR) occurs following androgen deprivation, the precise mechanism involved is unclear. Here we show that the receptor tyrosine kinase, RON alters mechanical properties of cells to influence epithelial to mesenchymal transition and functions as a transcription factor to differentially regulate AR signaling. RON inhibits AR activation and subset of AR-regulated transcripts in androgen responsive LNCaP cells. However in C4-2B, a castrate-resistant sub-line of LNCaP and AR-negative androgen independent DU145 cells, RON activates subset of AR-regulated transcripts. Expression of AR in PC-3 cells leads to activation of RON under androgen deprivation but not under androgen proficient conditions implicating a role for RON in androgen independence. Consistently, RON expression is significantly elevated in castrate resistant prostate tumors. Taken together our results suggest that RON activation could aid in promoting androgen independence and that inhibition of RON in combination with AR antagonist(s) merits serious consideration as a therapeutic option during hormone deprivation therapy. C1 [Batth, Izhar; Meng, Peng; Bedolla, Roble; Kumar, Addanki] Dept Urol, San Antonio, TX USA. [Yun, Huiyoung; Hussain, Suleman; Kumar, Addanki] Univ Texas San Antonio, Hlth Sci Ctr, Dept Pharmacol, 7703 Floyd Curl Dr, San Antonio, TX 78284 USA. [Osumulski, Powel; Huang, Tim Hui-Ming; Kumar, Addanki] Dept Mol Med, San Antonio, TX USA. [Profit, Amanda; Reddick, Robert] Univ Texas San Antonio, Hlth Sci Ctr, Dept Pathol, San Antonio, TX 78284 USA. [Huang, Tim Hui-Ming; Kumar, Addanki] Dept Canc Therapy & Res Ctr, San Antonio, TX USA. [Kumar, Addanki] Univ Texas Hlth Sci Ctr San Antonio, San Antonio, TX 78229 USA. [Kumar, Addanki] South Texas Vet Hlth Care Syst, San Antonio, TX USA. [Meng, Peng] Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA USA. [Batth, Izhar] Univ Texas MD Anderson Canc Ctr, Dept Pediat, Houston, TX 77030 USA. RP Kumar, A (reprint author), Dept Urol, San Antonio, TX USA.; Kumar, A (reprint author), Univ Texas San Antonio, Hlth Sci Ctr, Dept Pharmacol, 7703 Floyd Curl Dr, San Antonio, TX 78284 USA.; Kumar, A (reprint author), Dept Mol Med, San Antonio, TX USA.; Kumar, A (reprint author), Dept Canc Therapy & Res Ctr, San Antonio, TX USA.; Kumar, A (reprint author), Univ Texas Hlth Sci Ctr San Antonio, San Antonio, TX 78229 USA.; Kumar, A (reprint author), South Texas Vet Hlth Care Syst, San Antonio, TX USA. EM kumara3@uthscsa.edu FU Veterans Affairs-Merit Award [I01 BX 000766-01, 1R01CA135451, 1R01AT007448]; CTRC at UT Health Science Center San Antonio (UTHSCSA) through the National Cancer Institute [2P30 CA 054174-17]; CTRC 40th Anniversary Distinguished Professor of Oncology Endowment FX This work was supported in part by funds from Veterans Affairs-Merit Award I01 BX 000766-01, 1R01CA135451 and 1R01AT007448 (APK). We acknowledge support provided by CTRC at UT Health Science Center San Antonio (UTHSCSA) through the National Cancer Institute support grant #2P30 CA 054174-17. We acknowledge support provided by the CTRC 40th Anniversary Distinguished Professor of Oncology Endowment to APK. We thank Dr. JW Freeman, (UTHSCSA) for the RON-reporter; Dr. A. Lowey, (UC-San Diego) for the RON expression plasmid; Dr. D. Tindall, (Mayo Clinic Rochester) for pGL3-PSAARE constructs; and Dr. R. Vadlamudi (UTHSCSA) for providing PC-3AR cells. We sincerely thank Dr. R. Ghosh, (UTHSCSA) for critically reading the manuscript. NR 56 TC 1 Z9 1 U1 0 U2 0 PU IMPACT JOURNALS LLC PI ALBANY PA 6211 TIPTON HOUSE, STE 6, ALBANY, NY 12203 USA SN 1949-2553 J9 ONCOTARGET JI Oncotarget PD MAR 22 PY 2016 VL 7 IS 12 BP 14048 EP 14063 PG 16 WC Oncology; Cell Biology SC Oncology; Cell Biology GA DL5OT UT WOS:000375687200058 PM 26872377 ER PT J AU Deb, N Li, BH Skoda, M Rogers, S Sun, Y Gong, X Karim, A Sumpter, BG Bucknall, DG AF Deb, Nabankur Li, Bohao Skoda, Maximilian Rogers, Sarah Sun, Yan Gong, Xiong Karim, Alamgir Sumpter, Bobby G. Bucknall, David G. TI Harnessing Structure-Property Relationships for Poly(alkyl thiophene)-Fullerene Derivative Thin Films to Optimize Performance in Photovoltaic Devices SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID HETEROJUNCTION SOLAR-CELLS; TRIBLOCK COPOLYMER FILMS; ORGANIC PHOTOVOLTAICS; CONVERSION EFFICIENCY; INDUCED MORPHOLOGY; SELF-ORGANIZATION; SURFACE-ENERGY; POLYMER; P3HT/PCBM; POLY(3-HEXYLTHIOPHENE) AB Nanoscale bulk heterojunction (BHJ) systems, consisting of fullerenes dispersed in conjugated polymers have been actively studied in order to produce high performance organic photovoltaics. How the BHJ morphology affects device efficiency, is currently ill-understood. Neutron reflection together with grazing incidence X-ray and neutron scattering and X-ray photoelectron spectroscopy are utilized to gain understanding of the BHJ morphology in functional devices. For nine model systems, based on mixtures of three poly(3-alkyl thiophenes, P3AT) (A = butyl, hexyl, octyl) blended with three different fullerene derivatives, the BHJ morphology through the film thickness is determined. It is shown that fullerene enrichment occurs at both the electrode interfaces after annealing. The degree of fullerene enrichment is found to strongly correlate with the short circuit current (J(SC)) and to a lesser degree with the fill factor. Based on these findings, it is demonstrated that by deliberately adding a fullerene layer at the electron transport layer interface, J(SC) can be increased by up to 20%, resulting in an overall increase in power conversion efficiency of 5%. C1 [Deb, Nabankur; Bucknall, David G.] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. [Li, Bohao; Sun, Yan; Gong, Xiong; Karim, Alamgir] Univ Akron, Dept Polymer Engn, Akron, OH 44325 USA. [Skoda, Maximilian; Rogers, Sarah] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Sumpter, Bobby G.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Sumpter, Bobby G.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Bucknall, David G.] Heriot Watt Univ, Engn & Phys Sci, Edinburgh EH14 4AS, Midlothian, Scotland. RP Bucknall, DG (reprint author), Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA.; Bucknall, DG (reprint author), Heriot Watt Univ, Engn & Phys Sci, Edinburgh EH14 4AS, Midlothian, Scotland. EM bucknall@gatech.edu RI Sumpter, Bobby/C-9459-2013 OI Sumpter, Bobby/0000-0001-6341-0355 FU U.S. Department of Energy, Division of Basic Energy Sciences [DE-FG02-10ER4779] FX The authors gratefully acknowledge partial support by the U.S. Department of Energy, Division of Basic Energy Sciences under Contract No. DE-FG02-10ER4779. They also thank ISIS Facility, Harwell, UK, for neutron beam time access for the GISANS measurements on SANS2D and SSRL, Stanford, USA, for GIWAXS beam time access on beam line 11-3. They also thank Dr. S. Rogers and Dr. C. Tassone for help during these measurements. The work of B. G. S. was performed at the Center for Nanophase Materials Sciences, a DOE Office of Science User Facility. NR 68 TC 2 Z9 2 U1 8 U2 42 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAR 22 PY 2016 VL 26 IS 12 BP 1908 EP 1920 DI 10.1002/adfm.201502653 PG 13 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DH9QA UT WOS:000373129500005 ER PT J AU Gong, YJ Ye, GL Lei, SD Shi, G He, YM Lin, JH Zhang, X Vajtai, R Pantelides, ST Zhou, W Li, B Ajayan, PM AF Gong, Yongji Ye, Gonglan Lei, Sidong Shi, Gang He, Yongmin Lin, Junhao Zhang, Xiang Vajtai, Robert Pantelides, Sokrates T. Zhou, Wu Li, Bo Ajayan, Pulickel M. TI Synthesis of Millimeter-Scale Transition Metal Dichalcogenides Single Crystals SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID CHEMICAL-VAPOR-DEPOSITION; MOS2 ATOMIC LAYERS; LARGE-AREA; MOLYBDENUM-DISULFIDE; BORON-NITRIDE; COPPER FOILS; PHASE GROWTH; HIGH-QUALITY; GRAPHENE; MONOLAYER AB The emergence of semiconducting transition metal dichalcogenide (TMD) atomic layers has opened up unprecedented opportunities in atomically thin electronics. Yet the scalable growth of TMD layers with large grain sizes and uniformity has remained very challenging. Here is reported a simple, scalable chemical vapor deposition approach for the growth of MoSe2 layers is reported, in which the nucleation density can be reduced from 10(5) to 25 nuclei cm(-2), leading to millimeter-scale MoSe2 single crystals as well as continuous macrocrystalline films with millimeter size grains. The selective growth of monolayers and multilayered MoSe2 films with well-defined stacking orientation can also be controlled via tuning the growth temperature. In addition, periodic defects, such as nanoscale triangular holes, can be engineered into these layers by controlling the growth conditions. The low density of grain boundaries in the films results in high average mobilities, around approximate to 42 cm(2) V-1 s(-1), for back-gated MoSe2 transistors. This generic synthesis approach is also demonstrated for other TMD layers such as millimeter-scale WSe2 single crystals. C1 [Gong, Yongji; Ajayan, Pulickel M.] Rice Univ, Dept Chem, Houston, TX 77005 USA. [Ye, Gonglan; Lei, Sidong; Shi, Gang; He, Yongmin; Vajtai, Robert; Li, Bo; Ajayan, Pulickel M.] Rice Univ, Dept Mat Sci & NanoEngn, Houston, TX 77005 USA. [Lin, Junhao; Zhou, Wu] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Lin, Junhao; Pantelides, Sokrates T.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. RP Ajayan, PM (reprint author), Rice Univ, Dept Chem, Houston, TX 77005 USA.; Li, B; Ajayan, PM (reprint author), Rice Univ, Dept Mat Sci & NanoEngn, Houston, TX 77005 USA. EM Bo.Li@rice.edu; ajayan@rice.edu RI Zhou, Wu/D-8526-2011; Lin, Junhao/D-7980-2015; Gong, Yongji/L-7628-2016 OI Zhou, Wu/0000-0002-6803-1095; Lin, Junhao/0000-0002-2195-2823; FU Army Research Office MURI [W911NF-11-1-0362]; FAME Center, STARnet; Semiconductor Research Corporation program - MARCO; Semiconductor Research Corporation program - DARPA; U.S. Department of Energy, Office of Science, Basic Energy Science, Materials Sciences and Engineering Division; U.S. DOE [DE-FG02-09ER46554]; U.S. Office of Naval Research MURI grant [N000014-09-1-1066]; user project at ORNL's Center for Nanophase Materials Sciences (CNMS), DOE Office of Science User Facility FX Y.G. and G. Y. contributed equally to this work. This work was supported by the Army Research Office MURI grant W911NF-11-1-0362, the FAME Center, one of six centers of STARnet, a Semiconductor Research Corporation program sponsored by MARCO and DARPA, the U.S. Department of Energy, Office of Science, Basic Energy Science, Materials Sciences and Engineering Division (W. Z.), U.S. DOE grant DE-FG02-09ER46554 (J. L., S. T. P.), the U.S. Office of Naval Research MURI grant N000014-09-1-1066, and a user project at ORNL's Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. NR 35 TC 8 Z9 8 U1 43 U2 146 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAR 22 PY 2016 VL 26 IS 12 BP 2009 EP 2015 DI 10.1002/adfm.201504633 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DH9QA UT WOS:000373129500016 ER PT J AU Plonka, AM Chen, XY Wang, H Krishna, R Dong, X Banerjee, D Woerner, WR Han, Y Li, J Parise, JB AF Plonka, Anna M. Chen, Xianyin Wang, Hao Krishna, Rajamani Dong, Xinglong Banerjee, Debasis Woerner, William R. Han, Yu Li, Jing Parise, John B. TI Light Hydrocarbon Adsorption Mechanisms in Two Calcium-Based Microporous Metal Organic Frameworks SO CHEMISTRY OF MATERIALS LA English DT Article ID X-RAY-DIFFRACTION; CARBON-DIOXIDE; SELECTIVE ADSORPTION; GAS-ADSORPTION; COORDINATION NETWORKS; ACETYLENE STORAGE; XYLENE ISOMERS; HYDROGEN-BONDS; SEPARATION; SIMULATION AB The adsorption mechanism of ethane, ethylene, and acetylene (C2Hn = 2, 4, 6) on two microporous metal organic frameworks (MOFs) is described here that is consistent with observations from single crystal and powder X-ray diffraction, calorimetric measurements, and gas adsorption isotherm measurements. Two calcium-based MOFs, designated as SBMOF-1 and SBMOF-2 (SB: Stony Brook), form three-dimensional frameworks with one-dimensional open channels. As determined from single crystal diffraction experiments, channel geometries of both SBMOF-1 and SBMOF-2 provide multiple adsorption sites for hydrocarbon molecules through C-H-pi and C-H center dot center dot center dot interactions, similarly to interactions in the molecular and protein crystals. Both materials selectively adsorb C-2 hydrocarbon gases over methane as determined with LAST and breakthrough calculations as well as experimental breakthrough measurements, with C2H6/CH4 selectivity as high as 74 in SBMOF-1. C1 [Plonka, Anna M.; Woerner, William R.; Parise, John B.] SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA. [Chen, Xianyin; Parise, John B.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Wang, Hao; Banerjee, Debasis; Li, Jing] Rutgers State Univ, Dept Chem & Chem Biol, Piscataway, NJ 08854 USA. [Krishna, Rajamani] Univ Amsterdam, Vant Hoff Inst Mol Sci, Sci Pk 904, NL-1098 XH Amsterdam, Netherlands. [Dong, Xinglong; Han, Yu] King Abdullah Univ Sci & Technol, Thuwal 239556900, Saudi Arabia. [Parise, John B.] Brookhaven Natl Lab, Photon Sci, Upton, NY 11973 USA. [Plonka, Anna M.] Yeshiva Univ, Brookhaven Natl Lab, New York Off, Dept Phys, 342,Bldg 555, Upton, NY 11973 USA. [Banerjee, Debasis] Pacific NW Natl Lab, Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Plonka, AM (reprint author), SUNY Stony Brook, Dept Geosci, Stony Brook, NY 11794 USA.; Li, J (reprint author), Rutgers State Univ, Dept Chem & Chem Biol, Piscataway, NJ 08854 USA.; Krishna, R (reprint author), Univ Amsterdam, Vant Hoff Inst Mol Sci, Sci Pk 904, NL-1098 XH Amsterdam, Netherlands.; Plonka, AM (reprint author), Yeshiva Univ, Brookhaven Natl Lab, New York Off, Dept Phys, 342,Bldg 555, Upton, NY 11973 USA. EM anna.plonka@yu.edu; r.krishna@contact.uva.nl; jingli@rutgers.edu RI Krishna, Rajamani/A-1098-2012 OI Krishna, Rajamani/0000-0002-4784-8530 FU National Science Foundation [DMR-1231586]; NSF [CHE-0840483]; National Science Foundation/Department of Energy [NSF/CHE-0822838]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357, DE-FG02-08ER46491]; KAUST [URF/1/1672-01-01] FX Synthetic strategies for development of SBMOF-2, SCXRD and DSC-XRD characterization work, and analysis of synchrotron data at Stony Brook by A.M.P., X.C., J.B.P., and W.R.W were supported by National Science Foundation Grant DMR-1231586. Structures of SBMOF-1:C2H2, SBMOF-1:C2H4, SBMOF-2:C2H2, and SBMOF-2:C2H4 were determined using the Stony Brook University single crystal diffractometer, obtained through the support of the NSF (Grant CHE-0840483). Structures of SBMOF-1:C2H6 and SBMOF-2:C2H6 were determined in ChemMatCars (Sector 15), Advanced Photon Source (APS), principally supported by the National Science Foundation/Department of Energy (NSF/CHE-0822838). Use of APS was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. The RU team acknowledges partial support for the gas adsorption work and LAST calculations by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, through Grant DE-FG02-08ER46491. Y.H. thanks KAUST for the Competitive Research Funds under Awards URF/1/1672-01-01. NR 63 TC 7 Z9 7 U1 25 U2 64 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 22 PY 2016 VL 28 IS 6 BP 1636 EP 1646 DI 10.1021/acs.chemmater.5b03792 PG 11 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DH5UD UT WOS:000372856600008 ER PT J AU Thompson, MJ Blakeney, KJ Cady, SD Reichert, MD Del Pilar-Albaladejo, J White, ST Vela, J AF Thompson, Michelle J. Blakeney, Kyle J. Cady, Sarah D. Reichert, Malinda D. Del Pilar-Albaladejo, Joselyn White, Seth T. Vela, Javier TI Cu2ZnSnS4 Nanorods Doped with Tetrahedral, High Spin Transition Metal Ions: Mn2+, Co2+, and Ni2+ SO CHEMISTRY OF MATERIALS LA English DT Article ID ELECTRON-PARAMAGNETIC-RESONANCE; MAGNETIC QUANTUM DOTS; FILM SOLAR-CELLS; SEMICONDUCTOR NANOCRYSTALS; TEMPERATURE FERROMAGNETISM; COLLOIDAL NANOCRYSTALS; OPTICAL-PROPERTIES; EPR-SPECTRA; INORGANIC-CHEMISTRY; KESTERITE CU2ZNSNS4 AB Because of its useful optoelectronic properties and the relative abundance of its elements, the quaternary semiconductor Cu2ZnSnS4 (CZTS) has garnered considerable interest in recent years. In this work, we dope divalent, high spin transition metal ions (M2+ = Mn2+, Co2+, Ni2+) into the tetrahedral Zn2+ sites of wurtzite CZTS nanorods. The resulting Cu2MxZn1-xSnS4 (CMTS) nanocrystals retain the hexagonal crystalline structure, elongated morphology, and broad visible light absorption profile of the undoped CZTS nanorods. Electron paramagnetic resonance (EPR), X-ray photoelectron spectroscopy (XPS), and infrared (IR) spectroscopy help corroborate the composition and local ion environment of the doped nanocrystals. EPR shows that, similarly to MnxCd1-xSe, washing Cu2MxZn1-xSnS4 nanocrystals with trioctylphosphine oxide (TOPO) is an efficient way to remove excess Mn2+ ions from the particle surface. XPS and IR of as-isolated and thiol-washed samples show that, in contrast to binary chalcogenides, Cu2MxZn1-xSnS4 nanocrystals aggregate not through dichalcogenide bonds, but through excess metal ions cross-linking the sulfur-rich surfaces of neighboring particles. Our results may help in expanding the synthetic applicability of CZTS and CMTS materials beyond photovoltaics and into the fields of spintronics and magnetic data storage. C1 [Thompson, Michelle J.; Blakeney, Kyle J.; Cady, Sarah D.; Reichert, Malinda D.; Del Pilar-Albaladejo, Joselyn; White, Seth T.; Vela, Javier] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Thompson, Michelle J.; Reichert, Malinda D.; Vela, Javier] Ames Lab, Ames, IA 50011 USA. RP Vela, J (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA.; Vela, J (reprint author), Ames Lab, Ames, IA 50011 USA. EM vela@iastate.edu RI Vela, Javier/I-4724-2014 OI Vela, Javier/0000-0001-5124-6893 FU National Science Foundation through the Division of Materials Research, Solid State and Materials Chemistry program [NSF-DMR-1309510]; ISU FX J.V. thanks the National Science Foundation for funding of this work through the Division of Materials Research, Solid State and Materials Chemistry program (NSF-DMR-1309510). M.J.T. thanks ISU for a Joseph F. Nelson Fellowship and Jim Anderegg for assistance with XPS analysis. NR 116 TC 2 Z9 2 U1 22 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 22 PY 2016 VL 28 IS 6 BP 1668 EP 1677 DI 10.1021/acs.chemmater.5b04411 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DH5UD UT WOS:000372856600011 ER PT J AU Lin, YC Wen, BH Wiaderek, KM Sallis, S Liu, H Lapidus, SH Borkiewicz, OJ Quackenbush, NF Chernova, NA Karki, K Omenya, F Chupas, PJ Piper, LFJ Whittingham, MS Chapman, KW Ong, SP AF Lin, Yuh-Chieh Wen, Bohua Wiaderek, Kamila M. Sallis, Shawn Liu, Hao Lapidus, Saul H. Borkiewicz, Olaf J. Quackenbush, Nicholas F. Chernova, Natasha A. Karki, Khim Omenya, Fredrick Chupas, Peter J. Piper, Louis F. J. Whittingham, M. Stanley Chapman, Karena W. Ong, Shyue Ping TI Thermodynamics, Kinetics and Structural Evolution of epsilon-LiVOPO4 over Multiple Lithium Intercalation SO CHEMISTRY OF MATERIALS LA English DT Article ID MINIMUM ENERGY PATHS; ELASTIC BAND METHOD; LI-ION BATTERIES; AB-INITIO; ELECTRONIC-STRUCTURE; VANADIUM PHOSPHATE; SADDLE-POINTS; CATHODE; STORAGE; DENSITY AB In this work, we demonstrate the stable cycling of more than one Li in solid-state-synthesized epsilon-LiVOPO4 over more than 20 cycles for the first time. Using a combination of density functional theory (DFT) calculations, X-ray pair distribution function (PDF) analysis and X-ray absorption near edge structure (XANES) measurements, we present a comprehensive analysis of the thermodynamics, kinetics, and structural evolution of epsilon-LixVOPO4 over the entire lithiation range. We identify two intermediate phases at x = 1.5 and 1.75 in the low-voltage regime using DFT calculations, and the computed and electrochemical voltage profiles are in excellent agreement. Operando PDF and EXAFS techniques show a reversible hysteretic change in the short (<2 angstrom) V-O bond lengths coupled with an irreversible extension of the long V-O bond (>2.4 angstrom) during low-voltage cycling. Hydrogen intercalation from electrolyte decomposition is a possible explanation for the similar to 2.4 angstrom V-O bond and its irreversible extension. Finally, we show that e epsilon-LixVOPO4 is likely a pseudo-1D ionic diffuser with low electronic conductivity using DFT calculations, which suggests that nanosizing and carbon coating is necessary to achieve good electrochemical performance in this material. C1 [Lin, Yuh-Chieh; Ong, Shyue Ping] Univ Calif San Diego, Dept NanoEngn, 9500 Gilman Dr 0448, La Jolla, CA 92093 USA. [Wen, Bohua; Chernova, Natasha A.; Karki, Khim; Omenya, Fredrick; Whittingham, M. Stanley] SUNY Binghamton, NECCES, Binghamton, NY 13902 USA. [Wiaderek, Kamila M.; Liu, Hao; Lapidus, Saul H.; Borkiewicz, Olaf J.; Chupas, Peter J.; Chapman, Karena W.] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. [Sallis, Shawn; Piper, Louis F. J.] SUNY Binghamton, Mat Sci & Engn, Binghamton, NY 13902 USA. [Quackenbush, Nicholas F.; Piper, Louis F. J.] SUNY Binghamton, Dept Phys Appl Phys & Astron, Binghamton, NY 13902 USA. [Karki, Khim] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Ong, SP (reprint author), Univ Calif San Diego, Dept NanoEngn, 9500 Gilman Dr 0448, La Jolla, CA 92093 USA.; Whittingham, MS (reprint author), SUNY Binghamton, NECCES, Binghamton, NY 13902 USA.; Chapman, KW (reprint author), Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. EM stanwhit@gmail.com; chapmank@aps.anl.gov; ongsp@eng.ucsd.edu RI Piper, Louis/C-2960-2011 OI Piper, Louis/0000-0002-3421-3210 FU NorthEast Center for Chemical Energy Storage (NECCES), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0012583]; DOE Office of Science [DE-AC02-06CH11357] FX This research is supported as part of the NorthEast Center for Chemical Energy Storage (NECCES), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0012583. We thank Drs. T. Wu and G. Sterbinsky for supporting experiments at 9-BM. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 62 TC 6 Z9 6 U1 11 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 22 PY 2016 VL 28 IS 6 BP 1794 EP 1805 DI 10.1021/acs.chemmater.5b04880 PG 12 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DH5UD UT WOS:000372856600024 ER PT J AU Kan, WH Huq, A Manthiram, A AF Kan, Wang Hay Huq, Ashfia Manthiram, Arumugam TI Exploration of a Metastable Normal Spinel Phase Diagram for the Quaternary Li-Ni-Mn-Co-O System SO CHEMISTRY OF MATERIALS LA English DT Article ID LITHIUM-ION BATTERIES; POSITIVE-ELECTRODE MATERIALS; ELECTROCHEMICAL PROPERTIES; METAL-OXIDES; CATHODE; CELLS; LINI1/3MN1/3CO1/3O2; LIMN2O4; VOLTAGE; PERSPECTIVE AB In an attempt to enlarge the normal spinel phase diagram for the quaternary Li-Ni-Mn-Co-O system, the transformation at moderate temperatures (150-210 degrees C) of layered Li-0.5(Ni1-y-zMnyCoz)O-2 (R (3) over barm), which were obtained by an ambient-temperature extraction of lithium from Li-0.5(Ni1-y-zMnyCoz)O-2, into normal spinel-like (Fd (3) over barm) Li(Ni1-y-zMnyCoz)(2)O-4 has been investigated. The phase-conversion mechanism has been studied by joint time-of-flight (TOF) neutron and X-ray diffractions, thermogravimetric analysis, and bond valence sum map. The ionic diffusion of lithium (3a, 6c) and nickel (3a, 3b) ions has been quantified as a function of temperature. The investigated spinel phases are metastable, and they are subject to change into rock-salt phases at higher temperatures. The phases have been characterized as cathodes in lithium-ion cells. The study may serve as a strategic model to access other metastable phases by low-temperature synthesis approaches. C1 [Kan, Wang Hay; Manthiram, Arumugam] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA. [Kan, Wang Hay; Manthiram, Arumugam] Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. [Huq, Ashfia] Oak Ridge Natl Lab, Neutron Scattering Sci Div, Oak Ridge, TN 37831 USA. RP Manthiram, A (reprint author), Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA.; Manthiram, A (reprint author), Univ Texas Austin, Texas Mat Inst, Austin, TX 78712 USA. EM manth@austin.utexas.edu RI Huq, Ashfia/J-8772-2013 OI Huq, Ashfia/0000-0002-8445-9649 FU Welch Foundation [F-1254]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the Welch Foundation Grant F-1254. The neutron diffraction measurement at the POWGEN beamline at the Oak Ridge National Laboratory's (ORNL) Spallation Neutron Source (SNS) was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The authors appreciate the technical help and useful discussion with Drs. Melanie Kirkham and Pamela Whitfield at the POWGEN in ORNL, Dr. Bohang Song at the University of Texas at Austin, and Dr. Maxim Avdeev at Bragg Institute in Australian Nuclear Science and Technology Organization (ANSTO). Use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 35 TC 3 Z9 3 U1 17 U2 55 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 22 PY 2016 VL 28 IS 6 BP 1832 EP 1837 DI 10.1021/acs.chemmater.5b04994 PG 6 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DH5UD UT WOS:000372856600028 ER PT J AU Mouat, AR Mane, AU Elam, JW Delferro, M Marks, TJ Stair, PC AF Mouat, Aidan R. Mane, Anil U. Elam, Jeffrey W. Delferro, Massimiliano Marks, Tobin J. Stair, Peter C. TI Volatile Hexavalent Oxo-amidinate Complexes: Molybdenum and Tungsten Precursors for Atomic Layer Deposition SO CHEMISTRY OF MATERIALS LA English DT Article ID OXIDE THIN-FILMS; SUPPORTED METAL NANOPARTICLES; SURFACE ELECTRONIC-STRUCTURE; CHEMICAL-VAPOR-DEPOSITION; LITHIUM-ION BATTERIES; OXIDATIVE DEHYDROGENATION; OPTICAL-PROPERTIES; CATALYTIC-ACTIVITY; SELECTIVE OXIDATION; OLEFIN METATHESIS AB New complexes MoO2(tBuAMD)2 (1) and WO2((t)BuAMD)(2) (2) (AMD = acetamidinato) are synthesized and fully characterized as precursors for atomic layer deposition (ALD). They contain metal-oxo functionalities not previously utilized in ALD-type growth processes and are fully characterized by H-1 and C-13 NMR, X-ray diffraction (XRD), Fourier transform infrared, thermogravimetric analysis, single-crystal XRD, and elemental analysis. Guided by quartz crystal microbalance studies, ALD growth methodologies for both complexes have been developed. Remarkably, these isostructural compounds exhibit dramatic differences in ALD properties. Using 1 and O-3, amorphous, ultrathin molybdenum oxynitride (MoON) films are grown on Si(100) wafers. Using 2 and H2O yields amorphous WO3 films on Si(100) wafers that crystallize as WO3 nanowires upon annealing. Although 1/H2O and 2/O-3 growth was attempted, effective ALD growth could only be obtained with 1/O-3 and 2/H2O, underscoring reactivity differences in these precursors. Film thicknesses, compositions, and optical and electrical parameters are characterized by variable angle spectroscopic ellipsometry, X-ray reflectivity, grazing incidence X-ray diffraction, X-ray photoelectron spectroscopy, ultraviolet photoelectron spectroscopy, and atomic force microscopy techniques. The hitherto unknown ALD chemistry of group VI metal-oxo compounds lays a foundation for their use in the ALD synthesis of heterogeneous catalysts. C1 [Mouat, Aidan R.; Delferro, Massimiliano; Marks, Tobin J.; Stair, Peter C.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Mane, Anil U.; Elam, Jeffrey W.] Argonne Natl Lab, Energy Syst Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Stair, Peter C.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Delferro, M; Marks, TJ; Stair, PC (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Stair, PC (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM m-delferro@northwestern.edu; t-marks@northwestern.edu; pstair@northwestern.edu OI Delferro, Massimiliano/0000-0002-4443-165X FU Chemical Sciences, Geosciences, and Biosciences Division, U.S. Department of Energy [DE FG02-03ER15457]; Institute for Atom-Efficient Chemical Transformations (IACT), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX Research at Northwestern was supported by the Chemical Sciences, Geosciences, and Biosciences Division, U.S. Department of Energy through a grant (DE FG02-03ER15457) to the Institute of Catalysis in Energy Processes (ICEP) at Northwestern University. Work at Argonne was supported as part of the Institute for Atom-Efficient Chemical Transformations (IACT), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. NR 128 TC 4 Z9 4 U1 16 U2 44 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 22 PY 2016 VL 28 IS 6 BP 1907 EP 1919 DI 10.1021/acs.chemmater.6b00248 PG 13 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DH5UD UT WOS:000372856600037 ER PT J AU Luo, HX Xie, WW Tao, J Pletikosic, I Valla, T Sahasrabudhe, GS Osterhoudt, G Sutton, E Burch, KS Seibel, EM Krizan, JW Zhu, YM Cava, RJ AF Luo, Huixia Xie, Weiwei Tao, Jing Pletikosic, Ivo Valla, Tonica Sahasrabudhe, Girija S. Osterhoudt, Gavin Sutton, Erin Burch, Kenneth S. Seibel, Elizabeth M. Krizan, Jason W. Zhu, Yimei Cava, Robert J. TI Differences in Chemical Doping Matter: Superconductivity in Ti1-xTaxSe2 but Not in Ti1-xNbxSe2 SO CHEMISTRY OF MATERIALS LA English DT Article ID SUPERLATTICE FORMATION; SEMIMETAL TISE2; CHARGE-ORDER; TRANSITION; 1T-TISE2; RAMAN; PHASES; DOME AB We report that 1T-TiSe2, an archetypical layered transition metal dichalcogenide, becomes superconducting when Ta is substituted for Ti but not when Nb is substituted for Ti. This is unexpected because Nb and Ta should be chemically equivalent electron donors. Superconductivity emerges near x = 0.02 for Ti1-xTaxSe2, while, for Ti1-xNbxSe2, no superconducting transitions are observed above 0.4 K. The equivalent chemical nature of the dopants is confirmed by X-ray photoelectron spectroscopy. ARPES and Raman scattering studies show similarities and differences between the two systems, but the fundamental reasons why the Nb and Ta dopants yield such different behavior are unknown. We present a comparison of the electronic phase diagrams of many electron-doped 1T-TiSe2 systems, showing that they behave quite differently, which may have broad implications in the search for new superconductors. We propose that superconducting Ti0.8Ta0.2Se2 will be suitable for devices and other studies based on exfoliated crystal flakes. C1 [Luo, Huixia; Xie, Weiwei; Sahasrabudhe, Girija S.; Seibel, Elizabeth M.; Krizan, Jason W.; Cava, Robert J.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Tao, Jing; Pletikosic, Ivo; Valla, Tonica; Zhu, Yimei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Pletikosic, Ivo] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Osterhoudt, Gavin; Sutton, Erin; Burch, Kenneth S.] Boston Coll, Dept Phys, 140 Commonwealth Ave,Chestnut Hill, Boston, MA 02467 USA. RP Luo, HX (reprint author), Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. EM huixial@princeton.edu RI Luo, huixia/A-7544-2014; Pletikosic, Ivo/A-5683-2010; Luo, Huixia/D-8467-2017; OI Luo, huixia/0000-0003-0999-6441; Pletikosic, Ivo/0000-0003-4697-8912; Luo, Huixia/0000-0003-2703-5660; Seibel, Elizabeth/0000-0002-6728-5376 FU Department of Energy, division of basic energy sciences [DE-FG02-98ER45706]; Gordon and Betty Moore Foundation, EPiQS initiative [GBMF4412]; DOE BES, by the Materials Sciences and Engineering Division [DE-AC02-98CH10886]; BNL [DE-AC02-05CH11231, DE-SC0012704]; National Science Foundation [DMR-1410846] FX The materials synthesis and physical property characterization of this superconductor were supported by the Department of Energy, division of basic energy sciences, Grant DE-FG02-98ER45706. The single crystal structure determinations were supported by the Gordon and Betty Moore Foundation, EPiQS initiative, Grant GBMF4412. The electron diffraction study at Brookhaven National Laboratory was supported by the DOE BES, by the Materials Sciences and Engineering Division under Contract DE-AC02-98CH10886, and through the use of the Center for Functional Nanomaterials. The ARPES experiments were performed under the LBNL and BNL Grants DE-AC02-05CH11231 and DE-SC0012704. The Raman spectroscopy, AFM, and mechanical exfoliation were supported by the National Science Foundation, Grant DMR-1410846. NR 46 TC 2 Z9 2 U1 15 U2 40 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD MAR 22 PY 2016 VL 28 IS 6 BP 1927 EP 1935 DI 10.1021/acs.chemmater.6b00288 PG 9 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DH5UD UT WOS:000372856600039 ER PT J AU Carrillo, JMY Sakwa-Novak, MA Holewinski, A Potter, ME Rother, G Jones, CW Sumpter, BG AF Carrillo, Jan-Michael Y. Sakwa-Novak, Miles A. Holewinski, Adam Potter, Matthew E. Rother, Gernot Jones, Christopher W. Sumpter, Bobby G. TI Unraveling the Dynamics of Aminopolymer/Silica Composites SO LANGMUIR LA English DT Article ID POSTCOMBUSTION CO2 CAPTURE; MESOPOROUS MOLECULAR-SIEVE; SORPTION PERFORMANCE; VARYING QUALITY; CARBON CAPTURE; AMINE SORBENTS; SILICA; ADSORPTION; ADSORBENT; MCM-41 AB The structure and dynamics of a model branched polymer was investigated through molecular dynamics simulations and neutron scattering experiments. The polymer confinement, monomer concentration, and solvent quality were varied in the simulations and detailed comparisons between the calculated structural and dynamical properties of the unconfined polymer and those confined within an adsorbing and nonadsorbing cylindrical pore, representing the silica based structural support of the composite, were made. The simulations show a direct relationship in the structure of the polymer and the nonmonotonic dynamics as a function of monomer concentration within an adsorbing cylindrical pore. However, the nonmonotonic behavior disappears for the case of the branched polymer within a nonadsorbing cylindrical pore. Overall, the simulation results are in good agreement with quasi-elastic neutron scattering (QENS) studies of branched poly(ethylenimine) in mesoporous silica (SBA-15) of comparable size, suggesting an approach that can be a useful guide for understanding how to tune porous polymer composites for enhancing desired dynamical and structural behavior targeting carbon dioxide adsorption. C1 [Carrillo, Jan-Michael Y.; Sumpter, Bobby G.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Carrillo, Jan-Michael Y.; Sumpter, Bobby G.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Sakwa-Novak, Miles A.; Holewinski, Adam; Potter, Matthew E.; Jones, Christopher W.] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA. [Rother, Gernot] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Holewinski, Adam] Univ Colorado, Chem & Biol Engn, Boulder, CO 80309 USA. RP Carrillo, JMY (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.; Carrillo, JMY (reprint author), Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. EM carrillojy@ornl.gov RI Sumpter, Bobby/C-9459-2013; Rother, Gernot/B-7281-2008 OI Sumpter, Bobby/0000-0001-6341-0355; Rother, Gernot/0000-0003-4921-6294 FU Center for Understanding and Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME), an Energy Frontier Research Center - U.S. Department of Energy (US DoE), Office of Science, Basic Energy Sciences (BES) [DE-SC0012577]; US DoE, BES; Office of Science of the U.S. DoE [DE-AC05-00OR22725]; National Science Foundation [DMR-1508249] FX This work is supported by the Center for Understanding and Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME), an Energy Frontier Research Center funded by U.S. Department of Energy (US DoE), Office of Science, Basic Energy Sciences (BES) under Award no. DE-SC0012577. The authors acknowledge the Center for Accelerated Materials Modeling (CAMM) funded by US DoE, BES, Materials Science and Engineering Division (MSED) for helping with the analysis of MD simulations data and the support of the National Institute of Standards and Technology (NIST), U.S. Department of Commerce (US DoC), in providing the neutron research facilities used in this work. This research used resources of the Oak Ridge Leadership Computing Facility (OLCF) at the Oak Ridge National Laboratory (ORNL), which is supported by the Office of Science of the U.S. DoE under Contract No. DE-AC05-00OR22725. QENS measurements were performed on BASIS at the Spallation Neutron Source (SNS) at ORNL and at the High Flux Backscattering Spectrometer (HFBS) at the NIST Center for Neutron Research (NCNR) at NIST (Gaithersburg, MD, USA). The authors would like to thank S. O. Diallo and M. Tyagi for their discussion and assistance in performing experiments on the BASIS and HFBS spectrometers, respectively. This work utilized facilities supported in part by the National Science Foundation under Agreement No. DMR-1508249. NR 46 TC 2 Z9 2 U1 7 U2 30 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0743-7463 J9 LANGMUIR JI Langmuir PD MAR 22 PY 2016 VL 32 IS 11 BP 2617 EP 2625 DI 10.1021/acs.langmuir.5b04299 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DH5UF UT WOS:000372856800011 PM 26915732 ER PT J AU Sanoja, GE Popere, BC Beckingham, BS Evans, CM Lynd, NA Segalman, RA AF Sanoja, Gabriel E. Popere, Bhooshan C. Beckingham, Bryan S. Evans, Christopher M. Lynd, Nathaniel A. Segalman, Rachel A. TI Structure-Conductivity Relationships of Block Copolymer Membranes Based on Hydrated Protic Polymerized Ionic Liquids: Effect of Domain Spacing SO MACROMOLECULES LA English DT Article ID GAS SEPARATION PERFORMANCE; ELECTROLYTE MEMBRANES; PHASE-BEHAVIOR; TRANSPORT; TEMPERATURE; CONFINEMENT; SCATTERING; SOLVENTS; DYNAMICS; LONOMERS AB Elucidating the relationship between chemical structure, morphology, and ionic conductivity is essential for designing novel high-performance materials for electrochemical applications. In this work, the effect of lamellar domain spacing (d) on ionic conductivity (sigma) is investigated for a model system of hydrated diblock copolymer based on a protic polymerized ionic liquid. We present a strategy that allows for the synthesis of a well-defined series of narrowly dispersed PS-b-PIL with constant volume fraction of ionic liquid moieties (f(IL) approximate to 0.39) and with two types of mobile charge carriers: trifluoroacetate anions and protons. These materials self-assemble into ordered lamellar morphologies with variable domain spacing (ca. 20-70 nm) as demonstrated by small-angle X-ray scattering. PS-b-PIL membranes exhibit ionic conductivities above 10(-4) S/cm at room temperature, which are independent of domain spacing consistent with their nearly identical water content. The conductivity scaling relationship demonstrated in this paper suggests that a mechanically robust membrane can be designed without compromising its ability to transport ions. In addition, PIL-based membranes exhibit low water uptake (lambda approximate to 10) in comparison with many proton-conducting systems reported elsewhere. The low water content of the materials described herein makes them promising candidates for electrochemical devices operating in aqueous electrolytes at low current densities where moderate ion conduction and low product crossover are required. C1 [Sanoja, Gabriel E.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Sanoja, Gabriel E.; Beckingham, Bryan S.; Lynd, Nathaniel A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Lynd, Nathaniel A.] Univ Texas Austin, McKetta Dept Chem Engn, Austin, TX 78712 USA. [Sanoja, Gabriel E.; Popere, Bhooshan C.; Evans, Christopher M.; Segalman, Rachel A.] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. [Segalman, Rachel A.] Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. RP Lynd, NA (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA.; Lynd, NA (reprint author), Univ Texas Austin, McKetta Dept Chem Engn, Austin, TX 78712 USA.; Segalman, RA (reprint author), Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA.; Segalman, RA (reprint author), Univ Calif Santa Barbara, Dept Mat, Santa Barbara, CA 93106 USA. EM lynd@che.utexas.edu; segalman@engineering.ucsb.edu FU AFOSR MURI [FA9550-12-1]; Office of Science of the U.S. Department of Energy [DE-SC0004993]; California Energy Commission (CEC) [500-11-23]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; MRSEC Program of the National Science Foundation [DMR 1121053] FX We gratefully acknowledge Dr. Eric Schaible, Polite Stewart, and Chenhui Zhu for experimental assistance at the ALS. The authors also thank Prof. Nitash P. Balsara, Prof. Karen I. Winey, Prof. Andrew Herring, Dr. Adam Z. Weber, Dr. Pepa Cotanda, Dr. Daniel J. Miller, Dr. Miguel A. Modestino, and Christina Rodriguez for helpful discussions. The physical characterization of PS-b-PIL and data analysis were supported by the AFOSR MURI program under FA9550-12-1. The synthesis and molecular characterization of PS-b-PIL were performed at the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award DE-SC0004993. Work by Bryan S. Beckingham and Nathaniel A. Lynd was supported by the California Energy Commission (CEC) under Contract 500-11-23. Beamline 7.3.3 of the Advanced Light Source is supported by the Director of the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract DE-AC02-05CH11231. The ionic conductivity and water uptake measurements of PS-b-PIL were performed at the Materials Research Laboratory, a facility supported by the MRSEC Program of the National Science Foundation, under Award DMR 1121053. NR 62 TC 4 Z9 4 U1 17 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAR 22 PY 2016 VL 49 IS 6 BP 2216 EP 2223 DI 10.1021/acs.macromol.5b02614 PG 8 WC Polymer Science SC Polymer Science GA DH5UA UT WOS:000372856300026 ER PT J AU Maskey, S Osti, NC Grest, GS Perahia, D AF Maskey, Sabina Osti, Naresh C. Grest, Gary S. Perahia, Dvora TI Dynamics of Polydots: Soft Luminescent Polymeric Nanoparticles SO MACROMOLECULES LA English DT Article ID DEPENDENT SPECTROSCOPIC PROPERTIES; MOLECULAR-DYNAMICS; CROSS-LINKING; DOTS; FUNCTIONALIZATION; SIMULATION; SCATTERING; BEHAVIOR; CELLS; FIELD AB The conformation and dynamics of luminescent polymers collapsed into nanoparticles or polydots were studied using fully atomistic molecular dynamics (MD) simulations, providing a first insight into their internal dynamics. Controlling the conformation and dynamics of confined polymers is essential for realization of the full potential of polydots in nanomedicine and biotechnology. Specifically, the shape and internal dynamics of polydots that consist of highly rigid dialkyl p-phenylene ethynylene (PPE) are probed as a function of temperature. At room temperature, the polydots are spherical without any correlations between the aromatic rings on the PPE backbone. With increasing temperature, they expand and become slightly aspherical; however, the polymers remain confined. The coherent dynamic structure factor reveals that the internal motion of the polymer backbone is arrested, and the side chains dominate the internal dynamics of the polydots. These new soft nanoparticles retain their overall shape and dynamics over an extended temperature range, and their conformation is tunable via their degree of expansion. C1 [Maskey, Sabina; Osti, Naresh C.; Perahia, Dvora] Clemson Univ, Dept Chem, Clemson, SC 29634 USA. [Grest, Gary S.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Osti, Naresh C.] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Perahia, D (reprint author), Clemson Univ, Dept Chem, Clemson, SC 29634 USA. EM dperahi@g.clemson.edu FU NSF [CHE 1308298]; Office of Science of the U.S. Department of Energy [DEAC02-05CH11231]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors gratefully acknowledge financial support from NSF Grant CHE 1308298. This work was made possible by advanced computational resources deployed and maintained by Clemson Computing and Information Technology. This research used resources obtained through the Advanced Scientific Computing Research (ASCR) Leadership Computing Challenge (ALCC) at the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract DEAC02-05CH11231. The research was carried out, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy and Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 44 TC 1 Z9 1 U1 4 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD MAR 22 PY 2016 VL 49 IS 6 BP 2399 EP 2407 DI 10.1021/acs.macromol.5b02776 PG 9 WC Polymer Science SC Polymer Science GA DH5UA UT WOS:000372856300046 ER PT J AU Rangel, T Berland, K Sharifzadeh, S Brown-Altvater, F Lee, K Hyldgaard, P Kronik, L Neaton, JB AF Rangel, Tonatiuh Berland, Kristian Sharifzadeh, Sahar Brown-Altvater, Florian Lee, Kyuho Hyldgaard, Per Kronik, Leeor Neaton, Jeffrey B. TI Structural and excited-state properties of oligoacene crystals from first principles SO PHYSICAL REVIEW B LA English DT Article ID TETRACENE SINGLE-CRYSTALS; DENSITY-FUNCTIONAL THEORY; GENERALIZED GRADIENT APPROXIMATION; CHARGE-TRANSFER TRANSITIONS; TAMM-DANCOFF APPROXIMATION; NEUTRON POWDER DIFFRACTION; QUASI-PARTICLE ENERGIES; DER-WAALS COMPLEXES; ELECTRONIC-STRUCTURE; MOLECULAR-CRYSTALS AB Molecular crystals are a prototypical class of van der Waals (vdW) bound organic materials with excited-state properties relevant for optoelectronics applications. Predicting the structure and excited-state properties of molecular crystals presents a challenge for electronic structure theory, as standard approximations to density functional theory (DFT) do not capture long-range vdW dispersion interactions and do not yield excited-state properties. In this work, we use a combination of DFT including vdW forces, using both nonlocal correlation functionals and pairwise correction methods, together with many-body perturbation theory (MBPT) to study the geometry and excited states, respectively, of the entire series of oligoacene crystals, from benzene to hexacene. We find that vdW methods can predict lattice constants within 1% of the experimental measurements, on par with the previously reported accuracy of pairwise approximations for the same systems. We further find that excitation energies are sensitive to geometry, but if optimized geometries are used MBPT can yield excited-state properties within a few tenths of an eV from experiment. We elucidate trends in MBPT-computed charged and neutral excitation energies across the acene series and discuss the role of common approximations used in MBPT. C1 [Rangel, Tonatiuh; Brown-Altvater, Florian; Lee, Kyuho; Neaton, Jeffrey B.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Rangel, Tonatiuh; Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Berland, Kristian] Univ Oslo, Ctr Mat Sci & Nanotechnol, NO-0316 Oslo, Norway. [Sharifzadeh, Sahar] Boston Univ, Dept Elect & Comp Engn, Boston, MA 02215 USA. [Sharifzadeh, Sahar] Boston Univ, Div Mat Sci & Engn, Boston, MA 02215 USA. [Brown-Altvater, Florian] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Hyldgaard, Per] Chalmers, MC2, Dept Microtechnol & Nanosci, SE-41296 Gothenburg, Sweden. [Hyldgaard, Per] Malmo Univ, Mat Sci & Appl Math, SE-20506 Malmo, Sweden. [Kronik, Leeor] Weizmann Inst Sci, Dept Mat & Interfaces, IL-76100 Rehovot, Israel. [Neaton, Jeffrey B.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. RP Rangel, T; Neaton, JB (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.; Rangel, T; Neaton, JB (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Kronik, L (reprint author), Weizmann Inst Sci, Dept Mat & Interfaces, IL-76100 Rehovot, Israel.; Neaton, JB (reprint author), Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. EM trangel@lbl.gov; leeor.kronik@weizmann.ac.il; jbneaton@berkeley.edu RI Hyldgaard, Per/A-2038-2011; Sharifzadeh, Sahar/P-4881-2016; OI Hyldgaard, Per/0000-0001-5810-8119; Sharifzadeh, Sahar/0000-0003-4215-4668; Berland, Kristian/0000-0002-4655-1233 FU SciDAC Program on Excited State Phenomena in Energy Materials - U S Department of Energy, Office of Basic Energy Sciences and of Advanced Scientific Computing Research at Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; Office of Science, Office of Basic Energy Sciences, of the U S Department of Energy [DE-AC02-05CH11231]; Office of Science of the U S Department of Energy; Swedish Research Council; Chalmers Nanoscience Area of Advance; US-Israel Binational Science Foundation; computational resources of the National Energy Research Scientific Computing center FX T. Rangel thanks M. Torrent and M. Delaveau for addressing technical issues in ABINIT, related to the calculation of a large number of bands needed for GW calculations. This research was supported by the SciDAC Program on Excited State Phenomena in Energy Materials funded by the U S Department of Energy, Office of Basic Energy Sciences and of Advanced Scientific Computing Research, under Contract No. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U S Department of Energy under Contract No. DE-AC02-05CH11231. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U S Department of Energy. Work in Sweden supported by the Swedish Research Council and the Chalmers Nanoscience Area of Advance. Work in Israel was supported by the US-Israel Binational Science Foundation and the computational resources of the National Energy Research Scientific Computing center. NR 177 TC 13 Z9 13 U1 12 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 22 PY 2016 VL 93 IS 11 AR 115206 DI 10.1103/PhysRevB.93.115206 PG 16 WC Physics, Condensed Matter SC Physics GA DH3VR UT WOS:000372715400002 ER PT J AU Meisel, Z George, S Ahn, S Bazin, D Brown, BA Browne, J Carpino, JF Chung, H Cyburt, RH Estrade, A Famiano, M Gade, A Langer, C Matos, M Mittig, W Montes, F Morrissey, DJ Pereira, J Schatz, H Schatz, J Scott, M Shapira, D Sieja, K Smith, K Stevens, J Tan, W Tarasov, O Towers, S Wimmer, K Winkelbauer, JR Yurkon, J Zegers, RGT AF Meisel, Z. George, S. Ahn, S. Bazin, D. Brown, B. A. Browne, J. Carpino, J. F. Chung, H. Cyburt, R. H. Estrade, A. Famiano, M. Gade, A. Langer, C. Matos, M. Mittig, W. Montes, F. Morrissey, D. J. Pereira, J. Schatz, H. Schatz, J. Scott, M. Shapira, D. Sieja, K. Smith, K. Stevens, J. Tan, W. Tarasov, O. Towers, S. Wimmer, K. Winkelbauer, J. R. Yurkon, J. Zegers, R. G. T. TI Time-of-flight mass measurements of neutron-rich chromium isotopes up to N=40 and implications for the accreted neutron star crust SO PHYSICAL REVIEW C LA English DT Article ID SINGLE-PARTICLE; SHELL-MODEL; RAY-BURSTS; SPECTROMETER; DEFORMATIONS; TRANSITIONS; EMISSION; NUCLIDES; DETECTOR; NUCLEI AB We present the mass excesses of Cr59-64, obtained from recent time-of-flight nuclear mass measurements at the National Superconducting Cyclotron Laboratory at Michigan State University. The mass of Cr-64 is determined for the first time, with an atomic mass excess of -33.48(44) MeV. We find a significantly different two-neutron separation energy S-2n trend for neutron-rich isotopes of chromium, removing the previously observed enhancement in binding at N = 38. Additionally, we extend the S-2n trend for chromium to N = 40, revealing behavior consistent with the previously identified island of inversion in this region. We compare our results to state-of-the-art shell-model calculations performed with a modified Lenzi-Nowacki-Poves-Sieja interaction in the fp shell, including the g(9/2) and d(5/2) orbits for the neutron valence space. We employ our result for the mass of Cr-64 in accreted neutron star crust network calculations and find a reduction in the strength and depth of electron-capture heating from the A = 64 isobaric chain, resulting in a cooler than expected accreted neutron star crust. This reduced heating is found to be due to the >1-MeV reduction in binding for Cr-64 with respect to values from commonly used global mass models. C1 [Meisel, Z.] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Meisel, Z.; George, S.; Ahn, S.; Browne, J.; Cyburt, R. H.; Estrade, A.; Montes, F.; Pereira, J.; Schatz, H.; Stevens, J.; Zegers, R. G. T.] Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. [George, S.] Max Planck Inst Kernphys, D-69117 Heidelberg, Germany. [Ahn, S.; Bazin, D.; Brown, B. A.; Browne, J.; Cyburt, R. H.; Gade, A.; Mittig, W.; Montes, F.; Morrissey, D. J.; Pereira, J.; Schatz, H.; Schatz, J.; Scott, M.; Stevens, J.; Tarasov, O.; Winkelbauer, J. R.; Yurkon, J.; Zegers, R. G. T.] Michigan State Univ, Natl Supercond Cyclotron Lab, E Lansing, MI 48824 USA. [Brown, B. A.; Browne, J.; Gade, A.; Mittig, W.; Schatz, H.; Scott, M.; Stevens, J.; Winkelbauer, J. R.; Zegers, R. G. T.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Carpino, J. F.; Chung, H.; Famiano, M.; Towers, S.] Western Michigan Univ, Dept Phys, Kalamazoo, MI 49008 USA. [Estrade, A.] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. [Langer, C.] Goethe Univ Frankfurt, Inst Appl Phys, D-60438 Frankfurt, Germany. [Matos, M.] IAEA, Phys Sect, A-1400 Vienna, Austria. [Morrissey, D. J.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Shapira, D.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Sieja, K.] Univ Strasbourg, IPHC, CNRS, UMR 7178, F-67037 Strasbourg, France. [Smith, K.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Wimmer, K.] Univ Tokyo, Dept Phys, Bunkyo Ku, Hongo 7-3-1, Tokyo 1130033, Japan. RP Meisel, Z (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA.; Meisel, Z (reprint author), Michigan State Univ, Joint Inst Nucl Astrophys, E Lansing, MI 48824 USA. EM zmeisel@nd.edu RI Gade, Alexandra/A-6850-2008; Zegers, Remco/A-6847-2008; Langer, Christoph/L-3422-2016; Tan, Wanpeng/A-4687-2008 OI Gade, Alexandra/0000-0001-8825-0976; Tan, Wanpeng/0000-0002-5930-1823 FU NSF [PHY-0822648, PHY-1102511, PHY-1404442, PHY-1430152]; DFG [GE2183/1-1, GE2183/2-1] FX We thank C. Morse, C. Prokop, and J. Vredevoogd for many useful discussions. This project was funded by the NSF through Grant Nos. PHY-0822648, PHY-1102511, PHY-1404442, and PHY-1430152. S.G. acknowledges support from the DFG under Contract Nos. GE2183/1-1 and GE2183/2-1. NR 70 TC 2 Z9 2 U1 3 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 22 PY 2016 VL 93 IS 3 AR 035805 DI 10.1103/PhysRevC.93.035805 PG 14 WC Physics, Nuclear SC Physics GA DH3XH UT WOS:000372719600006 ER PT J AU Caputo, R Buckley, MR Martin, P Charles, E Brooks, AM Drlica-Wagner, A Gaskins, J Wood, M AF Caputo, R. Buckley, M. R. Martin, P. Charles, E. Brooks, A. M. Drlica-Wagner, A. Gaskins, J. Wood, M. TI Search for gamma-ray emission from dark matter annihilation in the Small Magellanic Cloud with the Fermi Large Area Telescope SO PHYSICAL REVIEW D LA English DT Article ID GALACTIC-CENTER; STAR-FORMATION; LAT OBSERVATIONS; MILKY-WAY; GALAXIES; MASS; CONSTRAINTS; HISTORIES; PROFILES; DISTANCE AB The Small Magellanic Cloud (SMC) is the second-largest satellite galaxy of the Milky Way and is only 60 kpc away. As a nearby, massive, and dense object with relatively low astrophysical backgrounds, it is a natural target for dark matter indirect detection searches. In this work, we use six years of Pass 8 data from the Fermi Large Area Telescope to search for gamma-ray signals of dark matter annihilation in the SMC. Using data-driven fits to the gamma-ray backgrounds, and a combination of N-body simulations and direct measurements of rotation curves to estimate the SMC DM density profile, we found that the SMC was well described by standard astrophysical sources, and no signal from dark matter annihilation was detected. We set conservative upper limits on the dark matter annihilation cross section. These constraints are in agreement with stronger constraints set by searches in the Large Magellanic Cloud and approach the canonical thermal relic cross section at dark matter masses lower than 10 GeV in the b (b) over bar and tau(+)tau(-) channels. C1 [Caputo, R.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Caputo, R.] Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA. [Buckley, M. R.; Brooks, A. M.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Martin, P.] CNRS, IRAP, F-31028 Toulouse 4, France. [Charles, E.; Wood, M.] Stanford Univ, Dept Phys, Kavli Inst Particle Astrophys & Cosmol, WW Hansen Expt Phys Lab, Stanford, CA 94305 USA. [Charles, E.; Wood, M.] Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA. [Drlica-Wagner, A.] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. [Gaskins, J.] Univ Amsterdam, GRAPPA, Sci Pk 904, NL-1098 XH Amsterdam, Netherlands. RP Caputo, R (reprint author), Univ Calif Santa Cruz, Dept Phys, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA.; Caputo, R (reprint author), Univ Calif Santa Cruz, Dept Astron & Astrophys, Santa Cruz, CA 95064 USA.; Buckley, MR (reprint author), Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA.; Charles, E (reprint author), Stanford Univ, Dept Phys, Kavli Inst Particle Astrophys & Cosmol, WW Hansen Expt Phys Lab, Stanford, CA 94305 USA.; Charles, E (reprint author), Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA. EM rcaputo@ucsc.edu; mbuckley@physics.rutgers.edu; echarles@slac.stanford.edu FU Istituto Nazionale di Astrofisica in Italy; Centre National d'Etudes Spatiales in France; NASA High-End Computing (HEC) Program through the NASA Advanced Supercomputing (NAS) Division at Ames Research Center; National Aeronautics and Space Administration in the United States; Department of Energy in the United States; Commissariat a l'Energie Atomique in France; Centre National de la Recherche Scientifique / Institut National de Physique Nucleaire et de Physique des Particules in France; Agenzia Spaziale Italiana in Italy; Istituto Nazionale di Fisica Nucleare in Italy; Ministry of Education, Culture, Sports, Science and Technology (MEXT) in Japan; High Energy Accelerator Research Organization (KEK) in Japan; Japan Aerospace Exploration Agency (JAXA) in Japan; K. A. Wallenberg Foundation; Swedish Research Council in Sweden; Swedish National Space Board in Sweden FX The Fermi-LAT Collaboration acknowledges generous ongoing support from a number of agencies and institutes that have supported both the development and the operation of the LAT as well as scientific data analysis. These include the National Aeronautics and Space Administration and the Department of Energy in the United States, the Commissariat a l'Energie Atomique and the Centre National de la Recherche Scientifique / Institut National de Physique Nucleaire et de Physique des Particules in France, the Agenzia Spaziale Italiana and the Istituto Nazionale di Fisica Nucleare in Italy, the Ministry of Education, Culture, Sports, Science and Technology (MEXT), High Energy Accelerator Research Organization (KEK) and Japan Aerospace Exploration Agency (JAXA) in Japan, and the K. A. Wallenberg Foundation, the Swedish Research Council and the Swedish National Space Board in Sweden. Additional support for science analysis during the operations phase is gratefully acknowledged from the Istituto Nazionale di Astrofisica in Italy and the Centre National d'Etudes Spatiales in France. Resources supporting this work were provided by the NASA High-End Computing (HEC) Program through the NASA Advanced Supercomputing (NAS) Division at Ames Research Center. NR 86 TC 3 Z9 3 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 22 PY 2016 VL 93 IS 6 AR 062004 DI 10.1103/PhysRevD.93.062004 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH3YI UT WOS:000372722300001 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Van de Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van 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Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Search for dark matter and unparticles produced in association with a Z boson in proton-proton collisions at root s=8 TeV SO PHYSICAL REVIEW D LA English DT Article ID PARTON DISTRIBUTIONS; LHC; COMPUTATION; SIMULATION; EXISTENCE; MODEL AB A search for evidence of particle dark matter (DM) and unparticle production at the LHC has been performed using events containing two charged leptons, consistent with the decay of a Z boson, and large missing transverse momentum. This study is based on data collected with the CMS detector corresponding to an integrated luminosity of 19.7 fb(-1) of pp collisions at the LHC at a center-of-mass energy of 8 TeV. No significant excess of events is observed above the number expected from the standard model contributions. The results are interpreted in terms of 90% confidence level limits on the DM-nucleon scattering cross section, as a function of the DM particle mass, for both spin-dependent and spin-independent scenarios. Limits are set on the effective cutoff scale., and on the annihilation rate for DM particles, assuming that their branching fraction to quarks is 100%. Additionally, the most stringent 95% confidence level limits to date on the unparticle model parameters are obtained. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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S.; Junkes, A.; Klanner, R.; Kogler, R.; Kovalchuk, N.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Meyer, M.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Rathjens, D.; Sander, C.; Scharf, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schwandt, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.; Vormwald, B.] Univ Hamburg, Hamburg, Germany. [Akbiyik, M.; Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Friese, R.; Giffels, M.; Gilbert, A.; Haitz, D.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Sieber, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.; Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Horvath, D.; Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, D. K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Jain, Sa; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Chauhan, S.; Dube, S.; Kothekar, K.; Sharma, S.] Indian Inst Sci Educ & Res IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Battilana, C.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Di Mattia, A.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. 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T.; Passaseo, M.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trent, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. 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[Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Mazza, G.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. 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[Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. 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[Matveev, V.; Bylinkin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Cirkovic, P.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, P.; Cirkovic, P.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Merlin, J. A.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Szillasi, Z.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Tosi, N.; Viliani, L.; Primavera, F.; Manzoni, R. A.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Pazzini, J.; Zucchetta, A.; Ciangottini, D.; Azzurri, P.; Donato, S.; D'imperio, G.; Del Re, D.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duggan, D.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Loureno, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Polatoz, A.; Tali, B.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Ctr Nat Sci, UA-310108 Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Bravo, C.; Cousins, R.; Everaerts, P.; Farrell, C.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Gleyzer, S. V.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois Chicago UIC, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Roskes, J.; Sady, A.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MA USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Saka, H.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; De Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Tan, P.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.; Foerster, M.; Riley, G.; Rose, K.; Spanier, S.] Rutgers State Univ, Piscataway, NJ USA. [York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Celik, A.; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Huang, T.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Rose, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Ni, H.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sinthuprasith, T.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C. -E.; Chinellato, J.] Vienna Univ Technol, A-1040 Vienna, Austria. [Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Assran, Y.] Suez Univ, Suez, Egypt. [Elgammal, S.] British Univ Egypt, Cairo, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.; Mohammed, Y.] Fayoum Univ, Al Fayyum, Egypt. 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[Heredia-De La Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Di Marco, E.] Univ Rome, Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Scuola Normale, Pisa, Italy. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cerci, S.; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Ozturk, S.] Gaziosmanpasa Univ, Tokat, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.; Hernandez, A. Castaneda] Texas A&M Univ Qatar, Doha, Qatar. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; TUVE', Cristina/P-3933-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Govoni, Pietro/K-9619-2016; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; Konecki, Marcin/G-4164-2015; Manganote, Edmilson/K-8251-2013; Della Ricca, Giuseppe/B-6826-2013; Dudko, Lev/D-7127-2012; Montanari, Alessandro/J-2420-2012; Lokhtin, Igor/D-7004-2012; Novaes, Sergio/D-3532-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Azarkin, Maxim/N-2578-2015; Chinellato, Jose Augusto/I-7972-2012; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Tinoco Mendes, Andre David/D-4314-2011 OI Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; Gallinaro, Michele/0000-0003-1261-2277; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; TUVE', Cristina/0000-0003-0739-3153; Androsov, Konstantin/0000-0003-2694-6542; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Govoni, Pietro/0000-0002-0227-1301; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Della Ricca, Giuseppe/0000-0003-2831-6982; Dudko, Lev/0000-0002-4462-3192; Montanari, Alessandro/0000-0003-2748-6373; Novaes, Sergio/0000-0003-0471-8549; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Tinoco Mendes, Andre David/0000-0001-5854-7699 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agency (CNPq); Brazilian Funding Agency (CAPES); Brazilian Funding Agency (FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences of China; Ministry of Science and Technology of China; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonia; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS, France; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, Republic of Korea; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education and University of Malaya, Malaysia; Mexican Funding Agency (CINVESTAV); Mexican Funding Agency (CONACYT); Mexican Funding Agency (SEP); Mexican Funding Agency (UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Spain; Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; Swiss Funding Agency (ETH Board); Swiss Funding Agency (ETH Zurich); Swiss Funding Agency (PSI); Swiss Funding Agency (SNF); Swiss Funding Agency (UniZH); Swiss Funding Agency (Canton Zurich); Swiss Funding Agency (SER); Ministry of Science and Technology of Taipei; Thailand Center of Excellence in Physics of Thailand; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research of Thailand; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, United Kingdom; US Department of Energy; US National Science Foundation; Marie-Curie program (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union, Regional Development Fund; OPUS program of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR Project (Italy) [20108T4XTM]; Thalis program EU-ESF; Aristeia program by EU-ESF; Thalis program Greek NSRF; Aristeia program by Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Welch Foundation [C-1845]; Estonian Research Council, Estonia [IUT23-4, IUT23-6] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education and University of Malaya, Malaysia; the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna, the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research, and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, United Kingdom; the US Department of Energy and the US National Science Foundation. Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced by the European Union, Regional Development Fund; the OPUS program of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR Project No. 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, Contract No. C-1845. NR 103 TC 0 Z9 0 U1 13 U2 36 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 22 PY 2016 VL 93 IS 5 AR 052011 DI 10.1103/PhysRevD.93.052011 PG 29 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH3XP UT WOS:000372720400001 ER PT J AU Nomura, Y Sanches, F Weinberg, SJ AF Nomura, Yasunori Sanches, Fabio Weinberg, Sean J. TI Flat-space quantum gravity in the AdS/CFT correspondence SO PHYSICAL REVIEW D LA English DT Article ID GENERALIZED 2ND LAW; BLACK-HOLE; GRAVITATIONAL WAVES; STRING THEORY; ENTROPY; COMPLEMENTARITY; THERMODYNAMICS; RELATIVITY; RADIATION; MECHANICS AB Motivated by the task of understanding microscopic dynamics of an evolving black hole, we present a scheme describing gauge-fixed continuous time evolution of quantum gravitational processes in asymptotically flat spacetime using the algebra of conformal field theory operators. This allows us to study the microscopic dynamics of the Hawking emission process, although obtaining a full S-matrix may require a modification of the minimal scheme. The role of the operator product expansion is to physically interpret the resulting time evolution by decomposing the Hilbert space of the states for the entire system into those for smaller subsystems. We translate the picture of an evaporating black hole previously proposed by the authors into predictions for nonperturbative properties of the conformal field theories that have weakly coupled dual gravitational descriptions. We also discuss a possible relationship between the present scheme and a reference frame change in the bulk. C1 [Nomura, Yasunori] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Nomura, Y (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. OI Nomura, Yasunori/0000-0002-1497-1479 FU Office of Science, Office of High Energy and Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [PHY-1214644, PHY-1521446]; MEXT KAKENHI [15H05895]; DOE National Nuclear Security Administration Stewardship Science Graduate Fellowship FX We would like to thank Yu Nakayama, Yuji Tachikawa, Tadashi Takayanagi, and Taizan Watari for useful conversations on this and related topics. We also thank Kavli Institute for the Physics and Mathematics of the Universe, University of Tokyo, for hospitality during the visit in which a part of this work was carried out. This work was supported in part by the Director, Office of Science, Office of High Energy and Nuclear Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, by the National Science Foundation under Grants No. PHY-1214644 and No. PHY-1521446, and by MEXT KAKENHI Grant No. 15H05895. The work of F. S. was supported in part by the DOE National Nuclear Security Administration Stewardship Science Graduate Fellowship. NR 77 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 22 PY 2016 VL 93 IS 6 AR 064049 DI 10.1103/PhysRevD.93.064049 PG 17 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH3YI UT WOS:000372722300003 ER PT J AU Kolos, K Miller, D Grzywacz, R Iwasaki, H Al-Shudifat, M Bazin, D Bingham, CR Braunroth, T Cerizza, G Gade, A Lemasson, A Liddick, SN Madurga, M Morse, C Portillo, M Rajabali, MM Recchia, F Riedinger, LL Voss, P Walters, WB Weisshaar, D Whitmore, K Wimmer, K Tostevin, JA AF Kolos, K. Miller, D. Grzywacz, R. Iwasaki, H. Al-Shudifat, M. Bazin, D. Bingham, C. R. Braunroth, T. Cerizza, G. Gade, A. Lemasson, A. Liddick, S. N. Madurga, M. Morse, C. Portillo, M. Rajabali, M. M. Recchia, F. Riedinger, L. L. Voss, P. Walters, W. B. Weisshaar, D. Whitmore, K. Wimmer, K. Tostevin, J. A. TI Direct Lifetime Measurements of the Excited States in Ni-72 SO PHYSICAL REVIEW LETTERS LA English DT Article ID ISOTOPES; NUCLEI; TOOL AB The lifetimes of the first excited 2(+) and 4(+) states in Ni-72 were measured at the National Superconducting Cyclotron Laboratory with the recoil-distance Doppler-shift method, a model-independent probe to obtain the reduced transition probability. Excited states in Ni-72 were populated by the one-proton knockout reaction of an intermediate energy Cu-73 beam. gamma-ray-recoil coincidences were detected with the gamma-ray tracking array GRETINA and the S800 spectrograph. Our results provide evidence of enhanced transition probability B(E2; 2(+) -> 0(+)) as compared to Ni-68, but do not confirm the trend of large B(E2) values reported in the neighboring isotope Ni-70 obtained from Coulomb excitation measurement. The results are compared to shell model calculations. The lifetime obtained for the excited 4(1)(+) state is consistent with models showing decay of a seniority nu = 4, 4(+) state, which is consistent with the disappearance of the 8(+) isomer in Ni-72. C1 [Kolos, K.; Grzywacz, R.; Al-Shudifat, M.; Bingham, C. R.; Cerizza, G.; Madurga, M.; Riedinger, L. L.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Kolos, K.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Miller, D.; Rajabali, M. M.] TRIUMF, 4004 Westbrook Mall, Vancouver, BC V6T 2A3, Canada. [Grzywacz, R.; Bingham, C. R.; Riedinger, L. L.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Iwasaki, H.; Bazin, D.; Gade, A.; Lemasson, A.; Liddick, S. N.; Morse, C.; Portillo, M.; Recchia, F.; Weisshaar, D.; Whitmore, K.] Michigan State Univ, Natl Superconducting Cyclotron Lab, E Lansing, MI 48824 USA. [Iwasaki, H.; Gade, A.; Morse, C.; Whitmore, K.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Braunroth, T.] Univ Cologne, Inst Kernphys, D-50937 Cologne, Germany. [Liddick, S. N.] Michigan State Univ, Dept Chem, E Lansing, MI 48824 USA. [Voss, P.] Simon Fraser Univ, Burnaby, BC V5A 1S6, Canada. [Walters, W. B.] Univ Maryland, College Pk, MD 20742 USA. [Wimmer, K.] Cent Michigan Univ, Dept Phys, Mt Pleasant, MI 48859 USA. [Tostevin, J. A.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. RP Kolos, K (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.; Kolos, K (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. EM kolos1@llnl.gov RI Gade, Alexandra/A-6850-2008 OI Gade, Alexandra/0000-0001-8825-0976 FU Department of Energy, Office of Science Nuclear Physics [DE-FG02-96ER40983]; National Nuclear Security Administration under the Stewardship Science Academic Alliances program through DOE Cooperative Agreement [DE-FG52-08NA28552]; National Science Foundation (NSF) [PHY-1102511]; Department of Energy (DOE) National Nuclear Security Administration [DE-NA0000979]; US DOE-Office of Science; NSF [PHY-1102511]; DOE [DE-AC02-05CH11231]; National Research Council of Canada FX We wish to acknowledge the National Superconducting Cyclotron Laboratory staff for assisting with the experiments and providing excellent quality radioactive beams. The authors would like to thank Kamila Sieja (University of Strasburg/IPHC), Takaharu Otsuka (University of Tokyo) and Alex Brown (NSCL/MSU) for providing us with the results of the theoretical calculations. This work was supported by the Department of Energy, Office of Science Nuclear Physics under Contracts No. DE-FG02-96ER40983 (UTK) and by the National Nuclear Security Administration under the Stewardship Science Academic Alliances program through DOE Cooperative Agreement No. DE-FG52-08NA28552. This work also is supported by the National Science Foundation (NSF) under Grant No. PHY-1102511 and by Department of Energy (DOE) National Nuclear Security Administration under Award No. DE-NA0000979. GRETINA was funded by the US DOE-Office of Science. Operation of the array at NSCL is supported by NSF under Cooperative Agreement No. PHY-1102511(NSCL) and DOE under Grant No. DE-AC02-05CH11231(LBNL). TRIUMF (M. M. R. and D. M.) received federal funding via a contribution agreement through the National Research Council of Canada. NR 29 TC 2 Z9 2 U1 2 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 22 PY 2016 VL 116 IS 12 AR 122502 DI 10.1103/PhysRevLett.116.122502 PG 5 WC Physics, Multidisciplinary SC Physics GA DH4AJ UT WOS:000372727600004 PM 27058074 ER PT J AU Miiller, W Wu, LS Kim, MS Orvis, T Simonson, JW Gamza, M McNally, DM Nelson, CS Ehlers, G Podlesnyak, A Helton, JS Zhao, Y Qiu, Y Copley, JRD Lynn, JW Zaliznyak, I Aronson, MC AF Miiller, W. Wu, L. S. Kim, M. S. Orvis, T. Simonson, J. W. Gamza, M. McNally, D. M. Nelson, C. S. Ehlers, G. Podlesnyak, A. Helton, J. S. Zhao, Y. Qiu, Y. Copley, J. R. D. Lynn, J. W. Zaliznyak, I. Aronson, M. C. TI Magnetic structure of Yb2Pt2Pb: Ising moments on the Shastry-Sutherland lattice SO PHYSICAL REVIEW B LA English DT Article ID NEUTRON-SCATTERING; SPIN SYSTEM; SRCU2(BO3)(2); SPECTROMETER; PLATEAUS; STATES; MODEL AB Neutron diffraction measurements were carried out on single crystals and powders of Yb2Pt2Pb, where Yb moments form two interpenetrating planar sublattices of orthogonal dimers, a geometry known as Shastry-Sutherland lattice, and are stacked along the c axis in a ladder geometry. Yb2Pt2Pb orders antiferromagnetically at T-N = 2.07 K, and the magnetic structure determined from these measurements features the interleaving of two orthogonal sublattices into a 5 x 5 x 1 magnetic supercell that is based on stripes with moments perpendicular to the dimer bonds, which are along (110) and (-110). Magnetic fields applied along (110) or (-110) suppress the antiferromagnetic peaks from an individual sublattice, but leave the orthogonal sublattice unaffected, evidence for the Ising character of the Yb moments in Yb2Pt2Pb that is supported by point charge calculations. Specific heat, magnetic susceptibility, and electrical resistivity measurements concur with neutron elastic scattering results that the longitudinal critical fluctuations are gapped with Delta E similar or equal to 0.07 meV. C1 [Miiller, W.; Wu, L. S.; Kim, M. S.; Orvis, T.; Simonson, J. W.; McNally, D. M.; Aronson, M. C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Gamza, M.; Zaliznyak, I.; Aronson, M. C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Nelson, C. S.] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. [Ehlers, G.; Podlesnyak, A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Helton, J. S.; Zhao, Y.; Qiu, Y.; Copley, J. R. D.; Lynn, J. W.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Zhao, Y.; Qiu, Y.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. RP Aronson, MC (reprint author), SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA.; Aronson, MC (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM maronson@bnl.gov RI Podlesnyak, Andrey/A-5593-2013; Wu, Liusuo/A-5611-2016; Ehlers, Georg/B-5412-2008 OI Podlesnyak, Andrey/0000-0001-9366-6319; Wu, Liusuo/0000-0003-0103-5267; Ehlers, Georg/0000-0003-3513-508X FU Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, U.S. Department of Energy (DOE) [DE-SC00112704]; National Science Foundation [DMR-0944772]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; [NSF-DMR-1310008] FX We acknowledge valuable discussions with T. Sakakibara. Work at Stony Brook University (W.M., L.S.W., M.S.K., T.O., J.W.S., D.M., M.C.A.) was supported by NSF-DMR-1310008. Work at BNL (M.G., I.Z., A.M.T.) and use of the NSLS were supported by Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, U.S. Department of Energy (DOE), under Contract No. DE-SC00112704. This work utilized facilities supported in part by the National Science Foundation under Agreement No. DMR-0944772. Research conducted at SNS was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 36 TC 2 Z9 2 U1 9 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 22 PY 2016 VL 93 IS 10 AR 104419 DI 10.1103/PhysRevB.93.104419 PG 10 WC Physics, Condensed Matter SC Physics GA DH3VD UT WOS:000372714000002 ER PT J AU Moran, MA Kujawinski, EB Stubbins, A Fatland, R Aluwihare, LI Buchan, A Crump, BC Dorrestein, PC Dyhrman, ST Hess, NJ Howe, B Longnecker, K Medeiros, PM Niggemann, J Obernosterer, I Repeta, DJ Waldbauer, JR AF Moran, Mary Ann Kujawinski, Elizabeth B. Stubbins, Aron Fatland, Rob Aluwihare, Lihini I. Buchan, Alison Crump, Byron C. Dorrestein, Pieter C. Dyhrman, Sonya T. Hess, Nancy J. Howe, Bill Longnecker, Krista Medeiros, Patricia M. Niggemann, Jutta Obernosterer, Ingrid Repeta, Daniel J. Waldbauer, Jacob R. TI Deciphering ocean carbon in a changing world SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE dissolved organic matter; marine microbes; cyberinfrastructure ID DISSOLVED ORGANIC-MATTER; NORTHWESTERN SARGASSO SEA; RESONANCE MASS-SPECTROMETRY; BIOSYNTHETIC GENE CLUSTERS; PACIFIC SUBTROPICAL GYRE; MARINE-BACTERIA; SURFACE OCEAN; DEEP-OCEAN; MICROBIAL OCEANOGRAPHY; LIQUID-CHROMATOGRAPHY AB Dissolved organic matter (DOM) in the oceans is one of the largest pools of reduced carbon on Earth, comparable in size to the atmospheric CO2 reservoir. A vast number of compounds are present in DOM, and they play important roles in all major element cycles, contribute to the storage of atmospheric CO2 in the ocean, support marine ecosystems, and facilitate interactions between organisms. At the heart of the DOM cycle lie molecular-level relationships between the individual compounds in DOM and the members of the ocean microbiome that produce and consume them. In the past, these connections have eluded clear definition because of the sheer numerical complexity of both DOM molecules and microorganisms. Emerging tools in analytical chemistry, microbiology, and informatics are breaking down the barriers to a fuller appreciation of these connections. Here we highlight questions being addressed using recent methodological and technological developments in those fields and consider how these advances are transforming our understanding of some of the most important reactions of the marine carbon cycle. C1 [Moran, Mary Ann; Medeiros, Patricia M.] Univ Georgia, Dept Marine Sci, Athens, GA 30602 USA. [Kujawinski, Elizabeth B.; Longnecker, Krista; Repeta, Daniel J.] Woods Hole Oceanog Inst, Dept Marine Chem & Geochem, Woods Hole, MA 02543 USA. [Stubbins, Aron] Univ Georgia, Dept Marine Sci, Skidaway Inst Oceanog, Savannah, GA 31411 USA. [Fatland, Rob] Univ Washington, Dept Informat Technol, Seattle, WA 98105 USA. [Aluwihare, Lihini I.] Univ Calif San Diego, Scripps Inst Oceanog, Geosci Res Div, La Jolla, CA 92093 USA. [Buchan, Alison] Univ Tennessee, Dept Microbiol, Knoxville, TN 37996 USA. [Crump, Byron C.] Oregon State Univ, Coll Earth Ocean & Atmospher Sci, Corvallis, OR 97331 USA. [Dorrestein, Pieter C.] Univ Calif San Diego, Skaggs Sch Pharm & Pharmaceut Sci, Dept Pharmacol, La Jolla, CA 92037 USA. [Dorrestein, Pieter C.] Univ Calif San Diego, Dept Chem, Skaggs Sch Pharm & Pharmaceut Sci, La Jolla, CA 92037 USA. [Dorrestein, Pieter C.] Univ Calif San Diego, Skaggs Sch Pharm & Pharmaceut Sci, Dept Biochem, La Jolla, CA 92037 USA. [Dyhrman, Sonya T.] Columbia Univ, Dept Earth & Environm Sci, Palisades, NY 10964 USA. [Dyhrman, Sonya T.] Columbia Univ, Lamont Doherty Earth Observ, Palisades, NY 10964 USA. [Hess, Nancy J.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Howe, Bill] Univ Washington, Dept Comp Sci & Engn, Seattle, WA 98195 USA. [Niggemann, Jutta] Carl von Ossietzky Univ Oldenburg, Inst Chem & Biol Marine Environm, Res Grp Marine Geochem, D-26129 Oldenburg, Germany. [Obernosterer, Ingrid] Univ Paris 06, Sorbonne Univ, CNRS, Observ Oceanol,Lab Oceanog Microbienne, F-66650 Banyuls Sur Mer, France. [Waldbauer, Jacob R.] Univ Chicago, Dept Geophys Sci, 5734 S Ellis Ave, Chicago, IL 60637 USA. RP Moran, MA (reprint author), Univ Georgia, Dept Marine Sci, Athens, GA 30602 USA.; Kujawinski, EB (reprint author), Woods Hole Oceanog Inst, Dept Marine Chem & Geochem, Woods Hole, MA 02543 USA.; Stubbins, A (reprint author), Univ Georgia, Dept Marine Sci, Skidaway Inst Oceanog, Savannah, GA 31411 USA.; Fatland, R (reprint author), Univ Washington, Dept Informat Technol, Seattle, WA 98105 USA. EM mmoran@uga.edu; ekujawinski@whoi.edu; aron.stubbins@skio.uga.edu; rob5@uw.edu RI Obernosterer, Ingrid/A-5434-2011; OI Hess, Nancy/0000-0002-8930-9500; Buchan, Alison/0000-0001-7420-985X; Moran, Mary Ann/0000-0002-0702-8167 FU Gordon and Betty Moore Foundation; Microsoft Research Corporation; National Science Foundation [OCE1356010, OCE1154320, OCE1356890]; Gordon and Betty Moore Foundation [3304] FX We thank Jack Cook for graphics expertise. Formative discussions for this perspective occurred at a workshop entitled "Linking Marine Microbes and the Molecules of Dissolved Organic Matter," held in New York City in November 2014. The workshop was supported by the Gordon and Betty Moore Foundation and Microsoft Research Corporation. Additional support was provided by National Science Foundation Grants OCE1356010, OCE1154320, and OCE1356890, and by Gordon and Betty Moore Foundation Grant 3304. NR 150 TC 5 Z9 5 U1 31 U2 73 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 22 PY 2016 VL 113 IS 12 BP 3143 EP 3151 DI 10.1073/pnas.1514645113 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH0QH UT WOS:000372488200031 PM 26951682 ER PT J AU Tjong, H Li, WY Kalhor, R Dai, C Hao, SL Gong, K Zhou, YG Li, HC Zhou, XJ Le Gros, MA Larabell, CA Chen, L Alber, F AF Tjong, Harianto Li, Wenyuan Kalhor, Reza Dai, Chao Hao, Shengli Gong, Ke Zhou, Yonggang Li, Haochen Zhou, Xianghong Jasmine Le Gros, Mark A. Larabell, Carolyn A. Chen, Lin Alber, Frank TI Population-based 3D genome structure analysis reveals driving forces in spatial genome organization SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE 3D genome organization; Hi-C data analysis; genome structure modeling; centromere clustering; human genome ID CHROMOSOME CONFORMATION; TRANSCRIPTIONAL REGULATION; NUCLEAR-ORGANIZATION; DROSOPHILA GENOME; YEAST GENOME; ARCHITECTURE; PRINCIPLES; DOMAINS; CELLS; MODEL AB Conformation capture technologies (e.g., Hi-C) chart physical interactions between chromatin regions on a genome-wide scale. However, the structural variability of the genome between cells poses a great challenge to interpreting ensemble-averaged Hi-C data, particularly for long-range and interchromosomal interactions. Here, we present a probabilistic approach for deconvoluting Hi-C data into a model population of distinct diploid 3D genome structures, which facilitates the detection of chromatin interactions likely to co-occur in individual cells. Our approach incorporates the stochastic nature of chromosome conformations and allows a detailed analysis of alternative chromatin structure states. For example, we predict and experimentally confirm the presence of large centromere clusters with distinct chromosome compositions varying between individual cells. The stability of these clusters varies greatly with their chromosome identities. We show that these chromosome-specific clusters can play a key role in the overall chromosome positioning in the nucleus and stabilizing specific chromatin interactions. By explicitly considering genome structural variability, our population-based method provides an important tool for revealing novel insights into the key factors shaping the spatial genome organization. C1 [Tjong, Harianto; Li, Wenyuan; Kalhor, Reza; Dai, Chao; Hao, Shengli; Gong, Ke; Zhou, Yonggang; Li, Haochen; Zhou, Xianghong Jasmine; Chen, Lin; Alber, Frank] Univ So Calif, Dept Biol Sci, Mol & Computat Biol, Los Angeles, CA 90089 USA. [Le Gros, Mark A.; Larabell, Carolyn A.] Univ Calif San Francisco, Dept Anat, San Francisco, CA 94148 USA. [Le Gros, Mark A.; Larabell, Carolyn A.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94702 USA. [Le Gros, Mark A.; Larabell, Carolyn A.] Lawrence Berkeley Natl Lab, Adv Light Source, Natl Ctr Xray Tomog, Berkeley, CA 94702 USA. [Chen, Lin] Univ So Calif, Dept Chem, Keck Sch Med, Los Angeles, CA 90089 USA. [Chen, Lin] Univ So Calif, Keck Sch Med, Norris Comprehens Canc Ctr, Los Angeles, CA 90089 USA. RP Alber, F (reprint author), Univ So Calif, Dept Biol Sci, Mol & Computat Biol, Los Angeles, CA 90089 USA. EM alber@usc.edu FU Arnold and Mabel Beckman Foundation (BYI Program); NIH [R01GM096089, 5R01 AI113009, U54DK107981-01]; National Heart, Lung, and Blood Institute MAP-GEN Grant [U01HL108634]; NSF CAREER Grant [1150287]; Pew Charitable Trusts; National Institute of General Medical Sciences of the National Institutes of Health [P41GM103445]; US Department of Energy, Office of Biological and Environmental Research Grant [DE-AC02-05CH11231] FX We thank Dr. Quan Chen for inspiring discussions about the methods formulations and Nan Hua and Qingjiao Li for helpful discussions to improve the manuscript. The authors wish to acknowledge the anonymous reviewers for their helpful comments on the manuscript. The work was supported by the Arnold and Mabel Beckman Foundation (BYI Program) (F.A.), NIH Grants R01GM096089 (to F.A.), 5R01 AI113009 (to L.C.), and U54DK107981-01 (to F.A., L.C., and X.J.Z.), National Heart, Lung, and Blood Institute MAP-GEN Grant U01HL108634 (to X.J.Z.), and NSF CAREER Grant 1150287 (to F.A.). F.A. is a Pew Scholar in Biomedical Sciences, supported by the Pew Charitable Trusts. The National Center for X-ray Tomography is supported by the National Institute of General Medical Sciences of the National Institutes of Health Grant P41GM103445 and the US Department of Energy, Office of Biological and Environmental Research Grant DE-AC02-05CH11231. NR 57 TC 9 Z9 10 U1 12 U2 19 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 22 PY 2016 VL 113 IS 12 BP E1663 EP E1672 DI 10.1073/pnas.1512577113 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH0QH UT WOS:000372488200012 PM 26951677 ER PT J AU Gardas, B Deffner, S Saxena, A AF Gardas, Bartlomiej Deffner, Sebastian Saxena, Avadh TI Non-hermitian quantum thermodynamics SO SCIENTIFIC REPORTS LA English DT Article ID FREE-ENERGY DIFFERENCES; MECHANICS; SYSTEMS; WORK; HAMILTONIANS; SYMMETRY AB Thermodynamics is the phenomenological theory of heat and work. Here we analyze to what extent quantum thermodynamic relations are immune to the underlying mathematical formulation of quantum mechanics. As a main result, we show that the Jarzynski equality holds true for all non-hermitian quantum systems with real spectrum. This equality expresses the second law of thermodynamics for isothermal processes arbitrarily far from equilibrium. In the quasistatic limit however, the second law leads to the Carnot bound which is fulfilled even if some eigenenergies are complex provided they appear in conjugate pairs. Furthermore, we propose two setups to test our predictions, namely with strongly interacting excitons and photons in a semiconductor microcavity and in the non-hermitian tight-binding model. C1 [Gardas, Bartlomiej; Deffner, Sebastian; Saxena, Avadh] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Gardas, Bartlomiej] Univ Silesia, Inst Phys, PL-40007 Katowice, Poland. [Deffner, Sebastian; Saxena, Avadh] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP Gardas, B (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA.; Gardas, B (reprint author), Univ Silesia, Inst Phys, PL-40007 Katowice, Poland. EM bartek.gardas@gmail.com RI Deffner, Sebastian/C-5170-2008 OI Deffner, Sebastian/0000-0003-0504-6932 FU Polish Ministry of Science and Higher Education [1060/MOB/2013/0]; U.S. Department of Energy through LANL FX This work was supported by the Polish Ministry of Science and Higher Education under project Mobility Plus 1060/MOB/2013/0 (B.G.); S.D. acknowledges financial support from the U.S. Department of Energy through a LANL Director's Funded Fellowship. NR 57 TC 4 Z9 4 U1 1 U2 5 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 22 PY 2016 VL 6 AR 23408 DI 10.1038/srep23408 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH1FZ UT WOS:000372531100001 PM 27003686 ER PT J AU Berman, GP Nesterov, AI Sayre, RT Still, S AF Berman, Gennady P. Nesterov, Alexander I. Sayre, Richard T. Still, Susanne TI On improving the performance of nonphotochemical quenching in CP29 light-harvesting antenna complex SO PHYSICS LETTERS A LA English DT Article DE Electron transfer; Photosynthesis; Noise; Correlations; Nonphotochemical quenching ID CHARGE-TRANSFER STATE; SUPERRADIANCE TRANSITION; PHOTOSYNTHETIC COMPLEXES; ELECTRON-TRANSFER; GREEN PLANTS AB We model and simulate the performance of charge-transfer in nonphotochemical quenching (NPQ) in the CP29 light-harvesting antenna-complex associated with photosystem II (PSII). The model consists of five discrete excitonic energy states and two sinks, responsible for the potentially damaging processes and charge-transfer channels, respectively. We demonstrate that by varying (i) the parameters of the chlorophyll-based dimer, (ii) the resonant properties of the protein-solvent environment interaction, and (iii) the energy transfer rates to the sinks, one can significantly improve the performance of the NPQ Our analysis suggests strategies for improving the performance of. the NPQ in response to environmental changes, and may stimulate experimental verification. (C) 2016 Elsevier B.V. All rights reserved. C1 [Berman, Gennady P.] Los Alamos Natl Lab, Div Theoret, T-4, Los Alamos, NM 87544 USA. [Berman, Gennady P.; Sayre, Richard T.] New Mexico Consortium, Los Alamos, NM 87544 USA. [Nesterov, Alexander I.] Univ Guadalajara, Dept Fis, CUCEI, Av Revoluc 1500, Guadalajara 44420, Jalisco, Mexico. [Sayre, Richard T.] Los Alamos Natl Lab, Div Biol, B-11, Los Alamos, NM 87544 USA. [Still, Susanne] Univ Hawaii Manoa, Dept Informat & Comp Sci, 1860 East West Rd, Honolulu, HI 96822 USA. RP Nesterov, AI (reprint author), Univ Guadalajara, Dept Fis, CUCEI, Av Revoluc 1500, Guadalajara 44420, Jalisco, Mexico. EM nesterov@cencar.udg.mx OI Sayre, Richard/0000-0002-3153-7084 FU National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory [DE-AC52-06NA25396]; CONACYT; LDRD program at LANL; Foundational Questions Institute [FQXi-RFP3-1345] FX This work was carried out under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy at Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396. A.I.N. acknowledges the support from the CONACYT and the support during his visit of the B-Division at LANL. G.P.B. and R.T.S. acknowledge the support from the LDRD program at LANL. S.S. is grateful for support from the Foundational Questions Institute (Grant No. FQXi-RFP3-1345). NR 27 TC 1 Z9 1 U1 0 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0375-9601 EI 1873-2429 J9 PHYS LETT A JI Phys. Lett. A PD MAR 22 PY 2016 VL 380 IS 13 BP 1279 EP 1283 DI 10.1016/j.physleta.2016.01.052 PG 5 WC Physics, Multidisciplinary SC Physics GA DF7PR UT WOS:000371550600011 ER PT J AU Huntemann, M Ivanova, NN Mavromatis, K Tripp, HJ Paez-Espino, D Palaniappan, K Szeto, E Pillay, M Chen, IMA Pati, A Nielsen, T Markowitz, VM Kyrpides, NC AF Huntemann, Marcel Ivanova, Natalia N. Mavromatis, Konstantinos Tripp, H. James Paez-Espino, David Palaniappan, Krishnaveni Szeto, Ernest Pillay, Manoj Chen, I-Min A. Pati, Amrita Nielsen, Torben Markowitz, Victor M. Kyrpides, Nikos C. TI The standard operating procedure of the DOE-JGI Microbial Genome Annotation Pipeline (MGAP v.4) (vol 10, 86, 2015) SO STANDARDS IN GENOMIC SCIENCES LA English DT Correction C1 [Huntemann, Marcel; Ivanova, Natalia N.; Mavromatis, Konstantinos; Tripp, H. James; Paez-Espino, David; Pati, Amrita; Nielsen, Torben; Kyrpides, Nikos C.] Joint Genome Inst, Dept Energy, Genome Biol Program, 2800 Mitchell Dr, Walnut Creek, CA 94598 USA. [Palaniappan, Krishnaveni; Szeto, Ernest; Pillay, Manoj; Chen, I-Min A.; Markowitz, Victor M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biosci Comp, Computat Res Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Mavromatis, Konstantinos] Celgene Corp, Computat Biol Grp, Summit, NJ USA. RP Huntemann, M (reprint author), Joint Genome Inst, Dept Energy, Genome Biol Program, 2800 Mitchell Dr, Walnut Creek, CA 94598 USA. EM mhuntemann@lbl.gov RI Kyrpides, Nikos/A-6305-2014 OI Kyrpides, Nikos/0000-0002-6131-0462 NR 1 TC 0 Z9 0 U1 2 U2 2 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD MAR 21 PY 2016 VL 11 AR 27 DI 10.1186/s40793-016-0148-8 PG 1 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DO7GZ UT WOS:000377951800001 PM 27004084 ER PT J AU Braun-Munzinger, P Koch, V Schafer, T Stachel, J AF Braun-Munzinger, Peter Koch, Volker Schaefer, Thomas Stachel, Johanna TI Properties of hot and dense matter from relativistic heavy ion collisions SO PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS LA English DT Review ID NUCLEUS-NUCLEUS COLLISIONS; QUARK-GLUON PLASMA; CHEMICAL FREEZE-OUT; PB-PB COLLISIONS; STRONGLY INTERACTING MATTER; CHIRAL-SYMMETRY RESTORATION; RANGE ANGULAR-CORRELATIONS; SUPER-PROTON SYNCHROTRON; COLOR GLASS CONDENSATE; QCD PHASE-TRANSITION AB We review the progress achieved in extracting the properties of hot and dense matter from relativistic heavy ion collisions at the relativistic heavy ion collider (RHIC) at Brookhaven National Laboratory and the large hadron collider (LHC) at CERN. We focus on bulk properties of the medium, in particular the evidence for thermalization, aspects of the equation of state, transport properties, as well as fluctuations and correlations. We also discuss the in-medium properties of hadrons with light and heavy quarks, and measurements of dileptons and quarkonia. This review is dedicated to the memory of Gerald E. Brown. (C) 2016 Elsevier B.V. All rights reserved. C1 [Braun-Munzinger, Peter] GSI Helmholtzzentrum Schwerionenforsch, EMMI, D-64291 Darmstadt, Germany. [Braun-Munzinger, Peter] Tech Univ Darmstadt, Petersenstr 30, D-64287 Darmstadt, Germany. [Braun-Munzinger, Peter] FIAS, D-60438 Frankfurt, Germany. [Koch, Volker] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Stachel, Johanna] Heidelberg Univ, Inst Phys, D-69120 Heidelberg, Germany. [Schaefer, Thomas] N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. RP Schafer, T (reprint author), N Carolina State Univ, Dept Phys, Raleigh, NC 27695 USA. EM p.braun-munzinger@gsi.de; vkoch@lbl.gov; tmschaef@ncsu.edu; stachel@physi.uni-heidelberg.de RI Fachbereich14, Dekanat/C-8553-2015; OI Schaefer, Thomas/0000-0002-2297-782X FU Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Divisions of Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231, DE-FG02-03ER41260]; German BMBF ministry [05P12VHCA1]; ExtreMe Matter Institute EMMI [HA216-UHD] FX The authors thank Jiangyong Jia, Klaus Reygers, Hans Specht, Joachim Stroth, and Zhangbu Xu for helpful communications. Two of us (PBM, JS) thank K. Redlich and A. Andronic for long time collaboration on issues related to the thermal/statistical model. V.K. and T.S. are supported by the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Divisions of Nuclear Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 and DE-FG02-03ER41260, respectively. J.S. is supported in part by the German BMBF ministry (Contract No. 05P12VHCA1) and by the ExtreMe Matter Institute EMMI (Contract No. HA216-UHD). NR 399 TC 8 Z9 8 U1 6 U2 17 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-1573 EI 1873-6270 J9 PHYS REP JI Phys. Rep.-Rev. Sec. Phys. Lett. PD MAR 21 PY 2016 VL 621 BP 76 EP 126 DI 10.1016/j.physrep.2015.12.003 PG 51 WC Physics, Multidisciplinary SC Physics GA DI3RN UT WOS:000373416300003 ER PT J AU Huang, Y Zang, HD Chen, JS Sutter, EA Sutter, PW Nam, CY Cotlet, M AF Huang, Yuan Zang, Huidong Chen, Jia-Shiang Sutter, Eli A. Sutter, Peter W. Nam, Chang-Yong Cotlet, Mircea TI Hybrid quantum dot-tin disulfide field-effect transistors with improved photocurrent and spectral responsivity SO APPLIED PHYSICS LETTERS LA English DT Article ID ULTRAFAST GRAPHENE PHOTODETECTOR; MOS2 AB We report an improved photosensitivity in few-layer tin disulfide (SnS2) field-effect transistors (FETs) following doping with CdSe/ZnS core/shell quantum dots (QDs). The hybrid QD-SnS2 FET devices achieve more than 500% increase in the photocurrent response compared with the starting SnS2-only FET device and a spectral responsivity reaching over 650 A/W at 400 nm wavelength. The negligible electrical conductance in a control QD-only FET device suggests that the energy transfer between QDs and SnS2 is the main mechanism responsible for the sensitization effect, which is consistent with the strong spectral overlap between QD photoluminescence and SnS2 optical absorption as well as the large nominal donor-acceptor interspacing between QD core and SnS2. We also find enhanced charge carrier mobility in hybrid QD-SnS2 FETs which we attribute to a reduced contact Schottky barrier width due to an elevated background charge carrier density. (C) 2016 AIP Publishing LLC. C1 [Huang, Yuan; Zang, Huidong; Chen, Jia-Shiang; Nam, Chang-Yong; Cotlet, Mircea] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. [Chen, Jia-Shiang; Cotlet, Mircea] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. [Sutter, Eli A.] Univ Nebraska, Dept Mech & Mat Engn, Lincoln, NE 68588 USA. [Sutter, Peter W.] Univ Nebraska, Dept Elect & Comp Engn, Lincoln, NE 68588 USA. RP Nam, CY; Cotlet, M (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA.; Cotlet, M (reprint author), SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA.; Sutter, PW (reprint author), Univ Nebraska, Dept Elect & Comp Engn, Lincoln, NE 68588 USA. EM psutter@unl.edu; cynam@bnl.gov; cotlet@bnl.gov RI Nam, Chang-Yong/D-4193-2009 OI Nam, Chang-Yong/0000-0002-9093-4063 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704] FX This research was carried out at the Center for Functional Nanomaterials, Brookhaven National Laboratory (BNL), which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. NR 27 TC 0 Z9 0 U1 19 U2 43 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 21 PY 2016 VL 108 IS 12 AR 123502 DI 10.1063/1.4944781 PG 5 WC Physics, Applied SC Physics GA DI2SD UT WOS:000373348000042 ER PT J AU Shirazi-HD, M Turkmeneli, K Liu, S Dai, S Edmunds, C Shao, J Gardner, G Zakharov, DN Manfra, MJ Malis, O AF Shirazi-HD, M. Turkmeneli, K. Liu, S. Dai, S. Edmunds, C. Shao, J. Gardner, G. Zakharov, D. N. Manfra, M. J. Malis, O. TI Dramatic enhancement of near-infrared intersubband absorption in c-plane AlInN/GaN superlattices SO APPLIED PHYSICS LETTERS LA English DT Article AB We report substantial improvement of near-infrared (2-2.6 mu m) intersubband absorption in c-plane AlInN/GaN superlattices grown by molecular beam epitaxy. Progress was obtained through optimization of AlInN growth conditions using an AlInN growth rate of 0.9-nm/min at substrate temperature of 550 degrees C, as well as by judiciously placing the charge into two delta-doping sheets. Structural characterization suggests that AlInN crystal quality is enhanced and interface roughness is reduced. Importantly, near-infrared absorption data indicate that the optical quality of the AlInN/GaN superlattices is now comparable with that of AlN/GaN superlattices designed to exploit near-infrared intersubband transitions. (C) 2016 AIP Publishing LLC. C1 [Shirazi-HD, M.; Liu, S.; Manfra, M. J.] Purdue Univ, Sch Elect & Comp Engn, W Lafayette, IN 47907 USA. [Shirazi-HD, M.; Shao, J.; Gardner, G.; Manfra, M. J.] Birck Nanotechnol Ctr, W Lafayette, IN 47907 USA. [Turkmeneli, K.; Dai, S.; Edmunds, C.; Shao, J.; Manfra, M. J.; Malis, O.] Purdue Univ, Dept Phys & Astron, W Lafayette, IN 47907 USA. [Gardner, G.; Manfra, M. J.] Purdue Univ, Sch Mat Engn, W Lafayette, IN 47907 USA. [Zakharov, D. N.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Malis, O (reprint author), Purdue Univ, Dept Phys & Astron, W Lafayette, IN 47907 USA. EM omalis@purdue.edu FU National Science Foundation; NSF [DMR-1206919, ECCS-1253720]; Center for Functional Nanomaterials, U.S. DOE Office of Science Facility, at Brookhaven National Laboratory [DE-SC0012704] FX We acknowledge support from the National Science Foundation. M.S.-HD and C.E. were supported by the NSF Award No. DMR-1206919. S.D., S.L., J.S., and O.M. acknowledge partial support from NSF Grant No. ECCS-1253720. This research also used resources of the Center for Functional Nanomaterials, which is a U.S. DOE Office of Science Facility, at Brookhaven National Laboratory under Contract No. DE-SC0012704. NR 20 TC 1 Z9 1 U1 7 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 21 PY 2016 VL 108 IS 12 AR 121108 DI 10.1063/1.4944847 PG 5 WC Physics, Applied SC Physics GA DI2SD UT WOS:000373348000008 ER PT J AU Pan, BF Huang, JH He, MN Brombosz, SM Vaughey, JT Zhang, L Burrell, AK Zhang, ZC Liao, C AF Pan, Baofei Huang, Jinhua He, Meinan Brombosz, Scott M. Vaughey, John T. Zhang, Lu Burrell, Anthony K. Zhang, Zhengcheng Liao, Chen TI The Role of MgCl2 as a Lewis Base in ROMgCl-MgCl2 Electrolytes for Magnesium-Ion Batteries SO CHEMSUSCHEM LA English DT Article DE electrolytes; lewis acid-free; magnesium-ion batteries; mechanism; magnesium chloride ID RECHARGEABLE MG BATTERIES; SECONDARY BATTERIES; ELECTROCHEMISTRY; CATHODE; COMPLEX; SALTS AB A series of strong Lewis acid-free alkoxide/siloxide-based Mg electrolytes were deliberately developed with remarkable oxidative stability up to 3.5V (vs. Mg/Mg2+). Despite the perception of ROMgCl (R=alkyl, silyl) as a strong base, ROMgCl acts like Lewis acid, whereas the role of MgCl2 in was unambiguously demonstrated as a Lewis base through the identification of the key intermediate using single crystal X-ray crystallography. This Lewis-acid-free strategy should provide a prototype system for further investigation of Mg-ion batteries. C1 [Pan, Baofei; Huang, Jinhua; He, Meinan; Vaughey, John T.; Zhang, Lu; Burrell, Anthony K.; Zhang, Zhengcheng; Liao, Chen] Argonne Natl Lab, Joint Ctr Energy Storage Res, Chem Sci & Engn Div, Lemont, IL 60439 USA. [Brombosz, Scott M.] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. RP Liao, C (reprint author), Argonne Natl Lab, Joint Ctr Energy Storage Res, Chem Sci & Engn Div, Lemont, IL 60439 USA. EM liaoc@anl.gov OI Liao, Chen/0000-0001-5168-6493 FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; [DE-AC02-06CH11357] FX This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract no. DE-AC02-06CH11357. The electron microscopy was accomplished at the Electron Microscopy Center at Argonne National Laboratory. NR 27 TC 2 Z9 2 U1 23 U2 78 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1864-5631 EI 1864-564X J9 CHEMSUSCHEM JI ChemSusChem PD MAR 21 PY 2016 VL 9 IS 6 BP 595 EP 599 DI 10.1002/cssc.201501557 PG 5 WC Chemistry, Multidisciplinary; GREEN & SUSTAINABLE SCIENCE & TECHNOLOGY SC Chemistry; Science & Technology - Other Topics GA DI5ZT UT WOS:000373579700005 PM 26845373 ER PT J AU Horn, PR Mao, YZ Head-Gordon, M AF Horn, Paul R. Mao, Yuezhi Head-Gordon, Martin TI Defining the contributions of permanent electrostatics, Pauli repulsion, and dispersion in density functional theory calculations of intermolecular interaction energies SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID ADAPTED PERTURBATION-THEORY; TRANSITION-STATE METHOD; GENERALIZED GRADIENT APPROXIMATION; NATURAL STERIC ANALYSIS; BOND ORBITAL ANALYSIS; DER-WAALS COMPLEXES; DECOMPOSITION ANALYSIS; CHARGE-TRANSFER; NONCOVALENT INTERACTIONS; MOLECULAR-INTERACTIONS AB In energy decomposition analysis of Kohn-Sham density functional theory calculations, the so-called frozen (or pre-polarization) interaction energy contains contributions from permanent electrostatics, dispersion, and Pauli repulsion. The standard classical approach to separate them suffers from several well-known limitations. We introduce an alternative scheme that employs valid antisymmetric electronic wavefunctions throughout and is based on the identification of individual fragment contributions to the initial supersystem wavefunction as determined by an energetic optimality criterion. The density deformations identified with individual fragments upon formation of the initial supersystem wavefunction are analyzed along with the distance dependence of the new and classical terms for test cases that include the neon dimer, ammonia borane, water-Na+, water-Cl-, and the naphthalene dimer. (C) 2016 AIP Publishing LLC. C1 [Horn, Paul R.; Head-Gordon, Martin] Univ Calif Berkeley, Kenneth S Pitzer Ctr Theoret Chem, Dept Chem, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Horn, PR; Head-Gordon, M (reprint author), Univ Calif Berkeley, Kenneth S Pitzer Ctr Theoret Chem, Dept Chem, Berkeley, CA 94720 USA. EM prhorn@berkeley.edu; mhg@cchem.berkeley.edu FU U.S. National Science Foundation [CHE-1363342] FX This work was supported by Grant No. CHE-1363342 from the U.S. National Science Foundation. NR 88 TC 11 Z9 11 U1 9 U2 36 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD MAR 21 PY 2016 VL 144 IS 11 AR 114107 DI 10.1063/1.4942921 PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DI3FO UT WOS:000373384100010 PM 27004862 ER PT J AU Haider, A Ibrahim, M Bassil, BS Carey, AM Viet, AN Xing, XL Ayass, WW Minambres, JF Liu, RJ Zhang, GJ Keita, B Mereacre, V Powell, AK Balinski, K N'Diaye, AT Kupper, K Chen, HY Stimming, U Kortz, U AF Haider, Ali Ibrahim, Masooma Bassil, Bassem S. Carey, Akina M. Anh Nguyen Viet Xing, Xiaolin Ayass, Wassim W. Minambres, Juan F. Liu, Rongji Zhang, Guangjin Keita, Bineta Mereacre, Valeriu Powell, Annie K. Balinski, Kamil N'Diaye, Alpha T. Kuepper, Karsten Chen, Han-Yi Stimming, Ulrich Kortz, Ulrich TI Mixed-Valent Mn-16-Containing Heteropolyanions: Tuning of Oxidation State and Associated Physicochemical Properties SO INORGANIC CHEMISTRY LA English DT Article ID SINGLE-MOLECULE MAGNET; DAWSON SANDWICH COMPLEXES; FREE AEROBIC OXIDATION; TRANSITION-METAL; CRYSTAL-STRUCTURE; BUILDING-BLOCKS; WATER OXIDATION; ELECTROCHEMICAL GENERATION; POLYOXOMETALATE CHEMISTRY; DIMERIC POLYOXOANIONS AB The two 16-manganese-containing, Keggin-based 36-tungsto-4-silicates [(Mn10Mn6O6)-Mn-III-O-II(OH)(6)(PO4)(4)(A-alpha-SiW9O34)(4)](28-) (1) and [(Mn4Mn12II)-Mn-III(OH)(12)(PO4)(4)(A-alpha-SiW9O34)(4)](28-) (2) have been prepared by reaction of the trilacunary Keggin precursor [A-alpha-SiW9O34](10-) with either Mn(OOCCH3)(3)center dot 2H(2)O (for 1) or MnCl2 center dot 4H2O (for 2), in aqueous phosphate solution at pH 9. Polyanions 1 and 2 comprise mixed-valent, cationic {(MnMnI6O6)-Mn-III-I-II(OH)(6)}(24+) and {(Mn10Mn6O6)-Mn-III-O-II(OH)(6)(PO4)(4) cores, respectively, encapsulated by four phosphate groups and four {SiW9} units in a tetrahedral fashion. Both polyanions were structurally and compositionally Characterized by single-crystal XRD, IR, therrnogravimetric analysis, and X-ray absorption,, spectroscopy. Furthermore, studies were performed probing, the magnetic, electrochemical, oxidation catalytic, and Li-ion battery performance of 1 and 2. C1 [Haider, Ali; Ibrahim, Masooma; Bassil, Bassem S.; Carey, Akina M.; Anh Nguyen Viet; Xing, Xiaolin; Ayass, Wassim W.; Minambres, Juan F.; Kortz, Ulrich] Jacobs Univ Bremen, Dept Life Sci & Chem, POB 750 561, D-28725 Bremen, Germany. [Bassil, Bassem S.] Univ Balamand, Dept Chem, Fac Sci, POB 100, Tripoli, Lebanon. [Liu, Rongji; Zhang, Guangjin] Chinese Acad Sci, Inst Proc Engn, Key Lab Green Proc & Engn, Beijing 100190, Peoples R China. [Keita, Bineta] Univ Paris 11, UMR CNRS 8000, Lab Chim Phys, F-91405 Orsay, France. [Ibrahim, Masooma; Mereacre, Valeriu; Powell, Annie K.] KIT, Inst Nanotechnol, Hermann von Helmholtz Pl 1, D-76344 Eggenstein Leopoldshafen, Germany. [Powell, Annie K.] KIT, Inst Inorgan Chem, Engesserstr 15, D-76131 Karlsruhe, Germany. [Balinski, Kamil; Kuepper, Karsten] Univ Osnabruck, Dept Phys, D-49069 Osnabruck, Germany. [Balinski, Kamil; Kuepper, Karsten] Univ Osnabruck, Ctr Phys & Chem New Mat, D-49069 Osnabruck, Germany. [N'Diaye, Alpha T.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Chen, Han-Yi; Stimming, Ulrich] TUM CREATE, 1 CREATE Way,10-02 CREATE Tower, Singapore 138602, Singapore. [Chen, Han-Yi; Stimming, Ulrich] Tech Univ Munich, Dept Chem, Lichtenbergstr 4, D-85748 Garching, Germany. [Stimming, Ulrich] Newcastle Univ, Sch Chem, Bedson Bldg, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. RP Kortz, U (reprint author), Jacobs Univ Bremen, Dept Life Sci & Chem, POB 750 561, D-28725 Bremen, Germany. EM u.kortz@jacobs-university.de RI Kupper, Karsten/G-1397-2016; Ibrahim, Masooma/P-1913-2016; Powell, Annie/B-8665-2012 OI Ibrahim, Masooma/0000-0002-8520-8585; Powell, Annie/0000-0003-3944-7427 FU German Science Foundation (DFG) [KO 2288/20-1]; CMST COST Action [CM1203]; Jacobs University; Chinese Academy of Sciences President's International Fellowship Initiative [2015VMA041]; DAAD; DFG; Institute of Nanotechnology, Karlsruhe Institute of Technology (KIT); Higher Education Commission of Pakistan; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation of China [21371173]; TUM CREATE; National Research Foundation of Singapore; Newcastle University FX U.K. thanks the German Science Foundation (DFG, KO 2288/20-1), the CMST COST Action CM1203 (PoCheMoN), and Jacobs University for research support, and kindly acknowledges the Chinese Academy of Sciences President's International Fellowship Initiative (Grant No. 2015VMA041). A.H. thanks DAAD for a doctoral fellowship. M.I. thanks DFG and Institute of Nanotechnology, Karlsruhe Institute of Technology (KIT), for a postdoctoral fellowship, and she also thanks DAAD and the Higher Education Commission of Pakistan for a doctoral fellowship (Jacobs University). She also acknowledges the University of Balochistan, Quetta, Pakistan, for allowing her to pursue Ph.D. (Jacobs University) and postdoctoral (KIT) studies in Germany. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. G.Z. thanks the National Science Foundation of China (No. 21371173) for the funding and research support. H.-Y.C. and U.S. thank TUM CREATE, National Research Foundation of Singapore, and Newcastle University for research and funding support. Figures 1 and 2 were generated by Diamond, Version 3.2 (copyright Crystal Impact GbR). NR 115 TC 1 Z9 1 U1 14 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAR 21 PY 2016 VL 55 IS 6 BP 2755 EP 2764 DI 10.1021/acs.inorgchem.5b02503 PG 10 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DH3HJ UT WOS:000372677800013 PM 26931312 ER PT J AU Arcos-Lopez, T Qayyum, M Rivillas-Acevedo, L Miotto, MC Grande-Aztatzi, R Fernandez, CO Hedman, B Hodgson, KO Vela, A Solomon, EI Quintanar, L AF Arcos-Lopez, Trinidad Qayyum, Munzarin Rivillas-Acevedo, Lina Miotto, Marco C. Grande-Aztatzi, Rafael Fernandez, Claudio O. Hedman, Britt Hodgson, Keith O. Vela, Alberto Solomon, Edward I. Quintanar, Liliana TI Spectroscopic and Theoretical Study of Cu-I Binding to His111 in the Human Prion Protein Fragment 106-115 SO INORGANIC CHEMISTRY LA English DT Article ID METHIONINE SULFOXIDE REDUCTASE; VALENCE SUM ANALYSIS; LIGAND BOND LENGTHS; REORGANIZATION ENERGY; COPPER-BINDING; AMYLOIDOGENIC FRAGMENT; HYDROGEN-PEROXIDE; OCTAREPEAT REGION; ELECTRON-TRANSFER; PHYSIOLOGICAL PH AB The ability of the cellular prion protein (PrPC) to bind copper in vivo points to a physiological role for PrPC in copper transport. Six copper binding sites have been identified in the nonstructured N-terminal region of human PrPC. Among these sites, the His111 site is unique in that it contains a MKHM motif that would confer interesting Cu-I and Cu-II binding properties. We have evaluated Cu-I coordination to the PrP(106-115) fragment of the human PrP protein, using NMR and X-ray absorption spectroscopies and electronic structure calculations. We find that Met109 and Met112 play an important role in anchoring this metal ion. Cu-I coordination to His111 is pH-dependent: at pH >8, 2N1O1S species are formed with one Met ligand in the range of pH 5-8, both methionine (Met) residues bind to Cu-I, forming a 1N1O2S species, where N is from His111 and O is from a backbone carbonyl or a water molecule; at pH <5, only the two Met residues remain coordinated. Thus, even upon drastic changes in the Chemical environment, such as those occurring during endocytosis of PrPC (decreased pH and a reducing potential), the two Met residues in the MKHM motif enable PrPC to maintain the bound Cu-I ions, consistent with a copper transport function for this protein. We also find that the physiologically relevant Cu-I-1N1O2S species activates dioxygen via an inner-sphere mechanism, likely involving the formation of a copper(II) superoxide complex. In this process, the Met residues are partially Oxidized to sulfoxide; this ability to scavenge superoxide may play a role in the proposed antioxidant properties of PrPC. This study provides further insight into the Cu-I coordination properties of His111 in human PrPC and the molecular mechanism of oxygen activation by this site. C1 [Arcos-Lopez, Trinidad; Rivillas-Acevedo, Lina; Grande-Aztatzi, Rafael; Vela, Alberto; Quintanar, Liliana] CINVESTAV, Dept Quim, Gustavo A Madero 07360, Mexico. [Qayyum, Munzarin; Hodgson, Keith O.; Solomon, Edward I.] Stanford Univ, Dept Chem, Stanford, CA 94395 USA. [Hedman, Britt; Hodgson, Keith O.; Solomon, Edward I.] Stanford Univ, SLAC, SSRL, Menlo Pk, CA 94025 USA. [Miotto, Marco C.; Fernandez, Claudio O.] Univ Nacl Rosario Ocampo & Esmeralda, UNR MPIbpC, MPLbioR, Max Planck Lab Struct Biol Chem & Mol Biophys Ros, S2002LRK Rosario, Buenos Aires, DF, Argentina. [Miotto, Marco C.; Fernandez, Claudio O.] Univ Nacl Rosario Ocampo & Esmeralda, UNR CONICET, IIDEFAR, Inst Invest Descubrimiento Farmacos Rosario, S2002LRK Rosario, Buenos Aires, DF, Argentina. RP Quintanar, L (reprint author), CINVESTAV, Dept Quim, Gustavo A Madero 07360, Mexico.; Solomon, EI (reprint author), Stanford Univ, Dept Chem, Stanford, CA 94395 USA.; Solomon, EI (reprint author), Stanford Univ, SLAC, SSRL, Menlo Pk, CA 94025 USA. EM edward.solomon@stanford.edu; lilianaq@cinvestav.mx RI Grande-Aztatzi, Rafael/G-4660-2015 OI Grande-Aztatzi, Rafael/0000-0002-1919-4883 FU CONACYT [221134, 193318, 601210, 128369, 128411]; National Institutes of Health (NIH) [DK31450]; Fulbright-Garcia Robles fellowship; U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; U.S. DOE, Office of Biological and Environmental Research; NIH, National Institute of General Medical Sciences (NIGMS) [P41GM103393] FX This research was supported by CONACYT (Grants 221134 and 193318 to L.Q., Grants 601210 and 128369 to A.V., grant 128411 to purchase stopped-flow instrument, and a graduate fellowship to T.A.-L., and by the National Institutes of Health (NIH; Grant DK31450 to E. I.S.). T.A.-L. is thankful for a Fulbright-Garcia Robles fellowship. The authors thank Dr. Patrick Frank for technical assistance in preparing the XAS samples, Dr. Federico del Rio (UNAM) for preliminary NMR tests, M. C. Emmanuel R. C. and LaNSE-Cinvestav (Unit of Genomics, Proteomics and Metabolomics) for assistance with MALDI-TOF experiments, Selena Martinez-Gomez and Atenea Villegas-Vargas for peptide synthesis, Carolina Sanchez-Lopez and Geiser Cuellar for assistance with the acquisition of ES-MS data, and CGSTIC-Cinvestav for providing computing time for the "Xiuhcoatl Hybrid Supercomputing Cluster". XAS data were measured at the SSRL, which is supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-76SF00515. The SSRL Structural Molecular Biology Program is supported by the U.S. DOE, Office of Biological and Environmental Research, and by the NIH, National Institute of General Medical Sciences (NIGMS; Grant P41GM103393). The contents of this publication are solely the responsibility of the authors and do not necessarily represent the official views of the NIGMS or NIH. NR 93 TC 1 Z9 1 U1 3 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAR 21 PY 2016 VL 55 IS 6 BP 2909 EP 2922 DI 10.1021/acs.inorgchem.5b02794 PG 14 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DH3HJ UT WOS:000372677800028 PM 26930130 ER PT J AU McWilliams, SF Rodgers, KR Lukat-Rodgers, G Mercado, BQ Grubel, K Holland, PL AF McWilliams, Sean F. Rodgers, Kenton R. Lukat-Rodgers, Gudrun Mercado, Brandon Q. Grubel, Katarzyna Holland, Patrick L. TI Alkali Metal Variation and Twisting of the FeNNFe Core in Bridging Diiron Dinitrogen Complexes SO INORGANIC CHEMISTRY LA English DT Article ID DENSITY-FUNCTIONAL THEORY; TRIAMIDOAMINE LIGANDS; CATALYTIC-REDUCTION; IRON COMPLEXES; END-ON; AMMONIA; N-2; ACTIVATION; NITROGEN; FE(111) AB Alkali metal cations can interact with Fe-N-2 complexes, potentially enhancing back-bonding or influencing the geometry of the iron atom. These influences are relevant to large-scale N-2 reduction by iron, such as in the FeMoco of nitrogenase and the alkali-promoted Haber-Bosch process. However, to our knowledge there have been no systematic studies of a large range of alkali metals regarding their influence on transition metal-dinitrogen complexes. In this work, we varied the alkali metal in [alkali cation](2)[LFeNNFeL] complexes (L = bulky beta-diketiminate ligand) through the size range from Na+ to K+, Rb+, and Cs+. The FeNNFe cores have similar Fe-N and N-N distances and N-N stretching frequencies despite the drastic change in alkali metal cation size. The two diketiminates twist relative to one another, with larger dihedral angles accommodating the larger cations. In order to explain why the twisting has so little influence on the core, we performed density functional theory calculations on a simplified LFeNNFeL model, which show that the two metals surprisingly do not compete for back-bonding to the same pi* orbital of N-2, even when the ligand planes are parallel. This diiron system can tolerate distortion of the ligand planes through compensating orbital energy changes, and thus, a range of ligand orientations can give very similar energies. C1 [McWilliams, Sean F.; Mercado, Brandon Q.; Grubel, Katarzyna; Holland, Patrick L.] Yale Univ, Dept Chem, 225 Prospect St, New Haven, CT 06520 USA. [Rodgers, Kenton R.; Lukat-Rodgers, Gudrun] N Dakota State Univ, Dept Chem & Biochem, Fargo, ND 58105 USA. [Grubel, Katarzyna] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. RP Holland, PL (reprint author), Yale Univ, Dept Chem, 225 Prospect St, New Haven, CT 06520 USA. EM patrick.holland@yale.edu OI McWilliams, Sean/0000-0001-8715-9230 FU National Institutes of Health [GM065313, GM116463]; Germany Fulbright Commission FX This work was supported by the National Institutes of Health (GM065313 to P.L.H.; GM116463 to S.F.M.). We thank Frank Neese and Shengfa Ye (Max Planck Institute for Chemical Energy Conversion, Mulheim an der Ruhr, Germany) for assistance and resources for some of the computations, which were performed during sabbatical work by P.L.H. and funded by the Germany Fulbright Commission. NR 61 TC 2 Z9 2 U1 8 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAR 21 PY 2016 VL 55 IS 6 BP 2960 EP 2968 DI 10.1021/acs.inorgchem.5b02841 PG 9 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DH3HJ UT WOS:000372677800034 PM 26925968 ER PT J AU Heathman, CR Grimes, TS Zalupski, PR AF Heathman, Colt R. Grimes, Travis S. Zalupski, Peter R. TI Thermodynamic and Spectroscopic Studies of Trivalent f-element Complexation with Ethylenediamine-N,N '-di(acetylglycine)N,N '-diacetic Acid SO INORGANIC CHEMISTRY LA English DT Article ID INTERFACIAL MASS-TRANSFER; MRI CONTRAST AGENTS; EQUILIBRIUM-CONSTANTS; MAGNETIC-RESONANCE; HYDRATION NUMBER; DODECANE-NACL; LUMINESCENCE; STABILITY; ACTINIDE; EXTRACTION AB The coordination behavior and thermodynamic features of complexation of trivalent lanthanides and americium by ethylenediamine-N,N'-di(acetylglycine)-N,N'-diacetic acid (EDDAG-DA) (bisamide-substituted-EDTA) were investigated by potentiometric and spectroscopic techniques. Add dissociation constants (K-a) and complexation constants (beta) of lanthanides (except Pm) were determined by potentiometric analysis. Absorption spectroscopy was used to determine stability constants for the binding of trivalent americium and neodymium by EDDAG-DA under similar conditions. The potentiometry revealed 5 discernible protonation constants and 3 distinct metal ligand complexes (identified as ML-, MHL, and MH2L+). Time-resolved fluorescence studies of Eu-(EDDAG-DA) solutions (at varying pH) identified a constant inner-sphere hydration number of 3, suggesting that glycine functionalities contained in the amide pendant arms are not involved in metal complexation and are protonated under more acidic conditions. The thermodynamic studies identified that f-element coordination by EDDAG-DA is similar to that observed for ethylenediamine-N,N,N',N'-tetraacetic acid (EDTA). However, coordination via two amidic oxygens of EDDAG-DA lowers its trivalent f-element complex stability by roughly 3 orders of magnitude relative to EDTA. C1 [Heathman, Colt R.; Grimes, Travis S.; Zalupski, Peter R.] Idaho Natl Lab, Aqueous Separat & Radiochem, Idaho Falls, ID 83415 USA. RP Heathman, CR; Zalupski, PR (reprint author), Idaho Natl Lab, Aqueous Separat & Radiochem, Idaho Falls, ID 83415 USA. EM colt.heathman@inl.gov; peter.zalupski@inl.gov RI Heathman, Colt/B-4783-2017 OI Heathman, Colt/0000-0001-9436-5972 FU U.S. Department of Energy, Office of Nuclear Energy, DOE Idaho Operations Office [DE-AC07-05ID14517] FX All experimental work was conducted at the Idaho National Laboratory and supported by the U.S. Department of Energy, Office of Nuclear Energy, DOE Idaho Operations Office, under contract DE-AC07-05ID14517. NR 42 TC 3 Z9 3 U1 5 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAR 21 PY 2016 VL 55 IS 6 BP 2977 EP 2985 DI 10.1021/acs.inorgchem.5b02865 PG 9 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DH3HJ UT WOS:000372677800036 PM 26930023 ER PT J AU Calta, NP Bud'ko, SL Rodriguez, AP Han, F Chung, DY Kanatzidis, MG AF Calta, Nicholas P. Bud'ko, Sergey L. Rodriguez, Alexandra P. Han, Fei Chung, Duck Young Kanatzidis, Mercouri G. TI Synthesis, Structure, and Complex Magnetism of MIr2In8 (M = Eu, Sr) SO INORGANIC CHEMISTRY LA English DT Article ID INTERMETALLIC COMPOUNDS; SINGLE-CRYSTALS; FILLED VARIANT; GROWTH; FLUX; IR; SUPERCONDUCTIVITY; ELECTRON; BEHAVIOR; ND AB We report the synthesis, crystal structure, and physical properties of two new polar intermetallic compounds, EuIr2In8 and SrIr2In8. Both were synthesized in good-yield using In metal as a reactive flux medium, enabling the growth of large crystals for physical property measurements. They crystallize in the orthorhombic space group Pbam with the CeFe2Al8 structure type, which is sometimes also referred to as the CaCo2Al8 structure type. The two analogues have unit cell parameters of a = 13.847(3) angstrom, b = 16.118(3) angstrom, and c = 4.3885(9) angstrom for M = Eu and a = 13.847(3) angstrom, b = 16.113(3) angstrom, and c = 4.3962(9) angstrom for M = Sr at room temperature. SrIr2In8 is a diamagnetic metal with no local magnetic moments on either the Sr or Ir sites, and the diamagnetic contribution from core electrons overwhelms the expected Pauli paramagnetism normally seen in intermetallic compounds. Magnetism in EuIr2In8 is dominated by the local Eu moments, which order antiferromagnetically at 5 K in low applied fields. Increasing,the field strength depresses the magnetic ordering temperature and also induces a spin reorientation at lower temperature, indicating complex competing magnetic interactions. Low temperature heat capacity measurements show a significant enhancement of the Sommerfeld coefficient in EuIr2In8 relative to that in SrIr2In8, with estimated values of gamma = 118(3) and 18.0(2) mJ mol(-1) K-2, respectively. C1 [Calta, Nicholas P.; Rodriguez, Alexandra P.; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Bud'ko, Sergey L.] Iowa State Univ, Dept Phys & Astron, 12 Phys Hall, Ames, IA 50011 USA. [Bud'ko, Sergey L.] Ames Lab, Div Engn & Mat Sci, Ames, IA 50011 USA. [Han, Fei; Chung, Duck Young; Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Kanatzidis, MG (reprint author), Northwestern Univ, Dept Chem, 2145 Sheridan Rd, Evanston, IL 60208 USA.; Kanatzidis, MG (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM m-kanatzidis@northwestern.edu RI Han, Fei/N-2021-2013 OI Han, Fei/0000-0001-7782-2713 FU U.S. Department of Energy (DOE), Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]; Northwestern University Office of Undergraduate Research; MRSEC program (NSF) at the Materials Research Center [DMR-1121262]; International Institute for Nanotechnology (IIN); State of Illinois, through the IIN; Materials Sciences and Engineerinng Division, Basic Energy Sciences, Office of Science, U.S. DOE; Northwestern University's IIN; State of Illinois Department of Commerce and Economic Opportunity [10-203031] FX Work at the Ames Laboratory (S.L.B.) was supported by the U.S. Department of Energy (DOE), Basic Energy Sciences, Division of Materials Sciences and Engineering, under Contract DE-AC02-07CH11358. A.P.R. acknowledges support through an Undergraduate Research Grant administered by the Northwestern University Office of Undergraduate Research. This work made use of the EPIC facility (NUANCE Center, Northwestern University), which has received support from the MRSEC program (NSF Grant DMR-1121262) at the Materials Research Center, the International Institute for Nanotechnology (IIN), and the State of Illinois, through the IIN. The work at Argonne National Laboratory was supported by Materials Sciences and Engineerinng Division, Basic Energy Sciences, Office of Science, U.S. DOE. We acknowledge Prof. Danna Freedman and Samantha Clarke for assistance with magnetic measurements, which were supported by Northwestern University's IIN and the State of Illinois Department of Commerce and Economic Opportunity under Award 10-203031. NR 42 TC 0 Z9 0 U1 4 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD MAR 21 PY 2016 VL 55 IS 6 BP 3128 EP 3135 DI 10.1021/acs.inorgchem.6b00059 PG 8 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DH3HJ UT WOS:000372677800053 PM 26949815 ER PT J AU Alves, DSM El Hedri, S Wacker, JG AF Alves, Daniele S. M. El Hedri, Sonia Wacker, Jay G. TI Dark matter in 3D SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Dark matter; Beyond Standard Model; Dark Matter and Double Beta Decay ID DIRECTIONAL DETECTION; DETECTOR; COSMOLOGY; EFFICIENT AB We discuss the relevance of directional detection experiments in the post-discovery era and propose a method to extract the local dark matter phase space distribution from directional data. The first feature of this method is a parameterization of the dark matter distribution function in terms of integrals of motion, which can be analytically extended to infer properties of the global distribution if certain equilibrium conditions hold. The second feature of our method is a decomposition of the distribution function in moments of a model independent basis, with minimal reliance on the ansatz for its functional form. We illustrate our method using the Via Lactea II N-body simulation as well as an analytical model for the dark matter halo. We conclude that O(1000) events are necessary to measure deviations from the Standard Halo Model and constrain or measure the presence of anisotropies. C1 [Alves, Daniele S. M.] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Wilson St & Kirk Rd, Batavia, IL 60510 USA. [El Hedri, Sonia; Wacker, Jay G.] Stanford Univ, SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [El Hedri, Sonia; Wacker, Jay G.] Stanford Univ, Stanford Inst Theoret Phys, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94305 USA. RP Alves, DSM (reprint author), Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, Wilson St & Kirk Rd, Batavia, IL 60510 USA.; El Hedri, S; Wacker, JG (reprint author), Stanford Univ, SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.; El Hedri, S; Wacker, JG (reprint author), Stanford Univ, Stanford Inst Theoret Phys, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94305 USA. EM alves@fnal.gov; soniaeh@slac.stanford.edu; jgwacker@stanford.edu FU US DOE [DE-AC02-76-SFO0515]; Stanford Graduate Fellowship; DOE; US Department of Energy; US Department [DE-AC02-07CH11359] FX We thank Robert Feldman, Mariangela Lisanti, Louie Strigari and Tom Theuns for useful discussions. Special thanks to Michael Kuhlen for having given us access to the Via Lactea II N-body simulation full dataset and for his enlightening explanations of it. SEH and JGW are supported by the US DOE under contract number DE-AC02-76-SFO0515. SEH is supported by a Stanford Graduate Fellowship. JGW is supported by the DOE's Outstanding Junior Investigator Award. DSMA acknowledges the hospitality of the Aspen Center for Theoretical Physics where this work was partially completed. DSMA is supported by the US Department of Energy. Fermilab is operated by Fermi Research Alliance, LLC under Contract No. DE-AC02-07CH11359 with the US Department. NR 70 TC 1 Z9 1 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 21 PY 2016 IS 3 AR 149 DI 10.1007/JHEP03(2016)149 PG 28 WC Physics, Particles & Fields SC Physics GA DH9RR UT WOS:000373133900001 ER PT J AU Chiang, CW Harigaya, K Ibe, M Yanagida, TT AF Chiang, Cheng-Wei Harigaya, Keisuke Ibe, Masahiro Yanagida, Tsutomu T. TI Revisiting R-invariant direct gauge mediation SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology ID DYNAMICAL SUPERSYMMETRY BREAKING; LIGHTEST HIGGS-BOSON; GRAVITINO DARK-MATTER; RADIATIVE-CORRECTIONS; GLUINO PRODUCTION; STANDARD MODEL; MU-PROBLEM; MASSES; LEPTOGENESIS; SQUARK AB We revisit a special model of gauge mediated supersymmetry breaking, the "R-invariant direct gauge mediation." We pay particular attention to whether the model is consistent with the minimal model of the mu-term, i.e., a simple mass term of the Higgs doublets in the superpotential. Although the incompatibility is highlighted in view of the current experimental constraints on the superparticle masses and the observed Higgs boson mass, the minimal mu-term can be consistent with the R-invariant gauge mediation model via a careful choice of model parameters. We derive an upper limit on the gluino mass from the observed Higgs boson mass. We also discuss whether the model can explain the 3 sigma excess of the Z + jets + E (T) (miss) events reported by the ATLAS collaboration. C1 [Chiang, Cheng-Wei] Natl Cent Univ, Ctr Math & Theoret Phys, Taoyuan 32001, Taiwan. [Chiang, Cheng-Wei] Natl Cent Univ, Dept Phys, Taoyuan 32001, Taiwan. [Chiang, Cheng-Wei] Acad Sinica, Inst Phys, Taipei 11529, Taiwan. [Chiang, Cheng-Wei] Natl Ctr Theoret Sci, Div Phys, Hsinchu 30013, Taiwan. [Chiang, Cheng-Wei; Ibe, Masahiro; Yanagida, Tsutomu T.] Univ Tokyo, UTIAS, Kavli IPMU WPI, Kashiwa, Chiba 2778583, Japan. [Harigaya, Keisuke] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Harigaya, Keisuke] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. [Harigaya, Keisuke; Ibe, Masahiro] Univ Tokyo, ICRR, Kashiwa, Chiba 2778582, Japan. RP Chiang, CW (reprint author), Natl Cent Univ, Ctr Math & Theoret Phys, Taoyuan 32001, Taiwan.; Chiang, CW (reprint author), Natl Cent Univ, Dept Phys, Taoyuan 32001, Taiwan.; Chiang, CW (reprint author), Acad Sinica, Inst Phys, Taipei 11529, Taiwan.; Chiang, CW (reprint author), Natl Ctr Theoret Sci, Div Phys, Hsinchu 30013, Taiwan.; Chiang, CW; Ibe, M; Yanagida, TT (reprint author), Univ Tokyo, UTIAS, Kavli IPMU WPI, Kashiwa, Chiba 2778583, Japan.; Harigaya, K (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Harigaya, K (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA.; Harigaya, K; Ibe, M (reprint author), Univ Tokyo, ICRR, Kashiwa, Chiba 2778582, Japan. EM chengwei@ncu.edu.tw; keisukeharigaya@berkeley.edu; ibe@icrr.u-tokyo.ac.jp; tsutomu.tyanagida@ipmu.jp OI Chiang, Cheng-Wei/0000-0003-1716-0169 FU Ministry of Science and Technology of Taiwan [MOST-100-2628-M-008-003-MY4, 104-2628-M-008-004-MY4]; Ministry of Education, Culture, Sports, Science, and Technology (MEXT) KAKENHI, Japan [24740151, 25105011, 15H05889, 26104009]; Japan Society for the Promotion of Science (JSPS) KAKENHI [26287039]; World Premier International Research Center Initiative (WPI), MEXT, Japan; JSPS Research Fellowship for Young Scientists; MEXT [15H05889] FX The authors thank S. Shirai for useful discussions on the realization of Z+jets+ETmiss signal in SUSY models. This work is supported in part by the Ministry of Science and Technology of Taiwan under Grant Nos. MOST-100-2628-M-008-003-MY4 and 104-2628-M-008-004-MY4 (C.-W. C); Grants-in-Aid for Scientific Research from the Ministry of Education, Culture, Sports, Science, and Technology (MEXT) KAKENHI, Japan, No. 24740151, No. 25105011 and No. 15H05889 (M. I.) as well as No. 26104009 (T. T. Y.); Grant-in-Aid No. 26287039 (M. I. and T. T. Y.) from the Japan Society for the Promotion of Science (JSPS) KAKENHI; and by the World Premier International Research Center Initiative (WPI), MEXT, Japan (M. I., and T. T. Y.). K.H. was supported in part by a JSPS Research Fellowship for Young Scientists. This work is also supported by MEXT Grant-in-Aid for Scientific research on Innovative Areas (No. 15H05889). NR 111 TC 0 Z9 0 U1 0 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 21 PY 2016 IS 3 AR 145 DI 10.1007/JHEP03(2016)145 PG 25 WC Physics, Particles & Fields SC Physics GA DI2QS UT WOS:000373342100001 ER PT J AU Nachman, B AF Nachman, Benjamin TI For a light stop, less is more when gluinos mediate SO MODERN PHYSICS LETTERS A LA English DT Article DE SUSY; stop ID PP COLLISIONS; ROOT-S=8 TEV; SEARCH; SQUARK; HIGGS; BOSON; LHC AB Compressed mass spectra are generally more difficult to identify than spectra with large splittings. In particular, gluino pair production with four high energy top or bottom quarks leaves a striking signature in a detector. However, if any of the mass splittings are compressed, the power of traditional techniques may deteriorate. Searches for direct stop/sbottom pair production can be recast as searches for gluinos in order to extend the sensitivitity. As a demonstration, we show that for (g) over tilde -> t (t) over tilde (1) and m (t) over tilde (1) similar to m (chi) over tilde (0)(1), limits on the stop mass at 8 TeV can be extended by least 300 GeV for a 1.1 TeV gluino using a pp -> (t) over tilde (1)(t) over tilde (1) search. At 13 TeV, the effective cross-section for the gluino mediated process is twice the direct stop pair production cross-section, suggesting that direct stop searches could be sensitive to discover new physics earlier than expected. C1 [Nachman, Benjamin] Stanford Univ, SLAC, Stanford, CA 94305 USA. RP Nachman, B (reprint author), Stanford Univ, SLAC, Stanford, CA 94305 USA. EM bnachman@cern.ch FU National Science Foundation Graduate Research Fellowship [DGE-4747]; Stanford Graduate Fellowship FX We would like to thank Till Eifert and Michael Peskin for useful discussions and Tommaso Lari for referring us to the limits in Ref. 8. B.N. is supported by the National Science Foundation Graduate Research Fellowship under Grant No. DGE-4747 and by the Stanford Graduate Fellowship. NR 43 TC 1 Z9 1 U1 0 U2 0 PU WORLD SCIENTIFIC PUBL CO PTE LTD PI SINGAPORE PA 5 TOH TUCK LINK, SINGAPORE 596224, SINGAPORE SN 0217-7323 EI 1793-6632 J9 MOD PHYS LETT A JI Mod. Phys. Lett. A PD MAR 21 PY 2016 VL 31 IS 9 AR 1650052 DI 10.1142/S0217732316500528 PG 15 WC Physics, Nuclear; Physics, Particles & Fields; Physics, Mathematical SC Physics GA DI1VG UT WOS:000373283900002 ER PT J AU Mun, E Bud'ko, SL Canfield, PC AF Mun, Eundeok Bud'ko, Sergey L. Canfield, Paul C. TI Robust tunability of magnetoresistance in half-Heusler RPtBi (R = Gd, Dy, Tm, and Lu) compounds SO PHYSICAL REVIEW B LA English DT Article ID DEPENDENT FERMI-SURFACE; LINEAR MAGNETORESISTANCE; GIANT MAGNETORESISTANCE; TRANSPORT-PROPERTIES; QUANTUM; MAGNETOTHERMOPOWER; CEBIPT AB We present the magnetic field dependencies of transport properties for RPtBi (R = Gd, Dy, Tm, and Lu) half-Heusler compounds. Temperature- and field-dependent resistivity measurements of high-quality RPtBi single crystals reveal an unusually large, nonsaturating magnetoresistance (MR) up to 300 K under a moderate magnetic field of H = 140 kOe. At 300 K, the large MR effect decreases as the rare earth is traversed from Gd to Lu and the magnetic field dependence of MR shows a deviation from the conventional H-2 behavior. The Hall coefficient (R-H) for R = Gd indicates a sign change around 120 K, whereas R-H curves for R = Dy, Tm, and Lu remain positive for all measured temperatures. At 300 K, the Hall resistivity reveals a deviation from the linear field dependence for all compounds. Thermoelectric power measurements on this family show strong temperature and magnetic field dependencies which are consistent with resistivity measurements. A highly enhanced thermoelectric power under applied magnetic field is observed as high as similar to 100 mu V/K at 140 kOe. Analysis of the transport data in this series reveals that the rare-earth-based half-Heusler compounds provide opportunities to tune MR effect through lanthanide contraction and to elucidate the mechanism of nontrivial MR. C1 [Mun, Eundeok; Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, Ames Lab US DOE, Ames, IA 50011 USA. [Mun, Eundeok; Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Mun, Eundeok] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. RP Mun, E (reprint author), Iowa State Univ, Ames Lab US DOE, Ames, IA 50011 USA.; Mun, E (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA.; Mun, E (reprint author), Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. FU U. S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering; U. S. Department of Energy by Iowa State University [DE-AC02-07CH11358]; Natural Sciences and Engineering Research Council of Canada FX This work was supported by the U. S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering. The research was performed at the Ames Laboratory. Ames Laboratory is operated for the U. S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. The work at Simon Fraser University was supported by Natural Sciences and Engineering Research Council of Canada. NR 35 TC 0 Z9 0 U1 16 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 21 PY 2016 VL 93 IS 11 AR 115134 DI 10.1103/PhysRevB.93.115134 PG 8 WC Physics, Condensed Matter SC Physics GA DH3VN UT WOS:000372715000002 ER PT J AU Aaltonen, T Amerio, S Amidei, D Anastassov, A Annovi, A Antos, J Apollinari, G Appel, JA Arisawa, T Artikov, A Asaadi, J Ashmanskas, W Auerbach, B Aurisano, A Azfar, F Badgett, W Bae, T Barbaro-Galtieri, A Barnes, VE Barnett, BA Barria, P Bartos, P Bauce, M Bedeschi, F Behari, S Bellettini, G Bellinger, J Benjamin, D Beretvas, A Bhatti, A Bland, KR Blumenfeld, B Bocci, A Bodek, A Bortoletto, D Boudreau, J Boveia, A Brigliadori, L Bromberg, C Brucken, E Budagov, J Budd, HS Burkett, K Busetto, G Bussey, P Butti, P Buzatu, A Calamba, A Camarda, S Campanelli, M Canelli, F Carls, B Carlsmith, D Carosi, R Carrillo, S Casal, B Casarsa, M Castro, A Catastini, P Cauz, D Cavaliere, V Cerri, A Cerrito, L Chen, YC Chertok, M Chiarelli, G Chlachidze, G Cho, K Chokheli, D Clark, A Clarke, C Convery, ME Conway, J Corbo, M Cordelli, M Cox, CA Cox, DJ Cremonesi, M Cruz, D Cuevas, J Culbertson, R d'Ascenzo, N Datta, M de Barbaro, P Demortier, L Deninno, M D'Errico, M Devoto, F Di Canto, A Di Ruzza, B Dittmann, JR Donati, S D'Onofrio, M Dorigo, M Driutti, A Ebina, K Edgar, R Elagin, A Erbacher, R Errede, S Esham, B Farrington, S Ramos, JPF Field, R Flanagan, G Forrest, R Franklin, M Freeman, JC Frisch, H Funakoshi, Y Galloni, C Garfinkel, AF Garosi, P Gerberich, H Gerchtein, E Giagu, S Giakoumopoulou, V Gibson, K Ginsburg, CM Giokaris, N Giromini, P Glagolev, V Glenzinski, D Gold, M Goldin, D Golossanov, A Gomez, G Gomez-Ceballos, G Goncharov, M Lopez, OG Gorelov, I Goshaw, AT Goulianos, K Gramellini, E Grosso-Pilcher, C Group, RC da Costa, JG Hahn, SR Han, JY Happacher, F Hara, K Hare, M Harr, RF Harrington-Taber, T Hatakeyama, K Hays, C Heinrich, J Herndon, M Hocker, A Hong, Z Hopkins, W Hou, S Hughes, RE Husemann, U Hussein, M Huston, J Introzzi, G Iori, M Ivanov, A James, E Jang, D Jayatilaka, B Jeon, EJ Jindariani, S Jones, M Joo, KK Jun, SY Junk, TR Kambeitz, M Kamon, T Karchin, PE Kasmi, A Kato, Y Ketchum, W Keung, J Kilminster, B Kim, DH Kim, HS Kim, JE Kim, MJ Kim, SH Kim, SB Kim, YJ Kim, YK Kimura, N Kirby, M Knoepfel, K Kondo, K Kong, DJ Konigsberg, J Kotwal, AV Kreps, M Kroll, J Kruse, M Kuhr, T Kurata, M Laasanen, AT Lammel, S Lancaster, M Lannon, K Latino, G Lee, HS Lee, JS Leo, S Leone, S Lewis, JD Limosani, A Lipeles, E Lister, A Liu, H Liu, Q Liu, T Lockwitz, S Loginov, A Lucchesi, D Luca, A Lueck, J Lujan, P Lukens, P Lungu, G Lys, J Lysak, R Madrak, R Maestro, P Malik, S Manca, G Manousakis-Katsikakis, A Marchese, L Margaroli, F Marino, P Matera, K Mattson, ME Mazzacane, A Mazzanti, P McNulty, R Mehta, A Mehtala, P Mesropian, C Miao, T Mietlicki, D Mitra, A Miyake, H Moed, S Moggi, N Moon, CS Moore, R Morello, MJ Mukherjee, A Muller, T Murat, P Mussini, M Nachtman, J Nagai, Y Naganoma, J Nakano, I Napier, A Nett, J Neu, C Nigmanov, T Nodulman, L Noh, SY Norniella, O Oakes, L Oh, SH Oh, YD Oksuzian, I Okusawa, T Orava, R Ortolan, L Pagliarone, C Palencia, E Palni, P Papadimitriou, V Parker, W Pauletta, G Paulini, M Paus, C Phillips, TJ Piacentino, G Pianori, E Pilot, J Pitts, K Plager, C Pondrom, L Poprocki, S Potamianos, K Pranko, A Prokoshin, F Ptohos, F Punzi, G Fernandez, IR Renton, P Rescigno, M Rimondi, F Ristori, L Robson, A Rodriguez, T Rolli, S Ronzani, M Roser, R Rosner, L Ruffini, F Ruiz, A Russ, J Rusu, V Sakumoto, WK Sakurai, Y Santi, L Sato, K Saveliev, V Savoy-Navarro, A Schlabach, P Schmidt, EE Schwarz, T Scodellaro, L Scuri, F Seidel, S Seiya, Y Semenov, A Sforza, F Shalhout, SZ Shears, T Shepard, PF Shimojima, M Shochet, M Shreyber-Tecker, I Simonenko, A Sliwa, K Smith, JR Snider, FD Song, H Sorin, V Denis, RS Stancari, M Stentz, D Strologas, J Sudo, Y Sukhanov, A Suslov, I Takemasa, K Takeuchi, Y Tang, J Tecchio, M Teng, PK Thom, J Thomson, E Thukral, V Toback, D Tokar, S Tollefson, K Tomura, T Tonelli, D Torre, S Torretta, D Totaro, P Trovato, M Ukegawa, F Uozumi, S Vazquez, F Velev, G Vellidis, C Vernieri, C Vidal, M Vilar, R Vizan, J Vogel, M Volpi, G Wagner, P Wallny, R Wang, SM Waters, D Wester, WC Whiteson, D Wicklund, AB Wilbur, S Williams, HH Wilson, JS Wilson, P Winer, BL Wittich, P Wolbers, S Wolfe, H Wright, T Wu, X Wu, Z Yamamoto, K Yamato, D Yang, T Yang, UK Yang, YC Yao, WM Yeh, GP Yi, K Yoh, J Yorita, K Yoshida, T Yu, GB Yu, I Zanetti, AM Zeng, Y Zhou, C Zucchelli, S AF Aaltonen, T. Amerio, S. Amidei, D. Anastassov, A. Annovi, A. Antos, J. Apollinari, G. Appel, J. A. Arisawa, T. Artikov, A. Asaadi, J. Ashmanskas, W. Auerbach, B. Aurisano, A. Azfar, F. Badgett, W. Bae, T. Barbaro-Galtieri, A. Barnes, V. E. Barnett, B. A. Barria, P. Bartos, P. Bauce, M. Bedeschi, F. Behari, S. Bellettini, G. Bellinger, J. Benjamin, D. Beretvas, A. Bhatti, A. Bland, K. R. Blumenfeld, B. Bocci, A. Bodek, A. Bortoletto, D. Boudreau, J. Boveia, A. Brigliadori, L. Bromberg, C. Brucken, E. Budagov, J. Budd, H. S. Burkett, K. Busetto, G. Bussey, P. Butti, P. Buzatu, A. Calamba, A. Camarda, S. Campanelli, M. Canelli, F. Carls, B. Carlsmith, D. Carosi, R. Carrillo, S. Casal, B. Casarsa, M. Castro, A. Catastini, P. Cauz, D. Cavaliere, V. Cerri, A. Cerrito, L. Chen, Y. C. Chertok, M. Chiarelli, G. Chlachidze, G. Cho, K. Chokheli, D. Clark, A. Clarke, C. Convery, M. E. Conway, J. Corbo, M. Cordelli, M. Cox, C. A. Cox, D. J. Cremonesi, M. Cruz, D. Cuevas, J. Culbertson, R. d'Ascenzo, N. 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Ivanov, A. James, E. Jang, D. Jayatilaka, B. Jeon, E. J. Jindariani, S. Jones, M. Joo, K. K. Jun, S. Y. Junk, T. R. Kambeitz, M. Kamon, T. Karchin, P. E. Kasmi, A. Kato, Y. Ketchum, W. Keung, J. Kilminster, B. Kim, D. H. Kim, H. S. Kim, J. E. Kim, M. J. Kim, S. H. Kim, S. B. Kim, Y. J. Kim, Y. K. Kimura, N. Kirby, M. Knoepfel, K. Kondo, K. Kong, D. J. Konigsberg, J. Kotwal, A. V. Kreps, M. Kroll, J. Kruse, M. Kuhr, T. Kurata, M. Laasanen, A. T. Lammel, S. Lancaster, M. Lannon, K. Latino, G. Lee, H. S. Lee, J. S. Leo, S. Leone, S. Lewis, J. D. Limosani, A. Lipeles, E. Lister, A. Liu, H. Liu, Q. Liu, T. Lockwitz, S. Loginov, A. Lucchesi, D. Luca, A. Lueck, J. Lujan, P. Lukens, P. Lungu, G. Lys, J. Lysak, R. Madrak, R. Maestro, P. Malik, S. Manca, G. Manousakis-Katsikakis, A. Marchese, L. Margaroli, F. Marino, P. Matera, K. Mattson, M. E. Mazzacane, A. Mazzanti, P. McNulty, R. Mehta, A. Mehtala, P. Mesropian, C. Miao, T. Mietlicki, D. Mitra, A. Miyake, H. Moed, S. Moggi, N. Moon, C. S. 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CA CDF Collaboration TI Measurement of vector boson plus D*(2010)(+) meson production in (p)over-barp collisions at root s=1.96 TeV SO PHYSICAL REVIEW D LA English DT Article AB A measurement of vector boson (V) production in conjunction with a D*(2010)(+) meson is presented. Using a data sample corresponding to 9.7 fb(-1) of proton-antiproton collisions at center-of-mass energy root s = 1.96 TeV produced by the Fermilab Tevatron, we reconstruct V + D*+ samples with the CDF II detector. The D*+ is fully reconstructed in the D*(2010)(+) -> D-0 (-> K-pi(+))pi(+) decay mode. This technique is sensitive to the associated production of vector boson plus charm or bottom mesons. We measure the ratio of production cross sections sigma(W + D*) = sigma(W) = [1.75 +/- 0.13(stat) +/- 0.09(stat)]% and sigma(Z + D*)/sigma(Z) = [1.5 +/- 0.4(stat) +/- 0.2(stat)]% and perform a differential measurement of d sigma(W + D*)/dp(T)(D*). 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[Barria, P.; Garosi, P.; Latino, G.; Maestro, P.; Ruffini, F.] Univ Siena, I-56127 Pisa, Italy. [Marino, P.; Morello, M. J.; Trovato, M.; Vernieri, C.] Scuola Normale Super Pisa, I-56127 Pisa, Italy. [Introzzi, G.] INFN Pavia, I-27100 Pavia, Italy. [Introzzi, G.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Boudreau, J.; Gibson, K.; Nigmanov, T.; Shepard, P. F.; Song, H.] Univ Pittsburgh, Pittsburgh, PA 15260 USA. [Barnes, V. E.; Bortoletto, D.; Garfinkel, A. F.; Jones, M.; Laasanen, A. T.; Liu, Q.; Vidal, M.] Purdue Univ, W Lafayette, IN 47907 USA. [Bodek, A.; Budd, H. S.; de Barbaro, P.; Han, J. Y.; Sakumoto, W. K.] Univ Rochester, Rochester, NY 14627 USA. [Bhatti, A.; Demortier, L.; Goulianos, K.; Lungu, G.; Malik, S.; Mesropian, C.] Rockefeller Univ, New York, NY 10065 USA. [Giagu, S.; Iori, M.; Margaroli, F.; Rescigno, M.] Ist Nazl Fis Nucl, Sez Roma 1, I-00185 Rome, Italy. [Iori, M.] Univ Roma La Sapienza, I-00185 Rome, Italy. [Asaadi, J.; Aurisano, A.; Cruz, D.; Elagin, A.; Goldin, D.; Hong, Z.; Kamon, T.; Nett, J.; Thukral, V.; Toback, D.] Texas A&M Univ, Mitchell Inst Fundamental Phys & Astron, College Stn, TX 77843 USA. [Cauz, D.; Dorigo, M.; Driutti, A.; Pagliarone, C.; Pauletta, G.; Santi, L.; Zanetti, A. M.] Ist Nazl Fis Nucl Trieste, I-33100 Udine, Italy. [Cauz, D.; Driutti, A.; Pauletta, G.; Santi, L.] Grp Coll Udine, I-33100 Udine, Italy. [Cauz, D.; Driutti, A.; Pauletta, G.; Santi, L.] Univ Udine, I-33100 Udine, Italy. [Dorigo, M.] Univ Trieste, I-34127 Trieste, Italy. [Hara, K.; Kim, S. H.; Kurata, M.; Miyake, H.; Nagai, Y.; Sato, K.; Shimojima, M.; Sudo, Y.; Takemasa, K.; Takeuchi, Y.; Tomura, T.; Ukegawa, F.] Univ Tsukuba, Tsukuba, Ibaraki 305, Japan. [Hare, M.; Napier, A.; Rolli, S.; Sliwa, K.] Tufts Univ, Medford, MA 02155 USA. [Group, R. C.; Liu, H.; Neu, C.; Oksuzian, I.] Univ Virginia, Charlottesville, VA 22906 USA. [Arisawa, T.; Ebina, K.; Funakoshi, Y.; Kimura, N.; Kondo, K.; Naganoma, J.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo 169, Japan. [Clarke, C.; Harr, R. F.; Karchin, P. E.; Mattson, M. E.] Wayne State Univ, Detroit, MI 48201 USA. [Bellinger, J.; Carlsmith, D.; Herndon, M.; Parker, W.; Pondrom, L.] Univ Wisconsin, Madison, WI 53706 USA. [Husemann, U.; Lockwitz, S.; Loginov, A.] Yale Univ, New Haven, CT 06520 USA. RP Aaltonen, T (reprint author), Univ Helsinki, Dept Phys, Div High Energy Phys, FIN-00014 Helsinki, Finland.; Aaltonen, T (reprint author), Helsinki Inst Phys, FIN-00014 Helsinki, Finland. RI Gorelov, Igor/J-9010-2015; Prokoshin, Fedor/E-2795-2012; Canelli, Florencia/O-9693-2016; Ruiz, Alberto/E-4473-2011; Paulini, Manfred/N-7794-2014 OI Gorelov, Igor/0000-0001-5570-0133; Prokoshin, Fedor/0000-0001-6389-5399; Canelli, Florencia/0000-0001-6361-2117; Ruiz, Alberto/0000-0002-3639-0368; Paulini, Manfred/0000-0002-6714-5787 FU U.S. Department of Energy and National Science Foundation; Italian Istituto Nazionale di Fisica Nucleare; Ministry of Education, Culture, Sports, Science and Technology of Japan; Natural Sciences and Engineering Research Council of Canada; National Science Council of the Republic of China; Swiss National Science Foundation; A. P. Sloan Foundation; Bundesministerium fur Bildung und Forschung, Germany; Korean World Class University Program, the National Research Foundation of Korea; Science and Technology Facilities Council, United Kingdom; Royal Society, United Kingdom; Russian Foundation for Basic Research; Ministerio de Ciencia e Innovacion, Spain; Slovak RD Agency; Academy of Finland; Australian Research Council (ARC); EU community Marie Curie Fellowship [302103]; Programa Consolider-Ingenio, Spain FX We thank the Fermilab staff and the technical staffs of the participating institutions for their vital contributions. This work was supported by the U.S. Department of Energy and National Science Foundation; the Italian Istituto Nazionale di Fisica Nucleare; the Ministry of Education, Culture, Sports, Science and Technology of Japan; the Natural Sciences and Engineering Research Council of Canada; the National Science Council of the Republic of China; the Swiss National Science Foundation; the A. P. Sloan Foundation; the Bundesministerium fur Bildung und Forschung, Germany; the Korean World Class University Program, the National Research Foundation of Korea; the Science and Technology Facilities Council and the Royal Society, United Kingdom; the Russian Foundation for Basic Research; the Ministerio de Ciencia e Innovacion, and Programa Consolider-Ingenio 2010, Spain; the Slovak R&D Agency; the Academy of Finland; the Australian Research Council (ARC); and the EU community Marie Curie Fellowship Contract No. 302103. NR 18 TC 1 Z9 1 U1 5 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 21 PY 2016 VL 93 IS 5 AR 052012 DI 10.1103/PhysRevD.93.052012 PG 9 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH3XN UT WOS:000372720200001 ER PT J AU Bukov, M Kolodrubetz, M Polkovnikov, A AF Bukov, Marin Kolodrubetz, Michael Polkovnikov, Anatoli TI Schrieffer-Wolff Transformation for Periodically Driven Systems: Strongly Correlated Systems with Artificial Gauge Fields SO PHYSICAL REVIEW LETTERS LA English DT Article ID TRIANGULAR LATTICE; OPTICAL LATTICES; MAGNETIC-FIELDS; ULTRACOLD ATOMS; HUBBARD-MODEL; LOCALIZATION; CHAIN AB We generalize the Schrieffer-Wolff transformation to periodically driven systems using Floquet theory. The method is applied to the periodically driven, strongly interacting Fermi-Hubbard model, for which we identify two regimes resulting in different effective low-energy Hamiltonians. In the nonresonant regime, we realize an interacting spin model coupled to a static gauge field with a nonzero flux per plaquette. In the resonant regime, where the Hubbard interaction is a multiple of the driving frequency, we derive an effective Hamiltonian featuring doublon association and dissociation processes. The ground state of this Hamiltonian undergoes a phase transition between an ordered phase and a gapless Luttinger liquid phase. One can tune the system between different phases by changing the amplitude of the periodic drive. C1 [Bukov, Marin; Kolodrubetz, Michael; Polkovnikov, Anatoli] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Kolodrubetz, Michael] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Kolodrubetz, Michael] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Bukov, M (reprint author), Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. EM mbukov@bu.edu FU AFOSR [FA9550-13-1-0039]; NSF [DMR-1506340]; ARO [W911NF1410540]; Laboratory Directed Research and Development (LDRD) from Berkeley Lab; Office of Science, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We thank L. D'Alessio, E. Altman, W. Bakr, E. Demler, M. Eckstein, A. Grushin, M. Heyl, D. Huse, A. Iaizzi, G. Jotzu, R. Kaul, S. Kourtis, M. Piraud, A. Sandvik, and R. Singh for insightful and interesting discussions. We are especially grateful to M. Dolfi and all contributors to the ALPS project [77,78] for developing the ALPS MPS and DMRG tools used in this work. We thank A. Rosch for pointing out to us the potential connection between the HFE and the SWT. This work was supported by AFOSR FA9550-13-1-0039, NSF DMR-1506340, and ARO W911NF1410540. M. K. was supported by Laboratory Directed Research and Development (LDRD) funding from Berkeley Lab, provided by the Director, Office of Science, of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. NR 87 TC 6 Z9 6 U1 2 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 21 PY 2016 VL 116 IS 12 AR 125301 DI 10.1103/PhysRevLett.116.125301 PG 6 WC Physics, Multidisciplinary SC Physics GA DH4AC UT WOS:000372726900005 PM 27058085 ER PT J AU O'Donnell, M Li, HL AF O'Donnell, Mike Li, Huilin TI The Eukaryotic Replisome Goes Under the Microscope SO CURRENT BIOLOGY LA English DT Review ID DNA-POLYMERASE-EPSILON; MINICHROMOSOME MAINTENANCE PROTEIN; REPLICATIVE HEXAMERIC HELICASE; SACCHAROMYCES-CEREVISIAE; STRUCTURAL BASIS; MCM2-7 HELICASE; POL ALPHA; CRYSTAL-STRUCTURE; III HOLOENZYME; FORK HELICASE AB The machinery at the eukaryotic replication fork has seen many new structural advances using electron microscopy and crystallography. Recent structures of eukaryotic replisome components include the Mcm2-7 complex, the CMG helicase, DNA polymerases, a Ctf4 trimer hub and the first look at a core replisome of 20 different proteins containing the helicase, primase, leading polymerase and a lagging strand polymerase. The eukaryotic core replisome shows an unanticipated architecture, with one polymerase sitting above the helicase and the other below. Additionally, structures of Mcm2 bound to an H3/H4 tetramer suggest a direct role of the replisome in handling nucleosomes, which are important to DNA organization and gene regulation. This review provides a summary of some of the many recent advances in the structure of the eukaryotic replisome. C1 [O'Donnell, Mike] Rockefeller Univ, DNA Replicat Lab, 1230 York Ave, New York, NY USA. [O'Donnell, Mike] SUNY Stony Brook, Howard Hughes Med Inst, Stony Brook, NY 11794 USA. [Li, Huilin] SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA. [Li, Huilin] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP O'Donnell, M (reprint author), Rockefeller Univ, DNA Replicat Lab, 1230 York Ave, New York, NY USA.; O'Donnell, M (reprint author), SUNY Stony Brook, Howard Hughes Med Inst, Stony Brook, NY 11794 USA.; Li, HL (reprint author), SUNY Stony Brook, Dept Biochem & Cell Biol, Stony Brook, NY 11794 USA.; Li, HL (reprint author), Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. EM odonnel@rockefeller.edu; hli@bnl.gov OI O'Donnell, Michael/0000-0001-9002-4214 FU US National Institutes of Health [GM111472, OD12272, GM115809]; Howard Hughes Medical Institute FX We appreciate help with some of the figures by Dr. Nina Yao (Rockefeller University). This work was funded by the US National Institutes of Health (GM111472 and OD12272 to H.L. and GM115809 to M.O.D.) and Howard Hughes Medical Institute (M.O.D.). NR 90 TC 4 Z9 4 U1 4 U2 22 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0960-9822 EI 1879-0445 J9 CURR BIOL JI Curr. Biol. PD MAR 21 PY 2016 VL 26 IS 6 BP R247 EP R256 DI 10.1016/j.cub.2016.02.034 PG 10 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA DG9NY UT WOS:000372411600014 PM 27003891 ER PT J AU Chao, P Karnesky, RA AF Chao, Paul Karnesky, Richard A. TI Hydrogen isotope trapping in Al-Cu binary alloys SO MATERIALS SCIENCE AND ENGINEERING A-STRUCTURAL MATERIALS PROPERTIES MICROSTRUCTURE AND PROCESSING LA English DT Article DE Age-hardening; Aluminum alloys; Hydrogen embrittlement; Al-Cu; Hydrogen diffusion and trapping; Hydrogen desorption ID HIGH-PURITY ALUMINUM; ELECTRICAL-RESISTIVITY; DIFFUSION; BEHAVIOR; PRECIPITATION; TEMPERATURES; DEPENDENCE; SYSTEMS AB The trapping mechanisms for hydrogen isotopes in Al-X Cu (0.0 at% < X < 3.5 at%) alloys were investigated using thermal desorption spectroscopy (TDS), electrical conductivity, and differential scanning calorimetry. Constant heating rate TDS was used to determine microstructural trap energies and occupancies. In addition to the trapping states in pure Al reported in the literature (interstitial lattice sites, dislocations, and vacancies), a trap site due to Al-Cu intermetallic precipitates is observed. The binding energy of this precipitate trap is (18 +/- 3) kJ mol(-1) (0.19 +/- 0.03 eV). Typical occupancy of this trap is high; for Al-2.6 at% Cu (a Cu composition comparable to that in AA2219) charged at 200 degrees C with 130 MPa D-2 for 68 days, there is ca. there is 3.15 x 10(-7) mol D bound to the precipitate trap per mol of Al, accounting for a third of the D in the charged sample. (C) 2016 Elsevier B.V. All rights reserved. C1 [Chao, Paul; Karnesky, Richard A.] Sandia Natl Labs, Livermore, CA USA. [Chao, Paul] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. RP Karnesky, RA (reprint author), Sandia Natl Labs, Livermore, CA USA. EM rakarne@sandia.gov OI Karnesky, Richard/0000-0003-4717-457X FU Sandia National Laboratories Laboratory Directed Research and Development (LDRD) Program [165724]; US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Drs. D.K. Ward, C. San Marchi, B.P. Somerday, and D.K. Balch are thanked for helpful discussions. The authors gratefully acknowledge support from the Sandia National Laboratories Laboratory Directed Research and Development (LDRD) Program (Project 165724). Sandia is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under Contract no. DE-AC04-94AL85000. NR 37 TC 0 Z9 0 U1 3 U2 9 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0921-5093 EI 1873-4936 J9 MAT SCI ENG A-STRUCT JI Mater. Sci. Eng. A-Struct. Mater. Prop. Microstruct. Process. PD MAR 21 PY 2016 VL 658 BP 422 EP 428 DI 10.1016/j.msea.2016.02.003 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DH1QU UT WOS:000372560800050 ER PT J AU Suchyta, E Huff, EM Aleksic, J Melchior, P Jouvel, S MacCrann, N Ross, AJ Crocce, M Gaztanaga, E Honscheid, K Leistedt, B Peiris, HV Rykoff, ES Sheldon, E Abbott, T Abdalla, FB Allam, S Banerji, M Benoit-Levy, A Bertin, E Burke, DL Burke, DL Rosell, AC Kind, MC Carretero, J Cunha, CE D'Andrea, CB da Costa, LN Depoy, DL Desai, S Diehl, HT Dietrich, JP Doel, P Eifler, TF Estrada, J Evrard, AE Flaugher, B Fosalba, P Frieman, J Gerdes, DW Gruen, D Gruendl, RA James, DJ Jarvis, M Kuehn, K Kuropatkin, N Lahav, O Lima, M Maia, MAG March, M Marshall, JL Miller, CJ Miquel, R Neilsen, E Nichol, RC Nord, B Ogando, R Percival, WJ Reil, K Roodman, A Sako, M Sanchez, E Scarpine, V Sevilla-Noarbe, I Smith, RC Soares-Santos, M Sobreira, F Swanson, MEC Tarle, G Thaler, J Thomas, D Vikram, V Walker, AR Wechsler, RH Zhang, Y AF Suchyta, E. Huff, E. M. Aleksic, J. Melchior, P. Jouvel, S. MacCrann, N. Ross, A. J. Crocce, M. Gaztanaga, E. Honscheid, K. Leistedt, B. Peiris, H. V. Rykoff, E. S. Sheldon, E. Abbott, T. Abdalla, F. B. Allam, S. Banerji, M. Benoit-Levy, A. Bertin, E. Brooks, D. Burke, D. L. Carnero Rosell, A. Carrasco Kind, M. Carretero, J. Cunha, C. E. D'Andrea, C. B. da Costa, L. N. DePoy, D. L. Desai, S. Diehl, H. T. Dietrich, J. P. Doel, P. Eifler, T. F. Estrada, J. Evrard, A. E. Flaugher, B. Fosalba, P. Frieman, J. Gerdes, D. W. Gruen, D. Gruendl, R. A. James, D. J. Jarvis, M. Kuehn, K. Kuropatkin, N. Lahav, O. Lima, M. Maia, M. A. G. March, M. Marshall, J. L. Miller, C. J. Miquel, R. Neilsen, E. Nichol, R. C. Nord, B. Ogando, R. Percival, W. J. Reil, K. Roodman, A. Sako, M. Sanchez, E. Scarpine, V. Sevilla-Noarbe, I. Smith, R. C. Soares-Santos, M. Sobreira, F. Swanson, M. E. C. Tarle, G. Thaler, J. Thomas, D. Vikram, V. Walker, A. R. Wechsler, R. H. Zhang, Y. CA DES Collaboration TI No galaxy left behind: accurate measurements with the faintest objects in the Dark Energy Survey SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE methods: data analysis; methods: miscellaneous; techniques: image processing; galaxies: statistics ID DIGITAL SKY SURVEY; REDSHIFT-SPACE DISTORTIONS; SCIENCE VERIFICATION DATA; PHOTOMETRIC REDSHIFTS; WIDE-FIELD; SDSS-III; CALIBRATION; COSMOS; SELECTION; UNCERTAINTIES AB Accurate statistical measurement with large imaging surveys has traditionally required throwing away a sizable fraction of the data. This is because most measurements have relied on selecting nearly complete samples, where variations in the composition of the galaxy population with seeing, depth, or other survey characteristics are small. We introduce a new measurement method that aims to minimize this wastage, allowing precision measurement for any class of detectable stars or galaxies. We have implemented our proposal in BALROG, software which embeds fake objects in real imaging to accurately characterize measurement biases. We demonstrate this technique with an angular clustering measurement using Dark Energy Survey (DES) data. We first show that recovery of our injected galaxies depends on a variety of survey characteristics in the same way as the real data. We then construct a flux-limited sample of the faintest galaxies in DES, chosen specifically for their sensitivity to depth and seeing variations. Using the synthetic galaxies as randoms in the Landy-Szalay estimator suppresses the effects of variable survey selection by at least two orders of magnitude. With this correction, our measured angular clustering is found to be in excellent agreement with that of a matched sample from much deeper, higher resolution space-based Cosmological Evolution Survey (COSMOS) imaging; over angular scales of 0 degrees.004 < theta < 0 degrees.2, we find a best-fitting scaling amplitude between the DES and COSMOS measurements of 1.00 +/- 0.09. We expect this methodology to be broadly useful for extending measurements' statistical reach in a variety of upcoming imaging surveys. C1 [Suchyta, E.; Huff, E. M.; Melchior, P.; Honscheid, K.] Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. [Suchyta, E.; Huff, E. M.; Melchior, P.; Ross, A. J.; Honscheid, K.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Aleksic, J.; Carretero, J.; Miquel, R.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Jouvel, S.; Leistedt, B.; Peiris, H. V.; Abdalla, F. B.; Brooks, D.; Doel, P.; Lahav, O.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [MacCrann, N.] Univ Manchester, Sch Phys & Astron, Jodrell Bank Ctr Astrophys, Oxford Rd, Manchester M13 9PL, Lancs, England. [Crocce, M.; Gaztanaga, E.; Carretero, J.; Fosalba, P.] CSIC, IEEC, Inst Ciencies Espai, Campus UAB,Carrer Can Magrans S-N, E-08193 Barcelona, Spain. [Rykoff, E. S.; Burke, D. L.; Cunha, C. E.; Roodman, A.; Wechsler, R. H.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, POB 2450, Stanford, CA 94305 USA. [Rykoff, E. S.; Burke, D. L.; Reil, K.; Roodman, A.; Wechsler, R. H.] Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Sheldon, E.] Brookhaven Natl Lab, Bldg 510, Upton, NY 11973 USA. [Abbott, T.; James, D. J.; Smith, R. C.; Walker, A. R.] Natl Opt Astron Observ, Cerro Tololo Inter Amer Observ, Casilla 603, La Serena, Chile. [Abdalla, F. B.; Estrada, J.] Rhodes Univ, Dept Phys Elect, POB 94, ZA-6140 Grahamstown, South Africa. [Allam, S.; Diehl, H. T.; Flaugher, B.; Frieman, J.; Kuropatkin, N.; Neilsen, E.; Nord, B.; Scarpine, V.; Soares-Santos, M.; Sobreira, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Banerji, M.] Univ Cambridge, Inst Astron, Madingley Rd, Cambridge CB3 0HA, England. [Banerji, M.] Univ Cambridge, Kavli Inst Cosmol, Madingley Rd, Cambridge CB3 0HA, England. [Bertin, E.] CNRS, UMR 7095, Inst Astrophys Paris, F-75014 Paris, France. [Bertin, E.] Univ Paris 06, Sorbonne Univ, UMR 7095, Inst Astrophys Paris, F-75014 Paris, France. [Carnero Rosell, A.; da Costa, L. N.; Lima, M.; Maia, M. A. G.; Ogando, R.; Sobreira, F.] Lab Interinst E Astron LIneA, Rua Gal Jose Cristino 77, BR-20921 Rio De Janeiro, RJ, Brazil. [Carnero Rosell, A.; da Costa, L. N.; Maia, M. A. G.; Ogando, R.] Observ Nacl, Rua Gal Jose Cristino 77, BR-20921 Rio De Janeiro, RJ, Brazil. [Carrasco Kind, M.; Gruendl, R. A.; Sevilla-Noarbe, I.] Univ Illinois, Dept Astron, 1002 W Green St, Urbana, IL 61801 USA. [Carrasco Kind, M.; Gruendl, R. A.; Swanson, M. E. C.] Univ Illinois, Natl Ctr Supercomp Applicat, 1205 West Clark St, Urbana, IL 61801 USA. [D'Andrea, C. B.; Nichol, R. C.; Percival, W. J.; Thomas, D.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [DePoy, D. L.; Marshall, J. L.] Texas A&M Univ, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [DePoy, D. L.; Marshall, J. L.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Desai, S.; Dietrich, J. P.] Excellence Cluster Univ, Boltzmannstr 2, D-85748 Garching, Germany. [Desai, S.] Univ Munich, Fac Phys, Scheinerstr 1, D-81679 Munich, Germany. [Dietrich, J. P.; Gruen, D.] Univ Munich, Univ Sternwarte, Fak Phys, Scheinerstr 1, D-81679 Munich, Germany. [Eifler, T. F.; Jarvis, M.; March, M.; Sako, M.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Eifler, T. F.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Evrard, A. E.; Miller, C. J.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Evrard, A. E.; Gerdes, D. W.; Miller, C. J.; Tarle, G.; Zhang, Y.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Frieman, J.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Gruen, D.] Max Planck Inst Extraterr Phys, Giessenbachstr, D-85748 Garching, Germany. [Kuehn, K.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Lima, M.] Univ Sao Paulo, Inst Fis, Dept Fis Matemat, CP 66318, BR-05314970 Sao Paulo, Brazil. [Miquel, R.] Inst Catalana Recerca & Estudis Avancats, E-08010 Barcelona, Spain. [Sanchez, E.; Sevilla-Noarbe, I.] CIEMAT, E-28040 Madrid, Spain. [Thaler, J.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Vikram, V.] Argonne Natl Lab, 9700 South Cass Ave, Lemont, IL 60439 USA. [Wechsler, R. H.] Stanford Univ, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94305 USA. RP Suchyta, E; Huff, EM (reprint author), Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA.; Suchyta, E; Huff, EM (reprint author), Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. EM eric.d.suchyta@gmail.com; emhuff@gmail.com RI Lima, Marcos/E-8378-2010; Fosalba Vela, Pablo/I-5515-2016; Ogando, Ricardo/A-1747-2010; Sobreira, Flavia/F-4168-2015; Gaztanaga, Enrique/L-4894-2014; OI Ogando, Ricardo/0000-0003-2120-1154; Sobreira, Flavia/0000-0002-7822-0658; Gaztanaga, Enrique/0000-0001-9632-0815; Suchyta, Eric/0000-0002-7047-9358; Carrasco Kind, Matias/0000-0002-4802-3194; Abdalla, Filipe/0000-0003-2063-4345 FU Ohio State University Graduate Presidential Fellowship; CCAPP postdoctoral fellowship; MINECO [FPA2012-39684, AYA2012-39559, ESP2013-48274, FPA2013-47986]; US Department of Energy [DE-FG02-91ER40690]; US National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Center for Cosmology and Astro-Particle Physics at The Ohio State University; Mitchell Institute for Fundamental Physics and Astronomy at Texas AM University; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia, Tecnologia e Inovacao; Deutsche Forschungsgemeinschaft; DES; National Science Foundation [AST-1138766]; Argonne National Laboratory; University of California at Santa Cruz; University of Cambridge; Centro de Investigaciones Energeticas; Medioambientales y Tecnologicas-Madrid; University of Chicago; University College London; DES-Brazil Consortium; University of Edinburgh; Eidgenossische Technische Hochschule (ETH) Zurich; Fermi National Accelerator Laboratory; University of Illinois at Urbana-Champaign; Institut de Ciencies de l'Espai (IEEC/CSIC); Institut de Fisica d'Altes Energies; Lawrence Berkeley National Laboratory; Ludwig-Maximilians Universitat Munchen; associated Excellence Cluster Universe; University of Michigan; National Optical Astronomy Observatory; University of Nottingham; Ohio State University; University of Pennsylvania; University of Portsmouth; SLAC National Accelerator Laboratory; Stanford University; University of Sussex; Texas AM University; Centro de Excelencia Severo Ochoa [SEV-2012-0234]; European Research Council under the European Union [240672, 291329, 306478] FX ES is supported by an Ohio State University Graduate Presidential Fellowship. EMH is funded by a CCAPP postdoctoral fellowship. JA is partially supported by MINECO under grant FPA2012-39684. PM is supported by the US Department of Energy under Contract No. DE-FG02-91ER40690.r Funding for the DES Projects has been provided by the US Department of Energy, the US National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, the Center for Cosmology and Astro-Particle Physics at The Ohio State University, the Mitchell Institute for Fundamental Physics and Astronomy at Texas A&M University, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia, Tecnologia e Inovacao, the Deutsche Forschungsgemeinschaft and the Collaborating Institutions in the DES. The DESDM system is supported by the National Science Foundation under Grant Number AST-1138766.r The Collaborating Institutions are Argonne National Laboratory, the University of California at Santa Cruz, the University of Cambridge, Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid, the University of Chicago, University College London, the DES-Brazil Consortium, the University of Edinburgh, the Eidgenossische Technische Hochschule (ETH) Zurich, Fermi National Accelerator Laboratory, the University of Illinois at Urbana-Champaign, the Institut de Ciencies de l'Espai (IEEC/CSIC), the Institut de Fisica d'Altes Energies, Lawrence Berkeley National Laboratory, the Ludwig-Maximilians Universitat Munchen and the associated Excellence Cluster Universe, the University of Michigan, the National Optical Astronomy Observatory, the University of Nottingham, The Ohio State University, the University of Pennsylvania, the University of Portsmouth, SLAC National Accelerator Laboratory, Stanford University, the University of Sussex, and Texas A&M University.r The DES participants from Spanish institutions are partially supported by MINECO under grants AYA2012-39559, ESP2013-48274, FPA2013-47986, and Centro de Excelencia Severo Ochoa SEV-2012-0234. Research leading to these results has received funding from the European Research Council under the European Unions Seventh Framework Programme (FP7/2007-2013) including ERC grant agreements 240672, 291329, and 306478. NR 66 TC 7 Z9 7 U1 0 U2 3 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD MAR 21 PY 2016 VL 457 IS 1 BP 786 EP 808 DI 10.1093/mnras/stv2953 PG 23 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DH2FM UT WOS:000372599600054 ER PT J AU Jennings, E Wechsler, RH Skillman, SW Warren, MS AF Jennings, Elise Wechsler, Risa H. Skillman, Samuel W. Warren, Michael S. TI Disentangling redshift-space distortions and non-linear bias using the 2D power spectrum SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE cosmology: theory; large-scale structure of Universe ID HALO OCCUPATION DISTRIBUTION; LUMINOUS RED GALAXIES; GROWTH-RATE; MASS; MODELS; GRAVITY AB We present the 2D redshift-space galaxy power spectrum, P(k, mu), measured from the Dark Sky simulations, using catalogues constructed with halo occupation distribution and subhalo abundance matching methods, chosen to represent an intermediate redshift sample of luminous red galaxies. We find that the information content in individual mu (cosine of the angle to the line of sight) bins is substantially richer then multipole moments, and show that this can be used to isolate the impact of non-linear growth and redshift-space distortion (RSD) effects. Using the mu < 0.2 simulation data, which is not impacted by RSD, we can successfully measure the non-linear bias to similar to 5 per cent at k < 0.6 h Mpc(-1). Using the low mu simulation data to constrain the non-linear bias, and mu >= 0.2 to constrain the growth rate, we show that f can be constrained to similar to 26(22) per cent to a k(max) < 0.4(0.6) h Mpc(-1) from clustering alone using a dispersion model, for a range of galaxy models. Our analysis of individual mu bins reveals interesting physical effects which arise from different methods of populating haloes with galaxies. We find a prominent turnaround scale, at which RSD damping effects are greater than the nonlinear growth, which differs for each galaxy model. The idea of separating non-linear growth and RSD effects making use of the full information in the 2D galaxy power spectrum yields significant improvements in constraining cosmological parameters and may be a promising probe of galaxy formation models. C1 [Jennings, Elise] Ctr Particle Astrophys, Fermi Natl Accelerator Lab MS209, POB 500,Kirk Rd & Pine St, Batavia, IL 60510 USA. [Jennings, Elise] Univ Chicago, Enrico Fermi Inst, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Wechsler, Risa H.; Skillman, Samuel W.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Dept Phys, Stanford, CA 94305 USA. [Wechsler, Risa H.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Warren, Michael S.] LANL, Theoret Div, Los Alamos, NM 87545 USA. RP Jennings, E (reprint author), Ctr Particle Astrophys, Fermi Natl Accelerator Lab MS209, POB 500,Kirk Rd & Pine St, Batavia, IL 60510 USA.; Jennings, E (reprint author), Univ Chicago, Enrico Fermi Inst, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. EM elise@fnal.gov FU Fermi Research Alliance, LLC under the US Department of Energy [DE-AC02-07CH11359]; US Department of Energy [DE-AC02-76SF00515] FX This research made use of the Dark Sky Simulations, which were produced using an INCITE 2014 allocation on the Oak Ridge Leadership Computing Facility at Oak Ridge National Laboratory. We are grateful to Matt Turk and the rest of our Dark Sky collaborators. We also thank Yao-Yuan Mao for running the merger trees, and to Benjamin Lehmann for assistance with galaxy catalogue production. We are grateful to the University of Chicago Research Computing Center and we thank the scientific computing team at SLAC for their support related to hosting data through the darksky server. We thank Eduardo Rozo for a careful reading of the first draft, and Carlton Baugh, Scott Dodelson and Andrey Kratsov for useful discussions. EJ is supported by Fermi Research Alliance, LLC under the US Department of Energy under contract No. DE-AC02-07CH11359. RHW received support from the US Department of Energy under contract number DE-AC02-76SF00515. NR 64 TC 4 Z9 4 U1 0 U2 1 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD MAR 21 PY 2016 VL 457 IS 1 BP 1076 EP 1088 DI 10.1093/mnras/stv2989 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DH2FM UT WOS:000372599600077 ER PT J AU Riedel, CJ Zurek, WH Zwolak, M AF Riedel, C. Jess Zurek, Wojciech H. Zwolak, Michael TI Objective past of a quantum universe: Redundant records of consistent histories SO PHYSICAL REVIEW A LA English DT Article ID ENVIRONMENT-INDUCED DECOHERENCE; YIELD CONTRARY INFERENCES; LOGICAL REFORMULATION; MECHANICS; DARWINISM; INFORMATION; STATES; SETS; PREDICTABILITY; EINSELECTION AB Motivated by the advances of quantum Darwinism and recognizing the role played by redundancy in identifying the small subset of quantum states with resilience characteristic of objective classical reality, we explore the implications of redundant records for consistent histories. The consistent histories formalism is a tool for describing sequences of events taking place in an evolving closed quantum system. A set of histories is consistent when one can reason about them using Boolean logic, i.e., when probabilities of sequences of events that define histories are additive. However, the vast majority of the sets of histories that are merely consistent are flagrantly nonclassical in other respects. This embarras de richesses (known as the set selection problem) suggests that one must go beyond consistency to identify how the classical past arises in our quantum universe. The key intuition we follow is that the records of events that define the familiar objective past are inscribed in many distinct systems, e.g., subsystems of the environment, and are accessible locally in space and time to observers. We identify histories that are not just consistent but redundantly consistent using the partial-trace condition introduced by Finkelstein as a bridge between histories and decoherence. The existence of redundant records is a sufficient condition for redundant consistency. It selects, from the multitude of the alternative sets of consistent histories, a small subset endowed with redundant records characteristic of the objective classical past. The information about an objective history of the past is then simultaneously within reach of many, who can independently reconstruct it and arrive at compatible conclusions in the present. C1 [Riedel, C. Jess] Perimeter Inst Theoret Phys, Waterloo, ON N2L 2Y5, Canada. [Riedel, C. Jess] IBM Watson Res Ctr, Yorktown Hts, NY 10598 USA. [Riedel, C. Jess; Zurek, Wojciech H.] LANL, Theoret Div, Los Alamos, NM 87545 USA. [Zwolak, Michael] Oregon State Univ, Dept Phys, Corvallis, OR 97331 USA. RP Riedel, CJ (reprint author), Perimeter Inst Theoret Phys, Waterloo, ON N2L 2Y5, Canada.; Riedel, CJ (reprint author), IBM Watson Res Ctr, Yorktown Hts, NY 10598 USA.; Riedel, CJ (reprint author), LANL, Theoret Div, Los Alamos, NM 87545 USA. EM jessriedel@gmail.com RI Zwolak, Michael/G-2932-2013 OI Zwolak, Michael/0000-0001-6443-7816 FU U.S. Department of Energy through the LANL/LDRD program; John Templeton Foundation; Foundational Questions Institute on "Physics of What Happens" [2015-144057]; Government of Canada through Industry Canada; Province of Ontario through the Ministry of Research and Innovation FX We thank Charles Bennett, Robert Griffiths, James Hartle, Adrian Kent, and Lev Vaidman for discussion. We also thank the University of Ulm for hosting us while this work was being prepared. This research was partially supported by the U.S. Department of Energy through the LANL/LDRD program, by the John Templeton Foundation, and by the Foundational Questions Institute Grant No. 2015-144057 on "Physics of What Happens." Research at the Perimeter Institute is supported by the Government of Canada through Industry Canada and by the Province of Ontario through the Ministry of Research and Innovation. NR 109 TC 3 Z9 3 U1 3 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9926 EI 2469-9934 J9 PHYS REV A JI Phys. Rev. A PD MAR 21 PY 2016 VL 93 IS 3 AR 032126 DI 10.1103/PhysRevA.93.032126 PG 16 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DH0PD UT WOS:000372485200002 ER PT J AU Homes, CC Dai, YM Schneeloch, J Zhong, RD Gu, GD AF Homes, C. C. Dai, Y. M. Schneeloch, J. Zhong, R. D. Gu, G. D. TI Phonon anomalies in some iron telluride materials SO PHYSICAL REVIEW B LA English DT Article ID SUPERCONDUCTIVITY; CHALCOGENIDES; PNICTIDES; STATES AB The detailed temperature dependence of the infrared-active mode in Fe1.03Te (T-N similar or equal to 68 K) and Fe1.13Te (T-N similar or equal to 56 K) has been examined, and the position, width, strength, and asymmetry parameter have been determined using an asymmetric Fano profile superimposed on an electronic background. In both materials the frequency of the mode increases as the temperature is reduced; however, there is also a slight asymmetry in the line shape, indicating that the mode is coupled to either spin or charge excitations. Below T-N there is an anomalous decrease in frequency, and the mode shows little temperature dependence, at the same time becoming more symmetric, suggesting a reduction in spin-or electron-phonon coupling. The frequency of the infrared-active mode and the magnitude of the shift below T-N are predicted reasonably well by first-principles calculations; however, the predicted splitting of the mode is not observed. In superconducting FeTe0.55Se0.45 (T-c similar or equal to 14 K) the infrared-active E-u mode displays asymmetric line shape at all temperatures, which is most pronounced between 100 and 200 K, indicating the presence of either spin- or electron-phonon coupling, which may be a necessary prerequisite for superconductivity in this class of materials. C1 [Homes, C. C.; Dai, Y. M.; Schneeloch, J.; Zhong, R. D.; Gu, G. D.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Homes, CC; Dai, YM (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM homes@bnl.gov; ymdai@lanl.gov RI Zhong, Ruidan/D-5296-2013; Dai, Yaomin/E-4259-2016 OI Zhong, Ruidan/0000-0003-1652-9454; Dai, Yaomin/0000-0002-2464-3161 FU Office of Science, US Department of Energy [DE-SC0012704]; Center for Emergent Superconductivity, an Energy Frontier Research Center - US Department of Energy, Office of Science FX We would like to acknowledge helpful discussions with T. Birol. We are indebted to S. V. Dordevic for referring us to a phenomenological Fano line shape, developed by A. Damascelli and A. Kuzmenko. This work is supported by the Office of Science, US Department of Energy under Contract No. DE-SC0012704. J.S. and R.D.Z. are supported by the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science. NR 53 TC 3 Z9 3 U1 6 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 21 PY 2016 VL 93 IS 12 AR 125135 DI 10.1103/PhysRevB.93.125135 PG 8 WC Physics, Condensed Matter SC Physics GA DH3VV UT WOS:000372715800006 ER PT J AU Biswas, S Palit, R Navin, A Rejmund, M Bisoi, A Sarkar, MS Sarkar, S Bhattacharyya, S Biswas, DC Caamano, M Carpenter, MP Choudhury, D Clement, E Danu, LS Delaune, O Farget, F de France, G Hota, SS Jacquot, B Lemasson, A Mukhopadhyay, S Nanal, V Pillay, RG Saha, S Sethi, J Singh, P Srivastava, PC Tandel, SK AF Biswas, S. Palit, R. Navin, A. Rejmund, M. Bisoi, A. Sarkar, M. Saha Sarkar, S. Bhattacharyya, S. Biswas, D. C. Caamano, M. Carpenter, M. P. Choudhury, D. Clement, E. Danu, L. S. Delaune, O. Farget, F. de France, G. Hota, S. S. Jacquot, B. Lemasson, A. Mukhopadhyay, S. Nanal, V. Pillay, R. G. Saha, S. Sethi, J. Singh, Purnima Srivastava, P. C. Tandel, S. K. TI Structure of Te-132(52)80: The two-particle and two-hole spectrum of Sn-132(50)82 SO PHYSICAL REVIEW C LA English DT Article ID FISSION FRAGMENTS; EXCITED-STATES; SHELL-MODEL; GAMMA-RAY; NUCLEI; SPECTROMETER; ARRAY AB High-spin states in Te-132, an isotope with two proton particles and two neutron holes outside of the Sn-132 doubly magic core, have been extended up to an excitation energy of 6.17 MeV. The prompt-delayed coincidence technique has been used to correlate states above the T-1/2 = 3.70(9) mu s isomer in Te-132 to the lower states using Th-232(Li-7, f) at 5.4 MeV/u and the Indian National Gamma Array (INGA). With Be-9(U-238, f) at 6.2 MeV/u and EXOGAM gamma-array coupled with the VAMOS++ spectrometer, the level scheme was extended to higher excitation energies. The high-spin positive-parity states, above J(pi) = 10(+), in Te-132 are expected to arise from the alignment of the particles in the high-j orbitals lying close to the Fermi surface, the pi g(7/2)(2), and the nu h(11/2)(-2) configurations. The experimental level scheme has been compared with the large scale shell model calculations. A reduction in the p-n interaction strength resulted in an improved agreement with the measurements up to the spin of 15 (h) over bar. In contrast, the comparison of the differences between the experiment and these calculations for the N = 76,78 isotones of Te and Sn shows the increasing disagreement as a function of spin, where the magnitude is larger in Te than in Sn. This behavior could possibly be attributed to the deficiencies in the p-n correlations, in addition to the n-n correlations in Sn. C1 [Biswas, S.; Palit, R.; Choudhury, D.; Nanal, V.; Pillay, R. G.; Saha, S.; Sethi, J.; Singh, Purnima] Tata Inst Fundamental Res, Dept Nucl & Atom Phys, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Navin, A.; Rejmund, M.; Clement, E.; Delaune, O.; Farget, F.; de France, G.; Jacquot, B.; Lemasson, A.] CEA, GANIL, CNRS, DRF,IN2P3, Bd Henri Becquerel,BP 55027, F-14076 Caen 5, France. [Bisoi, A.; Sarkar, S.] Indian Inst Engn Sci & Technol, Sibpur 711103, Howrah, India. [Sarkar, M. Saha] Saha Inst Nucl Phys, Kolkata 700064, W Bengal, India. [Bhattacharyya, S.] Ctr Variable Energy Cyclotron, Kolkata 700064, India. [Biswas, D. C.; Danu, L. S.; Mukhopadhyay, S.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Caamano, M.] Univ Santiago de Compostela, E-15706 Santiago De Compostela, Spain. [Carpenter, M. P.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Hota, S. S.] Australian Natl Univ, GPO Box 4, Canberra, ACT 2601, Australia. [Srivastava, P. C.] Indian Inst Technol, Dept Phys, Roorkee 247667, Uttar Pradesh, India. [Tandel, S. K.] UM DAE Ctr Excellence Basic Sci, Mumbai 400098, Maharashtra, India. RP Biswas, S (reprint author), Tata Inst Fundamental Res, Dept Nucl & Atom Phys, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. RI Palit, Rudrajyoti/F-5185-2012; caamano, manuel/A-1832-2013 OI caamano, manuel/0000-0002-5045-003X FU Department of Science and Technology, Government of India [IR/S2/PF-03/2003-II]; LIA France-India FX The authors would like to acknowledge the TIFR-BARC Pelletron Linac Facility for providing a good quality beam. The help and cooperation of the INGA collaboration in setting up the array is acknowledged. This work has been partially funded by the Department of Science and Technology, Government of India (No. IR/S2/PF-03/2003-II). We acknowledge B. S. Naidu, S. Jadhav, and R. Donthi for their technical help during the INGA experiment. We would also like to thank the GANIL accelerator staff and acknowledge the important technical contributions of J. Goupil, G. Fermont, L. Menager, J. Ropert, C. Spitaels. We thank C. Schmitt for help in various aspects related to the GANIL experiment. Two of us (S.Bi. and S.Bh.) acknowledge partial financial support through the LIA France-India agreement. NR 41 TC 1 Z9 1 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 21 PY 2016 VL 93 IS 3 AR 034324 DI 10.1103/PhysRevC.93.034324 PG 8 WC Physics, Nuclear SC Physics GA DH3XF UT WOS:000372719400002 ER PT J AU Urban, W Sieja, K Rzaca-Urban, T Czerwinski, M Naidja, H Nowacki, F Smith, AG Ahmad, I AF Urban, W. Sieja, K. Rzaca-Urban, T. Czerwinski, M. Naidja, H. Nowacki, F. Smith, A. G. Ahmad, I. TI First evidence of gamma collectivity close to the doubly magic core Sn-132 SO PHYSICAL REVIEW C LA English DT Article ID RICH XE ISOTOPES; NEUTRON-RICH; OCTUPOLE CORRELATIONS; SPONTANEOUS FISSION; EXCITED-STATES; SHELL-MODEL; TRANSITION; NUCLEI AB The Te-138 and Xe-140 nuclei have been reinvestigated using prompt gamma-ray data from spontaneous fission of Cm-248, collected with the EUROGAM2 Ge array. gamma bands have been identified in both nuclei. The gamma band observed in Te-138, a nucleus with only six valence nucleons, indicates the presence of collectivity very close to the doubly magic Sn-132 core. Such band is even more pronounced in Xe-140, the N = 86 isotone of Te-138. The newly observed bands are interpreted within the shell model, which reproduce well the. collectivity at N = 86. C1 [Urban, W.; Rzaca-Urban, T.; Czerwinski, M.] Univ Warsaw, Fac Phys, Ulica Pasteura 5, PL-02093 Warsaw, Poland. [Sieja, K.; Naidja, H.; Nowacki, F.] Univ Strasbourg, IPHC, 23 Rue Loess, F-67037 Strasbourg, France. [Sieja, K.; Naidja, H.; Nowacki, F.] CNRS, UMR7178, F-67037 Strasbourg, France. [Naidja, H.] GSI Helmholtzzentrum Schwerionenforsch GmbH, D-64291 Darmstadt, Germany. [Naidja, H.] Univ Constantine 1, LPMS, Route Ain El Bey, Constantine 25000, Algeria. [Smith, A. G.] Univ Manchester, Dept Phys & Astron, Manchester M13 9PL, Lancs, England. [Ahmad, I.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Urban, W (reprint author), Univ Warsaw, Fac Phys, Ulica Pasteura 5, PL-02093 Warsaw, Poland. FU US Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357]; Helmholtz association through the Nuclear Astrophysics Virtual Institute NAVI [VH-VI-417] FX This material is based upon work supported by the US Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357. The authors are grateful for the use of 248Cm to the Office of Basic Energy Sciences, US Department of Energy, through the transplutonium element production facilities at Oak Ridge National Laboratory. H.N. acknowledges support from the Helmholtz association through the Nuclear Astrophysics Virtual Institute NAVI (Grant No. VH-VI-417). NR 23 TC 2 Z9 2 U1 2 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 21 PY 2016 VL 93 IS 3 AR 034326 DI 10.1103/PhysRevC.93.034326 PG 10 WC Physics, Nuclear SC Physics GA DH3XF UT WOS:000372719400004 ER PT J AU Amole, C Ardid, M Arnquist, IJ Asner, DM Baxter, D Behnke, E Bhattacharjee, P Borsodi, H Bou-Cabo, M Brice, SJ Broemmelsiek, D Clark, K Collar, JI Cooper, PS Crisler, M Dahl, CE Das, M Debris, F Fallows, S Farine, J Felis, I Filgas, R Fines-Neuschild, M Girard, F Giroux, G Hall, J Harris, O Hoppe, EW Jackson, CM Jin, M Krauss, CB Lafreniere, M Laurin, M Lawson, I Leblanc, A Levine, I Lippincott, WH Mann, E Martin, JP Maurya, D Mitra, P Olson, S Neilson, R Noble, AJ Plante, A Podviianiuk, RB Priya, S Robinson, AE Ruschman, M Scallon, O Sonnenschein, A Starinski, N Stekl, I Vazquez-Jauregui, E Wells, J Wichoski, U Zacek, V Zhang, J AF Amole, C. Ardid, M. Arnquist, I. J. Asner, D. M. Baxter, D. Behnke, E. Bhattacharjee, P. Borsodi, H. Bou-Cabo, M. Brice, S. J. Broemmelsiek, D. Clark, K. Collar, J. I. Cooper, P. S. Crisler, M. Dahl, C. E. Das, M. Debris, F. Fallows, S. Farine, J. Felis, I. Filgas, R. Fines-Neuschild, M. Girard, F. Giroux, G. Hall, J. Harris, O. Hoppe, E. W. Jackson, C. M. Jin, M. Krauss, C. B. Lafreniere, M. Laurin, M. Lawson, I. Leblanc, A. Levine, I. Lippincott, W. H. Mann, E. Martin, J. P. Maurya, D. Mitra, P. Olson, S. Neilson, R. Noble, A. J. Plante, A. Podviianiuk, R. B. Priya, S. Robinson, A. E. Ruschman, M. Scallon, O. Sonnenschein, A. Starinski, N. Stekl, I. Vazquez-Jauregui, E. Wells, J. Wichoski, U. Zacek, V. Zhang, J. CA PICO Collaboration TI Improved dark matter search results from PICO-2L Run 2 SO PHYSICAL REVIEW D LA English DT Article ID CANDIDATES; CONSTRAINTS; DETECTOR AB New data are reported from a second run of the 2-liter PICO-2L C3F8 bubble chamber with a total exposure of 129 kg-days at a thermodynamic threshold energy of 3.3 keV. These data show that measures taken to control particulate contamination in the superheated fluid resulted in the absence of the anomalous background events observed in the first run of this bubble chamber. One single nuclear-recoil event was observed in the data, consistent both with the predicted background rate from neutrons and with the observed rate of unambiguous multiple-bubble neutron scattering events. The chamber exhibits the same excellent electron-recoil and alpha decay rejection as was previously reported. These data provide the most stringent direct detection constraints on weakly interacting massive particle (WIMP)-proton spin-dependent scattering to date for WIMP masses < 50 GeV/c(2). C1 [Amole, C.; Giroux, G.; Olson, S.; Noble, A. J.] Queens Univ, Dept Phys, Kingston, ON K7L 3N6, Canada. [Ardid, M.; Bou-Cabo, M.; Felis, I.] Univ Politecn Valencia, Dept Fis Aplicada, E-46022 Valencia, Spain. [Arnquist, I. J.; Asner, D. M.; Hall, J.; Hoppe, E. W.] Pacific NW Natl Lab, Richland, WA 99354 USA. [Baxter, D.; Dahl, C. E.; Jin, M.; Zhang, J.] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. [Behnke, E.; Borsodi, H.; Harris, O.; Levine, I.; Mann, E.; Wells, J.] Indiana Univ, Dept Phys, South Bend, IN 46634 USA. [Bhattacharjee, P.; Das, M.] Saha Inst Nucl Phys, AstroParticle Phys & Cosmol Div, Kolkata 700064, India. [Brice, S. J.; Broemmelsiek, D.; Cooper, P. S.; Crisler, M.; Dahl, C. E.; Lippincott, W. H.; Robinson, A. E.; Ruschman, M.; Sonnenschein, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Clark, K.] Univ Toronto, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada. [Collar, J. I.] Univ Chicago, Enrico Fermi Inst, KICP, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Collar, J. I.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Debris, F.; Fines-Neuschild, M.; Girard, F.; Jackson, C. M.; Lafreniere, M.; Laurin, M.; Martin, J. P.; Plante, A.; Scallon, O.; Starinski, N.; Zacek, V.] Univ Montreal, Dept Phys, CP 6128, Montreal, PQ H3C 3J7, Canada. [Fallows, S.; Krauss, C. B.; Mitra, P.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada. [Farine, J.; Girard, F.; Lawson, I.; Leblanc, A.; Podviianiuk, R. B.; Scallon, O.; Wichoski, U.] Laurentian Univ, Dept Phys, Sudbury, ON P3E 2C6, Canada. [Filgas, R.; Stekl, I.] Czech Tech Univ, Inst Expt & Appl Phys, CZ-12800 Prague, Czech Republic. [Lawson, I.] SNOLAB, Lively, ON P3Y 1N2, Canada. [Maurya, D.; Priya, S.] Virginia Tech, CEHMS, BMDL, Blacksburg, VA 24061 USA. [Neilson, R.] Drexel Univ, Dept Phys, Philadelphia, PA 19104 USA. [Vazquez-Jauregui, E.] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City 01000, DF, Mexico. RP Amole, C (reprint author), Queens Univ, Dept Phys, Kingston, ON K7L 3N6, Canada. EM camole@owl.phy.queensu.ca OI Dahl, Carl Eric/0000-0003-1637-2346 FU Fermi National Accelerator Laboratory [DE-AC02-07CH11359]; Pacific Northwest National Laboratory; National Sciences and Engineering Research Council of Canada (NSERC); Canada Foundation for Innovation (CFI); National Science Foundation (NSF) [PHY-1242637, PHY-0919526, PHY-1205987, PHY-1506377]; U.S. Department of Energy [DE-SC-0012161]; Department of Atomic Energy (DAE), Government of India, under the Center of AstroParticle Physics II project (CAPP-II) at Saha Institute of Physics (SINP); Czech Ministry of Education, Youth and Sports [LM2011027]; Spanish Ministerio de Economia y Competitividad, Consolider MultiDark [CSD2009-00064]; DGAPA-UNAM through grant PAPIIT [IA100316] FX The PICO Collaboration thanks SNOLAB for their exceptional laboratory space and technical support. We also thank Fermi National Accelerator Laboratory (Contract No. DE-AC02-07CH11359) and Pacific Northwest National Laboratory for their support. This work is supported by the National Sciences and Engineering Research Council of Canada (NSERC), the Canada Foundation for Innovation (CFI), the National Science Foundation (NSF) under the Grants No. PHY-1242637, No. PHY-0919526, No. PHY-1205987, and No. PHY-1506377 and by the U.S. Department of Energy under Award No. DE-SC-0012161. We also acknowledge the support of Department of Atomic Energy (DAE), Government of India, under the Center of AstroParticle Physics II project (CAPP-II) at Saha Institute of Physics (SINP); the Czech Ministry of Education, Youth and Sports (Grant No. LM2011027); the Spanish Ministerio de Economia y Competitividad, Consolider MultiDark (Grant No. CSD2009-00064) and DGAPA-UNAM through grant PAPIIT No. IA100316. NR 44 TC 22 Z9 22 U1 2 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 21 PY 2016 VL 93 IS 6 AR 061101 DI 10.1103/PhysRevD.93.061101 PG 5 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DH3YD UT WOS:000372721800001 ER PT J AU Yang, G Fragner, A Koolstra, G Ocola, L Czaplewski, DA Schoelkopf, RJ Schuster, DI AF Yang, Ge Fragner, A. Koolstra, G. Ocola, L. Czaplewski, D. A. Schoelkopf, R. J. Schuster, D. I. TI Coupling an Ensemble of Electrons on Superfluid Helium to a Superconducting Circuit SO PHYSICAL REVIEW X LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; LIQUID-HELIUM; QUANTUM ELECTRODYNAMICS; SURFACE; TRANSITION; STATE; QUBIT; SPIN AB The quantized lateral motional states and the spin states of electrons trapped on the surface of superfluid helium have been proposed as basic building blocks of a scalable quantum computer. Circuit quantum electrodynamics allows strong dipole coupling between electrons and a high-Q superconducting microwave resonator, enabling such sensitive detection and manipulation of electron degrees of freedom. Here, we present the first realization of a hybrid circuit in which a large number of electrons are trapped on the surface of superfluid helium inside a coplanar waveguide resonator. The high finesse of the resonator allows us to observe large dispersive shifts that are many times the linewidth and make fast and sensitive measurements on the collective vibrational modes of the electron ensemble, as well as the superfluid helium film underneath. Furthermore, a large ensemble coupling is observed in the dispersive regime during experiment, and it shows excellent agreement with our numeric model. The coupling strength of the ensemble to the cavity is found to be approximate to 1 MHz per electron, indicating the feasibility of achieving single electron strong coupling. C1 [Yang, Ge; Koolstra, G.; Schuster, D. I.] Univ Chicago, James Franck Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Yang, Ge; Koolstra, G.; Schuster, D. I.] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. [Fragner, A.; Schoelkopf, R. J.] Yale Univ, Dept Phys & Appl Phys, New Haven, CT 06520 USA. [Ocola, L.; Czaplewski, D. A.] Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Schuster, DI (reprint author), Univ Chicago, James Franck Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA.; Schuster, DI (reprint author), Univ Chicago, Dept Phys, Chicago, IL 60637 USA. EM David.Schuster@uchicago.edu FU NSF CAREER Grant [DMR 1151839]; University of Chicago MRSEC program of the NSF [DMR 1420709]; David and Lucile Packard Foundation; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The authors thank Mark Dykman, Steve Lyon, and David G. Rees for many helpful discussions, and the HOOMD molecular dynamics simulation package [37-39]. The authors thank C. Suzanne Miller and Ralu Divan for support with device fabrication. This work was supported by NSF CAREER Grant No. DMR 1151839, the University of Chicago MRSEC program of the NSF under Award No. DMR 1420709, and the David and Lucile Packard Foundation. Use of the Center for Nanoscale Materials, an Office of Science user facility, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 37 TC 2 Z9 2 U1 14 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD MAR 21 PY 2016 VL 6 IS 1 AR 011031 DI 10.1103/PhysRevX.6.011031 PG 7 WC Physics, Multidisciplinary SC Physics GA DH3ZU UT WOS:000372726100001 ER PT J AU Lewin, GR Johnson, AL Soto, RDM Perry, K Book, AJ Horn, HA Pinto-Tomas, AA Currie, CR AF Lewin, Gina R. Johnson, Amanda L. Moreira Soto, Rolando D. Perry, Kailene Book, Adam J. Horn, Heidi A. Pinto-Tomas, Adrian A. Currie, Cameron R. TI Cellulose-Enriched Microbial Communities from Leaf-Cutter Ant (Atta colombica) Refuse Dumps Vary in Taxonomic Composition and Degradation Ability SO PLOS ONE LA English DT Article ID THERMOPHILIC BACTERIAL CONSORTIA; SP-NOV.; CUTTING ANT; CD-HIT; SPOROCYTOPHAGA-MYXOCOCCOIDES; FUNGUS GARDENS; DIVERSITY; SOIL; DISCOVERY; SEQUENCES AB Deconstruction of the cellulose in plant cell walls is critical for carbon flow through ecosystems and for the production of sustainable cellulosic biofuels. Our understanding of cellulose deconstruction is largely limited to the study of microbes in isolation, but in nature, this process is driven by microbes within complex communities. In Neotropical forests, microbes in leaf-cutter ant refuse dumps are important for carbon turnover. These dumps consist of decaying plant material and a diverse bacterial community, as shown here by electron microscopy. To study the portion of the community capable of cellulose degradation, we performed enrichments on cellulose using material from five Atta colombica refuse dumps. The ability of enriched communities to degrade cellulose varied significantly across refuse dumps. 16S rRNA gene amplicon sequencing of enriched samples identified that the community structure correlated with refuse dump and with degradation ability. Overall, samples were dominated by Bacteroidetes, Gammaproteobacteria, and Betaproteobacteria. Half of abundant operational taxonomic units (OTUs) across samples were classified within genera containing known cellulose degraders, including Acidovorax, the most abundant OTU detected across samples, which was positively correlated with cellulolytic ability. A representative Acidovorax strain was isolated, but did not grow on cellulose alone. Phenotypic and compositional analyses of enrichment cultures, such as those presented here, help link community composition with cellulolytic ability and provide insight into the complexity of community-based cellulose degradation. C1 [Lewin, Gina R.; Johnson, Amanda L.; Perry, Kailene; Book, Adam J.; Currie, Cameron R.] Univ Wisconsin, Dept Energy, Great Lakes Bioenergy Res Ctr, Madison, WI USA. [Lewin, Gina R.; Johnson, Amanda L.; Perry, Kailene; Book, Adam J.; Horn, Heidi A.; Currie, Cameron R.] Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. [Moreira Soto, Rolando D.; Pinto-Tomas, Adrian A.] Univ Costa Rica, Ctr Invest Estruct Microscop, San Jose, Costa Rica. [Moreira Soto, Rolando D.] Univ Costa Rica, Ctr Invest Enfermedades Trop, San Jose, Costa Rica. [Pinto-Tomas, Adrian A.] Univ Costa Rica, Fac Med, Dept Bioquim, San Jose, Costa Rica. [Pinto-Tomas, Adrian A.] Univ Costa Rica, Ctr Invest Biol Celular & Mol, San Jose, Costa Rica. RP Currie, CR (reprint author), Univ Wisconsin, Dept Energy, Great Lakes Bioenergy Res Ctr, Madison, WI USA.; Currie, CR (reprint author), Univ Wisconsin, Dept Bacteriol, Madison, WI 53706 USA. EM currie@bact.wisc.edu FU Great Lakes Bioenergy Research Center [Department of Energy, Office of Science, Biological and Environmental Research] [DE-FC02-07ER64494]; National Science Foundation [DGE-1256259, DEB-0747002, MCB-0702025]; National Institutes of Health [National Research Service Award] [T32 GM07215]; UW-Madison's Hilldale Undergraduate/Faculty Research Fellowship; University of Costa Rica; Costa Rican Ministry of Science and Technology FX This work was supported by the Great Lakes Bioenergy Research Center [Department of Energy, Office of Science, Biological and Environmental Research DE-FC02-07ER64494, http://science.energy.gov/ber/]; the National Science Foundation [DGE-1256259 to GRL, DEB-0747002, and MCB-0702025, http://www.nsf.gov/]; the National Institutes of Health [National Research Service Award T32 GM07215, http://www.nih.gov/]; the UW-Madison's Hilldale Undergraduate/Faculty Research Fellowship to ALJ and CRC [http://awards.advising.wisc.edu/hilldale-undergraduatefaculty-research- fellowship/]; and support from the University of Costa Rica [http://www.ucr.ac.cr/] and the Costa Rican Ministry of Science and Technology [https://www.micit.go.cr/] to RDMS and AAPT. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 73 TC 0 Z9 0 U1 6 U2 9 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 21 PY 2016 VL 11 IS 3 AR e0151840 DI 10.1371/journal.pone.0151840 PG 22 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH3NW UT WOS:000372694700071 PM 26999749 ER PT J AU Lee, YL Xu, SZ Morgan, D AF Lee, Yueh-Lin Xu, Shenzhen Morgan, Dane TI Ab initio and empirical defect modeling of LaMnO3 +/-delta for solid oxide fuel cell cathodes (vol 14, pg 290, 2012) SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Correction C1 [Lee, Yueh-Lin; Xu, Shenzhen; Morgan, Dane] Univ Wisconsin, Mat Sci Program, 1509 Univ Ave, Madison, WI 53706 USA. [Morgan, Dane] Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. [Lee, Yueh-Lin] Natl Energy Technol Lab, 626 Cochrans Mill Rd,POB 10940, Pittsburgh, PA 15236 USA. RP Morgan, D (reprint author), Univ Wisconsin, Mat Sci Program, 1509 Univ Ave, Madison, WI 53706 USA.; Morgan, D (reprint author), Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. EM ddmorgan@wisc.edu RI LEE, YUEH-LIN/F-6274-2011 OI LEE, YUEH-LIN/0000-0003-2477-6412 NR 1 TC 0 Z9 0 U1 2 U2 10 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAR 21 PY 2016 VL 18 IS 11 BP 8242 EP 8242 DI 10.1039/c6cp90049f PG 1 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG6XP UT WOS:000372229700072 PM 26908310 ER PT J AU Telling, MTF Campbell, SI Engberg, D Marero, DMY Andersen, KH AF Telling, Mark T. F. Campbell, Stuart I. Engberg, Dennis Martin y Marero, David Andersen, Ken H. TI Spectroscopic characteristics of the OSIRIS near-backscattering crystal analyser spectrometer on the ISIS pulsed neutron source (vol 7, pg 1255, 2005) SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Correction C1 [Telling, Mark T. F.; Campbell, Stuart I.; Engberg, Dennis] Rutherford Appleton Lab, ISIS Facil, Chilton OX11 0QX, Oxon, England. [Martin y Marero, David] Univ Autonoma Madrid, Fac Ciencias, Dept Fis Aplicada, E-28049 Madrid, Spain. [Martin y Marero, David] Fdn Parque Cient Madrid, Campus Cantoblanco, Madrid 28049, Spain. [Martin y Marero, David] Univ Autonoma Madrid, Ctr Microanal Mat, E-28049 Madrid, Spain. [Martin y Marero, David] Univ Autonoma Madrid, Inst Nicolas Cabrera, E-28049 Madrid, Spain. [Andersen, Ken H.] Inst Laue Langevin, Grenoble, France. [Campbell, Stuart I.] Oak Ridge Natl Lab, Neutron Data Anal & Visualizat Div, Oak Ridge, TN USA. [Andersen, Ken H.] European Spallat Source ERIC, POB 176, S-22100 Lund, Sweden. RP Telling, MTF (reprint author), Rutherford Appleton Lab, ISIS Facil, Chilton OX11 0QX, Oxon, England. EM mark.telling@stfc.ac.uk RI Martin y Marero, David/B-3094-2008; Campbell, Stuart/A-8485-2010; Telling, Mark/F-3294-2014 OI Martin y Marero, David/0000-0002-8969-0735; Campbell, Stuart/0000-0001-7079-0878; NR 1 TC 2 Z9 2 U1 1 U2 6 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAR 21 PY 2016 VL 18 IS 11 BP 8243 EP 8243 DI 10.1039/c6cp90057g PG 1 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG6XP UT WOS:000372229700073 PM 26905035 ER PT J AU Bonicalzi, RM Aalseth, CE Day, AR Hoppe, EW Mace, EK Moran, JJ Overman, CT Panisko, ME Seifert, A AF Bonicalzi, R. M. Aalseth, C. E. Day, A. R. Hoppe, E. W. Mace, E. K. Moran, J. J. Overman, C. T. Panisko, M. E. Seifert, A. TI Optimization of simultaneous tritium-radiocarbon internal gas proportional counting SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Tritium; Radiocarbon; Optimization; Proportional counter; Environmental methane ID MASS-SPECTROMETRY; ENERGY-LEVELS AB Specific environmental applications can benefit from dual tritium and radiocarbon measurements in a single compound. Assuming typical environmental levels, it is often the low tritium activity relative to the higher radiocarbon activity that limits the dual measurement. In this paper, we explore the parameter space for a combined tritium and radiocarbon measurement using a natural methane sample mixed with an argon fill gas in low-background proportional counters of a specific design. We present an optimized methane percentage, detector fill pressure, and analysis energy windows to maximize measurement sensitivity while minimizing count time. The final optimized method uses a 9-atm fill of P35 (35% methane, 65% argon), and a tritium analysis window from 1.5 to 10.3 keV, which stops short of the tritium beta decay endpoint energy of 18.6 keV. This method optimizes tritium-counting efficiency while minimizing radiocarbon beta-decay interference. (C) 2016 Elsevier B.V. All rights reserved. C1 [Bonicalzi, R. M.] Seattle Cent Coll, 1701 Broadway, Seattle, WA 98122 USA. [Aalseth, C. E.; Day, A. R.; Hoppe, E. W.; Mace, E. K.; Moran, J. J.; Overman, C. T.; Panisko, M. E.; Seifert, A.] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. RP Mace, EK (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM Emily.Mace@pnl.gov OI Moran, James/0000-0001-9081-9017; Day, Anthony/0000-0002-1217-1822 NR 26 TC 1 Z9 1 U1 0 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAR 21 PY 2016 VL 813 BP 19 EP 28 DI 10.1016/j.nima.2015.12.062 PG 10 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DC6ZV UT WOS:000369369000004 ER PT J AU Favorite, JA AF Favorite, Jeffrey A. TI The solid angle (geometry factor) for a spherical surface source and an arbitrary detector aperture SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Solid angle; Geometry factor; Geometrical efficiency; Spherical surface source; Arbitrary detector aperture AB It is proved that the solid angle (or geometry factor, also called the geometrical efficiency) for a spherically symmetric outward-directed surface source with an arbitrary radius and polar angle distribution and an arbitrary detector aperture is equal to the solid angle for an isotropic point source located at the center of the spherical surface source and the same detector aperture. (C) 2016 The Authors. Published by Elsevier B.V. C1 [Favorite, Jeffrey A.] Los Alamos Natl Lab, Computat Phys X CP Div, MS F663, Los Alamos, NM 87545 USA. RP Favorite, JA (reprint author), Los Alamos Natl Lab, Computat Phys X CP Div, MS F663, Los Alamos, NM 87545 USA. EM fave@lanl.gov NR 15 TC 0 Z9 0 U1 2 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD MAR 21 PY 2016 VL 813 BP 29 EP 35 DI 10.1016/j.nima.2015.12.060 PG 7 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DC6ZV UT WOS:000369369000005 ER PT J AU Balbinot, E Yanny, B Li, TS Santiago, B Marshall, JL Finley, DA Pieres, A Abbott, TMC Abdalla, FB Allam, S Benoit-Levy, A Bernstein, GM Bertin, E Brooks, D Burke, DL Rosell, AC Kind, MC Carretero, J Cunha, CE Da Costa, LN DePoy, DL Desai, S Diehl, HT Doel, P Estrada, J Flaugher, B Frieman, J Gerdes, DW Gruen, D Gruendl, RA Honscheid, K James, DJ Kuehn, K Kuropatkin, N Lahav, O March, M Martini, P Miquel, R Nichol, RC Ogando, R Romer, AK Sanchez, E Schubnell, M Sevilla-Noarbe, I Smith, RC Soares-Santos, M Sobreira, F Suchyta, E Tarle, G Thomas, D Tucker, D Walker, AR AF Balbinot, E. Yanny, B. Li, T. S. Santiago, B. Marshall, J. L. Finley, D. A. Pieres, A. Abbott, T. M. C. Abdalla, F. B. Allam, S. Benoit-Levy, A. Bernstein, G. M. Bertin, E. Brooks, D. Burke, D. L. Rosell, A. Carnero Kind, M. Carrasco Carretero, J. Cunha, C. E. Da Costa, L. N. DePoy, D. L. Desai, S. Diehl, H. T. Doel, P. Estrada, J. Flaugher, B. Frieman, J. Gerdes, D. W. Gruen, D. Gruendl, R. A. Honscheid, K. James, D. J. Kuehn, K. Kuropatkin, N. Lahav, O. March, M. Martini, P. Miquel, R. Nichol, R. C. Ogando, R. Romer, A. K. Sanchez, E. Schubnell, M. Sevilla-Noarbe, I. Smith, R. C. Soares-Santos, M. Sobreira, F. Suchyta, E. Tarle, G. Thomas, D. Tucker, D. Walker, A. R. CA DES Collaboration TI THE PHOENIX STREAM: A COLD STREAM IN THE SOUTHERN HEMISPHERE SO ASTROPHYSICAL JOURNAL LA English DT Article DE Galaxy: halo; Galaxy: structure ID DARK ENERGY SURVEY; GLOBULAR-CLUSTER PALOMAR-5; SAGITTARIUS DWARF GALAXY; MILKY-WAY COMPANIONS; SKY SURVEY VIEW; STELLAR HALO; TIDAL STREAMS; DATA RELEASE; MATTER HALO; FAINT AB We report the discovery of a stellar stream in the Dark Energy Survey Year 1 (Y1A1) data. The discovery was made through simple color-magnitude filters and visual inspection of the Y1A1 data. We refer to this new object as the Phoenix stream, after its resident constellation. After subtraction of the background stellar population we detect a clear signal of a simple stellar population. By fitting the ridge line of the stream in color-magnitude space, we find that a stellar population with age tau = 11.5 +/- 0.5 Gyr and [Fe/H] < -1.6, located 17.5 +/- 0.9 kpc from the Sun, gives an adequate description of the stream stellar population. The stream is detected over an extension of 8 degrees.1 (2.5 kpc) and has a width of similar to 54 pc assuming a Gaussian profile, indicating that a globular cluster (GC) is a probable progenitor. There is no known GC within 5 kpc that is compatible with being the progenitor of the stream, assuming that the stream traces its orbit. We examined overdensities (ODs) along the stream, however, no obvious counterpart-bound stellar system is visible in the coadded images. We also find ODs along the stream that appear to be symmetrically distributed-consistent with the epicyclic OD scenario for the formation of cold streams-as well as a misalignment between the northern and southern part of stream. Despite the close proximity we find no evidence that this stream and the halo cluster NGC 1261 have a common accretion origin linked to the recently found EriPhe OD. C1 [Balbinot, E.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Yanny, B.; Finley, D. A.; Allam, S.; Benoit-Levy, A.; Diehl, H. T.; Estrada, J.; Flaugher, B.; Frieman, J.; Kuropatkin, N.; Soares-Santos, M.; Sobreira, F.; Tucker, D.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Li, T. S.; Marshall, J. L.; DePoy, D. L.] Texas A&M Univ, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [Li, T. S.; Marshall, J. L.; DePoy, D. L.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Santiago, B.; Pieres, A.] Univ Fed Rio Grande do Sul, Inst Fis, Caixa Postal 15051, BR-91501970 Porto Alegre, RS, Brazil. [Santiago, B.; Pieres, A.; Rosell, A. Carnero; Da Costa, L. N.; Ogando, R.; Sobreira, F.] Lab Interinst E Astron LIneA, Rua Gal Jose Cristino 77, BR-20921400 Rio De Janeiro, RJ, Brazil. [Abbott, T. M. C.; James, D. J.; Smith, R. C.; Walker, A. R.] Natl Opt Astron Observ, Cerro Tololo Inter Amer Observ, Casilla 603, La Serena, Chile. [Abdalla, F. B.; Benoit-Levy, A.; Brooks, D.; Doel, P.; Lahav, O.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Bertin, E.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Bertin, E.] CNRS, Inst Astrophys Paris, UMR 7095, F-75014 Paris, France. [Bertin, E.] Univ Paris 06, Sorbonne Univ, Inst Astrophys Paris, UMR 7095, F-75014 Paris, France. [Burke, D. L.; Cunha, C. E.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, POB 2450, Stanford, CA 94305 USA. [Burke, D. L.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Rosell, A. Carnero; Da Costa, L. N.; Ogando, R.] Observ Nacl, Rua Gal Jose Cristino 77, BR-20921400 Rio De Janeiro, RJ, Brazil. [Kind, M. Carrasco; Gruendl, R. A.; Sevilla-Noarbe, I.] Univ Illinois, Dept Astron, 1002 W Green St, Urbana, IL 61801 USA. [Kind, M. Carrasco; Gruendl, R. A.] Natl Ctr Supercomp Applicat, 1205 West Clark St, Urbana, IL 61801 USA. [Carretero, J.; Miquel, R.] IEEC CSIC, Inst Ciencies Espai, Campus UAB,Carrer Can Magrans S-N, E-08193 Barcelona, Spain. [Carretero, J.; Miquel, R.] Univ Autonoma Barcelona, Inst Fis Altes Energies, Carrer Can Magrans S-N, E-08193 Barcelona, Spain. [Desai, S.] Excellence Cluster Universe, Boltzmannstr 2, D-85748 Garching, Germany. [Desai, S.] Univ Munich, Fac Phys, Scheinerstr 1, D-81679 Munich, Germany. [Frieman, J.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 21 USA. [Gerdes, D. W.; Schubnell, M.; Tarle, G.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Gruen, D.] Max Planck Inst Extraterr Phys, Giessenbachstr, D-85748 Garching, Germany. [Gruen, D.] Univ Munich, Univ Sternwarte, Fak Phys, Scheinerstr 1, D-81679 Munich, Germany. [Honscheid, K.; Martini, P.; Suchyta, E.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Honscheid, K.; Suchyta, E.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Kuehn, K.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Martini, P.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Miquel, R.] Inst Catalana Recerca & Estudis Avancats, E-08010 Barcelona, Spain. [Nichol, R. C.; Thomas, D.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [Romer, A. K.] Univ Sussex, Dept Phys & Astron, Pevensey Bldg, Brighton BN1 9QH, E Sussex, England. [Sanchez, E.; Sevilla-Noarbe, I.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. RP Balbinot, E (reprint author), Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. EM e.balbinot@surrey.ac.uk RI Ogando, Ricardo/A-1747-2010; Sobreira, Flavia/F-4168-2015; Balbinot, Eduardo/E-8019-2015; OI Ogando, Ricardo/0000-0003-2120-1154; Sobreira, Flavia/0000-0002-7822-0658; Tucker, Douglas/0000-0001-7211-5729; Balbinot, Eduardo/0000-0002-1322-3153; Abdalla, Filipe/0000-0003-2063-4345 FU U.S. Department of Energy; U.S. National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Center for Cosmology and Astro-Particle Physics at the Ohio State University; Mitchell Institute for Fundamental Physics and Astronomy at Texas AM University; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia, Tecnologia e Inovacao; Deutsche Forschungsgemeinschaft; Argonne National Laboratory; University of California at Santa Cruz; University of Cambridge; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid; University of Chicago; University College London; DES-Brazil Consortium; University of Edinburgh; Eidgenossische Technische Hochschule (ETH) Zurich; Fermi National Accelerator Laboratory; University of Illinois at Urbana-Champaign; Institut de Ciencies de l'Espai (IEEC/CSIC); Institut de Fisica d'Altes Energies; Lawrence Berkeley National Laboratory; Ludwig-Maximilians Universitat Munchen; University of Michigan; National Optical Astronomy Observatory; University of Nottingham; Ohio State University; University of Pennsylvania; University of Portsmouth; SLAC National Accelerator Laboratory, Stanford University; University of Sussex; Texas AM University; National Science Foundation [AST-1138766]; MINECO [AYA2012-39559, ESP2013-48274, FPA2013-47986]; Centro de Excelencia Severo Ochoa [SEV-2012-0234]; ERDF funds from the European Union; European Research Council under the European Union's Seventh Framework Programme (FP7), ERC grant [240672, 291329, 306478]; European Research Council [ERC-StG-335936] FX Funding for the DES Projects has been provided by the U.S. Department of Energy, the U.S. National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, the Center for Cosmology and Astro-Particle Physics at the Ohio State University, the Mitchell Institute for Fundamental Physics and Astronomy at Texas A&M University, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia, Tecnologia e Inovacao, the Deutsche Forschungsgemeinschaft, and the Collaborating Institutions in the Dark Energy Survey.r The Collaborating Institutions are Argonne National Laboratory, the University of California at Santa Cruz, the University of Cambridge, Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid, the University of Chicago, University College London, the DES-Brazil Consortium, the University of Edinburgh, the Eidgenossische Technische Hochschule (ETH) Zurich, Fermi National Accelerator Laboratory, the University of Illinois at Urbana-Champaign, the Institut de Ciencies de l'Espai (IEEC/CSIC), the Institut de Fisica d'Altes Energies, Lawrence Berkeley National Laboratory, the Ludwig-Maximilians Universitat Munchen and the associated Excellence Cluster universe, the University of Michigan, the National Optical Astronomy Observatory, the University of Nottingham, The Ohio State University, the University of Pennsylvania, the University of Portsmouth, SLAC National Accelerator Laboratory, Stanford University, the University of Sussex, and Texas A&M University.r The DES data management system is supported by the National Science Foundation under grant No. AST-1138766. The DES participants from Spanish institutions are partially supported by MINECO under grants AYA2012-39559, ESP2013-48274, FPA2013-47986, and Centro de Excelencia Severo Ochoa SEV-2012-0234, some of which include ERDF funds from the European Union. Research leading to these results has received funding from the European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013), including ERC grant agreements 240672, 291329, and 306478.r E. Balbinot acknowledges financial support from the European Research Council (ERC-StG-335936, CLUSTERS). NR 49 TC 5 Z9 5 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 20 PY 2016 VL 820 IS 1 AR 58 DI 10.3847/0004-637X/820/1/58 PG 8 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DH4WT UT WOS:000372787000057 ER PT J AU de la Rosa, J Roming, P Pritchard, T Fryer, C AF de la Rosa, Janie Roming, Pete Pritchard, Tyler Fryer, Chris TI CHARACTERIZING MID-ULTRAVIOLET TO OPTICAL LIGHT CURVES OF NEARBY TYPE IIn SUPERNOVAE SO ASTROPHYSICAL JOURNAL LA English DT Article DE supernovae: general; ultraviolet: general ID SPECTRAL EVOLUTION; SN 2010JL; TELESCOPE; CORE; PROGENITOR; FRACTIONS; ERUPTIONS; 2011HT; RATES; RISE AB We present early mid-ultraviolet and optical observations of Type IIn supernovae (SNe IIn) observed from 2007 to 2013. Our results focus on the properties of UV light curves: peak absolute magnitudes, temporal decay, and color evolution. During early times, this sample demonstrates that UV light decays faster than optical, and each event transitions from a predominantly UV-bright phase to an optically bright phase. In order to understand early UV behavior, we generate and analyze the sample's blackbody luminosity, temperature, and radius as the SN ejecta expand and cool. Since most of our observations were detected post maximum luminosity, we introduce a method for estimating the date of peak magnitude. When our observations are compared based on filter, we find that even though these SNe IIn vary in peak magnitudes, there are similarities in UV decay rates. We use a simple semi-analytical SN model in order to understand the effects of the explosion environment on our UV observations. Understanding the UV characteristics of nearby SNe IIn during an early phase can provide valuable information about the environment surrounding these explosions, leading us to evaluating the diversity of observational properties in this subclass. C1 [de la Rosa, Janie; Roming, Pete] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. [Roming, Pete] SW Res Inst, San Antonio, TX 78228 USA. [Pritchard, Tyler] Swinburne Univ Technol, Ctr Astrophys & Supercomp, POB 218, Hawthorn, Vic 3122, Australia. [Fryer, Chris] Los Alamos Natl Lab, CCS 2, Los Alamos, NM 87545 USA. [Fryer, Chris] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Fryer, Chris] Univ Arizona, Steward Observ, Tucson, AZ 85721 USA. RP de la Rosa, J (reprint author), Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. NR 54 TC 1 Z9 1 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 20 PY 2016 VL 820 IS 1 AR 74 DI 10.3847/0004-637X/820/1/74 PG 21 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DH4WT UT WOS:000372787000073 ER PT J AU Ganot, N Gal-Yam, A Ofek, EO Sagiv, I Waxman, E Lapid, O Kulkarni, SR Ben-Ami, S Kasliwal, MM Chelouche, D Rafter, S Behar, E Laor, A Poznanski, D Nakar, E Maoz, D Trakhtenbrot, B Neill, JD Barlow, TA Martin, CD Gezari, S Arcavi, I Bloom, JS Nugent, PE Sullivan, M AF Ganot, Noam Gal-Yam, Avishay Ofek, Eran. O. Sagiv, Ilan Waxman, Eli Lapid, Ofer Kulkarni, Shrinivas R. Ben-Ami, Sagi Kasliwal, Mansi M. Chelouche, Doron Rafter, Stephen Behar, Ehud Laor, Ari Poznanski, Dovi Nakar, Ehud Maoz, Dan Trakhtenbrot, Benny Neill, James D. Barlow, Thomas A. Martin, Christofer D. Gezari, Suvi Arcavi, Iair Bloom, Joshua S. Nugent, Peter E. Sullivan, Mark CA ULTRASAT Sci Team WTTH Consortium GALEX Sci Team Palomar Transient Factory TI THE DETECTION RATE OF EARLY UV EMISSION FROM SUPERNOVAE: A DEDICATED GALEX/PTF SURVEY AND CALIBRATED THEORETICAL ESTIMATES SO ASTROPHYSICAL JOURNAL LA English DT Article DE supernovae: general ID CORE-COLLAPSE SUPERNOVAE; GAMMA-RAY BURSTS; II-P SUPERNOVAE; DENSE MASS-LOSS; SHOCK-BREAKOUT; LIGHT-CURVES; LUMINOUS SUPERNOVAE; FOLLOW-UP; STELLAR ENVELOPES; RED SUPERGIANT AB The radius and surface composition of an exploding massive star, as well as the explosion energy per unit mass, can be measured using early UV observations of core-collapse supernovae (SNe). We present the first results from a simultaneous GALEX/PTF search for early ultraviolet (UV) emission from SNe. Six SNe II and one Type II superluminous SN (SLSN-II) are clearly detected in the GALEX near-UV (NUV) data. We compare our detection rate with theoretical estimates based on early, shock-cooling UV light curves calculated from models that fit existing Swift and GALEX observations well, combined with volumetric SN rates. We find that our observations are in good agreement with calculated rates assuming that red supergiants (RSGs) explode with fiducial radii of 500 R-circle dot, explosion energies of 10(51) erg, and ejecta masses of 10M(circle dot). Exploding blue supergiants and Wolf-Rayet stars are poorly constrained. We describe how such observations can be used to derive the progenitor radius, surface composition, and explosion energy per unit mass of such SN events, and we demonstrate why UV observations are critical for such measurements. We use the fiducial RSG parameters to estimate the detection rate of SNe during the shock-cooling phase (<1 day after explosion) for several ground-based surveys (PTF, ZTF, and LSST). We show that the proposed wide-field UV explorer ULTRASAT mission is expected to find >85 SNe per year (similar to 0.5 SN per deg(2)), independent of host galaxy extinction, down to an NUV detection limit of 21.5 mag AB. Our pilot GALEX/PTF project thus convincingly demonstrates that a dedicated, systematic SN survey at the NUV band is a compelling method to study how massive stars end their life. C1 [Ganot, Noam; Gal-Yam, Avishay; Ofek, Eran. O.; Sagiv, Ilan; Waxman, Eli; Lapid, Ofer] Weizmann Inst Sci, Fac Phys, Dept Particle Phys & Astrophys, IL-76100 Rehovot, Israel. [Kulkarni, Shrinivas R.; Kasliwal, Mansi M.] CALTECH, Cahill Ctr Astrophys, Pasadena, CA 91125 USA. [Ben-Ami, Sagi] Harvard Smithsonian Ctr Astrophys, Smithsonian Astrophys Observ, 60 Garden St, Cambridge, MA 02138 USA. [Chelouche, Doron; Rafter, Stephen] Univ Haifa, Dept Phys, Fac Nat Sci, IL-31905 Haifa, Israel. [Behar, Ehud; Laor, Ari] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Poznanski, Dovi; Nakar, Ehud; Maoz, Dan] Tel Aviv Univ, Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Trakhtenbrot, Benny] ETH, Inst Astron, Wolfgang Pauli Str 27, CH-8093 Zurich, Switzerland. [Neill, James D.; Barlow, Thomas A.; Martin, Christofer D.] CALTECH, 1200 East Calif Blvd,MC 278-17, Pasadena, CA 91125 USA. [Gezari, Suvi] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Arcavi, Iair] Las Cumbres Observ Global Telescope, 6740 Cortona Dr,Suite 102, Goleta, CA 93111 USA. [Bloom, Joshua S.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Nugent, Peter E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Sullivan, Mark] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Arcavi, Iair] Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USA. RP Ganot, N (reprint author), Weizmann Inst Sci, Fac Phys, Dept Particle Phys & Astrophys, IL-76100 Rehovot, Israel. EM noam.ganot@gmail.com OI Sullivan, Mark/0000-0001-9053-4820; Trakhtenbrot, Benny/0000-0002-3683-7297 FU Israeli Space Agency (ISA); Ministry of Science, Technology and Space (MOS); EU via ERC grant [307260]; ISF; Kimmel award FX This research was supported by grants from the Israeli Space Agency (ISA) and the Ministry of Science, Technology and Space (MOS). Additional funding was provided by the EU via ERC grant 307260, the ISF, and a Kimmel award. NR 69 TC 1 Z9 1 U1 2 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 20 PY 2016 VL 820 IS 1 AR 57 DI 10.3847/0004-637X/820/1/57 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DH4WT UT WOS:000372787000056 ER PT J AU Garnavich, PM Tucker, BE Rest, A Shaya, EJ Olling, RP Kasen, D Villar, A AF Garnavich, P. M. Tucker, B. E. Rest, A. Shaya, E. J. Olling, R. P. Kasen, D. Villar, A. TI SHOCK BREAKOUT AND EARLY LIGHT CURVES OF TYPE II-P SUPERNOVAE OBSERVED WITH KEPLER SO ASTROPHYSICAL JOURNAL LA English DT Article DE shock waves; stars: mass-loss; supernovae: general; supernovae: individual (KSN2011a, KSN2011d, SN1999ig) ID CORE-COLLAPSE SUPERNOVAE; RED SUPERGIANTS; PROGENITOR; EMISSION; WIND AB We discovered two transient events in the Kepler field with light curves that strongly suggest they are type. II-P supernovae (SNe II-P). Using the fast cadence of the Kepler observations we precisely estimate the rise time to maximum for KSN2011a and KSN2011d as 10.5 +/- 0.4 and 13.3 +/- 0.4 rest-frame days, respectively. Based on fits to idealized analytic models, we find the progenitor radius of KSN2011a (280 +/- 20 R-circle dot) to be significantly smaller than that for KSN2011d (490 +/- 20 R-circle dot), but both have similar explosion energies of 2.0 +/- 0.3 x 10(51) erg. The rising light curve of KSN2011d is an excellent match to that predicted by simple models of exploding red supergiants (RSG). However, the early rise of KSN2011a is faster than the models predict, possibly due to the supernova shock wave moving into pre-existing wind or mass-loss from the RSG. A mass-loss rate of 10(-4)M(circle dot) yr(-1) from the RSG can explain the fast rise without impacting the optical flux at maximum light or the shape of the post-maximum light curve. No shock breakout emission is seen in KSN2011a, but this is likely due to the circumstellar interaction suspected in the fast rising light curve. The early light curve of KSN2011d does show excess emission consistent with model predictions of a shock breakout. This is the first optical detection of a shock breakout from a SNe II-P. C1 [Garnavich, P. M.] Univ Notre Dame, Dept Phys, 225 Nieuwland Sci Hall, Notre Dame, IN 46556 USA. [Tucker, B. E.] Australian Natl Univ, Mt Stromlo Observ, Res Sch Astron & Astrophys, Via Cotter Rd, Weston, ACT 2611, Australia. [Tucker, B. E.; Kasen, D.] Univ Calif Berkeley, Dept Phys & Astron, Berkeley, CA 94720 USA. [Rest, A.] Space Telescope Sci Inst, 3700 San Martin Dr, Baltimore, MD 21218 USA. [Shaya, E. J.; Olling, R. P.] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Kasen, D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Villar, A.] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. RP Garnavich, PM (reprint author), Univ Notre Dame, Dept Phys, 225 Nieuwland Sci Hall, Notre Dame, IN 46556 USA. FU Kepler grants [NNX12AC89G, NNX11AG95G]; DOE office of nuclear physics early career award FX This research has made use of the NASA/IPAC Extragalactic Database (NED), which is operated by the Jet Propulsion Laboratory, California Institute of Technology, under contract with the National Aeronautics and Space Administration. This research has made use of the NASA/IPAC Infrared Science Archive, which is operated by the Jet Propulsion Laboratory, California Institute of Technology, under contract with the National Aeronautics and Space Administration. This work was partly supported by Kepler grants NNX12AC89G and NNX11AG95G. D.K. is supported by a DOE office of nuclear physics early career award. NR 26 TC 9 Z9 9 U1 3 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 20 PY 2016 VL 820 IS 1 AR 23 DI 10.3847/0004-637X/820/1/23 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DH4WT UT WOS:000372787000023 ER PT J AU LaMassa, SM Ricarte, A Glikman, E Urry, CM Stern, D Yaqoob, T Lansbury, GB Civano, F Boggs, SE Brandt, WN Chen, CTJ Christensen, FE Craig, WW Hailey, CJ Harrison, F Hickox, RC Koss, M Ricci, C Treister, E Zhang, W AF LaMassa, Stephanie M. Ricarte, Angelo Glikman, Eilat Urry, C. Megan Stern, Daniel Yaqoob, Tahir Lansbury, George B. Civano, Francesca Boggs, Steve E. Brandt, W. N. Chen, Chien-Ting J. Christensen, Finn E. Craig, William W. Hailey, Chuck J. Harrison, Fiona Hickox, Ryan C. Koss, Michael Ricci, Claudio Treister, Ezequiel Zhang, Will TI PEERING THROUGH THE DUST: NuSTAR OBSERVATIONS OF TWO FIRST-2MASS RED QUASARS SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: active; infrared: galaxies; quasars: individual (F2M 0380+3759, F2M 1227+3214); X-rays: individual (F2M 0830+3759, F2M 1227+3214) ID ACTIVE GALACTIC NUCLEI; SUPERMASSIVE BLACK-HOLES; XMM-NEWTON OBSERVATIONS; DIGITAL SKY SURVEY; RAY SPECTRAL MODEL; WIDE-FIELD SURVEY; X-RAY; REDDENED QUASARS; COSMOS FIELD; SEYFERT-GALAXIES AB Some reddened quasars appear to be transitional objects in the paradigm of merger-induced black hole growth/galaxy evolution, where a heavily obscured nucleus starts to be unveiled by powerful quasar winds evacuating the surrounding cocoon of dust and gas. Hard X-ray observations are able to peer through this gas and dust, revealing the properties of circumnuclear obscuration. Here, we present NuSTAR and XMM-Newton/Chandra observations of FIRST-2MASS-selected red quasars F2M 0830+3759 and F2M 1227+3214. We find that though F2M 0830 +3759 is moderately obscured (N-H,(Z) = (2.1 +/- 0.2) x 10(22) cm(-2)) and F2M 1227+3214 is mildly absorbed (N-H,(Z) = 3.4(- 0.7)(+0.8) x 10(21) cm(-2)) along the line of sight, heavier global obscuration may be present in both sources, with N-H,(S) = 3.7(- 2.6)(+4.1) x 10(23) cm(-2) and <5.5 x 10(23) cm(-2) for F2M 0830+3759 and F2M 1227+3214, respectively. F2M 0830+3759 also has an excess of soft X-ray emission below 1 keV, which is well accommodated by a model where 7% of the intrinsic X-ray emission from the active galactic nucleus (AGN) is scattered into the line of sight. While F2M 1227+3214 has a dust-to-gas ratio (E(B - V)/N-H) consistent with the Galactic value, the value of E(B - V)/N-H for F2M 0830+3759 is lower than the Galactic standard, consistent with the paradigm that the dust resides on galactic scales while the X-ray reprocessing gas originates within the dust sublimation zone of the broad-line region. The X-ray and 6.1 mu m luminosities of these red quasars are consistent with the empirical relations derived for high-luminosity, unobscured quasars, extending the parameter space of obscured AGNs previously observed by NuSTAR to higher luminosities. C1 [LaMassa, Stephanie M.; Urry, C. Megan; Civano, Francesca] Yale Ctr Astron & Astrophys, Dept Phys, POB 208120, New Haven, CT 06520 USA. [LaMassa, Stephanie M.; Urry, C. Megan; Civano, Francesca] Yale Univ, Dept Phys, POB 208121, New Haven, CT 06520 USA. [LaMassa, Stephanie M.; Zhang, Will] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Ricarte, Angelo] Yale Univ, Dept Astron, New Haven, CT 06511 USA. [Glikman, Eilat] Middlebury Coll, Dept Phys, Middlebury, VT 05753 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr,Mail Stop 169-221, Pasadena, CA 91109 USA. [Yaqoob, Tahir] Univ Maryland Baltimore Cty, Dept Phys, 1000 Hilltop Circle, Baltimore, MD 21250 USA. [Lansbury, George B.] Univ Durham, Dept Phys, Ctr Extragalact Astron, South Rd, Durham DH1 3LE, England. [Civano, Francesca; Hickox, Ryan C.] Dartmouth Coll, Dept Phys & Astron, 6127 Wilder Lab, Hanover, NH 03755 USA. [Civano, Francesca] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. [Boggs, Steve E.; Craig, William W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Brandt, W. N.; Chen, Chien-Ting J.] Penn State Univ, Dept Astron & Astrophys, 525 Davey Lab, University Pk, PA 16802 USA. [Brandt, W. N.; Chen, Chien-Ting J.] Penn State Univ, Inst Gravitat & Cosmos, 525 Davey Lab, University Pk, PA 16802 USA. [Brandt, W. N.] Penn State Univ, Dept Phys, 525 Davey Lab, University Pk, PA 16802 USA. [Christensen, Finn E.] Tech Univ Denmark, Natl Space Inst, DTU Space, Elektrovej 327, DK-2800 Lyngby, Denmark. [Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hailey, Chuck J.] Columbia Univ, Columbia Astrophys Lab, 538 W 120th St, New York, NY 10027 USA. [Harrison, Fiona] CALTECH, Cahill Ctr Astron & Astrophys, 1216 E Calif Blvd, Pasadena, CA 91125 USA. [Koss, Michael] ETH, Inst Astron, Dept Phys, Wolfgang Pauli Str 27, CH-8093 Zurich, Switzerland. [Ricci, Claudio] Pontificia Univ Catolica Chile, Inst Astrofis, Vicuna Mackenna 4860, Santiago 7820436, Chile. [Treister, Ezequiel] Univ Concepcion, Dept Astron, Casilla 160-C, Concepcion, Chile. RP LaMassa, SM (reprint author), Yale Ctr Astron & Astrophys, Dept Phys, POB 208120, New Haven, CT 06520 USA. RI Boggs, Steven/E-4170-2015; OI Boggs, Steven/0000-0001-9567-4224; Urry, Meg/0000-0002-0745-9792 FU NASA [NNG08FD60C]; National Aeronautics and Space Administration; Gruber Science Fellowship; Cottrell College Award through the Research Corporation for Science Advancement; Caltech NuSTAR subcontract [44A-1092750]; NASA ADP grant [NNX10AC99G]; NASA through ADAP award [NNX12AE38G]; National Science Foundation [1211096, 1515364]; Sloan Research Fellowship; Dartmouth Class of Faculty Fellowship; CONICYT-Chile grants ["EMBIGGEN" Anillo ACT1101, FONDECYT 1141218, Basal-CATA PFB-06/2007] FX We thank the referee for a careful reading of this manuscript and helpful comments. This work was supported under NASA contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). AR is supported by the Gruber Science Fellowship. EG acknowledges the generous support of the Cottrell College Award through the Research Corporation for Science Advancement. WNB acknowledges support from Caltech NuSTAR subcontract 44A-1092750 and NASA ADP grant NNX10AC99G. RCH acknowledges support from NASA through ADAP award NNX12AE38G, the National Science Foundation through grant nos. 1211096 and 1515364, a Sloan Research Fellowship, and a Dartmouth Class of 1962 Faculty Fellowship. CR acknowledges financial support from the CONICYT-Chile grants "EMBIGGEN" Anillo ACT1101, FONDECYT 1141218, Basal-CATA PFB-06/2007. NR 108 TC 3 Z9 3 U1 2 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 20 PY 2016 VL 820 IS 1 AR 70 DI 10.3847/0004-637X/820/1/70 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DH4WT UT WOS:000372787000069 ER PT J AU Rubin, A Gal-Yam, A De Cia, A Horesh, A Khazov, D Ofek, EO Kulkarni, SR Arcavi, I Manulis, I Yaron, O Vreeswijk, P Kasliwal, MM Ben-Ami, S Perley, DA Cao, Y Cenko, SB Rebbapragada, UD Wozniak, PR Filippenko, AV Clubb, KI Nugent, PE Pan, YC Badenes, C Howell, DA Valenti, S Sand, D Sollerman, J Johansson, J Leonard, DC Horst, JC Armen, SF Fedrow, JM Quimby, RM Mazzali, P Pian, E Sternberg, A Matheson, T Sullivan, M Maguire, K Lazarevic, S AF Rubin, Adam Gal-Yam, Avishay De Cia, Annalisa Horesh, Assaf Khazov, Danny Ofek, Eran O. Kulkarni, S. R. Arcavi, Iair Manulis, Ilan Yaron, Ofer Vreeswijk, Paul Kasliwal, Mansi M. Ben-Ami, Sagi Perley, Daniel A. Cao, Yi Cenko, S. Bradley Rebbapragada, Umaa D. Wozniak, P. R. Filippenko, Alexei V. Clubb, K. I. Nugent, Peter E. Pan, Y-C. Badenes, C. Howell, D. Andrew Valenti, Stefano Sand, David Sollerman, J. Johansson, Joel Leonard, Douglas C. Horst, J. Chuck Armen, Stephen F. Fedrow, Joseph M. Quimby, Robert M. Mazzali, Paulo Pian, Elena Sternberg, Assaf Matheson, Thomas Sullivan, M. Maguire, K. Lazarevic, Sanja TI TYPE II SUPERNOVA ENERGETICS AND COMPARISON OF LIGHT CURVES TO SHOCK-COOLING MODELS SO ASTROPHYSICAL JOURNAL LA English DT Article DE supernovae: general ID P SUPERNOVAE; LUMINOUS SUPERNOVAE; CORE-COLLAPSE; PHOTOSPHERIC PHASE; LOW-RESOLUTION; IA SUPERNOVAE; RISE-TIME; FOLLOW-UP; MASS-LOSS; BREAKOUT AB During the first few days after explosion, Type II supernovae (SNe) are dominated by relatively simple physics. Theoretical predictions regarding early-time SN light curves in the ultraviolet (UV) and optical bands are thus quite robust. We present, for the first time, a sample of 57 R-band SN II light curves that are well-monitored during their rise, with > 5 detections during the first 10 days after discovery, and a well-constrained time of explosion to within 1-3 days. We show that the energy per unit mass (E/M) can be deduced to roughly a factor of five by comparing early-time optical data to the 2011 model of Rabinak & Waxman, while the progenitor radius cannot be determined based on R-band data alone. We find that SN II explosion energies span a range of E/M = (0.2-20) x 10(51) erg/(10 M-circle dot), and have a mean energy per unit mass of < E/M > = 0.85 x 10(51) erg/(10 M-circle dot), corrected for Malmquist bias. Assuming a small spread in progenitor masses, this indicates a large intrinsic diversity in explosion energy. Moreover, E/M is positively correlated with the amount of Ni-56 produced in the explosion, as predicted by some recent models of core-collapse SNe. We further present several empirical correlations. The peak magnitude is correlated with the decline rate (Delta m(15)), the decline rate is weakly correlated with the rise time, and the rise time is not significantly correlated with the peak magnitude. Faster declining SNe are more luminous and have longer rise times. This limits the possible power sources for such events. C1 [Rubin, Adam; Gal-Yam, Avishay; De Cia, Annalisa; Horesh, Assaf; Khazov, Danny; Ofek, Eran O.; Manulis, Ilan; Yaron, Ofer; Vreeswijk, Paul] Weizmann Inst Sci, Dept Particle Phys & Astrophys, 234 Herzl St, Rehovot, Israel. [Kulkarni, S. R.; Perley, Daniel A.; Cao, Yi] CALTECH, Dept Astron, Pasadena, CA 91125 USA. [Kulkarni, S. R.] CALTECH, Caltech Opt Observ, Pasadena, CA 91125 USA. [Arcavi, Iair; Howell, D. Andrew; Valenti, Stefano] Las Cumbres Observ Global Telescope Network, 6740 Cortona Dr,Suite 102, Goleta, CA 93117 USA. [Arcavi, Iair] Univ Calif Santa Barbara, Kavli Inst Theoret Phys, Santa Barbara, CA 93106 USA. [Kasliwal, Mansi M.] Observ Carnegie Inst Sci, 813 Santa Barbara St, Pasadena, CA 91101 USA. Harvard Smithsonian Ctr Astrophys, Smithsonian Astrophys Observ, 60 Garden St, Cambridge, MA 02138 USA. [Perley, Daniel A.] Univ Copenhagen, Niels Bohr Inst, Dark Cosmol Ctr, Juliane Maries Vej 30, DK-2100 Copenhagen O, Denmark. [Cenko, S. Bradley] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Mail Code 661, Greenbelt, MD 20771 USA. [Cenko, S. Bradley] Univ Maryland, Joint Space Sci Inst, College Pk, MD 20742 USA. [Rebbapragada, Umaa D.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Wozniak, P. R.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Filippenko, Alexei V.; Clubb, K. I.; Nugent, Peter E.] Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. [Nugent, Peter E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Pan, Y-C.] Univ Illinois, Dept Astron, 1002 W Green St, Urbana, IL 61801 USA. [Badenes, C.] Univ Pittsburgh, Dept Phys & Astron, 3941 OHara St, Pittsburgh, PA 15260 USA. [Badenes, C.] Univ Pittsburgh, Pittsburgh Particle Phys Astrophys & Cosmol Ctr P, 3941 OHara St, Pittsburgh, PA 15260 USA. [Howell, D. Andrew] Univ Calif Santa Barbara, Dept Phys, Broida Hall,Mail Code 9530, Santa Barbara, CA 93106 USA. [Sand, David] Texas Tech Univ, Dept Phys, Lubbock, TX 79409 USA. [Sollerman, J.] Stockholm Univ, Oskar Klein Ctr, Dept Astron, SE-10691 Stockholm, Sweden. [Johansson, Joel] Stockholm Univ, Oskar Klein Ctr, Dept Phys, SE-10691 Stockholm, Sweden. [Leonard, Douglas C.; Horst, J. Chuck; Armen, Stephen F.; Fedrow, Joseph M.; Quimby, Robert M.] San Diego State Univ, Dept Astron, San Diego, CA 92182 USA. [Fedrow, Joseph M.] Kyoto Univ, Yukawa Inst Theoret Phys, Kyoto 6068502, Japan. [Quimby, Robert M.] Univ Tokyo, UTIAS, Kavli IPMU WPI, Kashiwa, Chiba 2778583, Japan. [Mazzali, Paulo] Liverpool John Moores Univ, IC2, Astrophys Res Inst, Liverpool Sci Pk,146 Browlow Hill, Liverpool L3 5RF, Merseyside, England. [Mazzali, Paulo; Sternberg, Assaf] Max Planck Inst Astrophys, Karl Schwarzschild Str 1, D-85748 Garching, Germany. [Pian, Elena] Inst Space Astrophys & Cosm Phys, INAF, Via P Gobetti 101, I-40129 Bologna, Italy. [Pian, Elena] Scuola Normale Super Pisa, Piazza Cavalieri 7, I-56126 Pisa, Italy. [Sternberg, Assaf] Tech Univ Munich, Excellence Cluster Universe, Boltzmannstr 2, D-85748 Garching, Germany. [Matheson, Thomas] Natl Opt Astron Observ, 950 N Cherry Ave, Tucson, AZ 85719 USA. [Sullivan, M.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Maguire, K.] ESO, Karl Schwarzschild Str 2, D-85748 Garching, Germany. [Lazarevic, Sanja] Univ Belgrade, Fac Math, Dept Astron, Belgrade, Serbia. RP Rubin, A (reprint author), Weizmann Inst Sci, Dept Particle Phys & Astrophys, 234 Herzl St, Rehovot, Israel. EM adam.rubin@weizmann.ac.il RI Horesh, Assaf/O-9873-2016; OI Horesh, Assaf/0000-0002-5936-1156; Sollerman, Jesper/0000-0003-1546-6615; Wozniak, Przemyslaw/0000-0002-9919-3310; Sullivan, Mark/0000-0001-9053-4820 FU EU/FP7 via ERC [307260]; Quantum universe I-CORE Program by the Israeli Committee for Planning and Budgeting; Israel Science Foundation (ISF); Minerva grant; ISF grant; Weizmann-UK "making connections" program; Kimmel award; ARCHES award; Willner Family Leadership Institute Ilan Gluzman (Secaucus, NJ); Weizmann-UK; I-CORE Program of the Planning and Budgeting Committee; EU/FP7-ERC [615929]; NSF [AST-1009571, AST-1210311, AST-1211916]; Christopher R. Redlich Fund; TABASGO Foundation; W.M. Keck Foundation; Robert Martin Ayers Sciences Fund; US Department of Energy, Laboratory Directed Research and Development program; ISF; Royal Society; US Government; Minerva; European Community FX A.G.Y. is supported by the EU/FP7 via ERC grant No. 307260, the Quantum universe I-CORE Program by the Israeli Committee for Planning and Budgeting and the Israel Science Foundation (ISF); by Minerva and ISF grants; by the Weizmann-UK "making connections" program; and by Kimmel and ARCHES awards. E.O.O. is the incumbent of the Arye Dissentshik career development chair and is grateful for support by grants from the Willner Family Leadership Institute Ilan Gluzman (Secaucus, NJ), ISF, Minerva, Weizmann-UK, and the I-CORE Program of the Planning and Budgeting Committee and the ISF. M. S. acknowledges support from the Royal Society and EU/FP7-ERC grant No. [615929]. K. M. is grateful for a Marie Curie Intra-European Fellowship, within the 7th European Community Framework Programme (FP7). D.C.L., S.F.A., J.C.H., and J.M.F. are supported by NSF grants AST-1009571 and AST-1210311, under which part of this research (photometry data collected at MLO) was carried out. The supernova research of A.V.F.'s group at U.C. Berkeley presented herein is supported by Gary & Cynthia Bengier, the Christopher R. Redlich Fund, the TABASGO Foundation, and NSF grant AST-1211916.; Research at Lick Observatory is partially supported by a generous gift from Google. Some of the data presented here were obtained at the W.M. Keck Observatory, which is operated as a scientific partnership among the California Institute of Technology, the University of California, and NASA; the observatory was made possible by the generous financial support of the W.M. Keck Foundation. The William Herschel Telescope is operated on the island of La Palma by the Isaac Newton Group in the Spanish Observatorio del Roque de los Muchachos of the Instituto de Astrofisica de Canarias. This research has made use of the APASS database, located at the AAVSO web site. Funding for APASS has been provided by the Robert Martin Ayers Sciences Fund. A portion of this work was carried out at the Jet Propulsion Laboratory under a Research and Technology Development Grant, under contract with the National Aeronautics and Space Administration. US Government Support is acknowledged. LANL participation in iPTF is supported by the US Department of Energy as part of the Laboratory Directed Research and Development program. NR 75 TC 8 Z9 8 U1 1 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 20 PY 2016 VL 820 IS 1 AR 33 DI 10.3847/0004-637X/820/1/33 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DH4WT UT WOS:000372787000033 ER PT J AU Wyper, PF DeVore, CR AF Wyper, P. F. DeVore, C. R. TI SIMULATIONS OF SOLAR JETS CONFINED BY CORONAL LOOPS SO ASTROPHYSICAL JOURNAL LA English DT Article DE magnetic reconnection; Sun: activity; Sun: corona ID X-RAY JETS; EXTREME-ULTRAVIOLET JETS; H-ALPHA SURGES; MAGNETIC RECONNECTION MODEL; FLUX EMERGENCE; ACTIVE-REGION; CHROMOSPHERIC EVAPORATION; NUMERICAL SIMULATIONS; CURRENT SHEETS; BLOWOUT JETS AB Coronal jets are collimated, dynamic events that occur over a broad range of spatial scales in the solar corona. In the open magnetic field of coronal holes, jets form quasi-radial spires that can extend far out into the heliosphere, while in closed-field regions the jet outflows are confined to the corona. We explore the application of the embedded-bipole model to jets occurring in closed coronal loops. In this model, magnetic free energy is injected slowly by footpoint motions that introduce twist within the closed dome of the jet source region, and is released rapidly by the onset of an ideal kink-like instability. Two length scales characterize the system: the width (N) of the jet source region and the footpoint separation (L) of the coronal loop that envelops the jet source. We find that both the conditions for initiation and the subsequent dynamics are highly sensitive to the ratio L/N. The longest-lasting and most energetic jets occur along long coronal loops with large L/N ratios, and share many of the features of open-field jets, while smaller L/N ratios produce shorter-duration, less energetic jets that are affected by reflections from the far-loop footpoint. We quantify the transition between these behaviors and show that our model replicates key qualitative and quantitative aspects of both quiet Sun and active-region loop jets. We also find that the reconnection between the closed dome and surrounding coronal loop is very extensive: the cumulative reconnected flux at least matches the total flux beneath the dome for small L/N, and is more than double that value for large L/N. C1 [Wyper, P. F.] Oak Ridge Associated Univ, NASA, Goddard Space Flight Ctr, Heliophys Sci Div, 8800 Greenbelt Rd, Greenbelt, MD 20771 USA. [DeVore, C. R.] NASA, Goddard Space Flight Ctr, Heliophys Sci Div, 8800 Greenbelt Rd, Greenbelt, MD 20771 USA. RP Wyper, PF (reprint author), Oak Ridge Associated Univ, NASA, Goddard Space Flight Ctr, Heliophys Sci Div, 8800 Greenbelt Rd, Greenbelt, MD 20771 USA.; DeVore, CR (reprint author), NASA, Goddard Space Flight Ctr, Heliophys Sci Div, 8800 Greenbelt Rd, Greenbelt, MD 20771 USA. EM peter.f.wyper@nasa.gov; c.richard.devore@nasa.gov RI Wyper, Peter/H-9166-2013 FU ESA; NASA FX This work was supported by P.F.W.'s appointment to the NASA Postdoctoral Program, administered by Oak Ridge Associated Universities through a contract with NASA, and by C.R.D.'s participation with a NASA Living With a Star Focused Science Team on solar jets. The computer resources used to perform the numerical simulations were provided to C.R.D. by NASA's High-End Computing program at the NASA Center for Climate Simulation. Figure 1 and its animation were created using the ESA and NASA funded Helioviewer Project. We are grateful to our colleagues Spiro Antiochos, Judy Karpen, Etienne Pariat, and Kevin Dalmasse for numerous helpful discussions on the topic of solar jets, to David Pontin for ongoing discussions and insight regarding three-dimensional reconnection, and to our anonymous referee for suggesting clarifying changes to the original manuscript. NR 61 TC 4 Z9 4 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 20 PY 2016 VL 820 IS 1 AR 77 DI 10.3847/0004-637X/820/1/77 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DH4WT UT WOS:000372787000076 ER PT J AU Hannah, IG Grefenstette, BW Smith, DM Glesener, L Krucker, S Hudson, HS Madsen, KK Marsh, A White, SM Caspi, A Shih, AY Harrison, FA Stern, D Boggs, SE Christensen, FE Craig, WW Hailey, CJ Zhang, WW AF Hannah, Iain G. Grefenstette, Brian W. Smith, David M. Glesener, Lindsay Krucker, Saem Hudson, Hugh S. Madsen, Kristin K. Marsh, Andrew White, Stephen M. Caspi, Amir Shih, Albert Y. Harrison, Fiona A. Stern, Daniel Boggs, Steven E. Christensen, Finn E. Craig, William W. Hailey, Charles J. Zhang, William W. TI THE FIRST X-RAY IMAGING SPECTROSCOPY OF QUIESCENT SOLAR ACTIVE REGIONS WITH NuSTAR SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE Sun: activity; Sun: corona; Sun: X-rays, gamma rays ID HOT PLASMA; LOOPS OBSERVATIONS; ATOMIC DATABASE; CORONAL LOOPS; QUIET SUN; EMISSION; RHESSI; HINODE; TELESCOPE; SPECTRUM AB We present the first observations of quiescent active regions (ARs) using the Nuclear Spectroscopic Telescope Array (NuSTAR), a focusing hard X-ray telescope capable of studying faint solar emission from high-temperature and non-thermal sources. We analyze the first directly imaged and spectrally resolved X-rays above 2 keV from non-flaring ARs, observed near the west limb on 2014 November 1. The NuSTAR X-ray images match bright features seen in extreme ultraviolet and soft X-rays. The NuSTAR imaging spectroscopy is consistent with isothermal emission of temperatures 3.1-4.4 MK and emission measures 1-8 x 10(46) cm(-3). We do not observe emission above 5 MK, but our short effective exposure times restrict the spectral dynamic range. With few counts above 6 keV, we can place constraints on the presence of an additional hotter component between 5 and 12 MK of similar to 10(46) cm(-3) and similar to 10(43) cm(-3), respectively, at least an order of magnitude stricter than previous limits. With longer duration observations and a weakening solar cycle (resulting in an increased livetime), future NuSTAR observations will have sensitivity to a wider range of temperatures as well as possible non-thermal emission. C1 [Hannah, Iain G.; Hudson, Hugh S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow G12 8QQ, Lanark, Scotland. [Grefenstette, Brian W.; Madsen, Kristin K.; Harrison, Fiona A.] CALTECH, Cahill Ctr Astrophys, 1216 E Calif Blvd, Pasadena, CA 91125 USA. [Smith, David M.; Marsh, Andrew] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Smith, David M.; Marsh, Andrew] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Glesener, Lindsay] Univ Minnesota Twin Cities, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Glesener, Lindsay; Krucker, Saem; Hudson, Hugh S.; Boggs, Steven E.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Krucker, Saem] Univ Appl Sci & Arts Northwestern Switzerland, Sch Engn, Inst Technol 4D, CH-5210 Windisch, Switzerland. [White, Stephen M.] Air Force Res Lab, Space Vehicles Directorate, 3550 Aberdeen Ave SE, Kirtland AFB, NM 87117 USA. [Caspi, Amir] Southwest Res Inst, Boulder, CO 80302 USA. [Shih, Albert Y.] NASA, Goddard Space Flight Ctr, Solar Phys Lab, Greenbelt, MD 20771 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Christensen, Finn E.] Tech Univ Denmark, Natl Space Inst, DTU Space, Elektrovej 327, DK-2800 Lyngby, Denmark. [Craig, William W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Hailey, Charles J.] Columbia Univ, Columbia Astrophys Lab, 538 W 120th St, New York, NY 10027 USA. [Zhang, William W.] NASA, Goddard Space Flight Ctr, Astrophys Sci Div, Greenbelt, MD 20771 USA. RP Hannah, IG (reprint author), Univ Glasgow, SUPA Sch Phys & Astron, Glasgow G12 8QQ, Lanark, Scotland. EM iain.hannah@glasgow.ac.uk RI Hannah, Iain/F-1972-2011; Boggs, Steven/E-4170-2015; OI Hannah, Iain/0000-0003-1193-8603; Boggs, Steven/0000-0001-9567-4224; Hudson, Hugh/0000-0001-5685-1283; Madsen, Kristin/0000-0003-1252-4891; Caspi, Amir/0000-0001-8702-8273 FU National Aeronautics and Space Administration; NASA [NNX12AJ36G, NNX14AG07G, NNX13AM41H, 200021-140308, NASA NNX15AK26G, NNX14AN84G] FX This paper made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research made use of the NuSTAR Data Analysis Software (NUSTAR-DAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). This work is supported by: NASA grants NNX12AJ36G, NNX14AG07G, IGH (Royal Society University Research Fellowship), AM (NASA Earth Space Science Fellowship, NNX13AM41H), SK (Swiss National Science Foundation, 200021-140308), AC (NASA NNX15AK26G, NNX14AN84G). Thanks to Kim Tolbert for OSPEX help. NR 47 TC 7 Z9 7 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD MAR 20 PY 2016 VL 820 IS 1 AR L14 DI 10.3847/2041-8205/820/1/L14 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG8RT UT WOS:000372352000014 ER PT J AU Garrick, TR Diao, WJ Tengco, JM Stach, EA Senanayake, SD Chen, DA Monnier, JR Weidner, JW AF Garrick, Taylor R. Diao, Weijian Tengco, John M. Stach, Eric A. Senanayake, Sanjaya D. Chen, Donna A. Monnier, John R. Weidner, John W. TI The Effect of the Surface Composition of Ru-Pt Bimetallic Catalysts for Methanol Oxidation SO ELECTROCHIMICA ACTA LA English DT Article DE Electrochemical; Catalysts; Bimetallic; Methanol oxidation ID ELECTROOXIDATION; ALLOYS; ELECTROCATALYSTS; HYDROGENATION; PLATINUM AB A series of Ru-Pt bimetallic catalysts prepared by the electroless deposition of controlled and variable amounts of Ru on the Pt surface of a commercially-available 20 wt% Pt/C catalyst has been characterized and evaluated for the oxidation of methanol. The activity of each Ru-Pt catalyst was determined as a function of surface composition via cyclic voltammetry. For the Ru-Pt bimetallic catalysts, activity passed through a maximum at approximately 50% monodisperse Ru surface coverage. However, due to the monolayer coverage of Ru on Pt, the amount of metal in the catalyst is minimized compared to a bulk 1: 1 atomic ratio of Ru: Pt seen in commercial bimetallic catalysts. Chemisorption and temperature programmed reduction experiments confirmed that the surface had characteristics of a true bimetallic catalyst. On a mass of Pt basis, the activity of this composition for methanol oxidation was 7 times higher than pure Pt and 3.5 times higher than a commercial catalyst with a 1: 1 Pt: Ru bulk atomic ratio. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Garrick, Taylor R.; Diao, Weijian; Tengco, John M.; Monnier, John R.; Weidner, John W.] Univ S Carolina, Dept Chem Engn, Ctr Electrochem Engn, Columbia, SC 29208 USA. [Chen, Donna A.] Univ S Carolina, Dept Chem & Biochem, Columbia, SC 29208 USA. [Stach, Eric A.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11963 USA. [Senanayake, Sanjaya D.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11963 USA. RP Weidner, JW (reprint author), Univ S Carolina, Dept Chem Engn, Ctr Electrochem Engn, Columbia, SC 29208 USA. EM weidner@cec.sc.edu RI Stach, Eric/D-8545-2011; Senanayake, Sanjaya/D-4769-2009; OI Stach, Eric/0000-0002-3366-2153; Senanayake, Sanjaya/0000-0003-3991-4232; Tengco, John Meynard/0000-0002-3582-3766 FU University of South Carolina ASPIRE grant; University of South Carolina Magellan Program; University of South Carolina Honors College SURF Grant; Department of Energy FX The work presented here was partially funded by the University of South Carolina ASPIRE grant, the University of South Carolina Magellan Program, the University of South Carolina Honors College SURF Grant, and the Department of Energy. NR 19 TC 2 Z9 2 U1 7 U2 45 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD MAR 20 PY 2016 VL 195 BP 106 EP 111 DI 10.1016/j.electacta.2016.02.134 PG 6 WC Electrochemistry SC Electrochemistry GA DH1DJ UT WOS:000372524300013 ER PT J AU Colby, SM Kabilan, S Jacob, RE Kuprat, AP Einstein, DR Corley, RA AF Colby, Sean M. Kabilan, Senthil Jacob, Richard E. Kuprat, Andrew P. Einstein, Daniel R. Corley, Richard A. TI Comparison of realistic and idealized breathing patterns in computational models of airflow and vapor dosimetry in the rodent upper respiratory tract SO INHALATION TOXICOLOGY LA English DT Article DE PBPK; realistic breathing; tissue dose; olfaction; sniffing; CFD; Acetaldehyde ID ALDEHYDE DEHYDROGENASE; OLFACTORY-BULB; INHALATION TOXICITY; NASAL PASSAGES; RAT; ACETALDEHYDE; LUNG; IMAGE; FORMALDEHYDE; METABOLISM AB Context: Computational fluid dynamics (CFD) simulations of airflows coupled with physiologically based pharmacokinetic (PBPK) modeling of respiratory tissue doses of airborne materials have traditionally used either steady-state inhalation or a sinusoidal approximation of the breathing cycle for airflow simulations despite their differences from normal breathing patterns. Objective: Evaluate the impact of realistic breathing patterns, including sniffing, on predicted nasal tissue concentrations of a reactive vapor that targets the nose in rats as a case study. Materials and methods: Whole-body plethysmography measurements from a free-breathing rat were used to produce profiles of normal breathing, sniffing and combinations of both as flow inputs to CFD/PBPK simulations of acetaldehyde exposure. Results: For the normal measured ventilation profile, modest reductions in time- and tissue depth-dependent areas under the curve (AUC) acetaldehyde concentrations were predicted in the wet squamous, respiratory and transitional epithelium along the main airflow path, while corresponding increases were predicted in the olfactory epithelium, especially the most distal regions of the ethmoid turbinates, versus the idealized profile. The higher amplitude/frequency sniffing profile produced greater AUC increases over the idealized profile in the olfactory epithelium, especially in the posterior region. Conclusions: The differences in tissue AUCs at known lesion-forming regions for acetaldehyde between normal and idealized profiles were minimal, suggesting that sinusoidal profiles may be used for this chemical and exposure concentration. However, depending upon the chemical, exposure system and concentration and the time spent sniffing, the use of realistic breathing profiles, including sniffing, could become an important modulator for local tissue dose predictions. C1 [Colby, Sean M.; Kabilan, Senthil; Jacob, Richard E.; Kuprat, Andrew P.; Einstein, Daniel R.; Corley, Richard A.] Pacific NW Natl Lab, Richland, WA 99352 USA. RP Colby, SM (reprint author), Pacific NW Natl Lab, Div Biol Sci, 902 Battelle Blvd,POB 999,MSIN J4-18, Richland, WA 99352 USA. EM sean.colby@pnnl.gov FU National Heart, Lung, and Blood Institute of the National Institutes of Health [R01 HL073598] FX All model development and simulations were conducted under a grant from the National Heart, Lung, and Blood Institute of the National Institutes of Health (R01 HL073598). The authors have no conflicts of interest to declare. NR 32 TC 0 Z9 0 U1 2 U2 4 PU TAYLOR & FRANCIS LTD PI ABINGDON PA 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND SN 0895-8378 EI 1091-7691 J9 INHAL TOXICOL JI Inhal. Toxicol. 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Zeman, M. Zemla, A. Zeng, Q. Zengel, K. Zenin, O. Zenis, T. Zerwas, D. Zhang, D. Zhang, F. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for magnetic monopoles and stable particles with high electric charges in 8 TeV pp collisions with the ATLAS detector SO PHYSICAL REVIEW D LA English DT Article ID GEV CM ENERGY; IONIZING PARTICLES; MATTER; FIELD; LHC AB A search for highly ionizing particles produced in proton-proton collisions at 8 TeV center-of-mass energy is performed by the ATLAS Collaboration at the CERN Large Hadron Collider. The data set used corresponds to an integrated luminosity of 7.0 fb(-1). A customized trigger significantly increases the sensitivity, permitting a search for such particles with charges and energies beyond what was previously accessible. No events were found in the signal region, leading to production cross section upper limits in the mass range 200-2500 GeV for magnetic monopoles with magnetic charge in the range 0.5g(D) < vertical bar g vertical bar < 2.0g(D), where g(D) is the Dirac charge, and for stable particles with electric charge in the range 10 < vertical bar z vertical bar < 60. Model-dependent limits are presented in given pair-production scenarios, and model-independent limits are presented in fiducial regions of particle energy and pseudorapidity. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. 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L.; Bellagamba, L.; Biondi, S.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; Corradi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstrom, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Alberghi, G. L.; Biondi, S.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstrom, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Grefe, C.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.] Univ Bonn, Inst Phys, Nussallee 12, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Coffey, L.; Dhaliwal, S.; Fitzgerald, E. A.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Univ Fed Juiz de Fora, Elect Circuits Dept, Juiz de Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Oliveira Damazio, D.; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Alvarez Gonzalez, B.; Armbruster, A. J.; Boveia, A.; Catinaccio, A.; Cattai, A.; Dell'Acqua, A.; Di Girolamo, A.; Di Girolamo, B.; Dudarev, A.; Gorini, B.; Henriques Correia, A. M.; Hoecker, A.; Krasznahorkay, A.; Lapoire, C.; Lenzi, B.; Mandelli, B.; Marzin, A.; Milic, A.; Nairz, A. M.; Nicquevert, B.; Petersen, B. A.; Poppleton, A.; Rembser, C.; Ruiz-Martinez, A.; Salzburger, A.; Serfon, C.; Sfyrla, A.; Tricoli, A.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Salazar Loyola, J. E.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan 250100, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Romano Saez, S. M.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Romano Saez, S. M.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Blaise Pascal, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Romano Saez, S. M.; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand 2, Photochim Mol & Macromol Lab, CNRS, IN2P3, F-63177 Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, Lab Nazl Frascati, Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Naranjo Garcia, R. F.; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K-J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Naranjo Garcia, R. F.; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Olivares Pino, S. A.; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sch Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Oropeza Barrera, C.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Moreno Llacer, M.; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Lopez Mateos, D.; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Narrias Villar, D. I.; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores; Salvucci, A.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Lorenzo Martinez, N.; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Teixeira Dias Castanheira, M.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, London, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Vazquez Schroeder, T.; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Long, J. D.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Villaplana Perez, M.] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Villaplana Perez, M.] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, D-80805 Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Annovi, A.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Aloisio, A.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Natl Res Ctr Kurchatov Inst, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Bertolucci, F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. [Onofre, A.] Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] INFN Sez Pisa, Pisa, Italy. [Aloisio, A.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] INFN Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Cadi Ayyad, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Goncalves Pinto Firmino Da Costa, J.; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energie Al, IRFU Inst Rech Lois Fondamentales Univers, DSM, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; Sales De Bruin, P. H.; Torro Pastor, E.; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Lopez Paredes, B.; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Aloisio, A.; Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.; Lee, C. A.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hsu, C.; Kar, D.; March, L.; Mellado Garcia, B. R.; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Santoyo Castillo, I.; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Paredes Hernandez, D.; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Perez Codina, E.; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Della Mora, J.; Manjarres Ramos, J.; Noordeh, E.; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzaez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Annovi, A.; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzaez de la Hoz, S.; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Marti-Garcia, S.; Oliver Garcia, E.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. 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[Liu, B.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Nessi, M.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Stabile, Alberto/L-3419-2016; Villa, Mauro/C-9883-2009; Monzani, Simone/D-6328-2017; Fabbri, Laura/H-3442-2012; Brooks, William/C-8636-2013; Guo, Jun/O-5202-2015; Ippolito, Valerio/L-1435-2016; Livan, Michele/D-7531-2012; Gauzzi, Paolo/D-2615-2009; Warburton, Andreas/N-8028-2013; Di Domenico, Antonio/G-6301-2011; Li, Liang/O-1107-2015; Chekulaev, Sergey/O-1145-2015; Mashinistov, Ruslan/M-8356-2015; Staroba, Pavel/G-8850-2014; Kuday, Sinan/C-8528-2014; Goncalo, Ricardo/M-3153-2016; Solodkov, Alexander/B-8623-2017; BESSON, NATHALIE/L-6250-2015; Camarri, Paolo/M-7979-2015; messina, andrea/C-2753-2013; White, Ryan/E-2979-2015; Vranjes Milosavljevic, Marija/F-9847-2016; Vykydal, Zdenek/H-6426-2016; Snesarev, Andrey/H-5090-2013; Doyle, Anthony/C-5889-2009; Maneira, Jose/D-8486-2011; Ventura, Andrea/A-9544-2015; Gavrilenko, Igor/M-8260-2015; Kantserov, Vadim/M-9761-2015; Nechaeva, Polina/N-1148-2015; Smirnova, Oxana/A-4401-2013; Boyko, Igor/J-3659-2013; Vanadia, Marco/K-5870-2016; Gladilin, Leonid/B-5226-2011; Tikhomirov, Vladimir/M-6194-2015; Conde Muino, Patricia/F-7696-2011; Carvalho, Joao/M-4060-2013; Prokoshin, Fedor/E-2795-2012; Gorelov, Igor/J-9010-2015; Gutierrez, Phillip/C-1161-2011; Mitsou, Vasiliki/D-1967-2009; Zhukov, Konstantin/M-6027-2015; SULIN, VLADIMIR/N-2793-2015 OI Stabile, Alberto/0000-0002-6868-8329; Villa, Mauro/0000-0002-9181-8048; Monzani, Simone/0000-0002-0479-2207; Fabbri, Laura/0000-0002-4002-8353; Brooks, William/0000-0001-6161-3570; Guo, Jun/0000-0001-8125-9433; Ippolito, Valerio/0000-0001-5126-1620; Livan, Michele/0000-0002-5877-0062; Gauzzi, Paolo/0000-0003-4841-5822; Warburton, Andreas/0000-0002-2298-7315; Di Domenico, Antonio/0000-0001-8078-2759; Li, Liang/0000-0001-6411-6107; Smirnov, Sergei/0000-0002-6778-073X; Irles, Adrian/0000-0001-5668-151X; La Rosa, Alessandro/0000-0001-6291-2142; Beck, Hans Peter/0000-0001-7212-1096; Kukla, Romain/0000-0002-1140-2465; Prokofiev, Kirill/0000-0002-2177-6401; Vazquez Schroeder, Tamara/0000-0002-9780-099X; Chen, Chunhui /0000-0003-1589-9955; Terzo, Stefano/0000-0003-3388-3906; Mashinistov, Ruslan/0000-0001-7925-4676; Kuday, Sinan/0000-0002-0116-5494; Goncalo, Ricardo/0000-0002-3826-3442; Solodkov, Alexander/0000-0002-2737-8674; Camarri, Paolo/0000-0002-5732-5645; Farrington, Sinead/0000-0001-5350-9271; Robson, Aidan/0000-0002-1659-8284; White, Ryan/0000-0003-3589-5900; Vranjes Milosavljevic, Marija/0000-0003-4477-9733; Vykydal, Zdenek/0000-0003-2329-0672; Doyle, Anthony/0000-0001-6322-6195; Maneira, Jose/0000-0002-3222-2738; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Smirnova, Oxana/0000-0003-2517-531X; Boyko, Igor/0000-0002-3355-4662; Vanadia, Marco/0000-0003-2684-276X; Gladilin, Leonid/0000-0001-9422-8636; Tikhomirov, Vladimir/0000-0002-9634-0581; Conde Muino, Patricia/0000-0002-9187-7478; Carvalho, Joao/0000-0002-3015-7821; Prokoshin, Fedor/0000-0001-6389-5399; Gorelov, Igor/0000-0001-5570-0133; Mitsou, Vasiliki/0000-0002-1533-8886; SULIN, VLADIMIR/0000-0003-3943-2495 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern, Switzerland; Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon 2020, European Union; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex, France; Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos; Thales; Aristeia programmes - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We thank R. Koniuk for useful contributions. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 49 TC 3 Z9 3 U1 8 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 18 PY 2016 VL 93 IS 5 AR 052009 DI 10.1103/PhysRevD.93.052009 PG 25 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG9QF UT WOS:000372418200001 ER PT J AU Rykovanov, SG Geddes, CGR Schroeder, CB Esarey, E Leemans, WP AF Rykovanov, S. G. Geddes, C. G. R. Schroeder, C. B. Esarey, E. Leemans, W. P. TI Controlling the spectral shape of nonlinear Thomson scattering with proper laser chirping SO PHYSICAL REVIEW ACCELERATORS AND BEAMS LA English DT Article ID X-RAY SOURCE; COMPTON BACKSCATTERING; BEAMS; ELECTRONS; PULSES; FIELD AB Effects of nonlinearity in Thomson scattering of a high intensity laser pulse from electrons are analyzed. Analytic expressions for laser pulse shaping in frequency (chirping) are obtained which control spectrum broadening for high laser pulse intensities. These analytic solutions allow prediction of the spectral form and required laser parameters to avoid broadening. Results of analytical and numerical calculations agree well. The control over the scattered radiation bandwidth allows narrow bandwidth sources to be produced using high scattering intensities, which in turn greatly improves scattering yield for future x- and gamma-ray sources. C1 [Rykovanov, S. G.; Geddes, C. G. R.; Schroeder, C. B.; Esarey, E.; Leemans, W. P.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Rykovanov, S. G.] Helmholtz Inst Jena, Frobelstieg 3, D-07743 Jena, Germany. RP Rykovanov, SG (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.; Rykovanov, SG (reprint author), Helmholtz Inst Jena, Frobelstieg 3, D-07743 Jena, Germany. EM S.Rykovanov@gsi.de FU Office of Science Office of High Energy Physics [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Helmholtz Association (Helmholtz Young Investigators group) [VH-NG-1037]; U.S. Department of Energy National Nuclear Security administration [DNN RD/NA-22] FX This work was supported by the U.S. Department of Energy National Nuclear Security administration DNN R&D/NA-22, and by the Office of Science Office of High Energy Physics, under Contract No. DE-AC02-05CH11231. The simulations used the resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. S. G. R. would like to acknowledge support from Helmholtz Association (Helmholtz Young Investigators group VH-NG-1037). We would like to acknowledge fruitful discussions with M. Zolotorev, M. Efremov, C. Benedetti, D. Seipt and V. Kharin. NR 52 TC 5 Z9 5 U1 4 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9888 J9 PHYS REV ACCEL BEAMS JI Phys. Rev. Accel. Beams PD MAR 18 PY 2016 VL 19 IS 3 AR 030701 DI 10.1103/PhysRevAccelBeams.19.030701 PG 9 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DQ6VI UT WOS:000379343200001 ER PT J AU Turner, TJ Shade, PA Bernier, JV Li, SF Schuren, JC Lind, J Lienert, U Kenesei, P Suter, RM Blank, B Almer, J AF Turner, Todd J. Shade, Paul A. Bernier, Joel V. Li, Shiu Fai Schuren, Jay C. Lind, Jonathan Lienert, Ulrich Kenesei, Peter Suter, Robert M. Blank, Basil Almer, Jonathan TI Combined near- and far-field high-energy diffraction microscopy dataset for Ti-7Al tensile specimen elastically loaded in situ SO INTEGRATING MATERIALS AND MANUFACTURING INNOVATION LA English DT Article DE High-energy diffraction microscopy (HEDM); X-ray diffraction; Far-field diffraction; Near-field diffraction; Three-dimensional microstructure; Crystal plasticity finite element modeling (CPFEM) ID X-RAY-DIFFRACTION; ELECTRON-MICROSCOPY; CRYSTAL PLASTICITY; SINGLE-GRAIN; DEFORMATION; POLYCRYSTALS; MICROSTRUCTURE; SIMULATIONS; ORIENTATION; ALUMINUM AB High-energy diffraction microscopy (HEDM) constitutes a suite of combined X-ray characterization methods, which hold the unique advantage of illuminating the microstructure and micromechanical state of a material during concurrent in situ mechanical deformation. The data generated from HEDM experiments provides a heretofore unrealized opportunity to validate meso-scale modeling techniques, such as crystal plasticity finite element modeling (CPFEM), by explicitly testing the accuracy of these models at the length scales where the models predict their response. Combining HEDM methods with in situ loading under known and controlled boundary conditions represents a significant challenge, inspiring the recent development of a new high-precision rotation and axial motion system for simultaneously rotating and axially loading a sample. In this paper, we describe the initial HEDM dataset collected using this hardware on an alpha-titanium alloy (Ti-7Al) under in situ tensile deformation at the Advanced Photon Source, Argonne National Laboratory. We present both near-field HEDM data that maps out the grain morphology and intragranular crystallographic orientations and far-field HEDM data that provides the grain centroid, grain average crystallographic orientation, and grain average elastic strain tensor for each grain. Finally, we provide a finite element mesh that can be utilized to simulate deformation in the volume of this Ti-7Al specimen. The dataset supporting this article is available in the National Institute of Standards and Technology (NIST) repository (http://hdl.handle.net/11256/599). C1 [Turner, Todd J.; Shade, Paul A.; Schuren, Jay C.] Air Force Res Lab, Mat & Mfg Directorate, 2230 10th St, Wright Patterson AFB, OH 45433 USA. [Bernier, Joel V.; Li, Shiu Fai; Lind, Jonathan] Lawrence Livermore Natl Lab, Engn Directorate, 7000 East Ave, Livermore, CA 94550 USA. [Lind, Jonathan; Suter, Robert M.] Carnegie Mellon Univ, 5000 Forbes Ave, Pittsburgh, PA 15213 USA. [Lienert, Ulrich] DESY, DESY Petra 3 Notkestr 85, D-22603 Hamburg, Germany. [Kenesei, Peter; Almer, Jonathan] Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. [Blank, Basil] PulseRay, 4583 State Route 414, Beaver Dams, NY 14812 USA. RP Turner, TJ (reprint author), Air Force Res Lab, Mat & Mfg Directorate, 2230 10th St, Wright Patterson AFB, OH 45433 USA. EM Todd.Turner.5@us.af.mil RI Suter, Robert/P-2541-2014 OI Suter, Robert/0000-0002-0651-0437 NR 32 TC 1 Z9 1 U1 6 U2 9 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 2193-9764 EI 2193-9772 J9 INTEGR MATER MANUF I JI Integr. Mater. Manuf. Innov. PD MAR 18 PY 2016 VL 5 DI 10.1186/s40192-016-0048-1 PG 9 WC Materials Science, Multidisciplinary SC Materials Science GA DO7SX UT WOS:000377984400001 ER PT J AU Gault, B Saxey, DW Ashton, MW Sinnott, SB Chiaramonti, AN Moody, MP Schreiber, DK AF Gault, Baptiste Saxey, David W. Ashton, Michael W. Sinnott, Susan B. Chiaramonti, Ann N. Moody, Michael P. Schreiber, Daniel K. TI Behavior of molecules and molecular ions near a field emitter SO NEW JOURNAL OF PHYSICS LA English DT Article DE field evaporation; field ionization; atom probe tomography (APT); molecular dissociation ID ATOM-PROBE TOMOGRAPHY; POSITION-SENSITIVE DETECTOR; EVAPORATED IONS; POST-IONIZATION; DIRECTIONAL WALK; ELECTRIC-FIELDS; QUANTUM-THEORY; CHARGE STATES; CLUSTER IONS; DESORPTION AB The cold emission of particles from surfaces under intense electric fields is a process which underpins a variety of applications including atom probe tomography (APT), an analytical microscopy technique with near-atomic spatial resolution. Increasingly relying on fast laser pulsing to trigger the emission, APT experiments often incorporate the detection of molecular ions emitted from the specimen, in particular from covalently or ionically bonded materials. Notably, it has been proposed that neutral molecules can also be emitted during this process. However, this remains a contentious issue. To investigate the validity of this hypothesis, a careful review of the literature is combined with the development of new methods to treat experimental APT data, the modeling of ion trajectories, and the application of density-functional theory simulations to derive molecular ion energetics. It is shown that the direct thermal emission of neutral molecules is extremely unlikely. However, neutrals can still be formed in the course of an APT experiment by dissociation of metastable molecular ions. C1 [Gault, Baptiste; Moody, Michael P.] Univ Oxford, Dept Mat, Parks Rd, Oxford OX13PH, England. [Gault, Baptiste] Max Planck Inst Eisenforsch GmbH, Dept Microstruct Phys & Alloy Design, D-40237 Dusseldorf, Germany. [Saxey, David W.] Curtin Univ, Adv Resource Characterisat Facil, Perth, WA 6102, Australia. [Saxey, David W.] Curtin Univ, John Laeter Ctr, Perth, WA 6102, Australia. [Ashton, Michael W.] Univ Florida, Dept Mat Sci & Engn, Gainesville, FL 32611 USA. [Sinnott, Susan B.] Penn State Univ, Mat Sci & Engn, University Pk, PA 16802 USA. [Chiaramonti, Ann N.] NIST, Mat Measurement Lab, Boulder, CO 80305 USA. [Schreiber, Daniel K.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Gault, B (reprint author), Univ Oxford, Dept Mat, Parks Rd, Oxford OX13PH, England. EM b.gault@mpie.de RI Moody, Michael/H-9377-2013; OI Moody, Michael/0000-0002-9256-0966; Sinnott, Susan/0000-0002-3598-0403; Gault, Baptiste/0000-0002-4934-0458; Saxey, David/0000-0001-7433-946X FU Drs Brian Geiser & Drs David Larson (Cameca); EPSRC [GR/S49391/01]; UK Engineering and Physical Sciences Research Council (EPSRC) [EP/077664/1]; US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering FX BG acknowledges Shyeh Tjing (Cleo) Loi (University of Sydney) who performed the BEM simulations, with support from Drs Brian Geiser & Drs David Larson (Cameca). Dr Frederic De Geuser (CNRS, UJF, France) is acknowledged for fruitful discussions and commenting on the manuscript. Dr Lan Yao (U Michigan) is thanked for providing the code to compute the Kingham curves. The Cambridge Centre of Gallium Nitride is acknowledged as the source of the material used in some of these analyses, for work has been funded, in part, by the EPSRC (GR/S49391/01) and these atom probe analyses were performed at the UKAtom-probe Facility at the University of Oxford-funded by the UK Engineering and Physical Sciences Research Council (EPSRC) under grant no. EP/077664/1. DKS acknowledges support from the US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Pacific Northwest National Laboratory (PNNL) is a multiprogram national laboratory operated for DOE by Battelle. Lyle Gordon (PNNL) is acknowledged for providing the Fe3O4 sample described in this study. NR 107 TC 2 Z9 2 U1 8 U2 14 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD MAR 18 PY 2016 VL 18 AR 033031 DI 10.1088/1367-2630/18/3/033031 PG 16 WC Physics, Multidisciplinary SC Physics GA DI8CA UT WOS:000373727300003 ER PT J AU Adamczyk, L Adkins, JK Agakishiev, G Aggarwal, MM Ahammed, Z Alekseev, I Aparin, A Arkhipkin, D Aschenauer, EC Attri, A Averichev, GS Bai, X Bairathi, V Bellwied, R Bhasin, A Bhati, AK Bhattarai, P Bielcik, J Bielcikova, J Bland, LC Bordyuzhin, IG Bouchet, J Brandenburg, JD Brandin, AV Bunzarov, I Butterworth, J Caines, H Sanchez, MCD Campbell, JM Cebra, D Chakaberia, I Chaloupka, P Chang, Z Chatterjee, A Chattopadhyay, S Chen, JH Chen, X Cheng, J Cherney, M Christie, W Contin, G Crawford, HJ Das, S De Silva, LC Debbe, RR Dedovich, TG Deng, J Derevschikov, AA Di Ruzza, B Didenko, L Dilks, C Dong, X Drachenberg, JL Draper, JE Du, CM Dunkelberger, LE Dunlop, JC Efimov, LG Engelage, J Eppley, G Esha, R Evdokimov, O Eyser, O Fatemi, R Fazio, S Federic, P Fedorisin, J Feng, Z Filip, P Fisyak, Y Flores, CE Fulek, L Gagliardi, CA Garand, D Geurts, F Gibson, A Girard, M Greiner, L Grosnick, D Gunarathne, DS Guo, Y Gupta, S Gupta, A Guryn, W Hamad, AI Hamed, A Haque, R Harris, JW He, L Heppelmann, S Heppelmann, S Hirsch, A Hoffmann, GW Horvat, S Huang, T Huang, X Huang, B Huang, HZ Huck, P Humanic, TJ Igo, G Jacobs, WW Jang, H Jentsch, A Jia, J Jiang, K Judd, EG Kabana, S Kalinkin, D Kang, K Kauder, K Ke, HW Keane, D Kechechyan, A Khan, ZH Kikola, DP Kisel, I Kisiel, A Kochenda, L Koetke, DD Kosarzewski, LK Kraishan, AF Kravtsov, P Krueger, K Kumar, L Lamont, MAC Landgraf, JM Landry, KD Lauret, J Lebedev, A Lednicky, R Lee, JH Li, X Li, C Li, X Li, Y Li, W Lin, T Lisa, MA Liu, F Ljubicic, T Llope, WJ Lomnitz, M Longacre, RS Luo, X Ma, R Ma, GL Ma, YG Ma, L Magdy, N Majka, R Manion, A Margetis, S Markert, C Matis, HS McDonald, D McKinzie, S Meehan, K Mei, JC Minaev, NG Mioduszewski, S Mishra, D Mohanty, B Mondal, MM Morozov, DA Mustafa, MK Nandi, BK Nasim, M Nayak, TK Nigmatkulov, G Niida, T Nogach, LV Noh, SY Novak, J Nurushev, SB Odyniec, G Ogawa, A Oh, K Okorokov, VA Jr, DO Page, BS Pak, R Pan, YX Pandit, Y Panebratsev, Y Pawlik, B Pei, H Perkins, C Pile, P Pluta, J Poniatowska, K Porter, J Posik, M Poskanzer, AM Pruthi, NK Putschke, J Qiu, H Quintero, A Ramachandran, S Raniwala, S Raniwala, R Ray, RL Ritter, HG Roberts, JB Rogachevskiy, OV Romero, JL Ruan, L Rusnak, J Rusnakova, O Sahoo, NR Sahu, PK Sakrejda, I Salur, S Sandweiss, J Sarkar, A Schambach, J Scharenberg, RP Schmah, AM Schmidke, WB Schmitz, N Seger, J Seyboth, P Shah, N Shahaliev, E Shanmuganathan, PV Shao, M Sharma, A Sharma, B Sharma, MK Shen, WQ Shi, Z Shi, SS Shou, QY Sichtermann, EP Sikora, R Simko, M Singha, S Skoby, MJ Smirnov, N Smirnov, D Solyst, W Song, L Sorensen, P Spinka, HM Srivastava, B Stanislaus, TDS Stepanov, M Stock, R Strikhanov, M Stringfellow, B Sumbera, M Summa, B Sun, Z Sun, XM Sun, Y Surrow, B Svirida, DN Tang, Z Tang, AH Tarnowsky, T Tawfik, A Thader, J Thomas, JH Timmins, AR Tlusty, D Todoroki, T Tokarev, M Trentalange, S Tribble, RE Tribedy, P Tripathy, SK Tsai, OD Ullrich, T Underwood, DG Upsal, I Van Buren, G Van Nieuwenhuizen, G Vandenbroucke, M Varma, R Vasiliev, AN Vertesi, R Videbaek, F Vokal, S Voloshin, SA Vossen, A Wang, F Wang, G Wang, JS Wang, H Wang, Y Wang, Y Webb, G Webb, JC Wen, L Westfall, GD Wieman, H Wissink, SW Witt, R Wu, Y Xiao, ZG Xie, W Xie, G Xin, K Xu, YF Xu, QH Xu, N Xu, H Xu, Z Xu, J Yang, S Yang, Y Yang, Y Yang, C Yang, Y Yang, Q Ye, Z Ye, Z Yepes, P Yi, L Yip, K Yoo, IK Yu, N Zbroszczyk, H Zha, W Zhang, XP Zhang, Y Zhang, J Zhang, J Zhang, S Zhang, S Zhang, Z Zhang, JB Zhao, J Zhong, C Zhou, L Zhu, X Zoulkarneeva, Y Zyzak, M AF Adamczyk, L. Adkins, J. K. Agakishiev, G. Aggarwal, M. M. Ahammed, Z. Alekseev, I. Aparin, A. Arkhipkin, D. Aschenauer, E. C. Attri, A. Averichev, G. S. Bai, X. Bairathi, V. Bellwied, R. Bhasin, A. Bhati, A. K. Bhattarai, P. Bielcik, J. Bielcikova, J. Bland, L. C. Bordyuzhin, I. G. Bouchet, J. Brandenburg, J. D. Brandin, A. V. Bunzarov, I. Butterworth, J. Caines, H. Calderon de la Barca Sanchez, M. Campbell, J. M. Cebra, D. Chakaberia, I. Chaloupka, P. Chang, Z. Chatterjee, A. Chattopadhyay, S. Chen, J. H. Chen, X. Cheng, J. Cherney, M. Christie, W. Contin, G. Crawford, H. J. Das, S. De Silva, L. C. Debbe, R. R. Dedovich, T. G. Deng, J. Derevschikov, A. A. Di Ruzza, B. Didenko, L. Dilks, C. Dong, X. Drachenberg, J. L. Draper, J. E. Du, C. M. Dunkelberger, L. E. Dunlop, J. C. Efimov, L. G. Engelage, J. Eppley, G. Esha, R. Evdokimov, O. Eyser, O. Fatemi, R. Fazio, S. Federic, P. Fedorisin, J. Feng, Z. Filip, P. Fisyak, Y. Flores, C. E. Fulek, L. Gagliardi, C. A. Garand, D. Geurts, F. Gibson, A. Girard, M. Greiner, L. Grosnick, D. Gunarathne, D. S. Guo, Y. Gupta, S. Gupta, A. Guryn, W. Hamad, A. I. Hamed, A. Haque, R. Harris, J. W. He, L. Heppelmann, S. Heppelmann, S. Hirsch, A. Hoffmann, G. W. Horvat, S. Huang, T. Huang, X. Huang, B. Huang, H. Z. Huck, P. Humanic, T. J. Igo, G. Jacobs, W. W. Jang, H. Jentsch, A. Jia, J. Jiang, K. Judd, E. G. Kabana, S. Kalinkin, D. Kang, K. Kauder, K. Ke, H. W. Keane, D. Kechechyan, A. Khan, Z. H. Kikola, D. P. Kisel, I. Kisiel, A. Kochenda, L. Koetke, D. D. Kosarzewski, L. K. Kraishan, A. F. Kravtsov, P. Krueger, K. Kumar, L. Lamont, M. A. C. Landgraf, J. M. Landry, K. D. Lauret, J. Lebedev, A. Lednicky, R. Lee, J. H. Li, X. Li, C. Li, X. Li, Y. Li, W. Lin, T. Lisa, M. A. Liu, F. Ljubicic, T. Llope, W. J. Lomnitz, M. Longacre, R. S. Luo, X. Ma, R. Ma, G. L. Ma, Y. G. Ma, L. Magdy, N. Majka, R. Manion, A. Margetis, S. Markert, C. Matis, H. S. McDonald, D. McKinzie, S. Meehan, K. Mei, J. C. Minaev, N. G. Mioduszewski, S. Mishra, D. Mohanty, B. Mondal, M. M. Morozov, D. A. Mustafa, M. K. Nandi, B. K. Nasim, Md. Nayak, T. K. Nigmatkulov, G. Niida, T. Nogach, L. V. Noh, S. Y. Novak, J. Nurushev, S. B. Odyniec, G. Ogawa, A. Oh, K. Okorokov, V. A. Jr, D. Olvitt Page, B. S. Pak, R. Pan, Y. X. Pandit, Y. Panebratsev, Y. Pawlik, B. Pei, H. Perkins, C. Pile, P. Pluta, J. Poniatowska, K. Porter, J. Posik, M. Poskanzer, A. M. Pruthi, N. K. Putschke, J. Qiu, H. Quintero, A. Ramachandran, S. Raniwala, S. Raniwala, R. Ray, R. L. Ritter, H. G. Roberts, J. B. Rogachevskiy, O. V. Romero, J. L. Ruan, L. Rusnak, J. Rusnakova, O. Sahoo, N. R. Sahu, P. K. Sakrejda, I. Salur, S. Sandweiss, J. Sarkar, A. Schambach, J. Scharenberg, R. P. Schmah, A. M. Schmidke, W. B. Schmitz, N. Seger, J. Seyboth, P. Shah, N. Shahaliev, E. Shanmuganathan, P. V. Shao, M. Sharma, A. Sharma, B. Sharma, M. K. Shen, W. Q. Shi, Z. Shi, S. S. Shou, Q. Y. Sichtermann, E. P. Sikora, R. Simko, M. Singha, S. Skoby, M. J. Smirnov, N. Smirnov, D. Solyst, W. Song, L. Sorensen, P. Spinka, H. M. Srivastava, B. Stanislaus, T. D. S. Stepanov, M. Stock, R. Strikhanov, M. Stringfellow, B. Sumbera, M. Summa, B. Sun, Z. Sun, X. M. Sun, Y. Surrow, B. Svirida, D. N. Tang, Z. Tang, A. H. Tarnowsky, T. Tawfik, A. Thader, J. Thomas, J. H. Timmins, A. R. Tlusty, D. Todoroki, T. Tokarev, M. Trentalange, S. Tribble, R. E. Tribedy, P. Tripathy, S. K. Tsai, O. D. Ullrich, T. Underwood, D. G. Upsal, I. Van Buren, G. Van Nieuwenhuizen, G. Vandenbroucke, M. Varma, R. Vasiliev, A. N. Vertesi, R. Videbaek, F. Vokal, S. Voloshin, S. A. Vossen, A. Wang, F. Wang, G. Wang, J. S. Wang, H. Wang, Y. Wang, Y. Webb, G. Webb, J. C. Wen, L. Westfall, G. D. Wieman, H. Wissink, S. W. Witt, R. Wu, Y. Xiao, Z. G. Xie, W. Xie, G. Xin, K. Xu, Y. F. Xu, Q. H. Xu, N. Xu, H. Xu, Z. Xu, J. Yang, S. Yang, Y. Yang, Y. Yang, C. Yang, Y. Yang, Q. Ye, Z. Ye, Z. Yepes, P. Yi, L. Yip, K. Yoo, I. -K. Yu, N. Zbroszczyk, H. Zha, W. Zhang, X. P. Zhang, Y. Zhang, J. Zhang, J. Zhang, S. Zhang, S. Zhang, Z. Zhang, J. B. Zhao, J. Zhong, C. Zhou, L. Zhu, X. Zoulkarneeva, Y. Zyzak, M. CA STAR Collaboration TI Beam Energy Dependence of the Third Harmonic of Azimuthal Correlations in Au plus Au Collisions at RHIC SO PHYSICAL REVIEW LETTERS LA English DT Article ID HEAVY-ION COLLISIONS; QUARK-GLUON PLASMA; ELLIPTIC FLOW; AU+AU COLLISIONS; QUANTUM CHROMODYNAMICS; CENTRALITY DEPENDENCE; ROOT-S(NN)=130 GEV; PHASE-TRANSITION; QCD; MATTER AB We present results from a harmonic decomposition of two-particle azimuthal correlations measured with the STAR detector in Au + Au collisions for energies ranging from root s(NN) = 7.7 to 200 GeV. The third harmonic nu(2)(3){2} = cos 3(phi(1)-phi(2)), where phi(1)-phi(2) is the angular difference in azimuth, is studied as a function of the pseudorapidity difference between particle pairs Delta eta = eta(1) -eta(2). Nonzero nu(2)(3){2} is directly related to the previously observed large-Delta eta narrow-Delta phi ridge correlations and has been shown in models to be sensitive to the existence of a low viscosity quark gluon plasma phase. For sufficiently central collisions, nu(2)(3){2} persist down to an energy of 7.7 GeV, suggesting that quark gluon plasma may be created even in these low energy collisions. In peripheral collisions at these low energies, however, nu(2)(3){2} is consistent with zero. When scaled by the pseudorapidity density of charged-particle multiplicity per participating nucleon pair, nu(2)(3){2} for central collisions shows a minimum near root s(NN) = 20 GeV. C1 [Adamczyk, L.; Fulek, L.; Sikora, R.] AGH Univ Sci & Technol, FPACS, PL-30059 Krakow, Poland. [Krueger, K.; Spinka, H. M.; Underwood, D. G.] Argonne Natl Lab, Argonne, IL 60439 USA. [Arkhipkin, D.; Aschenauer, E. C.; Bland, L. C.; Chakaberia, I.; Christie, W.; Di Ruzza, B.; Didenko, L.; Dunlop, J. C.; Eyser, O.; Fazio, S.; Fisyak, Y.; Guryn, W.; Jia, J.; Ke, H. W.; Lamont, M. A. C.; Landgraf, J. M.; Lauret, J.; Lebedev, A.; Lee, J. H.; Ljubicic, T.; Longacre, R. S.; Ma, R.; Ogawa, A.; Page, B. S.; Pak, R.; Pile, P.; Ruan, L.; Schmidke, W. B.; Smirnov, D.; Sorensen, P.; Tang, A. H.; Todoroki, T.; Tribedy, P.; Ullrich, T.; Van Buren, G.; Van Nieuwenhuizen, G.; Videbaek, F.; Wang, H.; Webb, G.; Webb, J. C.; Xu, Z.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Crawford, H. J.; Engelage, J.; Judd, E. G.; Perkins, C.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Calderon de la Barca Sanchez, M.; Cebra, D.; Draper, J. E.; Flores, C. E.; Heppelmann, S.; Meehan, K.; Romero, J. L.] Univ Calif Davis, Davis, CA 95616 USA. [Debbe, R. R.; Dunkelberger, L. E.; Esha, R.; Huang, H. Z.; Igo, G.; Landry, K. D.; Nasim, Md.; Pan, Y. X.; Trentalange, S.; Tsai, O. D.; Wang, G.; Wen, L.] Univ Calif Los Angeles, Los Angeles, CA 90095 USA. [Bai, X.; Feng, Z.; Huck, P.; Liu, F.; Luo, X.; Pei, H.; Shi, S. S.; Sun, X. M.; Wang, Y.; Xu, J.; Yang, Y.; Yu, N.; Zhang, J. B.] Cent China Normal Univ, Wuhan 430079, Hubei, Peoples R China. [Evdokimov, O.; Huang, B.; Khan, Z. H.; Pandit, Y.; Ye, Z.] Univ Illinois, Chicago, IL 60607 USA. [Cherney, M.; De Silva, L. C.; Seger, J.] Creighton Univ, Omaha, NE 68178 USA. [Bielcik, J.; Chaloupka, P.; Rusnakova, O.] Czech Tech Univ, FNSPE, Prague 11519, Czech Republic. [Bielcikova, J.; Federic, P.; Rusnak, J.; Simko, M.; Sumbera, M.; Vertesi, R.] Nucl Phys Inst AS CR, Prague 25068, Czech Republic. [Kisel, I.; Stock, R.; Zyzak, M.] FIAS, D-60438 Frankfurt, Germany. [Das, S.; Sahu, P. K.; Tripathy, S. K.] Inst Phys, Bhubaneswar 751005, Orissa, India. [Nandi, B. K.; Sarkar, A.; Varma, R.] Indian Inst Technol, Mumbai 400076, Maharashtra, India. [Jacobs, W. W.; Kalinkin, D.; Lin, T.; Skoby, M. J.; Solyst, W.; Vossen, A.; Wissink, S. W.] Indiana Univ, Bloomington, IN 47408 USA. [Alekseev, I.; Bordyuzhin, I. G.; Svirida, D. N.] Alikhanov Inst Theoret & Expt Phys, Moscow 117218, Russia. [Bhasin, A.; Gupta, S.; Gupta, A.; Sharma, A.; Sharma, M. K.] Univ Jammu, Jammu 180001, India. [Agakishiev, G.; Aparin, A.; Averichev, G. S.; Bunzarov, I.; Dedovich, T. G.; Efimov, L. G.; Fedorisin, J.; Filip, P.; Kechechyan, A.; Lednicky, R.; Panebratsev, Y.; Rogachevskiy, O. V.; Shahaliev, E.; Tokarev, M.; Vokal, S.; Zoulkarneeva, Y.] Joint Inst Nucl Res, Dubna 141980, Russia. [Bouchet, J.; Hamad, A. I.; Kabana, S.; Keane, D.; Lomnitz, M.; Margetis, S.; Quintero, A.; Shanmuganathan, P. V.; Singha, S.; Wu, Y.] Kent State Univ, Kent, OH 44242 USA. [Adkins, J. K.; Fatemi, R.; Ramachandran, S.] Univ Kentucky, Lexington, KY 40506 USA. [Jang, H.; Noh, S. Y.] Korea Inst Sci & Technol Informat, Daejeon 305701, South Korea. [Chen, X.; Du, C. M.; Sun, Z.; Wang, J. S.; Xu, H.; Yang, Y.; Zhang, J.] Chinese Acad Sci, Inst Modern Phys, Lanzhou 730000, Gansu, Peoples R China. [Contin, G.; Dong, X.; Greiner, L.; Manion, A.; Matis, H. S.; McKinzie, S.; Mustafa, M. K.; Odyniec, G.; Porter, J.; Poskanzer, A. M.; Qiu, H.; Ritter, H. G.; Sakrejda, I.; Salur, S.; Schmah, A. M.; Shi, Z.; Sichtermann, E. P.; Thader, J.; Thomas, J. H.; Wieman, H.; Xu, N.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Schmitz, N.; Seyboth, P.] Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany. [Novak, J.; Tarnowsky, T.; Westfall, G. D.] Michigan State Univ, E Lansing, MI 48824 USA. [Brandin, A. V.; Kochenda, L.; Kravtsov, P.; Nigmatkulov, G.; Okorokov, V. A.; Strikhanov, M.] Natl Res Nucl Univ MEPhI, Moscow 115409, Russia. [Bairathi, V.; Haque, R.; Mishra, D.; Mohanty, B.] Natl Inst Sci Educ & Res, Bhubaneswar 751005, Orissa, India. [Huang, T.; Yang, Y.] Natl Cheng Kung Univ, Tainan 70101, Taiwan. [Campbell, J. M.; Humanic, T. J.; Lisa, M. A.; Upsal, I.] Ohio State Univ, Columbus, OH 43210 USA. [Pawlik, B.; Sharma, B.] Inst Nucl Phys PAN, PL-31342 Krakow, Poland. [Aggarwal, M. M.; Attri, A.; Bhati, A. K.; Kumar, L.; Pruthi, N. K.] Panjab Univ, Chandigarh 160014, India. [Dilks, C.; Heppelmann, S.; Summa, B.] Penn State Univ, University Pk, PA 16802 USA. [Derevschikov, A. A.; Minaev, N. G.; Morozov, D. A.; Nogach, L. V.; Nurushev, S. B.; Vasiliev, A. N.] Inst High Energy Phys, Protvino 142281, Russia. [Garand, D.; He, L.; Hirsch, A.; Scharenberg, R. P.; Srivastava, B.; Stepanov, M.; Stringfellow, B.; Wang, F.; Xie, W.; Zhao, J.] Purdue Univ, W Lafayette, IN 47907 USA. [Oh, K.; Yoo, I. -K.] Pusan Natl Univ, Pusan 46241, South Korea. [Raniwala, S.; Raniwala, R.] Univ Rajasthan, Jaipur 302004, Rajasthan, India. [Brandenburg, J. D.; Butterworth, J.; Eppley, G.; Geurts, F.; Roberts, J. B.; Tlusty, D.; Xin, K.; Yepes, P.] Rice Univ, Houston, TX 77251 USA. [Guo, Y.; Jiang, K.; Li, C.; Li, X.; Shao, M.; Sun, Y.; Tang, Z.; Xie, G.; Yang, S.; Yang, C.; Yang, Q.; Zha, W.; Zhang, Y.; Zhang, S.; Zhou, L.] Univ Sci & Technol China, Hefei 230026, Anhui, Peoples R China. [Deng, J.; Mei, J. C.; Xu, Q. H.; Zhang, J.] Shandong Univ, Jinan 250100, Shandong, Peoples R China. [Chen, J. H.; Li, W.; Ma, G. L.; Ma, Y. G.; Ma, L.; Shah, N.; Shen, W. Q.; Shou, Q. Y.; Xu, Y. F.; Zhang, S.; Zhang, Z.; Zhong, C.] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China. [Magdy, N.] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Gunarathne, D. S.; Kraishan, A. F.; Li, X.; Jr, D. Olvitt; Posik, M.; Surrow, B.; Vandenbroucke, M.] Temple Univ, Philadelphia, PA 19122 USA. [Chang, Z.; Gagliardi, C. A.; Hamed, A.; Mioduszewski, S.; Mondal, M. M.; Sahoo, N. R.; Tribble, R. E.] Texas A&M Univ, College Stn, TX 77843 USA. [Bhattarai, P.; Hoffmann, G. W.; Jentsch, A.; Markert, C.; Ray, R. L.; Schambach, J.] Univ Texas Austin, Austin, TX 78712 USA. [Bellwied, R.; McDonald, D.; Song, L.; Timmins, A. R.] Univ Houston, Houston, TX 77204 USA. [Cheng, J.; Huang, X.; Kang, K.; Li, Y.; Wang, Y.; Xiao, Z. G.; Zhang, X. P.; Zhu, X.] Tsinghua Univ, Beijing 100084, Peoples R China. [Witt, R.] US Naval Acad, Annapolis, MD 21402 USA. [Drachenberg, J. L.; Gibson, A.; Grosnick, D.; Koetke, D. D.; Stanislaus, T. D. S.] Valparaiso Univ, Valparaiso, IN 46383 USA. [Ahammed, Z.; Chatterjee, A.; Chattopadhyay, S.; Nayak, T. K.] Ctr Variable Energy Cyclotron, Kolkata 700064, India. [Girard, M.; Kikola, D. P.; Kisiel, A.; Kosarzewski, L. K.; Pluta, J.; Poniatowska, K.; Zbroszczyk, H.] Warsaw Univ Technol, PL-00661 Warsaw, Poland. [Kauder, K.; Llope, W. J.; Niida, T.; Putschke, J.; Voloshin, S. A.] Wayne State Univ, Detroit, MI 48201 USA. [Tawfik, A.] WLCAPP, Cairo 11571, Egypt. [Caines, H.; Harris, J. W.; Horvat, S.; Majka, R.; Sandweiss, J.; Smirnov, N.; Yi, L.] Yale Univ, New Haven, CT 06520 USA. RP Adamczyk, L (reprint author), AGH Univ Sci & Technol, FPACS, PL-30059 Krakow, Poland. RI Chaloupka, Petr/E-5965-2012; Huang, Bingchu/H-6343-2015; Fazio, Salvatore /G-5156-2010; Xin, Kefeng/O-9195-2016; Yi, Li/Q-1705-2016; Alekseev, Igor/J-8070-2014; Svirida, Dmitry/R-4909-2016; Tawfik, Abdel Nasser/M-6220-2013; Okorokov, Vitaly/C-4800-2017; Ma, Yu-Gang/M-8122-2013; Gunarathne, Devika/C-4903-2017 OI Sikora, Rafal/0000-0001-5185-2367; Ke, Hongwei/0000-0003-1463-7291; Sorensen, Paul/0000-0001-5056-9391; Thomas, James/0000-0002-6256-4536; Huang, Bingchu/0000-0002-3253-3210; Xin, Kefeng/0000-0003-4853-9219; Yi, Li/0000-0002-7512-2657; Alekseev, Igor/0000-0003-3358-9635; Tawfik, Abdel Nasser/0000-0002-1679-0225; Okorokov, Vitaly/0000-0002-7162-5345; Ma, Yu-Gang/0000-0002-0233-9900; Gunarathne, Devika/0000-0002-7155-7418 FU RHIC Operations Group and RCF at BNL; NERSC Center at LBNL; KISTI Center in Korea; Open Science Grid consortium; Office of Nuclear Physics within the U.S. DOE Office of Science; U.S. NSF; Ministry of Education and Science of the Russian Federation; NSFC; CAS; MoST; MoE of China; National Research Foundation of Korea; NCKU (Taiwan); GA of the Czech Republic; MSMT of the Czech Republic; FIAS of Germany; DAE; DST; UGC of India; National Science Centre of Poland; National Research Foundation; Ministry of Science, Education and Sports of the Republic of Croatia; RosAtom of Russia FX We thank the RHIC Operations Group and RCF at BNL, the NERSC Center at LBNL, the KISTI Center in Korea, and the Open Science Grid consortium for providing resources and support. This work was supported in part by the Office of Nuclear Physics within the U.S. DOE Office of Science, the U.S. NSF, the Ministry of Education and Science of the Russian Federation, NSFC, CAS, MoST, and MoE of China, the National Research Foundation of Korea, NCKU (Taiwan), GA and MSMT of the Czech Republic, FIAS of Germany, DAE, DST, and UGC of India, the National Science Centre of Poland, National Research Foundation, the Ministry of Science, Education and Sports of the Republic of Croatia, and RosAtom of Russia. NR 78 TC 4 Z9 4 U1 11 U2 25 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 18 PY 2016 VL 116 IS 11 AR 112302 DI 10.1103/PhysRevLett.116.112302 PG 9 WC Physics, Multidisciplinary SC Physics GA DG9WB UT WOS:000372433400003 PM 27035295 ER PT J AU Baczewski, AD Shulenburger, L Desjarlais, MP Hansen, SB Magyar, RJ AF Baczewski, A. D. Shulenburger, L. Desjarlais, M. P. Hansen, S. B. Magyar, R. J. TI X-ray Thomson Scattering in Warm Dense Matter without the Chihara Decomposition SO PHYSICAL REVIEW LETTERS LA English DT Article ID TOTAL-ENERGY CALCULATIONS; TIME-DEPENDENT ENSEMBLES; AUGMENTED-WAVE METHOD; ELECTRON-GAS; BASIS-SET; PLASMAS; METALS; STATE AB X-ray Thomson scattering is an important experimental technique used to measure the temperature, ionization state, structure, and density of warm dense matter (WDM). The fundamental property probed in these experiments is the electronic dynamic structure factor. In most models, this is decomposed into three terms [J. Chihara, J. Phys. F 17, 295 (1987)] representing the response of tightly bound, loosely bound, and free electrons. Accompanying this decomposition is the classification of electrons as either bound or free, which is useful for gapped and cold systems but becomes increasingly questionable as temperatures and pressures increase into the WDM regime. In this work we provide unambiguous first principles calculations of the dynamic structure factor of warm dense beryllium, independent of the Chihara form, by treating bound and free states under a single formalism. The computational approach is real-time finite-temperature time-dependent density functional theory (TDDFT) being applied here for the first time to WDM. We compare results from TDDFT to Chihara-based calculations for experimentally relevant conditions in shock-compressed beryllium. C1 [Baczewski, A. D.; Magyar, R. J.] Sandia Natl Labs, Ctr Comp Res, POB 5800, Albuquerque, NM 87185 USA. [Shulenburger, L.; Desjarlais, M. P.; Hansen, S. B.] Sandia Natl Labs, Pulsed Power Sci Ctr, POB 5800, Albuquerque, NM 87185 USA. RP Baczewski, AD (reprint author), Sandia Natl Labs, Ctr Comp Res, POB 5800, Albuquerque, NM 87185 USA. EM adbacze@sandia.gov FU Sandia's Laboratory Directed Research and Development (LDRD) Project [165731]; U.S. Department of Energy, Office of Science Early Career Research Program, Office of Fusion Energy Sciences; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Calculations were completed on Chama and Skybridge at Sandia National Laboratories and Sequoia at Lawrence Livermore National Laboratory. We are grateful for discussions with Stephen Bond, Kieron Burke, Hardy Gross, Ryan Hatcher, Neepa Maitra, Thomas Mattsson, Normand Modine, Jonathan Moussa, Kai-Uwe Plagemann, Aurora Pribram-Jones, Kenneth Rudinger, Travis Sjostrom, and Sam Trickey. A. D. B, L. S., M. P. D., and R. J. M. were supported by Sandia's Laboratory Directed Research and Development (LDRD) Project No. 165731. S. B. H. was supported by the U.S. Department of Energy, Office of Science Early Career Research Program, Office of Fusion Energy Sciences. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 52 TC 5 Z9 5 U1 4 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 18 PY 2016 VL 116 IS 11 AR 115004 DI 10.1103/PhysRevLett.116.115004 PG 6 WC Physics, Multidisciplinary SC Physics GA DG9WB UT WOS:000372433400004 PM 27035307 ER PT J AU Gray, AX Jeong, J Aetukuri, NP Granitzka, P Chen, Z Kukreja, R Higley, D Chase, T Reid, AH Ohldag, H Marcus, MA Scholl, A Young, AT Doran, A Jenkins, CA Shafer, P Arenholz, E Samant, MG Parkin, SSP Durr, HA AF Gray, A. X. Jeong, J. Aetukuri, N. P. Granitzka, P. Chen, Z. Kukreja, R. Higley, D. Chase, T. Reid, A. H. Ohldag, H. Marcus, M. A. Scholl, A. Young, A. T. Doran, A. Jenkins, C. A. Shafer, P. Arenholz, E. Samant, M. G. Parkin, S. S. P. Duerr, H. A. TI Correlation-Driven Insulator-Metal Transition in Near-Ideal Vanadium Dioxide Films SO PHYSICAL REVIEW LETTERS LA English DT Article ID X-RAY-ABSORPTION; MOTT-HUBBARD; BAND THEORY; VO2; SPECTROSCOPY; PEIERLS; OXIDES; VIEW AB We use polarization- and temperature-dependent x-ray absorption spectroscopy, in combination with photoelectron microscopy, x-ray diffraction, and electronic transport measurements, to study the driving force behind the insulator-metal transition in VO2. We show that both the collapse of the insulating gap and the concomitant change in crystal symmetry in homogeneously strained single-crystalline VO2 films are preceded by the purely electronic softening of Coulomb correlations within V-V singlet dimers. This process starts 7 K (+/- 0.3 K) below the transition temperature, as conventionally defined by electronic transport and x-ray diffraction measurements, and sets the energy scale for driving the near-roomtemperature insulator-metal transition in this technologically promising material. C1 [Gray, A. X.; Granitzka, P.; Chen, Z.; Kukreja, R.; Higley, D.; Chase, T.; Reid, A. H.; Duerr, H. A.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Gray, A. X.] Temple Univ, Dept Phys, 1925 North 12th St, Philadelphia, PA 19130 USA. [Jeong, J.; Aetukuri, N. P.; Samant, M. G.; Parkin, S. S. P.] IBM Almaden Res Ctr, 650 Harry Rd, San Jose, CA 95120 USA. [Granitzka, P.] Univ Amsterdam, Van der Waals Zeeman Inst, Kruislaan 403, NL-1018 XE Amsterdam, Netherlands. [Chen, Z.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Kukreja, R.] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. [Higley, D.; Chase, T.] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. [Ohldag, H.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Marcus, M. A.; Scholl, A.; Young, A. T.; Doran, A.; Jenkins, C. A.; Shafer, P.; Arenholz, E.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Gray, AX (reprint author), SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA.; Gray, AX (reprint author), Temple Univ, Dept Phys, 1925 North 12th St, Philadelphia, PA 19130 USA. EM axgray@temple.edu; hdurr@slac.stanford.edu RI Durr, Hermann/F-6205-2012 FU Stanford Institute for Materials and Energy Sciences (SIMES) [DE-AC02-76SF00515]; U.S. Department of Energy, Office of Basic Energy Sciences; Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC02-76SF00515, DE-AC02-05CH11231] FX Research at Stanford was supported through the Stanford Institute for Materials and Energy Sciences (SIMES) under Contract No. DE-AC02-76SF00515 and the LCLS by the U.S. Department of Energy, Office of Basic Energy Sciences. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, is supported by the Director, Office of Science, Office of Basic Energy Sciences, U.S. Department of Energy under Contract No. DE-AC02-76SF00515. The authors would like to thank C.-C. Chen, B. Moritz, T. P. Devereaux, and M. van Veenendaal for helpful discussions. NR 30 TC 6 Z9 6 U1 23 U2 70 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 18 PY 2016 VL 116 IS 11 AR 116403 DI 10.1103/PhysRevLett.116.116403 PG 6 WC Physics, Multidisciplinary SC Physics GA DG9WB UT WOS:000372433400008 PM 27035314 ER PT J AU Duran, BEL Duncan, DS Oates, LG Kucharik, CJ Jackson, RD AF Duran, Brianna E. L. Duncan, David S. Oates, Lawrence G. Kucharik, Christopher J. Jackson, Randall D. TI Nitrogen Fertilization Effects on Productivity and Nitrogen Loss in Three Grass-Based Perennial Bioenergy Cropping Systems SO PLOS ONE LA English DT Article ID TRACE-GAS FLUXES; SOUTHERN WISCONSIN; BIOMASS PRODUCTION; CURRENT KNOWLEDGE; SOIL RESPIRATION; PLANT DIVERSITY; SWITCHGRASS; USA; BIODIVERSITY; MANAGEMENT AB Nitrogen (N) fertilization can greatly improve plant productivity but needs to be carefully managed to avoid harmful environmental impacts. Nutrient management guidelines aimed at reducing harmful forms of N loss such as nitrous oxide (N2O) emissions and nitrate (NO3-) leaching have been tailored for many cropping systems. The developing bioenergy industry is likely to make use of novel cropping systems, such as polycultures of perennial species, for which we have limited nutrient management experience. We studied how a switchgrass (Panicum virgatum) monoculture, a 5-species native grass mixture and an 18-species restored prairie responded to annual fertilizer applications of 56 kg N ha(-1) in a field-scale agronomic trial in south-central Wisconsin over a 2-year period. We observed greater fertilizer-induced N2O emissions and sub-rooting zone NO3- concentrations in the switchgrass monoculture than in either polyculture. Fertilization increased aboveground net primary productivity in the polycultures, but not in the switchgrass monoculture. Switchgrass was generally more productive, while the two polycultures did not differ from each other in productivity or N loss. Our results highlight differences between polycultures and a switchgrass monoculture in responding to N fertilization. C1 [Duran, Brianna E. L.; Duncan, David S.; Oates, Lawrence G.; Kucharik, Christopher J.; Jackson, Randall D.] Univ Wisconsin, Dept Agron, 1575 Linden Dr, Madison, WI 53706 USA. [Duran, Brianna E. L.; Duncan, David S.; Oates, Lawrence G.; Kucharik, Christopher J.; Jackson, Randall D.] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI USA. RP Oates, LG (reprint author), Univ Wisconsin, Dept Agron, 1575 Linden Dr, Madison, WI 53706 USA.; Oates, LG (reprint author), Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI USA. EM oates@wisc.edu OI Kucharik, Christopher/0000-0002-0400-758X FU DOE Great Lakes Bioenergy Research Center (DOE BER Office of Science) [DE-FC02-07ER64494]; DOE OBP Office of Energy Efficiency and Renewable Energy [DE-AC05-76RL01830]; Water Sustainability and Climate Program of the National Science Foundation [DEB-1038759]; Multi-State Hatch Grant [WISO1420]; UW Department of Agronomy; D.C. Smith Wisconsin Distinguished Graduate Fellowship FX This work was funded in part by the DOE Great Lakes Bioenergy Research Center (https://www.glbrc.org/)(DOE BER Office of Science DE-FC02-07ER64494; http://science.energy.gov/) and DOE OBP Office of Energy Efficiency and Renewable Energy (DE-AC05-76RL01830; http://energy.gov/eere/office-energy-efficiency-renewable-energy), the Water Sustainability and Climate Program of the National Science Foundation (DEB-1038759), a Multi-State Hatch Grant (#WISO1420), the UW Department of Agronomy, and the D.C. Smith Wisconsin Distinguished Graduate Fellowship. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 55 TC 0 Z9 0 U1 12 U2 35 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 18 PY 2016 VL 11 IS 3 AR e0151919 DI 10.1371/journal.pone.0151919 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH1ZE UT WOS:000372582800117 PM 26991790 ER PT J AU Faria, JP Overbeek, R Taylor, RC Conrad, N Vonstein, V Goelzer, A Fromion, V Rocha, M Rocha, I Henry, CS AF Faria, Jose P. Overbeek, Ross Taylor, Ronald C. Conrad, Neal Vonstein, Veronika Goelzer, Anne Fromion, Vincent Rocha, Miguel Rocha, Isabel Henry, Christopher S. TI Reconstruction of the Regulatory Network for Bacillus subtilis and Reconciliation with Gene Expression Data SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE Atomic Regulon; regulatory network; stimuli; regulation; Bacillus subtilis ID TRANSCRIPTIONAL REGULATION; ESCHERICHIA-COLI; REPRESSOR TRER; OPERON; METABOLISM; REGULON; GENOME; MODEL; FUR; ARCHITECTURE AB We introduce a manually constructed and curated regulatory network model that describes the current state of knowledge of transcriptional regulation of Bacillus subtilis. The model corresponds to an updated and enlarged version of the regulatory model of central metabolism originally proposed in 2008. We extended the original network to the whole genome by integration of information from DBTBS, a compendium of regulatory data that includes promoters, transcription factors (TFs), binding sites, motifs, and regulated operons. Additionally, we consolidated our network with all the information on regulation included in the SporeWeb and Subtiwiki community-curated resources on B. subtilis. Finally, we reconciled our network with data from RegPrecise, which recently released their own less comprehensive reconstruction of the regulatory network for B. subtilis. Our model describes 275 regulators and their target genes, representing 30 different mechanisms of regulation such as TFs, RNA switches, Riboswitches, and small regulatory RNAs. Overall, regulatory information is included in the model for 2500 of the 4200 genes in B. subtilis 168. In an effort to further expand our knowledge of B. subtilis regulation, we reconciled our model with expression data. For this process, we reconstructed the Atomic Regulons (ARs) for B. subtilis, which are the sets of genes that share the same "ON" and "OFF" gene expression profiles across multiple samples of experimental data. We show how ARs for B. sub tills are able to capture many sets of genes corresponding to regulated operons in our manually curated network. Additionally, we demonstrate how ARs can be used to help expand or validate the knowledge of the regulatory networks by looking at highly correlated genes in the ARs for which regulatory information is lacking. During this process, we were also able to infer novel stimuli for hypothetical genes by exploring the genome expression metadata relating to experimental conditions, gaining insights into novel biology. C1 [Faria, Jose P.; Henry, Christopher S.] Univ Chicago, Computat Inst, Chicago, IL 60637 USA. [Faria, Jose P.; Conrad, Neal] Argonne Natl Lab, Comp Environm & Life Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Faria, Jose P.; Rocha, Miguel; Rocha, Isabel] Univ Minho, Ctr Biol Engn, Braga, Portugal. [Overbeek, Ross; Vonstein, Veronika] Interpretat Genomes, Burr Ridge, IL USA. [Taylor, Ronald C.] US DOE, Pacific NW Natl Lab, Computat Biol & Bioinformat Grp, Richland, WA USA. [Goelzer, Anne; Fromion, Vincent] Paris Saclay Univ, INRA, Appl Math & Comp Sci Genomes Environm UR1404, Jouy En Josas, France. [Henry, Christopher S.] Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Faria, JP; Henry, CS (reprint author), Univ Chicago, Computat Inst, Chicago, IL 60637 USA.; Faria, JP (reprint author), Argonne Natl Lab, Comp Environm & Life Sci, 9700 S Cass Ave, Argonne, IL 60439 USA.; Faria, JP (reprint author), Univ Minho, Ctr Biol Engn, Braga, Portugal.; Henry, CS (reprint author), Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jplfaria@uchiago.edu; chenry@mcs.anl.gov RI Rocha, Miguel/B-9404-2011; OI Rocha, Miguel/0000-0001-8439-8172; Faria, Jose/0000-0001-9302-7250 FU FCT (Portuguese Foundation for Science and Technology) Ph.D. program [FRH/BD/70824/2010]; National Science Foundation [EFRI-MIKS-1137089]; US Department of Energy [DE-ACO2-06CH11357]; Genomic Science Program (GSP); Office of Biological and Environmental Research (OBER) FX JF acknowledges funding from [FRH/BD/70824/2010] of the FCT (Portuguese Foundation for Science and Technology) Ph.D. program. CH was supported by the National Science Foundation under grant number EFRI-MIKS-1137089 and the US Department of Energy under contract DE-ACO2-06CH11357. RT was supported by the Genomic Science Program (GSP), Office of Biological and Environmental Research (OBER), U.S. Department of Energy (DOE), and his work is a contribution of the Pacific Northwest National Laboratory (PNNL) Foundational Scientific Focus Area. NR 49 TC 1 Z9 1 U1 4 U2 13 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD MAR 18 PY 2016 VL 7 AR 275 DI 10.3389/fmicb.2016.00275 PG 11 WC Microbiology SC Microbiology GA DH0PX UT WOS:000372487200001 PM 27047450 ER PT J AU Calafiore, G Fillot, Q Dhuey, S Sassolini, S Salvadori, F Mejia, CA Munechika, K Peroz, C Cabrini, S Pina-Hernandez, C AF Calafiore, Giuseppe Fillot, Quentin Dhuey, Scott Sassolini, Simone Salvadori, Filippo Mejia, Camilo A. Munechika, Keiko Peroz, Christophe Cabrini, Stefano Pina-Hernandez, Carlos TI Printable photonic crystals with high refractive index for applications in visible light SO NANOTECHNOLOGY LA English DT Article DE titanium dioxide; functional material; photonic crystal; nanoimprint lithography; reverse imprint; optical devices ID HIGH EXTRACTION EFFICIENCY; SPONTANEOUS EMISSION AB Nanoimprint lithography (NIL) of functional high-refractive index materials has proved to be a powerful candidate for the inexpensive manufacturing of high-resolution photonic devices. In this paper, we demonstrate the fabrication of printable photonic crystals (PhCs) with high refractive index working in the visible wavelengths. The PhCs are replicated on a titanium dioxide-based high-refractive index hybrid material by reverse NIL with almost zero shrinkage and high-fidelity reproducibility between mold and printed devices. The optical responses of the imprinted PhCs compare very well with those fabricated by conventional nanofabrication methods. This study opens the road for a low-cost manufacturing of PhCs and other nanophotonic devices for applications in visible light. C1 [Calafiore, Giuseppe; Mejia, Camilo A.; Munechika, Keiko; Peroz, Christophe; Pina-Hernandez, Carlos] ABeam Technol, 22290 Foothill Blvd St2, Hayward, CA 94541 USA. [Calafiore, Giuseppe] Polytech Univ Turin, Corso Duca Abruzzi 24, I-10129 Turin, Italy. [Fillot, Quentin; Dhuey, Scott; Sassolini, Simone; Salvadori, Filippo; Cabrini, Stefano] LBNL, Mol Foundry, One Cyclotron Rd, Berkeley, CA 94702 USA. RP Pina-Hernandez, C (reprint author), ABeam Technol, 22290 Foothill Blvd St2, Hayward, CA 94541 USA.; Cabrini, S (reprint author), LBNL, Mol Foundry, One Cyclotron Rd, Berkeley, CA 94702 USA. EM scabrini@lbl.gov; cpina@abeamtech.com FU US Air Force [FA9550-14-C-0020]; Office of Science; Office of Basic Energy Sciences of the United States Department of Energy [DE-AC02-05CH11231] FX The authors would like to thank Dr Deirdre Olynick for the useful discussion. This study is supported by the US Air Force under Contract No. FA9550-14-C-0020. Work at the Molecular Foundry was supported by the Office of Science and Office of Basic Energy Sciences of the United States Department of Energy under contract DE-AC02-05CH11231. NR 21 TC 1 Z9 1 U1 6 U2 34 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD MAR 18 PY 2016 VL 27 IS 11 AR 115303 DI 10.1088/0957-4484/27/11/115303 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DD9QD UT WOS:000370259800015 PM 26875825 ER PT J AU Doughty, B Simpson, MJ Yang, B Xiao, K Ma, YZ AF Doughty, Benjamin Simpson, Mary Jane Yang, Bin Xiao, Kai Ma, Ying-Zhong TI Simplification of femtosecond transient absorption microscopy data from CH3NH3PbI3 perovskite thin films into decay associated amplitude maps SO NANOTECHNOLOGY LA English DT Article DE nonlinear imaging; ultrafast imaging; decay associated spectrum; ultrafast dynamics; big data ID PUMP-PROBE MICROSCOPY; ORGANOMETAL HALIDE PEROVSKITE; SOLAR-CELLS; FLUORESCENCE MICROSCOPY; SILICON NANOWIRES; CARRIER LIFETIME; CHARGE-CARRIERS; TARGET ANALYSIS; TRAP STATES; RECOMBINATION AB This work aims to simplify multi-dimensional femtosecond transient absorption microscopy (TAM) data into decay associated amplitude maps (DAAMs) that describe the spatial distributions of dynamical processes occurring on various characteristic timescales. Application of this method to TAM data obtained from a model methyl-ammonium lead iodide (CH3NH3PbI3) perovskite thin film allows us to simplify the data set comprising 68 time-resolved images into four DAAMs. These maps offer a simple means to visualize the complex electronic excited-state dynamics in this system by separating distinct dynamical processes evolving on characteristic timescales into individual spatial images. This approach provides new insight into subtle aspects of ultrafast relaxation dynamics associated with excitons and charge carriers in the perovskite thin film, which have recently been found to coexist at spatially distinct locations. C1 [Doughty, Benjamin; Simpson, Mary Jane; Ma, Ying-Zhong] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Yang, Bin; Xiao, Kai] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Doughty, B (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM doughtyb1@ornl.gov RI Yang, Bin/P-8529-2014; Ma, Yingzhong/L-6261-2016; Doughty, Benjamin /M-5704-2016; OI Yang, Bin/0000-0002-5667-9126; Ma, Yingzhong/0000-0002-8154-1006; Doughty, Benjamin /0000-0001-6429-9329; Simpson, Mary Jane/0000-0002-3511-8370 FU Laboratory Directed Research and Development Program of Oak Ridge National Laboratory; US Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division FX BD's research sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the US Department of Energy. BD also recognizes fruitful conversations and feedback from Dr Tessa R Calhoun. Work by MJS and Y-ZM were supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. Work by BY and KX was conducted at the Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. NR 40 TC 2 Z9 2 U1 9 U2 96 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD MAR 18 PY 2016 VL 27 IS 11 AR 114002 DI 10.1088/0957-4484/27/11/114002 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DD9QD UT WOS:000370259800006 PM 26882434 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aring;kesson, TP Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A 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Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. zur Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Identification of boosted, hadronically decaying W bosons and comparisons with ATLAS data taken at root s=8 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID COLLISIONS AB This paper reports a detailed study of techniques for identifying boosted, hadronically decaying W bosons using 20.3 fb(-1) of proton-proton collision data collected by the ATLAS detector at the LHC at a centre-of-mass energy root s = 8 TeV. A range of techniques for optimising the signal jet mass resolution are combined with various jet substructure variables. The results of these studies in Monte Carlo simulations show that a simple pairwise combination of groomed jet mass and one substructure variable can provide a 50 % efficiency for identifying W bosons with transverse momenta larger than 200 GeV while maintaining multijet background efficiencies of 2-4% for jets with the same transverse momentum. These signal and background efficiencies are confirmed in data for a selection of tagging techniques. C1 [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. 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Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarra, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Alberghi, G. L.; Biondi, S.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Ehrenfeld, W.; Gaycken, G.; Geich-Gimbel, Ch.; Gonella, L.; Grefe, C.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hellmich, D.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mergelmeyer, S.; Mijovic, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Scutti, F.; Seema, P.; Stillings, J. A.; Tannoury, N.; Velz, T.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.] Univ Bonn, Phys Inst, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Artoni, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; de Andrade Filho, L. Manhaes] Univ Fed Juiz de Fora, Elect Circuits Dept, Juiz de Fora, Brazil. [do Vale, M. A. B.] Univ Fed Sao Joao del Rei, Sao Joao del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [Alexa, C.] Transilvania Univ Brasov, Natl Inst Phys & Nucl Engn, Brasov, Romania. [Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Horia Hulubei Natl Inst Phys & Nucl Engn, Bucharest 077125, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Warburton, A.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Loyola, J. E. Salazar; Araya, S. Tapia; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Ma, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan 250100, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Nazl Frascati Lab, Grp Collegato Cosenza, I-00044 Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Washbrook, A.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Washbrook, A.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Wardrope, D. R.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Collot, J.; Crape-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores; Salvucci, A.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Pokfulam, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Ellert, M.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Ward, C. P.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Lang, V. S.; Le Guirriec, E.; Liu, J.; Liu, K.; Macina, D.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Lang, V. S.; Le Guirriec, E.; Liu, J.; Liu, K.; Macina, D.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Wanotayaroj, C.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Guo, Y.; Hu, X.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J. -F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Inst Phys, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Morvaj, L.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C. -L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Amor Dos Santos, S. P.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrument & Fis Expt Particulas LIP, Lisbon, Portugal. [Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Silva, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Fiolhais, M. C. N.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dep Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Piazzale Aldo Moro 5, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Bacci, C.; Baroncelli, A.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Reseau Univ Phys Hautes Energies Univ Hassan II, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Techn Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J. -P.; Nicolaidou, R.; Ouraou, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, Commissariat Energie Atom & Energies Alternati, DSM IRFU, Inst Rech Lois Fondamentlaes Univers, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F. -W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Lee, C. A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hsu, C.; Kar, D.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Astron & Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Cabrera Urban, S.; Castillo Gimenez, V.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. 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[Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), CNRS, IN2P3, Marseille, France. RI Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Brooks, William/C-8636-2013; Zhukov, Konstantin/M-6027-2015; Conde Muino, Patricia/F-7696-2011; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Villa, Mauro/C-9883-2009; Guo, Jun/O-5202-2015; Gladilin, Leonid/B-5226-2011; Tikhomirov, Vladimir/M-6194-2015; Warburton, Andreas/N-8028-2013; Livan, Michele/D-7531-2012; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; Carvalho, Joao/M-4060-2013; Kantserov, Vadim/M-9761-2015; Mitsou, Vasiliki/D-1967-2009; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Carli, Ina/C-2189-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015 OI Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Brooks, William/0000-0001-6161-3570; Conde Muino, Patricia/0000-0002-9187-7478; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Villa, Mauro/0000-0002-9181-8048; Guo, Jun/0000-0001-8125-9433; Gladilin, Leonid/0000-0001-9422-8636; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315; Livan, Michele/0000-0002-5877-0062; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Carvalho, Joao/0000-0002-3015-7821; Kantserov, Vadim/0000-0001-8255-416X; Mitsou, Vasiliki/0000-0002-1533-8886; Solodkov, Alexander/0000-0002-2737-8674; Carli, Ina/0000-0002-0411-1141; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon, European Union; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme - EU-ESF; Thales programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 83 TC 6 Z9 6 U1 20 U2 39 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAR 17 PY 2016 VL 76 IS 3 AR 154 DI 10.1140/epjc/s10052-016-3978-z PG 47 WC Physics, Particles & Fields SC Physics GA DL0DY UT WOS:000375303400005 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TP Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Altheimer, A Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnal, V Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Auerbach, B Augsten, K Aurousseau, M Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bacci, C Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Bain, T Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Banas, E Banerjee, S Bannoura, AAE Bansil, HS Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Becker, S Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besana, MI Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bieniek, SP Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Borroni, S Bortfeldt, J Bortolotto, V Bos, K Boscherini, D Bosman, M Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Bousson, N Boveia, A Boyd, J Boyko, IR Bozic, I Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Brazzale, SF Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristowc, K Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Bronner, J Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Brown, J De Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Bruschi, M Bruscino, N Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Buda, SI Budagov, IA 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A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.; ATLAS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. [Jackson, P.; Lee, L.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.; Saddique, A.; Vaque, F. 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N.; Karakostas, K.; Karastathis, N.; Karentzos, E.; Leontsinis, S.; Maltezos, S.; Ntekas, K.; Panagiotopoulou, E.; Papadopoulou, Th. D.; Tsipolitis, G.; Vlachos, S.] Natl Tech Univ Athens, Dept Phys, Zografos, Greece. [Abdinov, O.; Ahmadov, F.; Huseynov, N.; Javadov, N.; Khalil-zada, F.] Azerbaijan Acad Sci, Inst Phys, Baku 370143, Azerbaijan. [Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Helsens, C.; Rozas, A. Juste; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Anjos, N.; Bosman, M.; Casado, M. P.; Casolino, M.; Cavalli-Sforza, M.; Cortes-Gonzalez, A.; Farooque, T.; Fischer, C.; Fracchia, S.; Giangiobbe, V.; Parra, G. Gonzalez; Grinstein, S.; Helsens, C.; Rozas, A. Juste; Korolkov, I.; Lange, J. C.; Le Menedeu, E.; Paz, I. Lopez; Martinez, M.; Mir, L. M.; Berlingen, J. Montejo; Pages, A. Pacheco; Aranda, C. Padilla; Riu, I.; Sorin, V.; Succurro, A.; Tripiana, M. F.; Tsiskaridze, S.; Valery, L.] Univ Autonoma Barcelona, Dept Fis, E-08193 Barcelona, Spain. [Agatonovic-Jovin, T.; Bogavac, D.; Bozic, I.; Dimitrievska, A.; Krstic, J.; Marjanovic, M.; Popovic, D. S.; Sijacki, Dj.; Simic, Lj.; Vranjes, N.; Milosavljevic, M. Vranjes; Zivkovic, L.] Univ Belgrade, Inst Phys, Belgrade, Serbia. [Buanes, T.; Dale, O.; Eigen, G.; Kastanas, A.; Liebig, W.; Lipniacka, A.; Maeland, S.; Latour, B. Martin dit; Rosendahl, P. L.; Sjursen, T. B.; Smestad, L.; Stugu, B.; Ugland, M.; Zalieckas, J.] Univ Bergen, Dept Phys & Technol, Bergen, Norway. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. C.; Ovcharova, A.; Griso, S. Pagan; Potamianos, K.; Pranko, A.; Quayle, W. B.; Shapiro, M.; Sood, A.; Tibbetts, M. J.; Trottier-McDonald, M.; Tsulaia, V.; Viel, S.; Wang, H.; Yao, W. -M.; Yu, D. R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Amadio, B. T.; Axen, B.; Barnett, R. M.; Beringer, J.; Bhimji, W.; Brosamer, J.; Calafiura, P.; Cerutti, F.; Ciocio, A.; Clarke, R. N.; Cooke, M.; Einsweiler, K.; Farrell, S.; Garcia-Sciveres, M.; Gilchriese, M.; Haber, C.; Hance, M.; Heinemann, B.; Hinchliffe, I.; Hinman, R. R.; Holmes, T. R.; Jeanty, L.; Lavrijsen, W.; Leggett, C.; Loscutoff, P.; Marshall, Z.; Ohm, C. 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[Alexa, C.; Boldea, V.; Buda, S. I.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Dos Santos, S. P. Amor; Carvalho, J.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Politehn Bucuresti, Bucharest, Romania. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] West Univ Timisoara, Timisoara, Romania. [Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Assamagan, K.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. 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[Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Nazl Frascati Lab, Grp Coll Cosenza, I-00044 Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; De Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Experimentelle Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenn, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Sammel, D.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Delitzsch, C. M.; Della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, INFN Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Raddum, S.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Dunforda, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Lisovyi, M.; Schaetzelb, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Jussel, P.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kishimoto, T.; Kurashige, H.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumid, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [Akesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, D-55122 Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Quilty, D.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Davies, E.; Diaconu, C.; Diglio, S.; Djama, F.; Djuvsland, J. I.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Coadou, Y.; Davies, E.; Diaconu, C.; Diglio, S.; Djama, F.; Djuvsland, J. I.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Hu, X.; Levin, D.; Liu, H.; Long, J. D.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Xu, L.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Meroni, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr, Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J. -F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Becker, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. 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[Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; van Huysduynen, L. Hooft; Kaplan, B.; Karthik, K.; Konoplich, R.; Kreiss, S.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Moss, J.; Nagarkar, A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Yu, J.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Radeka, V.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Tseng, J. C. -L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartmento Fis, Via Palestro 3, I-27100 Pavia, Italy. [Brendlinger, K.; Fletcher, R. R. M.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Reichert, J.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Natl Res Ctr, Kurchatov Inst BP Konstantinov, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Pretea, T.; Dell'Orsoa, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Chiarelli, G.; Del Pretea, T.; Dell'Orsoa, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousaa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrumentacao Fisa Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousaa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, P-1699 Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dep Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Rome, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartmento Fis, Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Reseau Univ Phys Hautes Energies Univ Hassan II, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. 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R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, DSM IRFU Inst Rech Lois Fondamentales Univers, Commissariat Energie Atom & Energies Alternat, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F. -W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehan, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connell, S. H.; Govender, N.; Lee, C. A.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristowc, K.; Hamity, G. N.; Hsu, C.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Astron & Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Lerner, G.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Queitsch-Maitland, M.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Queitsch-Maitland, M.; Serkin, L.; Shaw, K.; Soualah, R.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Miglioranzi, S.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Valladolid Gallego, E.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. P.; McPherson, R. A.; Ouellette, E. A.; Pearce, J.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Farrington, S. M.; Harrison, P. F.; Janus, M.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Pan, Y. B.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Beermann, T. A.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Fleischmann, S.; Flick, T.; Gabizon, O.; Hamacher, K.; Harenberg, T.; Heim, T.; Hirschbuehl, D.; Kersten, S.; Kohlmann, S.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fachbereich C Phys, Wuppertal, Germany. [Baker, O. K.; Cummings, J.; Demers, S.; Garberson, F.; Guest, D.; Henrichs, A.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Thomsen, L. A.; Tipton, P.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Rahal, G.] Inst Natl Phys Nucl & Phys Particules IN2P3, Ctr Calcul, Villeurbanne, France. [Acharya, B. S.; Piccinini, M.; Pinamonti, M.] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] Novosibirsk State Univ, Novosibirsk 630090, Russia. [Bawa, H. S.] Calif State Univ Fresno, Dept Phys, Fresno, CA 93740 USA. [Beck, H. P.] Univ Fribourg, Dept Phys, CH-1700 Fribourg, Switzerland. [Castro, N. F.] Univ Porto, Fac Ciencias, Dept Fis & Astron, Rua Campo Alegre 823, P-4100 Oporto, Portugal. [Chelkov, G. A.] Tomsk State Univ, Tomsk 634050, Russia. [Conventi, F.; Della Pietra, M.] Univ Napoli Parthenope, Naples, Italy. [Corriveau, F.; McPherson, R. A.; Robertson, S. H.; Sobie, R.; Teuscher, R. J.] IPP, Waterloo, ON, Canada. [Davies, E.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Fedin, O. L.] St Petersburg State Polytechn Univ, Dept Phys, St Petersburg, Russia. [Greenwood, Z. D.; Sawyer, L.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Rozas, A. Juste; Martinez, M.] ICREA, Barcelona, Spain. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Hsinchu 30013, Taiwan. [Ilchenko, Y.; Onyisi, P. U. E.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Li, B.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Lin, S. 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RI Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Brooks, William/C-8636-2013; Zhukov, Konstantin/M-6027-2015; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Mitsou, Vasiliki/D-1967-2009; Villa, Mauro/C-9883-2009; Guo, Jun/O-5202-2015; Gladilin, Leonid/B-5226-2011; Tikhomirov, Vladimir/M-6194-2015; Warburton, Andreas/N-8028-2013; Livan, Michele/D-7531-2012; Gorelov, Igor/J-9010-2015; Ventura, Andrea/A-9544-2015; Carvalho, Joao/M-4060-2013; Kantserov, Vadim/M-9761-2015; Carli, Ina/C-2189-2017; Zaitsev, Alexandre/B-8989-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Di Domenico, Antonio/G-6301-2011; Gauzzi, Paolo/D-2615-2009; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017 OI Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Brooks, William/0000-0001-6161-3570; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559; Mitsou, Vasiliki/0000-0002-1533-8886; Villa, Mauro/0000-0002-9181-8048; Guo, Jun/0000-0001-8125-9433; Gladilin, Leonid/0000-0001-9422-8636; Tikhomirov, Vladimir/0000-0002-9634-0581; Warburton, Andreas/0000-0002-2298-7315; Livan, Michele/0000-0002-5877-0062; Gorelov, Igor/0000-0001-5570-0133; Ventura, Andrea/0000-0002-3368-3413; Carvalho, Joao/0000-0002-3015-7821; Kantserov, Vadim/0000-0001-8255-416X; Carli, Ina/0000-0002-0411-1141; Zaitsev, Alexandre/0000-0002-4961-8368; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Goncalo, Ricardo/0000-0002-3826-3442; Di Domenico, Antonio/0000-0001-8078-2759; Gauzzi, Paolo/0000-0003-4841-5822; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674 NR 1 TC 10 Z9 10 U1 15 U2 36 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. 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R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Fitzgerald, E. A.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchika, C.; Marroquima, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; de Andrade Filho, L. Manhaes] Fed Univ Juiz De Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [Do Vale, M. A. B.] Fed Univ Sao Joao Del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, CP 20516, BR-01498 Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lissauer, D.; Lynn, D.; Ma, H.; Maeno, T.; Metcalfe, J.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. 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R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Robinson, D.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feigl, S.; Perez, S. Fernandez; Francis, D.; Froidevaux, D.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Hawkings, R. J.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaekel, M. R.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lantzsch, K.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sfyrla, A.; Solans, C. A.; Spigo, G.; Stelzer, H. J.; Teischinger, F. A.; TenKate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Fiascaris, M.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Vukotic, I.; Webster, J. S.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshinb, F.; White, R.] Univ Tecn Feder Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Wang, J.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Guanb, L.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Xu, L.; Zhang, R.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Chen, S.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing 210008, Jiangsu, Peoples R China. [Chen, L.; Feng, C.; Ge, P.; Liu, B.; Mad, L. L.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Brete, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai, Peoples R China. [Chen, X.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Theveneaux-Pelzer, T.; Vazeille, F.] CNRS, IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Altheimer, A.; Andeen, T.; Angerami, A.; Bain, T.; Brooijmans, G.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Joergensen, M. D.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Grp Coll Cosenza, POB 13, I-00044 Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartmento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyka, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindura, B.; Przybyciena, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Dallas, TX 75230 USA. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Argyropoulos, S.; Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Glazov, A.; Grahn, K. -J.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hengler, C.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; Sedov, G.; Shushkevich, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Starovoitov, P.; Styles, N. A.; Tackmann, K.; Wang, J.; Wasicki, C.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Jung, C. A.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gumpert, C.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Morgenstern, M.; Novgorodova, O.; Rudolph, C.; Schnoor, U.; Siegert, F.; Socher, F.; Staerz, S.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bhimji, W.; Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; O'Brien, B. J.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Giromini, P.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Nazl Frascati Lab, I-00044 Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Giuliani, C.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Mahboubi, K.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Ruthmann, N.; Schillo, C.; Schmidt, E.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Temming, K. K.; Tsiskaridze, V.; Ungaro, F. C.; Von Radziewski, H.; Warsinsky, M.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Fribourg, Switzerland. [Ancu, L. S.; Barone, G.; Bell, W. H.; Noccioli, E. Benhar; De Mendizabal, J. Bilbao; Clark, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Muenstermann, D.; Nessi, M.; Paolozzi, L.; Picazio, A.; Ristic, B.; Schramm, S.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Durren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Ortiz, N. G. Gutierrez; Kar, D.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Annovi, A.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; George, M.; Graber, L.; Grosse-Knetter, J.; Hamer, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Llacer, M. Moreno; Musheghyan, H.; Nackenhorst, O.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Brown, J.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J. -Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subat & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Da Costa, J. Barreiro Guimaraes; Catastini, P.; Clark, B. L.; Franklin, M.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baasa, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Lisovyi, M.; Schaetzelb, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Castillo, L. R. Flores] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Mallik, U.; Mandrysch, R.; Zaidan, R.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Krumnack, N.; Pluth, D.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Aleksandrov, I. N.; Aloisio, A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Kazarinov, M. Y.; Khramov, E.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Plotnikova, E.; Potrap, I. N.; Sapronov, A.; Shiyakova, M.; Sisakyan, A. N.; Soloshenko, A.; Yeletskikh, I.; Zhemchugov, A.] Joint Inst Nucl Res Dubna, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kishimoto, T.; Kurashige, H.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Allport, P. P.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Mandic, I.; Mikuz, M.; Sfiligoj, T.] Univ Ljubljana, Ljubljana, Slovenia. [Alpigiani, C.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.; Castanheira, M. Teixeira Dias] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bieniek, S. P.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Ochoa, I.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.] CNRS, IN2P3, Paris, France. [AKesson, T. P.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Arnal, V.; Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Karnevskiy, M.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schott, M.; Schroeder, C.; Schuh, N.; Simioni, E.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Robinson, J. E. M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Serre, T.; Talby, M.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.] CNRS, IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Hanninger, G. Nunes; Nuti, F.; Rados, P.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Hu, X.; Levin, D.; Liu, H.; Long, J. D.; Lu, N.; Marley, D. E.; Mckee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Thun, R. P.; Wilson, A.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Ta, D.; Tollefson, K.; True, P.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimontia, G.; Andreazza, A.; Annovi, A.; Besana, M. I.; Carminati, L.; Cavalli, D.; Consonni, S. M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Mazza, S. M.; Meronia, C.; Perini, L.; Pizio, C.; Ragusa, F.; Resconi, S.; Shojaii, S.; Simoniello, R.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Consonni, S. M.; Fanti, M.; Mazza, S. M.; Perini, L.; Pizio, C.; Ragusa, F.; Shojaii, S.; Simoniello, R.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Arguin, J. -F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. 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J.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Nunnemann, T.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Bronner, J.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Maier, T.; Manfredini, A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; Von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst Phys, Max Planck Inst Phys, Munich, Germany. [Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Hasegawa, S.; Horii, Y.; Morvaj, L.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; De Asmundis, R.; Della Pietra, M.; Di Donato, C.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Di Donato, C.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Seidel, S. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Salvucci, A.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; De Jong, P.; De Nooij, L.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Gadatsch, S.; Geerts, D. A. A.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Linde, F.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; van der Graaf, H.; Van Der Leeuw, R.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Suhr, C.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. 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[Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Ptacek, E.; Radloff, P.; Shamim, M.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; DeVivieDeRegie, J. B.; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris 11, LAL, Orsay, France. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; DeVivieDeRegie, J. B.; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J. -F.; Guillemin, T.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Poggioli, L.; Puzo, P.; Renaud, A.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] CNRS, IN2P3, F-91405 Orsay, France. [Endo, M.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C. -L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanzaa, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Via Palestro 3, I-27100 Pavia, Italy. [Brendlinger, K.; Fletcher, R. R. M.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Stahlman, J.; Thomson, E.; Tuna, A. N.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Sedykh, E.; Seliverstov, D. M.; Solovyev, V.] Petersburg Nucl Phys Inst, Kurchatov Inst BP Konstantinov, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Cavasinni, V.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Cleland, W.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Parodi, A. Ferretto; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Pinto, B.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] Lab Instrument Fis & Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Carvalho, J.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Parodi, A. Ferretto; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Fac Ciencias & Tecnol, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Cerny, K.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Pleskot, V.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] Inst High Energy Phys, State Res Ctr, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McCubbin, N. A.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bauce, M.; Bini, C.; Ciapetti, G.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Falciano, S.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzanoa, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Di Domenico, A.; Gabrielli, A.; Gauzzi, P.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Piazzale Aldo Moro 5, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mazzaferro, L.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Mazzaferro, L.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Bacci, C.; Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Bacci, C.; Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed V Agdal, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Kivernyk, O.; Kozanecki, W.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J. -P.; Nicolaidou, R.; Ouraou, A.; E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.; Sobie, R.] CEA Saclay, DSM IRFU, Inst Rech Lois Fondamentales Univers, Commissariat Energie Atom & Energies Alternat, F-91191 Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grabas, H. M. X.; Grillo, A. A.; Kuhl, A.; LaRosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Manning, P. M.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F. -W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Blackburn, D.; Coccaro, A.; Goussiou, A. G.; Hsu, S. -C.; Lubatti, H. J.; Marx, M.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Ikematsu, K.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Bartoldus, R.; Bawa, H. S.; Black, J. E.; Cogan, J. G.; Fulsom, B. G.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Malone, C.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Strauss, E.; Su, D.; Swiatlowski, M.; Tompkins, L.; Wittgen, M.; Young, C.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Federic, P.; Plazak, L.; Stavina, P.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Hamilton, A.; Meehana, S.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Castaneda-Miranda, E.; Connellb, S. H.; Govender, N.; Lee, C. A.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Bristow, K.; Hamity, G. N.; Hsu, C.; March, L.; Garciac, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaitia, Y.; Akerstedt, H.; Annovi, A.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Poettgen, R.; Shcherbakova, A.; Silverstein, S. B.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaitia, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Kim, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Petridis, A.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjoelin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Morley, A. K.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Di Simone, A.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Grassi, V.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; Mastrandrea, P.; McCarthy, R. L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Potter, C. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Musto, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Silver, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgio, K.; Hernandez, D. Paredes; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Spreitzer, T.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaeva, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Rolli, S.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Relich, M.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.; Zhou, N.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharyaa, B. S.; Barisonzi, M.; Brazzale, S. F.; Cobal, M.; Cribbs, W. A.; Giordani, M. P.; Hellman, S.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Rossetti, V.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Grp Coll Udine, Sez Trieste, Udine, Italy. [Acharyaa, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Brazzale, S. F.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Lie, K.; Liss, T. M.; Liu, L.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Isaksson, C.; Madsen, A.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; van der Geer, R.; Vos, M.] Univ Valencia, Inst Fis Corpuscular ISIC, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; van der Geer, R.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; van der Geer, R.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; van der Geer, R.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Piqueras, D. Alvarez; Urban, S. Cabrera; Gimenez, V. Castillo; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; de la Hoz, S. Gonzalez; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Quiles, A. Irles; Pena, J. Jimenez; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Moles-Valls, R.; Garcia, E. Oliver; Lopez, S. Pedraza; Garcia-Estan, M. T. Perez; Adam, E. Romero; Ros, E.; Salt, J.; Sanchez, J.; Martinez, V. Sanchez; Soldevila, U.; Pastor, E. Torro; Valero, A.; Gallego, E. Valladolid; Ferrer, J. A. Valls; van der Geer, R.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; King, S. B.; Lister, A.; Swedish, S.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada. [Albert, J.; Berghaus, F.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; Marino, C. 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C PD MAR 17 PY 2016 VL 76 IS 3 AR 152 DI 10.1140/epjc/s10052-016-3934-y PG 14 WC Physics, Particles & Fields SC Physics GA DL0DY UT WOS:000375303400003 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Rougny, R Van de Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Brun, H Caillol, C Clerbaux, B De Lentdecker, G Fasanella, G Favart, L Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-conde, A Reis, T Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Strobbe, N Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L Da Silveira, GG Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Assran, Y Elgammal, S Kamel, AE Mahmoud, MA Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C 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Walker, M. Foerster, M. Riley, G. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dalchenko, M. De Mattia, M. Delgado, A. Dildick, S. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Krutelyov, V. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Ff, A. Perlo Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Ni, H. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Sun, X. Wang, Y. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Christian, A. Dasu, S. Dodd, L. Duric, S. Friis, E. Gomber, B. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Search for excited leptons in proton-proton collisions at root s=8 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Exotics; Hadron-Hadron scattering ID PP COLLISIONS; HADRON-COLLISIONS; COMPOSITE MODELS; QUARKS; HEAVY; SUBSTRUCTURE; RESONANCES; LEP AB A search for compositeness of electrons and muons is presented using a data sample of proton-proton collisions at a center-of-mass energy of root s = 8TeV collected with the CMS detector at the LHC and corresponding to an integrated luminosity of 19.7 fb(-1). Excited leptons (l*) produced via contact interactions in conjunction with a standard model lepton are considered, and a search is made for their gauge decay modes. The decays considered are l* -> l gamma and l* -> lZ , which give final states of two leptons and a photon or, depending on the Z-boson decay mode, four leptons or two leptons and two jets. The number of events observed in data is consistent with the standard model prediction. Exclusion limits are set on the excited lepton mass, and the compositeness scale Lambda. For the case M-l* = Lambda the existence of excited electrons (muons) is excluded up to masses of 2.45 (2.47) TeV at 95% confidence level. Neutral current decays of excited leptons are considered for the first time, and limits are extended to include the possibility that the weight factors f and f', which determine the couplings between standard model leptons and excited leptons via gauge mediated interactions, have opposite sign. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Knuenz, V.; Koenig, A.; Krammer, M.; Kraetschmer, I.; Liko, D.; Matsushita, T.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schieck, J.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] OeAW, Inst Hochenergiephys, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Lauwers, J.; Luyckx, S.; Rougny, R.; Van de Klundert, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, B-2020 Antwerp, Belgium. 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[Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; De Remigis, P.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Lee, S.; Kim, H.; Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Kim, H.; Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmad, A.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bylinkin, A.] Natl Res Nucl Univ Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Ershow, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; Manzano, P. De Castro; Duarte Campderros, J.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Cortabitarte, R. Vilar] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Mussgiller, A.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Unser, M. D.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Gutho, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Fi, F. Pandol; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Mai, S. H.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarl, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. 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[Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Berry, E.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Sinthuprasith, T.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Chauhan, S.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado Boulder, Boulder, CO USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Banerjee, S.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; No, J. M. Marra Ffi; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Wang, J.; Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Verzetti, M.] Univ Rochester, Rochester, NY USA. [Demortier, L.] Rockefeller Univ, 1230 York Ave, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Eld, D. She Ffi; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Prosper, H.; Bouhali, O.; Hernandez, A. Castaneda; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Ff, A. Perlo; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Melo, A.; Ni, H.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Sharma, A.; Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Christian, A.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Gomber, B.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Krammer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Rabady, D.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Marzocchi, B.; Di Guida, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Arcidiacono, R.; Candelise, V.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Zhang, F.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Beluffi, C.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS,IN2P3, Strasbourg, France. [Giammanco, A.] NICPB, Tallinn, Estonia. [Popov, A.; Zhukov, V.; Katkov, I.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Plestina, R.] Ecole Polytech, CNRS, Lab Leprince Ringuet, IN2P3, F-91128 Palaiseau, France. [Finger, M.; Finger, M., Jr.] Joint Inst Nucl Res, Dubna, Russia. [Assran, Y.] Suez Univ, Suez, Egypt. [Elgammal, S.] British Univ Egypt, Cairo, Egypt. [Kamel, A. Ellithi] Cairo Univ, Cairo, Egypt. [Mahmoud, M. A.] Fayoum Univ, Al Fayyum, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Toriashvili, T.] Tbilisi State Univ, GE-380086 Tbilisi, Rep of Georgia. [Bagaturia, I.] Ilia State Univ, Tbilisi, Rep of Georgia. [Gallo, E.] Univ Hamburg, Hamburg, Germany. [Hempel, M.; Karacheban, O.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Karancsi, J.] Univ Debrecen, Debrecen, Hungary. [Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Savoy-Navarro, A.] Purdue Univ, W Lafayette, IN 47907 USA. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] Agensi Nuklear Malaysia, MOSTI, Kajang, Malaysia. [Heredia-de La Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Matveev, V.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Dubinin, M.] CALTECH, Pasadena, CA 91125 USA. [Adzic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. Univ Rome, Fac Ingn, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Scuola Normale Super Pisa, Pisa, Italy. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Starodumov, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cerci, S.] Adiyaman Univ, Adiyaman, Turkey. Mersin Univ, Mersin, Turkey. Cag Univ, Mersin, Turkey. Piri Reis Univ, Istanbul, Turkey. Gaziosmanpasa Univ, Tokat, Turkey. Ozyegin Univ, Istanbul, Turkey. Izmir Inst Technol, Izmir, Turkey. Mimar Sinan Univ, Istanbul, Turkey. Marmara Univ, Istanbul, Turkey. Kafkas Univ, Kars, Turkey. Yildiz Tekn Univ, Istanbul, Turkey. Hacettepe Univ, Ankara, Turkey. Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. Utah Valley Univ, Orem, UT USA. Vinca Inst Nucl Sci, Belgrade, Serbia. Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. Erzincan Univ, Erzincan, Turkey. Texas A&M Univ Qatar, Doha, Qatar. Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Dudko, Lev/D-7127-2012; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; Konecki, Marcin/G-4164-2015; Novaes, Sergio/D-3532-2012; Dubinin, Mikhail/I-3942-2016; TUVE', Cristina/P-3933-2015; Tinoco Mendes, Andre David/D-4314-2011; Lokhtin, Igor/D-7004-2012; Della Ricca, Giuseppe/B-6826-2013; Azarkin, Maxim/N-2578-2015; VARDARLI, Fuat Ilkehan/B-6360-2013; Chinellato, Jose Augusto/I-7972-2012; Manganote, Edmilson/K-8251-2013; Tomei, Thiago/E-7091-2012 OI Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Androsov, Konstantin/0000-0003-2694-6542; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Novaes, Sergio/0000-0003-0471-8549; Dubinin, Mikhail/0000-0002-7766-7175; TUVE', Cristina/0000-0003-0739-3153; Tinoco Mendes, Andre David/0000-0001-5854-7699; Della Ricca, Giuseppe/0000-0003-2831-6982; Chinellato, Jose Augusto/0000-0002-3240-6270; Tomei, Thiago/0000-0002-1809-5226 FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; Brazilian Funding Agency (CNPq); Brazilian Funding Agency (CAPES); Brazilian Funding Agency (FAPERJ); Brazilian Funding Agency (FAPESP); Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research, Estonia; Estonian Research Council, Estonia [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules / CNRS, France; Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; Bundesministerium fur Bildung und Forschung, Germany; Deutsche Forschungsgemeinschaft, Germany; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, Hungary; National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, Republic of Korea; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education (Malaysia); University of Malaya (Malaysia); Mexican Funding Agency (CINVESTAV); Mexican Funding Agency (CONACYT); Mexican Funding Agency (SEP); Mexican Funding Agency (UASLP-FAI); Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; Swiss Funding Agency (ETH Board); Swiss Funding Agency (ETH Zurich); Swiss Funding Agency (PSI); Swiss Funding Agency (SNF); Swiss Funding Agency (UniZH); Swiss Funding Agency (Canton Zurich); Swiss Funding Agency (SER); Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine, Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, U.K.; US Department of Energy; US National Science Foundation; Marie-Curie programme (European Union); European Research Council (European Union); EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science; European Union, Regional Development Fund; OPUS programme of the National Science Center (Poland); Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR project (Italy) [20108T4XTM]; Thalis programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Welch Foundation [C-1845]; Institute for the Promotion of Teaching Science and Technology of Thailand; Finnish Ministry of Education and Culture; Ministry of Science and Technology FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules / CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives / CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, U.K.; the US Department of Energy, and the US National Science Foundation.; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Center (Poland); the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, contract C-1845. NR 63 TC 1 Z9 1 U1 15 U2 39 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 17 PY 2016 IS 3 AR 125 DI 10.1007/JHEP03(2016)125 PG 54 WC Physics, Particles & Fields SC Physics GA DH9HU UT WOS:000373107900001 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyka, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexab, C Alexander, G Alexopoulos, T Alhroob, M Alimontia, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P 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Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for charged Higgs bosons in the H-+/- -> tb decay channel in pp collisions at root s=8 TeV using the ATLAS detector SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron scattering; Higgs physics ID NEUTRINO MASSES; MONTE-CARLO; TOP-PAIR; PARTON DISTRIBUTIONS; HADRON COLLIDERS; CROSS-SECTION; PLUS PLUS; LHC; SUPERSYMMETRY; PHYSICS AB Charged Higgs bosons heavier than the top quark and decaying via H-+/- -> tb are searched for in proton-proton collisions measured with the ATLAS experiment at root s = 8 TeV corresponding to an integrated luminosity of 20.3 fb(-1). The production of a charged Higgs boson in association with a top quark, gb -> tH(+/-), is explored in the mass range 200 to 600 GeV using multi-jet final states with one electron or muon. In order to separate the signal from the Standard Model background, analysis techniques combining several kinematic variables are employed. An excess of events above the background only hypothesis is observed across a wide mass range, amounting to up to 2.4 standard deviations. Upper limits are set on the gb -> tH(+/-) production cross section times the branching fraction BR(H-+/- -> tb). Additionally, the complementary s-channel production, qq' -> H-+/-, is investigated through a reinterpretation of W' -> tb searches in ATLAS. Final states with one electron or muon are relevant for H-+/- masses from 0.4 to 2.0 TeV, whereas the all-hadronic final state covers the range 1.5 to 3.0 TeV. 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M.; Carter, J. R.; Chapman, J. D.; Cottin, G.; French, S. T.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Potter, C. J.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Tarrade, F.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON K1S 5B6, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Diihrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feng, E. J.; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Gillberg, D.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gurnpert, C.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jaeke, M. R.; Jakobsen, S.; Jenni, P.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Macina, D.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; Milic, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Prasad, S.; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Solans, C. A.; Spigo, G.; Staerz, S.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Tsarouchas, C.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Andeen, T.; Anderson, K. J.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Alameda 340, Santiago, Chile. [Brooks, W. K.; Pezoa, R.; Prokoshin, F.; Salazar Loyola, J. E.; Tapia Araya, S.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Fang, Y.; Jin, S.; Lou, X.; Ma, L. L.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Har, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Li, L.; Li, Y.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Chen, L.; Du, Y.; Feng, C.; Liu, B.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreui, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreui, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreui, E.; Gilles, G.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] IN2P3, CNRS, Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Nikiforou, N.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Lab Nazl Frascati, INFN Grp Collegato Cosenza, Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyka, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flasche, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Borroni, S.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flasche, N.; Glazov, A.; Gregor, I. M.; Grohsjean, A.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Petit, E.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Wang, J.; Yildirim, E.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Rudolph, C.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Amoroso, S.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buscher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mahboubi, K.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; von Radziewski, H.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Nessi, M.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Tykhonov, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gu, U.; Knue, A.; Morton, A.; Mullen, P.; O'Shea, V.; Barrera, C. Oropeza; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareern, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Monini, C.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS, IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Catastini, P.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Spearman, W. R.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E-E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Philosophenweg 12, Heidelberg, Germany. [Colombo, T.; Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Pre, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] Joint Inst Nucl Res Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegarni, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamada, M.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Maddocks, H. J.; Muenstermann, D.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kerevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kerevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Goddard, J. R.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Vannucci, F.; Varouchas, D.; Yap, Y. C.] IN2P3, CNRS, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buscher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Erte, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Barnes, S. L.; Cox, B. E.; Da Via, C.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Joshi, K. D.; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Chen, L.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Feligioni, L.; Gao, J.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Zhang, R.] IN2P3, CNRS, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Picazio, A.; Pueschel, E.; Ventura, D.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Geng, C.; Goldfarb, S.; Guan, L.; Guo, Y.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Linnemann, J. T.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Tollefson, K.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimontia, G.; Andreazza, A.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Perini, L.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Manzoni, S.; Mazza, S. M.; Perini, L.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Phys Inst, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Taylor, F. E.] MIT, Dept Phys, Cambridge, MA 02139 USA. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Tikhomirov, V. O.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Vladoiu, D.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagell, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richterl, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst Phys, Max Planck Inst Phys, Munich, Germany. [Fusayasul, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi 4648601, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; De Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelovl, I.; Hoeferkamp, M. R.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galeal, C.; Koenig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bassalat, A.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkinal, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedtl, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subatom Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkinal, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedtl, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakrabortyl, D.; Cole, S.; Saha, P.; Yurkewicz, A.] No Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Pignotti, D. T.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Saleem, M.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hama, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Ayoub, M. K.; Bassalat, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Grivaz, J-F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Li, Y.; Lounis, A.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Scifo, E.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris Saclay, Univ Paris 11, LAL, CNRS,IN2P3, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Okamura, W.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feig, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlic, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hal, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Lewis, A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L.; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, I-27100 Pavia, Italy. [Amorim, A.; Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejba, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Jakubek, J.; Kohout, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Solc, J.; Sopczak, A.; Sopko, B.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Davies, E.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Monzani, S.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] INFN Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Monzani, S.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] INFN Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, Lphea Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Calandri, A.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Maiani, C.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Peyaud, A.; Protopapadaki, E.; Royon, C. R.; Sairnpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] Commissariat Energie Atom & Energies Alternat, CEA Saclay, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; La Rosa, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Paganis, E.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Nei, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazeka, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Hsu, C.; Lee, C. A.; Garcia, B. R. Mellado; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Aurousseau, M.; Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; March, L.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Wallangen, V.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finei, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Pate, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.; Zhang, G.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Cheatham, S.; Di Mattia, A.; Gozani, E.; Kopeliansky, R.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Cohen, H.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.; Tsionou, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Nagai, R.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Koutsman, A.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Urban, S. Cabrera; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Tries Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Tries Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Tries Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Tries Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Urban, S. Cabrera; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Tries Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Perez Garcia-Estan, M. T.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. 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M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou 510275, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur 59100, Malaysia. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), IN2P3, CNRS, Marseille, France. RI Nechaeva, Polina/N-1148-2015; Mashinistov, Ruslan/M-8356-2015; Vykydal, Zdenek/H-6426-2016; Fedin, Oleg/H-6753-2016; Guo, Jun/O-5202-2015; Ventura, Andrea/A-9544-2015; Kantserov, Vadim/M-9761-2015; Mitsou, Vasiliki/D-1967-2009; Villa, Mauro/C-9883-2009; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Ippolito, Valerio/L-1435-2016; Smirnova, Oxana/A-4401-2013; Gladilin, Leonid/B-5226-2011; Carvalho, Joao/M-4060-2013; Chekulaev, Sergey/O-1145-2015; Livan, Michele/D-7531-2012; Tikhomirov, Vladimir/M-6194-2015; White, Ryan/E-2979-2015; Zhukov, Konstantin/M-6027-2015; SULIN, VLADIMIR/N-2793-2015; Warburton, Andreas/N-8028-2013; Snesarev, Andrey/H-5090-2013; Brooks, William/C-8636-2013; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Di Domenico, Antonio/G-6301-2011; Maleev, Victor/R-4140-2016; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Owen, Mark/Q-8268-2016; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015 OI Mashinistov, Ruslan/0000-0001-7925-4676; Vykydal, Zdenek/0000-0003-2329-0672; Guo, Jun/0000-0001-8125-9433; Ventura, Andrea/0000-0002-3368-3413; Kantserov, Vadim/0000-0001-8255-416X; Mitsou, Vasiliki/0000-0002-1533-8886; Villa, Mauro/0000-0002-9181-8048; Vanadia, Marco/0000-0003-2684-276X; Ippolito, Valerio/0000-0001-5126-1620; Smirnova, Oxana/0000-0003-2517-531X; Gladilin, Leonid/0000-0001-9422-8636; Carvalho, Joao/0000-0002-3015-7821; Livan, Michele/0000-0002-5877-0062; Tikhomirov, Vladimir/0000-0002-9634-0581; White, Ryan/0000-0003-3589-5900; SULIN, VLADIMIR/0000-0003-3943-2495; Warburton, Andreas/0000-0002-2298-7315; Brooks, William/0000-0001-6161-3570; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Di Domenico, Antonio/0000-0001-8078-2759; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Owen, Mark/0000-0001-6820-0488; Fabbri, Laura/0000-0002-4002-8353; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, China; Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon 2020, European Union; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. NR 112 TC 7 Z9 7 U1 17 U2 44 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 17 PY 2016 IS 3 AR 127 DI 10.1007/JHEP03(2016)127 PG 48 WC Physics, Particles & Fields SC Physics GA DH9RJ UT WOS:000373133100001 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Eroe, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S De Klundert, MV Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Brun, H Caillol, C Clerbaux, B De Lentdecker, G Fasanella, G Favart, L Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-Conde, A Seva, T Velde, CV Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L Da Silveira, GG Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Musich, M Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, FL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Herrera, CM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Abdelalim, AA Awad, A Mahrous, A Mohammed, Y Radi, A Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Antropov, I Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Dahms, T Davignon, O Filipovic, N de Cassagnac, RG Jo, M Lisniak, S Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Pigard, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Bernet, C Boudoul, G Bouvier, E Montoya, CAC Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Lagarde, F Laktineh, IB Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Donckt, MV Verdier, P Viret, S Toriashvili, T Lomidze, D Autermann, C Beranek, S Edelhoff, M Feld, L Heister, A Kiesel, MK Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Schael, S Schulte, JF Verlage, T Weber, H Wittmer, B Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Scheuch, F Sonnenschein, L Teyssier, D Thuer, S Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Hoehle, F Kargoll, B Kress, T Kuessel, Y Kunsken, A Lingemann, J Nehrkorn, A Nowack, A Nugent, IM Pistone, C Pooth, O Stahl, A Martin, MA 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Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Event generator tunes obtained from underlying event and multiparton scattering measurements SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID DOUBLE PARTON SCATTERING; CROSS-SECTIONS; PYTHIA; COLLISIONS AB New sets of parameters ("tunes")for the underlying-event (UE) modelling of the PYTHIA8, PYTHIA6 and HERWIG++ MonteCarlo event generators are constructed using different parton distribution functions. Combined fits to CMS UE proton-proton (pp) data at root s = 7 TeV and to UE proton-antiproton (p (P) over bar) data from the CDF experiment at lower root s, are used to study the UE models and constrain their parameters, providing thereby improved predictions for proton-proton collisions at 13 TeV. In addition, it is investigated whether the values of the parameters obtained from fits to UE observables are consistent with the values determined from fitting observables sensitive to double-parton scattering processes. Finally, comparisons are presented of the UE tunes to "minimum bias" (MB) events, multijet, and Drell-Yan (q (Q) over bar -> Z/gamma* -> lepton-antilepton+jets) observables at 7 and 8 TeV, as well as predictions for MB and UE observables at 13 TeV. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Friese, R.; Giffels, M.; Gilbert, A.; Haitz, D.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Sieber, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Williamson, S.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, Inst Nucl & Particle Phys, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.; Sphicas, P.] Univ Athens, Athens, Greece. 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[Cappello, G.; Chiorboli, M.; Costa, S.; Di Mattia, A.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, Via Celoria 16, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.; Thyssen, F.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Fantinel, S.; Fanzago, F.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Awad, A.; Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.; Di Marco, E.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.; Di Marco, E.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.] Ist Nazl Fis Nucl, Sez Torino, Turin, Torino, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Torino, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Lee, S.; Kim, H.; Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Kim, H.; Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Linares, E. Casimiro; Castilla-Valdez, H.; De la Cruz-Burelo, E.; Heredia-De la Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, M.; Ahmad, A.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Da Cruz E Silva, C. Beirao; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M.; Finger, M., Jr.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Matveev, V.; Bylinkin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Cirkovic, P.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, P.; Cirkovic, P.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Maestre, J. Alcaraz; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De la Cruz, B.; Delgado Peris, A.; Del Valle, A. Escalante; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; De Martino, E. Navarro; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.] CIEMAT, E-28040 Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Merlin, J. A.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Szillasi, Z.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Tosi, N.; Viliani, L.; Primavera, F.; Manzoni, R. A.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Pazzini, J.; Zucchetta, A.; Ciangottini, D.; Azzurri, P.; Donato, S.; D'imperio, G.; Del Re, D.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duggan, D.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Cerci, S.; Ozdemir, K.; Polatoz, A.; Cerci, D. Sunar; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Guelmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Newbold, D. M.; Bell, K. W.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Bhattacharya, S.; Alimena, J.; Berry, E.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Chauhan, S.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Funk, G.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Bravo, C.; Cousins, R.; Everaerts, P.; Farrell, C.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Schnaible, C.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Incandela, J. Gran J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Banerjee, S.; Abdullin, S.; Albrow, M.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Gleyzer, S. V.; Hugon, J.; Konigsberg, J.; Korytov, A.; Kotov, K.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Chicago, Chicago, IL 60637 USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Roskes, J.; Sady, A.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Wang, J.; Apyan, A.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.; Barberis, E.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Saka, H.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Tan, P.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Hernandez, A. Castaneda; Celik, A.; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Huang, T.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Melo, A.; Ni, H.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sinthuprasith, T.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Sharma, A.; Levin, A.; Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI 53706 USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Abdelalim, A. A.; Mahrous, A.] Helwan Univ, Cairo, Egypt. [Abdelalim, A. A.] Zewail City Sci & Technol, Zewail, Egypt. [Mohammed, Y.] Fayoum Univ, Al Fayyum, Egypt. [Radi, A.] British Univ Egypt, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Choudhury, S.] Indian Inst Sci Educ & Res Bhopal, Bhopal 462066, India. [Hempel, M.; Karacheban, O.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] Agensi Nuklear Malaysia, MOSTI, Kajang, Malaysia. [Heredia-De la Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Scuola Normale, Pisa, Italy. [Rolandi, G.] Sezione Ist Nazl Fis Nucl, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, S.; Cerci, D. Sunar] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ Qatar, Doha, Qatar. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. EM cms-publication-committee-chair@cern.ch RI Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; TUVE', Cristina/P-3933-2015; Tomei, Thiago/E-7091-2012; Dubinin, Mikhail/I-3942-2016; Tinoco Mendes, Andre David/D-4314-2011; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Stahl, Achim/E-8846-2011; Da Silveira, Gustavo Gil/N-7279-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Manganote, Edmilson/K-8251-2013; Lokhtin, Igor/D-7004-2012; Andreev, Vladimir/M-8665-2015; Chinellato, Jose Augusto/I-7972-2012; Perez-Calero Yzquierdo, Antonio/F-2235-2013; Novaes, Sergio/D-3532-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Della Ricca, Giuseppe/B-6826-2013; Dudko, Lev/D-7127-2012; Montanari, Alessandro/J-2420-2012; Azarkin, Maxim/N-2578-2015; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012 OI ORTONA, Giacomo/0000-0001-8411-2971; Gallinaro, Michele/0000-0003-1261-2277; Chapon, Emilien/0000-0001-6968-9828; Reis, Thomas/0000-0003-3703-6624; Luukka, Panja/0000-0003-2340-4641; Jacob, Jeson/0000-0001-6895-5493; Androsov, Konstantin/0000-0003-2694-6542; Saka, Halil/0000-0001-7616-2573; Brianza, Luca/0000-0001-5770-6037; Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; TUVE', Cristina/0000-0003-0739-3153; HSIUNG, YEE/0000-0003-4801-1238; Tomei, Thiago/0000-0002-1809-5226; Dubinin, Mikhail/0000-0002-7766-7175; Tinoco Mendes, Andre David/0000-0001-5854-7699; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Stahl, Achim/0000-0002-8369-7506; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Chinellato, Jose Augusto/0000-0002-3240-6270; Perez-Calero Yzquierdo, Antonio/0000-0003-3036-7965; Novaes, Sergio/0000-0003-0471-8549; Della Ricca, Giuseppe/0000-0003-2831-6982; Dudko, Lev/0000-0002-4462-3192; Montanari, Alessandro/0000-0003-2748-6373; Mundim, Luiz/0000-0001-9964-7805; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Ruiz, Alberto/0000-0002-3639-0368; FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research; Estonian Research Council [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Innovation Office, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education, and University of Malaya (Malaysia); CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science; European Union, Regional Development Fund; OPUS programme of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR project (Italy) [20108T4XTM]; Thalis programme; Aristeia programme; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; r Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation. Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; r Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, contract C-1845. NR 39 TC 4 Z9 4 U1 18 U2 51 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAR 17 PY 2016 VL 76 IS 3 AR 155 DI 10.1140/epjc/s10052-016-3988-x PG 52 WC Physics, Particles & Fields SC Physics GA DH1UP UT WOS:000372570700001 ER PT J AU Shokri, A Wang, XB Wang, YP O'Doherty, GA Kass, SR AF Shokri, Alireza Wang, Xue-Bin Wang, Yanping O'Doherty, George A. Kass, Steven R. TI Flexible Acyclic Polyol-Chloride Anion Complexes and Their Characterization by Photoelectron Spectroscopy and Variable Temperature Binding Constant Determinations SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID ENTHALPY-ENTROPY COMPENSATION; INTRAMOLECULAR COULOMB REPULSION; MULTIPLE HYDROGEN-BONDS; MOLECULAR RECOGNITION; DENSITY FUNCTIONALS; NONCOVALENT INTERACTIONS; CALORIMETRIC TITRATION; INCLUSION COMPLEXATION; RECEPTORS; CHANNEL AB Flexible acyclic alcohols with one to five hydroxyl groups were bound to a chloride anion and these complexes were interrogated by negative ion photoelectron spectroscopy and companion density functional theory computations. The resulting vertical detachment energies are reproduced on average to 0.10 eV by M06-2X/aug-cc-pVTZ predictions and range from 4.45-5.96 eV. These values are 0.84-2.35 eV larger than the adiabatic detachment energy of Cl- as a result of the larger hydrogen bond networks in the bigger polyols. Adiabatic detachment energies of the alcohol-Cl- clusters are more difficult to determine both experimentally and computationally. This is due to the large geometry changes that occur upon photodetachment and the large bond dissociation energy of H-Cl which enables the resulting chlorine atom to abstract a hydrogen from any of the methylene (CH2) or methine (CH) positions. Both ionic and nonionic hydrogen bonds (i.e., OH center dot center dot center dot Cl- and OH center dot center dot center dot OH center dot center dot center dot Cl-) form in the larger polyols complexes and are found to be energetically comparable. Subtle structural differences, consequently can lead to the formation of different types of hydrogen bonds, and maximizing the ionic ones is not always preferred. Solution equilibrium binding constants between the alcohols and tetrabutylammonium chloride (TBACl) in acetonitrile at -24.2, +22.0, and +53.6 degrees C were also determined. The free energies of association are nearly identical for all of the substrates (i.e., Delta G degrees = -2.8 +/- 0.7 kcal mol(-1)). Compensating enthalpy and entropy values reveal, contrary to expectation and the intrinsic gas-phase preferences, that the bigger systems with more hydroxyl groups are entropically favored and enthalpically disfavored relative to the smaller species. This suggests that more solvent molecules are released upon binding TBACl to alcohols with more hydroxyl groups and is consistent with the measured negative heat capacities. These quantities increase with molecular complexity of the substrate, however, contrary to common interpretation of these values. C1 [Shokri, Alireza; Kass, Steven R.] Univ Minnesota, Dept Chem, 207 Pleasant St SE, Minneapolis, MN 55455 USA. [Wang, Xue-Bin] Pacific NW Natl Lab, Div Phys Sci, POB 999,MS K8-88, Richland, WA 99352 USA. [Wang, Yanping; O'Doherty, George A.] Northeastern Univ, Dept Chem & Chem Biol, Boston, MA 02115 USA. RP Kass, SR (reprint author), Univ Minnesota, Dept Chem, 207 Pleasant St SE, Minneapolis, MN 55455 USA.; Wang, XB (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999,MS K8-88, Richland, WA 99352 USA. EM xuebin.wang@pnnl.gov; kass@umn.edu FU National Science Foundation [CHE-1111678, 1361766]; Minnesota Supercomputer Institute for Advanced Computational Research; U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences; DOE's Office of Biological and Environmental Research FX Generous support from the National Science Foundation (CHE-1111678 and 1361766) and the Minnesota Supercomputer Institute for Advanced Computational Research are gratefully acknowledged. The photoelectron spectra work was supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences, and was performed at the EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is operated by Battelle for DOE. NR 62 TC 1 Z9 1 U1 3 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAR 17 PY 2016 VL 120 IS 10 BP 1661 EP 1668 DI 10.1021/acs.jpca.5b12286 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DH1RI UT WOS:000372562200004 PM 26909527 ER PT J AU Muller, G Scheer, A Osborn, DL Taatjes, CA Meloni, G AF Muller, Giel Scheer, Adam Osborn, David L. Taatjes, Craig A. Meloni, Giovanni TI Low Temperature Chlorine-Initiated Oxidation of Small-Chain Methyl Esters: Quantification of Chain-Terminating HO2-Elimination Channels SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID CHEMICAL KINETIC MECHANISM; SET MODEL CHEMISTRY; PHOTOIONIZATION MASS-SPECTROMETRY; DENSITY-FUNCTIONAL THEORIES; DIESEL FUEL SURROGATE; COMBUSTION CHEMISTRY; SYNCHROTRON-PHOTOIONIZATION; HYDROCARBON AUTOIGNITION; OIL BIODIESEL; ENGINE AB Cl-initiated oxidation reactions of three small-chain methyl esters, methyl propanoate (CH3CH2COOCH3; MP), methyl butanoate (CH3CH2CH2COOCH3; MB), and methyl valerate (CH3CH2CH2CH2COOCH3; MV), are studied at 1 or 8 Torr and 550 and 650 K. Products are monitored as a function of mass, time, and photoionization energy using multiplexed photoionization mass spectrometry coupled to tunable synchrotron photoionization radiation. Pulsed photolysis of molecular chlorine is the source of Cl radicals, which remove an H atom from the ester, forming a free radical. In each case, after addition of O-2 to the initial radicals, chain-terminating HO2-elimination reactions are observed to be important. Branching ratios among competing HO2-elimination channels are determined via absolute photoionization spectra of the unsaturated methyl ester coproducts. At 550 K, HO2-elimination is observed to be selective, resulting in nearly exclusive production of the conjugated methyl ester coproducts, methyl propenoate, methyl-2-butenoate, and methyl-2-pentenoate, respectively. However, in MV, upon raising the temperature to 650 K, other HO2-elimination pathways are observed that yield methyl-3-pentenoate and methyl-4-pentenoate. In each methyl ester oxidation reaction, a peak is observed at a mass consistent with cyclic ether formation, indicating chain-propagating OH loss/ring formation pathways via QOOH intermediates. Evidence is observed for the participation of resonance-stabilized QOOH in the most prominent cyclic ether pathways. Stationary point energies for HO2-elimination pathways and select cyclic ether formation channels are calculated at the CBS-QB3 level of theory and assist in the assignment of reaction pathways and final products. C1 [Muller, Giel; Meloni, Giovanni] Univ San Francisco, San Francisco, CA 94117 USA. [Scheer, Adam] Pacific Gas & Elect Co, 245 Market St, San Francisco, CA 94111 USA. [Osborn, David L.; Taatjes, Craig A.] Sandia Natl Labs, Livermore, CA 94551 USA. RP Meloni, G (reprint author), Univ San Francisco, San Francisco, CA 94117 USA.; Taatjes, CA (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM cataatj@sandia.gov; gmeloni@usfca.edu FU University of San Francisco Faculty Development Fund; Laboratory Directed Research and Development program at Sandia National Laboratories; United States Department of Energy (USDOE)'s National Nuclear Security Administration [DEAC04-94AL85000]; Division of Chemical Sciences, Geosciences, and Biosciences; Office of Basic Energy Sciences (BES), USDOE; Lawrence Berkeley National Laboratory [DE-AC02- 05CH11231]; USDOE [DE-AC02- 05CH11231] FX We thank Mr. Howard Johnsen and Mr. Kendrew Au for technical support of these experiments. Additional thanks is given to professors Claire Castro and William Karney for their support and use of the USF chemistry cluster. This work is supported by the University of San Francisco Faculty Development Fund, as well as the Laboratory Directed Research and Development program at Sandia National Laboratories, a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy (USDOE)'s National Nuclear Security Administration under contract DEAC04-94AL85000. The development of the experimental apparatus and the participation of DLO were supported by the Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences (BES), USDOE. The Advanced Light Source is supported by the Director, Office of Science, BES/USDOE, under contract DE-AC02- 05CH11231 between Lawrence Berkeley National Laboratory and the USDOE. This research used resources of the Advanced Light Source of Lawrence Berkeley National Laboratory, which is a USDOE Office of Science User Facility. NR 66 TC 1 Z9 1 U1 5 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAR 17 PY 2016 VL 120 IS 10 BP 1677 EP 1690 DI 10.1021/acs.jpca.6b00148 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DH1RI UT WOS:000372562200006 PM 26910881 ER PT J AU Pelliccione, CJ Timofeeva, EV Segre, CU AF Pelliccione, Christopher J. Timofeeva, Elena V. Segre, Carlo U. TI Potential-Resolved In Situ X-ray Absorption Spectroscopy Study of Sn and SnO2 Nanomaterial Anodes for Lithium-Ion Batteries SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID REACTION-MECHANISM; CRYSTAL-STRUCTURE; TIN OXIDE; ELECTRODES; CAPACITY; XAFS; INTERCALATION; DIFFRACTION; IFEFFIT; INSIGHT AB This work provides detailed analysis of processes occurring in metallic Sn and SnO2 anode materials for lithium ion batteries during first lithiation, studied in situ with rapid continuous X-ray absorption spectroscopy (XAS). The X-ray absorption near edge structure (XANES) and extended X-ray absorption fine structure (EXAFS) spectra provide information on dynamic changes in the Sn atomic environment, including type and number of neighboring atoms and interatomic distances. A unique methodology was used to model insertion of Li atoms into the electrode material structure and to analyze the formation of SnLi phases within the electrodes. Additionally, analysis of fully lithiated and delithiated states of Sn and SnO2 electrodes in the first two cycles provides insight into the reasons for poor electrochemical performance and rapid capacity decline. Results indicate that use of SnO2 is more promising than metallic Sn as an anode material, but more effort in nanoscale and atomic engineering of anodes is required for commercially feasible use of Sn-based materials. C1 [Pelliccione, Christopher J.; Segre, Carlo U.] IIT, Dept Phys, 3101 S Dearborn St, Chicago, IL 60616 USA. [Pelliccione, Christopher J.; Segre, Carlo U.] IIT, CSRRI, 3101 S Dearborn St, Chicago, IL 60616 USA. [Timofeeva, Elena V.] Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Pelliccione, CJ (reprint author), IIT, Dept Phys, 3101 S Dearborn St, Chicago, IL 60616 USA.; Pelliccione, CJ (reprint author), IIT, CSRRI, 3101 S Dearborn St, Chicago, IL 60616 USA. EM cpellic1@hawk.iit.edu; segre@iit.edu RI Segre, Carlo/B-1548-2009; ID, MRCAT/G-7586-2011; OI Segre, Carlo/0000-0001-7664-1574; Timofeeva, Elena V./0000-0001-7839-2727 FU Department of Education GAANN Fellowship [P200A090137]; U.S. Department of Energy, Office of Basic Energy Science; Advanced Research Project Agency Energy (ARPA-E) [AR-000387]; Department of Energy; MRCAT member institutions; U.S. Department of Energy [DE-AC02-06CH11357] FX C.J.P. was supported by a Department of Education GAANN Fellowship, award no. P200A090137. The project is supported by the U.S. Department of Energy, Office of Basic Energy Science and the Advanced Research Project Agency Energy (ARPA-E) under Award no. AR-000387. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. Use of the Argonne National Laboratory Advanced Photon Source is supported by the U.S. Department of Energy, under Contract no. DE-AC02-06CH11357. NR 37 TC 6 Z9 6 U1 20 U2 56 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 17 PY 2016 VL 120 IS 10 BP 5331 EP 5339 DI 10.1021/acs.jpcc.5b12279 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH1QY UT WOS:000372561200008 ER PT J AU Pham, VH Dickerson, JH AF Viet Hung Pham Dickerson, James H. TI Reduced Graphene Oxide Hydrogels Deposited in Nickel Foam for Supercapacitor Applications: Toward High Volumetric Capacitance SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID HIGH-PERFORMANCE SUPERCAPACITORS; ELECTROCHEMICAL CAPACITORS; ENERGY-STORAGE; REDUCTION; FILMS; DISPERSIONS; FABRICATION; RESTACKING; PREVENTION; FRAMEWORKS AB Graphene hydrogels have been considered as ideal materials for high-performance supercapacitors. However, their low volumetric capacitance significantly limits its real application. In this study, we report an environment-friendly and scalable method to prepare high packing density, electrochemically reduced graphene oxide hydrogels (ERGO) for supercapacitor application by the electrophoretic deposition of graphene oxide onto nickel foam, followed by the electrochemical reduction and hydraulic compression of the deposited materials. The as-prepared ERGO on nickel foam was hydraulic compressed up to 20 tons, resulting in an increase of the packing density of ERGO from 0.0098 to 1.32 g cm(-3). Consequently, the volumetric capacitance and volumetric energy density of ERGOs greatly increased from 1.58 F cm(-3) and 0.053 Wh cm(-3) (as-prepared ERGO) to 176.5 F cm(-3) and 6.02 Wh cm(-3) (ERGO compressed at 20 tons), respectively. The ERGOs also exhibited long-term electrochemical stability with a capacitance retention in the range of approximately 79-90% after 10 000 cycles. We believe that these high packing density ERGOs are promising for real-world energy storage devices for which scalable, cost-effective manufacturing is of significance and for which space constraints are paramount. C1 [Viet Hung Pham; Dickerson, James H.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Dickerson, JH (reprint author), Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. EM jdickerson@bnl.gov FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-SC0012704] FX This work was performed at the Center for Functional Nanomaterials, Brookhaven National Laboratory, which is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, under Contract no. DE-SC0012704. NR 33 TC 5 Z9 5 U1 21 U2 78 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 17 PY 2016 VL 120 IS 10 BP 5353 EP 5360 DI 10.1021/acs.jpcc.6b00326 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH1QY UT WOS:000372561200011 ER PT J AU Felts, AC Andrus, MJ Knowles, ES Quintero, PK Ahir, AR Risset, ON Li, CH Maurin, I Halder, GJ Abboud, KA Meisel, MW Talham, DR AF Felts, Ashley C. Andrus, Matthew J. Knowles, Elizabeth S. Quintero, Pedro K. Ahir, Akhil R. Risset, Olivia N. Li, Carissa H. Maurin, Isabelle Halder, Gregory J. Abboud, Khalil A. Meisel, Mark W. Talham, Daniel R. TI Evidence for Interface-Induced Strain and Its Influence on Photomagnetism in Prussian Blue Analogue Core-Shell Heterostructures, RbaCob[Fe(CN)(6)](c)center dot mH(2)O@KjNik[Cr(CN)(6)](l)center dot nH(2)O SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID COORDINATION POLYMER HETEROSTRUCTURE; PHOTOINDUCED FERRIMAGNETIC SYSTEMS; ALKALI CATION; C-I; MAGNETISM; LIGHT; MAGNETIZATION; NANOPARTICLES; TEMPERATURE; PARTICLES AB A series of photomagnetic coordination polymer core-shell heterostructures, based on the light-switchable Prussian blue analogue RbaCob[Fe(CN)(6)](c)center dot mH(2)O (RbCoFe-PBA) as the core and the ferromagnetic KjNik[Cr(CN)(6)](l)center dot nH(2)O (KNiCr-PBA) as the shell, was studied using powder X-ray diffraction, down to 100 K, and magnetometry, down to 2 K, to investigate the influence of the shell thickness on light-induced magnetization changes and gain insight into the mechanism. The core material is known to undergo a charge-transfer induced spin transition (CTIST), and synchrotron powder diffraction was used to monitor structural changes in both the core and the shell associated with the thermally and optically induced CTIST of the core. Significant lattice contraction in the RbCoFe-PBA core upon cooling through the high-spin to the low-spin state transition near similar to 260 K induces strain on the KNiCr-PBA shells. This lattice strain in the shell can be relieved either by thermal cycling back to high temperature or by using light to access the metastable high-spin state of the core at low temperature. The different extents of strain in the KNiCr-PBA shell are reflected in low-temperature, low-field magnetization versus temperature data in the light and dark states. A broader magnetic transition at T-c approximate to 70 K in the dark state relative to the light state reflects the greater dispersion of nearest-neighbor contacts and exchange energies induced by the structural distortions of the strained state. Analyses for different shell thicknesses, coupled with high-field magnetization data, support a mechanism whereby the light-induced magnetization changes in the KNiCr-PBA shell are due to realignment of the local magnetic anisotropy as a result of the structural changes in the shell associated with the optical CTIST of the core. Through magnetization and structural analyses, the depth to which the properties of the shell are influenced by the core-shell architecture was estimated to be between 40 and 50 nm. C1 [Felts, Ashley C.; Andrus, Matthew J.; Ahir, Akhil R.; Risset, Olivia N.; Li, Carissa H.; Abboud, Khalil A.; Talham, Daniel R.] Univ Florida, Dept Chem, Gainesville, FL 32611 USA. [Knowles, Elizabeth S.; Quintero, Pedro K.; Meisel, Mark W.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Knowles, Elizabeth S.; Quintero, Pedro K.; Meisel, Mark W.] Univ Florida, Natl High Magnet Field Lab, Gainesville, FL 32611 USA. [Maurin, Isabelle] Ecole Polytech, CNRS, UMR 7643, Phys Mat Condensee, F-91128 Palaiseau, France. [Halder, Gregory J.] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Talham, DR (reprint author), Univ Florida, Dept Chem, Gainesville, FL 32611 USA.; Meisel, MW (reprint author), Univ Florida, Dept Phys, Gainesville, FL 32611 USA.; Meisel, MW (reprint author), Univ Florida, Natl High Magnet Field Lab, Gainesville, FL 32611 USA. EM meisel@phys.ufl.edu; talham@chem.ufl.edu FU National Science Foundation [DMR-1005581, DMR-1405439, DMR-1202033, DMR-1157490]; State of Florida; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX This work was supported by the National Science Foundation through Grants DMR-1005581 and DMR-1405439 (D.R.T.), DMR-1202033 (M.W.M.), and DMR-1157490 (National High Magnetic Field Laboratory, NHMFL) and the State of Florida. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract DE-AC02-06CH11357. We thank K.A.A. for use of the Bruker DUO diffractometer for screening PXRD experiments and Mr. John Cain for his help with the magnetometry measurements. NR 47 TC 2 Z9 2 U1 18 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 17 PY 2016 VL 120 IS 10 BP 5420 EP 5429 DI 10.1021/acs.jpcc.5b10761 PG 10 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH1QY UT WOS:000372561200018 ER PT J AU Estes, SL Antonio, MR Soderholm, L AF Estes, Shanna L. Antonio, Mark R. Soderholm, L. TI Tetravalent Ce in the Nitrate-Decorated Hexanuclear Cluster [Ce-6(mu(3)-O)(4)(mu(3)-OH)(4)](12+): A Structural End Point for Ceria Nanoparticles SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID OXIDE NANOPARTICLES; AQUEOUS-SOLUTION; NITRIC-ACID; HYDROLYSIS PRODUCTS; CYCLIC VOLTAMMETRY; LATTICE EXPANSION; CRYSTAL-STRUCTURE; CHEMISTRY; COMPLEXES; SIZE AB We describe the synthesis and characterization of three glycine-stabilized hexanuclear Cely cluster compounds, each containing the [Ce-6(mu(3)-O)(4)(mu(3)-OH)(4)](12+) core structure. Crystallized from aqueous nitrate solutions with pH < 0, the core cluster structures exhibit variable decoration by nitrate, glycine, and water ligands depending on solution conditions, where increased nitrate and glycine decoration of the cluster core was observed for crystals synthesized at high Ce and nitrate concentrations. No other crystalline products were observed using this synthetic route. In addition to confirming the tetravalent oxidation state of cerium in one of the reported clusters, cyclic voltammetry also indicates that Ce-IV is reduced at similar to+0.60 V vs Ag/AgCl (3 M NaCl), which is significantly less than the standard electrode potential. This large decrease in the Ce-IV/Ce-III reduction potential suggests that Ce-IV is significantly stabilized relative to Ce-III within the examined cluster. These compounds are discussed in terms of their importance as small, end member, ceric oxide nanoparticles. Single-crystal structural solutions, together with voltammetry and electrolysis data, permit the decoupling of Ce-III defects and substoichiometry. In addition, Ce-Ce distances can be used to determine an "effective" CeO2-x lattice constant, providing a simple method for comparing literature descriptions. The results are discussed in terms of their potential implications for the mechanisms by which nanoparticle ceria serve as catalysts and oxygen-storage materials. C1 [Estes, Shanna L.; Antonio, Mark R.; Soderholm, L.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Soderholm, L (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM LS@anl.gov RI Estes, Shanna/M-2834-2013 OI Estes, Shanna/0000-0002-5210-3365 FU UChicago Argonne, LLC (Argonne National Laboratory); U.S. Department of Energy; BES Heavy Elements Program [DE-AC02-06CH11357] FX The work is supported at UChicago Argonne, LLC (Argonne National Laboratory), by the U.S. Department of Energy, BES Heavy Elements Program under Contract No. DE-AC02-06CH11357. NR 76 TC 4 Z9 4 U1 4 U2 21 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 17 PY 2016 VL 120 IS 10 BP 5810 EP 5818 DI 10.1021/acs.jpcc.6b00644 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DH1QY UT WOS:000372561200060 ER PT J AU Matsuda, M Ye, F Dissanayake, SE Cheng, JG Chi, S Ma, J Zhou, HD Yan, JQ Kasamatsu, S Sugino, O Kato, T Matsubayashi, K Okada, T Uwatoko, Y AF Matsuda, M. Ye, F. Dissanayake, S. E. Cheng, J. -G. Chi, S. Ma, J. Zhou, H. D. Yan, J. -Q. Kasamatsu, S. Sugino, O. Kato, T. Matsubayashi, K. Okada, T. Uwatoko, Y. TI Pressure dependence of the magnetic ground states in MnP SO PHYSICAL REVIEW B LA English DT Article ID PHASE; SUPERCONDUCTIVITY; CRAS AB MnP, a superconductor under pressure, exhibits a ferromagnetic order below T-C similar to 290 K followed by a helical order with the spins lying in the ab plane and the helical rotation propagating along the c axis below T-s similar to 50 K at ambient pressure. We performed single-crystal neutron diffraction experiments to determine the magnetic ground states under pressure. Both T-C and T-s are gradually suppressed with increasing pressure and the helical order disappears at similar to 1.2 GPa. At intermediate pressures of 1.8 and 2.0 GPa, the ferromagnetic order first develops and changes to a conical or two-phase (ferromagnetic and helical) structure with the propagation along the b axis below a characteristic temperature. At 3.8 GPa, a helical magnetic order appears below 208 K, which hosts the spins in the ac plane and the propagation along the b axis. The period of this b axis modulation is shorter than that at 1.8 GPa. Our results indicate that the magnetic phase in the vicinity of the superconducting phase may have a helical magnetic correlation along the b axis. C1 [Matsuda, M.; Ye, F.; Dissanayake, S. E.; Chi, S.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Cheng, J. -G.] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Cheng, J. -G.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Ma, J.; Zhou, H. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Yan, J. -Q.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Yan, J. -Q.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Kasamatsu, S.; Sugino, O.; Kato, T.; Matsubayashi, K.; Okada, T.; Uwatoko, Y.] Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan. [Matsubayashi, K.] Univ Electrocommun, Dept Engn Sci, Grad Sch Informat & Engn, Chofu, Tokyo 1828585, Japan. RP Matsuda, M (reprint author), Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RI Matsuda, Masaaki/A-6902-2016; Ye, Feng/B-3210-2010; SNS, Corelli/O-8443-2015; Kasamatsu, Shusuke/A-7189-2012; Matsubayashi, Kazuyuki/F-7696-2013; Cheng, Jinguang/A-8342-2012; Zhou, Haidong/O-4373-2016; Chi, Songxue/A-6713-2013; Ma, Jie/C-1637-2013; OI Matsuda, Masaaki/0000-0003-2209-9526; Ye, Feng/0000-0001-7477-4648; SNS, Corelli/0000-0001-5563-3292; Chi, Songxue/0000-0002-3851-9153; Dissanayake, Sachith/0000-0002-4703-6516 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; U.S.-Japan Cooperative Program on Neutron Scattering; MOST; NSF of China [2014CB921500, 11574377, 11304371]; Chinese Academy of Sciences [XDB07020100]; NSF [DMR-1350002]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; JSPS KAKENHI [15H03681]; U.S. Department of Energy [DE-AC05-00OR22725] FX We are grateful to Kazuki Komatsu (University of Tokyo) and Yoshihiko Yokoyama (IMR, Tohoku University) for use of the pressure cell. Research conducted at ORNL's HFIR and SNS was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. This study was supported in part by the U.S.-Japan Cooperative Program on Neutron Scattering. J.G.C. is supported by the MOST and NSF of China (Grants No. 2014CB921500, No. 11574377, and No. 11304371), and the Strategic Priority Research Program (B) of the Chinese Academy of Sciences (Grant No. XDB07020100). H.D.Z. acknowledges the support from NSF-DMR-1350002. J.Q.Y. acknowledges the support by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Y.U. was supported by JSPS KAKENHI (Grant No. 15H03681). This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 23 TC 3 Z9 3 U1 13 U2 39 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 17 PY 2016 VL 93 IS 10 AR 100405 DI 10.1103/PhysRevB.93.100405 PG 5 WC Physics, Condensed Matter SC Physics GA DG9MF UT WOS:000372406400001 ER PT J AU Diakaki, M Karadimos, D Vlastou, R Kokkoris, M Demetriou, P Skordis, E Tsinganis, A Abbondanno, U Aerts, G Alvarez, H Alvarez-Velarde, F Andriamonje, S Andrzejewski, J Assimakopoulos, P Audouin, L Badurek, G Baumann, P Becvar, F Berthoumieux, E Calviani, M Calvino, F Cano-Ott, D Capote, R de Albornoz, AC Cennini, P Chepel, V Chiaveri, E Colonna, N Cortes, G Couture, A Cox, J David, S Dolfini, R Domingo-Pardo, C Dorochenko, A Dridi, W Duran, I Eleftheriadis, C Embid-Segura, M Ferrant, L Ferrari, A Ferreira-Marques, R Fitzpatrick, L Frais-Koelbl, H Fuji, K Furman, W Goncalves, I Gallino, R Gonzalez-Romero, E Goverdovski, A Gramegna, F Griesmayer, E Guerrero, C Gunsing, F Haas, B Haight, R Heil, M Herrera-Martinez, A Igashira, M Ioannidis, K Isaev, S Jericha, E Kadi, Y Kappeler, F Karamanis, D Kerveno, M Ketlerov, V Koehler, P Kolokolov, D Konovalov, V Krticka, M Lamboudis, C Leeb, H Lindote, A Lopes, I Lozano, M Lukic, S Marganiec, J Marques, L Marrone, S Massimi, C Mastinu, P Mengoni, A Milazzo, PM Moreau, C Mosconi, M Neves, F Oberhummer, H O'Brien, S Oshima, M Pancin, J Papadopoulos, C Paradela, C Patronis, N Pavlik, A Pavlopoulos, P Perrot, L Plag, R Plompen, A Plukis, A Poch, A Pretel, C Quesada, J Rauscher, T Reifarth, R Rosetti, M Rubbia, C Rudolf, G Rullhusen, P Salgado, J Sarchiapone, L Savvidis, I Sedysheva, M Stamoulis, K Stephan, C Tagliente, G Tain, JL Tassan-Got, L Tavora, L Terlizzi, R Vannini, G Vaz, P Ventura, A Villamarin, D Vincente, MC Vlachoudis, V Voss, F Wendler, H Wiescher, M Wisshak, K AF Diakaki, M. Karadimos, D. Vlastou, R. Kokkoris, M. Demetriou, P. Skordis, E. Tsinganis, A. Abbondanno, U. Aerts, G. Alvarez, H. Alvarez-Velarde, F. Andriamonje, S. Andrzejewski, J. Assimakopoulos, P. Audouin, L. Badurek, G. Baumann, P. Becvar, F. Berthoumieux, E. Calviani, M. Calvino, F. Cano-Ott, D. Capote, R. de Albornoz, A. Carrillo Cennini, P. Chepel, V. Chiaveri, E. Colonna, N. Cortes, G. Couture, A. Cox, J. David, S. Dolfini, R. Domingo-Pardo, C. Dorochenko, A. Dridi, W. Duran, I. Eleftheriadis, Ch. Embid-Segura, M. Ferrant, L. Ferrari, A. Ferreira-Marques, R. Fitzpatrick, L. Frais-Koelbl, H. Fuji, K. Furman, W. Goncalves, I. Gallino, R. Gonzalez-Romero, E. Goverdovski, A. Gramegna, F. Griesmayer, E. Guerrero, C. Gunsing, F. Haas, B. Haight, R. Heil, M. Herrera-Martinez, A. Igashira, M. Ioannidis, K. Isaev, S. Jericha, E. Kadi, Y. Kaeppeler, F. Karamanis, D. Kerveno, M. Ketlerov, V. Koehler, P. Kolokolov, D. Konovalov, V. Krticka, M. Lamboudis, C. Leeb, H. Lindote, A. Lopes, I. Lozano, M. Lukic, S. Marganiec, J. Marques, L. Marrone, S. Massimi, C. Mastinu, P. Mengoni, A. Milazzo, P. M. Moreau, C. Mosconi, M. Neves, F. Oberhummer, H. O'Brien, S. Oshima, M. Pancin, J. Papadopoulos, C. Paradela, C. Patronis, N. Pavlik, A. Pavlopoulos, P. Perrot, L. Plag, R. Plompen, A. Plukis, A. Poch, A. Pretel, C. Quesada, J. Rauscher, T. Reifarth, R. Rosetti, M. Rubbia, C. Rudolf, G. Rullhusen, P. Salgado, J. Sarchiapone, L. Savvidis, I. Sedysheva, M. Stamoulis, K. Stephan, C. Tagliente, G. Tain, J. L. Tassan-Got, L. Tavora, L. Terlizzi, R. Vannini, G. Vaz, P. Ventura, A. Villamarin, D. Vincente, M. C. Vlachoudis, V. Voss, F. Wendler, H. Wiescher, M. Wisshak, K. CA Collaboration, NT TI Neutron-induced fission cross section of Np-237 in the keV to MeV range at the CERN n_TOF facility SO PHYSICAL REVIEW C LA English DT Article ID NUCLEAR-DATA; ACTINIDES; LIBRARY; SCIENCE; EMPIRE; U-235; CODE AB The neutron-induced fission cross section of Np-237 was experimentally determined at the high-resolution and high-intensity facility n_TOF, at CERN, in the energy range 100 keV to 9 MeV, using the U-235(n, f) and U-238(n, f) cross section standards below and above 2 MeV, respectively. A fast ionization chamber was used in order to detect the fission fragments from the reactions and the targets were characterized as far as their mass and homogeneity are concerned by means of a spectroscopy and Rutherford backscattering spectroscopy respectively. Theoretical calculations within the Hauser-Feshbach formalism have been performed, employing the EMPIRE code, and the model parameters were tuned in order to successfully reproduce the experimental fission cross-sectional data and simultaneously all the competing reaction channels. C1 [Diakaki, M.; Aerts, G.; Andriamonje, S.; Berthoumieux, E.] CEA Saclay, DSM, F-91191 Gif Sur Yvette, France. [Diakaki, M.; Aerts, G.; Andriamonje, S.; Berthoumieux, E.] Natl Tech Univ Athens, Athens, Greece. [Demetriou, P.; Capote, R.] IAEA, Nucl Data Sect, A-1400 Vienna, Austria. [Skordis, E.; Tsinganis, A.; Calviani, M.; Cennini, P.; Chiaveri, E.; Ferrari, A.; Fitzpatrick, L.; Herrera-Martinez, A.; Kadi, Y.; Mengoni, A.; Sarchiapone, L.; Vlachoudis, V.; Wendler, H.] CERN, Geneva, Switzerland. [Abbondanno, U.; Milazzo, P. M.; Moreau, C.] Ist Nazl Fis Nucl, Trieste, Italy. [Alvarez, H.; Duran, I.; Paradela, C.] Univ Santiago de Compostela, Santiago De Compostela, Spain. [Alvarez-Velarde, F.; Cano-Ott, D.; Embid-Segura, M.; Gonzalez-Romero, E.; Guerrero, C.; Villamarin, D.; Vincente, M. C.] Ctr Invest Energet Medioambientales & Technol, Madrid, Spain. [Andrzejewski, J.; Marganiec, J.] Univ Lodz, PL-90131 Lodz, Poland. [Assimakopoulos, P.; Ioannidis, K.; Karamanis, D.; Patronis, N.; Stamoulis, K.] Univ Ioannina, GR-45110 Ioannina, Greece. [Audouin, L.; David, S.; Ferrant, L.; Isaev, S.; Stephan, C.; Tassan-Got, L.] CNRS, IN2P3, IPN, F-91405 Orsay, France. [Badurek, G.; Oberhummer, H.; Pavlik, A.] Univ Vienna, Inst Isotopenforsch & Kernphys, Vienna, Austria. [Baumann, P.; Kerveno, M.; Lukic, S.; Rudolf, G.] CNRS, IN2P3, IReS, Strasbourg, France. [Becvar, F.; Krticka, M.] Charles Univ Prague, Prague, Czech Republic. [Calvino, F.; Cortes, G.; Poch, A.; Pretel, C.] Univ Politecn Cataluna, Barcelona, Spain. [de Albornoz, A. Carrillo; Goncalves, I.; Marques, L.; Salgado, J.; Tavora, L.; Vaz, P.] Inst Tecnol & Nucl, Lisbon, Portugal. [Chepel, V.; Ferreira-Marques, R.; Lindote, A.; Lopes, I.; Neves, F.] LIP, Coimbra, Portugal. [Chepel, V.; Ferreira-Marques, R.; Lindote, A.; Lopes, I.; Neves, F.] Univ Coimbra, Dept Fis, P-3000 Coimbra, Portugal. [Colonna, N.; Fuji, K.; Marrone, S.; Tagliente, G.; Terlizzi, R.] Ist Nazl Fis Nucl, I-70126 Bari, Italy. [Couture, A.; Cox, J.; O'Brien, S.; Wiescher, M.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Dolfini, R.; Rubbia, C.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Domingo-Pardo, C.; Tain, J. L.] Univ Valencia, CSIC, Valencia, Spain. [Dorochenko, A.; Goverdovski, A.; Ketlerov, V.; Kolokolov, D.] Inst Phys & Power Engn, Obninsk, Kaluga Region, Russia. [Dridi, W.; Gunsing, F.; Pancin, J.; Perrot, L.; Plukis, A.] CEA Saclay, DSM, F-91191 Gif Sur Yvette, France. [Eleftheriadis, Ch.; Lamboudis, C.; Savvidis, I.] Aristotle Univ Thessaloniki, Thessaloniki, Greece. [Frais-Koelbl, H.; Griesmayer, E.] Fachhsch Wiener Neustadt, Wiener Neustadt, Austria. [Furman, W.; Konovalov, V.; Sedysheva, M.] Joint Nucl Res Inst, Frank Lab Neutron Phys, Dubna, Russia. [Gallino, R.] Univ Torino, Dipartimento Fis Gen, I-10125 Turin, Italy. [Gallino, R.] Sezione INFN Torino, I-10125 Turin, Italy. [Gramegna, F.; Mastinu, P.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Legnaro, Italy. [Haas, B.] CNRS, IN2P3, CENBG, Bordeaux, France. [Haight, R.; Reifarth, R.] Los Alamos Natl Lab, Los Alamos, NM USA. [Heil, M.; Kaeppeler, F.; Mosconi, M.; Plag, R.; Voss, F.; Wisshak, K.] Karlsruhe Inst Technol, Inst Kernphys, D-76021 Karlsruhe, Germany. [Igashira, M.] Tokyo Inst Technol, Tokyo 152, Japan. [Jericha, E.; Leeb, H.] Vienna Univ Technol, Atominst Osterreich Univ, A-1060 Vienna, Austria. [Koehler, P.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Lozano, M.; Quesada, J.] Univ Seville, Seville, Spain. [Massimi, C.; Vannini, G.] Univ Bologna, Dipartmento Fis, Bologna, Italy. [Massimi, C.; Vannini, G.] Sez INFN Bologna, Bologna, Italy. [Oshima, M.] Japan Atom Energy Res Inst, Tokai, Ibaraki 31911, Japan. [Pavlopoulos, P.] Pole Univ Leonard de Vinci, Paris, France. [Plompen, A.; Rullhusen, P.] CEC JRC IRMM, Geel, Belgium. [Rauscher, T.] Univ Basel, Dept Phys & Astron, Basel, Switzerland. [Rosetti, M.] ENEA, Bologna, Italy. [Ventura, A.] Ist Nazl Fis Nucl, I-40126 Bologna, Italy. RP Diakaki, M (reprint author), CEA Saclay, DSM, F-91191 Gif Sur Yvette, France.; Diakaki, M (reprint author), Natl Tech Univ Athens, Athens, Greece. EM maria.diakaki@cea.fr RI Vaz, Pedro/K-2464-2013; Rauscher, Thomas/D-2086-2009; Calvino, Francisco/K-5743-2014; Capote Noy, Roberto/M-1245-2014; Massimi, Cristian/K-2008-2015; Quesada Molina, Jose Manuel/K-5267-2014; Mengoni, Alberto/I-1497-2012 OI Vaz, Pedro/0000-0002-7186-2359; Rauscher, Thomas/0000-0002-1266-0642; Calvino, Francisco/0000-0002-7198-4639; Capote Noy, Roberto/0000-0002-1799-3438; Massimi, Cristian/0000-0003-2499-5586; Quesada Molina, Jose Manuel/0000-0002-2038-2814; Mengoni, Alberto/0000-0002-2537-0038 FU European Union (European Social Fund - ESF); Greek national funds through the Operational Program "Education and Life-long Learning" of the National Strategic Reference Framework (NSRF) - Research Funding Program: Heracleitus II FX This research has been cofinanced by the European Union (European Social Fund - ESF) and Greek national funds through the Operational Program "Education and Life-long Learning" of the National Strategic Reference Framework (NSRF) - Research Funding Program: Heracleitus II. NR 56 TC 1 Z9 1 U1 12 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 17 PY 2016 VL 93 IS 3 AR 034614 DI 10.1103/PhysRevC.93.034614 PG 12 WC Physics, Nuclear SC Physics GA DG9PF UT WOS:000372415600004 ER PT J AU Laskin, M Casten, RF Macchiavelli, AO Clark, RM Bucurescu, D AF Laskin, M. Casten, R. F. Macchiavelli, A. O. Clark, R. M. Bucurescu, D. TI Population of the giant pairing vibration SO PHYSICAL REVIEW C LA English DT Article ID UNBOUND LEVELS; EXCITATION; NUCLEI AB Background: The giant pairing vibration (GPV), a correlated two-nucleon mode in the second shell above the Fermi surface, has long been predicted and expected to be strongly populated in two-nucleon transfer cross sections similar to those of the normal pairing vibration. Recent experiments have provided evidence for this mode in C-14,C-15 but, despite sensitive studies, it has not been definitively identified in either Sn or Pb nuclei where pairing correlations are known to play a crucial role. Purpose: Our aim is to test whether features inherent to the mixing of bound and unbound levels might account for this and to study the effect in a simple and intuitively clear approach. Method: We study the mixing of unbound levels in a set of toy models that capture the essential physics of the GPV, along with a more realistic calculation including distorted-wave Born approximation transfer amplitudes. Results: The calculated (relative) cross section to populate a simulated GPV state is effectively low, compared to the case of bound levels with no widths Conclusions: The mixing turns out to be only a minor contributor to the weak population. Rather, the main reason is the melting of the GPV peak due to the width it acquires from the low orbital angular momentum single-particle states playing a dominant role in two-nucleon transfer amplitudes. This effect, in addition to a severe Q-value mismatch, may account for the elusive nature of this mode in (t,p) and (p, t) reactions. C1 [Laskin, M.; Casten, R. F.] Yale Univ, Wright Lab, Dept Phys, New Haven, CT 06520 USA. [Macchiavelli, A. O.; Clark, R. M.] Lawrence Berkeley Natl Lab, Nucl Sci Div, Berkeley, CA 94720 USA. [Bucurescu, D.] Natl Inst Phys & Nucl Engn, R-77125 Bucharest, Romania. [Laskin, M.] Univ Chicago, Dept Phys, 929 57th St, Chicago, IL 60637 USA. RP Laskin, M (reprint author), Yale Univ, Wright Lab, Dept Phys, New Haven, CT 06520 USA.; Laskin, M (reprint author), Univ Chicago, Dept Phys, 929 57th St, Chicago, IL 60637 USA. FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-05CH11231(LBNL), DE-FG02-91Er40609(Yale)]; Romanian UEFISCDI [PN-II-ID-PCE-2011-3-0140] FX We are grateful to Peter von Brentano for his research on the mixing of unbound levels and the sometimes unexpected effects encountered and for initial advice on calculations for such cases. We thank Witek Nazarewicz for pointing out to us the issues concerning the vanishing widths for bound levels. We greatly appreciate the extensive help of Hans Weidenmuller in understanding the formalism. This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-05CH11231(LBNL) and Grant No. DE-FG02-91Er40609(Yale), and the Romanian UEFISCDI, Project No. PN-II-ID-PCE-2011-3-0140. NR 28 TC 1 Z9 1 U1 2 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 17 PY 2016 VL 93 IS 3 AR 034321 DI 10.1103/PhysRevC.93.034321 PG 7 WC Physics, Nuclear SC Physics GA DG9PF UT WOS:000372415600003 ER PT J AU Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Agnew, JP Alexeev, GD Alkhazov, G Alton, A Askew, A Atkins, S Augsten, K Aushev, V Aushev, Y Avila, C Badaud, F Bagby, L Baldin, B Bandurin, DV Banerjee, S Barberis, E Baringer, P Bartlett, JF Bassler, U Bazterra, V Bean, A Begalli, M Bellantoni, L Beri, SB Bernardi, G Bernhard, R Bertram, I Besancon, M Beuselinck, R Bhat, PC Bhatia, S Bhatnagar, V Blazey, G Blessing, S Bloom, K Boehnlein, A Boline, D Boos, EE Borissov, G Borysova, M Brandt, A Brandt, O Brock, R Bross, A Brown, D Bu, XB Buehler, M Buescher, V Bunichev, V Burdin, S Buszello, CP Camacho-Perez, E Casey, BCK Castilla-Valdez, H Caughron, S Chakrabarti, S Chan, KM Chandra, A Chapon, E Chen, G Cho, SW Choi, S Choudhary, B Cihangir, S Claes, D Clutter, J Cooke, M Cooper, WE Corcoran, M Couderc, F Cousinou, MC Cuth, J Cutts, D Das, A Davies, G de Jong, SJ De La Cruz-Burelo, E Deliot, F Demina, R Denisov, D Denisov, SP Desai, S Deterre, C DeVaughan, K Diehl, HT Diesburg, M Ding, PF Dominguez, A Dubey, A Dudko, LV Duperrin, A Dutt, S Eads, M Edmunds, D Ellison, J Elvira, VD Enari, Y Evans, H Evdokimov, A Evdokimov, VN Faure, A Feng, L Ferbel, T Fiedler, F Filthaut, F Fisher, W Fisk, HE Fortner, M Fox, H Franc, J Fuess, S Garbincius, PH Garcia-Bellido, A Garcia-Gonzalez, JA Gaspar, P Gavrilov, V Geng, W Gerber, CE Gershtein, Y Ginther, G Gogota, O Golovanov, G Grannis, PD Greder, S Greenlee, H Grenier, G Gris, P Grivaz, JF Grohsjean, A Grunendahl, S Gruenewald, MW Guillemin, T Gutierrez, G Gutierrez, P Haley, J Han, L Harder, K Harel, A Hauptman, JM Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinson, AP Heintz, U Hensel, C Heredia-De La Cruz, I Herner, K Hesketh, G Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hoeneisen, B Hogan, J Hohlfeld, M Holzbauer, JL Howley, I Hubacek, Z Hynek, V Iashvili, I Ilchenko, Y Illingworth, R Ito, AS Jabeen, S Jaffre, M Jayasinghe, A Jeong, MS Jesik, R Jiang, P Johns, K Johnson, E Johnson, M Jonckheere, A Jonsson, P Joshi, J Jung, AW Juste, A Kajfasz, E Karmanov, D Katsanos, I Kaur, M Kehoe, R Kermiche, S Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Kiselevich, I Kohli, JM Kozelov, AV Kraus, J Kumar, A Kupco, A Kurca, T Kuzmin, VA Lammers, S Lebrun, P Lee, HS Lee, SW Lee, WM Lei, X Lellouch, J Li, D Li, H Li, L Li, QZ Lim, JK Lincoln, D Linnemann, J Lipaev, VV Lipton, R Liu, H Liu, Y Lobodenko, A Lokajicek, M de Sa, RL Luna-Garcia, R Lyon, AL Maciel, AKA Madar, R Magana-Villalba, R Malik, S Malyshev, VL Mansour, J Martinez-Ortega, J McCarthy, R McGivern, CL Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Meyer, A Meyer, J Miconi, F Mondal, NK Mulhearn, M Nagy, E Narain, M Nayyar, R Neal, HA Negret, JP Neustroev, P Nguyen, HT Nunnemann, T Orduna, J Osman, N Osta, J Pal, A Parashar, N Parihar, V Park, SK Partridge, R Parua, N Patwa, A Penning, B Perfilov, M Peters, Y Petridis, K Petrillo, G Petroff, P Pleier, MA Podstavkov, VM Popov, AV Prewitt, M Price, D Prokopenko, N Qian, J Quadt, A Quinn, B Ratoff, PN Razumov, I Ripp-Baudot, I Rizatdinova, F Rominsky, M Ross, A Royon, C Rubinov, P Ruchti, R Sajot, G Sanchez-Hernandez, A Sanders, MP Santos, AS Savage, G Savitskyi, M Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schott, M Schwanenberger, C Schwienhorst, R Sekaric, J Severini, H Shabalina, E Shary, V Shaw, S Shchukin, AA Simak, V Skubic, P Slattery, P Smirnov, D Snow, GR Snow, J Snyder, S Soeldner-Rembold, S Sonnenschein, L Soustruznik, K Stark, J Stefaniuk, N Stoyanova, DA Strauss, M Suter, L Svoisky, P Titov, M Tokmenin, VV Tsai, YT Tsybychev, D Tuchming, B Tully, C Uvarov, L Uvarov, S Uzunyan, S van Kooten, R van Leeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Verkheev, AY Vertogradov, LS Verzocchi, M Vesterinen, M Vilanova, D Vokac, P Wahl, HD Wang, MHLS Warchol, J Watts, G Wayne, M Weichert, J Welty-Rieger, L Williams, MRJ Wilson, GW Wobisch, M Wood, DR Wyatt, TR Xie, Y Yamada, R Yang, S Yasuda, T Yatsunenko, YA Ye, W Ye, Z Yin, H Yip, K Youn, SW Yu, JM Zennamo, J Zhao, TG Zhou, B Zhu, J Zielinski, M Zieminska, D Zivkovic, L AF Abazov, V. 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De La Cruz-Burelo, E. Deliot, F. Demina, R. Denisov, D. Denisov, S. P. Desai, S. Deterre, C. DeVaughan, K. Diehl, H. T. Diesburg, M. Ding, P. F. Dominguez, A. Dubey, A. Dudko, L. V. Duperrin, A. Dutt, S. Eads, M. Edmunds, D. Ellison, J. Elvira, V. D. Enari, Y. Evans, H. Evdokimov, A. Evdokimov, V. N. Faure, A. Feng, L. Ferbel, T. Fiedler, F. Filthaut, F. Fisher, W. Fisk, H. E. Fortner, M. Fox, H. Franc, J. Fuess, S. Garbincius, P. H. Garcia-Bellido, A. Garcia-Gonzalez, J. A. Gaspar, P. Gavrilov, V. Geng, W. Gerber, C. E. Gershtein, Y. Ginther, G. Gogota, O. Golovanov, G. Grannis, P. D. Greder, S. Greenlee, H. Grenier, G. Gris, Ph. Grivaz, J. -F. Grohsjean, A. Gruenendahl, S. Gruenewald, M. W. Guillemin, T. Gutierrez, G. Gutierrez, P. Haley, J. Han, L. Harder, K. Harel, A. Hauptman, J. M. Hays, J. Head, T. Hebbeker, T. Hedin, D. Hegab, H. Heinson, A. P. Heintz, U. Hensel, C. Heredia-De La Cruz, I. Herner, K. Hesketh, G. Hildreth, M. D. Hirosky, R. Hoang, T. Hobbs, J. D. Hoeneisen, B. Hogan, J. Hohlfeld, M. Holzbauer, J. L. Howley, I. Hubacek, Z. Hynek, V. Iashvili, I. Ilchenko, Y. Illingworth, R. Ito, A. S. Jabeen, S. Jaffre, M. Jayasinghe, A. Jeong, M. S. Jesik, R. Jiang, P. Johns, K. Johnson, E. Johnson, M. Jonckheere, A. Jonsson, P. Joshi, J. Jung, A. W. Juste, A. Kajfasz, E. Karmanov, D. Katsanos, I. Kaur, M. Kehoe, R. Kermiche, S. Khalatyan, N. Khanov, A. Kharchilava, A. Kharzheev, Y. N. Kiselevich, I. Kohli, J. M. Kozelov, A. V. Kraus, J. Kumar, A. Kupco, A. Kurca, T. Kuzmin, V. A. Lammers, S. Lebrun, P. Lee, H. S. Lee, S. W. Lee, W. M. Lei, X. Lellouch, J. Li, D. Li, H. Li, L. Li, Q. Z. Lim, J. K. Lincoln, D. Linnemann, J. Lipaev, V. V. Lipton, R. Liu, H. Liu, Y. Lobodenko, A. Lokajicek, M. de Sa, R. Lopes Luna-Garcia, R. Lyon, A. L. Maciel, A. K. A. Madar, R. Magana-Villalba, R. Malik, S. Malyshev, V. L. Mansour, J. Martinez-Ortega, J. McCarthy, R. McGivern, C. L. Meijer, M. M. Melnitchouk, A. Menezes, D. Mercadante, P. G. Merkin, M. Meyer, A. Meyer, J. Miconi, F. Mondal, N. K. Mulhearn, M. Nagy, E. Narain, M. Nayyar, R. Neal, H. A. Negret, J. P. Neustroev, P. Nguyen, H. T. Nunnemann, T. Orduna, J. Osman, N. Osta, J. Pal, A. Parashar, N. Parihar, V. Park, S. K. Partridge, R. Parua, N. Patwa, A. Penning, B. Perfilov, M. Peters, Y. Petridis, K. Petrillo, G. Petroff, P. Pleier, M. -A. Podstavkov, V. M. Popov, A. V. Prewitt, M. Price, D. Prokopenko, N. Qian, J. Quadt, A. Quinn, B. Ratoff, P. N. Razumov, I. Ripp-Baudot, I. Rizatdinova, F. Rominsky, M. Ross, A. Royon, C. Rubinov, P. Ruchti, R. Sajot, G. Sanchez-Hernandez, A. Sanders, M. P. Santos, A. S. Savage, G. Savitskyi, M. Sawyer, L. Scanlon, T. Schamberger, R. D. Scheglov, Y. Schellman, H. Schott, M. Schwanenberger, C. Schwienhorst, R. Sekaric, J. Severini, H. Shabalina, E. Shary, V. Shaw, S. Shchukin, A. A. Simak, V. Skubic, P. Slattery, P. Smirnov, D. Snow, G. R. Snow, J. Snyder, S. Soeldner-Rembold, S. Sonnenschein, L. Soustruznik, K. Stark, J. Stefaniuk, N. Stoyanova, D. A. Strauss, M. Suter, L. Svoisky, P. Titov, M. Tokmenin, V. V. Tsai, Y. -T. Tsybychev, D. Tuchming, B. Tully, C. Uvarov, L. Uvarov, S. Uzunyan, S. van Kooten, R. van Leeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verkheev, A. Y. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vokac, P. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weichert, J. Welty-Rieger, L. Williams, M. R. J. Wilson, G. W. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Yamada, R. Yang, S. Yasuda, T. Yatsunenko, Y. A. Ye, W. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. M. Zennamo, J. Zhao, T. G. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. CA D0 Collaboration TI Study of double parton interactions in diphoton plus dijet events in p<(p)over bar> collisions at root s = 1.96 TeV SO PHYSICAL REVIEW D LA English DT Article ID (P)OVER-BARP COLLISIONS; HADRONIC COLLISIONS; 4-JET EVENTS; SCATTERING AB We use a sample of diphoton + dijet events to measure the effective cross section of double parton interactions, which characterizes the area containing the interacting partons in proton-antiproton collisions, and find it to be sigma(eff) = 19.3 +/- 1.4(stat) +/- 7.8(syst) mb. The sample was collected by the D0 detector at the Fermilab Tevatron collider in p (p) over bar collisions at root s = 1.96 TeV and corresponds to an integrated luminosity of 8.7 fb(-1). C1 [Borysova, M.; Hensel, C.; Maciel, A. K. A.; Santos, A. S.] Ctr Brasileiro Pesquisas Fis, LAFEX, Rio De Janeiro, Brazil. [Begalli, M.; Gaspar, P.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Mercadante, P. G.] Univ Fed ABC, Santo Andre, Brazil. 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R.] Univ Nebraska, Lincoln, NE 68588 USA. [Gershtein, Y.] Rutgers State Univ, Piscataway, NJ 08855 USA. [Tully, C.] Princeton Univ, Princeton, NJ 08544 USA. [Iashvili, I.; Kharchilava, A.; Kumar, A.; Zennamo, J.] SUNY Buffalo, Buffalo, NY 14260 USA. [Demina, R.; Ferbel, T.; Garcia-Bellido, A.; Harel, A.; Petrillo, G.; Slattery, P.; Tsai, Y. -T.; Zielinski, M.] Univ Rochester, Rochester, NY 14627 USA. [Boline, D.; Chakrabarti, S.; Grannis, P. D.; Hobbs, J. D.; McCarthy, R.; Schamberger, R. D.; Tsybychev, D.; Ye, W.] SUNY Stony Brook, Stony Brook, NY 11794 USA. [Patwa, A.; Pleier, M. -A.; Snyder, S.; Yip, K.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Snow, J.] Langston Univ, Langston, OK 73050 USA. [Abbott, B.; Gutierrez, P.; Jayasinghe, A.; Severini, H.; Skubic, P.] Univ Oklahoma, Norman, OK 73019 USA. [Haley, J.; Hegab, H.; Khanov, A.; Rizatdinova, F.] Oklahoma State Univ, Stillwater, OK 74078 USA. [Schellman, H.; Strauss, M.] Oregon State Univ, Corvallis, OR 97331 USA. [Cutts, D.; Heintz, U.; Narain, M.; Parihar, V.; Partridge, R.] Brown Univ, Providence, RI 02912 USA. [Brandt, A.; Howley, I.; Pal, A.] Univ Texas Arlington, Arlington, TX 76019 USA. [Das, A.; Ilchenko, Y.; Kehoe, R.; Liu, H.] So Methodist Univ, Dallas, TX 75275 USA. [Chandra, A.; Corcoran, M.; Hogan, J.; Orduna, J.; Prewitt, M.] Rice Univ, Houston, TX 77005 USA. [Bandurin, D. V.; Hirosky, R.; Li, H.; Mulhearn, M.; Nguyen, H. T.; Svoisky, P.] Univ Virginia, Charlottesville, VA 22904 USA. [Watts, G.] Univ Washington, Seattle, WA 98195 USA. [Alton, A.] Augustana Coll, Sioux Falls, SD 57197 USA. [Burdin, S.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Deterre, C.; Grohsjean, A.] DESY, Notkestr 85, Hamburg, Germany. [Heredia-De La Cruz, I.] CONACyT, Mexico City, DF, Mexico. [Partridge, R.] SLAC, Menlo Pk, CA 94025 USA. [Hesketh, G.] UCL, London, England. [Luna-Garcia, R.] IPN, Ctr Invest Comp, Mexico City 07738, DF, Mexico. [Santos, A. S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Meyer, J.] KIT, SCC, D-76128 Karlsruhe, Germany. [Patwa, A.] US DOE, Off Sci, Washington, DC 20585 USA. [Cooke, M.] Amer Assoc Advancement Sci, Washington, DC 20005 USA. Kiev Inst Nucl Res, Kiev, Ukraine. [Jabeen, S.] Univ Maryland, College Pk, MD 20742 USA. [Williams, M. R. J.] European Org Nucl Res CERN, Geneva, Switzerland. [Jung, A. W.] Purdue Univ, W Lafayette, IN 47907 USA. RP Abazov, VM (reprint author), Inst Theoret & Expt Phys, Moscow 117259, Russia. RI Dudko, Lev/D-7127-2012; Merkin, Mikhail/D-6809-2012; Gutierrez, Phillip/C-1161-2011; Li, Liang/O-1107-2015 OI Dudko, Lev/0000-0002-4462-3192; Li, Liang/0000-0001-6411-6107 FU Department of Energy and National Science Foundation (USA); Alternative Energies and Atomic Energy Commission (France); National Center for Scientific Research/National Institute of Nuclear and Particle Physics (France); Ministry of Education and Science of the Russian Federation (Russia); National Research Center "Kurchatov Institute" of the Russian Federation (Russia); Russian Foundation for Basic Research (Russia); National Council for the Development of Science and Technology in the State of Rio de Janeiro (Brazil); Carlos Chagas Filho Foundation in the State of Rio de Janeiro (Brazil); Department of Atomic Energy and Department of Science and Technology (India); Administrative Department of Science, Technology and Innovation (Colombia); National Council of Science and Technology (Mexico); National Research Foundation of Korea (Korea); Foundation for Fundamental Research on Matter (Netherlands); Science and Technology Facilities Council (United Kingdom); Royal Society (United Kingdom); Ministry of Education, Youth and Sports (Czech Republic); Bundesministerium fur Bildung und Forschung (Federal Ministry of Education and Research) (Germany); Deutsche Forschungsgemeinschaft (German Research Foundation) (Germany); Science Foundation Ireland (Ireland); Swedish Research Council (Sweden); China Academy of Sciences (China); National Natural Science Foundation of China (China); Ministry of Education and Science of Ukraine (Ukraine) FX We thank the staff at Fermilab and collaborating institutions and acknowledge support from the Department of Energy and National Science Foundation (USA); Alternative Energies and Atomic Energy Commission and National Center for Scientific Research/National Institute of Nuclear and Particle Physics (France); Ministry of Education and Science of the Russian Federation, National Research Center "Kurchatov Institute" of the Russian Federation, and Russian Foundation for Basic Research (Russia); National Council for the Development of Science and Technology and Carlos Chagas Filho Foundation for the Support of Research in the State of Rio de Janeiro (Brazil); Department of Atomic Energy and Department of Science and Technology (India); Administrative Department of Science, Technology and Innovation (Colombia); National Council of Science and Technology (Mexico); National Research Foundation of Korea (Korea); Foundation for Fundamental Research on Matter (Netherlands); Science and Technology Facilities Council and The Royal Society (United Kingdom); Ministry of Education, Youth and Sports (Czech Republic); Bundesministerium fur Bildung und Forschung (Federal Ministry of Education and Research) and Deutsche Forschungsgemeinschaft (German Research Foundation) (Germany); Science Foundation Ireland (Ireland); Swedish Research Council (Sweden); China Academy of Sciences and National Natural Science Foundation of China (China); and Ministry of Education and Science of Ukraine (Ukraine). NR 49 TC 2 Z9 2 U1 6 U2 17 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 17 PY 2016 VL 93 IS 5 AR 052008 DI 10.1103/PhysRevD.93.052008 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG9QC UT WOS:000372417900001 ER PT J AU Bourgalais, J Roussel, V Capron, M Benidar, A Jasper, AW Klippenstein, SJ Biennier, L Le Picard, SD AF Bourgalais, J. Roussel, V. Capron, M. Benidar, A. Jasper, A. W. Klippenstein, S. J. Biennier, L. Le Picard, S. D. TI Low Temperature Kinetics of the First Steps of Water Cluster Formation SO PHYSICAL REVIEW LETTERS LA English DT Article ID NUCLEATION KINETICS; CHEMICAL-KINETICS; MASTER EQUATION; ENERGY; COMPUTATIONS; DIMERIZATION; DYNAMICS; (H2O)(N); RATES; DIMER AB We present a combined experimental and theoretical low temperature kinetic study of water cluster formation. Water cluster growth takes place in low temperature (23-69 K) supersonic flows. The observed kinetics of formation of water clusters are reproduced with a kinetic model based on theoretical predictions for the first steps of clusterization. The temperature-and pressure-dependent association and dissociation rate coefficients are predicted with an ab initio transition state theory based master equation approach over a wide range of temperatures (20-100 K) and pressures (10(-6) - 10 bar). C1 [Bourgalais, J.; Roussel, V.; Capron, M.; Benidar, A.; Biennier, L.; Le Picard, S. D.] Univ Rennes 1, CNRS, Inst Phys Rennes, UMR 6251, 263 Ave Gen Leclerc, F-35042 Rennes, France. [Jasper, A. W.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94551 USA. [Klippenstein, S. J.] Argonne Natl Lab, Div Chem, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Capron, M; Le Picard, SD (reprint author), Univ Rennes 1, CNRS, Inst Phys Rennes, UMR 6251, 263 Ave Gen Leclerc, F-35042 Rennes, France.; Klippenstein, SJ (reprint author), Argonne Natl Lab, Div Chem, 9700 S Cass Ave, Argonne, IL 60439 USA. EM michael.capron@univ-rennes1.fr; sjk@anl.gov; sebastien.le-picard@univ-rennes1.fr RI Jasper, Ahren/A-5292-2011 FU Agence Nationale de la Recherche [ANR-11-BS04-024-CRESUSOL-01]; Institut de Physique (INP-CNRS); Region Bretagne; Universite de Rennes 1; Institut Universitaire de France; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences at Argonne [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences at Sandia [DE-AC04-94AL85000] FX The Rennes team acknowledges support from the Agence Nationale de la Recherche, Contract No. ANR-11-BS04-024-CRESUSOL-01, the Institut de Physique (INP-CNRS), the Region Bretagne, and the Universite de Rennes 1. S. D. L. P. acknowledges financial support from the Institut Universitaire de France. The Rennes group wishes to express their thanks to Professor P. Casavecchia and Dr. R. Thissen and Dr. E. Hugo for his help in the design of the experiment. This study is based in part on work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences at Argonne under Contract No. DE-AC02-06CH11357, and at Sandia under Contract No. DE-AC04-94AL85000. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the National Nuclear Security Administration. NR 45 TC 3 Z9 3 U1 6 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 17 PY 2016 VL 116 IS 11 AR 113401 DI 10.1103/PhysRevLett.116.113401 PG 5 WC Physics, Multidisciplinary SC Physics GA DG9VU UT WOS:000372432700006 PM 27035301 ER PT J AU Bucher, B Zhu, S Wu, CY Janssens, RVF Cline, D Hayes, AB Albers, M Ayangeakaa, AD Butler, PA Campbell, CM Carpenter, MP Chiara, CJ Clark, JA Crawford, HL Cromaz, M David, HM Dickerson, C Gregor, ET Harker, J Hoffman, CR Kay, BP Kondev, FG Korichi, A Lauritsen, T Macchiavelli, AO Pardo, RC Richard, A Riley, MA Savard, G Scheck, M Seweryniak, D Smith, MK Vondrasek, R Wiens, A AF Bucher, B. Zhu, S. Wu, C. Y. Janssens, R. V. F. Cline, D. Hayes, A. B. Albers, M. Ayangeakaa, A. D. Butler, P. A. Campbell, C. M. Carpenter, M. P. Chiara, C. J. Clark, J. A. Crawford, H. L. Cromaz, M. David, H. M. Dickerson, C. Gregor, E. T. Harker, J. Hoffman, C. R. Kay, B. P. Kondev, F. G. Korichi, A. Lauritsen, T. Macchiavelli, A. O. Pardo, R. C. Richard, A. Riley, M. A. Savard, G. Scheck, M. Seweryniak, D. Smith, M. K. Vondrasek, R. Wiens, A. TI Direct Evidence of Octupole Deformation in Neutron-Rich Ba-144 SO PHYSICAL REVIEW LETTERS LA English DT Article ID GROUND-STATE; BARIUM ISOTOPES; RADIOACTIVE BEAMS; DEFORMED-NUCLEI; PARITY; ENERGY AB The neutron-rich nucleus Ba-144 (t(1/2) = 11.5 s) is expected to exhibit some of the strongest octupole correlations among nuclei with mass numbers A less than 200. Until now, indirect evidence for such strong correlations has been inferred from observations such as enhanced E1 transitions and interleaving positive- and negative-parity levels in the ground-state band. In this experiment, the octupole strength was measured directly by sub-barrier, multistep Coulomb excitation of a post-accelerated 650-MeV Ba-144 beam on a 1.0-mg/cm(2) Pb-208 target. The measured value of the matrix element, < 3(1)(-)parallel to M(E3)parallel to 0(1)(+)> = 0.65((+17)(-23)) eb(3/2,) corresponds to a reduced Bd(E3) transition probability of 48((+25)(-34)) W.u. This result represents an unambiguous determination of the octupole collectivity, is larger than any available theoretical prediction, and is consistent with octupole deformation. C1 [Bucher, B.; Wu, C. Y.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Zhu, S.; Janssens, R. V. F.; Albers, M.; Ayangeakaa, A. D.; Carpenter, M. P.; Chiara, C. J.; Clark, J. A.; David, H. M.; Dickerson, C.; Harker, J.; Hoffman, C. R.; Kay, B. P.; Kondev, F. G.; Korichi, A.; Lauritsen, T.; Pardo, R. C.; Savard, G.; Seweryniak, D.; Vondrasek, R.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Cline, D.; Hayes, A. B.] Univ Rochester, 601 Elmwood Ave, Rochester, NY 14627 USA. [Butler, P. A.] Univ Liverpool, Liverpool L69 7ZE, Merseyside, England. [Campbell, C. M.; Crawford, H. L.; Cromaz, M.; Macchiavelli, A. O.; Wiens, A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Chiara, C. J.; Harker, J.] Univ Maryland, College Pk, MD 20742 USA. [Crawford, H. L.; Richard, A.] Ohio Univ, Athens, OH 45701 USA. [Gregor, E. T.; Scheck, M.] Univ West Scotland, Paisley PA1 2BE, Renfrew, Scotland. [Gregor, E. T.; Scheck, M.] SUPA, Glasgow G12 8QQ, Lanark, Scotland. [Korichi, A.] IN2P3 CNRS, CSNSM, Batiment 104-108, F-91405 Orsay, France. [Riley, M. A.] Florida State Univ, Tallahassee, FL 32306 USA. [Smith, M. K.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Chiara, C. J.] US Army Res Lab, Adelphi, MD 20783 USA. [David, H. M.] GSI Helmholtzzentrum Schwerionenforsch, D-64291 Darmstadt, Germany. RP Bucher, B (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM bucher3@llnl.gov RI Hoffman, Calem/H-4325-2016; Kay, Benjamin/F-3291-2011 OI Hoffman, Calem/0000-0001-7141-9827; Kay, Benjamin/0000-0002-7438-0208 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357, DE-AC02-05CH11231, DE-AC52-07NA27344]; DOE [DE-FG02-94ER40834]; National Science Foundation [PHY-01401574, PHY-1068192]; STFC (UK) [ST/L005808/1] FX This work was funded by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, under Contract No. DE-AC02-06CH11357 (ANL), No. DE-AC02-05CH11231 (LBNL, GRETINA), No. DE-AC52-07NA27344 (LLNL), DOE Grant No. DE-FG02-94ER40834 (UM), and the National Science Foundation Grant No. PHY-01401574 (FSU) and PHY-1068192 (ND). M. S. and E. T. G. were supported by STFC (UK) Grant No. ST/L005808/1. This research used resources of ANL's ATLAS facility, which is a DOE Office of Science User Facility. NR 29 TC 11 Z9 11 U1 2 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 17 PY 2016 VL 116 IS 11 AR 112503 DI 10.1103/PhysRevLett.116.112503 PG 5 WC Physics, Multidisciplinary SC Physics GA DG9VU UT WOS:000372432700004 PM 27035298 ER PT J AU Clerouin, J Arnault, P Ticknor, C Kress, JD Collins, LA AF Clerouin, Jean Arnault, Philippe Ticknor, Christopher Kress, Joel D. Collins, Lee A. TI Unified Concept of Effective One Component Plasma for Hot Dense Plasmas SO PHYSICAL REVIEW LETTERS LA English DT Article ID EQUATION-OF-STATE; STATISTICAL-MECHANICS; DYNAMICAL PROPERTIES; MOLECULAR-DYNAMICS; IONIZED MATTER; YUKAWA SYSTEMS; SIMULATIONS; SCATTERING; PHYSICS; ENERGY AB Orbital-free molecular dynamics simulations are used to benchmark two popular models for hot dense plasmas: the one component plasma (OCP) and the Yukawa model. A unified concept emerges where an effective OCP (EOCP) is constructed from the short-range structure of the plasma. An unambiguous ionization and the screening length can be defined and used for a Yukawa system, which reproduces the long-range structure with finite compressibility. Similarly, the dispersion relation of longitudinal waves is consistent with the screened model at vanishing wave number but merges with the OCP at high wave number. Additionally, the EOCP reproduces the overall relaxation time scales of the correlation functions associated with ionic motion. In the hot dense regime, this unified concept of EOCP can be fruitfully applied to deduce properties such as the equation of state, ionic transport coefficients, and the ion feature in x-ray Thomson scattering experiments. C1 [Clerouin, Jean; Arnault, Philippe] CEA, DAM, DIF, F-91297 Arpajon, France. [Ticknor, Christopher; Kress, Joel D.; Collins, Lee A.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Clerouin, J (reprint author), CEA, DAM, DIF, F-91297 Arpajon, France. EM jean.clerouin@cea.fr RI Ticknor, Christopher/B-8651-2014; Clerouin, jean/D-8528-2015; OI Clerouin, jean/0000-0003-2144-2759; Ticknor, Christopher/0000-0001-9972-4524 FU National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX This work has been performed under the NNSA/DAM collaborative agreement P184. We specially thank Flavien Lambert for providing his OFMD code. P. A. would like to thank Nicolas Desbiens for fruitful discussions. The Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 53 TC 3 Z9 3 U1 6 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 17 PY 2016 VL 116 IS 11 AR 115003 DI 10.1103/PhysRevLett.116.115003 PG 5 WC Physics, Multidisciplinary SC Physics GA DG9VU UT WOS:000372432700008 PM 27035306 ER PT J AU Kang, CJ Denlinger, JD Allen, JW Min, CH Reinert, F Kang, BY Cho, BK Kang, JS Shim, JH Min, BI AF Kang, Chang-Jong Denlinger, J. D. Allen, J. W. Min, Chul-Hee Reinert, F. Kang, B. Y. Cho, B. K. Kang, J. -S. Shim, J. H. Min, B. I. TI Electronic Structure of YbB6: Is it a Topological Insulator or Not? SO PHYSICAL REVIEW LETTERS LA English DT Article ID BAND-STRUCTURE; SMB6; HEXABORIDE; PHOTOEMISSION; TRANSPORT; CAB6 AB To finally resolve the controversial issue of whether or not the electronic structure of YbB6 is nontrivially topological, we have made a combined study using angle-resolved photoemission spectroscopy (ARPES) of the nonpolar (110) surface and density functional theory (DFT). The flat-band conditions of the (110) ARPES avoid the strong band bending effects of the polar (001) surface and definitively show that YbB6 has a topologically trivial B 2p-Yb 5d semiconductor band gap of similar to 0.3 eV. Accurate determination of the low energy band topology in DFT requires the use of a modified Becke-Johnson exchange potential incorporating spin-orbit coupling and an on-site Yb 4f Coulomb interaction U as large as 7 eV. The DFT result, confirmed by a more precise GW band calculation, is similar to that of a small gap non-Kondo nontopological semiconductor. Additionally, the pressure-dependent electronic structure of YbB6 is investigated theoretically and found to transform into a p-d overlap semimetal with small Yb mixed valency. C1 [Kang, Chang-Jong; Shim, J. H.; Min, B. I.] Pohang Univ Sci & Technol, Dept Phys, PCTP, POSTECH, Pohang 37673, South Korea. [Denlinger, J. D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Allen, J. W.] Univ Michigan, Dept Phys, Randall Lab, Ann Arbor, MI 48109 USA. [Min, Chul-Hee; Reinert, F.] Univ Wurzburg, Expt Phys 7, D-97074 Wurzburg, Germany. [Kang, B. Y.; Cho, B. K.] GIST, Sch Mat Sci & Engn, Gwangju 61005, South Korea. [Kang, J. -S.] Catholic Univ Korea, Dept Phys, Bucheon 14662, South Korea. [Shim, J. H.] POSTECH, Dept Chem, Pohang 37673, South Korea. [Shim, J. H.] POSTECH, Div Adv Nucl Engn, Pohang 37673, South Korea. RP Min, BI (reprint author), Pohang Univ Sci & Technol, Dept Phys, PCTP, POSTECH, Pohang 37673, South Korea.; Denlinger, JD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. EM jddenlinger@lbl.gov; bimin@postech.ac.kr FU Korean NRF [2011-0028736, 2013R1A1A2006416, 2014R1A1A2056546, 2015R1A2A1A15053564]; Max-Plank POSTECH/KOREA Research Initiative [KR 2011-0031558]; KISTI supercomputing center [KSC-2015-C3-007]; Deutsche Forschungsgemeinschaft [SFB 1170 (C06)]; U.S. DOE at the Advanced Light Source [DE-AC02-05CH11231] FX This work was supported by the Korean NRF (No. 2011-0028736, No. 2013R1A1A2006416, No. 2014R1A1A2056546, No. 2015R1A2A1A15053564), Max-Plank POSTECH/KOREA Research Initiative (No. KR 2011-0031558), the KISTI supercomputing center (No. KSC-2015-C3-007), and the Deutsche Forschungsgemeinschaft via SFB 1170 (C06). Experiments were supported by the U.S. DOE at the Advanced Light Source (DE-AC02-05CH11231). NR 63 TC 4 Z9 4 U1 14 U2 51 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 17 PY 2016 VL 116 IS 11 AR 116401 DI 10.1103/PhysRevLett.116.116401 PG 6 WC Physics, Multidisciplinary SC Physics GA DG9VU UT WOS:000372432700011 PM 27035312 ER PT J AU Remillieux, MC Guyer, RA Payan, C Ulrich, TJ AF Remillieux, Marcel C. Guyer, Robert A. Payan, Cedric Ulrich, T. J. TI Decoupling Nonclassical Nonlinear Behavior of Elastic Wave Types SO PHYSICAL REVIEW LETTERS LA English DT Article ID RESONANT ULTRASOUND SPECTROSCOPY; DAMAGE ASSESSMENT; THERMAL-DAMAGE; SLOW DYNAMICS; ROCK; HYSTERESIS; CONCRETE; MEMORY; BONE AB In this Letter, the tensorial nature of the nonequilibrium dynamics in nonlinear mesoscopic elastic materials is evidenced via multimode resonance experiments. In these experiments the dynamic response, including the spatial variations of velocities and strains, is carefully monitored while the sample is vibrated in a purely longitudinal or a purely torsional mode. By analogy with the fact that such experiments can decouple the elements of the linear elastic tensor, we demonstrate that the parameters quantifying the nonequilibrium dynamics of the material differ substantially for a compressional wave and for a shear wave. This result could lead to further understanding of the nonlinear mechanical phenomena that arise in natural systems as well as to the design and engineering of nonlinear acoustic metamaterials. C1 [Remillieux, Marcel C.; Guyer, Robert A.; Ulrich, T. J.] Los Alamos Natl Lab, Geophys Grp EES 17, POB 1663, Los Alamos, NM 87545 USA. [Guyer, Robert A.] Univ Nevada, Dept Phys, Reno, NV 89577 USA. [Payan, Cedric] Aix Marseille Univ, LMA CNRS UPR 7051, Lab Mecan & Acoust, F-13402 Marseille 20, France. RP Remillieux, MC (reprint author), Los Alamos Natl Lab, Geophys Grp EES 17, POB 1663, Los Alamos, NM 87545 USA. EM mcr1@lanl.gov FU U.S. Department of Energy, Fuel Cycle R&D, Used Fuel Disposition (Storage) campaign FX This work was funded by the U.S. Department of Energy, Fuel Cycle R&D, Used Fuel Disposition (Storage) campaign. We are grateful to J. A. Ten Cate, P. A. Johnson, and P.-Y. Le Bas at Los Alamos National Laboratory for fruitful discussions. NR 33 TC 4 Z9 4 U1 9 U2 22 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 17 PY 2016 VL 116 IS 11 AR 115501 DI 10.1103/PhysRevLett.116.115501 PG 5 WC Physics, Multidisciplinary SC Physics GA DG9VU UT WOS:000372432700009 PM 27035309 ER PT J AU Aranson, IS AF Aranson, Igor S. TI MICROROBOTICS Swimmers by design SO NATURE LA English DT Editorial Material C1 [Aranson, Igor S.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Aranson, IS (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM aronson@anl.gov NR 13 TC 1 Z9 1 U1 5 U2 18 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAR 17 PY 2016 VL 531 IS 7594 BP 312 EP 313 PG 2 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG4TA UT WOS:000372064300039 PM 26983536 ER PT J AU Yang, B Zhang, YC Qian, Y Tang, J Liu, DQ AF Yang, Ben Zhang, Yaocun Qian, Yun Tang, Jian Liu, Dongqing TI Climatic effects of irrigation over the Huang-Huai-Hai Plain in China simulated by the weather research and forecasting model SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE irrigation; climatic effects; East Asian summer monsoon region; WRF ID ASIAN SUMMER MONSOON; CONVECTIVE PARAMETERIZATION SCHEME; SOUTHERN GREAT-PLAINS; SURFACE FLUXES; LAND-SURFACE; ANTHROPOGENIC AEROSOLS; ATMOSPHERIC RESPONSE; SEASON PRECIPITATION; EASTERN CHINA; LATE 1970S AB The climatic effects of irrigation over the Huang-Huai-Hai Plain (3HP) in China are investigated by using the weather research and forecasting model coupled with an operational-like irrigation scheme. Multiple numerical experiments with irrigation off/on during spring, summer, and both spring and summer are conducted. Results show that the warm bias in surface temperature and dry bias in soil moisture are reduced over the 3HP region during the growing seasons by considering the irrigation in the model. The air temperature during nongrowing seasons is also affected by irrigation because of the persistent effects of soil moisture on land-air energy exchanges and ground heat storage. Irrigation can induce significant cooling in the planetary boundary layer (PBL) during the growing seasons and lead to a relatively wet PBL with increased low-level clouds during spring but a relatively dry condition in summer. Further analyses indicate that irrigation leads to increased summer precipitation over the Yangtze River Basin and decreased summer precipitation in southern and northern China. These responses are associated with the changes in the large-scale circulation induced by irrigation. Irrigation tends to cool the atmosphere and forces a possible southward shift of the upper level jet that can further affect the precipitation distribution. Our model results suggest that in addition to local-scale processes, large-scale impacts should also be considered when studying the precipitation response to irrigation over East Asia. C1 [Yang, Ben; Zhang, Yaocun] Sch Atmospher Sci, Inst Climate & Global Change Res, CMA NJU Joint Lab Climate Predict Studies, Nanjing, Jiangsu, Peoples R China. [Yang, Ben; Zhang, Yaocun] Collaborat Innovat Ctr Climate Change, Nanjing, Jiangsu, Peoples R China. [Qian, Yun] Pacific NW Natl Lab, Richland, WA 99352 USA. [Tang, Jian] China Meteorol Adm, Beijing, Peoples R China. [Liu, Dongqing] Nanjing Meteorol Bur, Nanjing, Jiangsu, Peoples R China. RP Yang, B (reprint author), Sch Atmospher Sci, Inst Climate & Global Change Res, CMA NJU Joint Lab Climate Predict Studies, Nanjing, Jiangsu, Peoples R China.; Yang, B (reprint author), Collaborat Innovat Ctr Climate Change, Nanjing, Jiangsu, Peoples R China. EM byang@nju.edu.cn RI qian, yun/E-1845-2011; Yang, Ben/O-8548-2015 FU National Natural Science Foundation of China [41305084, 41475092]; Fundamental Research Funds for the Central Universities [20620140049]; Special Program for China Meteorology Trade [GYHY201306020]; Jiangsu Collaborative Innovation Center for Climate Change; U.S. Department of Energy's Office of Science as part of the Atmospheric System Research (ASR) program; DOE [DE-AC05-76RL01830] FX The authors acknowledge the three anonymous reviewers and Editor for their constructive comments and suggestions. Zhiyuan Hu, Anning Huang, Guoyong Leng, Xin Xu, and Chuliang Xiao are thanked for their valuable discussions. This work is jointly supported by the National Natural Science Foundation of China (41305084 and 41475092), the Fundamental Research Funds for the Central Universities (20620140049), Special Program for China Meteorology Trade (GYHY201306020), and the Jiangsu Collaborative Innovation Center for Climate Change. The contribution of Yun Qian in this study is supported by the U.S. Department of Energy's Office of Science as part of the Atmospheric System Research (ASR) program. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RL01830. The Global Map of Irrigation Areas version 5.0 was obtained from FAO's global water information system AQUASTAT at http://www.fao.org/nr/water/aquastat/irrigationmap/index10.stm. The weekly GVF data were obtained from NOAA/NESDIS/STAR at http://www.star.nesdis.noaa.gov/smcd/emb/vci/gvps/gvps_realtime_data.php . Surface air temperature and soil moisture observations were acquired from the National Meteorological Information Center of China Meteorological Administration at http://data.cma.gov.cn/data/index/6d1b5efbdcbf9a58.html. ChinaFLUX observations were obtained from Chinese FLUX observation and research network at http://159.226.111.42/pingtai/LoginRe/opendata.jsp. GPCP 1 degrees daily precipitation data were obtained from NCDC available online at http://www1.ncdc.noaa.gov/pub/data/gpcp/1dd-v1.2. The NCEP FNL analysis data set was downloaded from CISL Research Data Archive at http://rda.ucar.edu/datasets/ds083.2/. To request copies of the model data used in this study, please contact Ben Yang byang@nju.edu.cn. NR 65 TC 1 Z9 1 U1 10 U2 18 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAR 16 PY 2016 VL 121 IS 5 BP 2246 EP 2264 DI 10.1002/2015JD023736 PG 19 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DI6HB UT WOS:000373598700013 ER PT J AU Lim, KSS Riihimaki, L Comstock, JM Schmid, B Sivaraman, C Shi, Y McFarquhar, GM AF Lim, Kyo-Sun Sunny Riihimaki, Laura Comstock, Jennifer M. Schmid, Beat Sivaraman, Chitra Shi, Yan McFarquhar, Greg M. TI Evaluation of long-term surface-retrieved cloud droplet number concentration with in situ aircraft observations SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE cloud droplet number concentration; multifilter rotating shadow band radiometer; microwave radiometer; cloud droplet effective radius; RACORO field campaign; ARM SGP ID BOUNDARY-LAYER CLOUDS; LIQUID WATER PATH; GROUND-BASED MEASUREMENTS; RADIATIVE PROPERTIES; STRATUS CLOUD; MICROWAVE RADIOMETERS; CLIMATE FEEDBACKS; EFFECTIVE RADIUS; ENTRAINMENT; EVOLUTION AB A new operational retrieval of cloud droplet number concentration (N-D) at cloud base has been produced from surface remote sensors at the Atmospheric Radiation Measurement (ARM) Southern Great Plains site for 13years from January 1998 to January 2011. The retrieval is based on surface radiometer measurements of cloud optical depth from the multifilter rotating shadow band radiometer and liquid water path from the microwave radiometer (MWR). It is only applicable for single-layered overcast warm (stratus or stratocumulus) clouds. Evaluation with in situ aircraft measurements during the extended-term aircraft field campaign, Routine ARM Aerial Facility (AAF) Clouds with Low Optical Water Depths (CLOWD) Optical Radiative Observations (RACORO), shows that the retrieved N-D robustly reproduces the primary mode of the in situ measured probability density function (PDF) but produces too wide a distribution, primarily caused by frequent high cloud droplet number concentration. Our analysis shows that the error in the MWR retrievals at low liquid water paths is one possible reason for this deficiency. Modification through the diagnosed liquid water path from the coordinate solution improves not only the PDF of the retrieved N-D but also the relationship between the cloud droplet number concentration and cloud droplet effective radius. Consideration of entrainment effects rather than assuming an adiabatic cloud improves the values of the N-D retrieval by reducing the magnitude of cloud droplet number concentration. Aircraft measurements and retrieval comparisons suggest that retrieving the vertical distribution of cloud droplet number concentration and effective radius is feasible with an improvement of the parameter representing the mixing effects between environment and clouds and with a better understanding of the effect of mixing degree on cloud properties. C1 [Lim, Kyo-Sun Sunny; Riihimaki, Laura; Comstock, Jennifer M.; Schmid, Beat; Sivaraman, Chitra; Shi, Yan] Pacific NW Natl Lab, Richland, WA 99352 USA. [McFarquhar, Greg M.] Univ Illinois, Dept Atmospher Sci, Urbana, IL USA. RP Riihimaki, L (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM Laura.Riihimaki@pnnl.gov RI Lim, Kyo-Sun/I-3811-2012; OI McFarquhar, Greg/0000-0003-0950-0135 FU Office of Biological and Environmental Research of the U.S. Department of Energy as part of the Atmospheric Radiation Measurement (ARM) Climate Research Facility, an Office of Science user facility; Office of Biological and Environmental Research; DOE [DE-AC05-76RLO 1830] FX We greatly express our thanks to Haf Jonsson and Andy Vogelmann for their help providing in situ airborne measurement data. Our thanks also extend to the value-added products (VAP) science sponsors and scientists, Qilong Min, Allison McComiskey, Graham Feingold, and David D. Turner, for their helpful discussions and contributions to VAP development. The first author would like to express her thanks to Hyeyum Hailey Shin, Zhe Feng, and Jinho Yoon for their helpful review and suggestion. This research was supported by the Office of Biological and Environmental Research of the U.S. Department of Energy as part of the Atmospheric Radiation Measurement (ARM) Climate Research Facility, an Office of Science user facility. Data were obtained from the Atmospheric Radiation Measurement (ARM) Climate Research Facility, a U.S. Department of Energy Office of Science user facility sponsored by the Office of Biological and Environmental Research. The surface retrieval and the in situ aircraft data during RACORO field campaign used in this study can be freely downloadable at https://www.arm.gov/data/vaps and https://www.arm.gov/campaigns/aaf2009racoro, respectively. The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under contract DE-AC05-76RLO 1830. NR 53 TC 1 Z9 1 U1 1 U2 2 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAR 16 PY 2016 VL 121 IS 5 BP 2318 EP 2331 DI 10.1002/2015JD024082 PG 14 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DI6HB UT WOS:000373598700017 ER PT J AU Mills, MJ Schmidt, A Easter, R Solomon, S Kinnison, DE Ghan, SJ Neely, RR Marsh, DR Conley, A Bardeen, CG Gettelman, A AF Mills, Michael J. Schmidt, Anja Easter, Richard Solomon, Susan Kinnison, Douglas E. Ghan, Steven J. Neely, Ryan R., III Marsh, Daniel R. Conley, Andrew Bardeen, Charles G. Gettelman, Andrew TI Global volcanic aerosol properties derived from emissions, 1990-2014, using CESM1(WACCM) SO JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES LA English DT Article DE aerosol; climate; stratosphere; volcanoes; radiative forcing; ozone loss ID SIZE DISTRIBUTION MEASUREMENTS; EARTH SYSTEM MODEL; ANTHROPOGENIC OZONE DEPLETION; COMMUNITY ATMOSPHERE MODEL; SULFURIC-ACID-SOLUTIONS; STRATOSPHERIC AEROSOL; CLIMATE MODEL; SAGE-II; PINATUBO ERUPTION; CARBONYL SULFIDE AB Accurate representation of global stratospheric aerosols from volcanic and nonvolcanic sulfur emissions is key to understanding the cooling effects and ozone losses that may be linked to volcanic activity. Attribution of climate variability to volcanic activity is of particular interest in relation to the post-2000 slowing in the rate of global average temperature increases. We have compiled a database of volcanic SO2 emissions and plume altitudes for eruptions from 1990 to 2014 and developed a new prognostic capability for simulating stratospheric sulfate aerosols in the Community Earth System Model. We used these combined with other nonvolcanic emissions of sulfur sources to reconstruct global aerosol properties from 1990 to 2014. Our calculations show remarkable agreement with ground-based lidar observations of stratospheric aerosol optical depth (SAOD) and with in situ measurements of stratospheric aerosol surface area density (SAD). These properties are key parameters in calculating the radiative and chemical effects of stratospheric aerosols. Our SAOD calculations represent a clear improvement over available satellite-based analyses, which generally ignore aerosol extinction below 15km, a region that can contain the vast majority of stratospheric aerosol extinction at middle and high latitudes. Our SAD calculations greatly improve on that provided for the Chemistry-Climate Model Initiative, which misses about 60% of the SAD measured in situ on average during both volcanically active and volcanically quiescent periods. C1 [Mills, Michael J.; Kinnison, Douglas E.; Marsh, Daniel R.; Conley, Andrew; Bardeen, Charles G.; Gettelman, Andrew] Natl Ctr Atmospher Res, Atmospher Chem Observat & Modeling Lab, POB 3000, Boulder, CO 80307 USA. [Schmidt, Anja; Neely, Ryan R., III] Univ Leeds, Sch Earth & Environm, Leeds, W Yorkshire, England. [Easter, Richard; Ghan, Steven J.] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. [Solomon, Susan] MIT, Dept Earth Atmospher & Planetary Sci, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Neely, Ryan R., III] Univ Leeds, Natl Ctr Atmospher Sci, Leeds, W Yorkshire, England. RP Mills, MJ (reprint author), Natl Ctr Atmospher Res, Atmospher Chem Observat & Modeling Lab, POB 3000, Boulder, CO 80307 USA. EM mmills@ucar.edu RI Ghan, Steven/H-4301-2011; Marsh, Daniel/A-8406-2008; Schmidt, Anja/C-9617-2012; Mills, Michael/B-5068-2010; OI Ghan, Steven/0000-0001-8355-8699; Marsh, Daniel/0000-0001-6699-494X; Mills, Michael/0000-0002-8054-1346; Schmidt, Anja/0000-0001-8759-2843 FU National Science Foundation; NSF atmospheric chemistry program [1539972] FX We thank David Ridley for providing lidar extinction measurements shown in Figure 5 and Nicolas Theys for providing SO2 flux data for the database. Mauna Loa lidar data were provided by NOAA ESRL Global Monitoring Division, Boulder, Colorado, USA (http://esrl.noaa.gov/gmd/). Ny-Alesund lidar data were provided by Christoph Ritter. We thank Anne Smith, Jean-Francois Lamarque, and two anonymous reviewers for their many helpful comments on this manuscript. The National Center for Atmospheric Research is sponsored by the National Science Foundation. Any opinions, findings, and conclusions or recommendations expressed in the publication are those of the author(s) and do not necessarily reflect the views of the National Science Foundation. S.S. was supported by NSF atmospheric chemistry program grant 1539972. Our global volcanic aerosol reconstruction may be accessed via doi: 10.5065/D6S180JM. Supporting data are included as four tables in .xlsx format files and one figure; any additional data, including the source code used for these simulations, may be obtained from M.J.M. (email: mmills@ucar.edu). NR 90 TC 12 Z9 12 U1 10 U2 21 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-897X EI 2169-8996 J9 J GEOPHYS RES-ATMOS JI J. Geophys. Res.-Atmos. PD MAR 16 PY 2016 VL 121 IS 5 BP 2332 EP 2348 DI 10.1002/2015JD024290 PG 17 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DI6HB UT WOS:000373598700018 ER PT J AU Turner, AJ Jacob, DJ Benmergui, J Wofsy, SC Maasakkers, JD Butz, A Hasekamp, O Biraud, SC AF Turner, A. J. Jacob, D. J. Benmergui, J. Wofsy, S. C. Maasakkers, J. D. Butz, A. Hasekamp, O. Biraud, S. C. TI A large increase in US methane emissions over the past decade inferred from satellite data and surface observations SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE methane; GOSAT ID COMPARISON PROJECT WETCHIMP; HIGH-SPATIAL-RESOLUTION; GLOBAL WETLAND EXTENT; ATMOSPHERIC METHANE; PRESENT STATE; ETHANE; INVERSIONS; AIR AB The global burden of atmospheric methane has been increasing over the past decade, but the causes are not well understood. National inventory estimates from the U.S. Environmental Protection Agency indicate no significant trend in U.S. anthropogenic methane emissions from 2002 to present. Here we use satellite retrievals and surface observations of atmospheric methane to suggest that U.S. methane emissions have increased by more than 30% over the 2002-2014 period. The trend is largest in the central part of the country, but we cannot readily attribute it to any specific source type. This large increase in U.S. methane emissions could account for 30-60% of the global growth of atmospheric methane seen in the past decade. C1 [Turner, A. J.; Jacob, D. J.; Benmergui, J.; Wofsy, S. C.; Maasakkers, J. D.] Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Jacob, D. J.; Wofsy, S. C.] Harvard Univ, Dept Earth & Planetary Sci, 20 Oxford St, Cambridge, MA 02138 USA. [Butz, A.] Karlsruhe Inst Technol, IMK ASF, D-76021 Karlsruhe, Germany. [Hasekamp, O.] SRON Netherlands Inst Space Res, Utrecht, Netherlands. [Biraud, S. C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA 94720 USA. RP Jacob, DJ (reprint author), Harvard Univ, Sch Engn & Appl Sci, Cambridge, MA 02138 USA.; Jacob, DJ (reprint author), Harvard Univ, Dept Earth & Planetary Sci, 20 Oxford St, Cambridge, MA 02138 USA. EM djacob@fas.harvard.edu RI Biraud, Sebastien/M-5267-2013 OI Biraud, Sebastien/0000-0001-7697-933X FU NASA Carbon Monitoring System and a Department of Energy (DOE) Computational Science Graduate Fellowship (CSGF); Office of Biological and Environmental Research of the U.S. Department of Energy [DE-AC02-05CH11231]; ARM Aerial Facility; Terrestrial Ecosystem Science Program; Deutsche Forschungsgemeinschaft through the Emmy-Noether programme [BU2599/1-1]; ESA GHG-CCI project FX This work was supported by the NASA Carbon Monitoring System and a Department of Energy (DOE) Computational Science Graduate Fellowship (CSGF) to A.J.T. Observations collected in the Southern Great Plains were supported by the Office of Biological and Environmental Research of the U.S. Department of Energy under contract DE-AC02-05CH11231 as part of the Atmospheric Radiation Measurement Program (ARM), ARM Aerial Facility, and Terrestrial Ecosystem Science Program. A.B. is supported by Deutsche Forschungsgemeinschaft through the Emmy-Noether programme, grant BU2599/1-1 (RemoTeC). GOSAT retrieval algorithm development and processing was partly funded by the ESA GHG-CCI project. We thank E. Dlugokencky for providing data from the MLO and BMW sites. NR 45 TC 6 Z9 7 U1 16 U2 39 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAR 16 PY 2016 VL 43 IS 5 BP 2218 EP 2224 DI 10.1002/2016GL067987 PG 7 WC Geosciences, Multidisciplinary SC Geology GA DH9IN UT WOS:000373109800053 ER PT J AU Yang, Y Russell, LM Lou, SJ Liu, Y Singh, B Ghan, SJ AF Yang, Yang Russell, Lynn M. Lou, Sijia Liu, Ying Singh, Balwinder Ghan, Steven J. TI Rain-aerosol relationships influenced by wind speed SO GEOPHYSICAL RESEARCH LETTERS LA English DT Article DE rain; aerosol; wind; AOD ID COMMUNITY ATMOSPHERE MODEL; GENERAL-CIRCULATION MODEL; OPTICAL DEPTH; CLOUD MICROPHYSICS; CONVECTIVE CLOUDS; PRECIPITATION; SATELLITE; PARAMETERIZATION; INVIGORATION; POLLUTION AB Aerosol optical depth (AOD) has been shown to correlate with precipitation rate (R) in recent studies. The R-AOD relationships over oceans are examined in this study using 150year simulations with the Community Earth System Model. Through partial correlation analysis, with the influence of 10m wind speed removed, R-AOD relationships exert a change from positive to negative over the midlatitude oceans, indicating that wind speed makes a large contribution to the relationships by changing the sea-salt emissions. A simulation with prescribed sea-salt emissions shows that wind speed leads to increasing R by +0.99mmd(-1) averaged globally, offsetting 64% of the wet scavenging-induced decrease between polluted and clean conditions, defined according to percentiles of AOD. These demonstrate that wind speed is one of the major drivers of R-AOD relationships. Relative humidity at 915hPa can also result in the positive relationships; however, its role is smaller than that of wind speed. C1 [Yang, Yang; Russell, Lynn M.; Lou, Sijia] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. [Liu, Ying; Singh, Balwinder; Ghan, Steven J.] Pacific NW Natl Lab, Atmospher Sci & Global Change Div, Richland, WA 99352 USA. RP Russell, LM (reprint author), Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA. EM lmrussell@ucsd.edu RI Ghan, Steven/H-4301-2011 OI Ghan, Steven/0000-0001-8355-8699 FU National Science Foundation (NSF) [AGS1048995]; DOE as part of the U.S. Department of Energy, Office of Science, Biological and Environmental Research, Decadal and Regional Climate Prediction using Earth System Models (EaSM) program [DE-SC0006679]; Department of Energy's (DOE) by Battelle Memorial Institute of Columbus, Ohio [DE-AC05-76RLO 1830]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This research was supported by National Science Foundation (NSF) AGS1048995 and by DOE DE-SC0006679 as part of the U.S. Department of Energy, Office of Science, Biological and Environmental Research, Decadal and Regional Climate Prediction using Earth System Models (EaSM) program. The Pacific Northwest National Laboratory is operated for the Department of Energy's (DOE) by Battelle Memorial Institute of Columbus, Ohio under contract DE-AC05-76RLO 1830. Observed 10m wind speed data are obtained from the ERA-Interim reanalysis at the European Center for Medium Range Weather Forecasts (ECMWF). CMAP precipitation data are provided by the NOAA/OAR/ESRL PSD, Boulder, Colorado, USA, from their website at http://www.esrl.noaa.gov/psd/. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under contract DE-AC02-05CH11231. The data and codes for these results are posted at http://portal.nersc.gov/project/m1374/AOD_R. NR 36 TC 2 Z9 2 U1 1 U2 10 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0094-8276 EI 1944-8007 J9 GEOPHYS RES LETT JI Geophys. Res. Lett. PD MAR 16 PY 2016 VL 43 IS 5 BP 2267 EP 2274 DI 10.1002/2016GL067770 PG 8 WC Geosciences, Multidisciplinary SC Geology GA DH9IN UT WOS:000373109800059 ER PT J AU Sun, Q Wang, ZJ Zhang, ZJ Yu, Q Qu, Y Zhang, JY Yu, Y Xiang, B AF Sun, Qi Wang, Zhijie Zhang, Zijiao Yu, Qian Qu, Yan Zhang, Jingyu Yu, Yan Xiang, Bin TI Rational Design of Graphene-Reinforced MnO Nanowires with Enhanced Electrochemical Performance for Li-Ion Batteries SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE lithium-ion battery; MnO; graphene nanosheets; anode; nanowire morphology ID ENERGY-STORAGE; INTERCALATION PSEUDOCAPACITANCE; ANODE MATERIAL; OXIDE; GREEN; MICROSPHERES; NANOSHEETS; HYBRID; FILMS AB Recently, transition metal oxides (TMOs) mixed with carbon materials have attracted attention as lithium-ion battery (LIB) anode materials. However, the aggregation issue in TMOs hinders the development of an ideal encapsulation structure with carbon materials. In this paper, we report graphene reinforced MnO nanowires with enhanced electrochemical performance as an anode in LIB. The graphene nanosheets (GNs)/MnO feature was confirmed by transmission electron microscopy, X-ray diffraction, Raman scattering, and X-ray photoelectron spectroscopy. The GNs/MnO nanowires delivered a highly stable discharge capacity of similar to 815 mAh g(-1) at a current density of 100 mA g(-1) after 200 cycles, which is 1.5 times higher than that of pure MnO nanowires. This GNs/MnO structure with a specific capacity of similar to 995 mAh g(-1) at a current density of 50 mA g(-1) also exhibited excellent Li storage properties. The superior cycling and high rate capability were attributed to the intimate incorporation between the MnO and GNs. The structure of the GNs/MnO nanowires effectively accommodated the volume change of the MnO nanowires and prevented structure collapse during cycling. C1 [Sun, Qi; Wang, Zhijie; Yu, Yan; Xiang, Bin] Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Synerget Innovat Ctr Quantum Informat Quantum Phy, Dept Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China. [Zhang, Zijiao; Yu, Qian] Zhejiang Univ, Ctr Electron Microscopy, Hangzhou 310027, Zhejiang, Peoples R China. [Zhang, Zijiao; Yu, Qian] Zhejiang Univ, Dept Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China. [Qu, Yan] Sixth Element Mat Technol Co Ltd, Changzhou 213145, Jiangsu, Peoples R China. [Zhang, Jingyu] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Xiang, B (reprint author), Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Synerget Innovat Ctr Quantum Informat Quantum Phy, Dept Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China.; Yu, Q (reprint author), Zhejiang Univ, Ctr Electron Microscopy, Hangzhou 310027, Zhejiang, Peoples R China.; Yu, Q (reprint author), Zhejiang Univ, Dept Mat Sci & Engn, State Key Lab Silicon Mat, Hangzhou 310027, Zhejiang, Peoples R China. EM yu_qian@zju.edu.cn; binxiang@ustc.edu.cn RI Xiang, Bin/C-9192-2012; wang, zhijie/R-8576-2016 FU National Natural Science Foundation of China [21373196, 11434009]; National Program for Thousand Young Talents of China; Fundamental Research Funds for the Central Universities [WK2340000050, WK2060140014]; 973 Program of China [2015CB65930] FX This work was supported by the National Natural Science Foundation of China (21373196, 11434009), the National Program for Thousand Young Talents of China and the Fundamental Research Funds for the Central Universities (WK2340000050, WK2060140014). Q.Y. was supported by the 973 Program of China 2015CB65930. NR 29 TC 11 Z9 11 U1 42 U2 146 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD MAR 16 PY 2016 VL 8 IS 10 BP 6303 EP 6308 DI 10.1021/acsami.6b00122 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DH0MW UT WOS:000372479300001 PM 26894410 ER PT J AU Jiang, JC Zhao, YB Yaghi, OM AF Jiang, Juncong Zhao, Yingbo Yaghi, Omar M. TI Covalent Chemistry beyond Molecules SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Review ID METAL-ORGANIC FRAMEWORKS; ZEOLITIC IMIDAZOLATE FRAMEWORKS; ENHANCED CATALYTIC PERFORMANCE; CARBON-DIOXIDE CAPTURE; POSTSYNTHETIC MODIFICATION; HETEROGENEOUS CATALYSTS; GAS-ADSORPTION; MODULATED SYNTHESIS; DESIGNED SYNTHESIS; FUNCTIONAL-GROUPS AB Linking molecular building units by covalent bonds to make crystalline extended structures has given rise to metal organic frameworks (MOFs) and covalent organic frameworks (COFs), thus bringing the precision and versatility of covalent chemistry beyond discrete molecules to extended structures. The key advance in this regard has been the development of strategies to overcome the "crystallization problem", which is usually encountered when attempting to link molecular building units into covalent solids. Currently, numerous MOFs and COFs are made as crystalline materials in which the large size of the constituent units provides for open frameworks. The molecular units thus reticulated become part of a new environment where they have (a) lower degrees of freedom because they are fixed into position within the framework; (b) well-defined spatial arrangements where their properties are influenced by the intricacies of the pores; and (c) ordered patterns onto which functional groups can be covalently attached to produce chemical complexity. The notion of covalent chemistry beyond molecules is further strengthened by the fact that covalent reactions can be carried out on such frameworks, with full retention of their crystallinity and porosity. MOFs are exemplars of how this chemistry has led to porosity with designed metrics and functionality, chemically-rich sequences of information within their frameworks, and well-defined mesoscopic constructs in which nanoMOFs enclose inorganic nanocrystals and give them new levels of spatial definition, stability, and functionality. C1 [Jiang, Juncong; Zhao, Yingbo; Yaghi, Omar M.] Univ Calif Berkeley, Dept Chem, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Jiang, Juncong; Zhao, Yingbo; Yaghi, Omar M.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. [Yaghi, Omar M.] King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. RP Yaghi, OM (reprint author), Univ Calif Berkeley, Dept Chem, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Yaghi, OM (reprint author), Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA.; Yaghi, OM (reprint author), King Abdulaziz City Sci & Technol, Riyadh 11442, Saudi Arabia. EM yaghi@berkeley.edu OI Yaghi, Omar/0000-0002-5611-3325 FU BASF SE (Ludwigshafen, Germany); King Abdulaziz City for Science and Technology (Riyadh, Saudi Arabia); U.S. Department of Defense, Defense Threat Reduction Agency [HDTRA 1-12-1-0053]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Energy Frontier Research Center [DE-SC0001015] FX We gratefully acknowledge Drs. H. Furukawa, A. M. Fracaroli and A. Schodel and Mr. C. S. Diercks for their valuable discussion, and Prof. Walter G. Klemperer and Dr. J. Yuan for their contributions to the idea of enzyme-like constructs. Financial support for related research in O.M.Y. laboratories is provided by BASF SE (Ludwigshafen, Germany); King Abdulaziz City for Science and Technology (Riyadh, Saudi Arabia); U.S. Department of Defense, Defense Threat Reduction Agency Grant HDTRA 1-12-1-0053; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Energy Frontier Research Center grant DE-SC0001015. NR 143 TC 22 Z9 23 U1 94 U2 258 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD MAR 16 PY 2016 VL 138 IS 10 BP 3255 EP 3265 DI 10.1021/jacs.5b10666 PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA DH0MG UT WOS:000372477700001 PM 26863450 ER PT J AU Herlitschke, M Klobes, B Sergueev, I Hering, P Peron, J Hermann, RP AF Herlitschke, M. Klobes, B. Sergueev, I. Hering, P. Peron, J. Hermann, R. P. TI Elasticity and magnetocaloric effect in MnFe4Si3 SO PHYSICAL REVIEW B LA English DT Article ID NUCLEAR INELASTIC-SCATTERING; SYSTEM MN5SI3-FE5SI3; REFRIGERATION; MAGNETISM; MOSSBAUER AB The room temperature magnetocaloric material MnFe4Si3 was investigated with nuclear inelastic scattering (NIS) and resonant ultrasound spectroscopy (RUS) at different temperatures and applied magnetic fields in order to assess the influence of the magnetic transition and the magnetocaloric effect on lattice dynamics. The NIS data give access to phonons with energies above 3 meV, whereas RUS probes the elasticity of the material in the MHz frequency range and thus low-energy, neV, phonon modes. A significant influence of the magnetic transition on the lattice dynamics is observed only in the low-energy, long-wavelength limit. MnFe4Si3 and other compounds in the Mn(5-x)Ye(x)Si(3) series were also investigated with vibrating sample magnetometry, resistivity measurements, and Mossbauer spectroscopy in order to study the magnetic transitions and to complement the results obtained on the lattice dynamics. C1 [Herlitschke, M.; Sergueev, I.] Deutsch Elektronen Synchrotron DESY, FS PE, D-22607 Hamburg, Germany. [Herlitschke, M.; Klobes, B.; Hering, P.; Peron, J.; Hermann, R. P.] Forschungszentrum Julich, Julich Ctr Neutron Sci JCNS, D-52425 Julich, Germany. [Herlitschke, M.; Klobes, B.; Hering, P.; Peron, J.; Hermann, R. P.] Forschungszentrum Julich, Peter Grunberg Inst PGI, JARA FIT, D-52425 Julich, Germany. [Herlitschke, M.; Hermann, R. P.] Univ Liege, Fac Sci, B-4000 Liege, Belgium. [Hermann, R. P.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Herlitschke, M (reprint author), Deutsch Elektronen Synchrotron DESY, FS PE, D-22607 Hamburg, Germany.; Herlitschke, M; Hermann, RP (reprint author), Forschungszentrum Julich, Julich Ctr Neutron Sci JCNS, D-52425 Julich, Germany.; Herlitschke, M; Hermann, RP (reprint author), Forschungszentrum Julich, Peter Grunberg Inst PGI, JARA FIT, D-52425 Julich, Germany.; Herlitschke, M; Hermann, RP (reprint author), Univ Liege, Fac Sci, B-4000 Liege, Belgium.; Hermann, RP (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM marcus.herlitschke@desy.de; hermannrp@ornl.gov RI Hermann, Raphael/F-6257-2013 OI Hermann, Raphael/0000-0002-6138-5624 FU Helmholtz Association of German Research Centers [VH NG-407]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX R.P.H. acknowledges the Helmholtz Association of German Research Centers for funding VH NG-407 "Lattice dynamics in emerging functional materials" and support from the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Portions of this research were carried out at the light source PETRA III at DESY, a member of the Helmholtz Association (HGF). We would like to thank H.-C. Wille and K. Schlage for assistance in using beamline P01 and for support in analyzing the NIS data. We acknowledge helpful comments from M. Manley, J. Budai, and T. Watkins. NR 44 TC 0 Z9 0 U1 6 U2 27 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 16 PY 2016 VL 93 IS 9 AR 094304 DI 10.1103/PhysRevB.93.094304 PG 10 WC Physics, Condensed Matter SC Physics GA DG9KI UT WOS:000372401000002 ER PT J AU Bousso, R Fisher, Z Leichenauer, S Wall, AC AF Bousso, Raphael Fisher, Zachary Leichenauer, Stefan Wall, Aron C. TI Quantum focusing conjecture SO PHYSICAL REVIEW D LA English DT Article ID BLACK-HOLE ENTROPY; ONE-LOOP RENORMALIZATION; NOETHER CHARGE; ENTANGLEMENT ENTROPY; DYNAMICAL ORIGIN; FIELD-THEORY; GRAVITY; ENERGY; SUPERGRAVITY; THERMODYNAMICS AB We propose a universal inequality that unifies the Bousso bound with the classical focusing theorem. Given a surface sigma that need not lie on a horizon, we define a finite generalized entropy S-gen as the area of sigma in Planck units, plus the von Neumann entropy of its exterior. Given a null congruence N orthogonal to sigma, the rate of change of S-gen per unit area defines a quantum expansion. We conjecture that the quantum expansion cannot increase along N. This extends the notion of universal focusing to cases where quantum matter may violate the null energy condition. Integrating the conjecture yields a precise version of the Strominger-Thompson quantum Bousso bound. Applied to locally parallel light-rays, the conjecture implies a novel inequality, the quantum null energy condition, a lower bound on the stress tensor in terms of the second derivative of the von Neumann entropy. We sketch a proof of the latter relation in quantum field theory. C1 [Bousso, Raphael; Fisher, Zachary; Leichenauer, Stefan] Univ Calif Berkeley, Ctr Theoret Phys, Berkeley, CA 94720 USA. [Bousso, Raphael; Fisher, Zachary; Leichenauer, Stefan] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bousso, Raphael; Fisher, Zachary; Leichenauer, Stefan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Wall, Aron C.] Inst Adv Study, Olden Lane, Princeton, NJ 08540 USA. RP Bousso, R (reprint author), Univ Calif Berkeley, Ctr Theoret Phys, Berkeley, CA 94720 USA.; Bousso, R (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Bousso, R (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. OI Wall, Aron/0000-0002-6968-0425 FU Berkeley Center for Theoretical Physics; National Science Foundation [1214644, 1316783]; fqxi Grant [RFP3-1323]; US Department of Energy [DE-AC02-05CH11231]; NSF [PHY-1314311]; Institute for Advanced Study FX It is a pleasure to thank C. Akers, E. Bianchi, W. Donnelly, N. Engelhardt, B. Freivogel, M. Headrick, G. Horowitz, T. Jacobson, J. Koeller, J. Maldacena, D. Marolf, and D. Simmons-Duffin for discussions. The work of R. B., Z. F., and S. L. is supported in part by the Berkeley Center for Theoretical Physics, by the National Science Foundation (Awards No. 1214644 and No. 1316783), by fqxi Grant No. RFP3-1323, and by the US Department of Energy under Contract No. DE-AC02-05CH11231. The work of A. W. is supported in part by NSF Grant No. PHY-1314311 and the Institute for Advanced Study. NR 126 TC 13 Z9 13 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 16 PY 2016 VL 93 IS 6 AR 064044 DI 10.1103/PhysRevD.93.064044 PG 20 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG9RA UT WOS:000372420300006 ER PT J AU Upadhye, A Kwan, J Pope, A Heitmann, K Habib, S Finkel, H Frontiere, N AF Upadhye, Amol Kwan, Juliana Pope, Adrian Heitmann, Katrin Habib, Salman Finkel, Hal Frontiere, Nicholas TI Redshift-space distortions in massive neutrino and evolving dark energy cosmologies SO PHYSICAL REVIEW D LA English DT Article ID MICROWAVE BACKGROUND ANISOTROPIES; MATTER POWER SPECTRUM; CONSTANT PROBLEM; PARAMETER CONSTRAINTS; COSMIC ACCELERATION; GALAXIES; PROBE; INTEGRATION; UNIVERSES; EMULATION AB Large-scale structure surveys in the coming years will measure the redshift-space power spectrum to unprecedented accuracy, allowing for powerful new tests of the Lambda cold dark matter (Lambda CDM) picture as well as measurements of particle physics parameters such as the neutrino masses. We extend the time-renormalization-group (RG) perturbative framework to redshift space, computing the power spectrum P-s(k, mu) in massive neutrino cosmologies with time-dependent dark energy equations of state w(z). Time-RG is uniquely capable of incorporating scale-dependent growth into the P-s(k, mu) computation, which is important for massive neutrinos as well as modified gravity models. Although changes to w(z) and the neutrino mass fraction both affect the late-time scale dependence of the nonlinear power spectrum, we find that the two effects depend differently on the line-of-sight angle mu. Finally, we use the HACC N-body code to quantify errors in the perturbative calculations. For a Lambda CDM model at redshift z = 1, our procedure predicts the monopole (quadrupole) to 1% accuracy up to a wave number 0.19h/Mpc (0.28h/Mpc), compared to 0.08h/Mpc (0.07h/Mpc) for the Kaiser approximation and 0.19h/Mpc (0.16h/Mpc) for the current state-of-the-art perturbation scheme. Our calculation agrees with the simulated redshift-space power spectrum even for neutrino masses above the current bound, and for rapidly evolving dark energy equations of state, vertical bar dw/dz vertical bar similar to 1. Along with this article, we make our redshift-space time-RG implementation publicly available as the code REDTIME. C1 [Upadhye, Amol] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kwan, Juliana] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Pope, Adrian; Heitmann, Katrin; Habib, Salman; Frontiere, Nicholas] Argonne Natl Lab, Div High Energy Phys, 9700 South Cass Ave, Lemont, IL 60439 USA. [Heitmann, Katrin; Habib, Salman] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Heitmann, Katrin; Habib, Salman] Argonne Natl Lab, Div Math & Comp Sci, 9700 S Cass Ave, Lemont, IL 60439 USA. [Finkel, Hal] Argonne Natl Lab, ALCF, 9700 S Cass Ave, Lemont, IL 60439 USA. [Frontiere, Nicholas] Univ Chicago, Dept Phys, Chicago, IL 60637 USA. RP Upadhye, A (reprint author), Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. FU U.S. Department of Energy, Basic Energy Sciences, Office of Science [DE-AC02-06CH11357]; DOE/SC [DE-AC02-06CH11357, DE-AC05-00OR22725]; Argonne, a U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX We are grateful to D. Chung, E. Jennings, T. Okumura, and M. Takada for the insightful discussions. The authors were supported by the U.S. Department of Energy, Basic Energy Sciences, Office of Science, under Contract No. DE-AC02-06CH11357. This research used resources of the ALCF, which is supported by the DOE/SC under Contract No. DE-AC02-06CH11357 and the resources of the OLCF, which is supported by the DOE/SC under Contract No. DE-AC05-00OR22725. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. NR 69 TC 2 Z9 2 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 16 PY 2016 VL 93 IS 6 AR 063515 DI 10.1103/PhysRevD.93.063515 PG 18 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG9RA UT WOS:000372420300002 ER PT J AU Ross, DE Marshall, CW May, HD Norman, RS AF Ross, Daniel E. Marshall, Christopher W. May, Harold D. Norman, R. Sean TI Comparative Genomic Analysis of Sulfurospirillum cavolei MES Reconstructed from the Metagenome of an Electrosynthetic Microbiome SO PLOS ONE LA English DT Article ID SULFUR-REDUCING BACTERIUM; NITROUS-OXIDE REDUCTASE; DNA-DNA HYBRIDIZATION; WOLINELLA-SUCCINOGENES; SP-NOV.; DEHALOSPIRILLUM-MULTIVORANS; EPSILON-PROTEOBACTERIA; SUBSYSTEMS TECHNOLOGY; SPECIES DEFINITION; GENE-CLUSTER AB Sulfurospirillum spp. play an important role in sulfur and nitrogen cycling, and contain metabolic versatility that enables reduction of a wide range of electron acceptors, including thiosulfate, tetrathionate, polysulfide, nitrate, and nitrite. Here we describe the assembly of a Sulfurospirillum genome obtained from the metagenome of an electrosynthetic microbiome. The ubiquity and persistence of this organismin microbial electrosynthesis systems suggest it plays an important role in reactor stability and performance. Understanding why this organism is present and elucidating its genetic repertoire provide a genomic and ecological foundation for future studies where Sulfurospirillum are found, especially in electrode-associated communities. Metabolic comparisons and in-depth analysis of unique genes revealed potential ecological niche-specific capabilities within the Sulfurospirillum genus. The functional similarities common to all genomes, i.e., core genome, and unique gene clusters found only in a single genome were identified. Based upon 16S rRNA gene phylogenetic analysis and average nucleotide identity, the Sulfurospirillum draft genome was found to be most closely related to Sulfurospirillum cavolei. Characterization of the draft genome described herein provides pathway-specific details of the metabolic significance of the newly described Sulfurospirillum cavolei MES and, importantly, yields insight to the ecology of the genus as a whole. Comparison of eleven sequenced Sulfurospirillum genomes revealed a total of 6246 gene clusters in the pan-genome. Of the total gene clusters, 18.5% were shared among all eleven genomes and 50% were unique to a single genome. While most Sulfurospirillum spp. reduce nitrate to ammonium, five of the eleven Sulfurospirillum strains encode for a nitrous oxide reductase (nos) cluster with an atypical nitrous-oxide reductase, suggesting a utility for this genus in reduction of the nitrous oxide, and as a potential sink for this potent greenhouse gas. C1 [Ross, Daniel E.; Norman, R. Sean] Univ S Carolina, Arnold Sch Publ Hlth, Dept Environm Hlth Sci, Columbia, SC 29208 USA. [Marshall, Christopher W.; May, Harold D.] Med Univ S Carolina, Dept Microbiol & Immunol, Marine Biomed & Environm Sci Ctr, Charleston, SC 29425 USA. [Ross, Daniel E.] Natl Energy Technol Lab, Pittsburgh, PA USA. [Marshall, Christopher W.] Argonne Natl Lab, Lemont, IL USA. RP Norman, RS (reprint author), Univ S Carolina, Arnold Sch Publ Hlth, Dept Environm Hlth Sci, Columbia, SC 29208 USA. EM rsnorman@mailbox.sc.edu FU U.S. Department of Energy, Advanced Research Project Agency-Energy [DE-AR0000089] FX Funding was provided by the U.S. Department of Energy, Advanced Research Project Agency-Energy (award DE-AR0000089).; Funding was provided by the U.S. Department of Energy, Advanced Research Project Agency-Energy (award DE-AR0000089). We would like to thank JGI and Barbara Campbell (Clemson University) for permission to utilize the Sulfurospirillum sp. Am-N assembled contigs in our comparative genome analysis. These sequence data were produced by the US Department of Energy Joint Genome Institute (http://www.jgi.doe.gov/) in collaboration with the user community. We would also like to thank the editor and reviewers of the manuscript for the helpful comments. NR 85 TC 2 Z9 2 U1 3 U2 12 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 16 PY 2016 VL 11 IS 3 AR e0151214 DI 10.1371/journal.pone.0151214 PG 26 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH1WF UT WOS:000372574900069 PM 26983005 ER PT J AU Carrigan, CR Sun, YW Hunter, SL Ruddle, DG Wagoner, JL Myers, KBL Emer, DF Drellack, SL Chipman, VD AF Carrigan, Charles R. Sun, Yunwei Hunter, Steven L. Ruddle, David G. Wagoner, Jeffrey L. Myers, Katherine B. L. Emer, Dudley F. Drellack, Sigmund L. Chipman, Veraun D. TI Delayed signatures of underground nuclear explosions SO SCIENTIFIC REPORTS LA English DT Article ID GAS-TRANSPORT; NORTH-KOREA AB Radionuclide signals from underground nuclear explosions (UNEs) are strongly influenced by the surrounding hydrogeologic regime. One effect of containment is delay of detonation-produced radioxenon reaching the surface as well as lengthening of its period of detectability compared to uncontained explosions. Using a field-scale tracer experiment, we evaluate important transport properties of a former UNE site. We observe the character of signals at the surface due to the migration of gases from the post-detonation chimney under realistic transport conditions. Background radon signals are found to be highly responsive to cavity pressurization suggesting that large local radon anomalies may be an indicator of a clandestine UNE. Computer simulations, using transport properties obtained from the experiment, track radioxenon isotopes in the chimney and their migration to the surface. They show that the chimney surrounded by a fractured containment regime behaves as a leaky chemical reactor regarding its effect on isotopic evolution introducing a dependence on nuclear yield not previously considered. This evolutionary model for radioxenon isotopes is validated by atmospheric observations of radioxenon from a 2013 UNE in the Democratic People's Republic of Korea (DPRK). Our model produces results similar to isotopic observations with nuclear yields being comparable to seismic estimates. C1 [Carrigan, Charles R.; Sun, Yunwei; Hunter, Steven L.; Ruddle, David G.; Wagoner, Jeffrey L.; Myers, Katherine B. L.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Emer, Dudley F.; Drellack, Sigmund L.; Chipman, Veraun D.] Natl Secur Technol, Las Vegas, NV USA. RP Carrigan, CR (reprint author), Lawrence Livermore Natl Lab, Livermore, CA USA. EM carrigan1@llnl.gov FU Office of Proliferation Detection [NA-221]; U.S. Department of Energy; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX We thank Nathan G. Wimer, Steven A. Kreek, David LaGraffe, Donald J. Felske and Kevin Grot for critical reviews, helpful discussions, field support and gas analyses; the National Nuclear Security Administration, Office of Defense Nuclear Nonproliferation Research and Development (DNN R&D) and the Comprehensive Inspection Technologies working group, a multi-institutional and interdisciplinary group of scientists and engineers. We also thank the Defense Logistics Agency for their support in obtaining bottles of the Freon tracer gas. Finally, we thank five anonymous reviewers for constructive reviews of this work. This research was funded by the Office of Proliferation Detection (NA-221), U.S. Department of Energy and performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 24 TC 0 Z9 0 U1 6 U2 14 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 16 PY 2016 VL 6 AR 23032 DI 10.1038/srep23032 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG4RE UT WOS:000372059200001 PM 26979288 ER PT J AU Sun, ZQ Song, G Sisneros, TA Clausen, B Pu, C Li, L Gao, YF Liaw, PK AF Sun, Zhiqian Song, Gian Sisneros, Thomas A. Clausen, Bjorn Pu, Chao Li, Lin Gao, Yanfei Liaw, Peter K. TI Load partitioning between the bcc-iron matrix and NiAl-type precipitates in a ferritic alloy on multiple length scales SO SCIENTIFIC REPORTS LA English DT Article ID NEUTRON-DIFFRACTION; MECHANICAL-PROPERTIES; INTERMETALLIC COMPOUND; STRAIN-RATE; FE-19WT-PERCENT-CR ALLOYS; TENSILE DEFORMATION; CREEP-RESISTANT; AL; TEMPERATURE; STEELS AB An understanding of load sharing among constituent phases aids in designing mechanical properties of multiphase materials. Here we investigate load partitioning between the body-centered-cubic iron matrix and NiAl-type precipitates in a ferritic alloy during uniaxial tensile tests at 364 and 506 degrees C on multiple length scales by in situ neutron diffraction and crystal plasticity finite element modeling. Our findings show that the macroscopic load-transfer efficiency is not as high as that predicted by the Eshelby model; moreover, it depends on the matrix strain-hardening behavior. We explain the grain-level anisotropic load-partitioning behavior by considering the plastic anisotropy of the matrix and elastic anisotropy of precipitates. We further demonstrate that the partitioned load on NiAl-type precipitates relaxes at 506 degrees C, most likely through thermally-activated dislocation rearrangement on the microscopic scale. The study contributes to further understanding of load-partitioning characteristics in multiphase materials. C1 [Sun, Zhiqian; Song, Gian; Pu, Chao; Li, Lin; Gao, Yanfei; Liaw, Peter K.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Sisneros, Thomas A.; Clausen, Bjorn] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Liaw, PK (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM pliaw@utk.edu RI Gao, Yanfei/F-9034-2010; Clausen, Bjorn/B-3618-2015; Song, Gian/F-8880-2016; Pu, Chao/F-4256-2016 OI Gao, Yanfei/0000-0003-2082-857X; Clausen, Bjorn/0000-0003-3906-846X; Song, Gian/0000-0001-7462-384X; FU Department of Energy (DOE), Office of Fossil Energy Program [DE-09NT0008089, DE-FE0005868, DE-FE0011194, DE-FE0024054]; National Science Foundation [CMMI 0926798, CMMI 1300223, CMMI 1100080]; DOE Office of Science, Basic Energy Sciences, Materials Science and Engineering Division; Office of Basic Energy Science, DOE; DOE [DE-AC52-06NA-25396] FX The research is supported by the Department of Energy (DOE), Office of Fossil Energy Program, under Grants of DE-09NT0008089, DE-FE0005868, DE-FE0011194, and DE-FE0024054 (ZS, GS, and PKL) with Richard Dunst, Vito Cedro, Patricia Rawls, and Jessica Mullen as the program managers, by the National Science Foundation under grants CMMI 0926798 (LL) CMMI 1300223 (CP), and CMMI 1100080 (PKL), and by DOE Office of Science, Basic Energy Sciences, Materials Science and Engineering Division (YFG). The work has benefitted from the use of the Lujan Neutron Scattering Center at LANSCE, which is funded by the Office of Basic Energy Science, DOE. Los Alamos National Laboratory is operated by the Los Alamos National Security LLC under the DOE contract of DE-AC52-06NA-25396. NR 58 TC 0 Z9 0 U1 3 U2 20 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 16 PY 2016 VL 6 AR 23137 DI 10.1038/srep23137 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG4PV UT WOS:000372055100003 PM 26979660 ER PT J AU Manaa, MR Fried, LE Kuo, IFW AF Manaa, M. Riad Fried, Laurence E. Kuo, I-Feng W. TI Determination of enthalpies of formation of energetic molecules with composite quantum chemical methods SO CHEMICAL PHYSICS LETTERS LA English DT Article ID DENSITY-FUNCTIONAL THEORIES; PENTAERYTHRITOL TETRANITRATE; MECHANICAL CALCULATIONS; DETONATION PROPERTIES; APPROACH CCCA; HEAT; EXPLOSIVES; SUBLIMATION; GAUSSIAN-3; NITROTOLUENES AB We report gas-phase enthalpies of formation for the set of energetic molecules NTO, DADE, LLM-105, TNT, RDX, TATB, HMX, and PETN using the G2, G3, G4, and ccCA-PS3 quantum composite methods. Calculations for HMX and PETN hitherto represent the largest molecules attempted with these methods. G3 and G4 calculations are typically close to one another, with a larger difference found between these methods and ccCA-PS3. Although there is significant uncertainty in experimental values, the mean absolute deviation between the average experimental value and calculations are 12, 6, 7, and 3 kcal/mol for G2, G3, G4, and ccCA-PS3, respectively. (C) 2016 Elsevier B.V. All rights reserved. C1 [Manaa, M. Riad; Fried, Laurence E.; Kuo, I-Feng W.] Lawrence Livermore Natl Lab, Energet Mat Ctr, 7000 East Ave, Livermore, CA 94551 USA. RP Manaa, MR (reprint author), Lawrence Livermore Natl Lab, Energet Mat Ctr, 7000 East Ave, Livermore, CA 94551 USA. EM manaa1@llnl.gov FU U.S. Department of Energy Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Advanced Scientific Computation (ASC) program FX This work is performed under the auspices of the U.S. Department of Energy Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The extensive computational calculations reported in this work would not have been possible without the computational resources provided by the Computational Grand Challenge Program at LLNL. Support from the Advanced Scientific Computation (ASC) program is also greatly appreciated. NR 36 TC 0 Z9 0 U1 9 U2 16 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD MAR 16 PY 2016 VL 648 DI 10.1016/j.cplett.2016.01.071 PG 5 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DF5OS UT WOS:000371402100006 ER PT J AU Zhao, RN Yuan, YH Han, JG Duan, YH AF Zhao, Run-Ning Yuan, Yan-Hong Han, Ju-Guang Duan, Yuhua TI Geometries, stabilities, and electronic properties of tungsten encapsulated nanosize irregular B-n (n=20, 24, 28, and 32) fullerenes: A density functional investigation SO CHEMICAL PHYSICS LETTERS LA English DT Article ID ALL-BORON FULLERENE; CLUSTERS; POTENTIALS AB Geometries associated with relative stabilities and energy gaps of W@B-n (n = 20, 24, 28, 32) are systematically investigated by density functional theory. The calculated averaged atomic binding energies reveal that the W@B-20 has enhanced stability over other clusters. Interestingly, the irregular W@B-24 fullerene with bigger HOMO-LUMO gap is supposed to have stronger chemical activity. Moreover, the interactions between W and B24 cage is strongest one based upon the calculated binding energy between W and B cage, the doped W changes the properties of pure cages. The calculated dipoles of W@B-n reveal that the irregular W@B-24 cage is a nonpolar molecule. (C) 2016 Elsevier B.V. All rights reserved. C1 [Zhao, Run-Ning; Yuan, Yan-Hong] Shanghai Dianji Univ, Inst Appl Math & Phys, Shanghai 201306, Peoples R China. [Han, Ju-Guang] Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Peoples R China. [Duan, Yuhua] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Han, JG (reprint author), Univ Sci & Technol China, Natl Synchrotron Radiat Lab, Hefei 230029, Peoples R China. EM jghan@ustc.edu.cn FU National Natural Science Foundation of China [11179035] FX This work is supported by National Natural Science Foundation of China (11179035). Young Teacher Training Program of Shanghai Education Committee as well as Physical Electronics Disciplines (No. 12XKJC01). NR 25 TC 4 Z9 4 U1 14 U2 24 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2614 EI 1873-4448 J9 CHEM PHYS LETT JI Chem. Phys. Lett. PD MAR 16 PY 2016 VL 648 DI 10.1016/j.cplett.2016.01.052 PG 6 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DF5OS UT WOS:000371402100008 ER PT J AU Nasreen, F Antonio, D VanGennep, D Booth, CH Kothapalli, K Bauer, ED Sarrao, JL Lavina, B Iota-Herbei, V Sinogeikin, S Chow, P Xiao, YM Zhao, YS Cornelius, AL AF Nasreen, Farzana Antonio, Daniel VanGennep, Derrick Booth, Corwin H. Kothapalli, Karunakar Bauer, Eric D. Sarrao, John L. Lavina, Barbara Iota-Herbei, Valentin Sinogeikin, Stanislav Chow, Paul Xiao, Yuming Zhao, Yusheng Cornelius, Andrew L. TI High pressure effects on U L-3 x-ray absorption in partial fluorescence yield mode and single crystal x-ray diffraction in the heavy fermion compound UCd11 SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Article DE high pressure; x-ray absorption; single crystal x-ray diffraction; uranium intermetallic; heavy fermion; UCd11 ID PLUTONIUM INTERMETALLICS; ANTIFERROMAGNET UCD11; SYSTEM UCD11; 5F ORBITALS; TRANSITION; SCATTERING; URANIUM; SOLIDS; STATE; HPCAT AB We report a study of high pressure x-ray absorption (XAS) performed in the partial fluorescence yield mode (PFY) at the U L-3 edge (0-28.2 GPa) and single crystal x-ray diffraction (SXD) (0-20 GPa) on the UCd11 heavy fermion compound at room temperature. Under compression, the PFY-XAS results show that the white line is shifted by +4.1(3) eV at the highest applied pressure of 28.2 GPa indicating delocalization of the 5f electrons. The increase in full width at half maxima and decrease in relative amplitude of the white line with respect to the edge jump point towards 6d band broadening under high pressure. A bulk modulus of K-0 = 62(1) GPa and its pressure derivative, K-0(') = 4.9(2) was determined from high pressure SXD results. Both the PFY-XAS and diffraction results do not show any sign of a structural phase transition in the applied pressure range. C1 [Nasreen, Farzana; Antonio, Daniel; Lavina, Barbara; Iota-Herbei, Valentin; Zhao, Yusheng; Cornelius, Andrew L.] Univ Nevada, High Pressure Sci & Engn Ctr HiPSEC, Las Vegas, NV 89154 USA. [Nasreen, Farzana; Antonio, Daniel; Lavina, Barbara; Iota-Herbei, Valentin; Zhao, Yusheng; Cornelius, Andrew L.] Univ Nevada, Dept Phys & Astron, Las Vegas, NV 89154 USA. [VanGennep, Derrick] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Booth, Corwin H.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Kothapalli, Karunakar] US DOE, Ames Lab, Ames, IA 50011 USA. [Kothapalli, Karunakar] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Bauer, Eric D.; Sarrao, John L.] Los Alamos Natl Lab, POB 1663,MS K764, Los Alamos, NM 87545 USA. [Sinogeikin, Stanislav; Chow, Paul; Xiao, Yuming] Argonne Natl Lab, Carnegie Inst Washington, High Pressure Collaborat Access Team, Argonne, IL 60439 USA. RP Nasreen, F (reprint author), Univ Nevada, High Pressure Sci & Engn Ctr HiPSEC, Las Vegas, NV 89154 USA.; Nasreen, F (reprint author), Univ Nevada, Dept Phys & Astron, Las Vegas, NV 89154 USA. EM farzana6109@gmail.com RI Lavina, Barbara/A-1015-2010; OI Lavina, Barbara/0000-0002-8556-7916; Bauer, Eric/0000-0003-0017-1937 FU DOE/EPSCoR (Experimental Program to Stimulate Competitive Research) University/National Laboratory Partnership [DE-SC0005278]; National Nuclear Security Administration (NNSA) under the Stewardship Science Academic Alliances program through DOE Cooperative Agreement [DE-NA0001982]; Office of Science, Office of Basic Energy Sciences (OBES), of the U.S. DOE [DE-AC02-05CH11231]; DOE-NNSA [DE-NA0001974]; DOE-BES [DE-FG02-99ER45775]; NSF; ANL [DE-AC02-06CH11357]; U.S. DOE, OBES, Division of Materials Sciences and Engineering FX We acknowledge fruitful discussion with Ladislav Havela and Jon Lawrence. We thank Curtis Kenney-Benson for his assistance at HPCAT (Sector 16), APS, Argonne National Laboratory (ANL). This work was supported by DOE/EPSCoR (Experimental Program to Stimulate Competitive Research) University/National Laboratory Partnership (DE-SC0005278). The research work at High Pressure Science and Engineering Center (HiPSEC) at University of Nevada at Las Vegas (UNLV) was sponsored by the National Nuclear Security Administration (NNSA) under the Stewardship Science Academic Alliances program through DOE Cooperative Agreement #DE-NA0001982. Work at Lawrence Berkeley National Laboratory was supported by the Director, Office of Science, Office of Basic Energy Sciences (OBES), of the U.S. DOE under Contract No. DE-AC02-05CH11231. Portions of this work were performed at HPCAT (Sector 16), APS, ANL. HPCAT operations are supported by DOE-NNSA under Award No. DE-NA0001974 and DOE-BES under Award No. DE-FG02-99ER45775, with partial instrumentation funding by NSF. APS is a U.S. DOE Office of Science User Facility operated for the DOE Office of Science by ANL under Contract No. DE-AC02-06CH11357. Sample preparation at LANL was performed under the auspices of the U.S. DOE, OBES, Division of Materials Sciences and Engineering. NR 46 TC 1 Z9 1 U1 7 U2 22 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD MAR 16 PY 2016 VL 28 IS 10 AR 105601 DI 10.1088/0953-8984/28/10/105601 PG 7 WC Physics, Condensed Matter SC Physics GA DF0CY UT WOS:000371007800011 PM 26877538 ER PT J AU Chen, CR Cheng, HC Low, I AF Chen, Chuan-Ren Cheng, Hsin-Chia Low, Ian TI Same-sign dilepton excesses and vector-like quarks SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadronic Colliders; Phenomenological Models ID MASS; PAIR AB Multiple analyses from ATLAS and CMS collaborations, including searches for ttH production, supersymmetric particles and vector-like quarks, observed excesses in the same-sign dilepton channel containing b-jets and missing transverse energy in the LHC Run 1 data. In the context of little Higgs theories with T parity, we explain these excesses using vector-like T-odd quarks decaying into a top quark, a W boson and the lightest T-odd particle (LTP). For heavy vector -like quarks, decay topologies containing the LTP have not been searched for at the LHC. The bounds on the masses of the T -odd quarks can be estimated in a simplified model approach by adapting the search limits for top/bottom squarks in supersymmetry. Assuming a realistic decay branching fraction, a benchmark with a 750 GeV T-odd b' quark is proposed. We also comment on the possibility to fit excesses in different analyses in a common framework. C1 [Chen, Chuan-Ren] Natl Taiwan Normal Univ, Dept Phys, Ting Chou Rd, Taipei 116, Taiwan. [Cheng, Hsin-Chia] Univ Calif Davis, Dept Phys, One Shields Ave, Davis, CA 95616 USA. [Low, Ian] Northwestern Univ, Dept Phys & Astron, Sheridan Rd, Evanston, IL 60208 USA. [Low, Ian] Argonne Natl Lab, Div High Energy Phys, S Cass Ave, Argonne, IL 60439 USA. RP Chen, CR (reprint author), Natl Taiwan Normal Univ, Dept Phys, Ting Chou Rd, Taipei 116, Taiwan.; Cheng, HC (reprint author), Univ Calif Davis, Dept Phys, One Shields Ave, Davis, CA 95616 USA.; Low, I (reprint author), Northwestern Univ, Dept Phys & Astron, Sheridan Rd, Evanston, IL 60208 USA.; Low, I (reprint author), Argonne Natl Lab, Div High Energy Phys, S Cass Ave, Argonne, IL 60439 USA. EM crchen@ntnu.edu; cheng@physics.ucdavis.edu; ilow@northwestern.edu FU National Center for Theoretical Sciences (NCTS); National Science Council of R.O.C. [NSC 102-2112-M-003-001-MY3]; U.S. Department of Energy [DE-SC-000999, DE-AC02-06CH11357, DE-SC0010143] FX C.-R. C. would like to acknowledge the support of National Center for Theoretical Sciences (NCTS). H.-C. C. would like to thank Academia Sinica in Taiwan for hospitality while part of this work was done. I. L. acknowledges helpful discussions with Aurelio Juste regarding the ATLAS exotica search. We thank the authors of ref. [1] for providing the event file for the stop benchmark used in their study. The work of C.-R. C. is supported in part by the National Science Council of R.O.C. under Grants No. NSC 102-2112-M-003-001-MY3. H.-C. C is supported in part by U.S. Department of Energy grant DE-SC-000999. I. L. is supported in part by the U.S. Department of Energy under Contracts No. DE-AC02-06CH11357 and No. DE-SC0010143. NR 50 TC 4 Z9 4 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 15 PY 2016 IS 3 AR 098 DI 10.1007/JHEP03(2016)098 PG 16 WC Physics, Particles & Fields SC Physics GA DL0HE UT WOS:000375312300007 ER PT J AU Cohen, T Craig, N Knapen, S AF Cohen, Timothy Craig, Nathaniel Knapen, Simon TI Gauge mediated mini-split SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Supersymmetry Phenomenology ID RENORMALIZATION-GROUP EQUATIONS; QUANTUM-FIELD THEORY; SUPERSYMMETRY BREAKING; SYMMETRY-BREAKING; STANDARD MODEL; SCALE; CONSTRAINTS; BOSON; MASS; LHC AB We propose a simple model of split supersymmetry from gauge mediation. This model features gauginos that are parametrically a loop factor lighter than scalars, accommodates a Higgs boson mass of 125 GeV, and incorporates a simple solution to the mu - b(mu) problem. The gaugino mass suppression can be understood as resulting from collective symmetry breaking. Imposing collider bounds on mu and requiring viable electroweak symmetry breaking implies small a-terms and small tan beta - the stop mass ranges from 10(5) to 10(8) GeV. In contrast with models with anomaly + gravity mediation (which also predict a one-loop loop suppression for gaugino masses), our gauge mediated scenario predicts aligned squark masses and a gravitino LSP. Gluinos, electroweakinos and Higgsinos can be accessible at the LHC and/or future colliders for a wide region of the allowed parameter space. C1 [Cohen, Timothy] Univ Oregon, Inst Theoret Sci, Eugene, OR 97403 USA. [Craig, Nathaniel] Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA. [Knapen, Simon] Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. [Knapen, Simon] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Cohen, T (reprint author), Univ Oregon, Inst Theoret Sci, Eugene, OR 97403 USA.; Craig, N (reprint author), Univ Calif Santa Barbara, Dept Phys, Santa Barbara, CA 93106 USA.; Knapen, S (reprint author), Univ Calif Berkeley, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA.; Knapen, S (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. EM tcohen@uoregon.edu; ncraig@physics.ucsb.edu; smknapen@lbl.gov FU LHC Theory Initiative Postdoctoral Fellowship, under the National Science Foundation [PHY-0969510]; Department of Energy [DE-SC0014129]; LDRD program of LBNL under under DoE [DE-AC02-05CH11231]; National Science Foundation [PHY-1066293] FX We thank Csaba Csaki, Keiseke Harigaya, Markus Luty, Diego Redigolo, Giovanni Villadoro for useful discussions. TC is supported by an LHC Theory Initiative Postdoctoral Fellowship, under the National Science Foundation grant PHY-0969510. NC is supported by the Department of Energy under the grant DE-SC0014129. The work of SK is supported in part by the LDRD program of LBNL under under DoE contract DE-AC02-05CH11231. We acknowledge the hospitality of the Aspen Center for Physics, supported by the National Science Foundation Grant number PHY-1066293, where parts of this work were completed. NR 69 TC 3 Z9 3 U1 0 U2 1 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 15 PY 2016 IS 3 AR 103 DI 10.1007/JHEP03(2016)103 PG 17 WC Physics, Particles & Fields SC Physics GA DL0GO UT WOS:000375310600002 ER PT J AU Mueller, AH Szymanowski, L Wallon, S Xiao, BW Yuan, F AF Mueller, A. H. Szymanowski, Lech Wallon, Samuel Xiao, Bo-Wen Yuan, Feng TI Sudakov resummations in Mueller-Navelet dijet production SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Jets; QCD Phenomenology ID TRANSVERSE-MOMENTUM DISTRIBUTION; NLO JET VERTEX; BFKL POMERON; SCATTERING; QCD; UNIVERSALITY; PART AB In high energy hadron-hadron collisions, dijet production with large rapidity separation proposed by Mueller and Navelet, is one of the most interesting processes which can help us to directly access the well-known Balitsky-Fadin-Kuraev-Lipatov evolution dynamics. The objective of this work is to study the Sudakov resummation of Mueller-Navelet jets. Through the one-loop calculation, Sudakov type logarithms are obtained for this process when the produced dijets are almost back-to-back. These results could play an important role in the phenomenological study of dijet correlations with large rapidity separation at the LHC. C1 [Mueller, A. H.] Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA. [Szymanowski, Lech] Natl Ctr Nucl Res NCBJ, Warsaw, Poland. [Wallon, Samuel] Univ Paris Saclay, Univ Paris Sud, CNRS, Lab Phys Theor,CNRS,UMR 8627, F-91405 Orsay, France. [Wallon, Samuel] Univ Paris 06, Fac Phys, 4 Pl Jussieu, F-75252 Paris 05, France. [Xiao, Bo-Wen] Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China. [Xiao, Bo-Wen] Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China. [Yuan, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Mueller, AH (reprint author), Columbia Univ, Dept Phys, 538 W 120th St, New York, NY 10027 USA.; Szymanowski, L (reprint author), Natl Ctr Nucl Res NCBJ, Warsaw, Poland.; Wallon, S (reprint author), Univ Paris Saclay, Univ Paris Sud, CNRS, Lab Phys Theor,CNRS,UMR 8627, F-91405 Orsay, France.; Wallon, S (reprint author), Univ Paris 06, Fac Phys, 4 Pl Jussieu, F-75252 Paris 05, France.; Xiao, BW (reprint author), Cent China Normal Univ, Key Lab Quark & Lepton Phys MOE, Wuhan 430079, Peoples R China.; Xiao, BW (reprint author), Cent China Normal Univ, Inst Particle Phys, Wuhan 430079, Peoples R China.; Yuan, F (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Nucl Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM amh@phys.columbia.edu; lech@cpht.polytechnique.fr; Samuel.Wallon@th.u-psud.fr; bxiao@mail.ccnu.edu.cn; fyuan@lbl.gov FU U.S. Department of Energy [DE-AC02-05CH11231]; NSFC [11575070]; National Science Center, Poland [2015/17/B/ST2/01838] FX This work was supported in part by the U.S. Department of Energy under the contracts DE-AC02-05CH11231 and by the NSFC under Grant No. 11575070. B.X. wishes to thank Dr. F. Yuan and the nuclear theory group at LBNL for hospitality and support during his visit when this work is initiated. L.Sz. was supported by grant of National Science Center, Poland, No. 2015/17/B/ST2/01838. NR 35 TC 2 Z9 2 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 15 PY 2016 IS 3 AR 096 DI 10.1007/JHEP03(2016)096 PG 24 WC Physics, Particles & Fields SC Physics GA DL0HE UT WOS:000375312300005 ER PT J AU Hong, TZ Taylor-Lange, SC D'Oca, S Yang, D Corgnati, SP AF Hong, Tianzhen Taylor-Lange, Sarah C. D'Oca, Simona Yang, Da Corgnati, Stefano P. TI Advances in research and applications of energy-related occupant behavior in buildings SO ENERGY AND BUILDINGS LA English DT Article DE Occupant behavior; Behavior modeling; Building performance simulation; Energy use; Building design and operation ID RESIDENTIAL BUILDINGS; PERFORMANCE SIMULATION; THERMAL SENSATION; OFFICE BUILDINGS; USER BEHAVIOR; CONSUMPTION; DEMAND; COMFORT; IMPACT; FRAMEWORK AB Occupant behavior is one of the major factors influencing building energy consumption and contributing to uncertainty in building energy use prediction and simulation. Currently the understanding of occupant behavior is insufficient both in building design, operation and retrofit, leading to incorrect simplifications in modeling and analysis. This paper introduced the most recent advances and current obstacles in modeling occupant behavior and quantifying its impact on building energy use. The major themes include advancements in data collection techniques, analytical and modeling methods, and simulation applications which provide insights into behavior energy savings potential and impact. There has been growing research and applications in this field, but significant challenges and opportunities still lie ahead. (C) 2015 The Authors. Published by Elsevier B.V. This is an open access article under the CC BY-NC-ND license. C1 [Hong, Tianzhen; Taylor-Lange, Sarah C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [D'Oca, Simona; Corgnati, Stefano P.] Politecn Torino, Corso Duca Abruzzi 24, I-10129 Turin, Italy. [Yang, Da] Tsinghua Univ, 30 Shuangqing Rd, Beijing 100084, Peoples R China. RP Hong, TZ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM thong@lbl.gov FU United States Department of Energy under the U.S.-China Clean Energy Research Center for Building Energy Efficiency [DE-AC02-05CH11231] FX This work was sponsored by the United States Department of Energy (Contract No. DE-AC02-05CH11231) under the U.S.-China Clean Energy Research Center for Building Energy Efficiency. This work is also part of the research activities of the International Energy Agency Energy in Buildings and Communities Program Annex 66, Definition and Simulation of Occupant Behavior in Buildings. NR 71 TC 6 Z9 6 U1 3 U2 8 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0378-7788 EI 1872-6178 J9 ENERG BUILDINGS JI Energy Build. PD MAR 15 PY 2016 VL 116 BP 694 EP 702 DI 10.1016/j.enbuild.2015.11.052 PG 9 WC Construction & Building Technology; Energy & Fuels; Engineering, Civil SC Construction & Building Technology; Energy & Fuels; Engineering GA DJ0AH UT WOS:000373863300062 ER PT J AU Ilton, ES Post, JE Heaney, PJ Ling, FT Kerisit, SN AF Ilton, Eugene S. Post, Jeffrey E. Heaney, Peter J. Ling, Florence T. Kerisit, Sebastien N. TI XPS determination of Mn oxidation states in Mn (hydr)oxides SO APPLIED SURFACE SCIENCE LA English DT Article DE XPS; Manganese; Valence; Birnessite; Catalysis; Oxidation ID X-RAY-DIFFRACTION; MANGANESE OXIDE MINERALS; NA-RICH BIRNESSITE; CHROMIUM(III) OXIDATION; WATER OXIDATION; HEXAGONAL BIRNESSITE; MULTIPLET STRUCTURE; CR(III) OXIDATION; RIETVELD REFINEMENT; XANES SPECTROSCOPY AB Hydrous manganese oxides are an important class of minerals that help regulate the geochemical redox cycle in near-surface environments and are also considered to be promising catalysts for energy applications such as the oxidation of water. A complete characterization of these minerals is required to better understand their catalytic and redox activity. In this contribution an empirical methodology using X-ray photoelectron spectroscopy (XPS) is developed to quantify the oxidation state of hydrous multivalent manganese oxides with an emphasis on birnessite, a layered structure that occurs commonly in soils but is also the oxidized endmember in biomimetic water-oxidation catalysts. The Mn2p(3/2), Mn3p, and Mn3s lines of near monovalent Mn(II), Mn(III), and Mn(IV) oxides were fit with component peaks; after the best fit was obtained the relative widths, heights and binding energies of the components were fixed. Unknown multivalent samples were fit such that binding energies, intensities, and peak-widths of each oxidation state, composed of a packet of correlated component peaks, were allowed to vary. Peak-widths were constrained to maintain the difference between the standards. Both average and individual mole fraction oxidation states for all three energy levels were strongly correlated, with close agreement between Mn3s and Mn3p analyses, whereas calculations based on the Mn2p(3/2) spectra gave systematically more reduced results. Limited stoichiometric analyses were consistent with Mn3p and Mn3s. Further, evidence indicates the shape of the Mn3p line was less sensitive to the bonding environment than that for Mn2p. Consequently, fitting the Mn3p and Mn3s lines yielded robust quantification of oxidation states over a range of Mn (hydr)oxide phases. In contrast, a common method for determining oxidation states that utilizes the multiplet splitting of the Mn3s line was found to be not appropriate for birnessites. (C) 2016 Published by Elsevier B.V. C1 [Ilton, Eugene S.; Kerisit, Sebastien N.] Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. [Post, Jeffrey E.] Smithsonian Inst, Dept Mineral Sci, NHB 119,POB 37012, Washington, DC 20013 USA. [Heaney, Peter J.; Ling, Florence T.] Penn State Univ, Dept Geosci, University Pk, PA 16802 USA. RP Ilton, ES (reprint author), Pacific NW Natl Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM eugene.ilton@pnnl.gov OI Ling, Florence/0000-0002-2576-3608 FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; U.S. DOE's Office of Biological and Environmental Research; DOE by Battelle Memorial Institute [DE-AC06-76RLO-1830]; NSF [EAR11-47728] FX ESI and SNK were supported by the PNNL managed Geosciences Research Program of the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. The research was performed in part using the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the U.S. DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory (PNNL). PNNL is operated for DOE by Battelle Memorial Institute under Contract# DE-AC06-76RLO-1830. We also acknowledge support from NSF EAR11-47728. We thank Paul Bagus for comments on an earlier version of the manuscript and both Manjula Nandasiri and Ashleigh Schwarz for operating the XPS facility. Comments by two anonymous reviewers are greatly appreciated. NR 64 TC 10 Z9 10 U1 43 U2 88 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0169-4332 EI 1873-5584 J9 APPL SURF SCI JI Appl. Surf. Sci. PD MAR 15 PY 2016 VL 366 BP 475 EP 485 DI 10.1016/j.apsusc.2015.12.159 PG 11 WC Chemistry, Physical; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter SC Chemistry; Materials Science; Physics GA DH1AT UT WOS:000372517500058 ER PT J AU Xu, SC Zhao, ZC Hu, MY Han, XW Hu, JZ Bao, XH AF Xu, Suochang Zhao, Zhenchao Hu, Mary Y. Han, Xiuwen Hu, Jian Zhi Bao, Xinhe TI Investigation of water assisted phase transformation process from AlPO4-5 to AlPO4-tridymite SO MICROPOROUS AND MESOPOROUS MATERIALS LA English DT Article DE AlPO4-5; Molecular sieves; In situ; Multinuclear NMR; Phase transformation ID ALUMINOPHOSPHATE MOLECULAR-SIEVES; IONOTHERMAL SYNTHESIS; MAS NMR; CRYSTALLIZATION; ZEOLITES; DIFFRACTION; CONVERSION; FRAMEWORKS; SAPO-34 AB Water assisted phase transformation process from crystalized AlPO4-5 to AlPO4-tridymite was studied by the combination of X-ray diffraction (XRD), Scanning Electron Microscopy (SEM) and in situ multinuclear MAS NMR. It is found that water first activates the residue amorphous aluminophosphate in crystalized AlPO4-5 sample through hydrolysis and condensation reactions. Then the activated aluminophosphate species reassemble into AlPO4-tridymite crystalline. Meanwhile, AlPO4-5 transforms into orthorhombic phase during heating process. With further crystallization of AlPO4-tridymite, the amorphous phase is gradually consumed, and mass transportation between AlPO4-5 and AlPO4-tridymite is established through gradually amorphization of AlPO4-5. Finally, most of the AlPO4-5 transforms into the thermodynamically stable dense phase AlPO4-tridymite. (C) 2015 Elsevier Inc. All rights reserved. C1 [Xu, Suochang; Han, Xiuwen; Bao, Xinhe] Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China. [Xu, Suochang; Zhao, Zhenchao; Hu, Mary Y.; Hu, Jian Zhi] Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99354 USA. [Xu, Suochang; Zhao, Zhenchao; Hu, Mary Y.; Hu, Jian Zhi] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. [Xu, Suochang] Univ Chinese Acad Sci, Beijing 100039, Peoples R China. RP Bao, XH (reprint author), Chinese Acad Sci, Dalian Inst Chem Phys, State Key Lab Catalysis, Dalian 116023, Peoples R China.; Hu, JZ (reprint author), Pacific NW Natl Lab, Inst Integrated Catalysis, Richland, WA 99354 USA.; Hu, JZ (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. EM Jianzhi.Hu@pnnl.gov; xhbao@dicp.ac.cn RI Hu, Jian Zhi/F-7126-2012 FU National Natural Science Foundation of China [21321002, 11079005]; U. S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences; DOE's Office of Biological and Environmental Research; DOE by Battelle Memorial Institute [DE-AC06-76RLO 1830] FX This work was financially supported by the National Natural Science Foundation of China (Nos. 21321002 and 11079005). It was also supported by the U. S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Chemical Sciences, Biosciences and Geosciences. All of the NMR experiments were performed in the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research, and located at Pacific Northwest National Laboratory (PNNL). PNNL is a multi-program national laboratory operated for the DOE by Battelle Memorial Institute under Contract DE-AC06-76RLO 1830. NR 32 TC 0 Z9 0 U1 10 U2 26 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-1811 EI 1873-3093 J9 MICROPOR MESOPOR MAT JI Microporous Mesoporous Mat. PD MAR 15 PY 2016 VL 223 BP 241 EP 246 DI 10.1016/j.micromeso.2015.10.039 PG 6 WC Chemistry, Applied; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DI1JE UT WOS:000373251600030 ER PT J AU Doyle, BL AF Doyle, Barney L. TI Parameterization of ion channeling half-angles and minimum yields SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 22nd International Conference on Ion Beam Analysis (IBA) CY JUN 14-19, 2015 CL Opatija, CROATIA SP Ruder Boskovic Inst, Int Atom Energy Agcy, Croatian Ctr Excellence Adv Mat & Sensing Dev, Croatian Minist Sci, Educ & Sports, Fdn Croatian Acad Sci & Arts, CERIC ERIC, Elsevier, FEI, High Voltage Engn Europa B V, IONTOF, Kurt J Lesker Co, Natl Electrostat Corp, Pantechnik, Pfeiffer Vacuum DE Ion channeling; Half-angles; Minimum yields ID SI AB A MS Excel program has been written that calculates ion channeling half-angles and minimum yields in cubic bcc, fcc and diamond lattice crystals. All of the tables and graphs in the three Ion Beam Analysis Handbooks that previously had to be manually looked up and read from were programed into Excel in handy lookup tables, or parameterized, for the case of the graphs, using rather simple exponential functions with different power functions of the arguments. The program then offers an extremely convenient way to calculate axial and planar half-angles, minimum yields, effects on half-angles and minimum yields of amorphous overlayers. The program can calculate these half-angles and minimum yields for < uvw > axes and [hkl] planes up to (555). The program is open source and available at http://www.sandia.govipcnscidepartmentsiibaiibatable.html. (C) 2015 Elsevier B.V. All rights reserved. C1 [Doyle, Barney L.] Sandia Natl Labs, Radiat Solid Interact Dept 01111, POB 5800, Albuquerque, NM 87185 USA. RP Doyle, BL (reprint author), Sandia Natl Labs, Radiat Solid Interact Dept 01111, POB 5800, Albuquerque, NM 87185 USA. NR 13 TC 1 Z9 1 U1 1 U2 4 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD MAR 15 PY 2016 VL 371 BP 63 EP 68 DI 10.1016/j.nimb.2015.08.047 PG 6 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DI3PX UT WOS:000373412000012 ER PT J AU Vizkelethy, G Foiles, SM AF Vizkelethy, Gyorgy Foiles, Stephen M. TI Determination of recombination radius in Si for binary collision approximation codes SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 22nd International Conference on Ion Beam Analysis (IBA) CY JUN 14-19, 2015 CL Opatija, CROATIA SP Ruder Boskovic Inst, Int Atom Energy Agcy, Croatian Ctr Excellence Adv Mat & Sensing Dev, Croatian Minist Sci, Educ & Sports, Fdn Croatian Acad Sci & Arts, CERIC ERIC, Elsevier, FEI, High Voltage Engn Europa B V, IONTOF, Kurt J Lesker Co, Natl Electrostat Corp, Pantechnik, Pfeiffer Vacuum DE Binary Collision Approximation; Molecular Dynamics; Recombination radius; Displacement threshold energy ID COMPUTER-SIMULATION; DISPLACEMENT; SOLIDS; ENERGY; CASCADES; IONS AB Displacement damage caused by ions or neutrons in microelectronic devices can have significant effect on the performance of these devices. Therefore, it is important to predict not only the displacement damage profile, but also its magnitude precisely. Analytical methods and binary collision approximation codes working with amorphous targets use the concept of displacement energy, the energy that a lattice atom has to receive to create a permanent replacement. It was found that this "displacement energy" is direction dependent; it can range from 12 to 32 eV in silicon. Obviously, this model fails in BCA codes that work with crystalline targets, such as Marlowe. Marlowe does not use displacement energy; instead, it uses lattice binding energy only and then pairs the interstitial atoms with vacancies. Then based on the configuration of the Frenkel pairs it classifies them as close, near, or distant pairs, and considers the distant pairs the permanent replacements. Unfortunately, this separation is an ad hoc assumption, and the results do not agree with molecular dynamics calculations. After irradiation, there is a prompt recombination of interstitials and vacancies if they are nearby, within a recombination radius. In order to implement this recombination radius in Marlowe, we used the comparison of MD and Marlowe calculation in a range of ion energies in single crystal silicon target. The calculations showed that a single recombination radius of similar to 7.4 angstrom in Marlowe for a range of ion energies gives an excellent agreement with MD. (C) 2015 Elsevier B.V. All rights reserved. C1 [Vizkelethy, Gyorgy; Foiles, Stephen M.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Vizkelethy, G (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM gvizkel@sandia.gov OI Foiles, Stephen/0000-0002-1907-454X NR 18 TC 0 Z9 0 U1 3 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD MAR 15 PY 2016 VL 371 BP 111 EP 115 DI 10.1016/j.nimb.2015.08.088 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DI3PX UT WOS:000373412000021 ER PT J AU Lanford, WA Parenti, M Nordell, BJ Paquette, MM Caruso, AN Mantymaki, M Hamalainen, J Ritala, M Klepper, KB Miikkulainen, V Nilsen, O Tenhaeff, W Dudney, N Koh, D Banerjee, SK Mays, E Bielefeld, J King, SW AF Lanford, W. A. Parenti, M. Nordell, B. J. Paquette, M. M. Caruso, A. N. Mantymaki, M. Hamalainen, J. Ritala, M. Klepper, K. B. Miikkulainen, V. Nilsen, O. Tenhaeff, W. Dudney, N. Koh, D. Banerjee, S. K. Mays, E. Bielefeld, J. King, S. W. TI Nuclear reaction analysis for H, Li, Be, B, C, N, O and F with an RBS check SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS LA English DT Article; Proceedings Paper CT 22nd International Conference on Ion Beam Analysis (IBA) CY JUN 14-19, 2015 CL Opatija, CROATIA SP Ruder Boskovic Inst, Int Atom Energy Agcy, Croatian Ctr Excellence Adv Mat & Sensing Dev, Croatian Minist Sci, Educ & Sports, Fdn Croatian Acad Sci & Arts, CERIC ERIC, Elsevier, FEI, High Voltage Engn Europa B V, IONTOF, Kurt J Lesker Co, Natl Electrostat Corp, Pantechnik, Pfeiffer Vacuum DE NRA; Light elements; Electronic materials ID TRANSFORM-INFRARED-SPECTROSCOPY; CHEMICAL-VAPOR-DEPOSITION; SICH THIN-FILMS; DIELECTRIC-CONSTANT; CRYSTAL AB N-15 nuclear reaction analysis (NRA) for H is combined with 1.2 MeV deuteron (D) NRA which provides a simultaneous analysis for Li, Be, B, C, N, O and F. The energy dependence of the D NRA has been measured and used to correct for the D energy loss in film being analyzed. A 2 MeV He RBS measurement is made. Film composition is determined by a self-consistent analysis of the light element NRA data combined with an RBS analysis for heavy elements. This composition is used to simulate, with no adjustable parameters, the complete RBS spectrum. Comparison of this simulated RBS spectrum with the measured spectrum provides a powerful check of the analysis. (C) 2015 Elsevier B.V. All rights reserved. C1 [Lanford, W. A.; Parenti, M.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Nordell, B. J.; Paquette, M. M.; Caruso, A. N.] Univ Missouri, Dept Phys & Astron, Kansas City, MO 64110 USA. [Mantymaki, M.; Hamalainen, J.; Ritala, M.] Univ Helsinki, Dept Chem, Box 55, FI-00014 Helsinki, Finland. [Klepper, K. B.; Miikkulainen, V.; Nilsen, O.] Univ Oslo, Dept Chem, POB 1033, N-0315 Oslo, Norway. [Tenhaeff, W.; Dudney, N.] Oak Ridge Natl Lab, Div Solid State, POB 2008, Oak Ridge, TN 37831 USA. [Koh, D.; Banerjee, S. K.] Univ Texas Austin, Dept Elect & Comp Engn, 10100 Burnet Rd, Austin, TX 78758 USA. [Mays, E.; Bielefeld, J.; King, S. W.] Intel Corp, Log Technol Dev, Hillsboro, OR 97124 USA. RP Lanford, WA (reprint author), SUNY Albany, Dept Phys, Albany, NY 12222 USA. EM wlanford@albany.edu RI Ritala, Mikko/N-7268-2013; OI Ritala, Mikko/0000-0002-6210-2980; Miikkulainen, Ville/0000-0002-9398-2319; Mantymaki, Miia/0000-0003-0880-0427; Hamalainen, Jani/0000-0002-2903-1199 NR 34 TC 4 Z9 4 U1 2 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-583X EI 1872-9584 J9 NUCL INSTRUM METH B JI Nucl. Instrum. Methods Phys. Res. Sect. B-Beam Interact. Mater. Atoms PD MAR 15 PY 2016 VL 371 BP 211 EP 215 DI 10.1016/j.nimb.2015.10.052 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Atomic, Molecular & Chemical; Physics, Nuclear SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DI3PX UT WOS:000373412000040 ER PT J AU Stavila, V Schneider, C Mowry, C Zeitler, TR Greathouse, JA Robinson, AL Denning, JM Volponi, J Leong, K Quan, W Tu, M Fischer, RA Allendorf, MD AF Stavila, Vitalie Schneider, Christian Mowry, Curtis Zeitler, Todd R. Greathouse, Jeffery A. Robinson, Alex L. Denning, Julie M. Volponi, Joanne Leong, Kirsty Quan, William Tu, Min Fischer, Roland A. Allendorf, Mark D. TI Thin Film Growth of nbo MOFs and their Integration with Electroacoustic Devices SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article ID METAL-ORGANIC FRAMEWORKS; HIGH H-2 ADSORPTION; BY-STEP ROUTE; SITES; CONDUCTIVITY; FABRICATION; MECHANISM; KINETICS; COATINGS; HKUST-1 AB Metal-organic frameworks (MOFs) with the "nbo" topology constitute a diverse suite of more than 100 nanoporous materials, but their use in applications such as chemical sensing and membranes is inhibited by a lack of methods for growing them as thin films. Here, layer-by-layer (LBL) and solvothermal growth of "nbo" films is demonstrated and it is established for the first time that interlinker steric hindrance is a critical factor in determining the effectiveness of the LBL method. Film growth is demonstrated for three "nbo" MOFs: NOTT-100 and NOTT-101, which have the R-3m space group and are deposited by the LBL method, and PCN-14, with the R-3c space group, which is deposited by a solvothermal approach. Continuous and dense films of NOTT-100 and NOTT-101 are obtained and LBL growth is verified by observing deposition with a quartz crystal microbalance technique, which also yields the temperature dependence. Oxygen plasma treatment is found to be a useful tool for promoting the MOF film growth under solvothermal conditions. Effective mechanical coupling of these films to the substrate is demonstrated by growing them on surface acoustic wave sensors, which respond reversibly to vapors of water, acetone, and n-hexane. C1 [Stavila, Vitalie; Volponi, Joanne; Leong, Kirsty; Quan, William; Allendorf, Mark D.] Sandia Natl Labs, Livermore, CA 94551 USA. [Schneider, Christian; Tu, Min; Fischer, Roland A.] Ruhr Univ Bochum, Inorgan Chem Organometall & Mat Chem 2, D-44780 Bochum, Germany. [Mowry, Curtis; Zeitler, Todd R.; Greathouse, Jeffery A.; Robinson, Alex L.; Denning, Julie M.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Stavila, V; Allendorf, MD (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA.; Fischer, RA (reprint author), Ruhr Univ Bochum, Inorgan Chem Organometall & Mat Chem 2, D-44780 Bochum, Germany. EM vnstavi@sandia.gov; roland.fischer@ch.tum.de; mdallen@sandia.gov RI Tu, Min/F-5224-2015; Fischer, Roland/B-4042-2011 FU Sandia Laboratory Directed Research and Development Program; Cluster of Excellence RESOLV - Deutsche Forschungsgemeinschaft (DFG) [EXC 1069]; Ruhr University Research School [GSC 98]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors gratefully acknowledge financial support from Sandia Laboratory Directed Research and Development Program. R.A.F. and M.T. are supported by the Cluster of Excellence RESOLV (EXC 1069) funded by the Deutsche Forschungsgemeinschaft (DFG) and by Ruhr University Research School (GSC 98). Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 48 TC 2 Z9 2 U1 57 U2 135 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD MAR 15 PY 2016 VL 26 IS 11 BP 1699 EP 1707 DI 10.1002/adfm.201504211 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DH6PV UT WOS:000372914200002 ER PT J AU Viera, JP Payri, R Swantek, AB Duke, DJ Sovis, N Kastengren, AL Powell, CF AF Viera, Juan P. Payri, Raul Swantek, Andrew B. Duke, Daniel J. Sovis, Nicolas Kastengren, Alan L. Powell, Christopher F. TI Linking instantaneous rate of injection to X-ray needle lift measurements for a direct-acting piezoelectric injector SO ENERGY CONVERSION AND MANAGEMENT LA English DT Article DE Diesel direct injection; Rate of injection; Synchrotron; X-ray imaging; Needle lift ID SPRAY CHARACTERISTICS; NOZZLE GEOMETRY; DIESEL; COMBUSTION; ENGINE; PENETRATION; FLOW AB Internal combustion engines have been and still are key players in today's world. Ever increasing fuel consumption standards and the ongoing concerns about exhaust emissions have pushed the industry to research new concepts and develop new technologies that address these challenges. To this end, the diesel direct injection system has recently seen the introduction of direct-acting piezoelectric injectors, which provide engineers with direct control over the needle lift, and thus instantaneous rate of injection (ROI). Even though this type of injector has been studied previously, no direct link between the instantaneous needle lift and the resulting rate of injection has been quantified. This study presents an experimental analysis of the relationship between instantaneous partial needle lifts and the corresponding ROI. A prototype direct-acting injector was utilized to produce steady injections of different magnitude by partially lifting the needle. The ROI measurements were carried out at CMT-Motores Termicos utilizing a standard injection rate discharge curve indicator based on the Bosch method (anechoic tube). The needle lift measurements were performed at the Advanced Photon Source at Argonne National Laboratory. The analysis seeks both to contribute to the current understanding of the influence that partial needle lifts have over the instantaneous ROI and to provide experimental data with parametric variations useful for numerical model validations. Results show a strong relationship between the steady partial needle lift and the ROI. The effect is non-linear, and also strongly dependent on the injection pressure. The steady lift value at which the needle ceases to influence the ROI increases with the injection pressure. Finally, a transient analysis is presented, showing that the needle velocity may considerably affect the instantaneous ROI, because of the volume displaced inside the nozzle. Results presented in this study show that at constant injection pressure and energizing time, this injector has the potential to control many aspects of the ROI and thus, the heat release rate. Also, data presented are useful for numerical model validations, which would provide detailed insight into the physical processes that drive these observations, and potentially, to the effects of these features on combustion performance. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Viera, Juan P.; Payri, Raul] Univ Politecn Valencia, CMT Motores Term, Camino Vera S-N, E-46022 Valencia, Spain. [Swantek, Andrew B.; Duke, Daniel J.; Sovis, Nicolas; Powell, Christopher F.] Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. [Kastengren, Alan L.] Argonne Natl Lab, Adv Photon Source, Xray Sci Div, Argonne, IL 60439 USA. RP Viera, JP (reprint author), Univ Politecn Valencia, CMT Motores Term, Camino Vera S-N, E-46022 Valencia, Spain. EM juavieso@mot.upv.es FU U.S. Department of Energy (DOE) [DE-AC02-06CH11357]; DOE Vehicle Technologies Program; Fulbright Visiting Scholar grant; Ministry of Education, Culture and Sports of Spain [PRX14/00331]; Spanish MINECO grant [EEBB-I-15-0976, TRA2012-36932]; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX This research was performed at the 32-ID beam line of the APS at Argonne National Laboratory. Use of the APS is supported by the U.S. Department of Energy (DOE) under Contract No. DE-AC02-06CH11357. The fuel spray research is sponsored by the DOE Vehicle Technologies Program. The authors wish to thank Gurpreet Singh and Leo Broten for their support of this work. Raul Payri was funded by a Fulbright Visiting Scholar grant in collaboration with the Ministry of Education, Culture and Sports of Spain (reference PRX14/00331) while performing this work. J.P. Viera was funded by the Spanish MINECO grant EEBB-I-15-0976 under project TRA2012-36932.; The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory (Argonne). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 28 TC 2 Z9 2 U1 6 U2 7 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0196-8904 EI 1879-2227 J9 ENERG CONVERS MANAGE JI Energy Conv. Manag. PD MAR 15 PY 2016 VL 112 BP 350 EP 358 DI 10.1016/j.enconman.2016.01.038 PG 9 WC Thermodynamics; Energy & Fuels; Mechanics SC Thermodynamics; Energy & Fuels; Mechanics GA DI1GV UT WOS:000373245500032 ER PT J AU Jiang, YS DeVore, PTS Jalali, B AF Jiang, Yunshan DeVore, Peter T. S. Jalali, Bahram TI Analog optical computing primitives in silicon photonics SO OPTICS LETTERS LA English DT Article ID WAVE-GUIDES; RAMAN AMPLIFICATION; ABSORPTION; TRANSFORM AB Optical computing accelerators help alleviate bandwidth and power consumption bottlenecks in electronics. We show an approach to implementing logarithmic-type analog co-processors in silicon photonics and use it to perform the exponentiation operation and the recovery of a signal in the presence of multiplicative distortion. The function is realized by exploiting nonlinear-absorption-enhanced Raman amplification saturation in a silicon waveguide. (C) 2016 Optical Society of America C1 [Jiang, Yunshan; DeVore, Peter T. S.; Jalali, Bahram] Univ Calif Los Angeles, Dept Elect Engn, Los Angeles, CA 90095 USA. [DeVore, Peter T. S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RP Jiang, YS (reprint author), Univ Calif Los Angeles, Dept Elect Engn, Los Angeles, CA 90095 USA. EM jiangyunshan@g.ucla.edu FU Office of Naval Research (ONR) MURI Program on Optical Computing; U.S. Department of Defense (DOD) MURI Program on Near-Field Nanophotonics for Energy Efficient Computing and Communication (NECom); U.S. Department of Energy (DOE); Lawrence Livermore National Laboratory (LLNL) [DE-AC52-07NA27344] FX Office of Naval Research (ONR) MURI Program on Optical Computing; U.S. Department of Defense (DOD) MURI Program on Near-Field Nanophotonics for Energy Efficient Computing and Communication (NECom); U.S. Department of Energy (DOE); Lawrence Livermore National Laboratory (LLNL) (DE-AC52-07NA27344). NR 20 TC 2 Z9 2 U1 1 U2 8 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 0146-9592 EI 1539-4794 J9 OPT LETT JI Opt. Lett. PD MAR 15 PY 2016 VL 41 IS 6 BP 1273 EP 1276 DI 10.1364/OL.41.001273 PG 4 WC Optics SC Optics GA DH8KS UT WOS:000373042600051 PM 26977687 ER PT J AU Shaw, JB Robinson, EW Pasa-Tolic, L AF Shaw, Jared B. Robinson, Errol W. Pasa-Tolic, Ljiljana TI Vacuum Ultraviolet Photodissociation and Fourier Transform-Ion Cyclotron Resonance (FT-ICR) Mass Spectrometry: Revisited SO ANALYTICAL CHEMISTRY LA English DT Article ID ELECTRON-CAPTURE DISSOCIATION; PEPTIDE IONS; 193-NM PHOTODISSOCIATION; PROTONATED PEPTIDES; MAGNETRON MOTION; PROTEIN CATIONS; LARGE MOLECULES; 157 NM; FRAGMENTATION; PHOTOFRAGMENTATION AB We revisited the implementation of 193 nm ultraviolet photodissociation (UVPD) within the ion cyclotron resonance (ICR) cell of a Fourier transform ion cyclotron resonance (FT-ICR) mass spectrometer. UVPD performance characteristics were examined in the context of recent developments in the understanding of UVPD and in-cell tandem mass spectrometry. Efficient UVPD and photo-ECD of a model peptide and proteins within the ICR cell of a FT-ICR mass spectrometer are accomplished through appropriate modulation of laser pulse timing, relative to ion magnetron motion and the potential applied, to an ion optical element upon which photons impinge. It is shown that UVPD yields efficient and extensive fragmentation, resulting in excellent sequence coverage for model peptide and protein cations. C1 [Shaw, Jared B.; Robinson, Errol W.; Pasa-Tolic, Ljiljana] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. RP Pasa-Tolic, L (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. EM ljiljana.pasatolic@pnnl.gov FU Office of Biological and Environmental Research FX This research is part of the "High Resolution and Mass Accuracy Capability" development project at EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at the Pacific Northwest National Laboratory (PNNL) in Richland, WA. NR 36 TC 1 Z9 1 U1 4 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD MAR 15 PY 2016 VL 88 IS 6 BP 3019 EP 3023 DI 10.1021/acs.analchem.6b00148 PG 5 WC Chemistry, Analytical SC Chemistry GA DG9GT UT WOS:000372391500008 PM 26882021 ER PT J AU Hosseinzadeh, P Mirts, EN Pfister, TD Gao, YG Mayne, C Robinson, H Tajkhorshid, E Lu, Y AF Hosseinzadeh, Parisa Mirts, Evan N. Pfister, Thomas D. Gao, Yi-Gui Mayne, Christopher Robinson, Howard Tajkhorshid, Emad Lu, Yi TI Enhancing Mn(II)-Binding and Manganese Peroxidase Activity in a Designed Cytochrome c Peroxidase through Fine-Tuning Secondary-Sphere Interactions SO BIOCHEMISTRY LA English DT Article ID PHANEROCHAETE-CHRYSOSPORIUM; CRYSTAL-STRUCTURE; LIGNIN BIOSYNTHESIS; HEME PEROXIDASE; MN-PEROXIDASE; BINDING-SITE; AMINO-ACIDS; OXIDATION; SUBSTRATE; REDUCTION AB Noncovalent second-shell interactions are important in controlling metal-binding affinity and activity in metalloenzymes, but fine-tuning these interactions in designed metalloenzymes has not been fully explored. As a result, most,designed metalloenzymes have low metal-binding affinity and activity. Here we identified three mutations in the second coordination shell of an engineered Mn(II)-binding site in cytochrome c peroxidase (called MnCcP.1, containing Glu45, Glu37, and Glu181 ligands) that mimics the native manganese peroxidase (MnP), and explored their effects on both Mn(II)-binding affinity and MnP activity. First, removing a hydrogen bond to Glu45 through Tyr36Phe mutation enhanced Mn(II)-binding affinity, as evidenced by a 2.8-fold decrease in the K-M of Mn(II) oxidation. Second, introducing a salt bridge through Lys179Arg mutation improved Glu35 and Glu181 coordination to Mn(II), decreasing Km 2.6-fold. Third, eliminating a steric clash that prevented Glu37 from orienting toward Mn(II) resulted in an 8.6-fold increase in k(cat)/K-M, arising primarily from a 3.6-fold decrease in K-M, with a K-M value comparable to that of the native enzyme (0.28 mM vs 0.19 mM for Pleurotus eryngii MnP PS3). We further demonstrated that while the effects of Tyr36Phe and Lys179Arg mutations are additive, because involved in secondary-shell interactions to different ligands, other combinations of mutations were antagonistic because they act on, different aspects of the Mn(II) coordination at the same residues. Finally, we showed that these MnCcP variants are functional models of MnP that mimic its activity in both Mn(II) oxidation and degradation of a phenolic lignin model compound and kraft lignin. In addition to achieving KM in a designed protein that is similar to the that of native enzyme, our results offer molecular insight into the role of noncovalent interactions around metal-binding sites for improving metal binding and overall activity; such insight can be applied to rationally enhance these properties in other metalloenzyrnes and their models. C1 [Hosseinzadeh, Parisa; Pfister, Thomas D.; Tajkhorshid, Emad; Lu, Yi] Univ Illinois, Dept Biochem, Urbana, IL 61801 USA. [Gao, Yi-Gui; Lu, Yi] Univ Illinois, Dept Chem, Urbana, IL 61801 USA. [Mirts, Evan N.; Tajkhorshid, Emad; Lu, Yi] Univ Illinois, Ctr Biophys & Quantitat Biol, Urbana, IL 61801 USA. [Mayne, Christopher; Tajkhorshid, Emad] Univ Illinois, Beckman Inst Adv Sci & Technol, Urbana, IL 61801 USA. [Robinson, Howard] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. [Pfister, Thomas D.] Leidos Biomed Res Inc, Frederick Natl Lab Canc Res, Lab Human Toxicol & Pharmacol, Appl Dev Directorate, Frederick, MD 21702 USA. RP Lu, Y (reprint author), Univ Illinois, Dept Biochem, Urbana, IL 61801 USA.; Lu, Y (reprint author), Univ Illinois, Dept Chem, Urbana, IL 61801 USA.; Lu, Y (reprint author), Univ Illinois, Ctr Biophys & Quantitat Biol, Urbana, IL 61801 USA. EM yi-lu@illinois.edu RI Lu, Yi/B-5461-2010 OI Lu, Yi/0000-0003-1221-6709 FU National Institutes of Health [R01GM062211, P41-GM104601] FX This material is based on work supported by the National Institutes of Health via Grant R01GM062211 (to Y.L.) and Grant P41-GM104601 (E.T. and C.M.). NR 70 TC 3 Z9 3 U1 7 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0006-2960 J9 BIOCHEMISTRY-US JI Biochemistry PD MAR 15 PY 2016 VL 55 IS 10 BP 1494 EP 1502 DI 10.1021/acs.biochem.5b01299 PG 9 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DG9GY UT WOS:000372392000008 PM 26885726 ER PT J AU Zachara, J Brantley, S Chorover, J Ewing, R Kerisit, S Liu, CX Perfect, E Rother, G Stack, AG AF Zachara, John Brantley, Sue Chorover, Jon Ewing, Robert Kerisit, Sebastien Liu, Chongxuan Perfect, Edmund Rother, Gernot Stack, Andrew G. TI Internal Domains of Natural Porous Media Revealed: Critical Locations for Transport, Storage, and Chemical Reaction SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Review ID X-RAY MICROTOMOGRAPHY; MOLECULAR-DYNAMICS SIMULATIONS; ANGLE NEUTRON-SCATTERING; NANOSIZED MINERAL FRACTURES; INTERFACIAL WATER-STRUCTURE; ATOM-PROBE TOMOGRAPHY; LOW PORE CONNECTIVITY; SOIL ORGANIC-MATTER; DUAL-POROSITY MODEL; LONG-TERM SORPTION AB Internal pore domains exist within rocks, lithic fragments, subsurface sediments, and soil aggregates. These domains, termed internal domains in porous media (IDPM), represent a subset of a material's porosity; contain a significant fraction of their porosity as nanopores, dominate the reactive surface area of diverse media types; and are important locations for chemical reactivity and fluid storage. IDPM are key features controlling hydrocarbon release from shales in hydraulic fracture systems, organic matter decomposition in soil, weathering and soil formation, and contaminant behavior in the vadose zone and groundwater. Traditionally difficult to interrogate, advances in instrumentation and imaging methods are providing new insights on the physical structures and chemical attributes of IDPM, and their contributions to system behaviors. Here we discuss analytical methods to characterize IDPM, evaluate information on their size distributions, connectivity, and extended structures; determine whether they exhibit unique chemical reactivity; and assess the potential for their inclusion in reactive transport models. Ongoing developments in measurement technologies and sensitivity, and computer assisted interpretation will improve understanding of these critical features in the future. Impactful research opportunities exist to advance understanding of IDPM, and to incorporate their effects in reactive transport models for improved environmental simulation and prediction. C1 [Zachara, John; Kerisit, Sebastien; Liu, Chongxuan] Pacific NW Natl Lab, Richland, WA 99352 USA. [Brantley, Sue] Penn State Univ, University Pk, PA 16802 USA. [Chorover, Jon] Univ Arizona, Tucson, AZ 85721 USA. [Ewing, Robert] Iowa State Univ, Ames, IA 50011 USA. [Perfect, Edmund] Univ Tennessee, Knoxville, TN 37996 USA. [Rother, Gernot; Stack, Andrew G.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Zachara, J (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM john.zachara@pnnl.gov RI Rother, Gernot/B-7281-2008; Liu, Chongxuan/C-5580-2009 OI Rother, Gernot/0000-0003-4921-6294; FU DOE BER/SBR [54737]; DOE BES Geosciences [56674, ERKCC72]; DOE BES [DE-FG02-OSER15675]; Laboratory Directed Research and Development Program, ORNL FX This manuscript resulted from a U.S. Department of Energy (DOE), Basic Energy Science (BES) Geosciences Council Workshop on "Internal Domains in Porous Media" held in December 2012. The following sources/contracts provided funding to the authors: J.Z., DOE BER/SBR (54737) and DOE BES Geosciences (56674); S.B., DOE BES (DE-FG02-OSER15675); J.C., DOE BER/SBR (DE-SC0006781); RE., DOE BER/SBR (54737); S.K., DOE BES Geosciences (56674); C.L., DOE BER/SBR (54737); E.P., Laboratory Directed Research and Development Program, ORNL; GR; and A.S., DOE BES Geosciences (ERKCC72). BER/SBR is Biological and Environmental Research, Subsurface Biogeochemical Research Program. David Cole, Ohio State University, provided an initial concept for the abstract graphic. The helpful comments of three anonymous reviewers are acknowledged. NR 320 TC 4 Z9 4 U1 24 U2 97 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAR 15 PY 2016 VL 50 IS 6 BP 2811 EP 2829 DI 10.1021/acs.est.5b05015 PG 19 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DG9GZ UT WOS:000372392100009 PM 26849204 ER PT J AU Mehta, VS Maillot, F Wang, ZM Catalano, JG Giammar, DE AF Mehta, Vrajesh S. Maillot, Fabien Wang, Zheming Catalano, Jeffrey G. Giammar, Daniel E. TI Effect of Reaction Pathway on the Extent and Mechanism of Uranium(VI) Immobilization with Calcium and Phosphate SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; OCTACALCIUM PHOSPHATE; AUTUNITE; IFEFFIT; XAFS; HYDROXYAPATITE; REMEDIATION; GROUNDWATER; SEDIMENTS; APATITE AB Phosphate addition to subsurface environments contaminated with uranium can be used as an in situ remediation approach. Batch experiments were conducted to evaluate the dependence of the extent and mechanism of uranium uptake on the pathway for reaction with calcium phosphates. At pH 4.0 and 6.0 uranium uptake from solution occurred via autunite (Ca(UO2)(2)(PO4)(2)) precipitation irrespective of the starting forms of calcium and phosphate. At pH 7.5, a condition at which calcium phosphate solids could form, the uptake mechanism depended on the nature of the calcium and phosphate as determined by X-ray absorption spectroscopy and laser-induced fluorescence spectroscopy. When dissolved uranium, calcium, and phosphate were added simultaneously, uranium was structurally incorporated into a newly formed amorphous calcium phosphate solid. Adsorption was the dominant removal mechanism for uranium contacted with preformed amorphous calcium phosphate solids. When U(VI) was added to a suspension containing amorphous calcium phosphate solids as well as dissolved calcium and phosphate, then removal occurred through precipitation (57 +/- 4%) of autunite and adsorption (43 +/- 4%) onto calcium phosphate. Dissolved uranium, calcium, and phosphate concentrations with saturation index calculations helped identify removal mechanisms and determine thermodynamically favorable solid phases. C1 [Mehta, Vrajesh S.; Giammar, Daniel E.] Washington Univ, Dept Energy Environm & Chem Engn, St Louis, MO 63130 USA. [Maillot, Fabien; Catalano, Jeffrey G.] Washington Univ, Dept Earth & Planetary Sci, St Louis, MO 63130 USA. [Wang, Zheming] Pacific NW Natl Lab, Dept Fundamental & Computat Sci Directorate, Richland, WA 99352 USA. RP Giammar, DE (reprint author), Washington Univ, Dept Energy Environm & Chem Engn, St Louis, MO 63130 USA. EM giammar@wustl.edu RI Catalano, Jeffrey/A-8322-2013; Wang, Zheming/E-8244-2010 OI Catalano, Jeffrey/0000-0001-9311-977X; Wang, Zheming/0000-0002-1986-4357 FU U.S. Department of Energy (DOE) Subsurface Biogeochemical Research program [DE-SC0006857]; National Science Foundation [ECS-0335765]; DOE Office of Biological and Environmental Research; DOE by Battelle Memorial Institute [DE-AC06-76RLO-1830]; DOE Office of Basic Energy Sciences; Canadian Light Source; University of Washington; APS; U.S. DOE [DE-AC02-06CH11357] FX We are grateful to the McDonnell International Scholars Academy at Washington University for providing the Ameren corporate fellowship for Vrajesh Mehta. This work was supported by the U.S. Department of Energy (DOE) Subsurface Biogeochemical Research program (Award No. DE-SC0006857). Lyndsay Troyer assisted in the fitting of EXAFS data and the preparation of associated figures. ICP-MS analysis was performed in the Nano Research Facility (NRF), a member of the National Nanotechnology Infrastructure Network (NNIN), which was supported by the National Science Foundation under Grant No. ECS-0335765. LIPS measurements were performed at the Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by the DOE Office of Biological and Environmental Research and located at the Pacific Northwest National Laboratory (PNNL). PNNL is operated for DOE by Battelle Memorial Institute under Contract # DE-AC06-76RLO-1830. EXAFS measurements were performed at Sector 20 of the Advanced Photon Source (APS), which is supported by DOE Office of Basic Energy Sciences, the Canadian Light Source and its funding partners, the University of Washington, and the APS. Use of the APS, a user facility operated for the DOE Office of Science by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. We are grateful to Dr. Timothy Strathmann and three anonymous reviewers whose comments helped us improve the presentation of this study. NR 44 TC 5 Z9 5 U1 14 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAR 15 PY 2016 VL 50 IS 6 BP 3128 EP 3136 DI 10.1021/acs.est.5b06212 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DG9GZ UT WOS:000372392100042 PM 26934085 ER PT J AU Horner, RM Harto, CB Jackson, RB Lowry, ER Brandt, AR Yeskoo, TW Murphy, DJ Clark, CE AF Horner, R. M. Harto, C. B. Jackson, R. B. Lowry, E. R. Brandt, A. R. Yeskoo, T. W. Murphy, D. J. Clark, C. E. TI Water Use and Management in the Bakken Shale Oil Play in North Dakota SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID UNITED-STATES; GAS AB Oil and natural gas development in the Bakken shale play of North Dakota has grown substantially since 2008. This study provides a comprehensive overview and analysis of water quantity and management impacts from this development by (1) estimating water demand for hydraulic fracturing in the Bakken from 2008 to 2012; (2) compiling volume estimates for maintenance water, or brine dilution water; (3) calculating water intensities normalized by the amount of oil produced, or estimated ultimate recovery (EUR); (4) estimating domestic water demand associated with the large oil services population; (5) analyzing the change in wastewater volumes from 2005 to 2012; and (6) examining existing water sources used to meet demand. Water use for hydraulic fracturing in the North Dakota Bakken grew 5-fold from 770 million gallons in 2008 to 4.3 billion gallons in 2012. First-year wastewater volumes grew in parallel, from an annual average of 1 135 000 gallons per well in 2008 to 2 905 000 gallons in 2012, exceeding the mean volume of water used in hydraulic fracturing and surpassing typical 4-year wastewater totals for the Barnett, Denver, and Marcellus basins. Surprisingly, domestic water demand from the temporary oilfield services population in the region may be comparable to the regional water demand from hydraulic fracturing activities. Existing groundwater resources are inadequate to meet the demand for hydraulic fracturing, but there appear to be adequate surface water resources, provided that access is available. C1 [Horner, R. M.] US DOE, 1000 Independence Ave SW, Washington, DC 20585 USA. [Harto, C. B.; Clark, C. E.] Argonne Natl Lab, Div Environm Sci, 955 Enfant Plaza SW,Suite 6000, Washington, DC 20024 USA. [Jackson, R. B.] Stanford Univ, Woods Inst Environm, Sch Earth Energy & Environm Sci, Stanford, CA 94305 USA. [Jackson, R. B.; Brandt, A. R.] Stanford Univ, Precourt Inst Energy, Stanford, CA 94305 USA. [Lowry, E. R.; Brandt, A. R.] Stanford Univ, Sch Earth Energy & Environm Sci, Stanford, CA 94305 USA. [Murphy, D. J.] St Lawrence Univ, 23 Romoda Dr, Canton, NY 13617 USA. RP Horner, RM (reprint author), US DOE, 1000 Independence Ave SW, Washington, DC 20585 USA. EM robert.horner@hq.doe.gov FU U.S. Department Energy [DE-AC02-06CH11357]; Natural Resources Defense Council; Stanford's Natural Gas Initiative; Stanford University FX Argonne National Laboratory's work was funded by U.S. Department Energy under contract DE-AC02-06CH11357. We also acknowledge the Natural Resources Defense Council, Stanford University, and Stanford's Natural Gas Initiative for support. Scott Schlueter, Argonne GIS analyst, generated the figures in the report and in the Supporting Information. NR 42 TC 2 Z9 2 U1 9 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD MAR 15 PY 2016 VL 50 IS 6 BP 3275 EP 3282 DI 10.1021/acs.est.5b04079 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DG9GZ UT WOS:000372392100058 PM 26866674 ER PT J AU Uphoff, H AF Uphoff, Heidi TI Until We Are Free: My Fight for Human Rights in Iran SO LIBRARY JOURNAL LA English DT Book Review C1 [Uphoff, Heidi] Sandia Natl Labs, Livermore, CA 94550 USA. RP Uphoff, H (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. NR 1 TC 0 Z9 0 U1 0 U2 0 PU REED BUSINESS INFORMATION PI NEW YORK PA 360 PARK AVENUE SOUTH, NEW YORK, NY 10010 USA SN 0363-0277 J9 LIBR J JI Libr. J. PD MAR 15 PY 2016 VL 141 IS 5 BP 122 EP 122 PG 1 WC Information Science & Library Science SC Information Science & Library Science GA DH1RV UT WOS:000372563500172 ER PT J AU Gubler, P Hattori, K Lee, SH Oka, M Ozaki, S Suzuki, K AF Gubler, Philipp Hattori, Koichi Lee, Su Houng Oka, Makoto Ozaki, Sho Suzuki, Kei TI D mesons in a magnetic field SO PHYSICAL REVIEW D LA English DT Article ID QCD SUM-RULES; HEAVY-ION COLLISIONS; SOFT GAMMA-REPEATERS; NEUTRON-STARS; QUANTUM CHROMODYNAMICS; VACUUM POLARIZATION; FINITE-TEMPERATURE; RESONANCE PHYSICS; ELECTRIC-FIELDS; NUCLEAR-MATTER AB We investigate the mass spectra of open heavy flavor mesons in an external constant magnetic field within QCD sum rules. Spectral Ansatze on the phenomenological side are proposed in order to properly take into account mixing effects between the pseudoscalar and vector channels, and the Landau levels of charged mesons. The operator product expansion is implemented up to dimension-5 operators. As a result, we find for neutral D mesons a significant positive mass shift that goes beyond simple mixing effects. In contrast, charged D mesons are further subject to Landau level effects, which together with the mixing effects almost completely saturate the mass shifts obtained in our sum rule analysis. C1 [Gubler, Philipp] ECT, Villa Tambosi, I-38123 Villazzano, Trento, Italy. [Hattori, Koichi] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Bldg 510A, Upton, NY 11973 USA. [Hattori, Koichi; Suzuki, Kei] RIKEN, Nishina Ctr, Theoret Res Div, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. [Lee, Su Houng] Yonsei Univ, Dept Phys, Seoul 120749, South Korea. [Lee, Su Houng] Yonsei Univ, Inst Phys & Appl Phys, Seoul 120749, South Korea. [Oka, Makoto] Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan. [Oka, Makoto] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan. [Ozaki, Sho] High Energy Accelerator Res Org KEK, IPNS, Theory Ctr, 1-1 Oho, Tsukuba, Ibaraki 3050801, Japan. RP Gubler, P (reprint author), ECT, Villa Tambosi, I-38123 Villazzano, Trento, Italy.; Hattori, K (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Bldg 510A, Upton, NY 11973 USA.; Hattori, K; Suzuki, K (reprint author), RIKEN, Nishina Ctr, Theoret Res Div, 2-1 Hirosawa, Wako, Saitama 3510198, Japan.; Lee, SH (reprint author), Yonsei Univ, Dept Phys, Seoul 120749, South Korea.; Lee, SH (reprint author), Yonsei Univ, Inst Phys & Appl Phys, Seoul 120749, South Korea.; Oka, M (reprint author), Tokyo Inst Technol, Dept Phys, Meguro Ku, Tokyo 1528551, Japan.; Oka, M (reprint author), Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan.; Ozaki, S (reprint author), High Energy Accelerator Res Org KEK, IPNS, Theory Ctr, 1-1 Oho, Tsukuba, Ibaraki 3050801, Japan. EM pgubler@riken.jp; koichi.hattori@riken.jp; suhoung@yonsei.ac.kr; oka@th.phys.titech.ac.jp; sho@post.kek.jp; kei.suzuki@riken.jp FU Korean Research Foundation [KRF-2011-0020333, KRF-2011-0030621]; JSPS [25287066]; RIKEN Foreign Postdoctoral Researcher Program, the RIKEN iTHES Project; KAKENHI [25247036]; Japan Society for the Promotion of Science (JSPS) [26-8288] FX The authors thank Sungtae Cho and Kenji Morita for useful discussions. K. H. thanks Jorge Noronha for a discussion. This work was supported by the Korean Research Foundation under Grants No. KRF-2011-0020333 and No. KRF-2011-0030621. The research of K. H. is supported by JSPS Grant-in-Aid No. 25287066. At an early stage of this work, P. G. was supported by the RIKEN Foreign Postdoctoral Researcher Program, the RIKEN iTHES Project. Four of the authors (P. G., K. H., S. O. and K. S.) thank the Yukawa Institute for Theoretical Physics, Kyoto University, where some parts of this work were discussed during the YIPQS international workshops "New Frontiers in QCD 2013" and "Hadrons and Hadron Interactions in QCD 2015." K. H. is grateful to the hospitality of ECT*, where this work was finalized during the ECT* workshop "New Perspectives on Photons and Dileptons in Ultrarelativistic Heavy-Ion Collisions at RHIC and LHC." This work was partially supported by KAKENHI under Contract No. 25247036. K. S. was supported by Grant-in-Aid for JSPS Fellows from Japan Society for the Promotion of Science (JSPS) (No. 26-8288). NR 96 TC 5 Z9 5 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 15 PY 2016 VL 93 IS 5 AR 054026 DI 10.1103/PhysRevD.93.054026 PG 21 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG9PV UT WOS:000372417200001 ER PT J AU Bilgin, CC Fontenay, G Cheng, QS Chang, H Han, J Parvin, B AF Bilgin, Cemal Cagatay Fontenay, Gerald Cheng, Qingsu Chang, Hang Han, Ju Parvin, Bahram TI BioSig3D: High Content Screening of Three-Dimensional Cell Culture Models SO PLOS ONE LA English DT Article ID FLUORESCENCE MICROSCOPY; GENE-EXPRESSION; VISUALIZATION; ELEGANS; SYSTEM; ASSAYS AB BioSig3D is a computational platform for high-content screening of three-dimensional (3D) cell culture models that are imaged in full 3D volume. It provides an end-to-end solution for designing high content screening assays, based on colony organization that is derived from segmentation of nuclei in each colony. BioSig3D also enables visualization of raw and processed 3D volumetric data for quality control, and integrates advanced bioinformatics analysis. The system consists of multiple computational and annotation modules that are coupled together with a strong use of controlled vocabularies to reduce ambiguities between different users. It is a web-based system that allows users to: design an experiment by defining experimental variables, upload a large set of volumetric images into the system, analyze and visualize the dataset, and either display computed indices as a heatmap, or phenotypic subtypes for heterogeneity analysis, or download computed indices for statistical analysis or integrative biology. BioSig3D has been used to profile baseline colony formations with two experiments: (i) morphogenesis of a panel of human mammary epithelial cell lines (HMEC), and (ii) heterogeneity in colony formation using an immortalized non-transformed cell line. These experiments reveal intrinsic growth properties of well-characterized cell lines that are routinely used for biological studies. BioSig3D is being released with seed datasets and video-based documentation. C1 [Cheng, Qingsu; Chang, Hang; Han, Ju; Parvin, Bahram] Univ Nevada, Dept Elect & Biomed Engn, Reno, NV 89557 USA. [Bilgin, Cemal Cagatay; Fontenay, Gerald; Cheng, Qingsu; Chang, Hang; Han, Ju; Parvin, Bahram] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Parvin, B (reprint author), Univ Nevada, Dept Elect & Biomed Engn, Reno, NV 89557 USA.; Parvin, B (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. EM bparvin@unr.edu FU National Cancer Institute [RO1CA140663]; Parvin's startup funds at UNR FX This work was supported by a grant from the National Cancer Institute (Grant RO1CA140663) and Parvin's startup funds at UNR. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 33 TC 2 Z9 2 U1 2 U2 12 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 15 PY 2016 VL 11 IS 3 AR e0148379 DI 10.1371/journal.pone.0148379 PG 19 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH1VK UT WOS:000372572800011 PM 26978075 ER PT J AU Morgan, TJ Turn, SQ Sun, N George, A AF Morgan, Trevor James Turn, Scott Q. Sun, Ning George, Anthe TI Fast Pyrolysis of Tropical Biomass Species and Influence of Water Pretreatment on Product Distributions SO PLOS ONE LA English DT Article ID FLUIDIZED-BED PYROLYSIS; BIO-OIL; FLASH PYROLYSIS; ELEPHANT GRASS; SECONDARY REACTIONS; EUCALYPTUS-GRANDIS; REACTOR; LIGNIN; CONVERSION; BANAGRASS AB The fast pyrolysis behaviour of pretreated banagrass was examined at four temperatures (between 400 and 600 C) and four residence times (between similar to 1.2 and 12 s). The pretreatment used water washing/leaching to reduce the inorganic content of the banagrass. Yields of bio-oil, permanent gases and char were determined at each reaction condition and compared to previously published results from untreated banagrass. Comparing the bio-oil yields from the untreated and pretreated banagrass shows that the yields were greater from the pretreated banagrass by 4 to 11 wt%(absolute) at all reaction conditions. The effect of pretreatment (i.e. reducing the amount of ash, and alkali and alkali earth metals) on pyrolysis products is: 1) to increase the dry bio-oil yield, 2) to decrease the amount of undetected material, 3) to produce a slight increase in CO yield or no change, 4) to slightly decrease CO2 yield or no change, and 5) to produce a more stable bio-oil (less aging). Char yield and total gas yield were unaffected by feedstock pretreatment. Four other tropical biomass species were also pyrolyzed under one condition (450 degrees C and 1.4 s residence time) for comparison to the banagrass results. The samples include two hardwoods: leucaena and eucalyptus, and two grasses: sugarcane bagasse and energy-cane. A sample of pretreated energy-cane was also pyrolyzed. Of the materials tested, the best feedstocks for fast pyrolysis were sugarcane bagasse, pretreated energy cane and eucalyptus based on the yields of 'dry bio-oil', CO and CO2. On the same basis, the least productive feedstocks are untreated banagrass followed by pretreated banagrass and leucaena. C1 [Morgan, Trevor James; Turn, Scott Q.] Univ Hawaii Manoa, Hawaii Nat Energy Inst, Honolulu, HI 96822 USA. [Sun, Ning] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [George, Anthe] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. RP Morgan, TJ (reprint author), Univ Hawaii Manoa, Hawaii Nat Energy Inst, Honolulu, HI 96822 USA. EM morgatr@gmail.com FU U.S. Department of Energy [DE-EE0003507] FX This work was conducted under the Hawai'i Energy Sustainability Program with funding from the U.S. Department of Energy (Cooperative Agreement #DE-EE0003507). The funding was provided to the Hawaii Natural Energy Institute. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 41 TC 1 Z9 1 U1 8 U2 23 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 15 PY 2016 VL 11 IS 3 AR e0151368 DI 10.1371/journal.pone.0151368 PG 27 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH1VK UT WOS:000372572800068 PM 26978265 ER PT J AU Bouskill, NJ Wood, TE Baran, R Hao, Z Ye, Z Bowen, BP Lim, HC Nico, PS Holman, HY Gilbert, B Silver, WL Northen, TR Brodie, EL AF Bouskill, Nicholas J. Wood, Tana E. Baran, Richard Hao, Zhao Ye, Zaw Bowen, Ben P. Lim, Hsiao Chien Nico, Peter S. Holman, Hoi-Ying Gilbert, Benjamin Silver, Whendee L. Northen, Trent R. Brodie, Eoin L. TI Belowground Response to Drought in a Tropical Forest Soil. II. Change in Microbial Function Impacts Carbon Composition SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE tropical forest; drought; microbial functions; carbon dioxide; soil carbon ID DISSOLVED ORGANIC-MATTER; RAIN-FOREST; BACTERIAL COMMUNITIES; ANTIBIOTIC PRODUCTION; FTIR SPECTROSCOPY; IRON REDUCTION; DIOXIDE LOSSES; CLIMATE; MODELS; MICROORGANISMS AB Climate model projections for tropical regions show clear perturbation of precipitation patterns leading to increased frequency and severity of drought in some regions. Previous work has shown declining soil moisture to be a strong driver of changes in microbial trait distribution, however, the feedback of any shift in functional potential on ecosystem properties related to carbon cycling are poorly understood. Here we show that drought-induced changes in microbial functional diversity and activity shape, and are in turn shaped by, the composition of dissolved and soil-associated carbon. We also demonstrate that a shift in microbial functional traits that favor the production of hygroscopic compounds alter the efflux of carbon dioxide following soil rewetting. Under drought the composition of the dissolved organic carbon pool changed in a manner consistent with a microbial metabolic response. We hypothesize that this microbial ecophysiological response to changing soil moisture elevates the intracellular carbon demand stimulating extracellular enzyme production, that prompts the observed decline in more complex carbon compounds (e.g., cellulose and lignin). Furthermore, a metabolic response to drought appeared to condition (biologically and physically) the soil, notably through the production of polysaccharides, particularly in experimental plots that had been pre-exposed to a short-term drought. This hysteretic response, in addition to an observed drought-related decline in phosphorus concentration, may have been responsible for a comparatively modest CO2 efflux following wet-up in drought plots relative to control plots. C1 [Bouskill, Nicholas J.; Hao, Zhao; Ye, Zaw; Lim, Hsiao Chien; Nico, Peter S.; Holman, Hoi-Ying; Gilbert, Benjamin; Brodie, Eoin L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Climate & Ecosyst Sci, Earth & Environm Sci, Berkeley, CA 94720 USA. [Wood, Tana E.] US Forest Serv, Int Inst Trop Forestry, USDA, Rio Piedras, PR USA. [Wood, Tana E.] Fdn Puertorriquena Conservac, San Juan, PR USA. [Baran, Richard; Bowen, Ben P.; Northen, Trent R.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Genom & Syst Biol, Div Life Sci, Berkeley, CA 94720 USA. [Silver, Whendee L.; Brodie, Eoin L.] Univ Calif Berkeley, Dept Environm Sci Policy & Management, Berkeley, CA 94720 USA. RP Bouskill, NJ; Brodie, EL (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Climate & Ecosyst Sci, Earth & Environm Sci, Berkeley, CA 94720 USA. EM njbouskill@lbl.gov; elbrodie@lbl.gov RI Bouskill, Nick/G-2390-2015; Brodie, Eoin/A-7853-2008; Nico, Peter/F-6997-2010; Holman, Hoi-Ying/N-8451-2014; Hao, Zhao/G-2391-2015; Gilbert, Benjamin/E-3182-2010; OI Brodie, Eoin/0000-0002-8453-8435; Nico, Peter/0000-0002-4180-9397; Holman, Hoi-Ying/0000-0002-7534-2625; Hao, Zhao/0000-0003-0677-8529; Northen, Trent/0000-0001-8404-3259 FU Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory; U.S. Department of Energy, Office of Science, Office of Biological & Environmental Research [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; NSF grant [EAR-08199072]; Luquillo Critical Zone Observatory [EAR-0722476]; USGS Luquillo WEBB program; NSF [DEB 0620910] FX This work was partially supported by the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory. The Subsurface Biogeochemical Research program, the Next Generation Ecosystem Experiment (NGEE-Tropics), and ENIGMA- Ecosystems and Networks Integrated with Genes and Molecular Assemblies (http://enigma.lbl.gov). All Scientific Focus Area Programs at Lawrence Berkeley National Laboratory supported by the U.S. Department of Energy, Office of Science, Office of Biological & Environmental Research under contract number DE-AC02-05CH11231. This work was also partially funded by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research under contract number DE-AC02-05CH11231, and by NSF grant EAR-08199072 to WLS, the Luquillo Critical Zone Observatory (EAR-0722476) with additional support provided by the USGS Luquillo WEBB program, and grant DEB 0620910 from NSF to the Institute of Tropical Forest Ecosystem Studies, University of Puerto Rico, and to the International Institute of Tropical Forestry USDA Forest Service, as part of the Luquillo Long-Term Ecological Research Program. NR 114 TC 0 Z9 0 U1 18 U2 51 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD MAR 15 PY 2016 VL 7 AR 323 DI 10.3389/fmicb.2016.00323 PG 14 WC Microbiology SC Microbiology GA DG5KS UT WOS:000372117500003 PM 27014243 ER PT J AU Caspers, C Gloskovskii, A Gorgoi, M Besson, C Luysberg, M Rushchanskii, KZ Lezaic, M Fadley, CS Drube, W Muller, M AF Caspers, C. Gloskovskii, A. Gorgoi, M. Besson, C. Luysberg, M. Rushchanskii, K. Z. Lezaic, M. Fadley, C. S. Drube, W. Mueller, M. TI Interface Engineering to Create a Strong Spin Filter Contact to Silicon SO SCIENTIFIC REPORTS LA English DT Article ID FERROMAGNETIC SEMICONDUCTOR EUO; RAY PHOTOELECTRON-SPECTROSCOPY; EPITAXIAL INTEGRATION; GROWTH; TEMPERATURE; PROGRESS; SURFACE; OXIDES AB Integrating epitaxial and ferromagnetic Europium Oxide (EuO) directly on silicon is a perfect route to enrich silicon nanotechnology with spin filter functionality. To date, the inherent chemical reactivity between EuO and Si has prevented a heteroepitaxial integration without significant contaminations of the interface with Eu silicides and Si oxides. We present a solution to this long-standing problem by applying two complementary passivation techniques for the reactive EuO/Si interface: (i) an in situ hydrogen-Si (001) passivation and (ii) the application of oxygen-protective Eu monolayers-without using any additional buffer layers. By careful chemical depth profiling of the oxide-semiconductor interface via hard x-ray photoemission spectroscopy, we show how to systematically minimize both Eu silicide and Si oxide formation to the sub-monolayer regime-and how to ultimately interface-engineer chemically clean, heteroepitaxial and ferromagnetic EuO/Si (001) in order to create a strong spin filter contact to silicon. C1 [Caspers, C.; Besson, C.; Mueller, M.] Forschungszentrum Julich, PGI 6, D-52425 Julich, Germany. [Caspers, C.; Rushchanskii, K. Z.; Lezaic, M.; Mueller, M.] Forschungszentrum Julich, JARA, D-52425 Julich, Germany. [Gloskovskii, A.; Drube, W.] DESY Photon Sci, Deutsch Elektronen Synchrotron, D-22603 Hamburg, Germany. [Gorgoi, M.] BESSY II, Helmholtz Zentrum Mat & Energie, Berlin, Germany. [Luysberg, M.] Forschungszentrum Julich, PGI 5, D-52425 Julich, Germany. [Luysberg, M.] Forschungszentrum Julich, Ernst Ruska Ctr Mikroskopie & Spekt Elektronen, D-52425 Julich, Germany. [Rushchanskii, K. Z.; Lezaic, M.] Forschungszentrum Julich, PGI 1, D-52425 Julich, Germany. [Fadley, C. S.] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. [Fadley, C. S.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Mueller, M.] Univ Duisburg Essen, Fak Phys, D-47048 Duisburg, Germany. [Mueller, M.] Univ Duisburg Essen, Ctr Nanointegrat CENIDE, D-47048 Duisburg, Germany. RP Caspers, C; Muller, M (reprint author), Forschungszentrum Julich, PGI 6, D-52425 Julich, Germany.; Caspers, C; Muller, M (reprint author), Forschungszentrum Julich, JARA, D-52425 Julich, Germany.; Muller, M (reprint author), Univ Duisburg Essen, Fak Phys, D-47048 Duisburg, Germany.; Muller, M (reprint author), Univ Duisburg Essen, Ctr Nanointegrat CENIDE, D-47048 Duisburg, Germany. EM christian.caspers@gmx.de; mart.mueller@fz-juelich.de RI Hloskovsky, Andrei/A-3009-2012; Muller, Martina/O-2473-2015; Luysberg, Martina/B-6448-2014 OI Besson, Claire/0000-0002-0502-3610; Rushchanskii, Konstantin/0000-0003-3070-5725; Muller, Martina/0000-0001-6082-9038; Luysberg, Martina/0000-0002-5613-7570 FU Federal Ministry of Education and Research (BMBF) [05KS7UM1, 05K10UMA, 05KS7WW3, 05K10WW1]; Helmholtz Gemeinschaft [VH-NG-409]; Julich Supercomputing Centre [Jiff38]; DFG [MU3160/1-1]; HGF [VH-NG-811] FX We acknowledge experimental support by S. Doring and S. D. Flade. Funding by the Federal Ministry of Education and Research (BMBF) under contracts 05KS7UM1, 05K10UMA, 05KS7WW3, and 05K10WW1 is gratefully acknowledged. ML and KZR acknowledge the funding of the Helmholtz Gemeinschaft, grant VH-NG-409 and the support of the Julich Supercomputing Centre, grant Jiff38. M.L. K.Z.R. and M.M. acknowledges financial support by DFG under grant MU3160/1-1 and by HGF under No. VH-NG-811. NR 37 TC 2 Z9 2 U1 3 U2 20 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 15 PY 2016 VL 6 AR 22912 DI 10.1038/srep22912 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG4UA UT WOS:000372067100001 PM 26975515 ER PT J AU Chen, CL Mahjoubfar, A Tai, LC Blaby, IK Huang, A Niazi, KR Jalali, B AF Chen, Claire Lifan Mahjoubfar, Ata Tai, Li-Chia Blaby, Ian K. Huang, Allen Niazi, Kayvan Reza Jalali, Bahram TI Deep Learning in Label-free Cell Classification SO SCIENTIFIC REPORTS LA English DT Article ID CIRCULATING TUMOR-CELLS; IMAGE-ANALYSIS; GENE-EXPRESSION; FLOW-CYTOMETRY; PROTEIN-LEVELS; ROC CURVE; CHLAMYDOMONAS; VARIABILITY; SYSTEMS; TRANSFORMATION AB Label-free cell analysis is essential to personalized genomics, cancer diagnostics, and drug development as it avoids adverse effects of staining reagents on cellular viability and cell signaling. However, currently available label-free cell assays mostly rely only on a single feature and lack sufficient differentiation. Also, the sample size analyzed by these assays is limited due to their low throughput. Here, we integrate feature extraction and deep learning with high-throughput quantitative imaging enabled by photonic time stretch, achieving record high accuracy in label-free cell classification. Our system captures quantitative optical phase and intensity images and extracts multiple biophysical features of individual cells. These biophysical measurements form a hyperdimensional feature space in which supervised learning is performed for cell classification. We compare various learning algorithms including artificial neural network, support vector machine, logistic regression, and a novel deep learning pipeline, which adopts global optimization of receiver operating characteristics. As a validation of the enhanced sensitivity and specificity of our system, we show classification of white blood T-cells against colon cancer cells, as well as lipid accumulating algal strains for biofuel production. This system opens up a new path to data-driven phenotypic diagnosis and better understanding of the heterogeneous gene expressions in cells. C1 [Chen, Claire Lifan; Mahjoubfar, Ata; Huang, Allen; Jalali, Bahram] Univ Calif Los Angeles, Dept Elect Engn, Los Angeles, CA 90095 USA. [Chen, Claire Lifan; Mahjoubfar, Ata; Tai, Li-Chia; Niazi, Kayvan Reza; Jalali, Bahram] Calif NanoSyst Inst, Los Angeles, CA 90095 USA. [Blaby, Ian K.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Niazi, Kayvan Reza] NantWorks LLC, Culver City, CA 90232 USA. [Niazi, Kayvan Reza; Jalali, Bahram] Univ Calif Los Angeles, Dept Bioengn, Los Angeles, CA 90095 USA. [Jalali, Bahram] Univ Calif Los Angeles, David Geffen Sch Med, Dept Surg, Los Angeles, CA 90095 USA. [Blaby, Ian K.] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. RP Chen, CL (reprint author), Univ Calif Los Angeles, Dept Elect Engn, Los Angeles, CA 90095 USA.; Chen, CL (reprint author), Calif NanoSyst Inst, Los Angeles, CA 90095 USA. EM l.chen@ucla.edu FU Office of Naval Research (ONR) Multidisciplinary University Research Initiative (MURI) program on Optical Computing; U.S. Department of Energy [DE-FC02-02ER63421]; NantWorks, LLC, Culver City, California FX This work was partially supported by the Office of Naval Research (ONR) Multidisciplinary University Research Initiative (MURI) program on Optical Computing and NantWorks, LLC, Culver City, California. Ian K. Blaby was supported by the U.S. Department of Energy (grant no. DE-FC02-02ER63421) to Sabeeha Merchant. NR 69 TC 15 Z9 15 U1 11 U2 40 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 15 PY 2016 VL 6 AR 21471 DI 10.1038/srep21471 PG 16 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG4OV UT WOS:000372052400001 PM 26975219 ER PT J AU Isaienko, O Robel, I AF Isaienko, Oleksandr Robel, Istvan TI Phonon-assisted nonlinear optical processes in ultrashort-pulse pumped optical parametric amplifiers SO SCIENTIFIC REPORTS LA English DT Article ID STIMULATED POLARITON SCATTERING; POTASSIUM TITANYL PHOSPHATE; PERIODICALLY POLED KTIOPO4; RAMAN-SCATTERING; SILICA SURFACES; TERAHERTZ LASER; GENERATION; CRYSTALS; KTIOASO4; AMPLIFICATION AB Optically active phonon modes in ferroelectrics such as potassium titanyl phosphate (KTP) and potassium titanyl arsenate (KTA) in the similar to 7-20 THz range play an important role in applications of these materials in Raman lasing and terahertz wave generation. Previous studies with picosecond pulse excitation demonstrated that the interaction of pump pulses with phonons can lead to efficient stimulated Raman scattering (SRS) accompanying optical parametric oscillation or amplification processes (OPO/OPA), and to efficient polariton-phonon scattering. In this work, we investigate the behavior of infrared OPAs employing KTP or KTA crystals when pumped with similar to 800-nm ultrashort pulses of duration comparable to the oscillation period of the optical phonons. We demonstrate that under conditions of coherent impulsive Raman excitation of the phonons, when the effective chi((2)) nonlinearity cannot be considered instantaneous, the parametrically amplified waves (most notably, signal) undergo significant spectral modulations leading to an overall redshift of the OPA output. The pump intensity dependence of the redshifted OPA output, the temporal evolution of the parametric gain, as well as the pump spectral modulations suggest the presence of coupling between the nonlinear optical polarizations P-NL of the impulsively excited phonons and those of parametrically amplified waves. C1 [Isaienko, Oleksandr; Robel, Istvan] Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. RP Isaienko, O; Robel, I (reprint author), Los Alamos Natl Lab, Div Chem, POB 1663, Los Alamos, NM 87545 USA. EM oleksandr.isaienko@gmail.com; robel@lanl.gov RI Robel, Istvan/D-4124-2011 OI Robel, Istvan/0000-0002-9738-7728 FU Chemical Sciences, Biosciences and Geosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy FX These studies were supported by the Chemical Sciences, Biosciences and Geosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy. The authors wish to thank Pamela Bowlan, Dmitry Yarotski (both at MPA-CINT, LANL) and Jeffrey Moses (Cornell University, Ithaca, NY) for helpful discussions. NR 45 TC 0 Z9 0 U1 2 U2 11 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 15 PY 2016 VL 6 AR 23031 DI 10.1038/srep23031 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG4GP UT WOS:000372030100001 PM 26975881 ER PT J AU Zhang, RF Wen, XD Legut, D Fu, ZH Veprek, S Zurek, E Mao, HK AF Zhang, R. F. Wen, X. D. Legut, D. Fu, Z. H. Veprek, S. Zurek, E. Mao, H. K. TI Crystal Field Splitting is Limiting the Stability and Strength of Ultra-incompressible Orthorhombic Transition Metal Tetraborides SO SCIENTIFIC REPORTS LA English DT Article ID SOURCE EVOLUTIONARY ALGORITHM; TUNGSTEN TETRABORIDE; 1ST PRINCIPLES; HIGH-PRESSURE; MECHANICAL-PROPERTIES; ELECTRONIC-STRUCTURES; STRUCTURE PREDICTION; SUPERHARD; BORIDES; CRB4 AB The lattice stability and mechanical strengths of the supposedly superhard transition metal tetraborides (TmB4, Tm = Cr, Mn and Fe) evoked recently much attention from the scientific community due to the potential applications of these materials, as well as because of general scientific interests. In the present study, we show that the surprising stabilization of these compounds from a high symmetry to a low symmetry structure is accomplished by an in-plane rotation of the boron network, which maximizes the in- plane hybridization by crystal field splitting between d orbitals of Tm and p orbitals of B. Studies of mechanical and electronic properties of TmB4 suggest that these tetraborides cannot be intrinsically superhard. The mechanical instability is facilitated by a unique in-plane or out-of-plane weakening of the three-dimensional covalent bond network of boron along different shear deformation paths. These results shed a novel view on the origin of the stability and strength of orthorhombic TmB4, highlighting the importance of combinational analysis of a variety of parameters related to plastic deformation of the crystalline materials when attempting to design new ultra-incompressible, and potentially strong and hard solids. C1 [Zhang, R. F.; Fu, Z. H.] Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China. [Zhang, R. F.; Fu, Z. H.] Beihang Univ, Int Res Inst Multidisciplinary Sci, Beijing 100191, Peoples R China. [Zhang, R. F.; Wen, X. D.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Wen, X. D.] Chinese Acad Sci, Inst Coal Chem, State Key Lab Coal Convers, POB 165, Taiyuan 030001, Shanxi, Peoples R China. [Legut, D.] VSB Tech Univ Ostrava, Ctr IT4Innovat, CZ-70833 Ostrava, Czech Republic. [Veprek, S.] Tech Univ Munich, Dept Chem, Lichtenbergstr 4, D-85747 Garching, Germany. [Zurek, E.] SUNY Buffalo, Dept Chem, Buffalo, NY 14260 USA. [Mao, H. K.] Carnegie Inst Sci, Geophys Lab, Washington, DC 20015 USA. [Mao, H. K.] Ctr High Pressure Sci & Technol Adv Res, Shanghai 201203, Peoples R China. RP Zhang, RF (reprint author), Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China.; Zhang, RF (reprint author), Beihang Univ, Int Res Inst Multidisciplinary Sci, Beijing 100191, Peoples R China.; Zhang, RF (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM zrf@buaa.edu.cn RI Veprek, Stan/C-1248-2008; Zurek, Eva/J-4387-2012 OI Veprek, Stan/0000-0002-6016-3093; Zurek, Eva/0000-0003-0738-867X FU Fundamental Research Funds for the Central Universities; National Natural Science Foundation of China [51471018, 24173229, 91545121]; National Thousand Young Talents Program of China; Los Alamos National Laboratory Director's Postdoctoral Fellowship; European Regional Development Fund [CZ.1.05/1.1.00/02.0070]; Grant Agency of the Czech Republic [15-08971S]; national budget of the Czech Republic via the Research and Development for Innovations Operational Programme; Czech Ministry of Education, Youth and Sports via the project Large Research, Development and Innovations Infrastructures [LM2011033]; Company SHM; NSF [DMR-1505817] FX R.F.Z. and Z.H.F. is supported by the Fundamental Research Funds for the Central Universities, National Natural Science Foundation of China (51471018), National Thousand Young Talents Program of China, and Los Alamos National Laboratory Director's Postdoctoral Fellowship. D.L. acknowledges IT4Innovations Centre of Excellence project (CZ.1.05/1.1.00/02.0070) funded by the European Regional Development Fund, partial support by the Grant Agency of the Czech Republic (15-08971S), and the national budget of the Czech Republic via the Research and Development for Innovations Operational Programme, as well as Czech Ministry of Education, Youth and Sports via the project Large Research, Development and Innovations Infrastructures (LM2011033). S.V. would like to thank Company SHM for financial support of his research. E.Z. acknowledges the NSF (DMR-1505817) for financial support, and the Center for Computational Research (CCR) at SUNY Buffalo for computational support. X.D.W. are grateful for the financial support from the National Natural Science Foundation of China (No. 24173229, No. 91545121), also acknowledge the innovation foundation of Institute of Coal Chemistry, Chinese Academy of Sciences (No. Y4SC821981), Hundred-Talent Program (Chinese Academy of Sciences, No. Y5YCR41981) and Shanxi Hundred-Talent Program. The computational resources for the project were supplied by the Tianhe-2 in Lvliang, Shanxi and National Supercomputing Center in Shenzhen. We would also like to thank Prof. G. Kresse for valuable advice for the application of VASP and Dr. Maritza Veprek-Heijman for useful comments to the manuscript. NR 57 TC 9 Z9 9 U1 14 U2 40 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 15 PY 2016 VL 6 AR 23088 DI 10.1038/srep23088 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG4GT UT WOS:000372030600001 PM 26976479 ER PT J AU Hu, L Montzka, SA Miller, BR Andrews, AE Miller, JB Lehman, SJ Sweeney, C Miller, SM Thoning, K Siso, C Atlas, EL Blake, DR de Gouw, J Gilman, JB Dutton, G Elkins, JW Hall, B Chen, HL Fischer, ML Mountain, ME Nehrkorn, T Biraud, SC Moore, FL Tans, P AF Hu, Lei Montzka, Stephen A. Miller, Ben R. Andrews, Arlyn E. Miller, John B. Lehman, Scott J. Sweeney, Colm Miller, Scot M. Thoning, Kirk Siso, Carolina Atlas, Elliot L. Blake, Donald R. de Gouw, Joost Gilman, Jessica B. Dutton, Geoff Elkins, James W. Hall, Bradley Chen, Huilin Fischer, Marc L. Mountain, Marikate E. Nehrkorn, Thomas Biraud, Sebastien C. Moore, Fred L. Tans, Pieter TI Continued emissions of carbon tetrachloride from the United States nearly two decades after its phaseout for dispersive uses SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE carbon tetrachloride; emissions; United States; ozone-depleting substances; greenhouse gases ID CONTAINING HOUSEHOLD PRODUCTS; VOLATILE ORGANIC-COMPOUNDS; GAS REFERENCE NETWORK; INFORMATION CRITERION; EUROPEAN EMISSIONS; MODEL SELECTION; FLUX ESTIMATION; OCEANIC UPTAKE; TRACE GASES; STILT MODEL AB National-scale emissions of carbon tetrachloride (CCl4) are derived based on inverse modeling of atmospheric observations at multiple sites across the United States from the National Oceanic and Atmospheric Administration's flask air sampling network. We estimate an annual average US emission of 4.0 (2.0-6.5) Gg CCl4 y(-1) during 2008-2012, which is almost two orders of magnitude larger than reported to the US Environmental Protection Agency (EPA) Toxics Release Inventory (TRI) (mean of 0.06 Gg y(-1)) but only 8% (3-22%) of global CCl4 emissions during these years. Emissive regions identified by the observations and consistently shown in all inversion results include the Gulf Coast states, the San Francisco Bay Area in California, and the Denver area in Colorado. Both the observation-derived emissions and the US EPA TRI identified Texas and Louisiana as the largest contributors, accounting for one-to two-thirds of the US national total CCl4 emission during 2008-2012. These results are qualitatively consistent with multiple aircraft and ship surveys conducted in earlier years, which suggested significant enhancements in atmospheric mole fractions measured near Houston and surrounding areas. Furthermore, the emission distribution derived for CCl4 throughout the United States is more consistent with the distribution of industrial activities included in the TRI than with the distribution of other potential CCl4 sources such as uncapped landfills or activities related to population density (e.g., use of chlorine-containing bleach). C1 [Hu, Lei; Miller, Ben R.; Miller, John B.; Sweeney, Colm; Siso, Carolina; de Gouw, Joost; Gilman, Jessica B.; Dutton, Geoff; Chen, Huilin; Moore, Fred L.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Hu, Lei; Montzka, Stephen A.; Miller, Ben R.; Andrews, Arlyn E.; Miller, John B.; Sweeney, Colm; Thoning, Kirk; Siso, Carolina; Dutton, Geoff; Elkins, James W.; Hall, Bradley; Moore, Fred L.; Tans, Pieter] NOAA, Earth Syst Res Lab, Global Monitoring Div, Boulder, CO 80305 USA. [Lehman, Scott J.] Univ Colorado, Inst Arctic & Alpine Res, Boulder, CO 80309 USA. [Miller, Scot M.] Stanford Univ, Carnegie Inst Sci, Dept Global Ecol, Stanford, CA 94305 USA. [Atlas, Elliot L.] Univ Miami, Rosenstiel Sch Marine & Atmospher Sci, Miami, FL 33149 USA. [Blake, Donald R.] Univ Calif Irvine, Sch Phys Sci, Irvine, CA 92697 USA. [de Gouw, Joost; Gilman, Jessica B.] NOAA, Chem Sci Div, Earth Syst Res Lab, Boulder, CO 80305 USA. [Chen, Huilin] Univ Groningen, Ctr Isotope Res, Energy & Sustainabil Res Inst Groningen, NL-9747 AG Groningen, Netherlands. [Fischer, Marc L.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Energy Technol Area, Berkeley, CA 94720 USA. [Mountain, Marikate E.; Nehrkorn, Thomas] Atmospher & Environm Res, Lexington, MA 02421 USA. [Biraud, Sebastien C.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Earth & Environm Sci Area, Berkeley, CA 94720 USA. RP Hu, L (reprint author), Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA.; Hu, L; Montzka, SA (reprint author), NOAA, Earth Syst Res Lab, Global Monitoring Div, Boulder, CO 80305 USA. EM leihutx@gmail.com; Stephen.A.Montzka@noaa.gov RI de Gouw, Joost/A-9675-2008; Biraud, Sebastien/M-5267-2013; Gilman, Jessica/E-7751-2010; Chen, Huilin/J-9479-2012; Manager, CSD Publications/B-2789-2015; OI de Gouw, Joost/0000-0002-0385-1826; Biraud, Sebastien/0000-0001-7697-933X; Gilman, Jessica/0000-0002-7899-9948; Chen, Huilin/0000-0002-1573-6673; Montzka, Stephen/0000-0002-9396-0400; Nehrkorn, Thomas/0000-0003-0637-3468 FU National Oceanic and Atmospheric Administration (NOAA) Climate Program Office's AC4 program; California Energy Commission Public Interest Environmental Research Program Grant [DE-AC02-05CH11231] FX We thank J. Daniel, D. Godwin, S. Yvon-Lewis, A. Jacobson, K. Masarie, L. Bruhwiler, D. Baker, and S. Basu for discussion, R. Draxler and A. Stein for advice on running Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) simulations, and J. Butler, M. S. Torn, D. Mondeel, J. Higgs, M. Crotwell, P. Lang, W. Wolter, D. Neff, J. Kofler, I. Simpson, N. Blake, and others involved with program management, sampling, analysis, and logistics. We also thank members of the HIAPER HIPPO team, particularly S. Wofsy, for enabling flask sampling during that mission and Earth Networks for sample collection at the LEW site. This study was supported in part by National Oceanic and Atmospheric Administration (NOAA) Climate Program Office's AC4 program. Flask sampling at the tower sites WGC and STR was partially supported by a California Energy Commission Public Interest Environmental Research Program Grant to the Lawrence Berkeley National Laboratory under Contract DE-AC02-05CH11231. NR 49 TC 3 Z9 3 U1 4 U2 19 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 15 PY 2016 VL 113 IS 11 BP 2880 EP 2885 DI 10.1073/pnas.1522284113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG4BF UT WOS:000372014200042 PM 26929368 ER PT J AU Sung, N Lee, J Kim, JH Chang, C Joachimiak, A Lee, S Tsai, FTF AF Sung, Nuri Lee, Jungsoon Kim, Ji-Hyun Chang, Changsoo Joachimiak, Andrzej Lee, Sukyeong Tsai, Francis T. F. TI Mitochondrial Hsp90 is a ligand-activated molecular chaperone coupling ATP binding to dimer closure through a coiled-coil intermediate SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE TRAP1; Hsp90; molecular chaperone ID SHOCK-PROTEIN 90; ESCHERICHIA-COLI HSP90; N-TERMINAL DOMAIN; IN-VIVO; CONFORMATIONAL DYNAMICS; CRYSTAL-STRUCTURES; HYDROLYSIS; TRAP1; MECHANISM; HSP70 AB Heat-shock protein of 90 kDa (Hsp90) is an essential molecular chaperone that adopts different 3D structures associated with distinct nucleotide states: a wide-open, V-shaped dimer in the apo state and a twisted, N-terminally closed dimer with ATP. Although the N domain is known to mediate ATP binding, how Hsp90 senses the bound nucleotide and facilitates dimer closure remains unclear. Here we present atomic structures of human mitochondrial Hsp90(N) (TRAP1(N)) and a composite model of intact TRAP1 revealing a previously unobserved coiled-coil dimer conformation that may precede dimer closure and is conserved in intact TRAP1 in solution. Our structure suggests that TRAP1 normally exists in an autoinhibited state with the ATP lid bound to the nucleotide-binding pocket. ATP binding displaces the ATP lid that signals the cis-bound ATP status to the neighboring subunit in a highly cooperative manner compatible with the coiled-coil intermediate state. We propose that TRAP1 is a ligand-activated molecular chaperone, which couples ATP binding to dramatic changes in local structure required for protein folding. C1 [Sung, Nuri; Lee, Jungsoon; Kim, Ji-Hyun; Lee, Sukyeong; Tsai, Francis T. F.] Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. [Chang, Changsoo; Joachimiak, Andrzej] Argonne Natl Lab, Biosci Div, Struct Biol Ctr, Argonne, IL 60439 USA. [Tsai, Francis T. F.] Baylor Coll Med, Dept Mol & Cellular Biol, Houston, TX 77030 USA. [Tsai, Francis T. F.] Baylor Coll Med, Dept Mol Virol & Microbiol, Houston, TX 77030 USA. [Kim, Ji-Hyun] Louisiana State Univ, Pennington Biomed Res Ctr, Baton Rouge, LA 70808 USA. RP Lee, S; Tsai, FTF (reprint author), Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA.; Tsai, FTF (reprint author), Baylor Coll Med, Dept Mol & Cellular Biol, Houston, TX 77030 USA.; Tsai, FTF (reprint author), Baylor Coll Med, Dept Mol Virol & Microbiol, Houston, TX 77030 USA. EM slee@bcm.edu; ftsai@bcm.edu FU US Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357]; National Institutes of Health [R01 GM111084, R01 GM104980]; Welch Foundation [Q-1530] FX We thank Drs. D. Toft, S. Felts, J. Silberg, J. Barral, and E. Craig for expression constructs. Use of the Structural Biology Center (SBC) beamlines at the Advanced Photon Source was supported by the US Department of Energy, Office of Biological and Environmental Research (Contract DE-AC02-06CH11357). This work was supported by the National Institutes of Health (Grants R01 GM111084 and R01 GM104980) and the Welch Foundation (Grant Q-1530). J.L. was a Welch fellow. NR 57 TC 4 Z9 4 U1 4 U2 9 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD MAR 15 PY 2016 VL 113 IS 11 BP 2952 EP 2957 DI 10.1073/pnas.1516167113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG4BF UT WOS:000372014200054 PM 26929380 ER PT J AU Bai, Y Yan, D Yu, CY Cao, LN Wang, CL Zhang, JS Zhu, HY Hu, YS Dai, S Lu, JL Zhang, WF AF Bai, Ying Yan, Dong Yu, Caiyan Cao, Lina Wang, Chunlei Zhang, Jinshui Zhu, Huiyuan Hu, Yong-Sheng Dai, Sheng Lu, Junling Zhang, Weifeng TI Core-shell Si@TiO2 nanosphere anode by atomic layer deposition for Li-ion batteries SO JOURNAL OF POWER SOURCES LA English DT Article DE Silicon nanospheres; Titanium dioxide overcoating; Atomic layer deposition (ALD); Cycling performance; Buffering effect ID LITHIUM RECHARGEABLE BATTERIES; TIO2 THIN-FILMS; SILICON NANOWIRES; COMPOSITE ELECTRODES; COULOMBIC EFFICIENCY; XPS CHARACTERIZATION; PERFORMANCE; NANOPARTICLES; SIZE; NANOCOMPOSITE AB Silicon (Si) has been regarded as next-generation anode for high-energy lithium-ion batteries (LIBs) due to its high Li storage capacity (4200 mA h g(-1)). However, the mechanical degradation and resultant capacity fade critically hinder its practical application. In this regard, we demonstrate that nanocoating of Si spheres with a 3 nm titanium dioxide (TiO2) layer via atomic layer deposition (ALD) can utmostly balance the high conductivity and the good structural stability to improve the cycling stability of Si core material. The resultant sample, Si@TiO2-3 nm core-shell nanospheres, exhibits the best electrochemical performance of all with a highest initial Coulombic efficiency and specific charge capacity retention after 50 cycles at 0.1C (82.39% and 1580.3 mA h g(-1)). In addition to making full advantage of the ALD technique, we believe that our strategy and comprehension in coating the electrode and the active material could provide a useful pathway towards enhancing Si anode material itself and community of LIBs. (C) 2016 Elsevier B.V. All rights reserved. C1 [Bai, Ying; Yan, Dong; Yu, Caiyan; Zhang, Weifeng] Henan Univ, Key Lab Photovolta Mat Henan Prov, Kaifeng 475004, Peoples R China. [Bai, Ying; Yan, Dong; Yu, Caiyan; Zhang, Weifeng] Henan Univ, Sch Phys & Elect, Kaifeng 475004, Peoples R China. [Cao, Lina; Wang, Chunlei; Lu, Junling] Univ Sci & Technol China, iChem, Hefei Natl Lab Phys Sci Microscale, Dept Chem Phys, Hefei 230026, Peoples R China. [Cao, Lina; Wang, Chunlei; Lu, Junling] Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Hefei 230026, Peoples R China. [Bai, Ying; Zhang, Jinshui; Zhu, Huiyuan; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Hu, Yong-Sheng] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. RP Zhang, WF (reprint author), Henan Univ, Key Lab Photovolta Mat Henan Prov, Kaifeng 475004, Peoples R China.; Zhang, WF (reprint author), Henan Univ, Sch Phys & Elect, Kaifeng 475004, Peoples R China.; Lu, JL (reprint author), Univ Sci & Technol China, iChem, Hefei Natl Lab Phys Sci Microscale, Dept Chem Phys, Hefei 230026, Peoples R China.; Lu, JL (reprint author), Univ Sci & Technol China, CAS Key Lab Mat Energy Convers, Hefei 230026, Peoples R China. EM junling@ustc.edu.cn; wfzhang@henu.edu.cn RI Dai, Sheng/K-8411-2015; zhang, Jinshui/D-9749-2016; Hu, Yong-Sheng/H-1177-2011 OI Dai, Sheng/0000-0002-8046-3931; zhang, Jinshui/0000-0003-4649-6526; Hu, Yong-Sheng/0000-0002-8430-6474 FU National Natural Science Foundation of China [50902044, 21473169, 51402283]; 863 Program of China [2015AA034201]; State Scholarship Fund from China Scholarship Council [201308410027]; Program for Science & Technology Innovation Talents in Universities of Henan Province, China [16HASTIT042]; Recruitment Program of Global Youth Experts; Scientific Research Foundation for the Returned Overseas Chinese Scholars; U.S. Department of Energy's Office of Basic Energy Science, Division of Materials Sciences and Engineering; UT-Battelle, LLC FX This work was supported by the National Natural Science Foundation of China (50902044, 21473169, and 51402283), the 863 Program of China (2015AA034201), the State Scholarship Fund from China Scholarship Council (201308410027), the Program for Science & Technology Innovation Talents in Universities of Henan Province, China (16HASTIT042), and the Recruitment Program of Global Youth Experts, the Scientific Research Foundation for the Returned Overseas Chinese Scholars, and the U.S. Department of Energy's Office of Basic Energy Science, Division of Materials Sciences and Engineering, under contract with UT-Battelle, LLC (SD). NR 59 TC 7 Z9 7 U1 62 U2 250 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD MAR 15 PY 2016 VL 308 BP 75 EP 82 DI 10.1016/j.jpowsour.2016.01.049 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DF5AJ UT WOS:000371363900010 ER PT J AU Deng, XC Hu, M Wei, XL Wang, W Mueller, KT Chen, Z Hu, JZ AF Deng, Xuchu Hu, Mary Wei, Xiaoliang Wang, Wei Mueller, Karl T. Chen, Zhong Hu, Jian Zhi TI Nuclear magnetic resonance studies of the solvation structures of a high-performance nonaqueous redox flow electrolyte SO JOURNAL OF POWER SOURCES LA English DT Article DE Electrolyte; Nuclear magnetic resonance; Nonaqueous redox flow battery; Solvation structures; Molecular dynamics ID RESEARCH-AND-DEVELOPMENT; ELECTROCHEMICAL PROPERTIES; ENERGY-STORAGE; BATTERY; PROGRESS; IMPACT; ION AB Understanding the solvation structures of electrolytes is important for developing nonaqueous redox flow batteries that hold considerable potential for future large scale energy storage systems. The utilization of an emerging ionic-derivatived ferrocene compound, ferrocenylmethyl dimethyl ethyl ammonium bis(trifluoromethanesulfonyl)imide (Fc1N112-TFSI), has recently overcome the issue of solubility in the supporting electrolyte. In this work, C-13, H-1 and O-17 NMR investigations were carried out using electrolyte solutions consisting of Fc1N112-TFSI as the solute and the mixed alkyl carbonate as the solvent. It was observed that the spectra of C-13 experience changes of chemical shifts while those of O-17 undergo linewidth broadening, indicating interactions between solute and solvent molecules. Quantum chemistry calculations of both molecular structures and chemical shifts (C-13, H-1 and O-17) are performed for interpreting experimental results and for understanding the detailed solvation structures. The results indicate that Fc1N112-TFSI is dissociated at varying degrees in mixed solvent depending on concentrations. At dilute solute concentrations, most Fc1N112(+) and TFSI- are fully disassociated with their own solvation shells formed by solvent molecules. At saturated concentration, Fc1N112(+)-TFSI- contact ion pairs are formed and the solvent molecules are preferentially interacting with the Fc rings rather than interacting with the ionic pendant arm of Fc1N112-TFSI. (C) 2016 Elsevier B.V. All rights reserved. C1 [Deng, Xuchu; Chen, Zhong] Xiamen Univ, Dept Elect Sci, Xiamen 361005, Peoples R China. [Deng, Xuchu; Hu, Mary; Wei, Xiaoliang; Wang, Wei; Mueller, Karl T.; Hu, Jian Zhi] Pacific NW Natl Lab, JCESR, Richland, WA 99352 USA. [Mueller, Karl T.] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. RP Chen, Z (reprint author), Xiamen Univ, Dept Elect Sci, Xiamen 361005, Peoples R China.; Hu, JZ (reprint author), Pacific NW Natl Lab, JCESR, Richland, WA 99352 USA. EM chenz@xmu.edu.cn; Jianzhi.Hu@pnnl.gov RI Hu, Jian Zhi/F-7126-2012; Wang, Wei/F-4196-2010; Chen, Zhong/G-4601-2010 OI Wang, Wei/0000-0002-5453-4695; FU U.S. Department of Energy, Office of Science, Basic Energy Sciences (BES); U.S. Department of Energy's (DOE's) Office of Electricity Delivery and Energy Reliability (OE) [57558]; DOE's Office of Biological and Environmental Research (BER); National Natural Science Fund of China [21327001]; Department of Energy [DE-AC05-76RLO1830] FX This work was led intellectually as part of the Joint Center for Energy Storage Research (JCESR), an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences (BES). The NMR sample preparations were supported by the funding from the U.S. Department of Energy's (DOE's) Office of Electricity Delivery and Energy Reliability (OE) (under Contract No. 57558). The NMR, and computational studies were conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research (BER) and located at PNNL. Xuchu Deng was partially supported by the National Natural Science Fund of China under Grant 21327001. PNNL is operated by Battelle for the Department of Energy under Contract DE-AC05-76RLO1830. NR 28 TC 3 Z9 3 U1 9 U2 24 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD MAR 15 PY 2016 VL 308 BP 172 EP 179 DI 10.1016/j.jpowsour.2015.12.005 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DF5AJ UT WOS:000371363900019 ER PT J AU Visser, A Moran, JE Hillegonds, D Singleton, MJ Kulongoski, JT Belitz, K Esser, BK AF Visser, A. Moran, J. E. Hillegonds, Darren Singleton, M. J. Kulongoski, Justin T. Belitz, Kenneth Esser, B. K. TI Geostatistical analysis of tritium, groundwater age and other noble gas derived parameters in California SO WATER RESEARCH LA English DT Article DE Groundwater; Water age; Geostatistics; Tritium; Noble gas ID THICK UNSATURATED ZONE; SAN-JOAQUIN VALLEY; SHALLOW GROUNDWATER; ARTIFICIAL RECHARGE; EXCESS AIR; ARSENIC CONCENTRATIONS; NITRATE CONTAMINATION; ENVIRONMENTAL TRACERS; SEASONAL-VARIATION; MASS-SPECTROMETRY AB Key characteristics of California groundwater systems related to aquifer vulnerability, sustainability, recharge locations and mechanisms, and anthropogenic impact on recharge are revealed in a spatial geostatistical analysis of a unique data set of tritium, noble gases and other isotopic analyses unprecedented in size at nearly 4000 samples. The correlation length of key groundwater residence time parameters varies between tens of kilometers (H-3; age) to the order of a hundred kilometers (He-4(ter); C-14; He-3(trit)). The correlation length of parameters related to climate, topography and atmospheric processes is on the order of several hundred kilometers (recharge temperature; delta O-18). Young groundwater ages that highlight regional recharge areas are located in the eastern San Joaquin Valley, in the southern Santa Clara Valley Basin, in the upper LA basin and along unlined canals carrying Colorado River water, showing that much of the recent recharge in central and southern California is dominated by river recharge and managed aquifer recharge. Modern groundwater is found in wells with the top open intervals below 60 m depth in the southeastern San Joaquin Valley, Santa Clara Valley and Los Angeles basin, as the result of intensive pumping and/or managed aquifer recharge operations. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Visser, A.; Singleton, M. J.; Esser, B. K.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Moran, J. E.] Calif State Univ East Bay, Hayward, CA USA. [Hillegonds, Darren] IAEA, Vienna, Austria. [Kulongoski, Justin T.; Belitz, Kenneth] USGS Calif Water Sci Ctr, Livermore, CA USA. RP Visser, A (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. EM visser3@llnl.gov RI Visser, Ate/G-8826-2012; OI Kulongoski, Justin/0000-0002-3498-4154 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Groundwater Ambient Monitoring and Assessment Program [LLNL-JRNL-674881] FX This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. This data were collected in collaboration with the U.S. Geological Survey, and funded by the Groundwater Ambient Monitoring and Assessment Program. LLNL-JRNL-674881. NR 126 TC 0 Z9 0 U1 8 U2 28 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0043-1354 J9 WATER RES JI Water Res. PD MAR 15 PY 2016 VL 91 BP 314 EP 330 DI 10.1016/j.watres.2016.01.004 PG 17 WC Engineering, Environmental; Environmental Sciences; Water Resources SC Engineering; Environmental Sciences & Ecology; Water Resources GA DF2QO UT WOS:000371189100032 PM 26803267 ER PT J AU Xie, J Chen, JQ Sun, G Zha, TS Yang, B Chu, HS Liu, JG Wan, SQ Zhou, CX Ma, H Bourque, CPA Shao, CL John, R Ouyang, ZT AF Xie, Jing Chen, Jiquan Sun, Ge Zha, Tianshan Yang, Bai Chu, Housen Liu, Junguo Wan, Shiqiang Zhou, Caixian Ma, Hong Bourque, Charles P. -A. Shao, Changliang John, Ranjeet Ouyang, Zutao TI Ten-year variability in ecosystem water use efficiency in an oak-dominated temperate forest under a warming climate SO AGRICULTURAL AND FOREST METEOROLOGY LA English DT Article DE Dryness index; Eddy covariance; Evapotranspiration; Gross ecosystem production; Long-term variability; Water use efficiency ID CARBON-DIOXIDE; EDDY COVARIANCE; TERRESTRIAL ECOSYSTEMS; ENVIRONMENTAL CONTROLS; SOIL RESPIRATION; SONIC ANEMOMETER; ASPEN FOREST; LONG-TERM; FLUXES; EXCHANGE AB The impacts of extreme weather events on water-carbon (C) coupling and ecosystem-scale water use efficiency (WUE) over a long term are poorly understood. We analyzed the changes in ecosystem water use efficiency (WUE) from 10 years of eddy-covariance measurements (2004-2013) over an oak-dominated temperate forest in Ohio, USA. The aim was to investigate the long-term response of ecosystem WUE to measured changes in site-biophysical conditions and ecosystem attributes. The oak forest produced new plant biomass of 2.5 +/- 0.2 gC kg(-1) of water loss annually. Monthly evapotranspiration (ET) and gross ecosystem production (GEP) were tightly coupled over the 10-year study period (R-2=0.94). Daily WUE had a linear relationship with air temperature (T-a) in low-temperature months and a unimodal relationship with T-a in high-temperature months during the growing season. On average, daily WUE ceased to increase when T-a exceeded 22 degrees C in warm months for both wet and dry years. Monthly WUE had a strong positive linear relationship with leaf area index (LAI), net radiation (R-n), and T-a and weak logarithmic relationship with water vapor pressure deficit (VPD) and precipitation (P) on a growing-season basis. When exploring the regulatory mechanisms on WUE within each season, spring LAI and P, summer R-n and T-a, and autumnal VPD and R-n were found to be the main explanatory variables for seasonal variation in WUE. The model developed in this study was able to capture 78% of growing-season variation in WUE on a monthly basis. The negative correlation between WUE and A in spring was mainly due to the high precipitation amounts in spring, decreasing GEP and WUE when LAI was still small, adding ET being observed to increase with high levels of evaporation as a result of high SWC in spring. Summer WUE had a significant decreasing trend across the 10 years mainly due to the combined effect of seasonal drought and increasing potential and available energy increasing ET, but decreasing GEP in summer. We concluded that seasonal dynamics of the interchange between precipitation and drought status of the system was an important variable in controlling seasonal WUE in wet years. In contrast, despite the negative impacts of unfavorable warming, available groundwater and an early start of the growing season were important contributing variables in high seasonal GEP, and thus, high seasonal WUE in dry years. (C) 2015 Elsevier B.V. All rights reserved. C1 [Xie, Jing; Zha, Tianshan] Beijing Forestry Univ, Coll Soil & Water Conservat, Beijing 100083, Peoples R China. [Chen, Jiquan; Shao, Changliang; John, Ranjeet; Ouyang, Zutao] Michigan State Univ, CGCEO Geog, E Lansing, MI 48823 USA. [Xie, Jing; Zhou, Caixian; Ma, Hong] Beijing Forestry Carbon Sequestrat Adm, Beijing 100013, Peoples R China. [Sun, Ge] US Forest Serv, USDA, Southern Res Stn, Eastern Forest Environm Threat Assessment Ctr, Raleigh, NC 27606 USA. [Yang, Bai] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37931 USA. [Chu, Housen] Univ Calif Berkeley, Dept Environm Sci, Berkeley, CA 94720 USA. [Liu, Junguo] Beijing Forestry Univ, Coll Nat Conservat, Beijing 100083, Peoples R China. [Wan, Shiqiang] Henan Univ, Coll Life Sci, Key Lab Plant Stress Biol, Kaifeng 475004, Henan, Peoples R China. [Bourque, Charles P. -A.] Univ New Brunswick, Forestry & Environm Management, POB 4400, Fredericton, NB E3B 5A3, Canada. RP Xie, J (reprint author), Beijing Forestry Univ, Coll Soil & Water Conservat, Beijing 100083, Peoples R China.; Chen, JQ (reprint author), Michigan State Univ, CGCEO Geog, E Lansing, MI 48823 USA.; Xie, J (reprint author), Beijing Forestry Carbon Sequestrat Adm, Beijing 100013, Peoples R China. EM xiejingbj@126.com; jqchen@msu.edu RI Wan, Shiqiang/B-5799-2009; Chu, Housen/Q-6517-2016; Chen, Jiquan/D-1955-2009; OI Chu, Housen/0000-0002-8131-4938; Liu, Junguo/0000-0002-5745-6311 FU Eastern Forest Environmental Threat Assessment Center; Southern Research Station [03-CA-11330147-073, 04-CA-11330147-238]; Toledo Area Metropark; US-China Carbon Consortium (USCCC) FX This study was funded by Eastern Forest Environmental Threat Assessment Center, Southern Research Station (Cooperative Agreements 03-CA-11330147-073 and 04-CA-11330147-238), the Toledo Area Metropark, and the US-China Carbon Consortium (USCCC) that promotes collaborative research among interested institutions in the US and China. We are thankful to many members of the Landscape Ecology and Ecosystem Sciences (LEES) Lab at Michigan State University, including Gabriela Shirkey, for their thoughtful comments and language assistance. NR 50 TC 4 Z9 4 U1 14 U2 53 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-1923 EI 1873-2240 J9 AGR FOREST METEOROL JI Agric. For. Meteorol. PD MAR 15 PY 2016 VL 218 BP 209 EP 217 DI 10.1016/j.agrformet.2015.12.059 PG 9 WC Agronomy; Forestry; Meteorology & Atmospheric Sciences SC Agriculture; Forestry; Meteorology & Atmospheric Sciences GA DE8RT UT WOS:000370905100020 ER PT J AU Nandasiri, MI Jambovane, SR McGrail, BP Schaef, HT Nune, SK AF Nandasiri, Manjula I. Jambovane, Sachin R. McGrail, B. Peter Schaef, Herbert T. Nune, Satish. K. TI Adsorption, separation, and catalytic properties of densified metal-organic frameworks SO COORDINATION CHEMISTRY REVIEWS LA English DT Review DE MOF pellets; Densification; Hydrogen storage; Volumetric adsorption; Thermal conductivity; MOF composites ID ZEOLITIC IMIDAZOLATE FRAMEWORKS; LIQUID-CHROMATOGRAPHIC SEPARATION; HYDROGEN STORAGE; POWDER DENSIFICATION; THERMAL-CONDUCTIVITY; METHANE ADSORPTION; MIL-101 MONOLITHS; AQUEOUS-SOLUTIONS; PHASE ADSORPTION; MOF-5 COMPOSITES AB Metal-organic frameworks (MOFs) are one of the widely investigated materials of 21st century due to their unique properties such as structural tailorability, controlled porosity, and crystallinity. These exceptional properties make them promising candidates for various applications including gas adsorption and storage, separation, and catalysis. However, commercial applications of MOFs produced by conventional methods including solvothermal or hydrothermal synthesis are rather limited or restricted because they often produce fine powders. The use of MOF powders for industrial applications often results in pressure drop problems similar to the case with zeolites and limited robustness against water. To realize these materials for practical applications, densification of MOFs (by increasing pellet density) is routinely employed to form pellets, extrudates or beads to improve the overall density, volumetric adsorption, mechanical and thermal properties. However, the improvements come with some drawbacks such as reduction in overall porosity, surface area, and gravimetric adsorption capacity. Thus, optimizing the properties of densified MOF's by tuning the pellet density is very crucial for realizing these materials for industrial applications. Methods that increase the packing density in MOFs (for example by intentional interpenetration, etc.), which is different from pellet density, is not the scope of this review. In this review, the properties and applications of densified MOFs with different metal clusters and organic linkers are discussed. (C) 2016 Elsevier B.V. All rights reserved. C1 [Nandasiri, Manjula I.; Jambovane, Sachin R.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. [McGrail, B. Peter; Nune, Satish. K.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. [Schaef, Herbert T.] Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99354 USA. RP Nune, SK (reprint author), Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. EM satish.nune@pnnl.gov RI Jambovane, Sachin/G-2865-2016 OI Jambovane, Sachin/0000-0002-5063-6969 FU U.S. Department of Energy (DOE), Office of Fossil Energy; DOE by Battelle Memorial Institute [DE-AC06-76RLO-1830] FX The U.S. Department of Energy (DOE), Office of Fossil Energy, supported this work. The Pacific Northwest National Laboratory (PNNL) is operated for DOE by Battelle Memorial Institute under Contract# DE-AC06-76RLO-1830. NR 144 TC 25 Z9 25 U1 143 U2 484 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0010-8545 EI 1873-3840 J9 COORDIN CHEM REV JI Coord. Chem. Rev. PD MAR 15 PY 2016 VL 311 BP 38 EP 52 DI 10.1016/j.ccr.2015.12.004 PG 15 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DE8LP UT WOS:000370887800003 ER PT J AU Sikes, EL Cook, MS Guilderson, TP AF Sikes, Elisabeth L. Cook, Mea S. Guilderson, Thomas P. TI Reduced deep ocean ventilation in the Southern Pacific Ocean during the last glaciation persisted into the deglaciation SO EARTH AND PLANETARY SCIENCE LETTERS LA English DT Article DE radiocarbon; reservoir ages; Southern Ocean; last glaciation; CO2; climate change ID ATMOSPHERIC CO2 CONCENTRATIONS; WESTERN NORTH-ATLANTIC; CARBON-DIOXIDE RELEASE; ANTARCTIC SEA-ICE; NEW-ZEALAND; RADIOCARBON-AGE; YOUNGER DRYAS; OVERTURNING CIRCULATION; CLIMATE CHANGES; NZ-INTIMATE AB Marine radiocarbon (C-14) is widely used to trace ocean circulation and the C-14 levels of interior ocean water masses can provide insight into atmosphere-ocean exchange of CO2 the since the last glaciation. Using tephras as stratigraphic tie points with which to estimate past atmospheric Delta C-14, we reconstructed a series of deep radiocarbon ages for several time slices from the last glaciation through the deglaciation and Holocene in the Southwestern Pacific. Glacial ventilation ages were much greater in magnitude than modern and had a strong mid-depth Delta C-14 minimum centered on similar to 2500 m. Glacial radiocarbon ages of intermediate depth waters (600-1200 m) were similar to 800 to 1600 C-14 years, about twice modern and persisted through the early deglaciation. Notably, in the glaciation shallower depths were significantly more enriched in C-14 than waters between 1600 and 3800 m, which were similar to 4000 to 6200 C-14 years, or about 3-5 times older than modern. Abyssal waters deeper than 4000 m were also more C-14 rich than the overlying deep water. With radiocarbon ages of 1800-2300 C-14 years, this was similar to modern values. In the early deglaciation, Delta C-14 depleted waters were flushed from shallower depths first and replaced with progressively younger waters such that by 18 ka, the deep to intermediate age difference was reduced by half, and by similar to 14 ka a modern-type Delta C-14 profile for deep ocean water masses was in place. Our results 1) confirm a deep C-14 depleted water mass during the LGM and early deglaciation, and 2) constrain the extent of this "old" water in the Southern Pacific as between 1600 m and 3800 m. The availability of atmospheric ages from tephras reveals that the presence of older surface reservoir ages in the glaciation caused the estimation of ventilation ages from simple benthic-planktonic offsets to significantly underestimate the depletion of Delta C-14 in deep waters. This may have had a role in masking the large change in reservoir ages since the glaciation when using benthic-planktonic reservoir age estimates. (C) 2016 Elsevier B.V. All rights reserved. C1 [Sikes, Elisabeth L.] Rutgers State Univ, Inst Marine & Coastal Sci, 71 Dudley Rd, New Brunswick, NJ 08903 USA. [Cook, Mea S.] Williams Coll, Dept Geosci, 947 Main St, Williamstown, MA 01267 USA. [Guilderson, Thomas P.] Univ Calif Santa Cruz, Dept Ocean Sci, Santa Cruz, CA 95064 USA. [Guilderson, Thomas P.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Sikes, EL (reprint author), Rutgers State Univ, Inst Marine & Coastal Sci, 71 Dudley Rd, New Brunswick, NJ 08903 USA. EM sikes@marine.rutgers.edu OI Sikes, Elisabeth/0000-0003-2900-3283 FU NSF [OCE-0136651, OCE-0425053, OCE 0823487]; Hanse Wischenschaftkollege FX We thank the crew of the R/V Roger Revelle for assistance in obtaining the RR0503 cores. We thank NIWA for providing cores from their collection. NSF grants OCE-0136651, OCE-0425053, OCE 0823487 to ELS, TPG and MYC funded this work. A fellowship from the Hanse Wischenschaftkollege to ELS supported writing of the manuscript. NR 78 TC 5 Z9 5 U1 8 U2 22 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0012-821X EI 1385-013X J9 EARTH PLANET SC LETT JI Earth Planet. Sci. Lett. PD MAR 15 PY 2016 VL 438 BP 130 EP 138 DI 10.1016/j.epsl.2015.12.039 PG 9 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DE8UV UT WOS:000370913100014 ER PT J AU Heck, PR Schmitz, B Rout, SS Tenner, T Villalon, K Cronholm, A Terfelt, F Kita, NT AF Heck, Philipp R. Schmitz, Birger Rout, Surya S. Tenner, Travis Villalon, Krysten Cronholm, Anders Terfelt, Fredrik Kita, Noriko T. TI A search for H-chondritic chromite grains in sediments that formed immediately after the breakup of the L-chondrite parent body 470 Ma ago SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID ORDOVICIAN LOCKNE CRATER; EXTRATERRESTRIAL CHROMITE; SOUTHERN SWEDEN; TRANSANTARCTIC MOUNTAINS; MARINE LIMESTONE; OXYGEN-ISOTOPE; NOBLE-GASES; METEORITE; MICROMETEORITES; EVENT AB A large abundance of L-chondritic material, mainly in the form of fossil meteorites and chromite grains from micrometeorites, has been found in mid-Ordovician 470 Ma old sediments globally. The material has been determined to be ejecta from the L chondrite parent body breakup event, a major collision in the asteroid belt 470 Ma ago. In this study we search the same sediments for H-chondritic chromite grains in order to improve our understanding of the extraterrestrial flux to Earth after the asteroid breakup event. We have used SIMS in conjunction with quantitative SEM/EDS to determine the three oxygen isotopic and elemental compositions, respectively, of a total of 120 randomly selected, sediment-dispersed extraterrestrial chromite grains mainly representing micrometeorites from 470 Ma old post-breakup limestone from the Thorsberg quarry in Sweden and the Lynna River site in Russia. We show that 99% or more of the grains are L-chondritic, whereas the H-chondritic fraction is 1% or less. The L-/H-chondrite ratio after the breakup thus was >99 compared to 1.1 in today's meteoritic flux. This represents independent evidence, in agreement with previous estimates based on sediment-dispersed extraterrestrial chromite grain abundances and sedimentation rates, of a two orders of magnitude higher post-breakup flux of L-chondritic material in the micrometeorite fraction. Finally, we confirm the usefulness of three oxygen isotopic SIMS analyses of individual extraterrestrial chromite grains for classification of equilibrated ordinary chondrites. The H-and L-chondritic chromites differ both in their three oxygen isotopic and elemental compositions, but there is some overlap between the groups. In chromite, TiO2 is the oxide most resistant to diagenesis, and the combined application of TiO2 and oxygen three-isotope analysis can resolve uncertainties arising from the compositional overlaps. (C) 2016 The Authors. Published by Elsevier Ltd. C1 [Heck, Philipp R.; Schmitz, Birger; Rout, Surya S.; Villalon, Krysten] Field Museum Nat Hist, Robert A Pritzker Ctr Meteorit & Polar Studies, 1400 S Lake Shore Dr, Chicago, IL 60605 USA. [Heck, Philipp R.; Rout, Surya S.; Villalon, Krysten] Univ Chicago, Chicago Ctr Cosmochem, 5734 S Ellis Ave, Chicago, IL 60637 USA. [Heck, Philipp R.; Villalon, Krysten] Univ Chicago, Dept Geophys Sci, 5734 S Ellis Ave, Chicago, IL 60637 USA. [Schmitz, Birger; Cronholm, Anders; Terfelt, Fredrik] Lund Univ, Dept Phys, Astrogeobiol Lab, POB 118, SE-22100 Lund, Sweden. [Tenner, Travis; Kita, Noriko T.] Univ Wisconsin, Dept Geosci, WiscSIMS, 1215 W Dayton St, Madison, WI 53706 USA. [Tenner, Travis] Los Alamos Natl Lab, Chem Div Nucl & Radiochem, MSJ514, Los Alamos, NM 87545 USA. RP Heck, PR (reprint author), Field Museum Nat Hist, Robert A Pritzker Ctr Meteorit & Polar Studies, 1400 S Lake Shore Dr, Chicago, IL 60605 USA. EM prheck@fieldmuseum.org RI Kita, Noriko/H-8035-2016 OI Kita, Noriko/0000-0002-0204-0765 FU ERC-Advanced Grant (ASTROGEOBIO-SPHERE); NSF; NSEC [NSF EEC-0647560]; MRSEC [NSF DMR-1121262]; Keck Foundation; State of Illinois; Northwestern University; Tawani Foundation; NASA; W.H. Ganz III FX The authors acknowledge maintenance by B. Strack for the Field Museum's SEM laboratory and J. Kern for the WiscSIMS laboratory, F. Iqbal for support in the AGB laboratory, A. Lindskog for providing the Ly2U grains, and L. Koop, A. M. Davis, and T. Stephan for helpful discussions. We thank an anonymous reviewer and M. M. M. Meier for constructive reviews. The study was supported by an ERC-Advanced Grant (ASTROGEOBIO-SPHERE) to BS. The WiscSIMS lab is partially supported by NSF. 3D microscopy was performed in the Keck-II facility of the NUANCE Center at Northwestern University. The NUANCE Center is supported by NSEC (NSF EEC-0647560), MRSEC (NSF DMR-1121262), the Keck Foundation, the State of Illinois, and Northwestern University. PRH acknowledges funding from the Tawani Foundation and from W.H. Ganz III. KV was supported by NASA through grants to A.M. Davis. NR 30 TC 3 Z9 3 U1 1 U2 6 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD MAR 15 PY 2016 VL 177 BP 120 EP 129 DI 10.1016/j.gca.2015.11.042 PG 10 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DE9PH UT WOS:000370969700008 ER PT J AU Tinnacher, RM Holmboe, M Tournassat, C Bourg, IC Davis, JA AF Tinnacher, Ruth M. Holmboe, Michael Tournassat, Christophe Bourg, Ian C. Davis, James A. TI Ion adsorption and diffusion in smectite: Molecular, pore, and continuum scale views SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID SOCIETY SOURCE CLAYS; ELECTRICAL DOUBLE-LAYER; COMPACTED BENTONITE; OPALINUS CLAY; BASE-LINE; DYNAMICS SIMULATIONS; OSMOTIC EFFICIENCY; CONFINING PRESSURE; THROUGH-DIFFUSION; ARGILLACEOUS ROCK AB Clay-rich media have been proposed as engineered barrier materials or host rocks for high level radioactive waste repositories in several countries. Hence, a detailed understanding of adsorption and diffusion in these materials is needed, not only for radioactive contaminants, but also for predominant earth metals, which can affect radionuclide speciation and diffusion. The prediction of adsorption and diffusion in clay-rich media, however, is complicated by the similarity between the width of clay nanopores and the thickness of the electrical double layer (EDL) at charged clay mineral-water interfaces. Because of this similarity, the distinction between 'bulk liquid' water and 'surface' water (i.e., EDL water) in clayey media can be ambiguous. Hence, the goal of this study was to examine the ability of existing pore scale conceptual models (single porosity models) to link molecular and macroscopic scale data on adsorption and diffusion in compacted smectite. Macroscopic scale measurements of the adsorption and diffusion of calcium, bromide, and tritiated water in Na-montmorillonite were modeled using a multi-component reactive transport approach while testing a variety of conceptual models of pore scale properties (adsorption and diffusion in individual pores). Molecular dynamics (MD) simulations were carried out under conditions similar to those of our macroscopic scale diffusion experiments to help constrain the pore scale models. Our results indicate that single porosity models cannot be simultaneously consistent with our MD simulation results and our macroscopic scale diffusion data. A dual porosity model, which allows for the existence of a significant fraction of bulk liquid water-even at conditions where the average pore width is only a few nanometers-may be required to describe both pore scale and macroscopic scale data. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Tinnacher, Ruth M.; Holmboe, Michael; Tournassat, Christophe; Bourg, Ian C.; Davis, James A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Earth & Environm Sci Area, Berkeley, CA 94720 USA. [Holmboe, Michael] Umea Univ, Dept Chem, Uppsala, Sweden. [Tournassat, Christophe] French Geol Survey, BRGM, Orleans, France. [Bourg, Ian C.] Princeton Univ, Dept Civil & Environm Engn CEE, Princeton, NJ 08544 USA. [Bourg, Ian C.] Princeton Univ, PEI, Princeton, NJ 08544 USA. RP Tinnacher, RM (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Earth & Environm Sci Area, Berkeley, CA 94720 USA. EM RMTinnacher@lbl.gov RI Tournassat, Christophe/A-1353-2010; Davis, James/G-2788-2015; OI Tournassat, Christophe/0000-0003-2379-431X; Holmboe, Michael/0000-0003-3927-6197; Bourg, Ian/0000-0002-5265-7229 FU U.S. Department of Energy under the Used Fuel Disposition program (Office of Nuclear Energy) [DE-AC02-05CH11231]; U.S. Department of Energy under the Geosciences program (Office of Science, Office of Basic Energy Sciences) [DE-AC02-05CH11231]; French Geologic Survey (BRGM) through the Institut Carnot BRGM; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Carl Tryggers Foundation; Galo Foundation; foundation BLANCEFLOR FX This research was supported by the U.S. Department of Energy under Contract DE-AC02-05CH11231 under the auspices of the Used Fuel Disposition program (Office of Nuclear Energy) and the Geosciences program (Office of Science, Office of Basic Energy Sciences) as well as by the French Geologic Survey (BRGM) through the Institut Carnot BRGM. It used resources of the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy under Contract DE-AC02-05CH11231. Financial support to M.H. by the Carl Tryggers Foundation, the Galo Foundation, and the foundation BLANCEFLOR is gratefully acknowledged. The authors would like to thank Prof. Jonsson and co-workers at the Applied Physical Chemistry, KTH, Sweden, for providing the diffusion cells used in this study. NR 107 TC 3 Z9 3 U1 19 U2 53 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD MAR 15 PY 2016 VL 177 BP 130 EP 149 DI 10.1016/j.gca.2015.12.010 PG 20 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DE9PH UT WOS:000370969700009 ER PT J AU Collins, RN Rosso, KM Rose, AL Glover, CJ Waite, TD AF Collins, Richard N. Rosso, Kevin M. Rose, Andrew L. Glover, Chris J. Waite, T. David TI An in situ XAS study of ferric iron hydrolysis and precipitation in the presence of perchlorate, nitrate, chloride and sulfate SO GEOCHIMICA ET COSMOCHIMICA ACTA LA English DT Article ID RAY-ABSORPTION-SPECTROSCOPY; REVISED STRUCTURAL MODEL; PAIR DISTRIBUTION FUNCTION; DENSITY-FUNCTIONAL THEORY; ACID-MINE DRAINAGE; FE K-EDGE; AQUEOUS-SOLUTIONS; 2-LINE FERRIHYDRITE; MU-OXO; FE(II)-CATALYZED TRANSFORMATION AB Using a novel combination of in situ potentiometric experiments and quick-scanning XAS we present Fe K-edge XAS spectra (to k = 12 angstrom(-1)) during Fe-III hydrolysis and precipitation in 0.33M Fe(ClO4)(3), Fe(NO3)(3), FeCl3 and Fe-2(SO4)(3) solutions up to pH 4.8. Edge-sharing Fe-III polymers appeared almost immediately upon hydrolysis with strong evidence for a mu-oxo dimer species forming in the Fe(ClO4)(3), Fe(NO3)(3) and FeCl3 solutions. The effects of SO4 on hydrolysis and polymerization pathways included inhibition of both the formation of the mu-oxo dimer and double corner Fe-III bonding, ultimately resulting in the precipitation of schwertmannite. As such, under these experimental conditions, double corner Fe-III bonding appears to be critical to the formation of ferrihydrite. The spectral trends indicated that the decomposition/transformation of the dimer was sudden and broadly coincident with shortening average Fe-O bond distances, increased Fe neighbors at similar to 3.43 angstrom and a pre-edge energy transformation suggestive of decreased ligand field strength as well as increasing proportions of tetrahedral Fe-III. This result suggests that the incorporation of tetrahedral Fe-III into ferrihydrite occurs only at the latter stages of extended polymerization. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Collins, Richard N.; Waite, T. David] UNSW Australia, Sch Civil & Environm Engn, UNSW Water Res Ctr, Sydney, NSW 2052, Australia. [Rosso, Kevin M.] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99336 USA. [Rose, Andrew L.] So Cross Univ, So Cross Geosci, POB 157, Lismore, NSW 2480, Australia. [Glover, Chris J.] Australian Synchrotron Co Ltd, Xray Absorpt Spect Beamline, 800 Blackburn Rd, Clayton, Vic 3168, Australia. RP Collins, RN (reprint author), UNSW Australia, Sch Civil & Environm Engn, UNSW Water Res Ctr, Sydney, NSW 2052, Australia. EM richard.collins@unsw.edu.au FU Australian Research Council Future Fellowship [FT110100067]; Australian-American Fulbright Commission; U.S. Department of Energy's (DOE) Office of Basic Energy Sciences, Chemical Sciences, Geosciences, AMP; Biosciences (CSGB) Division through the Geosciences program at Pacific Northwest National Laboratory (PNNL); Australian Research Council QEII Fellowship [DP0987351]; Australian Research Council [DP120103234]; U.S. DOE Office of Biological and Environmental Research FX Richard Collins is a recipient of an Australian Research Council Future Fellowship (FT110100067) and also acknowledges the support of the Australian-American Fulbright Commission for a Senior Scholarship in Nuclear Science and Technology to work at Pacific Northwest National Laboratory. Kevin Rosso gratefully acknowledges the U.S. Department of Energy's (DOE) Office of Basic Energy Sciences, Chemical Sciences, Geosciences, & Biosciences (CSGB) Division for support through the Geosciences program at Pacific Northwest National Laboratory (PNNL). Andrew Rose is a recipient of an Australian Research Council QEII Fellowship (DP0987351). Funding support was also provided by the Australian Research Council project DP120103234. The DFT calculations were performed using either EMSL, a national scientific user facility sponsored by the U.S. DOE Office of Biological and Environmental Research and located at PNNL or the Leonardi Engineering Research Computing Cluster, UNSW Australia. NR 96 TC 1 Z9 1 U1 21 U2 50 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0016-7037 EI 1872-9533 J9 GEOCHIM COSMOCHIM AC JI Geochim. Cosmochim. Acta PD MAR 15 PY 2016 VL 177 BP 150 EP 169 DI 10.1016/j.gca.2016.01.021 PG 20 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DE9PH UT WOS:000370969700010 ER PT J AU Maurya, A Kulkarni, R Thamizhavel, A Paudyal, D Dhar, SK AF Maurya, Arvind Kulkarni, Ruta Thamizhavel, Arumugam Paudyal, Durga Dhar, Sudesh Kumar TI Kondo Lattice and Antiferromagnetic Behavior in Quaternary CeTAl4Si2 (T = Rh, Ir) Single Crystals SO JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN LA English DT Article ID ELECTRONIC-STRUCTURE; MAGNETIC-STRUCTURE; EUTAL4SI2 T; RARE-EARTH; INTERMETALLICS; CEAL2; ALUMINUM; SYSTEMS; METALS; HEAT AB We have explored in detail the anisotropic magnetic properties of CeRhAl4Si2 and CeIrAl4Si2, which undergo two antiferromagnetic transitions, at TN1 = 12.6 and 15.5 K, followed by a second transition at TN2 = 9.4 and 13.8 K, respectively, with the [001]-axis as the relatively easy axis of magnetization. The electrical resistivity at ambient and applied pressure provides evidence of Kondo interaction in both compounds, further supported by a reduced value of the entropy associated with the magnetic ordering. The Sommerfeld coefficient gamma is inferred to be 195.6 and 49.4 mJ/(molK(2)) for CeRhAl4Si2 and CeIrAl4Si2, respectively, classifying these materials as moderate heavy-fermion compounds. The crystal electric field energy levels are derived from the peak seen in the Schottky heat capacity. Furthermore, we have also performed electronic structure calculations by using the local spin density approximation + U [LSDA+U] approach, which provide physical insights on the observed magnetic behavior of these two compounds. C1 [Maurya, Arvind; Kulkarni, Ruta; Thamizhavel, Arumugam; Dhar, Sudesh Kumar] Tata Inst Fundamental Res, Dept Condensed Matter Phys & Mat Sci, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Paudyal, Durga] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. RP Dhar, SK (reprint author), Tata Inst Fundamental Res, Dept Condensed Matter Phys & Mat Sci, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. EM sudesh@tifr.res.in FU U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering; U.S. Department of Energy [DE-AC02-07CH11358] FX The electronic structure part of the work was supported by the U.S. Department of Energy, Office of Basic Energy Science, Division of Materials Sciences and Engineering. The Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. NR 27 TC 5 Z9 5 U1 8 U2 13 PU PHYSICAL SOC JAPAN PI TOKYO PA YUSHIMA URBAN BUILDING 5F, 2-31-22 YUSHIMA, BUNKYO-KU, TOKYO, 113-0034, JAPAN SN 0031-9015 J9 J PHYS SOC JPN JI J. Phys. Soc. Jpn. PD MAR 15 PY 2016 VL 85 IS 3 AR 034720 DI 10.7566/JPSJ.85.034720 PG 12 WC Physics, Multidisciplinary SC Physics GA DF1HS UT WOS:000371091100028 ER PT J AU Motoya, K Hagihala, M Takabatake, T Matsuda, M AF Motoya, Kiyoichiro Hagihala, Masato Takabatake, Toshiro Matsuda, Masaaki TI Long-Time Variation in Magnetic Structure of CeIr3Si2: Observation of a Nucleation-and-Growth Process of Magnetic Domains SO JOURNAL OF THE PHYSICAL SOCIETY OF JAPAN LA English DT Article ID PHASE-TRANSITION; KINETICS; CRYSTAL AB CeIr3Si2 is the first three-dimensional uniform magnet in which the long-time variation in magnetic structure was observed. To clarify the microscopic mechanism of this magnetic structural change, time-resolved neutron scattering measurements have been reinvestigated. Clear time variations in the line widths as well as the amplitudes of magnetic Bragg diffractions have been observed in this improved instrumentation. On the basis of this observation, a nucleation-and-growth model of magnetic structural change has been presented. The numerical calculation with this model reproduces well the observation. C1 [Motoya, Kiyoichiro; Hagihala, Masato] Tokyo Univ Sci, Fac Sci & Technol, Dept Phys, Noda, Chiba 2788510, Japan. [Takabatake, Toshiro] Hiroshima Univ, Dept Quantum Matter, ADSM, Higashihiroshima, Hiroshima 7398530, Japan. [Matsuda, Masaaki] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Hagihala, Masato] Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan. RP Motoya, K (reprint author), Tokyo Univ Sci, Fac Sci & Technol, Dept Phys, Noda, Chiba 2788510, Japan. EM motoya@ph.noda.tus.ac.jp RI Matsuda, Masaaki/A-6902-2016; Takabatake, Toshiro/L-2882-2014 OI Matsuda, Masaaki/0000-0003-2209-9526; Takabatake, Toshiro/0000-0002-3293-8592 FU US-Japan Cooperative Program on Neutron Scattering; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; Ministry of Education, Culture, Sports, Science and Technology [24540351] FX The neutron scattering experiment at Oak Ridge National Laboratory was supported by the US-Japan Cooperative Program on Neutron Scattering. Research conducted at ORNL's High Flux Isotope Reactor was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. This work was partly supported by a Grant-in-Aid for Scientific Research from the Ministry of Education, Culture, Sports, Science and Technology (No. 24540351). NR 12 TC 1 Z9 1 U1 0 U2 6 PU PHYSICAL SOC JAPAN PI TOKYO PA YUSHIMA URBAN BUILDING 5F, 2-31-22 YUSHIMA, BUNKYO-KU, TOKYO, 113-0034, JAPAN SN 0031-9015 J9 J PHYS SOC JPN JI J. Phys. Soc. Jpn. PD MAR 15 PY 2016 VL 85 IS 3 AR 034722 DI 10.7566/JPSJ.85.034722 PG 8 WC Physics, Multidisciplinary SC Physics GA DF1HS UT WOS:000371091100030 ER PT J AU Barker, BJ Berg, JM Kozimor, SA Wozniak, NR Wilkerson, MP AF Barker, Beau J. Berg, John M. Kozimor, Stosh A. Wozniak, Nicholas R. Wilkerson, Marianne P. TI Visible and near-infrared excitation spectra from the neptunyl ion doped into a uranyl tetrachloride lattice SO JOURNAL OF MOLECULAR STRUCTURE LA English DT Article DE Actinide; Electronic structure; Excitation spectrum; Intra-5f; Ligand-to-metal charge-transfer; Neptunyl ID ELECTRONIC-STRUCTURE; ACTINYL IONS; INTRA-5F FLUORESCENCE; TRANSITIONS; CS2UO2CL4; CS2U(NP)O2CL4; TEMPERATURE; COMPLEXES; NP(VI) AB Visible and near-infrared illumination induces 5f-5f and ligand-to-metal charge-transfer (LMCT) transitions of the neptunyl tetrachloride anion in polycrystalline Cs2U(Np)O2Cl4, and results in near-infrared luminescence from the second electronically excited state to the ground state. This photoluminescence is used as a detection method to collect excitation spectra throughout the near-infrared and visible regions. The excitation spectra of LMCT transitions in excitation spectra were identified in previous work. Here the measurement and analysis is extended to include both LMCT and intra-5f transitions. The results manifest variation in structural properties of the neptunium-oxo bond among the low-lying electronic states. Vibronic intensity patterns and energy spacings are used to compare bond lengths and vibrational frequencies in the excited states, confirming significant characteristic differences between those excited by 5f-5f transitions from those due to LMCT transitions. Results are compared with recently published RASPT2/SO calculations of [NpO2Cl4](2-). (C) 2015 Elsevier B.V. All rights reserved. C1 [Barker, Beau J.; Berg, John M.; Kozimor, Stosh A.; Wozniak, Nicholas R.; Wilkerson, Marianne P.] Los Alamos Natl Lab, POB 1663,Mail Stop J514, Los Alamos, NM 87545 USA. RP Wilkerson, MP (reprint author), Los Alamos Natl Lab, POB 1663,Mail Stop J514, Los Alamos, NM 87545 USA. EM mpw@lanl.gov RI Barker, Beau/S-5494-2016; OI Barker, Beau/0000-0001-6680-6814; Berg, John/0000-0002-6533-3573; Wilkerson, Marianne/0000-0001-8540-0465 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Science; U.S. Department of Energy's National Nuclear Security Administration (NNSA) [DE-AC52-06NA25396]; LANL LDRD program office FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Science. Los Alamos National Laboratory is managed and operated by Los Alamos National Security, LLC (LANS), under contract number DE-AC52-06NA25396 for the U.S. Department of Energy's National Nuclear Security Administration (NNSA). B. J. B. gratefully acknowledges a LANL Seaborg Institute Fellowship. N. R. W. gratefully acknowledges support from the LANL LDRD program office. NR 27 TC 1 Z9 1 U1 2 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0022-2860 EI 1872-8014 J9 J MOL STRUCT JI J. Mol. Struct. PD MAR 15 PY 2016 VL 1108 BP 594 EP 601 DI 10.1016/j.molstruc.2015.12.027 PG 8 WC Chemistry, Physical SC Chemistry GA DD7EQ UT WOS:000370086900065 ER PT J AU Cahill, JF Kertesz, V Van Berkel, GJ AF Cahill, John F. Kertesz, Vilmos Van Berkel, Gary J. TI Laser dissection sampling modes for direct mass spectral analysis SO RAPID COMMUNICATIONS IN MASS SPECTROMETRY LA English DT Article ID VORTEX CAPTURE/ELECTROSPRAY IONIZATION; CAPTURE MICRODISSECTION; ELECTROSPRAY-IONIZATION; CHLAMYDOMONAS-REINHARDTII; SPECTROMETRY; ABLATION; CELLS; TISSUES; LIPIDS; BRAIN AB RationaleLaser microdissection coupled directly with mass spectrometry provides the capability of on-line analysis of substrates with high spatial resolution, high collection efficiency, and freedom on shape and size of the sampling area. Establishing the merits and capabilities of the different sampling modes that the system provides is necessary in order to select the best sampling mode for characterizing analytically challenging samples. MethodsThe capabilities of laser ablation spot sampling, laser ablation raster sampling, and laser 'cut and drop' sampling modes of a hybrid optical microscopy/laser ablation liquid vortex capture electrospray ionization mass spectrometry system were compared for the analysis of single cells and tissue. ResultsSingle Chlamydomonas reinhardtii cells were monitored for their monogalactosyldiacylglycerol (MGDG) and diacylglyceryltrimethylhomo-Ser (DGTS) lipid content using the laser spot sampling mode, which was capable of ablating individual cells (4-15 m) even when agglomerated together. Turbid Allium Cepa cells (150 m) having unique shapes difficult to precisely measure using the other sampling modes could be ablated in their entirety using laser raster sampling. Intact microdissections of specific regions of a cocaine-dosed mouse brain tissue were compared using laser 'cut and drop' sampling. Since in laser 'cut and drop' sampling whole and otherwise unmodified sections are captured into the probe, 100% collection efficiencies were achieved. Laser ablation spot sampling has the highest spatial resolution of any sampling mode, while laser ablation raster sampling has the highest sampling area adaptability of the sampling modes. ConclusionsLaser ablation spot sampling has the highest spatial resolution of any sampling mode, useful in this case for the analysis of single cells. Laser ablation raster sampling was best for sampling regions with unique shapes that are difficult to measure using other sampling modes. Laser 'cut and drop' sampling can be used for cases where the highest sensitivity is needed, for example, monitoring drugs present in trace amounts in tissue. Published in 2016. This article is a U.S. Government work and is in the public domain in the USA. C1 [Cahill, John F.; Kertesz, Vilmos; Van Berkel, Gary J.] Oak Ridge Natl Lab, Div Chem Sci, Mass Spectrometry & Laser Spect Grp, Oak Ridge, TN 37831 USA. RP Van Berkel, GJ (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Mass Spectrometry & Laser Spect Grp, Oak Ridge, TN 37831 USA. EM vanberkelgj@ornl.gov RI Kertesz, Vilmos/M-8357-2016; OI Kertesz, Vilmos/0000-0003-0186-5797; Cahill, John/0000-0002-9866-4010 FU SCIEX [CRADA NFE-10-02966]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; U.S. Department of Energy [DE-AC05-00OR22725] FX Amina S. Woods, Shelley Jackson, and Aurelie Roux (National Institute of Drug Abuse-Intramural Research Program, National Institutes of Health) are thanked for supplying the mouse brain tissue. The TripleTOF (R) 5600+ mass spectrometer used in this work was provided on loan and the brain tissue studies funded by SCIEX through a Cooperative Research and Development Agreement (CRADA NFE-10-02966). Julian Burke (Leica Microsystems) is thanked for the loan of the LMD7000 instrument. The fundamental instrumental advancement and algae and plant studies were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. This manuscript has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 40 TC 1 Z9 1 U1 5 U2 14 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0951-4198 EI 1097-0231 J9 RAPID COMMUN MASS SP JI Rapid Commun. Mass Spectrom. PD MAR 15 PY 2016 VL 30 IS 5 BP 611 EP 619 DI 10.1002/rcm.7477 PG 9 WC Biochemical Research Methods; Chemistry, Analytical; Spectroscopy SC Biochemistry & Molecular Biology; Chemistry; Spectroscopy GA DD5WU UT WOS:000369996300007 PM 26842582 ER PT J AU Kholod, N Evans, M Gusev, E Yu, S Malyshev, V Tretyakova, S Barinov, A AF Kholod, N. Evans, M. Gusev, E. Yu, S. Malyshev, V. Tretyakova, S. Barinov, A. TI A methodology for calculating transport emissions in cities with limited traffic data: Case study of diesel particulates and black carbon emissions in Murmansk SO SCIENCE OF THE TOTAL ENVIRONMENT LA English DT Article DE Emission inventory; Transport; Diesel; Russia; Black carbon ID ROAD TRANSPORT; STRATEGIES; CHINA AB This paper presents a methodology for calculating exhaust emissions from on-road transport in cities with low-quality traffic data and outdated vehicle registries. The methodology consists of data collection approaches and emission calculation methods. For data collection, the paper suggests using video survey and parking lot survey methods developed for the International Vehicular Emissions model. Additional sources of information include data from the largest transportation companies, vehicle inspection stations, and official vehicle registries. The paper suggests using the European Computer Programme to Calculate Emissions from Road Transport (COPERT) 4 model to calculate emissions, especially in countries that implemented European emissions standards. If available, the local emission factors should be used instead of the default COPERT emission factors. The paper also suggests additional steps in the methodology to calculate emissions only from diesel vehicles. We applied this methodology to calculate black carbon emissions from diesel on-road vehicles in Murmansk, Russia. The results from Murmansk show that diesel vehicles emitted 11.7 tons of black carbon in 2014. The main factors determining the level of emissions are the structure of the vehicle fleet and the level of vehicle emission controls. Vehicles without controls emit about 55% of black carbon emissions. (C) 2015 Elsevier B.V. All rights reserved. C1 [Kholod, N.; Evans, M.; Yu, S.] Pacific NW Natl Lab, Joint Global Change Res Inst, 5825 Univ Res Court,Suite 3500, College Pk, MD 20740 USA. [Gusev, E.; Malyshev, V.; Barinov, A.] Murmansk State Tech Univ, Dept Energy & Transport, Murmansk, Russia. [Tretyakova, S.] Murmansk State Tech Univ, Dept Environm, Murmansk, Russia. RP Kholod, N (reprint author), Pacific NW Natl Lab, Joint Global Change Res Inst, 5825 Univ Res Court,Suite 3500, College Pk, MD 20740 USA. EM nazar.kholod@pnnl.gov OI Kholod, Nazar/0000-0002-4716-8770; Malyshev, Vladimir/0000-0002-1178-1776 FU U.S. Environmental Protection Agency, Office of International and Tribal Affairs [X4-83527901] FX The authors are grateful for the research support provided by the U.S. Environmental Protection Agency, Office of International and Tribal Affairs (grant No. X4-83527901). We appreciate the valuable advice and comments from Vadim Donchenko and Yuliy Kunin from the Russian Scientific Research Institute for Automobile Transport (NIIAT) and James Lents from the International Sustainable Systems Research Center. The views and opinions expressed in this paper are those of the authors alone. NR 36 TC 0 Z9 1 U1 5 U2 27 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0048-9697 EI 1879-1026 J9 SCI TOTAL ENVIRON JI Sci. Total Environ. PD MAR 15 PY 2016 VL 547 BP 305 EP 313 DI 10.1016/j.scitotenv.2015.12.151 PG 9 WC Environmental Sciences SC Environmental Sciences & Ecology GA DD0ST UT WOS:000369630600033 PM 26789368 ER PT J AU Polishook, D Moskovitz, N Binzel, RP Burt, B DeMeo, FE Hinkle, ML Lockhart, M Mommert, M Person, M Thirouin, A Thomas, CA Trilling, D Willman, M Aharonson, O AF Polishook, D. Moskovitz, N. Binzel, R. P. Burt, B. DeMeo, F. E. Hinkle, M. L. Lockhart, M. Mommert, M. Person, M. Thirouin, A. Thomas, C. A. Trilling, D. Willman, M. Aharonson, O. TI A 2 km-size asteroid challenging the rubble-pile spin barrier - A case for cohesion SO ICARUS LA English DT Article DE Asteroids; Asteroids, rotation; Rotational dynamics; Photometry ID NEAR-EARTH ASTEROIDS; MAIN BELT ASTEROIDS; 29075 1950 DA; PHYSICAL-PROPERTIES; ROTATIONAL BREAKUP; BINARY ASTEROIDS; P/2013 R3; DISRUPTION; ORIGIN; REGOLITH AB The rubble pile spin barrier is an upper limit on the rotation rate of asteroids larger than similar to 200-300 m. Among thousands of asteroids with diameters larger than similar to 300 m, only a handful of asteroids are known to rotate faster than 2.0 h, all are in the sub-km range (<= 0.6 km). Here we present photometric measurements suggesting that (60716) 2000 GD65, an S-complex, inner-main belt asteroid with a relatively large diameter of 2.3(-0.7)(+0.6) km, completes one rotation in 1.9529 +/- 0.0002 h. Its unique diameter and rotation period allow us to examine scenarios about asteroid internal structure and evolution: a rubble pile bound only by gravity; a rubble-pile with strong cohesion; a monolithic structure; an asteroid experiencing mass shedding; an asteroid experiencing YORP spin-up/down; and an asteroid with a unique octahedron shape results with a four-peak lightcurve and a 3.9 h period. We find that the most likely scenario includes a lunar-like cohesion that can prevent (60716) 2000 GD65 from disrupting without requiring a monolithic structure or a unique shape. Due to the uniqueness of (60716)2000 GD65, we suggest that most asteroids typically have smaller cohesion than that of lunar regolith. (C) 2015 Elsevier Inc. All rights reserved. C1 [Polishook, D.; Aharonson, O.] Weizmann Inst Sci, Dept Earth & Planetary Sci, IL-7610001 Rehovot, Israel. [Moskovitz, N.; Hinkle, M. L.; Thirouin, A.] Lowell Observ, 1400 West Mars Hill Rd, Flagstaff, AZ 86001 USA. [Binzel, R. P.; Burt, B.; DeMeo, F. E.; Person, M.] MIT, Dept Earth Atmospher & Planetary Sci, Cambridge, MA 02139 USA. [Lockhart, M.] POB 391274, Cambridge, MA 02139 USA. [Mommert, M.; Trilling, D.] No Arizona Univ, Dept Phys & Astron, POB 6010, Flagstaff, AZ 86011 USA. [Thomas, C. A.] NASA, Goddard Space Flight Ctr, 8800 Greenbelt Rd, Greenbelt, MD 20771 USA. [Thomas, C. A.] Oak Ridge Associated Univ, NASA Postdoctoral Program, POB 117,MS 36, Oak Ridge, TN 37831 USA. [Thomas, C. A.] Planetary Sci Inst, 1700 East Ft Lowell,Suite 106, Tucson, AZ 85719 USA. [Trilling, D.] S African Astron Observ, Cape Town, South Africa. [Trilling, D.] Univ Western Cape, ZA-7535 Bellville, South Africa. [Willman, M.] Univ Hawaii, Inst Astrophys, Honolulu, HI 96822 USA. RP Polishook, D (reprint author), Weizmann Inst Sci, Dept Earth & Planetary Sci, IL-7610001 Rehovot, Israel. FU Ministry of Science, Technology and Space of the Israeli government; AXA Research Fund; NASA [NNX12AL26G]; NASA; Helen Kimmel Center for Planetary Science; ISF I-CORE program "Origins: From the Big Bang to Planets"; NASA NEOO Grant [NNX14AN82G] FX We are grateful to the referees for their thorough reports that improve the manuscript. We thank William Bottke and Dave O'Brien for their insights and fruitful discussion. DP is grateful to the Ministry of Science, Technology and Space of the Israeli government for their Ramon fellowship for post-docs, and the AXA Research Fund for their generous post-doc fellowship, during the years of observations and analysis. FED acknowledges funding from NASA under Grant No. NNX12AL26G. CAT was supported by an appointment to the NASA Postdoctoral Program at Goddard Space Flight Center, administrated by Oak Ridge Associated Universities through a contract with NASA. OA would like to acknowledge support from the Helen Kimmel Center for Planetary Science and the ISF I-CORE program "Origins: From the Big Bang to Planets".; We acknowledge support from NASA NEOO Grant No. NNX14AN82G, awarded to the Mission Accessible Near-Earth Object Survey (MANOS). We are thankful to the Wise Observatory staff for their continuous help and generous time allocation. Observations for this study were performed in Arizona, Chile, Hawaii and Israel. The people of all nations that support hosting professional observatories are praised for understanding and supporting the importance of astronomical studies. NR 79 TC 2 Z9 2 U1 0 U2 3 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0019-1035 EI 1090-2643 J9 ICARUS JI Icarus PD MAR 15 PY 2016 VL 267 BP 243 EP 254 DI 10.1016/j.icarus.2015.12.031 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DC3NJ UT WOS:000369125700017 ER PT J AU Thuresson, A Segad, M Turesson, M Skepo, M AF Thuresson, A. Segad, M. Turesson, M. Skepo, M. TI Flocculated Laponite-PEG/PEO dispersions with monovalent salt, a SAXS and simulation study SO JOURNAL OF COLLOID AND INTERFACE SCIENCE LA English DT Article DE Laponite; Polyethylene glycol; Polyethylene oxide; Polymer bridging; Laponite-PEG composites; Laponite-PEO composites; Coarse-grained simulation; Molecular dynamics; Electrostatic interactions; Salt effects; Platelet polymer interaction; Tactoid; Bragg peak; Total structure factor; Aggregate ID X-RAY-SCATTERING; ANGLE NEUTRON-SCATTERING; POLY(ETHYLENE OXIDE); CLAY SUSPENSIONS; SWELLING PROPERTIES; NA-MONTMORILLONITE; TACTOID FORMATION; COLLOIDAL DISKS; PARTICLE-SIZE; NANOCOMPOSITES AB It is well-known that clay can form lamellar structures i.e. tactoids, and recently it has been shown that the tactoid formation is dependent on the platelet diameter. To the authors knowledge, no tactoid formation has been observed for montmorillonite platelets with a diameter less than 60 nm. In this study, small angle X-ray scattering in combination with coarse-grained modeling and molecular dynamics simulations have been utilized to study the sediment of Laponite-polyethylene glycol/polyethylene oxide (PEG/PEO) at elevated salt concentrations (150 mM-1 M). Laponite consists of platelets with a diameter of 25 nm and it is known to have a relatively monodisperse size-distribution. At pH 10, the face of the platelets has a strong negative charge, whereas the rim is slightly positive. Here we show that it is possible to induce tactoids for Laponite if two constraints are fulfilled: (1) addition of high amount of salt such as NaCl, and (2) addition of a neutral polymer such as PEG. The role of the salt is to screen the repulsive interactions between the platelets and the role of the polymer is to bridge the platelets together: hence the loss in configurational entropy of the polymer is counteracted by the gain in attractive polymer-platelet interaction. As the concentration of NaCl and/or PEG increases, the Bragg peak becomes sharper, which is an indication of that larger tactoids are formed. Comparison between Laponite and montmorillonite shows that the interlayer distance between the platelets increases linearly with an increased Debye screening length for both type of clays, whereas the structure peaks of Laponite are broader compared to the montmorillonite. We argue that the main reason to the latter is due to the size of the platelets: (i) smaller platelets are less rotationally restricted and (ii) the effect of positive edge charges is larger when the platelets are smaller, which results in more irregular aggregates. In absence of the polymer, montmorillonite form tactoids above similar to 0.3 M NaCl whereas Laponite does not. Even though the model used is simple, we find qualitative agreement between experiments and simulations, which verifies that the underlying physics for tactoid formation is captured. (C) 2015 Elsevier Inc. All rights reserved. C1 [Thuresson, A.; Turesson, M.; Skepo, M.] Lund Univ, Theoret Chem, POB 124, SE-22100 Lund, Sweden. [Segad, M.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Thuresson, A (reprint author), Lund Univ, Theoret Chem, POB 124, SE-22100 Lund, Sweden. EM axel.thuresson@teokem.lu.se NR 53 TC 0 Z9 0 U1 11 U2 38 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9797 EI 1095-7103 J9 J COLLOID INTERF SCI JI J. Colloid Interface Sci. PD MAR 15 PY 2016 VL 466 BP 330 EP 342 DI 10.1016/j.jcis.2015.12.033 PG 13 WC Chemistry, Physical SC Chemistry GA DC3KV UT WOS:000369119100038 PM 26748065 ER PT J AU Kaminski, MD Lee, SD Magnuson, M AF Kaminski, Michael D. Lee, Sang Don Magnuson, Matthew TI Wide-area decontamination in an urban environment after radiological dispersion: A review and perspectives SO JOURNAL OF HAZARDOUS MATERIALS LA English DT Review DE Decontamination; Remediation; Radionuclide dispersal device; Nuclear fallout; Radioactive contamination ID COATINGS; SURFACES; SORPTION AB Nuclear or radiological terrorism in the form of uncontrolled radioactive contamination presents a unique challenge in the field of nuclear decontamination. Potential targets require an immediate decontamination response, or mitigation plan to limit the social and economic impact. To date, experience with urban decontamination of building materials - specifically hard, porous, external surfaces - is limited to nuclear weapon fallout and nuclear reactor accidents. Methods are lacking for performing wide-area decontamination in an urban environment so that in all release scenarios the area may be re -occupied without evaluation and/or restriction. Also lacking is experience in developing mitigation strategies, that is, methods of mitigating contamination and its resultant radiation dose in key areas during the immediate aftermath of an event and after lifesaving operations. To date, the tremendous strategy development effort primarily by the European community has focused on the recovery phase, which extends years beyond the release event. In this review, we summarize the methods and data collected over the past 70 years in the field of hard, external surface decontamination of radionuclide contaminations, with emphasis on methods suitable for response to radiological dispersal devices and their potentially unique physico-chemical characteristics. This review concludes that although a tremendous amount of work has been completed primarily by the European Community (EU) and the United Kingdom (UK), the few studies existing on each technique permit only very preliminary estimates of decontamination factors for various building materials and methods and extrapolation of those values for use in environments outside the EU and UK. This data shortage prevents us from developing an effective and detailed mitigation response plan and remediation effort. Perhaps most importantly, while the data available does include valuable information on the practical aspects of performing the various remediation methods including costs, coverage rates, manpower, pitfalls, etc., it lacks the details on lessons learned, best practices, and standard procedures, for instance, that would be required to develop a mitigation strategy. While the urban decontamination problem is difficult and there is much more research to do, the existing literature provides a framework for a response plan. Using this framework, in conjunction with computer modeling and relevant data collection, can lead to development of appropriate plans and exercises that would permit development of a mitigation and remediation response. (C) 2015 Elsevier B.V. All rights reserved. C1 [Kaminski, Michael D.] Argonne Natl Lab, Nucl Engn Div, Nucl Decontaminat & Separat, Argonne, IL 60439 USA. [Lee, Sang Don; Magnuson, Matthew] US EPA, Off Res & Dev, Natl Homeland Secur Res Ctr, Washington, DC USA. RP Kaminski, MD (reprint author), Argonne Natl Lab, Nucl Engn Div, Nucl Decontaminat & Separat, Argonne, IL 60439 USA. EM Kaminski@anl.gov FU United States Department of Homeland Security/Science and Technology Directorate; U.S. Environmental Protection Agency/National Homeland Security Research Center; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX The authors thank J. Harmon and J. T. Bursey for editing the document. This work was supported by the United States Department of Homeland Security/Science and Technology Directorate in collaboration with the U.S. Environmental Protection Agency/National Homeland Security Research Center through an interagency agreement. It has been subject to an administrative review but does not necessarily reflect the views of either Agency. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The U.S. Government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 100 TC 3 Z9 3 U1 3 U2 28 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3894 EI 1873-3336 J9 J HAZARD MATER JI J. Hazard. Mater. PD MAR 15 PY 2016 VL 305 BP 67 EP 86 DI 10.1016/j.jhazmat.2015.11.014 PG 20 WC Engineering, Environmental; Engineering, Civil; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DC8DZ UT WOS:000369451400009 PM 26642448 ER PT J AU Ang, C Silva, C Shih, CH Koyanagi, T Katoh, Y Zinkle, SJ AF Ang, Caen Silva, Chinthaka Shih, Chunghao Koyanagi, Takaaki Katoh, Yutai Zinkle, Steven J. TI Anisotropic swelling and microcracking of neutron irradiated Ti3AlC2-Ti5Al2C3 materials SO SCRIPTA MATERIALIA LA English DT Article DE Anisotropic swelling; Neutron irradiation; MAX phase; Microcracking; Lattice parameter ID MAX PHASES; BERYLLIUM OXIDE; TI3ALC2; DAMAGE; RESISTANCE; NITRIDE; CERAMICS; TI3SIC2; AL2O3; MGO AB M(n + 1)AX(n). (MAX) phase materials based on Ti-Al-C have been irradiated at 400 degrees C (673 K) with fission neutrons to a fluence of 2 x 10(25) n/m(2) (E > 0.1 MeV), corresponding to similar to 2 displacements per atom (dpa). We report preliminary results of microcracking in the Al-containing MAX phase, which contained the phases Ti3AlC2 and Ti5Al2C3. Equibiaxial ring-on-ring tests of irradiated coupons showed that samples retained 10% of pre-irradiated strength. Volumetric swelling of up to 4% was observed. Phase analysis and microscopy suggest that anisotropic lattice parameter swelling caused microcracking. Variants of titanium aluminum carbide may be unsuitable materials for irradiation at light water reactor-relevant temperatures. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Ang, Caen; Silva, Chinthaka; Shih, Chunghao; Koyanagi, Takaaki; Katoh, Yutai; Zinkle, Steven J.] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. [Zinkle, Steven J.] Univ Tennessee, Knoxville, TN USA. RP Ang, C (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. RI Koyanagi, Takaaki/D-9841-2017 OI Koyanagi, Takaaki/0000-0001-7272-4049 NR 31 TC 5 Z9 5 U1 6 U2 31 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD MAR 15 PY 2016 VL 114 BP 74 EP 78 DI 10.1016/j.scriptamat.2015.11.008 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DC8GC UT WOS:000369456900017 ER PT J AU Luo, LL Zou, LF Schreiber, DK Baer, DR Bruemmer, SM Zhou, GW Wang, CM AF Luo, Langli Zou, Lianfeng Schreiber, Daniel K. Baer, Donald R. Bruemmer, Stephen M. Zhou, Guangwen Wang, Chong-Min TI In-situ transmission electron microscopy study of surface oxidation for Ni-10Cr and Ni-20Cr alloys SO SCRIPTA MATERIALIA LA English DT Article DE Ni-Cr; Oxidation; Oxidation kinetics; Environmental TEM ID NICKEL CHROMIUM-ALLOYS; NI-CR ALLOYS; TRANSIENT OXIDATION; 304-STAINLESS-STEEL; MECHANISM AB The early-stage oxidation of Ni (001) thin films alloyed with 10 or 20 at.% Cr at 700 degrees C has been directly visualized using in-situ TEM. Independent of Cr concentration, the oxidation initiates via nucleation of surface NiO islands and subsurface Cr2O3. The NiO grows and transitions into a continuous film, followed by the nucleation and growth of NiCr2O4 islands. For Ni-20 at.% Cr, a continuous Cr2O3 was developed, but not for Ni-10 at.% Cr. NiO whiskers are observed to preferentially nucleate/grow from the NiCr2O4 islands through a short-circuit diffusion of Ni along the NiCr2O4 interfaces in Ni-10 at.% Cr. (C) 2015 Scripta Materialia. Published by ELSEVIER Ltd. All rights reserved. C1 [Luo, Langli; Baer, Donald R.; Wang, Chong-Min] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Zou, Lianfeng; Zhou, Guangwen] SUNY Binghamton, Dept Mech Engn, Binghamton, NY 13902 USA. [Zou, Lianfeng; Zhou, Guangwen] SUNY Binghamton, Multidisciplinary Program Mat Sci & Engn, Binghamton, NY 13902 USA. [Schreiber, Daniel K.; Bruemmer, Stephen M.] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99352 USA. RP Wang, CM (reprint author), Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA.; Zhou, GW (reprint author), SUNY Binghamton, Dept Mech Engn, Binghamton, NY 13902 USA.; Zhou, GW (reprint author), SUNY Binghamton, Multidisciplinary Program Mat Sci & Engn, Binghamton, NY 13902 USA. EM gzhou@binghamton.edu; chongmin.wang@pnnl.gov RI Luo, Langli/B-5239-2013; OI Luo, Langli/0000-0002-6311-051X FU U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; DOE [DE-AC06-76RLO 1830]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-SC0001135] FX This work was supported by the U.S. Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. The work was conducted in the William R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a DOE User Facility operated by Battelle for the DOE Office of Biological and Environmental Research. Pacific Northwest National Laboratory is operated for the DOE under Contract DE-AC06-76RLO 1830. Authors 12 and GZ acknowledge support from the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award No. DE-SC0001135. NR 23 TC 0 Z9 0 U1 10 U2 37 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD MAR 15 PY 2016 VL 114 BP 129 EP 132 DI 10.1016/j.scriptamat.2015.11.031 PG 4 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DC8GC UT WOS:000369456900029 ER PT J AU Aidhy, DS Lu, CY Jin, K Bei, HB Zhang, YW Wang, LM Weber, WJ AF Aidhy, Dilpuneet S. Lu, Chenyang Jin, Ke Bei, Hongbin Zhang, Yanwen Wang, Lumin Weber, William J. TI Formation and growth of stacking fault tetrahedra in Ni via vacancy aggregation mechanism SO SCRIPTA MATERIALIA LA English DT Article DE Molecular dynamics; Diffusion; Point defect; Stacking fault tetrahedra ID DIPOLE ANNIHILATION; QUENCHED GOLD; CU; DEFECTS; COPPER; CASCADES; AL AB Using molecular dynamics simulations, the formation and growth of stacking fault tetrahedra (SFT) are captured by vacancy cluster diffusion and aggregation mechanisms in Ni. The vacancy-tetrahedron acts as a nucleation point for SFT formation. Simulations show that perfect SFT can grow to the next size perfect SFT via a vacancy aggregation mechanism. The stopping and range of ions in matter (SRIM) calculations and transmission electron microscopy (TEM) observations reveal that SFT can form farther away from the initial cascade-event locations, indicating the operation of diffusion-based vacancy-aggregation mechanism. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Aidhy, Dilpuneet S.] Univ Wyoming, Dept Mech Engn, Laramie, WY 82071 USA. [Aidhy, Dilpuneet S.; Jin, Ke; Bei, Hongbin; Zhang, Yanwen; Weber, William J.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Lu, Chenyang; Wang, Lumin] Univ Michigan, Dept Nucl Engn & Radiol Sci, Ann Arbor, MI 48109 USA. [Weber, William J.] Univ Tennessee, Mat Sci & Engn, Knoxville, TN 37996 USA. RP Aidhy, DS (reprint author), Univ Wyoming, Dept Mech Engn, Laramie, WY 82071 USA.; Aidhy, DS (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. EM daidhy@uwyo.edu RI Weber, William/A-4177-2008; OI Weber, William/0000-0002-9017-7365; Bei, Hongbin/0000-0003-0283-7990 FU Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences; Office of Science, U.S. Department of Energy [DEAC02-05CH11231] FX This work was supported by Energy Dissipation to Defect Evolution (EDDE), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. The computer simulations were performed at the National Energy Research Scientific Computing Center at Lawrence Berkeley National Laboratory, which is supported by the Office of Science, U.S. Department of Energy under Contract No. DEAC02-05CH11231. NR 24 TC 3 Z9 3 U1 7 U2 20 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD MAR 15 PY 2016 VL 114 BP 137 EP 141 DI 10.1016/j.scriptamat.2015.12.020 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DC8GC UT WOS:000369456900031 ER PT J AU Miao, YB Mo, K Ye, B Jamison, L Mei, ZG Gan, J Miller, B Madden, J Park, JS Almer, J Bhattacharya, S Kim, YS Hofman, GL Yacout, AM AF Miao, Yinbin Mo, Kun Ye, Bei Jamison, Laura Mei, Zhi-Gang Gan, Jian Miller, Brandon Madden, James Park, Jun-Sang Almer, Jonathan Bhattacharya, Sumit Kim, Yeon Soo Hofman, Gerard L. Yacout, Abdellatif M. TI High-energy synchrotron study of in-pile-irradiated U-Mo fuels SO SCRIPTA MATERIALIA LA English DT Article DE X-ray diffraction; Synchrotron radiation; Superlattice; Recrystallization; Metallic nuclear fuel ID RAY-DIFFRACTION ANALYSIS; DISPERSION FUEL; STEEL; BEHAVIOR; NANOPARTICLES; TEMPERATURE; PERFORMANCE; ALUMINUM AB Here synchrotron scattering analysis results on U-7wt.%Mo fuel specimens irradiated in the Advanced Test Reactor to three burnup levels (3.0, 5.2, and 63 x 10(21) fission/cm(3)) are reported. Mature fission gas bubble superlattice was observed to form at intermediate burnup. The superlattice constant was determined to be 11.7 and 12.0 nm by wide-angle and small-angle scattering respectively. Grain sub-division takes place throughout the irradiation and causes the collapse of the superlattice at high burnup. The bubble superlattice expands the U-Mo lattice and acts as strong sink for radiation-induced defects. The evolution of dislocation loops was, therefore, suppressed until the bubble superlattice collapsed. (C) 2015 Published by Elsevier Ltd. C1 [Miao, Yinbin; Mo, Kun; Ye, Bei; Jamison, Laura; Mei, Zhi-Gang; Park, Jun-Sang; Almer, Jonathan; Kim, Yeon Soo; Hofman, Gerard L.; Yacout, Abdellatif M.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Gan, Jian; Miller, Brandon; Madden, James] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Bhattacharya, Sumit] Northwestern Univ, Evanston, IL 60208 USA. RP Miao, YB (reprint author), 9700 S Cass Ave, Argonne, IL 60439 USA. EM ymiao@anl.gov OI Jamison, Laura/0000-0003-2759-6310; Miao, Yinbin/0000-0002-3128-4275 FU U.S. Department of Energy, National Nuclear Safety Administration (NNSA), Office of Material Management and Minimization Reactor Conversion Program [NA-23]; UChicago Argonne, LLC [DE-AC-02-06CH11357]; U.S. Department of Energy [DE-AC-02-06CH11357] FX This research was sponsored by the U.S. Department of Energy, National Nuclear Safety Administration (NNSA), Office of Material Management and Minimization (NA-23) Reactor Conversion Program. This research used the resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory. Both programs are supported under Contract No. DE-AC-02-06CH11357 between UChicago Argonne, LLC and the U.S. Department of Energy. NR 32 TC 3 Z9 3 U1 6 U2 15 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD MAR 15 PY 2016 VL 114 BP 146 EP 150 DI 10.1016/j.scriptamat.2015.12.019 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DC8GC UT WOS:000369456900033 ER PT J AU Johansson, A Garzon, M Sethian, JA AF Johansson, A. Garzon, M. Sethian, J. A. TI A three-dimensional coupled Nitsche and level set method for electrohydrodynamic potential flows in moving domains SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Nitsche finite element method; Level set method; Potential flow; Electrostatic driven flows ID BOUNDARY INTEGRAL METHOD; FINITE-ELEMENT-METHOD; ELECTRIC-FIELD; CHARGED DROPS; PINCH-OFF; DISINTEGRATION; SIMULATION; PENALTY AB In this paper we present a new algorithm for computing three-dimensional electrohydrodynamic flow in moving domains which can undergo topological changes. We consider a non-viscous, irrotational, perfect conducting fluid and introduce a way to model the electrically charged flow with an embedded potential approach. To numerically solve the resulting system, we combine a level set method to track both the free boundary and the surface velocity potential with a Nitsche finite element method for solving the Laplace equations. This results in an algorithmic framework that does not require body-conforming meshes, works in three dimensions, and seamlessly tracks topological change. Assembling this coupled system requires care: while convergence and stability properties of Nitsche's methods have been well studied for static problems, they have rarely been considered for moving domains or for obtaining the gradients of the solution on the embedded boundary. We therefore investigate the performance of the symmetric and non-symmetric Nitsche formulations, as well as two different stabilization techniques. The global algorithm and in particular the coupling between the Nitsche solver and the level set method are also analyzed in detail. Finally we present numerical results for several time-dependent problems, each one designed to achieve a specific objective: (a) The oscillation of a perturbed sphere, which is used for convergence studies and the examination of the Nitsche methods; (b) The break-up of a two lobe droplet with axial symmetry, which tests the capability of the algorithm to go past flow singularities such as topological changes and preservation of an axi-symmetric flow, and compares results to previous axi-symmetric calculations; (c) The electrohydrodynamical deformation of a thin film and subsequent jet ejection, which will account for the presence of electrical forces in a non-axi-symmetric geometry. (C) 2016 Elsevier Inc. All rights reserved. C1 [Johansson, A.] Simula Res Lab, Ctr Biomed Comp, POB 134, N-1325 Lysaker, Norway. [Garzon, M.] Univ Oviedo, Dept Appl Math, Oviedo, Spain. [Sethian, J. A.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Dept Math, Berkeley, CA 94720 USA. RP Johansson, A (reprint author), Simula Res Lab, Ctr Biomed Comp, POB 134, N-1325 Lysaker, Norway. EM august@simula.no; maria.garzon.martin@gmail.com; sethian@math.berkeley.edu FU Applied Mathematical Science subprogram of the Office of Energy Research, U.S. Department of Energy [DE-AC02-05CH11231]; Research Council of Norway through Centres of Excellence [179578]; Spanish Ministry of Science and Innovation [MTM2013-43671-P]; Division of Mathematical Sciences of the U.S. National Science Foundation FX This work was supported in part by the Applied Mathematical Science subprogram of the Office of Energy Research, U.S. Department of Energy, under contract Number DE-AC02-05CH11231. The first author was also supported by the Research Council of Norway through a Centres of Excellence grant to the Center for Biomedical Computing at Simula Research Laboratory, Project Number 179578. The second author was also supported by the Spanish Ministry of Science and Innovation, Project Number MTM2013-43671-P. The third author was also supported by the Division of Mathematical Sciences of the U.S. National Science Foundation, and acknowledges the support as an Einstein Visiting Fellow of the Einstein Stiftung Berlin, Germany. NR 43 TC 1 Z9 1 U1 5 U2 14 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD MAR 15 PY 2016 VL 309 BP 88 EP 111 DI 10.1016/j.jcp.2015.12.026 PG 24 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DC2YU UT WOS:000369085900006 ER PT J AU Lichterman, MF Sun, K Hu, S Zhou, XH McDowell, MT Shaner, MR Richter, MH Crumlin, EJ Carim, AI Saadi, FH Brunschwig, BS Lewis, NS AF Lichterman, Michael F. Sun, Ke Hu, Shu Zhou, Xinghao McDowell, Matthew T. Shaner, Matthew R. Richter, Matthias H. Crumlin, Ethan J. Carim, Azhar I. Saadi, Fadl H. Brunschwig, Bruce S. Lewis, Nathan S. TI Protection of inorganic semiconductors for sustained, efficient photoelectrochemical water oxidation SO CATALYSIS TODAY LA English DT Review DE Artificial photosynthesis; Photoelectrochemistry; Corrosion; Catalysis ID HYDROGEN-EVOLUTION REACTION; ATOMIC LAYER DEPOSITION; N-SILICON ELECTRODES; OXYGEN-EVOLUTION; SOLAR-CELL; THIN-FILMS; AQUEOUS KOH; PHOTOANODES; SI; DRIVEN AB Small-band-gap (E-g < 2 eV) semiconductors must be stabilized for use in integrated devices that convert solar energy into the bonding energy of a reduced fuel, specifically H-2(g) or a reduced-carbon species such as CH3OH or CH4. To sustainably and scalably complete the fuel cycle, electrons must be liberated through the oxidation of water to O-2(g). Strongly acidic or strongly alkaline electrolytes are needed to enable efficient and intrinsically safe operation of a full solar-driven water-splitting system. However, under water-oxidation conditions, the small-band-gap semiconductors required for efficient cell operation are unstable, either dissolving or forming insulating surface oxides. We describe herein recent progress in the protection of semiconductor photoanodes under such operational conditions. We specifically describe the properties of two protective overlayers, TiO2/Ni and NiOx, both of which have demonstrated the ability to protect otherwise unstable semiconductors for > 100 h of continuous solar-driven water oxidation when in contact with a highly alkaline aqueous electrolyte (1.0 M KOH(aq)). The stabilization of various semiconductor photoanodes is reviewed in the context of the electronic characteristics and a mechanistic analysis of the TiO2 films, along with a discussion of the optical, catalytic, and electronic nature of NiOx films for stabilization of semiconductor photoanodes for water oxidation. (C) 2015 Elsevier B.V. All rights reserved. C1 [Lichterman, Michael F.; Sun, Ke; Hu, Shu; McDowell, Matthew T.; Shaner, Matthew R.; Carim, Azhar I.; Lewis, Nathan S.] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. [Lichterman, Michael F.; Sun, Ke; Hu, Shu; Zhou, Xinghao; McDowell, Matthew T.; Shaner, Matthew R.; Richter, Matthias H.; Saadi, Fadl H.; Lewis, Nathan S.] CALTECH, Joint Ctr Artificial Photosynth, Pasadena, CA 91125 USA. [Hu, Shu; Brunschwig, Bruce S.; Lewis, Nathan S.] CALTECH, Beckman Inst, Pasadena, CA 91125 USA. [Crumlin, Ethan J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Lewis, Nathan S.] CALTECH, Kavli Nanosci Inst, Pasadena, CA 91125 USA. RP Lewis, NS (reprint author), CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA. EM nslewis@caltech.edu RI Sun, Ke /L-4709-2013 OI Sun, Ke /0000-0001-8209-364X FU Office of Science of the U.S. Department of Energy (DOE) [DE-SC0004993]; Moore Foundation; Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; DOE Energy Innovation Hub FX This work was supported through the Office of Science of the U.S. Department of Energy (DOE) under award no. DE-SC0004993 to the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, as well as by the Moore Foundation. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract no. DE-AC02-05CH11231. The authors thank Van Seebass for assistance in the preparation of this manuscript. NR 82 TC 8 Z9 8 U1 42 U2 316 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD MAR 15 PY 2016 VL 262 BP 11 EP 23 DI 10.1016/j.cattod.2015.08.017 PG 13 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA CY1IP UT WOS:000366160200003 ER PT J AU Lopes, PP Strmcnik, D Jirkovsky, JS Connell, JG Stamenkovic, V Markovic, N AF Lopes, Pietro P. Strmcnik, Dusan Jirkovsky, Jakub S. Connell, Justin G. Stamenkovic, Vojislav Markovic, Nenad TI Double layer effects in electrocatalysis: The oxygen reduction reaction and ethanol oxidation reaction on Au(111), Pt(111) and Ir(111) in alkaline media containing Na and Li cations SO CATALYSIS TODAY LA English DT Article DE Electrocatalysis; Surface spectators; Non covalent interactions; Cation effect; Oxygen reduction; Ethanol ID SINGLE-CRYSTAL ELECTRODES; ELECTROOXIDATION REACTION; NONCOVALENT INTERACTIONS; SURFACE-STRUCTURE; CARBON-MONOXIDE; PLATINUM; ADSORPTION; INTERFACES; PROMOTION; CATALYSTS AB Oxygen reduction and ethanol oxidation reactions were studied on Au(1 11), Pt(1 1 1) and Ir(1 1 1) in alkaline solutions containing sodium and/or lithium cations. By keeping the same (1 1 1) surface orientation and exploring oxophilicity trends and non-covalent interactions between OHad and alkali metal cations (AMC(n+)), we were able to gain deep insights into the multiple roles that OHad plays in these important electrocatalytic reactions. Cyclic voltammetry experiments revealed that OHad formation initiates at distinct electrode potentials, governed by the oxophilicity of the specific metal surface, with further OHad adlayer stabilization by non-covalent alkali-cation interactions and affecting the formation of a "true oxide" layer at higher electrode potentials. Although OHad is a simple spectator for the ORR, it promotes the ethanol oxidation reaction (EOR) at lower potentials and act as spectator at high OHad coverages. By changing the alkali metal cation at the interface (Li+) on more oxophilic surfaces, it was possible to promote the EOR even more, relative to Na+, without changing the product distribution for the reaction. This cation effect suggests that OHad-Li+(H2O)(x) clusters can stabilize the ethoxide adlayer, thus improving the EOR activity. Our results indicate the importance of the entire electrochemical interface in determining the electrocatalytic activity during reaction. (C) 2015 Elsevier B.V. All rights reserved. C1 [Lopes, Pietro P.; Strmcnik, Dusan; Jirkovsky, Jakub S.; Connell, Justin G.; Stamenkovic, Vojislav; Markovic, Nenad] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. RP Markovic, N (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Lemont, IL 60439 USA. EM nmarkovic@anl.gov RI Lopes, Pietro/E-2724-2013 OI Lopes, Pietro/0000-0003-3211-470X FU Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences [DE-AC0206CH11357] FX This work is supported by the Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Sciences, under contract DE-AC0206CH11357. NR 30 TC 6 Z9 6 U1 16 U2 121 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD MAR 15 PY 2016 VL 262 BP 41 EP 47 DI 10.1016/j.cattod.2015.09.010 PG 7 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA CY1IP UT WOS:000366160200006 ER PT J AU Ayers, KE Renner, JN Danilovic, N Wang, JX Zhang, Y Maric, R Yu, HR AF Ayers, Katherine E. Renner, Julie N. Danilovic, Nemanja Wang, Jia X. Zhang, Yu Maric, Radenka Yu, Haoran TI Pathways to ultra-low platinum group metal catalyst loading in proton exchange membrane electrolyzers SO CATALYSIS TODAY LA English DT Article DE Electrolysis; Catalyst; Manufacturing; Hydrogen; Core-shell; Platinum ID OXYGEN REDUCTION REACTION; FUEL-CELL CATALYSTS; RU NANOPARTICLES; DEPOSITION; ELECTROCATALYST; SURFACES; CO; STABILITY; EVOLUTION; WATER AB Hydrogen is one of the world's most important chemicals, with global production of about 50 billion kg/year. Currently, hydrogen is mainly produced from fossil fuels such as natural gas and coal, producing CO2. Water electrolysis is a promising technology for fossil-free, CO2-free hydrogen production. Proton exchange membrane (PEM)-based water electrolysis also eliminates the need for caustic electrolyte, and has been proven at megawatt scale. However, a major cost driver is the electrode, specifically the cost of electrocatalysts used to improve the reaction efficiency, which are applied at high loadings (>3 mg/cm(2) total platinum group metal (PGM) content). Core-shell catalysts have shown improved activity for hydrogen production, enabling reduced catalyst loadings, while reactive spray deposition techniques (RSDT) have been demonstrated to enable manufacture of catalyst layers more uniformly and with higher repeatability than existing techniques. Core-shell catalysts have also been fabricated with RSDT for fuel cell electrodes with good performance. Manufacturing and materials need to go hand in hand in order to successfully fabricate electrodes with ultra-low catalyst loadings (<0.5 mg/cm(2) total PGM content) without significant variation in performance. This paper describes the potential for these two technologies to work together to enable low cost PEM electrolysis systems. (C) 2015 Elsevier B.V. All rights reserved. C1 [Ayers, Katherine E.; Renner, Julie N.; Danilovic, Nemanja] Proton OnSite, Wallingford, CT 06492 USA. [Wang, Jia X.; Zhang, Yu] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Maric, Radenka; Yu, Haoran] Univ Connecticut, Mat Sci & Engn Dept, Chem & Biomol Engn Dept, Storrs, CT 06269 USA. RP Ayers, KE (reprint author), Proton OnSite, 10 Technol Dr, Wallingford, CT 06492 USA. EM kayers@protononsite.com RI Wang, Jia/B-6346-2011; OI Ayers, Katherine/0000-0003-3246-1744; Zhang, Yu/0000-0002-0814-2965 FU Office of Energy Efficiency and Renewable Energy [DE-SC0008251]; Advanced Manufacturing Office of the Department of Energy [DE-SC0009213] FX Research reported in this publication was supported by the Office of Energy Efficiency and Renewable Energy under award number DE-SC0008251, and the Advanced Manufacturing Office of the Department of Energy under award number DE-SC0009213. The content is solely the responsibility of the authors and does not necessarily represent the official views of the Department of Energy. NR 33 TC 3 Z9 3 U1 13 U2 108 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD MAR 15 PY 2016 VL 262 BP 121 EP 132 DI 10.1016/j.cattod.2015.10.019 PG 12 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA CY1IP UT WOS:000366160200016 ER PT J AU Harigaya, K Nomura, Y AF Harigaya, Keisuke Nomura, Yasunori TI A composite model for the 750 GeV diphoton excess SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; Technicolor and Composite Models ID PROTON-PROTON COLLISIONS; ROOT-S=8 TEV; DARK-MATTER; SEARCH; BOSON; U(1) AB We study a simple model in which the recently reported 750 GeV diphoton excess arises from a composite pseudo Nambu-Goldstone boson - hidden pion - produced by gluon fusion and decaying into two photons. The model only introduces an extra hidden gauge group at the TeV scale with a vectorlike quark in the bifundamental representation of the hidden and standard model gauge groups. We calculate the masses of all the hidden pions and analyze their experimental signatures and constraints. We find that two colored hidden pions must be near the current experimental limits, and hence are probed in the near future. We study physics of would-be stable particles - the composite states that do not decay purely by the hidden and standard model gauge dynamics - in detail, including constraints from cosmology. We discuss possible theoretical structures above the TeV scale, e.g. conformal dynamics and supersymmetry, and their phenomenological implications. We also discuss an extension of the minimal model in which there is an extra hidden quark that is singlet under the standard model and has a mass smaller than the hidden dynamical scale. This provides two standard model singlet hidden pions that can both be viewed as diphoton/diboson resonances produced by gluon fusion. We discuss several scenarios in which these (and other) resonances can be used to explain various excesses seen in the LHC data. C1 [Harigaya, Keisuke; Nomura, Yasunori] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, Berkeley, CA 94720 USA. RP Harigaya, K; Nomura, Y (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, Berkeley, CA 94720 USA. EM keisukeharigaya@berkeley.edu; ynomura@berkeley.edu OI Nomura, Yasunori/0000-0002-1497-1479 FU Office of Science, Office of High Energy and Nuclear Physics, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Science Foundation [PHY-1316783, PHY-1521446]; MEXT KAKENHI [15H05895] FX This work was supported in part by the Director, Office of Science, Office of High Energy and Nuclear Physics, of the U.S. Department of Energy under Contract DE-AC02-05CH11231, by the National Science Foundation under grants PHY-1316783 and PHY-1521446, and by MEXT KAKENHI Grant Number 15H05895. NR 56 TC 15 Z9 15 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 14 PY 2016 IS 3 AR 091 DI 10.1007/JHEP03(2016)091 PG 32 WC Physics, Particles & Fields SC Physics GA DL0GL UT WOS:000375310300001 ER PT J AU Firlar, E Perez-Gonzalez, T Olszewska, A Faivre, D Prozorov, T AF Firlar, Emre Perez-Gonzalez, Teresa Olszewska, Agata Faivre, Damien Prozorov, Tanya TI Following iron speciation in the early stages of magnetite magnetosome biomineralization SO JOURNAL OF MATERIALS RESEARCH LA English DT Review ID ENERGY-LOSS-SPECTROSCOPY; MAGNETOTACTIC BACTERIA; MAGNETOSPIRILLUM-GRYPHISWALDENSE; CIRCULAR-DICHROISM; PROTEOMIC ANALYSIS; OXIDE MATERIALS; CRYSTAL-GROWTH; NANOPARTICLES; MEMBRANE; MINERALIZATION AB Understanding magnetosome magnetite biomineralization is of fundamental interest to devising the strategies for bioinspired synthesis of magnetic materials at the nanoscale. Thus, we investigated the early stages of magnetosome formation in this work and correlated the size and emergent crystallinity of magnetosome nanoparticles with the changes in chemical environment of iron and oxygen by utilizing advanced analytical electron microscopy techniques. We observed that magnetosomes in the early stages of biomineralization with the sizes of 5-10 nm were amorphous, with a majority of iron present as Fe3+, indicative of ferric hydroxide. The magnetosomes with intermediate sizes showed partially crystalline structure with a majority of iron present as Fe3+ and trace amounts of Fe2+. The fully maturated magnetosomes were indexed to magnetite. Our approach provides spatially resolved structural and chemical information of individual magnetosomes with different particle sizes, attributed to magnetosomes at different stages of biomineralization. C1 [Firlar, Emre] US DOE, Emergent Atom & Magnet Struct, Div Mat Sci & Engn, Ames Lab, Ames, IA 50011 USA. [Perez-Gonzalez, Teresa; Olszewska, Agata; Faivre, Damien] Max Planck Inst Colloids & Interfaces, Dept Biomat, Sci Pk Golm, D-14424 Potsdam, Germany. [Prozorov, Tanya] Ames Lab, Emergent Atom & Magnet Struct, Div Mat Sci & Engn, Ames, IA 50011 USA. RP Prozorov, T (reprint author), Ames Lab, Emergent Atom & Magnet Struct, Div Mat Sci & Engn, Ames, IA 50011 USA. EM tprozoro@ameslab.gov RI faivre, damien/D-3713-2009 OI faivre, damien/0000-0001-6191-3389 FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Division of Materials Sciences and Engineering; Department of Energy Office of Science Early Career Research Award, Biomolecular Materials Program; U.S. Department of Energy [DE-AC02-07CH11358]; Max Planck Society; European Research Council [256915] FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Division of Materials Sciences and Engineering. T.P. acknowledges support from the Department of Energy Office of Science Early Career Research Award, Biomolecular Materials Program. The research was performed at the Ames Laboratory, which is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. D.F. acknowledges financial support from the Max Planck Society and the European Research Council (Starting Grant MB2 No. 256915). NR 70 TC 3 Z9 3 U1 13 U2 29 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0884-2914 EI 2044-5326 J9 J MATER RES JI J. Mater. Res. PD MAR 14 PY 2016 VL 31 IS 5 BP 547 EP 555 DI 10.1557/jmr.2016.33 PG 9 WC Materials Science, Multidisciplinary SC Materials Science GA DI4KF UT WOS:000373468100003 ER PT J AU Grate, JW Mo, KF Daily, MD AF Grate, Jay W. Mo, Kai-For Daily, Michael D. TI Triazine-Based Sequence-Defined Polymers with Side-Chain Diversity and Backbone-Backbone Interaction Motifs SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE biomimetics; macromolecules; sequence-defined polymers; simulations; solid-phase synthesis ID PHASE SYNTHESIS; OLIGOMERS; FOLDAMERS; MACROMOLECULES; SCAFFOLD; DESIGN; BLOCK; FIELD AB Sequence control in polymers, well-known in nature, encodes structure and functionality. Here we introduce a new architecture, based on the nucleophilic aromatic substitution chemistry of cyanuric chloride, that creates a new class of sequence-defined polymers dubbed TZPs. Proof of concept is demonstrated with two synthesized hexamers, having neutral and ionizable side chains. Molecular dynamics simulations show backbone-backbone interactions, including H-bonding motifs and pi-pi interactions. This architecture is arguably biomimetic while differing from sequence-defined polymers having peptide bonds. The synthetic methodology supports the structural diversity of side chains known in peptides, as well as backbone-backbone hydrogen-bonding motifs, and will thus enable new macromolecules and materials with useful functions. C1 [Grate, Jay W.; Mo, Kai-For; Daily, Michael D.] Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. RP Grate, JW (reprint author), Pacific NW Natl Lab, POB 999, Richland, WA 99352 USA. EM jwgrate@pnnl.gov FU Materials Synthesis and Simulation across Scales (MS3); Laboratory Directed Research and Development program at Pacific Northwest National Laboratory (PNNL) FX This research was supported as part of the Materials Synthesis and Simulation across Scales (MS3) initiative by the Laboratory Directed Research and Development program at Pacific Northwest National Laboratory (PNNL), a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy(DOE). NR 44 TC 6 Z9 6 U1 13 U2 48 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD MAR 14 PY 2016 VL 55 IS 12 BP 3925 EP 3930 DI 10.1002/anie.201509864 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA DH3AW UT WOS:000372660400009 PM 26865312 ER PT J AU Alikin, DO Ievlev, AV Luchkin, SY Turygin, AP Shur, VY Kalinin, SV Kholkin, AL AF Alikin, D. O. Ievlev, A. V. Luchkin, S. Yu. Turygin, A. P. Shur, V. Ya. Kalinin, S. V. Kholkin, A. L. TI Characterization of LiMn2O4 cathodes by electrochemical strain microscopy SO APPLIED PHYSICS LETTERS LA English DT Article AB Electrochemical strain microscopy (ESM) is a scanning probe microscopy (SPM) method in which the local electrodiffusion is probed via application of AC voltage to the SPM tip and registration of resulting electrochemical strain. Here, we implemented ESM to measure local strain in bulk LiMn2O4 cathodes of a commercial Li-battery in different states of charge to investigate distribution of Li-ion mobility and concentration. Ramped AC ESM imaging and voltage spectroscopy were used to find the most reliable regime of measurements allowing separating and diminishing different contributions to ESM. This is not a trivial task due to complex geometry of the sample and various obstacles resulting in less predictable contributions of different origins into ESM response: electrostatic tip-surface interactions, charge injection, electrostriction, and flexoelectricity. Understanding and control of these contributions is an important step towards quantitative interpretation of ESM data. (C) 2016 AIP Publishing LLC. C1 [Alikin, D. O.; Turygin, A. P.; Shur, V. Ya.; Kholkin, A. L.] Ural Fed Univ, Inst Nat Sci, 51 Lenin Ave, Ekaterinburg 620000, Russia. [Ievlev, A. V.; Kalinin, S. V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Ievlev, A. V.; Kalinin, S. V.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Luchkin, S. Yu.; Kholkin, A. L.] Univ Aveiro, Dept Phys, P-3810193 Aveiro, Portugal. [Luchkin, S. Yu.; Kholkin, A. L.] Univ Aveiro, CICECO, Aveiro Inst Mat, P-3810193 Aveiro, Portugal. RP Alikin, DO (reprint author), Ural Fed Univ, Inst Nat Sci, 51 Lenin Ave, Ekaterinburg 620000, Russia. RI Kholkin, Andrei/G-5834-2010; Luchkin, Sergey/K-3466-2015; Ievlev, Anton/H-3678-2012; Alikin, Denis/K-7914-2015 OI Kholkin, Andrei/0000-0003-3432-7610; Luchkin, Sergey/0000-0003-1923-7449; Ievlev, Anton/0000-0003-3645-0508; Alikin, Denis/0000-0001-9330-7463 FU UrFU development program; Government of the Russian Federation [02.A03.21.0006]; State Task from the Ministry of Education and Science of Russian Federation [1366.2014/236]; CNMS [2013-130]; European Commission within FP7 Marie Curie Initial Training Network "Nanomotion" [290158]; project CICECO-Aveiro Institute of Materials [FCT UID/CTM/50011/2013]; national funds through the FCT/MEC; FEDER under the PT2020 Partnership Agreement FX The equipment of the Ural Center for Shared Use "Modern nanotechnology" UrFU was used. The research was made possible in part by UrFU development program with the financial support of young scientists. The work was partially supported by Government of the Russian Federation (Act 211, Agreement 02.A03.21.0006). V.Y.S. acknowledges financial support within the State Task from the Ministry of Education and Science of Russian Federation (Project No. 1366.2014/236).; A portion of this research (A.V.I. and S.V.K.) was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. V.Y.S., D.O.A., A.I.L., and A.P.T. acknowledge CNMS user proposal (Project 2013-130).; The work was supported by the European Commission within FP7 Marie Curie Initial Training Network "Nanomotion" (Grant Agreement No. 290158). The authors gratefully acknowledge H.-Y. Amanieu and D. Rosato (Robert Bosch GmbH) for providing the samples and useful discussion.; This work was developed in the scope of the project CICECO-Aveiro Institute of Materials (Ref. FCT UID/CTM/50011/2013), financed by national funds through the FCT/MEC and, when applicable, co-financed by FEDER under the PT2020 Partnership Agreement. NR 26 TC 0 Z9 0 U1 10 U2 43 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 14 PY 2016 VL 108 IS 11 AR 113106 DI 10.1063/1.4943944 PG 5 WC Physics, Applied SC Physics GA DH8PY UT WOS:000373058400040 ER PT J AU Leroy, F Passanante, T Cheynis, F Curiotto, S Bussmann, EB Muller, P AF Leroy, F. Passanante, T. Cheynis, F. Curiotto, S. Bussmann, E. B. Mueller, P. TI Catalytically enhanced thermal decomposition of chemically grown silicon oxide layers on Si(001) SO APPLIED PHYSICS LETTERS LA English DT Article ID SCANNING-TUNNELING-MICROSCOPY; VOID FORMATION; ULTRATHIN OXIDE; NATIVE OXIDES; SI SURFACES; DESORPTION; SI(111); IMPURITIES; INTERFACE; OXIDATION AB The thermal decomposition of Si dioxide layers formed by wet chemical treatment on Si(001) has been studied by low-energy electron microscopy. Independent nucleations of voids occur into the Si oxide layers that open by reaction at the void periphery. Depending on the voids, the reaction rates exhibit large differences via the occurrence of a nonlinear growth of the void radius. This non-steady state regime is attributed to the accumulation of defects and silicon hydroxyl species at the SiO2/Si interface that enhances the silicon oxide decomposition at the void periphery. (C) 2016 AIP Publishing LLC. C1 [Leroy, F.; Passanante, T.; Cheynis, F.; Curiotto, S.; Bussmann, E. B.; Mueller, P.] Aix Marseille Univ, CINaM UMR 7325, Campus Luminy,Case 913, F-13288 Marseille, France. [Bussmann, E. B.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Leroy, F (reprint author), Aix Marseille Univ, CINaM UMR 7325, Campus Luminy,Case 913, F-13288 Marseille, France. EM leroy@cinam.univ-mrs.fr RI Muller, Pierre/M-2654-2016; OI Muller, Pierre/0000-0003-0911-1308; Curiotto, Stefano/0000-0002-7332-0836 FU ANR grant LOTUS [13 BS-000-402] FX The authors thank O. Ourdjini, F. Bedu, and I. Ozerov for sample preparation at PLANETE (C'Nano PACA) and Y. Saito for fruitful discussions. We acknowledge ANR 13 BS-000-402 grant LOTUS for financial support. NR 26 TC 1 Z9 1 U1 4 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD MAR 14 PY 2016 VL 108 IS 11 AR 111601 DI 10.1063/1.4941799 PG 4 WC Physics, Applied SC Physics GA DH8PY UT WOS:000373058400010 ER PT J AU Castro, KP Clikeman, TT DeWeerd, NJ Bukovsky, EV Rippy, KC Kuvychko, IV Hou, GL Chen, YS Wang, XB Strauss, SH Boltalina, OV AF Castro, Karlee P. Clikeman, Tyler T. DeWeerd, Nicholas J. Bukovsky, Eric V. Rippy, Kerry C. Kuvychko, Igor V. Hou, Gao-Lei Chen, Yu-Sheng Wang, Xue-Bin Strauss, Steven H. Boltalina, Olga V. TI Incremental Tuning Up of Fluorous Phenazine Acceptors SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE azaacenes; electrochemistry; electron affinity; semiconductors; trifluoromethyl groups ID ELECTRON-AFFINITIES; ORGANIC SEMICONDUCTORS; TRANSPORT-PROPERTIES; CRYSTAL-STRUCTURE; DERIVATIVES; PERFLUORO-4-AZIDOTOLUENE; AMINOPERFLUOROPHENAZINES; FERROELECTRICITY; FLUOROPHENAZINES; SPECTROSCOPY AB In a simple, one-step direct trifluoromethylation of phenazine with CF3I we prepared and characterized nine (poly)trifluoromethyl derivatives with up to six CF3 groups. The electrochemical reduction potentials and gas-phase electron affinities show a direct, strict linear relation to the number of CF3 groups, with phenazine(CF3)(6) reaching a record-high electron affinity of 3.24eV among perfluoroalkylated polyaromatics. C1 [Castro, Karlee P.; Clikeman, Tyler T.; DeWeerd, Nicholas J.; Bukovsky, Eric V.; Rippy, Kerry C.; Kuvychko, Igor V.; Strauss, Steven H.; Boltalina, Olga V.] Colorado State Univ, Dept Chem, Ft Collins, CO 80523 USA. [Hou, Gao-Lei; Wang, Xue-Bin] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. [Chen, Yu-Sheng] Univ Chicago, ChemMatCARS, Adv Photon Source, Argonne, IL 60439 USA. RP Strauss, SH; Boltalina, OV (reprint author), Colorado State Univ, Dept Chem, Ft Collins, CO 80523 USA. EM steven.strauss@colostate.edu; olga.boltalina@colostate.edu FU National Science Foundation [NSF/CHE-1362302, CHE-1012468, NSF/CHE-1346572]; Office of Basic Energy Sciences; Colorado State University Research Foundation; U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences [DE-AC02-06CH11357]; US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences; US Department of Energy's Office of Biological and Environmental Research FX We thank the National Science Foundation (grants NSF/CHE-1362302, and CHE-1012468 (S.H.S. and O.V.B.), the Office of Basic Energy Sciences, and the Colorado State University Research Foundation for partial financial support. ChemMatCARS Sector 15 is principally supported by the National Science Foundation under grant number NSF/CHE-1346572. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, and Office of Basic Energy Sciences under Contract DE-AC02-06CH11357. The low temperature PES work was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences (G.-L.H. and X.-B.W.) and was performed at EMSL, a national scientific user facility sponsored by the US Department of Energy's Office of Biological and Environmental Research and located at PNNL, which is operated by Battelle Memorial Institute for the DOE. NR 49 TC 0 Z9 0 U1 11 U2 20 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD MAR 14 PY 2016 VL 22 IS 12 BP 3930 EP + DI 10.1002/chem.201504122 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA DH1EF UT WOS:000372526500001 PM 26617289 ER PT J AU Alexander, CS Ding, JL Asay, JR AF Alexander, C. S. Ding, J. L. Asay, J. R. TI Experimental characterization and constitutive modeling of the mechanical behavior of molybdenum under electromagnetically applied compression-shear ramp loading SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID MAGNETIC-FIELD; ISENTROPIC COMPRESSION; SHOCK COMPRESSION; ANNEALING BEHAVIOR; 6061-T6 ALUMINUM; SELF-CONSISTENT; EXPERIMENTS ICE; Z-ACCELERATOR; FLYER PLATES; STRENGTH AB Magnetically applied pressure-shear (MAPS) is a new experimental technique that provides a platform for direct measurement of material strength at extreme pressures. The technique employs an imposed quasi-static magnetic field and a pulsed power generator that produces an intense current on a planar driver panel, which in turn generates high amplitude magnetically induced longitudinal compression and transverse shear waves into a planar sample mounted on the drive panel. In order to apply sufficiently high shear traction to the test sample, a high strength material must be used for the drive panel. Molybdenum is a potential driver material for the MAPS experiment because of its high yield strength and sufficient electrical conductivity. To properly interpret the results and gain useful information from the experiments, it is critical to have a good understanding and a predictive capability of the mechanical response of the driver. In this work, the inelastic behavior of molybdenum under uniaxial compression and biaxial compression-shear ramp loading conditions is experimentally characterized. It is observed that an imposed uniaxial magnetic field ramped to approximately 10 T through a period of approximately 2500 mu s and held near the peak for about 250 mu s before being tested appears to anneal the molybdenum panel. In order to provide a physical basis for model development, a general theoretical framework that incorporates electromagnetic loading and the coupling between the imposed field and the inelasticity of molybdenum was developed. Based on this framework, a multi-axial continuum model for molybdenum under electromagnetic loading is presented. The model reasonably captures all of the material characteristics displayed by the experimental data obtained from various experimental configurations. In addition, data generated from shear loading provide invaluable information not only for validating but also for guiding the development of the material model for multiaxial loadings. (C) 2016 AIP Publishing LLC. C1 [Alexander, C. S.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Ding, J. L.] Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. RP Ding, JL (reprint author), Washington State Univ, Sch Mech & Mat Engn, Pullman, WA 99164 USA. EM ding@mme.wsu.edu FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 50 TC 0 Z9 0 U1 4 U2 15 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 14 PY 2016 VL 119 IS 10 AR 105901 DI 10.1063/1.4943496 PG 11 WC Physics, Applied SC Physics GA DH7MA UT WOS:000372976900039 ER PT J AU Armstrong, AM Crawford, MH Jayawardena, A Ahyi, A Dhar, S AF Armstrong, Andrew M. Crawford, Mary H. Jayawardena, Asanka Ahyi, Ayayi Dhar, Sarit TI Role of self-trapped holes in the photoconductive gain of beta-gallium oxide Schottky diodes SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID SOLAR-BLIND PHOTODETECTORS; FILMS; CONTACTS AB Solar-blind photodetection and photoconductive gain >50 corresponding to a responsivity >8 A/W were observed for beta-Ga2O3 Schottky photodiodes. The origin of photoconductive gain was investigated. Current-voltage characteristics of the diodes did not indicate avalanche breakdown, which excludes carrier multiplication by impact ionization as the source for gain. However, photocapacitance measurements indicated a mechanism for hole localization for above-band gap illumination, suggesting self-trapped hole formation. Comparison of photoconductivity and photocapacitance spectra indicated that self-trapped hole formation coincides with the strong photoconductive gain. It is concluded that self-trapped hole formation near the Schottky diode lowers the effective Schottky barrier in reverse bias, producing photoconductive gain. Ascribing photoconductive gain to an inherent property like self-trapping of holes can explain the operation of a variety of beta-Ga2O3 photodetectors. (C) 2016 AIP Publishing LLC. C1 [Armstrong, Andrew M.; Crawford, Mary H.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Jayawardena, Asanka; Ahyi, Ayayi; Dhar, Sarit] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. RP Armstrong, AM (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM aarmstr@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 23 TC 4 Z9 4 U1 5 U2 20 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 14 PY 2016 VL 119 IS 10 AR 103102 DI 10.1063/1.4943261 PG 6 WC Physics, Applied SC Physics GA DH7MA UT WOS:000372976900002 ER PT J AU Bronkhorst, CA Gray, GT Addessio, FL Livescu, V Bourne, NK McDonald, SA Withers, PJ AF Bronkhorst, C. A. Gray, G. T., III Addessio, F. L. Livescu, V. Bourne, N. K. McDonald, S. A. Withers, P. J. TI Response and representation of ductile damage under varying shock loading conditions in tantalum (vol 119, 085103, 2016) SO JOURNAL OF APPLIED PHYSICS LA English DT Correction C1 [Bronkhorst, C. A.; Gray, G. T., III; Addessio, F. L.; Livescu, V.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. [Bourne, N. K.; McDonald, S. A.; Withers, P. J.] Univ Manchester, Sch Mat, Manchester M13 9PL, Lancs, England. RP Bronkhorst, CA (reprint author), Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. EM cabronk@lanl.gov NR 1 TC 0 Z9 0 U1 3 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 14 PY 2016 VL 119 IS 10 AR 109901 PG 1 WC Physics, Applied SC Physics GA DH7MA UT WOS:000372976900041 ER PT J AU Cochrane, KR Lemke, RW Riford, Z Carpenter, JH AF Cochrane, K. R. Lemke, R. W. Riford, Z. Carpenter, J. H. TI Magnetically launched flyer plate technique for probing electrical conductivity of compressed copper SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID INITIO MOLECULAR-DYNAMICS; TOTAL-ENERGY CALCULATIONS; AUGMENTED-WAVE METHOD; TRANSPORT-COEFFICIENTS; CONSTITUTIVE MODEL; LIQUID-METALS; DENSE-PLASMAS; BASIS-SET; RESISTIVITY; TRANSITION AB The electrical conductivity of materials under extremes of temperature and pressure is of crucial importance for a wide variety of phenomena, including planetary modeling, inertial confinement fusion, and pulsed power based dynamic materials experiments. There is a dearth of experimental techniques and data for highly compressed materials, even at known states such as along the principal isentrope and Hugoniot, where many pulsed power experiments occur. We present a method for developing, calibrating, and validating material conductivity models as used in magnetohydrodynamic (MHD) simulations. The difficulty in calibrating a conductivity model is in knowing where the model should be modified. Our method isolates those regions that will have an impact. It also quantitatively prioritizes which regions will have the most beneficial impact. Finally, it tracks the quantitative improvements to the conductivity model during each incremental adjustment. In this paper, we use an experiment on Sandia National Laboratories Z-machine to isentropically launch multiple flyer plates and, with the MHD code ALEGRA and the optimization code DAKOTA, calibrated the conductivity such that we matched an experimental figure of merit to +/-1%. (C) 2016 AIP Publishing LLC. C1 [Cochrane, K. R.; Lemke, R. W.; Riford, Z.; Carpenter, J. H.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Cochrane, KR (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX We would like to thank Sandia's Z operations, target fabrication, and HW design teams. We would also like to thank Michael Desjarlais for insightful discussions pertaining to the conductivity calculations, Marcus Knudson for converting VISAR data to velocities, and Stephanie Hansen for discussions on Ziman and Inferno. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 57 TC 2 Z9 3 U1 0 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 14 PY 2016 VL 119 IS 10 AR 105902 DI 10.1063/1.4943417 PG 10 WC Physics, Applied SC Physics GA DH7MA UT WOS:000372976900040 ER PT J AU Pei, F Jadhav, N Buchovecky, E Bower, AF Chason, E Liu, WJ Tischler, JZ Ice, GE Xu, RQ AF Pei, Fei Jadhav, Nitin Buchovecky, Eric Bower, Allan F. Chason, Eric Liu, Wenjun Tischler, Jonathan Z. Ice, Gene E. Xu, Ruqing TI In-situ synchrotron micro-diffraction study of surface, interface, grain structure, and strain/stress evolution during Sn whisker/hillock formation SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID DYNAMIC RECRYSTALLIZATION DRX; WHISKER GROWTH; HILLOCK FORMATION; STRESS EVOLUTION; TIN WHISKERS; CU; MECHANISM; FILMS AB We have performed X-ray synchrotron micro-diffraction measurements to study the processes controlling the formation of hillocks and whiskers in Sn layers on Cu. The studies were done in realtime on Sn layers that were electro-deposited immediately before the X-ray measurements were started. This enabled a region of the sample to be monitored from the as-deposited state until after a hillock feature formed. In addition to measuring the grain orientation and deviatoric strain (via Laue diffraction), the X-ray fluorescence was monitored to quantify the evolution of the Sn surface morphology and the formation of intermetallic compound (IMC) at the Sn-Cu interface. The results capture the simultaneous growth of the feature and the corresponding film stress, grain orientation, and IMC formation. The observations are compared with proposed mechanisms for whisker/hillock growth and nucleation. (C) 2016 AIP Publishing LLC. C1 [Pei, Fei; Bower, Allan F.; Chason, Eric] Brown Univ, Sch Engn, Providence, RI 02912 USA. [Jadhav, Nitin] IBM Corp, New York, NY 12533 USA. [Buchovecky, Eric] St Gobain, Northboro R&D Ctr, Northborough, MA 01532 USA. [Liu, Wenjun; Tischler, Jonathan Z.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Ice, Gene E.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Pei, F (reprint author), Brown Univ, Sch Engn, Providence, RI 02912 USA. FU NSF-DMR [DMR1206138, DMR1501411]; Brown MRSEC Program [DMR0079964]; DOE Office of Science [DE-AC02-06CH11357]; U.S. DOE Office of Science FX F.P. and E.C. gratefully acknowledge the support from the NSF-DMR under Contract Nos. DMR1206138 and DMR1501411. The work of A.F.B., E.B., and N.J. was supported by the Brown MRSEC Program (No. DMR0079964). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. The work of W.L., J.Z.T., G.E.I., and R.X. was supported by the U.S. DOE Office of Science. NR 42 TC 0 Z9 0 U1 13 U2 17 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD MAR 14 PY 2016 VL 119 IS 10 AR 105302 DI 10.1063/1.4942920 PG 11 WC Physics, Applied SC Physics GA DH7MA UT WOS:000372976900028 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahn, SU Aiola, S Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Almaraz, JRM Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Arnaldi, R Arnold, OW Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Baldisseri, A Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F Martinez, HB Bellwied, R Belmont, R Belmont-Moreno, E Belyaev, V Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bertens, RA Berzano, D Betev, L Bhasin, A Bhat, IR Bhati, AK Bhattacharjee, B Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Biswas, R Biswas, S Bjelogrlic, S Blair, JT Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Borri, M Bossu, F Botta, E Bottger, S Bourjau, C Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brucken, EJ Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Butt, JB Buxton, JT Caffarri, D Cai, X Caines, H Diaz, LC Caliva, A Villar, EC Camerini, P Carena, F Carena, W Carnesecchi, F Castellanos, JC Castro, AJ Casula, EAR Sanchez, CC Cepila, J Cerello, P Cerkala, J Chang, B Chapeland, S Chartier, M Charvet, JL Chattopadhyay, S Chattopadhyay, S Chelnokov, V Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Cho, S Chochula, P Choi, K Chojnacki, M Choudhury, S Christakoglou, P Christensen, CH Christiansen, P Chujo, T Chung, SU Cicalo, C Cifarelli, L Cindolo, F Cleymans, J Colamaria, F Colella, D Collu, A Colocci, M Balbastre, GC del Valle, ZC Connors, ME Contreras, JG Cormier, TM Morales, YC Maldonado, IC Cortese, P Cosentino, MR Costa, F Crochet, P Albino, RC Cuautle, E Cunqueiro, L Dahms, T Dainese, A Danu, A Das, D Das, I Das, S Dash, A Dash, S De, S De Caro, A de Cataldo, G de Conti, C de Cuveland, J De Falco, A De Gruttola, D De Marco, N De Pasquale, S Deisting, A Deloff, A Denes, E Deplano, C Dhankher, P Di Bari, D Di Mauro, A Di Nezza, P Corchero, MAD Dietel, T Dillenseger, P Divia, R Djuvsland, O Dobrin, A Gimenez, DD Donigus, B Dordic, O Drozhzhova, T Dubey, AK Dubla, A Ducroux, L Dupieux, P Ehlers, RJ Elia, D Engel, H Epple, E Erazmus, B Erdemir, I Erhardt, F Espagnon, B Estienne, M Esumi, S Eum, J Evans, D Evdokimov, S Eyyubova, G Fabbietti, L Fabris, D Faivre, J Fantoni, A Fasel, M Feldkamp, L Feliciello, A Feofilov, G Ferencei, J Tellez, AF Ferreiro, EG Ferretti, A Festanti, A Feuillard, VJG Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Fleck, MG Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fuchs, U Furget, C Furs, A Girard, MF Gaardhoje, JJ Gagliardi, M Gago, AM Gallio, M Gangadharan, DR Ganoti, P Gao, C Garabatos, C Garcia-Solis, E Gargiulo, C Gasik, P Gauger, EF Germain, M Gheata, A Gheata, M Ghosh, P Ghosh, SK Gianotti, P Giubellino, P Giubilato, P Gladysz-Dziadus, E Glassel, P Coral, DMG Ramirez, AG Gonzalez, V Gonzalez-Zamora, P Gorbunov, S Gorlich, L Gotovac, S Grabski, V Grachov, OA Graczykowski, LK Graham, KL Grelli, A Grigoras, A Grigoras, C Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Gronefeld, JM Grosse-Oetringhaus, JF Grossiord, JY Grosso, R Guber, F Guernane, R Guerzoni, B Gulbrandsen, K Gunji, T Gupta, A Gupta, R Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H Hamar, G Harris, JW Harton, A Hatzifotiadou, D Hayashi, S Heckel, ST Heide, M Helstrup, H Herghelegiu, A Corral, GH Hess, BA Hetland, KF Hillemanns, H Hippolyte, B Hosokawa, R Hristov, P Huang, M Humanic, TJ Hussain, N Hussain, T Hutter, D Hwang, DS Ilkaev, R Inaba, M Innocenti, GM Ippolitov, M Irfan, M Ivanov, M Ivanov, V Izucheev, V Jacobs, PM Jadhav, MB Jadlovska, S Jadlovsky, J Jahnke, C Jakubowska, MJ Jang, HJ Janik, MA Jayarathna, PHSY Jena, C Jena, S Bustamante, RTJ Jones, PG Jung, H Jusko, A Kalinak, P Kalweit, A Kamin, J Kang, JH Kaplin, V Kar, S Uysal, AK Karavichev, O Karavicheva, T Karayan, L Karpechev, E Kebschull, U Keidel, R Keijdener, DLD Keil, M Khan, MM Khan, P Khan, SA Khanzadeev, A Kharlov, Y Kileng, B Kim, DW Kim, DJ Kim, D Kim, H Kim, JS Kim, M Kim, M Kim, S Kim, T Kirsch, S Kisel, I Kiselev, S Kisiel, A Kiss, G Klay, JL Klein, C Klein, J Klein-Bosing, C Klewin, S Kluge, A Knichel, ML Knospe, AG Kobayashi, T Kobdaj, C Kofarago, M Kollegger, T Kolojvari, A Kondratiev, V Kondratyeva, N Kondratyuk, E Konevskikh, A Kopcik, M Kour, M Kouzinopoulos, C Kovalenko, O Kovalenko, V Kowalski, M Meethaleveedu, GK Kralik, I Kravcakova, A Kretz, M Krivda, M Krizek, F Kryshen, E Krzewicki, M Kubera, AM Kucera, V Kuhn, C Kuijer, PG Kumar, A Kumar, J Kumar, L Kumar, S Kurashvili, P Kurepin, A Kurepin, AB Kuryakin, A Kweon, MJ Kwon, Y La Pointe, SL La Rocca, P de Guevara, PL Fernandes, CL Lakomov, I Langoy, R Lara, C Lardeux, A Lattuca, A Laudi, E Lea, R Leardini, L Lee, GR Lee, S Lehas, F Lemmon, RC Lenti, V Leogrande, E Monzon, IL Vargas, HL Leoncino, M Levai, P Li, S Li, X Lien, J Lietava, R Lindal, S Lindenstruth, V Lippmann, C Lisa, MA Ljunggren, HM Lodato, DF Loenne, PI Loginov, V Loizides, C Lopez, X Torres, EL Lowe, A Luettig, P Lunardon, M Luparello, G Maevskaya, A Mager, M Mahajan, S Mahmood, SM Maire, A Majka, RD Malaev, M Cervantes, IM Malinina, L Mal'Kevich, D Malzacher, P Mamonov, A Manko, V Manso, F Manzari, V Marchisone, M Mares, J Margagliotti, GV 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CA ALICE Collaboration TI Measurement of D-s(+) product ion and nuclear modification factor in Pb-Pb collisions at root S-NN=2.76 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Hadron-Hadron scattering; Heavy ion Experiments; Quark gluon plasma ID HEAVY FLAVOR; STATISTICAL HADRONIZATION; J/PSI SUPPRESSION; CENTRAL RAPIDITY; STRANGENESS; MODEL; ENHANCEMENT AB The production of prompt D-s(+) mesons was measured for the first time in collisions of heavy nuclei with the ALICE detector at the LHC. The analysis was performed on a data sample of Pb-Pb collisions at a centre-of-mass energy per nucleon pair, root s(NN), of 2.76 TeV in two different centrality classes, namely 0-10% and 20-50%. D-s(+) mesons and their antiparticles were reconstructed at mid-rapidity from their hadronic decay channel D-s(+) -> phi pi(+), with phi -> K-K+, in the transverse momentum intervals 4 < p(T) < 12 GeV/c and 6 < p(T) < 12 GeV/c for the 0-10% and 20-50% centrality classes, respectively. The nuclear modi fication factor R-AA was computed by comparing the p(T)-differential production yields in Pb-Pb collisions to those in proton-proton (pp) collisions at the same energy. This pp reference was obtained using the cross section measured at root s = 7 TeV and scaled to root s = 2.76TeV. The R-AA of D-s(+) mesons was compared to that of non-strange D mesons in the 10% most central Pb-Pb collisions. At high p(T) (8 < p(T) < 12 GeV/c) a suppression of the D-s(+)-meson yield by a factor of about three, compatible within uncertainties with that of non-strange D mesons, is observed. At lower p(T) (4 < p(T) < 8 GeV/c) the values of the D-s(+)-meson R-AA are larger than those of non-strange D mesons, although compatible within uncertainties. The production ratios D-s(+)/D-0 and D-s(+)/D+ were also measured in Pb-Pb collisions and compared to their values in proton-proton collisions. C1 [Connors, M. E.] Georgia State Univ, Atlanta, GA 30303 USA. 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D.; Dash, A.; Takahashi, J.] Univ Estadual Campinas, UNICAMP, Campinas, SP, Brazil. [Bellwied, R.; Bianchi, L.; Jayarathna, P. H. S. Y.; Jena, S.; Mcdonald, D.; Ng, F.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.] Univ Houston, Houston, TX USA. [Chang, B.; Kim, D. J.; Rak, J.; Slupecki, M.; Snellman, T. W.; Trzaska, W. H.; Vargyas, M.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Borri, M.; Chartier, M.; Figueredo, M. A. S.; Norman, J.; Romita, R.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Castro, A. J.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.; Sorensen, S.] Univ Tennessee, Knoxville, TN USA. [Marchisone, M.; Vilakazi, Z.] Univ Witwatersrand, Johannesburg, South Africa. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Sekiguchi, Y.; Terasaki, K.; Tsuji, T.; Watanabe, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Busch, O.; Chujo, T.; Esumi, S.; Hosokawa, R.; Inaba, M.; Kobayashi, T.; Miake, Y.; Sano, M.; Tanaka, N.; Watanabe, D.; Yokoyama, H.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Erhardt, F.; Planinic, M.; Poljak, N.; Simatovic, G.; Utrobicic, A.] Univ Zagreb, Zagreb 41000, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Teyssier, B.; Tieulent, R.; Uras, A.] Univ Lyon 1, CNRS, IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Ahammed, Z.; Alam, S. N.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mitra, J.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Patra, R. N.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata, India. [Graczykowski, L. K.; Jakubowska, M. J.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pluta, J.; Szymanski, M.; Zaborowska, A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Belmont, R.; Bianchin, C.; Pan, J.; Pruneau, C. A.; Pujahari, P.; Putschke, J.; Reed, R. J.; Saleh, M. A.; Verweij, M.; Voloshin, S. A.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Barnafoeldi, G. G.; Bencedi, G.; Berenyi, D.; Boldizsar, L.; Denes, E.; Hamar, G.; Kiss, G.; Levai, P.; Lowe, A.; Olah, L.; Pochybova, S.; Varga, D.; Volpe, G.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Aiola, S.; Caines, H.; Connors, M. E.; Ehlers, R. J.; Epple, E.; Grachov, O. A.; Harris, J. W.; Majka, R. D.; Mulligan, J. D.; Oh, S.; Oliver, M. H.; Schuster, T.; Smirnov, N.] Yale Univ, New Haven, CT USA. [Kang, J. H.; Kim, D.; Kim, H.; Kim, M.; Kim, T.; Kwon, Y.; Lee, S.; Song, M.] Yonsei Univ, Seoul 120749, South Korea. [Keidel, R.] Fachhochschule Worms, ZTT, Worms, Germany. RP Adam, J (reprint author), Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic. RI Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Cosentino, Mauro/L-2418-2014; Suaide, Alexandre/L-6239-2016; Barnby, Lee/G-2135-2010; Peitzmann, Thomas/K-2206-2012; Kondratiev, Valery/J-8574-2013; Vinogradov, Leonid/K-3047-2013; Castillo Castellanos, Javier/G-8915-2013; Ferreiro, Elena/C-3797-2017; De Pasquale, Salvatore/B-9165-2008; de Cuveland, Jan/H-6454-2016; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Vechernin, Vladimir/J-5832-2013; Akindinov, Alexander/J-2674-2016; Takahashi, Jun/B-2946-2012; Chinellato, David/D-3092-2012; Pshenichnov, Igor/A-4063-2008; Bregant, Marco/I-7663-2012; Sevcenco, Adrian/C-1832-2012; Natal da Luz, Hugo/F-6460-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Kovalenko, Vladimir/C-5709-2013; Altsybeev, Igor/K-6687-2013; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; OI Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Cosentino, Mauro/0000-0002-7880-8611; Suaide, Alexandre/0000-0003-2847-6556; Barnby, Lee/0000-0001-7357-9904; Peitzmann, Thomas/0000-0002-7116-899X; Kondratiev, Valery/0000-0002-0031-0741; Vinogradov, Leonid/0000-0001-9247-6230; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; De Pasquale, Salvatore/0000-0001-9236-0748; de Cuveland, Jan/0000-0003-0455-1398; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Vechernin, Vladimir/0000-0003-1458-8055; Akindinov, Alexander/0000-0002-7388-3022; Takahashi, Jun/0000-0002-4091-1779; Chinellato, David/0000-0002-9982-9577; Pshenichnov, Igor/0000-0003-1752-4524; Sevcenco, Adrian/0000-0002-4151-1056; Natal da Luz, Hugo/0000-0003-1177-870X; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Kovalenko, Vladimir/0000-0001-6012-6615; Altsybeev, Igor/0000-0002-8079-7026; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Scarlassara, Fernando/0000-0002-4663-8216 FU Worldwide LHC Computing Grid (WLCG) collaboration; State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA); National Office for Research and Technology (NKTH); Department of Atomic Energy of the Government of India; Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT); Direccion General de Asuntos del Personal Academico(DGAPA), Mexico; Amerique Latine Formation academique - European Commission (ALFA-EC); EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); E-Infrastructure shared between Europe and Latin America (EELA); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN); Cubaenergia, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia; Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru FX The ALICE Collaboration would like to thank all its engineers and technicians for their-invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) collaboration. The ALICE Collaboration would like to thank M. He, R. Fries and R. Rapp for making available their model calculations.; The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA) and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico(DGAPA), Mexico, Amerique Latine Formation academique - European Commission (ALFA-EC) and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru. NR 72 TC 3 Z9 3 U1 7 U2 23 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 14 PY 2016 IS 3 AR 082 DI 10.1007/JHEP03(2016)082 PG 33 WC Physics, Particles & Fields SC Physics GA DH7IU UT WOS:000372967800002 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahn, SU Aiola, S Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Almaraz, JRM Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Arnaldi, R Arnold, OW Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Baldisseri, A Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B Batzing, PC Bearden, IG Beck, H Bedda, C Behera, NK Belikov, I Bellini, F Martinez, HB Bellwied, R Belmont, R Belmont-Moreno, E Belyaev, V Bencedi, G Beole, S Berceanu, I Bercuci, A Berdnikov, Y Berenyi, D Bertens, RA Berzano, D Betev, L Bhasin, A Bhat, IR Bhati, AK Bhattacharjee, B Bhom, J Bianchi, L Bianchi, N Bianchin, C Bielcik, J Bielcikova, J Bilandzic, A Biswas, R Biswas, S Bjelogrlic, S Blair, JT Blau, D Blume, C Bock, F Bogdanov, A Boggild, H Boldizsar, L Bombara, M Book, J Borel, H Borissov, A Borri, M Bossu, F Botta, E Bottger, S Bourjau, C Braun-Munzinger, P Bregant, M Breitner, T Broker, TA Browning, TA Broz, M Brucken, EJ Bruna, E Bruno, GE Budnikov, D Buesching, H Bufalino, S Buncic, P Busch, O Buthelezi, Z Butt, JB Buxton, JT Caffarri, D Cai, X Caines, H Diaz, LC Caliva, A Villar, EC Camerini, P Carena, F Carena, W Carnesecchi, F Castellanos, JC Castro, AJ Casula, EAR Sanchez, CC Cepila, J Cerello, P Cerkala, J Chang, B Chapeland, S Chartier, M Charvet, JL Chattopadhyay, S Chattopadhyay, S Chelnokov, V Cherney, M Cheshkov, C Cheynis, B Barroso, VC Chinellato, DD Cho, S 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Feldkamp, L Feliciello, A Feofilov, G Ferencei, J Tellez, AF Ferreiro, EG Ferretti, A Festanti, A Feuillard, VJG Figiel, J Figueredo, MAS Filchagin, S Finogeev, D Fionda, FM Fiore, EM Fleck, MG Floris, M Foertsch, S Foka, P Fokin, S Fragiacomo, E Francescon, A Frankenfeld, U Fuchs, U Furget, C Furs, A Girard, MF Gaardhoje, JJ Gagliardi, M Gago, AM Gallio, M Gangadharan, DR Ganoti, P Gao, C Garabatos, C Garcia-Solis, E Gargiulo, C Gasik, P Gauger, EF Germain, M Gheata, A Gheata, M Ghosh, P Ghosh, SK Gianotti, P Giubellino, P Giubilato, P Gladysz-Dziadus, E Glassel, P Coral, DMG Ramirez, AG Gonzalez, V Gonzalez-Zamora, P Gorbunov, S Gorlich, L Gotovac, S Grabski, V Grachov, OA Graczykowski, LK Graham, KL Grelli, A Grigoras, A Grigoras, C Grigoriev, V Grigoryan, A Grigoryan, S Grinyov, B Grion, N Gronefeld, JM Grosse-Oetringhaus, JF Grossiord, JY Grosso, R Guber, F Guernane, R Guerzoni, B Gulbrandsen, K Gunji, T Gupta, A Gupta, R Haake, R Haaland, O Hadjidakis, C Haiduc, M Hamagaki, H 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CA ALICE Collaboration TI Transverse momentum dependence of D-meson production in Pb-Pb collisions at root S-NN=2.76 TeV SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Heavy ion Experiments; Quark gluon plasma; Charm physics ID HEAVY-ION COLLISIONS; ENERGY-LOSS; ROOT-S(NN)=2.76 TEV; QCD MATTER; LHC; FLAVOR; CHARM; PROTONS; MODEL; FLOW AB The production of prompt charmed mesons D-0, D+ and D*(+), and their antiparticles, was measured with the ALICE detector in Pb-Pb collisions at the centre-of-mass energy per nucleon pair, root s(NN), of 2.76 TeV. The production yields for rapidity vertical bar y vertical bar < 0.5 are presented as a function of transverse momentum, p(T), in the interval 1-36 GeV/c for the centrality class 0-10% and in the interval 1-16 GeV/c for the centrality class 30-50%. The nuclear modification factor R-AA was computed using a proton-proton reference at root s = 2.76 TeV, based on measurements at root s = 7 TeV and on theoretical calculations. A maximum suppression by a factor of 5-6 with respect to binary-scaled pp yields is observed for the most central collisions at p(T) of about 10 GeV/c. A suppression by a factor of about 2-3 persists at the highest p(T) covered by the measurements. At low p(T) (1-3 GeV/c), the R-AA has large uncertainties that span the range 0.35 (factor of about 3 suppression) to 1 (no suppression). In all p(T) intervals, the R-AA is larger in the 30-50% centrality class compared to central collisions. The D-meson R-AA is also compared with that of charged pions and, at large p(T), charged hadrons, and with model calculations. C1 [Grigoryan, A.; Papikyan, V.] Yerevan Phys Inst, AI Alikhanyan Natl Sci Lab, Yerevan 375036, Armenia. [Bello Martinez, H.; Cortes Maldonado, I.; Fernandez Tellez, A.; Martinez, M. I.; Moreno, L. A. P.; Noris, J. C. C.; Rodriguez Cahuantzi, M.; Tejeda Munoz, G.; Vargas, A.; Vergara Limon, S.; Villatoro Tello, A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. 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A.; Buesching, H.; Dillenseger, P.; Doenigus, B.; Drozhzhova, T.; Erdemir, I.; Heckel, S. T.; Kamin, J.; Klein, C.; Luettig, P.; Marquard, M.; Ozdemir, M.; Lara, C. E. Perez; Lezama, E. Perez; Peskov, V.; Rascanu, B. T.; Reichelt, P.; Renfordt, R.; Sahlmuller, B.; Schuchmann, S.; Toia, A.] Goethe Univ Frankfurt, Inst Kernphys, D-60054 Frankfurt, Germany. [Anielski, J.; Bathen, B.; Feldkamp, L.; Haake, R.; Heide, M.; Klein-Boesing, C.; De Godoy, D. A. Moreira; Muehlheim, D.; Passfeld, A.; Wessels, J. P.; Westerhoff, U.; Wilde, M.; Zimmermann, M. B.] Univ Munster, Inst Kernphys, Wilhelm Klemm Str 9, D-48149 Munster, Germany. [Belikov, I.; Hippolyte, B.; Kuhn, C.; Maire, A.; Molnar, L.; Rami, F.; Roy, C.] Univ Strasbourg, CNRS, IN2P3, Inst Pluridisciplinaire Hubert Curien, Strasbourg, France. [Finogeev, D.; Furs, A.; Guber, F.; Karavichev, O.; Karavicheva, T.; Karpechev, E.; Konevskikh, A.; Kurepin, A.; Kurepin, A. 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[Danu, A.; Gheata, M.; Haiduc, M.; Mitu, C. M.; Niculescu, M.; Ristea, C.; Sevcenco, A.; Stan, I.; Zgura, I. S.] Inst Space Sci, Bucharest, Romania. [Cuautle, E.; Maldonado Cervantes, I.; Nellen, L.; Ortiz Velasquez, A.; Paic, G.] Univ Nacl Autonoma Mexico, Inst Ciencias Nucl, Mexico City 04510, DF, Mexico. [Alfaro Molina, R.; Belmont-Moreno, E.; Gomez Coral, D. M.; Grabski, V.; Leon Vargas, H.; Menchaca-Rocha, A.; Sandoval, A.; Serradilla, E.] Univ Nacl Autonoma Mexico, Inst Fis, Mexico City, DF, Mexico. [Bossu, F.; Buthelezi, Z.; Foertsch, S.; Marchisone, M.; Murray, S.; Senosi, K.; Steyn, G.] Natl Res Fdn, IThemba LABS, Somerset West, South Africa. [Batyunya, B.; Grigoryan, S.; Malinina, L.; Mikhaylov, K.; Nomokonov, P.; Rogochaya, E.; Vodopyanov, A.; Zaporozhets, S.] Joint Inst Nucl Res, Dubna, Russia. [Baek, Y. W.; Oh, S. K.] Konkuk Univ, Seoul, South Korea. [Ahn, S. U.; Jang, H. J.] Korea Inst Sci & Technol Informat, Daejeon, South Korea. [Uysal, A. 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S.; Evans, D.; Graham, K. L.; Jones, P. G.; Jusko, A.; Krivda, M.; Lee, G. R.; Lietava, R.; Baillie, O. Villalobos; Zardoshti, N.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Calvo Villar, E.; Gago, A. M.] Pontificia Univ Catolica Peru, Dept Ciencias, Secc Fis, Lima, Peru. [Evdokimov, S.; Izucheev, V.; Kharlov, Y.; Kondratyuk, E.; Petrov, V.; Polichtchouk, B.; Sadovsky, S.; Shangaraev, A.] NRC Kurchatov Inst, SSC IHEP, Protvino, Russia. [Weber, M.] Stefan Meyer Inst Subatomare Phys SMI, Vienna, Austria. [Aphecetche, L.; Audurier, B.; Batigne, G.; Erazmus, B.; Estienne, M.; Germain, M.; Blanco, J. Martin; Garcia, G. Martinez; Massacrier, L.; Molnar, L.; De Godoy, D. A. Moreira; Morreale, A.; Pillot, P.; Ette, L. Ron; Schutz, Y.; Shabetai, A.; Stocco, D.; Wang, M.; Zhu, J.] Univ Nantes, CNRS, IN2P3, SUBATECH,Ecole Mines Nantes, Nantes, France. [Kobdaj, C.; Poonsawat, W.] Suranaree Univ Technol, Nakhon Ratchasima, Thailand. [Cerkala, J.; Jadlovska, S.; Jadlovsky, J.; Kopcik, M.; Papcun, P.] Tech Univ Kosice, Kosice, Slovakia. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ Split FESB, Split, Croatia. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Goerlich, L.; Kowalski, M.; Matyja, A.; Mayer, C.; Otwinowski, J.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Blair, J. T.; Gauger, E. F.; Knospe, A. G.; Markert, C.; Thomas, D.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Almaraz, J. R. M.; Leon Monzon, I.; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Alves Garcia Prado, C.; Bregant, M.; Cosentino, M. R.; De, S.; de Conti, C.; Domenicis Gimenez, D.; Figueredo, M. A. S.; Jahnke, C.; Lagana Fernandes, C.; Mas, A.; Munhoz, M. G.; Natal da Luz, H.; Oliveira Da Silva, A. C.; Pereira De Oliveira Filho, E.; Suaide, A. A. P.; Szanto de Toledo, A.; Zanoli, H. J. C.] Univ Sao Paulo, Sao Paulo, Brazil. [Chinellato, D. D.; Dash, A.; Takahashi, J.] Univ Estadual Campinas UNICAMP, Campinas, SP, Brazil. [Bellwied, R.; Bianchi, L.; Jayarathna, P. H. S. Y.; Jena, S.; Mcdonald, D.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.] Univ Houston, Houston, TX USA. [Chang, B.; Kim, D. J.; Rak, J.; Slupecki, M.; Snellman, T. W.; Trzaska, W. H.; Vargyas, M.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Borri, M.; Chartier, M.; Figueredo, M. A. S.; Norman, J.; Romita, R.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Castro, A. J.; Mazer, J.; Nattrass, C.; Read, K. F.; Scott, R.; Sharma, N.; Sorensen, S.] Univ Tennessee, Knoxville, TN USA. [Marchisone, M.; Vilakazi, Z.] Univ Witwatersrand, Johannesburg, South Africa. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Sekiguchi, Y.; Terasaki, K.; Tsuji, T.; Watanabe, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Busch, O.; Chujo, T.; Esumi, S.; Hosokawa, R.; Inaba, M.; Kobayashi, T.; Miake, Y.; Sano, M.; Tanaka, N.; Watanabe, D.; Yokoyama, H.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Erhardt, F.; Planinic, M.; Poljak, N.; Simatovic, G.; Utrobicic, A.] Univ Zagreb, Zagreb 41000, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Teyssier, B.; Tieulent, R.; Uras, A.] Univ Lyon 1, CNRS, IN2P3, IPN Lyon, F-69622 Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Ahammed, Z.; Alam, S. N.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mitra, J.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Ng, F.; Pal, S. K.; Patra, R. N.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Ctr Variable Energy Cyclotron, Kolkata, India. [Graczykowski, L. K.; Jakubowska, M. J.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pluta, J.; Szymanski, M.; Zaborowska, A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Belmont, R.; Bianchin, C.; Pan, J.; Pruneau, C. A.; Pujahari, P.; Putschke, J.; Reed, R. J.; Saleh, M. A.; Verweij, M.; Voloshin, S. A.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Barnafoeldi, G. G.; Bencedi, G.; Berenyi, D.; Boldizsar, L.; Denes, E.; Hamar, G.; Kiss, G.; Levai, P.; Lowe, A.; Olah, L.; Pochybova, S.; Varga, D.; Volpe, G.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Aiola, S.; Caines, H.; Connors, M. E.; Ehlers, R. J.; Epple, E.; Grachov, O. A.; Harris, J. W.; Majka, R. D.; Mulligan, J. D.; Oh, S.; Oliver, M. H.; Schuster, T.; Smirnov, N.] Yale Univ, New Haven, CT USA. [Kang, J. H.; Kim, D.; Kim, H.; Kim, M.; Kim, T.; Kwon, Y.; Lee, S.; Song, M.] Yonsei Univ, Seoul 120749, South Korea. [Keidel, R.] Zentrum Technol Transfer & Telekommun ZTT, Fachhsch Worms, Worms, Germany. [Connors, M. E.] Georgia State Univ, Atlanta, GA 30303 USA. [Malinina, L.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl, Phys, Moscow, Russia. RP Adam, J (reprint author), Czech Tech Univ, Fac Nucl Sci & Phys Engn, CR-11519 Prague, Czech Republic. RI Natal da Luz, Hugo/F-6460-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Fernandez Tellez, Arturo/E-9700-2017; Kovalenko, Vladimir/C-5709-2013; Altsybeev, Igor/K-6687-2013; Vickovic, Linda/F-3517-2017; Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Cosentino, Mauro/L-2418-2014; Suaide, Alexandre/L-6239-2016; Barnby, Lee/G-2135-2010; Peitzmann, Thomas/K-2206-2012; Kondratiev, Valery/J-8574-2013; Vinogradov, Leonid/K-3047-2013; Castillo Castellanos, Javier/G-8915-2013; Ferreiro, Elena/C-3797-2017; Chinellato, David/D-3092-2012; Kurepin, Alexey/H-4852-2013; Jena, Deepika/P-2873-2015; Jena, Satyajit/P-2409-2015; Vechernin, Vladimir/J-5832-2013; Pshenichnov, Igor/A-4063-2008; Bregant, Marco/I-7663-2012; Akindinov, Alexander/J-2674-2016; Takahashi, Jun/B-2946-2012; Sevcenco, Adrian/C-1832-2012; De Pasquale, Salvatore/B-9165-2008; de Cuveland, Jan/H-6454-2016 OI Natal da Luz, Hugo/0000-0003-1177-870X; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Fernandez Tellez, Arturo/0000-0003-0152-4220; Kovalenko, Vladimir/0000-0001-6012-6615; Altsybeev, Igor/0000-0002-8079-7026; Vickovic, Linda/0000-0002-9820-7960; Scarlassara, Fernando/0000-0002-4663-8216; Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Cosentino, Mauro/0000-0002-7880-8611; Suaide, Alexandre/0000-0003-2847-6556; Barnby, Lee/0000-0001-7357-9904; Peitzmann, Thomas/0000-0002-7116-899X; Kondratiev, Valery/0000-0002-0031-0741; Vinogradov, Leonid/0000-0001-9247-6230; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; Chinellato, David/0000-0002-9982-9577; Kurepin, Alexey/0000-0002-1851-4136; Jena, Deepika/0000-0003-2112-0311; Jena, Satyajit/0000-0002-6220-6982; Vechernin, Vladimir/0000-0003-1458-8055; Pshenichnov, Igor/0000-0003-1752-4524; Akindinov, Alexander/0000-0002-7388-3022; Takahashi, Jun/0000-0002-4091-1779; Sevcenco, Adrian/0000-0002-4151-1056; De Pasquale, Salvatore/0000-0001-9236-0748; de Cuveland, Jan/0000-0003-0455-1398 FU State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; 'Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA); National Office for Research and Technology (NKTH); Department of Atomic Energy of the Government of India; Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT); Direccion General de Asuntos del Personal Academico(DGAPA), Mexico; Amerique Latine Formation academique - European Commission (ALFA-EC); EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovations; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); E-Infrastructure shared between Europe and Latin America (EELA; Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Educacion); Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN); Cubaenerga, Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia; Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) collaboration.; The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung und Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; Hungarian Orszagos Tudomanyos Kutatasi Alappgrammok (OTKA) and National Office for Research and Technology (NKTH); Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; MEXT Grant-in-Aid for Specially Promoted Research, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direccion General de Asuntos del Personal Academico(DGAPA), Mexico, ;Amerique Latine Formation academique - European Commission (ALFA-EC) and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovations and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Educacion), Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN), Cubaenerga, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru. NR 85 TC 11 Z9 11 U1 5 U2 21 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD MAR 14 PY 2016 IS 3 AR 081 DI 10.1007/JHEP03(2016)081 PG 43 WC Physics, Particles & Fields SC Physics GA DH7IU UT WOS:000372967800001 ER PT J AU Pagano, JK Dorhout, JM Czerwinski, KR Morris, DE Scott, BL Waterman, R Kiplinger, JL AF Pagano, Justin K. Dorhout, Jacquelyn M. Czerwinski, Kenneth R. Morris, David E. Scott, Brian L. Waterman, Rory Kiplinger, Jaqueline L. TI Tuning the Oxidation State, Nuclearity, and Chemistry of Uranium Hydrides with Phenylsilane and Temperature: The Case of the Classic Uranium(III) Hydride Complex [(C5Me5)(2)U(mu-H)](2) SO ORGANOMETALLICS LA English DT Article ID PENTAVALENT URANIUM; ELECTRONIC-STRUCTURE; MULTIELECTRON REDUCTANTS; REDOX ENERGETICS; HALIDE-COMPLEXES; ELEMENT; TETRAVALENT; REACTIVITY; REDUCTION; TRIVALENT AB This work demonstrates that the oxidation state and chemistry of uranium hydrides can be tuned with temperature and the stoichiometry of phenylsilane. The trivalent uranium hydride [(C5Me5)(2)UH](x) (5) was found to be comprised of an equilibrium mixture of U(III) hydrides in solution at ambient temperature. A single U(III) species can be selectively prepared by treating (C5Me5)(2)UMe2 (4) with 2 equiv of phenylsilane at 50 degrees C. The U(III) system is a potent reducing agent and displayed chemistry distinct from the U(IV) system [(C5Me5)(2)U(H)(-H)](2) (2), which was harnessed to prepare a variety of organometallic complexes, including (C5Me5)(2)U(dmpe)(H) (6), and the novel uranium(IV) metallacyclopentadiene complex (C5Me5)(2)U(C4Me4) (11) C1 [Pagano, Justin K.; Dorhout, Jacquelyn M.; Morris, David E.; Kiplinger, Jaqueline L.] Los Alamos Natl Lab, Div Chem, Mail Stop J514, Los Alamos, NM 87545 USA. [Scott, Brian L.] Los Alamos Natl Lab, Mat Phys & Applicat Div, Mail Stop J514, Los Alamos, NM 87545 USA. [Pagano, Justin K.; Waterman, Rory] Univ Vermont, Dept Chem, Cook Phys Sci Bldg, Burlington, VT 05405 USA. [Dorhout, Jacquelyn M.; Czerwinski, Kenneth R.] Univ Nevada, Dept Chem, 4505 South Maryland Pkwy,Box 454009, Las Vegas, NV 89154 USA. RP Kiplinger, JL (reprint author), Los Alamos Natl Lab, Div Chem, Mail Stop J514, Los Alamos, NM 87545 USA. EM kiplinger@lanl.gov RI Kiplinger, Jaqueline/B-9158-2011; Scott, Brian/D-8995-2017 OI Kiplinger, Jaqueline/0000-0003-0512-7062; Scott, Brian/0000-0003-0468-5396 FU U.S. Department of Energy through the Office of Workforce Development for Teachers and Scientists, Office of Science Graduate Student Research (SCGSR) program (GRA Fellowship); LANL LDRD Program; LANL G. T. Seaborg Institute for Transactinium Science (GRA Fellowship); Office of Basic Energy Sciences, Heavy Element Chemistry program; U.S. Department of Homeland Security (GRA fellowship) [2012-DN-130-NF0001]; U.S. National Science Foundation [CHE-1265608]; Oak Ridge Institute for Science and Education for the DOE [DE-AC05-06OR23100]; Los Alamos National Security, LLC, for the National Nuclear Security Administration of U.S. Department of Energy [DE-AC52-06NA25396] FX For financial support of this work, we acknowledge the U.S. Department of Energy through the Office of Workforce Development for Teachers and Scientists, Office of Science Graduate Student Research (SCGSR) program (GRA Fellowship to J.K.P.), the LANL LDRD Program and the LANL G. T. Seaborg Institute for Transactinium Science (GRA Fellowship to J.M.D.), and the Office of Basic Energy Sciences, Heavy Element Chemistry program (J.L.K., B.L.S., materials & supplies). We also acknowledge the U.S. Department of Homeland Security (GRA fellowship to J.M.D. under grant 2012-DN-130-NF0001) and the U.S. National Science Foundation (grant CHE-1265608 to R.W.). Finally, we thank Dr. Nicholas E. Travia for performing preliminary experiments and Drs. Karla A. Erickson and Marisa J. Monreal (all LANL) for helpful discussions. The SCGSR program is administered by the Oak Ridge Institute for Science and Education for the DOE (contract DE-AC05-06OR23100). Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of U.S. Department of Energy (contract DE-AC52-06NA25396). NR 25 TC 11 Z9 11 U1 5 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0276-7333 EI 1520-6041 J9 ORGANOMETALLICS JI Organometallics PD MAR 14 PY 2016 VL 35 IS 5 BP 617 EP 620 DI 10.1021/acs.organomet.6b00091 PG 4 WC Chemistry, Inorganic & Nuclear; Chemistry, Organic SC Chemistry GA DG6QD UT WOS:000372210300002 ER PT J AU Javidpour, P Deutsch, S Mutalik, VK Hillson, NJ Petzold, CJ Keasling, JD Beller, HR AF Javidpour, Pouya Deutsch, Samuel Mutalik, Vivek K. Hillson, Nathan J. Petzold, Christopher J. Keasling, Jay D. Beller, Harry R. TI Investigation of Proposed Ladderane Biosynthetic Genes from Anammox Bacteria by Heterologous Expression in E-coli SO PLOS ONE LA English DT Article ID ANAEROBIC AMMONIUM OXIDATION; ACID-DERIVED FUELS; MICROBIAL-PRODUCTION; BIOLOGY; CHEMICALS; PROTEIN; TRANSCRIPTION; METABOLISM; POLYMERASE; PRODUCTS AB Ladderanes are hydrocarbon chains with three or five linearly concatenated cyclobutane rings that are uniquely produced as membrane lipid components by anammox (anaerobic ammonia-oxidizing) bacteria. By virtue of their angle and torsional strain, ladderanes are unusually energetic compounds, and if produced biochemically by engineered microbes, could serve as renewable, high-energy-density jet fuel components. The biochemistry and genetics underlying the ladderane biosynthetic pathway are unknown, however, previous studies have identified a pool of 34 candidate genes from the anammox bacterium, Kuenenia stuttgartiensis, some or all of which may be involved with ladderane fatty acid biosynthesis. The goal of the present study was to establish a systematic means of testing the candidate genes from K. stuttgartiensis for involvement in ladderane biosynthesis through heterologous expression in E. coli under anaerobic conditions. This study describes an efficient means of assembly of synthesized, codon-optimized candidate ladderane biosynthesis genes in synthetic operons that allows for changes to regulatory element sequences, as well as modular assembly of multiple operons for simultaneous heterologous expression in E. coli (or potentially other microbial hosts). We also describe in vivo functional tests of putative anammox homologs of the phytoene desaturase CrtI, which plays an important role in the hypothesized ladderane pathway, and a method for soluble purification of one of these enzymes. This study is, to our knowledge, the first experimental effort focusing on the role of specific anammox genes in the production of ladderanes, and lays the foundation for future efforts toward determination of the ladderane biosynthetic pathway. Our substantial, but far from comprehensive, efforts at elucidating the ladderane biosynthetic pathway were not successful. We invite the scientific community to take advantage of the considerable synthetic biology resources and experimental results developed in this study to elucidate the biosynthetic pathway that produces unique and intriguing ladderane lipids. C1 [Javidpour, Pouya; Hillson, Nathan J.; Petzold, Christopher J.; Keasling, Jay D.; Beller, Harry R.] Joint BioEnergy Inst, 5885 Hollis Ave, Emeryville, CA USA. [Javidpour, Pouya; Hillson, Nathan J.; Petzold, Christopher J.; Keasling, Jay D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Syst & Engn, Berkeley, CA 94720 USA. [Deutsch, Samuel; Hillson, Nathan J.] Joint Genome Inst, 2800 Mitchell Dr, Walnut Creek, CA USA. [Mutalik, Vivek K.] LBNL, Environm Genom & Syst Biol, Berkeley, CA USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Beller, Harry R.] LBNL, Earth & Environm Sci, Berkeley, CA USA. RP Beller, HR (reprint author), Joint BioEnergy Inst, 5885 Hollis Ave, Emeryville, CA USA.; Beller, HR (reprint author), LBNL, Earth & Environm Sci, Berkeley, CA USA. EM HRBeller@lbl.gov RI Beller, Harry/H-6973-2014; OI Mutalik, Vivek/0000-0001-7934-0400; Deutsch, Samuel/0000-0001-9456-7101 FU U. S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was part of the DOE Joint BioEnergy Institute (http://www.jbei.org) supported by the U. S. Department of Energy (http://www.energy.gov/), Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U. S. Department of Energy. Work conducted by the Joint Genome Institute was supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 42 TC 2 Z9 2 U1 8 U2 17 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD MAR 14 PY 2016 VL 11 IS 3 AR e0151087 DI 10.1371/journal.pone.0151087 PG 21 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DH1UO UT WOS:000372570600047 PM 26975050 ER PT J AU Levin, I Krayzman, V Woicik, JC Bridges, F Sterbinsky, GE Usher, TM Jones, JL Torrejon, D AF Levin, I. Krayzman, V. Woicik, J. C. Bridges, F. Sterbinsky, G. E. Usher, T-M. Jones, J. L. Torrejon, D. TI Local structure in BaTiO3-BiScO3 dipole glasses SO PHYSICAL REVIEW B LA English DT Article ID SOLID-SOLUTIONS; PEROVSKITE; POLARIZATION; DIELECTRICS; CERAMICS; RELAXOR AB Local structures in cubic perovskite-type (Ba0.6Bi0.4)(Ti0.6Sc0.4)O-3 solid solutions that exhibit reentrant dipole glass behavior have been studied with variable-temperature x-ray/neutron total scattering, extended x-ray absorption fine structure, and electron diffraction methods. Simultaneous fitting of these data using a reverse Monte Carlo algorithm provided instantaneous atomic configurations, which have been used to extract local displacements of the constituent species. The smaller Bi and Ti atoms exhibit probability density distributions that consist of 14 and 8 split sites, respectively. In contrast, Ba and Sc feature single-site distributions. The multisite distributions arise from large and strongly anisotropic off-center displacements of Bi and Ti. The cation displacements are correlated over a short range, with a correlation length limited by chemical disorder. The magnitudes of these displacements and their anisotropy, which are largely determined by local chemistry, change relatively insignificantly on cooling from room temperature. The structure features a nonrandom distribution of local polarization with low-dimensional polar clusters that are several unit cells in size. In situ measurements of atomic pair-distribution function under applied electric field were used to study field-induced changes in the local structure; however, no significant effects besides lattice expansion in the direction of the field could be observed up to electric-field values of 4 kVmm(-1). C1 [Levin, I.; Krayzman, V.; Woicik, J. C.] NIST, Mat Measurement Sci Div, Gaithersburg, MD 20899 USA. [Bridges, F.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 95064 USA. [Sterbinsky, G. E.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Usher, T-M.; Jones, J. L.] N Carolina State Univ, Dept Mat Sci & Engn, Box 7907, Raleigh, NC 27695 USA. [Torrejon, D.] George Mason Univ, Dept Math Sci, Fairfax, VA 22030 USA. RP Levin, I (reprint author), NIST, Mat Measurement Sci Div, Gaithersburg, MD 20899 USA. EM igor.levin@nist.gov OI Usher, Tedi-Marie/0000-0001-8265-5972 FU Department of Energy (DOE), Office of Basic Energy Sciences; DOE [DE-AC52-06NA25396]; SSRL [DE-AC02-76SF00515]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]; APS [DE-AC02-06CH11357]; National Science Foundation Graduate Research Fellowship [DGE-1356109] FX This work benefited from the use of the Lujan Center at Los Alamos Neutron Science Center, while it was funded by the Department of Energy (DOE), Office of Basic Energy Sciences. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract No. DE-AC52-06NA25396. Portions of this research were carried out at the (i) SSRL Contract No. DE-AC02-76SF00515, a directorate of the stanford linear accelerator center (SLAC) National Accelerator Laboratory and an Office of Science User Facility operated for the U.S. Department of Energy, Office of Science, by Stanford University, (ii) National Synchrotron Light Source (NIST beamline X23A2), Brookhaven National Laboratory, supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886, and (iii) APS Contract No. DE-AC02-06CH11357 (beamline 11-ID-B). The authors are grateful to J. Siewenie (Oak Ridge National Laboratory) and E. Nelson (SSRL) for their technical assistance with the neutron scattering and x-ray absorption measurements, respectively, and to K. Beyer (APS) for his help with the x-ray PDF measurements. The work of D.T. has been supported by the National Science Foundation Graduate Research Fellowship under Grant No. DGE-1356109. NR 37 TC 0 Z9 0 U1 15 U2 33 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 14 PY 2016 VL 93 IS 10 AR 104106 DI 10.1103/PhysRevB.93.104106 PG 12 WC Physics, Condensed Matter SC Physics GA DG9LL UT WOS:000372404400003 ER PT J AU Ostlin, A Di Marco, I Locht, ILM Lashley, JC Vitos, L AF Ostlin, A. Di Marco, I. Locht, I. L. M. Lashley, J. C. Vitos, L. TI Stacking fault energetics of alpha- and gamma-cerium investigated with ab initio calculations SO PHYSICAL REVIEW B LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; MEAN-FIELD THEORY; CRYSTAL-STRUCTURE; ELECTRON-GAS; METALS; TRANSITION; ENERGY; PHASE; CE; TRANSFORMATION AB At ambient pressure the element cerium shows a metastable (t(1/2) similar to 40 years) double-hexagonal close-packed beta phase that is positioned between two cubic phases, gamma and alpha. With modest pressure the beta phase can be suppressed, and a volume contraction (17%) occurs between the gamma and the alpha phases as the temperature is varied. This phenomenon has been linked to subtle alterations in the 4f band. In order to rationalize the presence of the metastable beta phase, and its position in the phase diagram, we have computed the stacking fault formation energies of the cubic phases of cerium using an axial interaction model. This model links the total energy differences between hexagonal closed-packed stacking sequences and stacking fault energetics. Total energies are calculated by density functional theory and by dynamical mean-field theory merged with density functional theory. It is found that there is a large difference in the stacking fault energies between the alpha and the gamma phase. The beta-phase energy is nearly degenerate with the gamma phase, consistent with previous third-law calorimetry results, and dislocation dynamics explain the pressure and temperature hysteretic effects. C1 [Ostlin, A.; Vitos, L.] KTH Royal Inst Technol, Dept Mat Sci & Engn, Appl Mat Phys, SE-10044 Stockholm, Sweden. [Di Marco, I.; Locht, I. L. M.; Lashley, J. C.; Vitos, L.] Uppsala Univ, Dept Phys & Astron, POB 516, SE-75120 Uppsala, Sweden. [Locht, I. L. M.] Radboud Univ Nijmegen, Inst Mol & Mat, Heyendaalseweg 135, NL-6525 AJ Nijmegen, Netherlands. [Lashley, J. C.] Los Alamos Natl Lab, POB 1663,Bikini Atoll Rd, Los Alamos, NM 87545 USA. [Vitos, L.] Wigner Res Ctr Phys, Res Inst Solid State Phys & Opt, POB 49, H-1525 Budapest, Hungary. RP Ostlin, A (reprint author), KTH Royal Inst Technol, Dept Mat Sci & Engn, Appl Mat Phys, SE-10044 Stockholm, Sweden. EM andreas.oestlin@physik.uni-augsburg.de RI Di Marco, Igor/O-5190-2014 OI Di Marco, Igor/0000-0003-1714-0942 FU Swedish Research Council; Swedish Foundation for Strategic Research; Hungarian Scientific Research Fund [OTKA 84078, 109570]; Knut and Alice Wallenberg Foundation FX We thank Borje Johansson, Bob Albers, Angus Lawson, and Jon Lawrence for helpful discussions. A.O. and L.V. acknowledge financial support from the Swedish Research Council, the Swedish Foundation for Strategic Research, and the Hungarian Scientific Research Fund (research projects OTKA 84078 and 109570). I.D.M. and I.L. acknowledge financial support from the Swedish Research Council and the Knut and Alice Wallenberg Foundation (research projects of Prof. Olle Eriksson). Computations were performed using resources provided by the Swedish National Infrastructure for Computing (SNIC) at the National Supercomputer Centre in Linkoping and at the PDC Center for High Performance Computing in Stockholm. Work at the Los Alamos National Laboratory was carried out under the auspices of the United States Department of Energy. NR 65 TC 0 Z9 0 U1 4 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 14 PY 2016 VL 93 IS 9 AR 094103 DI 10.1103/PhysRevB.93.094103 PG 8 WC Physics, Condensed Matter SC Physics GA DG9KA UT WOS:000372400100001 ER PT J AU Wagman, JJ Carlo, JP Gaudet, J Van Gastel, G Abernathy, DL Stone, MB Granroth, GE Kolesnikov, AI Savici, AT Kim, YJ Zhang, H Ellis, D Zhao, Y Clark, L Kallin, AB Mazurek, E Dabkowska, HA Gaulin, BD AF Wagman, J. J. Carlo, J. P. Gaudet, J. Van Gastel, G. Abernathy, D. L. Stone, M. B. Granroth, G. E. Kolesnikov, A. I. Savici, A. T. Kim, Y. J. Zhang, H. Ellis, D. Zhao, Y. Clark, L. Kallin, A. B. Mazurek, E. Dabkowska, H. A. Gaulin, B. D. TI Neutron scattering studies of spin-phonon hybridization and superconducting spin gaps in the high-temperature superconductor La2-x(Sr, Ba)(x)CuO4 SO PHYSICAL REVIEW B LA English DT Article ID LA2-XSRXCUO4; LA2CUO4; ANTIFERROMAGNETISM; FLUCTUATIONS; EXCITATIONS; TRANSITION; PURE AB We present time-of-flight neutron scattering measurements on single crystals of La2-xBaxCuO4 (LBCO) with 0 <= x <= 0.095 and La2-xSrxCuO4 (LSCO) with x = 0.08 and 0.11. This range of dopings spans much of the phase diagram relevant to high-temperature cuprate superconductivity, ranging from insulating, three-dimensional commensurate long-range antiferromagnetic order, for x <= 0.02, to two-dimensional (2D) incommensurate antiferromagnetism coexisting with superconductivity for x >= 0.05. Previous work on lightly doped LBCO with x = 0.035 showed a clear enhancement of the inelastic scattering coincident with the low-energy crossings of the highly dispersive spin excitations and quasi-2D optic phonons. The present work extends these measurements across the phase diagram and shows this enhancement to be a common feature to this family of layered quantum magnets. Furthermore, we show that the low-temperature, low-energy magnetic spectral weight is substantially larger for samples with nonsuperconducting ground states relative to any of the samples with superconducting ground states. Spin gaps, suppression of low-energy magnetic spectral weight as a function of decreasing temperature, are observed in both superconducting LBCO and LSCO samples, consistent with previous observations for superconducting LSCO. C1 [Wagman, J. J.; Carlo, J. P.; Gaudet, J.; Van Gastel, G.; Clark, L.; Kallin, A. B.; Mazurek, E.; Gaulin, B. D.] McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. [Carlo, J. P.] Villanova Univ, Dept Phys, Villanova, PA 19085 USA. [Abernathy, D. L.; Stone, M. B.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Granroth, G. E.; Savici, A. T.] Oak Ridge Natl Lab, Neutron Data Anal & Visualizat Div, Oak Ridge, TN 37831 USA. [Kolesnikov, A. I.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Kim, Y. J.; Zhang, H.; Ellis, D.] Univ Toronto, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada. [Zhao, Y.] NIST, Gaithersburg, MD 20899 USA. [Zhao, Y.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. [Dabkowska, H. A.; Gaulin, B. D.] McMaster Univ, Brockhouse Inst Mat Res, Hamilton, ON L8S 4M1, Canada. [Gaulin, B. D.] Canadian Inst Adv Res, 180 Dundas St West, Toronto, ON M5G 1Z8, Canada. RP Wagman, JJ (reprint author), McMaster Univ, Dept Phys & Astron, Hamilton, ON L8S 4M1, Canada. RI Granroth, Garrett/G-3576-2012; Stone, Matthew/G-3275-2011; Abernathy, Douglas/A-3038-2012; BL18, ARCS/A-3000-2012; OI Granroth, Garrett/0000-0002-7583-8778; Stone, Matthew/0000-0001-7884-9715; Abernathy, Douglas/0000-0002-3533-003X; Clark, Lucy/0000-0002-6223-3622 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Natural Sciences and Engineering Research Council of Canada FX We would like to acknowledge useful conversations had with N. Christensen, E. Taylor, J. P. Carbotte, T. Timusk, J. Tranquada, I. Zaliznyak, and D. Fobes. We would also like to acknowledge T. E. Sherline and L. DeBeer Schmidt for technical assistance with the measurements on SEQUOIA, J. Niedziela and D. Maharaj for technical assistance with the ARCS measurements, and E. McNeice for assistance with sample growth. Research using ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. Work at McMaster was funded by Natural Sciences and Engineering Research Council of Canada. NR 57 TC 0 Z9 0 U1 3 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 14 PY 2016 VL 93 IS 9 AR 094416 DI 10.1103/PhysRevB.93.094416 PG 8 WC Physics, Condensed Matter SC Physics GA DG9KA UT WOS:000372400100005 ER PT J AU Xu, ZJ Schneeloch, JA Wen, JS Bozin, ES Granroth, GE Winn, BL Feygenson, M Birgeneau, RJ Gu, GD Zaliznyak, IA Tranquada, JM Xu, GY AF Xu, Zhijun Schneeloch, J. A. Wen, Jinsheng Bozin, E. S. Granroth, G. E. Winn, B. L. Feygenson, M. Birgeneau, R. J. Gu, Genda Zaliznyak, I. A. Tranquada, J. M. Xu, Guangyong TI Thermal evolution of antiferromagnetic correlations and tetrahedral bond angles in superconducting FeTe1-xSex SO PHYSICAL REVIEW B LA English DT Article ID IRON ARSENIDE SUPERCONDUCTOR; MAGNETIC ORDER; SPIN DYNAMICS; NEMATICITY; CHALCOGENIDES; FESE; FRUSTRATION; ANISOTROPY; STATE AB It has recently been demonstrated that dynamical magnetic correlations measured by neutron scattering in iron chalcogenides can be described with models of short-range correlations characterized by particular choices of four-spin plaquettes, where the appropriate choice changes as the parent material is doped towards superconductivity. Here we apply such models to describe measured maps of magnetic scattering as a function of two-dimensional wave vectors obtained for optimally superconducting crystals of FeTe1-xSex. We show that the characteristic antiferromagnetic wave vector evolves from that of the bicollinear structure found in underdoped chalcogenides (at high temperature) to that associated with the stripe structure of antiferromagnetic iron arsenides (at low temperature); these can both be described with the same local plaquette, but with different interplaquette correlations. While the magnitude of the low-energy magnetic spectral weight is substantial at all temperatures, it actually weakens somewhat at low temperature, where the charge carriers become more itinerant. The observed change in spin correlations is correlated with the dramatic drop in the electronic scattering rate and the growth of the bulk nematic response upon cooling. Finally, we also present powder neutron diffraction results for lattice parameters in FeTe1-xSex indicating that the tetrahedral bond angle tends to increase towards the ideal value upon cooling, in agreement with the increased screening of the crystal field by more itinerant electrons and the correspondingly smaller splitting of the Fe 3d orbitals. C1 [Xu, Zhijun; Birgeneau, R. J.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Xu, Zhijun; Birgeneau, R. J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Schneeloch, J. A.; Bozin, E. S.; Gu, Genda; Zaliznyak, I. A.; Tranquada, J. M.; Xu, Guangyong] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [Schneeloch, J. A.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Wen, Jinsheng] Nanjing Univ, Natl Lab Solid State Microstruct, Ctr Superconducting Phys & Mat, Nanjing 210093, Jiangsu, Peoples R China. [Wen, Jinsheng] Nanjing Univ, Dept Phys, Nanjing 210093, Jiangsu, Peoples R China. [Granroth, G. E.] Oak Ridge Natl Lab, Neutron Data Anal & Visualizat Div, Oak Ridge, TN 37831 USA. [Winn, B. L.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Feygenson, M.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Xu, GY (reprint author), Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. EM gxu@bnl.gov RI Granroth, Garrett/G-3576-2012; Wen, Jinsheng/F-4209-2010; Tranquada, John/A-9832-2009; xu, zhijun/A-3264-2013; OI Granroth, Garrett/0000-0002-7583-8778; Wen, Jinsheng/0000-0001-5864-1466; Tranquada, John/0000-0003-4984-8857; xu, zhijun/0000-0001-7486-2015; Feygenson, Mikhail /0000-0002-0316-3265 FU Office of Basic Energy Sciences, US Department of Energy [DE-SC00112704, DE-AC02-05CH11231]; NSFC [11374143, NCET-13-0282]; Division of Scientific User Facilities of the same office FX We are grateful for stimulating discussions with Wei Ku, Ian Fisher, Adriana Moreo, Elbio Dagotto, and Ming Yi. The work at Brookhaven National Laboratory was supported by the Office of Basic Energy Sciences, US Department of Energy, under Contract No. DE-SC00112704. Z.J.X. and R.J.B. are also supported by the Office of Basic Energy Sciences, US Department of Energy, through Contract No. DE-AC02-05CH11231. Research at Oak Ridge National Laboratory was sponsored by the Division of Scientific User Facilities of the same office. The work at Nanjing University was supported by NSFC No. 11374143, and NCET-13-0282. NR 85 TC 0 Z9 0 U1 5 U2 23 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 14 PY 2016 VL 93 IS 10 AR 104517 DI 10.1103/PhysRevB.93.104517 PG 9 WC Physics, Condensed Matter SC Physics GA DG9LL UT WOS:000372404400008 ER PT J AU Kanazawa, K Koike, Y Metz, A Pitonyak, D Schlegel, M AF Kanazawa, Koichi Koike, Yuji Metz, Andreas Pitonyak, Daniel Schlegel, Marc TI Operator constraints for twist-3 functions and Lorentz invariance properties of twist-3 observables SO PHYSICAL REVIEW D LA English DT Article ID SINGLE-SPIN ASYMMETRIES; PROTON-PROTON COLLISIONS; DEEP-INELASTIC SCATTERING; DIRECT PHOTON PRODUCTION; DRELL-YAN PROCESS; PION-PRODUCTION; Q(2) EVOLUTION; PARTON DISTRIBUTIONS; HADRON-PRODUCTION; ANALYZING POWER AB We investigate the behavior under Lorentz transformations of perturbative coefficient functions in a collinear twist-3 formalism relevant for high-energy observables including transverse polarization of hadrons. We argue that those perturbative coefficient functions can, a priori, acquire quite different yet Lorentz-invariant forms in various frames. This somewhat surprising difference can be traced back to a general dependence of the perturbative coefficient functions on light cone vectors which are introduced by the twist-3 factorization formulas and which are frame-dependent. One can remove this spurious frame dependence by invoking so-called Lorentz invariance relations (LIRs) between twist-3 parton correlation functions. Some of those relations for twist-3 distribution functions were discussed in the literature before. In this paper we derive the corresponding LIRs for twist-3 fragmentation functions. We explicitly demonstrate that these LIRs remove the light cone vector dependence by considering transverse spin observables in the single-inclusive production of hadrons in lepton-nucleon collisions, lN -> hX. With the LIRs in hand, we also show that twist-3 observables in general can be written solely in terms of three-parton correlation functions. C1 [Kanazawa, Koichi; Metz, Andreas] Temple Univ, Dept Phys, SERC, Philadelphia, PA 19122 USA. [Koike, Yuji] Niigata Univ, Dept Phys, Ikarashi, Niigata 9502181, Japan. [Pitonyak, Daniel] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Schlegel, Marc] Univ Tubingen, Inst Theoret Phys, Morgenstelle 14, D-72076 Tubingen, Germany. RP Kanazawa, K; Metz, A (reprint author), Temple Univ, Dept Phys, SERC, Philadelphia, PA 19122 USA.; Koike, Y (reprint author), Niigata Univ, Dept Phys, Ikarashi, Niigata 9502181, Japan.; Pitonyak, D (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA.; Schlegel, M (reprint author), Univ Tubingen, Inst Theoret Phys, Morgenstelle 14, D-72076 Tubingen, Germany. EM tuf29138@temple.edu; koike@phys.sc.niigata-u.ac.jp; metza@temple.edu; dpitonyak@quark.phy.bnl.gov; marc.schlegel@uni-tuebingen.de FU National Science Foundation [PHY-1516088]; Japanese Society of Promotion of Science [26287040]; RIKEN BNL Research Center; Bundesministerium fur Bildung und Forschung (BMBF) [05P12VTCTG] FX K. K. thanks S. Yoshida for useful discussions during his stay at Niigata University. This work has been supported by the National Science Foundation under Contract No. PHY-1516088 (K. K. and A. M.), the Grant-in-Aid for Scientific Research from the Japanese Society of Promotion of Science under Contract No. 26287040 (Y. K.), the RIKEN BNL Research Center (D. P.), and the Bundesministerium fur Bildung und Forschung (BMBF) Grant No. 05P12VTCTG (M. S.). NR 109 TC 5 Z9 5 U1 1 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 14 PY 2016 VL 93 IS 5 AR 054024 DI 10.1103/PhysRevD.93.054024 PG 20 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG9PN UT WOS:000372416400002 ER PT J AU Johnson, WR Nilsen, J AF Johnson, W. R. Nilsen, J. TI Average-atom treatment of relaxation time in x-ray Thomson scattering from warm dense matter SO PHYSICAL REVIEW E LA English DT Article ID IONIZED CARBON PLASMAS; ANOMALOUS-DISPERSION; OPTICAL-PROPERTIES; CONDUCTION; METALS AB The influence of finite relaxation times on Thomson scattering from warm dense plasmas is examined within the framework of the average-atom approximation. Presently most calculations use the collision-free Lindhard dielectric function to evaluate the free-electron contribution to the Thomson cross section. In this work, we use the Mermin dielectric function, which includes relaxation time explicitly. The relaxation time is evaluated by treating the average atom as an impurity in a uniform electron gas and depends critically on the transport cross section. The calculated relaxation rates agree well with values inferred from the Ziman formula for the static conductivity and also with rates inferred from a fit to the frequency-dependent conductivity. Transport cross sections determined by the phase-shift analysis in the average-atom potential are compared with those evaluated in the commonly used Born approximation. The Born approximation converges to the exact cross sections at high energies; however, differences that occur at low energies lead to corresponding differences in relaxation rates. The relative importance of including relaxation time when modeling x-ray Thomson scattering spectra is examined by comparing calculations of the free-electron dynamic structure function for Thomson scattering using Lindhard and Mermin dielectric functions. Applications are given to warm dense Be plasmas, with temperatures ranging from 2 to 32 eV and densities ranging from 2 to 64 g/cc. C1 [Johnson, W. R.] Univ Notre Dame, Dept Phys, 225 Nieuwland Sci Hall, Notre Dame, IN 46556 USA. [Nilsen, J.] Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. RP Johnson, WR (reprint author), Univ Notre Dame, Dept Phys, 225 Nieuwland Sci Hall, Notre Dame, IN 46556 USA. EM johnson@nd.edu FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors are grateful to K. T. Cheng, T. Doppner, and D. Krause for helpful discussions. The work of one author (J.N.) was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 37 TC 0 Z9 0 U1 4 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD MAR 14 PY 2016 VL 93 IS 3 AR 033205 DI 10.1103/PhysRevE.93.033205 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DG9SB UT WOS:000372423000016 PM 27078473 ER PT J AU Detmold, W Orginos, K Parreno, A Savage, MJ Tiburzi, BC Beane, SR Chang, E AF Detmold, William Orginos, Kostas Parreno, Assumpta Savage, Martin J. Tiburzi, Brian C. Beane, Silas R. Chang, Emmanuel CA NPLQCD Collaboration TI Unitary Limit of Two-Nucleon Interactions in Strong Magnetic Fields SO PHYSICAL REVIEW LETTERS LA English DT Article ID NEUTRON-STARS; QCD AB Two-nucleon systems are shown to exhibit large scattering lengths in strong magnetic fields at unphysical quark masses, and the trends toward the physical values indicate that such features may exist in nature. Lattice QCD calculations of the energies of one and two nucleons systems are performed at pion masses of m(pi) similar to 450 and 806 MeV in uniform, time-independent magnetic fields of strength vertical bar B vertical bar similar to 10(19)-10(20) G to determine the response of these hadronic systems to large magnetic fields. Fields of this strength may exist inside magnetars and in peripheral relativistic heavy ion collisions, and the unitary behavior at large scattering lengths may have important consequences for these systems. C1 [Detmold, William] MIT, Ctr Theoret Phys, Cambridge, MA 02139 USA. [Orginos, Kostas] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Orginos, Kostas] Jefferson Lab, 12000 Jefferson Ave, Newport News, VA 23606 USA. [Parreno, Assumpta] Univ Barcelona, Dept Estruct & Constituents Mat, ICC, Marti Franques 1, E-08028 Barcelona, Spain. [Savage, Martin J.; Chang, Emmanuel] Univ Washington, Inst Nucl Theory, Seattle, WA 98195 USA. [Tiburzi, Brian C.] CUNY City Coll, Dept Phys, New York, NY 10031 USA. [Tiburzi, Brian C.] CUNY Grad Sch & Univ Ctr, New York, NY 10016 USA. [Tiburzi, Brian C.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Beane, Silas R.] Univ Washington, Dept Phys, Box 351560, Seattle, WA 98195 USA. RP Detmold, W (reprint author), MIT, Ctr Theoret Phys, Cambridge, MA 02139 USA. FU National Science Foundation [NSF PHY11-25915, OCI-1053575]; NERSC (U.S. Department of Energy) [DE-AC02-05CH11231]; USQCD; Office of Science of the U.S. Department of Energy [DE-AC05-00OR22725]; NSF [PHY1206498]; U.S. Department of Energy [DE-SC001347, DE-FG02-04ER41302, DE-AC05-06OR23177]; U.S. Department of Energy Early Career Research Award [DE-SC0010495]; MEC (Spain) [FIS2011-24154]; FEDER; DOE [DE-FG02-00ER41132]; joint City College of New York-RIKEN/Brookhaven Research Center fellowship; U.S. National Science Foundation [PHY15-15738]; Professional Staff Congress of the CUNY FX We would like to thank Zohreh Davoudi, Daekyoung Kang, and Krishna Rajagopal for several interesting discussions. This research was supported in part by the National Science Foundation under Grant No. NSF PHY11-25915 and W. D. and M. J. S. acknowledge the Kavli Institute for Theoretical Physics for hospitality during completion of this work. Calculations were performed using computational resources provided by the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation Grant No. OCI-1053575, NERSC (supported by U.S. Department of Energy Grant No. DE-AC02-05CH11231), and by the USQCD collaboration. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. The PRACE Research Infrastructure resources Curie based in France at the Tres Grand Centre de Calcul and MareNostrum-III based in Spain at the Barcelona Supercomputing Center were also used. Parts of the calculations used the Chroma software suite [32]. S. R. B. was partially supported by NSF continuing Grant No. PHY1206498 and by U.S. Department of Energy through Grant No. DE-SC001347. W. D. was partially supported by the U.S. Department of Energy Early Career Research Award DE-SC0010495. K. O. was partially supported by the U.S. Department of Energy through Grant No. DE-FG02-04ER41302 and through Contract No. DE-AC05-06OR23177 under which JSA operates the Thomas Jefferson National Accelerator Facility. The work of A. P. was supported by the contract FIS2011-24154 from MEC (Spain) and FEDER. M. J. S. was supported by DOE Grant No. DE-FG02-00ER41132. B. C. T. was supported in part by a joint City College of New York-RIKEN/Brookhaven Research Center fellowship, a grant from the Professional Staff Congress of the CUNY, and by the U.S. National Science Foundation, under Grant No. PHY15-15738. NR 29 TC 3 Z9 3 U1 1 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 14 PY 2016 VL 116 IS 11 AR 112301 DI 10.1103/PhysRevLett.116.112301 PG 5 WC Physics, Multidisciplinary SC Physics GA DG9VH UT WOS:000372431400001 PM 27035294 ER PT J AU Wang, HW Wen, JG Miller, DJ Zhou, QB Chen, M Lee, HN Rabe, KM Wu, XF AF Wang, Hongwei Wen, Jianguo Miller, Dean J. Zhou, Qibin Chen, Mohan Lee, Ho Nyung Rabe, Karin M. Wu, Xifan TI Stabilization of Highly Polar BiFeO3-like Structure: A New Interface Design Route for Enhanced Ferroelectricity in Artificial Perovskite Superlattices SO PHYSICAL REVIEW X LA English DT Article ID POLARIZATION ENHANCEMENT; THIN-FILMS AB In ABO(3) perovskites, oxygen octahedron rotations are common structural distortions that can promote large ferroelectricity in BiFeO3 with an R3c structure [1] but suppress ferroelectricity in CaTiO3 with a Pbnm symmetry [2]. For many CaTiO3-like perovskites, the BiFeO3 structure is a metastable phase. Here, we report the stabilization of the highly polar BiFeO3-like phase of CaTiO3 in a BaTiO(3/)CaTiO3 superlattice grown on a SrTiO3 substrate. The stabilization is realized by a reconstruction of oxygen octahedron rotations at the interface from the pattern of nonpolar bulk CaTiO3 to a different pattern that is characteristic of a BiFeO3 phase. The reconstruction is interpreted through a combination of amplitude-contrast sub-0.1-nm high-resolution transmission electron microscopy and first-principles theories of the structure, energetics,and polarization of the superlattice and its constituents. We further predict a number of new artificial ferroelectric materials demonstrating that nonpolar perovskites can be turned into ferroelectrics via this interface mechanism. Therefore, a large number of perovskites with the CaTiO3 structure type, which include many magnetic representatives, are now good candidates as novel highly polar multiferroic materials [3]. C1 [Wang, Hongwei; Wu, Xifan] Temple Univ, Dept Phys, Philadelphia, PA 19122 USA. [Wen, Jianguo; Miller, Dean J.] Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. [Zhou, Qibin; Rabe, Karin M.] Rutgers State Univ, Dept Phys & Astron, POB 849, Piscataway, NJ 08854 USA. [Chen, Mohan] Princeton Univ, Dept Mech & Aerosp Engn, Princeton, NJ 08544 USA. [Lee, Ho Nyung] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Wu, XF (reprint author), Temple Univ, Dept Phys, Philadelphia, PA 19122 USA.; Wen, JG (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. RI Lee, Ho Nyung/K-2820-2012; Chen, Mohan/F-4621-2017 OI Lee, Ho Nyung/0000-0002-2180-3975; Chen, Mohan/0000-0002-8071-5633 FU Center for the Computational Design of Functional Layered Materials, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0012575]; DOE-BES [DE-AC02-06CH11357]; UChicago Argonne, LLC; National Science Foundation (NSF) [DMR-1334428]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This research was primarily supported as part of the Center for the Computational Design of Functional Layered Materials, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award No. DE-SC0012575 (the main ideas, theoretical models, calculations, and the analysis), by DOE-BES Facility supported under Contract No. DE-AC02-06CH11357 by UChicago Argonne, LLC (transmission electron microscopy measurement), by National Science Foundation (NSF) under Award No. DMR-1334428 (some of the first-principles calculations), and by U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division (superlattice synthesis). This research used resources of the National Energy Research Scientific Computing Center (NERSC), a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We thank Dr. Hua Zhou for useful discussions. X. W. is grateful for the useful discussions with Dr. Andrew J. Shanahan at University Medical Center of Princeton. NR 37 TC 0 Z9 0 U1 16 U2 50 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2160-3308 J9 PHYS REV X JI Phys. Rev. X PD MAR 14 PY 2016 VL 6 IS 1 AR 011027 DI 10.1103/PhysRevX.6.011027 PG 8 WC Physics, Multidisciplinary SC Physics GA DG9UN UT WOS:000372429400001 ER PT J AU Kumar, GR Savariraj, AD Karthick, SN Selvam, S Balamuralitharan, B Kim, HJ Viswanathan, KK Vijaykumar, M Prabakar, K AF Kumar, G. Rajendra Savariraj, A. Dennyson Karthick, S. N. Selvam, S. Balamuralitharan, B. Kim, Hee-Je Viswanathan, K. K. Vijaykumar, M. Prabakar, Kandasamy TI Phase transition kinetics and surface binding states of methylammonium lead iodide perovskite SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID HETEROJUNCTION SOLAR-CELLS; SEQUENTIAL DEPOSITION; HALIDE PEROVSKITES; CHARGE-TRANSPORT; LOW-COST; EFFICIENCY; SIZE; CH3NH3PBI3; SEMICONDUCTOR; FILMS AB We have presented a detailed analysis of the phase transition kinetics and binding energy states of solution processed methylammonium lead iodide (MAPbI(3)) thin films prepared at ambient conditions and annealed at different elevated temperatures. It is the processing temperature and environmental conditions that predominantly control the crystal structure and surface morphology of MAPbI3 thin films. The structural transformation from tetragonal to cubic occurs at 60 degrees C with a 30 minute annealing time while the 10 minute annealed films posses a tetragonal crystal structure. The transformed phase is greatly intact even at the higher annealing temperature of 150 degrees C and after a time of 2 hours. The charge transfer interaction between the Pb 4f and I 3d oxidation states is quantified using XPS. C1 [Kumar, G. Rajendra; Savariraj, A. Dennyson; Karthick, S. N.; Selvam, S.; Balamuralitharan, B.; Kim, Hee-Je; Prabakar, Kandasamy] Pusan Natl Univ, Dept Elect & Comp Engn, San 30, Busan 609735, South Korea. [Viswanathan, K. K.] Univ Teknol Malaysia, Fac Sci, Dept Math Sci, UTM Ctr Ind & Appl Math,Ibnu Sina Inst Sci & Ind, Johor Baharu 81310, Johor, Malaysia. [Vijaykumar, M.; Prabakar, Kandasamy] Pacific Northwest Natl Lab, Richland, WA 99354 USA. RP Prabakar, K (reprint author), Pusan Natl Univ, Dept Elect & Comp Engn, San 30, Busan 609735, South Korea.; Prabakar, K (reprint author), Pacific Northwest Natl Lab, Richland, WA 99354 USA. EM prabakar@pusan.ac.kr OI Gunasekaran, Rajendra Kumar/0000-0003-1360-0083 FU Basic Science Research Program through a National Research Foundation of Korea (NRF) grant - Korean government [2014005051] FX This work was supported by the Basic Science Research Program through a National Research Foundation of Korea (NRF) grant funded by the Korean government (No. 2014005051). NR 50 TC 2 Z9 2 U1 19 U2 66 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAR 14 PY 2016 VL 18 IS 10 BP 7284 EP 7292 DI 10.1039/c5cp06232b PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DF8LF UT WOS:000371608600038 ER PT J AU Dau, PD Armentrout, PB Michelini, MC Gibson, JK AF Dau, Phuong D. Armentrout, P. B. Michelini, Maria C. Gibson, John K. TI Activation of carbon dioxide by a terminal uranium-nitrogen bond in the gas-phase: a demonstration of the principle of microscopic reversibility SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID GUIDED ION-BEAM; SMALL-MOLECULE ACTIVATION; TRANSITION-METAL; BASIS-SETS; CO2; COMPLEXES; REACTIVITY; ENERGY; URANYL; OXIDATION AB Activation of CO2 is demonstrated by its spontaneous dissociative reaction with the gas-phase anion complex NUOCl2-, which can be considered as NUO+ coordinated by two chloride anion ligands. This reaction was previously predicted by density functional theory to occur exothermically, without barriers above the reactant energy. The present results demonstrate the validity of the prediction of microscopic reversibility, and provide a rare case of spontaneous dissociative addition of CO2 to a gas-phase complex. The activation of CO2 by NUOCl2- proceeds by conversion of a URN bond to a U=O bond and creation of an isocyanate ligand to yield the complex UO2(NCO)Cl-2(-), in which uranyl, UO22+, is coordinated by one isocyanate and two chloride anion ligands. This activation of CO2 by a uranium( VI) nitride complex is distinctive from previous reports of oxidative insertion of CO2 into lower oxidation state U(III) or U(IV) solid complexes, during which both C-O bonds remain intact. This unusual observation of spontaneous addition and activation of CO2 by NUOCl2- is a result of the high oxophilicity of uranium. If the computed Gibbs free energy of the reaction pathway, rather than the energy, is considered, there are barriers above the reactant asymptotes such that the observed reaction should not proceed under thermal conditions. This result provides a demonstration that energy rather than Gibbs free energy determines reactivity under low-pressure bimolecular conditions. C1 [Dau, Phuong D.; Gibson, John K.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Armentrout, P. B.] Univ Utah, Dept Chem, Salt Lake City, UT 84112 USA. [Michelini, Maria C.] Univ Calabria, Dipartimento Chim, I-87030 Arcavacata Di Rende, Italy. RP Gibson, JK (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM jkgibson@lbl.gov FU U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry Program, at LBNL [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry Program, at the University of Utah [DE-SC0012249]; Universita della Calabria, Italy; Office of Science of the U.S. D.O.E. [DE-AC02-05CH11231] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Heavy Element Chemistry Program, at LBNL under Contract No. DE-AC02-05CH11231 (P. D. D. and J. K. G.) and at the University of Utah by grant no. DE-SC0012249 (P. B. A.), and by Universita della Calabria, Italy (M. C. M.). This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. D.O.E. under Contract No. DE-AC02-05CH11231. NR 64 TC 4 Z9 4 U1 11 U2 33 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAR 14 PY 2016 VL 18 IS 10 BP 7334 EP 7340 DI 10.1039/c6cp00494f PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DF8LF UT WOS:000371608600043 PM 26898535 ER PT J AU Halliday, MTE Hess, WP Shluger, AL AF Halliday, M. T. E. Hess, W. P. Shluger, A. L. TI A mechanism of Cu work function reduction in CsBr/Cu photocathodes SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID SPACE GAUSSIAN PSEUDOPOTENTIALS; MINIMUM ENERGY PATHS; ELASTIC BAND METHOD; ALKALI HALIDES; SADDLE-POINTS; SURFACE; COEFFICIENTS; DESORPTION; ROUGHNESS; CRYSTAL AB Thin films of CsBr deposited on Cu(100) have been proposed as next-generation photocathode materials for applications in particle accelerators and free-electron lasers. However, the mechanisms underlying an improved photocathode performance as well as their long-term stability remain poorly understood. We present Density Functional Theory (DFT) calculations of the work function reduction following the application of CsBr thin film coatings to Cu photocathodes. The effects of both flat and rough interface and van der Waals forces are examined. Calculations suggest that CsBr films can reduce the Cu(100) work function by about 1.5 eV, which would explain the observed increase in quantum efficiency (QE) of coated vs. uncoated photocathodes. A model explaining the experimentally observed laser activation of photocathodes is provided whereby the photo-induced creation of Br vacancies and Cs-Br di-vacancies and their subsequent diffusion to the Cu/CsBr interface lead to a further increase in QE after a period of laser irradiation. C1 [Halliday, M. T. E.; Shluger, A. L.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Halliday, M. T. E.; Shluger, A. L.] UCL, London Ctr Nanotechnol, London WC1E 6BT, England. [Hess, W. P.] Pacific NW Natl Lab, Div Phys Sci, POB 999, Richland, WA 99352 USA. RP Halliday, MTE (reprint author), UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England.; Halliday, MTE (reprint author), UCL, London Ctr Nanotechnol, London WC1E 6BT, England. EM a.shluger@ucl.ac.uk FU EPSRC [EP/F067496]; US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences FX MTEH is grateful to EPSRC for financial support. WPH acknowledge support from the US Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences and Biosciences. Pacific Northwest National Laboratory is a multiprogram national laboratory operated for DOE by Battelle. Our access to the Archer facility is provided via our membership of the UK's HPC Materials Chemistry Consortium, which is funded by EPSRC grant EP/F067496. We are grateful to T. Durrant for useful discussions and help in calculations. NR 53 TC 0 Z9 0 U1 4 U2 16 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAR 14 PY 2016 VL 18 IS 10 BP 7427 EP 7434 DI 10.1039/c5cp07694c PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DF8LF UT WOS:000371608600055 PM 26899524 ER PT J AU Zhong, XL Rungger, I Zapol, P Nakamura, H Asai, Y Heinonen, O AF Zhong, Xiaoliang Rungger, Ivan Zapol, Peter Nakamura, Hisao Asai, Yoshihiro Heinonen, Olle TI The effect of a Ta oxygen scavenger layer on HfO2-based resistive switching behavior: thermodynamic stability, electronic structure, and low-bias transport SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article AB Reversible resistive switching between high-resistance and low-resistance states in metal-oxide-metal heterostructures makes them very interesting for applications in random access memories. While recent experimental work has shown that inserting a metallic "oxygen scavenger layer'' between the positive electrode and oxide improves device performance, the fundamental understanding of how the scavenger layer modifies the heterostructure properties is lacking. We use density functional theory to calculate thermodynamic properties and conductance of TiN/HfO2/TiN heterostructures with and without a Ta scavenger layer. First, we show that Ta insertion lowers the formation energy of low-resistance states. Second, while the Ta scavenger layer reduces the Schottky barrier height in the high-resistance state by modifying the interface charge at the oxide-electrode interface, the heterostructure maintains a high resistance ratio between high-and low-resistance states. Finally, we show that the low-bias conductance of device on-states becomes much less sensitive to the spatial distribution of oxygen removed from the HfO2 in the presence of the Ta layer. By providing a fundamental understanding of the observed improvements with scavenger layers, we open a path to engineer interfaces with oxygen scavenger layers to control and enhance device performance. In turn, this may enable the realization of a non-volatile low-power memory technology with concomitant reduction in energy consumption by consumer electronics and offering significant benefits to society. C1 [Zhong, Xiaoliang; Zapol, Peter; Heinonen, Olle] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. [Rungger, Ivan] Natl Phys Lab, Div Mat, Teddington TW11 0LW, Middx, England. [Nakamura, Hisao; Asai, Yoshihiro] Natl Inst Adv Ind Sci & Technol, Res Ctr Computat Design Adv Funct Mat CD FMat, Cent 2,Umezono 1-1-1, Tsukuba, Ibaraki 3058568, Japan. [Heinonen, Olle] Northwestern Univ, Northwestern Argonne Inst Sci & Engn, 2145 Sheridan Rd, Evanston, IL 60208 USA. RP Heinonen, O (reprint author), Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA.; Heinonen, O (reprint author), Northwestern Univ, Northwestern Argonne Inst Sci & Engn, 2145 Sheridan Rd, Evanston, IL 60208 USA. EM heinonen@anl.gov RI Zhong, Xiaoliang/B-2220-2012; OI Heinonen, Olle/0000-0002-3618-6092 FU U. S. DOE, Office of Science [DE-AC02-06CH11357]; European Union FX The work by X. Z., P. Z. and O. H. was supported by U. S. DOE, Office of Science under contract No. DE-AC02-06CH11357. I. R. acknowledges financial support from the European Union's Horizon2020 research and innovation programme within the PETMEM project. We gratefully acknowledge the computing resources provided for Blues and Fusion, high-performance computing clusters operated by the Laboratory Computing Resource Center at Argonne National Laboratory. (C) Queen's Printer and Controller of HMSO. NR 34 TC 4 Z9 4 U1 5 U2 23 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD MAR 14 PY 2016 VL 18 IS 10 BP 7502 EP 7510 DI 10.1039/c6cp00450d PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DF8LF UT WOS:000371608600064 PM 26902598 ER PT J AU Csanak, G Inal, MK Fontes, CJ Kilcrease, DP AF Csanak, G. Inal, M. K. Fontes, C. J. Kilcrease, D. P. TI The creation, destruction, and transfer of multipole moments in electron-ion three-body recombination using the Gell-Mann-Goldberger-Watson method SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE three-body recombination; multipole moments; electron-ion collisions; magnetic sublevels ID KINETIC-THEORY; SCATTERING; POLARIZATION; BEAM AB We use the Gell-Mann-Goldberger-Watson (GGW) method to further develop and elaborate on our earlier investigation of electron-ion three-body scattering. The GGW method is used to obtain multipole moment creation, destruction, and transfer rate formulae by the three-body recombination of electrons with ions assuming short-range interaction potentials. This approach leads to the derivation of the rate coefficient formula obtained previously via the alternative wave-packet propagation method. We show how to include exchange effects into the formalism, allowing extension of its validity to lower incident electron energies, and also introduce the Liouville-space formulation. Furthermore, we indicate that this method makes the relevance of the formulae to relativistic systems more transparent, demonstrating its validity for high incident electron energies and heavy ions. The Liouville-space formulation is used to facilitate the derivation of a selection rule for the rate coefficients for cylindrically symmetric plasmas, which is of practical importance for the proper formulation of population-alignment collisional-radiative modeling. C1 [Csanak, G.; Kilcrease, D. P.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. [Inal, M. K.] Univ Tlemcen, Fac Sci, Dept Phys, Tilimsen 13000, Algeria. [Fontes, C. J.] Los Alamos Natl Lab, Computat Phys Div, POB 1663, Los Alamos, NM 87545 USA. RP Inal, MK (reprint author), Univ Tlemcen, Fac Sci, Dept Phys, Tilimsen 13000, Algeria. EM cjf@lanl.gov OI Kilcrease, David/0000-0002-2319-5934 FU National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory; Algerian Ministry of Higher Education and Scientific Research [CNEPRU/D02020140022]; [DE-AC52-06NA25396] FX We would like to acknowledge Dr. P. Hakel for helpful discussions concerning potential applications of this work. This work was carried out in part under the auspices of the National Nuclear Security Administration of the US Department of Energy at Los Alamos National Laboratory and supported by contract no DE-AC52-06NA25396. One of us (MKI) gratefully acknowledges support from the Algerian Ministry of Higher Education and Scientific Research (CNEPRU/D02020140022). NR 33 TC 0 Z9 0 U1 0 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD MAR 14 PY 2016 VL 49 IS 5 AR 055202 DI 10.1088/0953-4075/49/5/055202 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DE4LS UT WOS:000370601400005 ER PT J AU Li, Y Pindzola, MS Colgan, J AF Li, Y. Pindzola, M. S. Colgan, J. TI Five-photon double ionization of helium SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE ionization; radiation; cross section AB A time-dependent close-coupling method is used to calculate the five-photon double ionization of He. It is found that the generalized cross section used in the past for two-photon double ionization of He cannot be extended to five-photon double ionization of He. Therefore only five-photon double ionization probabilities that depend on specific radiation field pulses can be calculated. C1 [Li, Y.; Pindzola, M. S.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Colgan, J.] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM USA. RP Li, Y (reprint author), Auburn Univ, Dept Phys, Auburn, AL 36849 USA. EM yzl0060@auburn.edu FU US National Science Foundation; US Department of Energy FX This work was supported in part by grants from the US National Science Foundation and the US Department of Energy. Computational work was carried out at the National Energy Research Scientific Computing Center (NERSC). NR 14 TC 2 Z9 2 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD MAR 14 PY 2016 VL 49 IS 5 AR 055401 DI 10.1088/0953-4075/49/5/055401 PG 5 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DE4LS UT WOS:000370601400008 ER PT J AU Menssen, A Trevisan, CS Schoffler, MS Jahnke, T Bocharova, I Sturm, F Gehrken, N Gaire, B Gassert, H Zeller, S Voigtsberger, J Kuhlins, A Trinter, F Gatton, A Sartor, J Reedy, D Nook, C Berry, B Zohrabi, M Kalinin, A Ben-Itzhak, I Belkacem, A Dorner, R Weber, T Landers, AL Rescigno, TN McCurdy, CW Williams, JB AF Menssen, A. Trevisan, C. S. Schoffler, M. S. Jahnke, T. Bocharova, I. Sturm, F. Gehrken, N. Gaire, B. Gassert, H. Zeller, S. Voigtsberger, J. Kuhlins, A. Trinter, F. Gatton, A. Sartor, J. Reedy, D. Nook, C. Berry, B. Zohrabi, M. Kalinin, A. Ben-Itzhak, I. Belkacem, A. Dorner, R. Weber, T. Landers, A. L. Rescigno, T. N. McCurdy, C. W. Williams, J. B. TI Molecular frame photoelectron angular distributions for core ionization of ethane, carbon tetrafluoride and 1,1-difluoroethylene SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE molecular photoionization; angular distribution; MFPAD ID DYNAMICS; PHOTOIONIZATION; FRAGMENTATION; ELECTRONS; REGION AB Molecular frame photoelectron angular distributions (MFPADs) are measured in electron-ion momentum imaging experiments and compared with complex Kohn variational calculations for carbon K-shell ionization of carbon tetrafluoride (CF4), ethane (C2H6) and 1,1-difluoroethylene (C2H2F2). While in ethane the polarization averaged MFPADs show a tendency at low energies for the photoelectron to be emitted in the directions of the bonds, the opposite effect is seen in CF4. A combination of these behaviors is seen in difluoroethylene where ionization from the two carbons can be distinguished experimentally because of their different K-shell ionization potentials. Excellent agreement is found between experiment and simple static-exchange or coupled two-channel theoretical calculations. However, simple electrostatics do not provide an adequate explanation of the suggestively simple angular distributions at low electron ejection energies. C1 [Menssen, A.; Schoffler, M. S.; Jahnke, T.; Gehrken, N.; Gassert, H.; Zeller, S.; Voigtsberger, J.; Kuhlins, A.; Trinter, F.; Kalinin, A.; Dorner, R.; Williams, J. B.] Goethe Univ Frankfurt, Inst Kernphys, Max von Laue Str 1, D-60438 Frankfurt, Germany. [Trevisan, C. S.] Calif State Univ, Maritime Acad, Dept Sci & Math, Vallejo, CA 94590 USA. [Menssen, A.; Bocharova, I.; Sturm, F.; Gaire, B.; Belkacem, A.; Weber, T.; Rescigno, T. N.; McCurdy, C. W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem Sci, Berkeley, CA 94720 USA. [Gatton, A.; Sartor, J.; Reedy, D.; Nook, C.; Landers, A. L.] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Berry, B.; Zohrabi, M.; Ben-Itzhak, I.] Kansas State Univ, JR McDonald Lab, Manhattan, KS 66506 USA. [McCurdy, C. W.] Univ Calif Davis, Dept Chem, Davis, CA 95616 USA. RP Menssen, A (reprint author), Goethe Univ Frankfurt, Inst Kernphys, Max von Laue Str 1, D-60438 Frankfurt, Germany.; Menssen, A (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Chem Sci, Berkeley, CA 94720 USA. RI Doerner, Reinhard/A-5340-2008; Schoeffler, Markus/B-6261-2008 OI Doerner, Reinhard/0000-0002-3728-4268; Schoeffler, Markus/0000-0001-9214-6848 FU German Academic Exchange Service (DAAD); German Research Foundation (DFG); US Department of Energy [DE-AC02-05CH11231]; US DOE Office of Basic Energy Sciences, Division of Chemical Sciences; US DOE Office of Basic Energy Sciences, Division of Chemical Sciences [DE-FG02-10ER16146]; US Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Visiting Faculty Program (VFP); Office of Science of the US Department of Energy [DE-AC02-05CH11231]; [DE-FG02-86ER13491] FX We acknowledge the financial support of the German Academic Exchange Service (DAAD) and the German Research Foundation (DFG). Work at the University of California, Lawrence Berkeley National Laboratory was performed under the auspices of the US Department of Energy under Contract No. DE-AC02-05CH11231 and was supported by the US DOE Office of Basic Energy Sciences, Division of Chemical Sciences. Work at Auburn University was supported by the US DOE Office of Basic Energy Sciences, Division of Chemical Sciences under grant number DE-FG02-10ER16146. The Kansas State University personnel were supported by grant number DE-FG02-86ER13491 from the same funding agency. One of us (CST) was supported by the US Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Visiting Faculty Program (VFP). This research used the Advanced Light Source and resources of the National Energy Research Scientific Computing Center, DOE Office of Science User Facilities supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. We thank the staff of the Advanced Light Source, in particular beamline 11.0.2 scientists H Bluhm and T Tyliszczak for outstanding support. NR 29 TC 0 Z9 0 U1 4 U2 13 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD MAR 14 PY 2016 VL 49 IS 5 AR 055203 DI 10.1088/0953-4075/49/5/055203 PG 11 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DE4LS UT WOS:000370601400006 ER PT J AU Shivaram, N Tong, XM Timmers, H Sandhu, A AF Shivaram, Niranjan Tong, Xiao-Min Timmers, Henry Sandhu, Arvinder TI Attosecond quantum-beat spectroscopy in helium SO JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS LA English DT Article DE attosecond; femtosecond; wavepacket; quantum beat; photoelectron; helium ID ABOVE-THRESHOLD-IONIZATION; ELECTRON WAVE-PACKETS; PULSE TRAINS; LASER-PULSES; DYNAMICS; TIME AB The evolution of electron wavepackets determines the course of many physical and chemical phenomena, and attosecond spectroscopy aims to measure and control such dynamics in real time. Here, we investigate radial electron wavepacket motion in helium by using an XUV attosecond pulse train to prepare a coherent superposition of excited states and a delayed femtosecond IR pulse to ionize them. Quantum-beat signals observed in the high resolution photoelectron spectrogram allow us to follow the field-free evolution of the bound electron wavepacket and determine the time-dependent ionization dynamics of the low-lying 2p state. C1 [Shivaram, Niranjan; Timmers, Henry; Sandhu, Arvinder] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Tong, Xiao-Min] Univ Tsukuba, Grad Sch Pure & Appl Sci, Tsukuba, Ibaraki 3058573, Japan. [Tong, Xiao-Min] Univ Tsukuba, Ctr Computat Sci, Tsukuba, Ibaraki 3058573, Japan. [Shivaram, Niranjan] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. RP Shivaram, N (reprint author), Univ Arizona, Dept Phys, Tucson, AZ 85721 USA.; Shivaram, N (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM nhshivaram@lbl.gov RI Tong, Xiao-Min/A-2748-2011; OI Tong, Xiao-Min/0000-0003-4898-3491; Shivaram, Niranjan/0000-0002-9550-3588 FU National Science Foundation (NSF) [PHY-1505556]; Japan Society for the Promotion of Science [C24540421]; HA-PACS (Highly Accelerated Parallel Advanced System for Computational Sciences) FX This work was supported by the National Science Foundation (NSF) under contract PHY-1505556. XMT was supported by a Grant-in-Aid for Scientific Research (C24540421) from the Japan Society for the Promotion of Science and the HA-PACS (Highly Accelerated Parallel Advanced System for Computational Sciences) Project for advanced interdisciplinary computational sciences by exascale computing technology. NR 29 TC 1 Z9 1 U1 3 U2 14 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-4075 EI 1361-6455 J9 J PHYS B-AT MOL OPT JI J. Phys. B-At. Mol. Opt. Phys. PD MAR 14 PY 2016 VL 49 IS 5 AR 055601 DI 10.1088/0953-4075/49/5/055601 PG 7 WC Optics; Physics, Atomic, Molecular & Chemical SC Optics; Physics GA DE4LS UT WOS:000370601400012 ER PT J AU Singh, RK Galvin, JE Sun, X AF Singh, Rajesh K. Galvin, Janine E. Sun, Xin TI Three-dimensional simulation of rivulet and film flows over an inclined plate: Effects of solvent properties and contact angle SO CHEMICAL ENGINEERING SCIENCE LA English DT Article DE VOF; Film flow; Rivulet flow; Interfacial area; Structure packing and contact angle ID THIN LIQUID-FILMS; STRUCTURED PACKING; SURFACE-TENSION; MASS-TRANSFER; PACKED-COLUMNS; GAS-LIQUID; DISTILLATION-COLUMNS; FLUID-DYNAMICS; CFD SIMULATION; FALLING FILMS AB We numerically investigated the film flow down an inclined plate using the volume of fluid (VOF) method. The flow simulations have been systematically carried out for a wide range of parameters, such as inlet size, inclination angle, contact angle, flow rates and solvent properties (viscosity and surface tension). Based on the simulation results, scaling theory is proposed for both interfacial area and for film thickness in terms of the Kapitza number (Ka).The Kapitza number is advantageous because it depends only on solvent properties. The Kapitza number decreases with increased solvent viscosity and is fixed for a given fluid. To investigate the effects of solvent properties on interfacial area a small inlet cross-section was used. The interfacial area decreases with increased value of Ka. The time to reach pseudo steady state of rivulet is also observed to increase with decreasing Ka. For a fixed flow rate, the inlet cross-section has marginal effect on the interfacial area; however, the developed width of the rivulet remains unchanged. In addition to inlet size, flow rate and solvent properties, the impact of contact angle on film thickness and interfacial area was also investigated. The contact angle has negligible effect for a fully wetted plate, but it significantly affects the interfacial area of the rivulet. A scaling theory for interfacial area in terms of the contact angle and Ka is presented. (C) 2015 Elsevier Ltd. All rights reserved. C1 [Singh, Rajesh K.; Galvin, Janine E.] Natl Energy Technol Lab, Computat Sci & Engn Div, Albany, OR 97321 USA. [Singh, Rajesh K.] Natl Energy Technol Lab, Albany, OR 97321 USA. [Sun, Xin] Pacific NW Natl Lab, Computat Sci Directorate, Richland, WA 99352 USA. RP Singh, RK (reprint author), Natl Energy Technol Lab, Computat Sci & Engn Div, Albany, OR 97321 USA. EM rajesh-kumar.singh@netl.doe.gov FU Office of Fossil Energy, U.S. Department of Energy, through Carbon Capture Simulation Initiative (CCSI) FX This research was supported in part by an appointment to the National Energy Technology Laboratory Research Participation Program, sponsored by the Office of Fossil Energy, U.S. Department of Energy, through Carbon Capture Simulation Initiative (CCSI) and administered by the Oak Ridge Institute for Science and Education. Authors would also like to thank Prof. Sankaran Sundaresan, Princeton University, for his valuable inputs and discussion on the project. NR 72 TC 0 Z9 0 U1 13 U2 28 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0009-2509 EI 1873-4405 J9 CHEM ENG SCI JI Chem. Eng. Sci. PD MAR 13 PY 2016 VL 142 BP 244 EP 257 DI 10.1016/j.ces.2015.11.029 PG 14 WC Engineering, Chemical SC Engineering GA DC2TE UT WOS:000369068500021 ER PT J AU Kanukollu, S Voget, S Pohlner, M Vandieken, V Petersen, J Kyrpides, NC Woyke, T Shapiro, N Goker, M Klenk, HP Cypionka, H Engelen, B AF Kanukollu, Saranya Voget, Sonja Pohlner, Marion Vandieken, Verona Petersen, Joern Kyrpides, Nikos C. Woyke, Tanja Shapiro, Nicole Goeker, Markus Klenk, Hans-Peter Cypionka, Heribert Engelen, Bert TI Genome sequence of Shimia str. SK013, a representative of the Roseobacter group isolated from marine sediment SO STANDARDS IN GENOMIC SCIENCES LA English DT Article DE Anaerobic metabolism; Cell-connecting filaments; Quorum quenching; Flagella gene cluster; DMSP; DMSO reductase; Denitrification ID HOMOSERINE LACTONE ACYLASE; ESCHERICHIA-COLI K-12; SP-NOV.; EMENDED DESCRIPTION; RNA GENES; BACTERIA; SYSTEM; CLADE; IDENTIFICATION; ANNOTATION AB Shimia strain SK013 is an aerobic, Gram-negative, rod shaped alphaproteobacterium affiliated with the Roseobacter group within the family Rhodobacteraceae. The strain was isolated from surface sediment (0-1 cm) of the Skagerrak at 114 m below sea level. The 4,049,808 bp genome of Shimia str. SK013 comprises 3,981 protein-coding genes and 47 RNA genes. It contains one chromosome and no extrachromosomal elements. The genome analysis revealed the presence of genes for a dimethylsulfoniopropionate lyase, demethylase and the trimethylamine methyltransferase (mttB) as well as genes for nitrate, nitrite and dimethyl sulfoxide reduction. This indicates that Shimia str. SK013 is able to switch from aerobic to anaerobic metabolism and thus is capable of aerobic and anaerobic sulfur cycling at the seafloor. Among the ability to convert other sulfur compounds it has the genetic capacity to produce climatically active dimethyl sulfide. Growth on glutamate as a sole carbon source results in formation of cell-connecting filaments, a putative phenotypic adaptation of the surface-associated strain to the environmental conditions at the seafloor. Genome analysis revealed the presence of a flagellum (fla1) and a type IV pilus biogenesis, which is speculated to be a prerequisite for biofilm formation. This is also related to genes responsible for signalling such as N-acyl homoserine lactones, as well as quip-genes responsible for quorum quenching and antibiotic biosynthesis. Pairwise similarities of 16S rRNA genes (98.56 % sequence similarity to the next relative S. haliotis) and the in silico DNA-DNA hybridization (21.20 % sequence similarity to S. haliotis) indicated Shimia str. SK013 to be considered as a new species. The genome analysis of Shimia str. SK013 offered first insights into specific physiological and phenotypic adaptation mechanisms of Roseobacter-affiliated bacteria to the benthic environment. C1 [Kanukollu, Saranya; Pohlner, Marion; Vandieken, Verona; Cypionka, Heribert; Engelen, Bert] Inst Chem & Biol Marine Environm ICBM, Oldenburg, Germany. [Voget, Sonja] Univ Gottingen, Dept Genom & Appl Microbiol, D-37073 Gottingen, Germany. [Voget, Sonja] Univ Gottingen, Inst Microbiol & Genet, Gottingen Genom Lab, D-37073 Gottingen, Germany. [Petersen, Joern; Goeker, Markus] Leibniz Inst DSMZ German Collect Microorganisms &, Braunschweig, Germany. [Kyrpides, Nikos C.; Woyke, Tanja; Shapiro, Nicole] Joint Genome Inst, Genome Biol Program, Dept Energy, Walnut Creek, CA USA. [Kyrpides, Nikos C.] King Abdulaziz Univ, Fac Sci, Dept Biol Sci, Jeddah 21413, Saudi Arabia. [Klenk, Hans-Peter] Newcastle Univ, Sch Biol, Newcastle Upon Tyne NE1 7RU, Tyne & Wear, England. RP Engelen, B (reprint author), Inst Chem & Biol Marine Environm ICBM, Oldenburg, Germany. EM engelen@icbm.de RI Kyrpides, Nikos/A-6305-2014; Faculty of, Sciences, KAU/E-7305-2017; Fac Sci, KAU, Biol Sci Dept/L-4228-2013 OI Kyrpides, Nikos/0000-0002-6131-0462; FU German Research Foundation (DFG) [Transregio-SFB 51]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors acknowledge the crew and the scientific party of the RV Heincke (expedition HE361), especially Judith Lucas for sampling and starting the enrichment cultures as well as Michael Pilzen and Jutta Graue for their assistance during sampling. Furthermore, we thank Jana Feldkamp and Frank Meyerjurgens for technical assistance and our students, Leon Dluglosch, David Nivia, Eva-Lena Nordmann and Katrin Grosser for preliminary physiological experiments and microscopy pictures. We would also extend our thanks to Marco Dogs, Sven Breider and Thorsten Brinkhoff for valuable discussions during genome analysis and Candice Raeburn for proofreading. This work was mainly conducted in the frame of the Roseobacter collaborative research center Transregio-SFB 51, supported by the German Research Foundation (DFG). The work conducted by the U.S. Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 53 TC 0 Z9 0 U1 1 U2 7 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1944-3277 J9 STAND GENOMIC SCI JI Stand. Genomic Sci. PD MAR 12 PY 2016 VL 11 AR 25 DI 10.1186/s40793-016-0143-0 PG 10 WC Genetics & Heredity; Microbiology SC Genetics & Heredity; Microbiology GA DO7GX UT WOS:000377951600001 PM 27042262 ER PT J AU Solomon, KV Haitjema, CH Henske, JK Gilmore, SP Borges-Rivera, D Lipzen, A Brewer, HM Purvine, SO Wright, AT Theodorou, MK Grigoriev, IV Regev, A Thompson, DA O'Malley, MA AF Solomon, Kevin V. Haitjema, Charles H. Henske, John K. Gilmore, Sean P. Borges-Rivera, Diego Lipzen, Anna Brewer, Heather M. Purvine, Samuel O. Wright, Aaron T. Theodorou, Michael K. Grigoriev, Igor V. Regev, Aviv Thompson, Dawn A. O'Malley, Michelle A. TI Early-branching gut fungi possess a large, comprehensive array of biomass-degrading enzymes SO SCIENCE LA English DT Article ID CELL-WALL; ANTISENSE TRANSCRIPTS; GENOME; RNA; EXPRESSION; RUMEN; ORPINOMYCES; DISCOVERY; REVEALS; HISTORY AB The fungal kingdom is the source of almost all industrial enzymes in use for lignocellulose bioprocessing. We developed a systems-level approach that integrates transcriptomic sequencing, proteomics, phenotype, and biochemical studies of relatively unexplored basal fungi. Anaerobic gut fungi isolated from herbivores produce a large array of biomass-degrading enzymes that synergistically degrade crude, untreated plant biomass and are competitive with optimized commercial preparations from Aspergillus and Trichoderma. Compared to these model platforms, gut fungal enzymes are unbiased in substrate preference due to a wealth of xylan-degrading enzymes. These enzymes are universally catabolite-repressed and are further regulated by a rich landscape of noncoding regulatory RNAs. Additionally, we identified several promising sequence-divergent enzyme candidates for lignocellulosic bioprocessing. C1 [Solomon, Kevin V.; Haitjema, Charles H.; Henske, John K.; Gilmore, Sean P.; O'Malley, Michelle A.] Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. [Borges-Rivera, Diego; Regev, Aviv; Thompson, Dawn A.] Broad Inst MIT & Harvard, Cambridge, MA 02143 USA. [Lipzen, Anna; Grigoriev, Igor V.] US DOE, Joint Genome Inst, 2800 Mitchell Dr, Walnut Creek, CA 94598 USA. [Brewer, Heather M.; Purvine, Samuel O.; Wright, Aaron T.] Pacific Northwest Natl Lab, Earth & Biol Sci Div, Richland, WA 99352 USA. [Brewer, Heather M.; Purvine, Samuel O.] Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Theodorou, Michael K.] Harper Adams Univ, Anim Prod Welf & Vet Sci, Newport TF10 8NB, Shrops, England. [Solomon, Kevin V.] Purdue Univ, Dept Agr & Biol Engn, W Lafayette, IN 47907 USA. [Thompson, Dawn A.] Ginkgo Bioworks, Boston, MA 02210 USA. RP O'Malley, MA (reprint author), Univ Calif Santa Barbara, Dept Chem Engn, Santa Barbara, CA 93106 USA. EM momalley@engineering.ucsb.edu OI Solomon, Kevin/0000-0003-2904-9118 FU Office of Science [Biological and Environmental Research (BER) program], DOE [DE-SC0010352]; U.S. Department of Agriculture [2011-67017-20459]; Institute for Collaborative Biotechnologies [W911NF-09-0001]; Office of Science BER program [DE-AC02-05CH11231, DE-AC05-76RL01830] FX We thank C. Ngan, C. Daum, E. Lindquist, and K. Barry for supervising library construction, transcriptome sequencing and analysis, and project management; K. Lee and L. Choe for proteomics support; P. Weimer for lignocellulosic substrates; and the Broad Institute core facilities for sequencing and computational assistance. Sequence and cluster descriptions are included in data S1 to S3, S8, and S9 in the supplementary materials. Raw sequence data and transcriptomic profiles reported in this study are deposited under BioProject accession no. PRJNA 291757 (www.ncbi.nlm.nih.gov/bioproject/291757). Expression data are deposited in the National Center for Biotechnology Information's Gene Expression Omnibus (GEO) (29) and are accessible through GEO Series accession no. GSE64834 (www.ncbi.nlm.nih.gov/geo/query/acc.cgi?acc=GSE64834). K.V.S., C.H.H., J.K.H., and M.A.O. are inventors on patent applications (UCSB 2014-075 and UCSB 2015-334), filed by The Reagents of the University of California, related to the production of anaerobic fungal enzymes. This work was supported by the Office of Science [Biological and Environmental Research (BER) program], DOE (grant DE-SC0010352); the U.S. Department of Agriculture (Award 2011-67017-20459); and the Institute for Collaborative Biotechnologies (grant W911NF-09-0001). A portion of this research was performed under the Joint Genome Institute (JGI)-Environmental Molecular Sciences Laboratory (EMSL) Collaborative Science Initiative and used resources at the DOE JGI and the EMSL, which are DOE Office of Science user facilities. Both facilities are sponsored by the Office of Science BER program and operated under contract nos. DE-AC02-05CH11231 (JGI) and DE-AC05-76RL01830 (EMSL). K.V.S., C.H.H., D.A.T., M.K.T., and M.A.O. planned the experiments. M.A.O., J.K.H., C.H.H., M.K.T., and K.V.S. isolated pure cultures of gut fungi. K.V.S., C.H.H., J.K.H., and M.A.O. performed growth and transcriptomic experiments. A.L. analyzed transcriptome sequencing. C.H.H., H.M.B., S.O.P., and A.T.W. performed proteomic analyses. S.P.G. performed enzyme characterization. K.V.S., D.B.-R., J.K.H., A.R., I.V.G., S.O.P., and S.P.G. facilitated bioinformatics analyses of the data sets. K.V.S., D.A.T., and M.A.O. wrote the manuscript. NR 29 TC 11 Z9 12 U1 22 U2 38 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD MAR 11 PY 2016 VL 351 IS 6278 BP 1192 EP 1195 DI 10.1126/science.aad1431 PG 4 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DZ8YI UT WOS:000386158400044 PM 26912365 ER PT J AU Campbell, JC Kim, JJ Li, KY Huang, GY Reger, AS Matsuda, S Sankaran, B Link, TM Yuasa, K Ladbury, JE Casteel, DE Kim, C AF Campbell, James C. Kim, Jeong Joo Li, Kevin Y. Huang, Gilbert Y. Reger, Albert S. Matsuda, Shinya Sankaran, Banumathi Link, Todd M. Yuasa, Keizo Ladbury, John E. Casteel, Darren E. Kim, Choel TI Structural Basis of Cyclic Nucleotide Selectivity in cGMP-dependent Protein Kinase II SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE allosteric regulation; cyclic nucleotide; ligand-binding protein; protein kinase G (PKG); receptor structure-function; serine; threonine protein kinase; X-ray crystallography; NO-cGMP signaling; cGMP-dependent protein kinase; cyclic nucleotide-binding domain (CNB); second messenger ID STRUCTURE REFINEMENT; ACTIVATION; MODEL; EXPRESSION; CLONING; DESIGN; PHENIX; GENE; CAMP AB Membrane-bound cGMP-dependent protein kinase (PKG) II is a key regulator of bone growth, renin secretion, and memory formation. Despite its crucial physiological roles, little is known about its cyclic nucleotide selectivity mechanism due to a lack of structural information. Here, we find that the C-terminal cyclic nucleotide binding (CNB-B) domain of PKG II binds cGMP with higher affinity and selectivity when compared with its N-terminal CNB (CNB-A) domain. To understand the structural basis of cGMP selectivity, we solved co-crystal structures of the CNB domains with cyclic nucleotides. Our structures combined with mutagenesis demonstrate that the guanine-specific contacts at Asp-412 and Arg-415 of the C-helix of CNB-B are crucial for cGMP selectivity and activation of PKG II. Structural comparison with the cGMP selective CNB domains of human PKG I and Plasmodium falciparum PKG (PfPKG) shows different contacts with the guanine moiety, revealing a unique cGMP selectivity mechanism for PKG II. C1 [Campbell, James C.; Ladbury, John E.; Kim, Choel] Baylor Coll Med, Struct & Computat Biol & Mol Biophys Program, Houston, TX 77030 USA. [Kim, Jeong Joo; Reger, Albert S.; Kim, Choel] Baylor Coll Med, Dept Pharmacol, Houston, TX 77030 USA. [Huang, Gilbert Y.; Kim, Choel] Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. [Kim, Jeong Joo] Univ Kassel, Dept Biochem, D-34132 Kassel, Hesse, Germany. [Li, Kevin Y.] Rice Univ, Dept Biochem & Cell Biol, Houston, TX 77005 USA. [Matsuda, Shinya; Yuasa, Keizo] Univ Tokushima, Dept Biol Sci & Technol, Grad Sch, Tokushima 7708506, Japan. [Sankaran, Banumathi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley Ctr Struct Biol, Berkeley, CA 94720 USA. [Link, Todd M.; Ladbury, John E.] Univ Texas MD Anderson Canc Ctr, Dept Biochem & Mol Biol, Houston, TX 77030 USA. [Casteel, Darren E.] Univ Calif San Diego, Dept Med, La Jolla, CA 92093 USA. [Ladbury, John E.] Univ Leeds, Sch Mol & Cellular Biol, Leeds LS2 9JT, W Yorkshire, England. RP Kim, C (reprint author), Baylor Coll Med, Struct & Computat Biol & Mol Biophys Program, Houston, TX 77030 USA.; Kim, C (reprint author), Baylor Coll Med, Dept Pharmacol, Houston, TX 77030 USA.; Kim, C (reprint author), Baylor Coll Med, Verna & Marrs McLean Dept Biochem & Mol Biol, Houston, TX 77030 USA. EM ckim@bcm.edu FU National Institutes of Health, NIGMS; Howard Hughes Medical Institute; Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy [DE-AC02-05CH11231] FX We thank A. Fields and H. Rehmann for critically reading the manuscript. We also thank M. Young and C. Zhao for their assistance with crystallization. The Berkeley Center for Structural Biology is supported in part by the National Institutes of Health, NIGMS, and the Howard Hughes Medical Institute. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy under Contract Number DE-AC02-05CH11231. NR 37 TC 1 Z9 1 U1 1 U2 2 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD MAR 11 PY 2016 VL 291 IS 11 BP 5623 EP 5633 DI 10.1074/jbc.M115.691303 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DH1NN UT WOS:000372551800015 PM 26769964 ER PT J AU Deng, XY Qin, XJ Chen, L Jia, Q Zhang, YH Zhang, ZY Lei, DS Ren, G Zhou, ZH Wang, Z Li, Q Xie, W AF Deng, Xiangyu Qin, Xiangjing Chen, Lei Jia, Qian Zhang, Yonghui Zhang, Zhiyong Lei, Dongsheng Ren, Gang Zhou, Zhihong Wang, Zhong Li, Qing Xie, Wei TI Large Conformational Changes of Insertion 3 in Human Glycyl-tRNA Synthetase (hGlyRS) during Catalysis SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE aminoacyl tRNA synthetase; Charcot-Marie-Tooth disease (CMT); conformational change; crystal structure; enzyme mechanism ID MARIE-TOOTH-DISEASE; PERIPHERAL NEUROPATHY; THERMUS-THERMOPHILUS; MOLECULAR SIMULATION; MUSCULAR-ATROPHY; GARS GENE; MUTATIONS; DYNAMICS; 2D; AMINOACYLATION AB Glycyl-tRNA synthetase (GlyRS) is the enzyme that covalently links glycine to cognate tRNA for translation. It is of great research interest because of its nonconserved quaternary structures, unique species-specific aminoacylation properties, and noncanonical functions in neurological diseases, but none of these is fully understood. We report two crystal structures of human GlyRS variants, in the free form and in complex with tRNA(Gly) respectively, and reveal new aspects of the glycylation mechanism. We discover that insertion 3 differs considerably in conformation in catalysis and that it acts like a switch and fully opens to allow tRNA to bind in a cross-subunit fashion. The flexibility of the protein is supported by molecular dynamics simulation, as well as enzymatic activity assays. The biophysical and biochemical studies suggest that human GlyRS may utilize its flexibility for both the traditional function (regulate tRNA binding) and alternative functions (roles in diseases). C1 [Deng, Xiangyu; Chen, Lei; Jia, Qian; Zhou, Zhihong; Xie, Wei] Sun Yat Sen Univ, Sch Life Sci, State Key Lab Biocontrol, 135 West Xingang Rd, Guangzhou 510275, Guangdong, Peoples R China. [Deng, Xiangyu; Chen, Lei; Jia, Qian; Zhou, Zhihong; Wang, Zhong; Li, Qing; Xie, Wei] Sun Yat Sen Univ, Ctr Cellular & Struct Biol, Guangzhou 510006, Guangdong, Peoples R China. [Wang, Zhong; Li, Qing] Sun Yat Sen Univ, Sch Pharmaceut Sci, Guangzhou 510006, Guangdong, Peoples R China. [Qin, Xiangjing] Chinese Acad Sci, South China Sea Inst, Guangzhou 510301, Guangdong, Peoples R China. [Zhang, Yonghui; Zhang, Zhiyong] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [Zhang, Yonghui; Zhang, Zhiyong] Univ Sci & Technol China, Sch Life Sci, Hefei 230026, Anhui, Peoples R China. [Lei, Dongsheng; Ren, Gang] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. RP Xie, W (reprint author), Sun Yat Sen Univ, Sch Life Sci, State Key Lab Biocontrol, 135 West Xingang Rd, Guangzhou 510275, Guangdong, Peoples R China. EM xiewei6@mail.sysu.edu.cn OI Xie, Wei/0000-0003-2410-2135 FU National Sciences Foundation of China [31100579, 31270760]; Guangdong Innovative Research Team Program [2011Y038] FX This work was supported by National Sciences Foundation of China Grants 31100579 and 31270760 and Guangdong Innovative Research Team Program 2011Y038. The authors declare that they have no conflicts of interest with the contents of this article. NR 60 TC 1 Z9 1 U1 0 U2 2 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD MAR 11 PY 2016 VL 291 IS 11 BP 5740 EP 5752 DI 10.1074/jbc.M115.679126 PG 13 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DH1NN UT WOS:000372551800023 PM 26797133 ER PT J AU Kitaura, FS Rodriguez-Torres, S Chuang, CH Zhao, C Prada, F Gil-Marin, H Guo, H Yepes, G Klypin, A Scoccola, CG Tinker, J McBride, C Reid, B Sanchez, AG Salazar-Albornoz, S Grieb, JN Vargas-Magana, M Cuesta, AJ Neyrinck, M Beutler, F Comparat, J Percival, WJ Ross, A AF Kitaura, Francisco-Shu Rodriguez-Torres, Sergio Chuang, Chia-Hsun Zhao, Cheng Prada, Francisco Gil-Marin, Hector Guo, Hong Yepes, Gustavo Klypin, Anatoly Scoccola, Claudia G. Tinker, Jeremy McBride, Cameron Reid, Beth Sanchez, Ariel G. Salazar-Albornoz, Salvador Grieb, Jan Niklas Vargas-Magana, Mariana Cuesta, Antonio J. Neyrinck, Mark Beutler, Florian Comparat, Johan Percival, Will J. Ross, Ashley TI The clustering of galaxies in the SDSS-III Baryon Oscillation Spectroscopic Survey: mock galaxy catalogues for the BOSS Final Data Release SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE methods: numerical; galaxies: haloes; galaxies: statistics; large-scale structure of Universe ID LARGE-SCALE STRUCTURE; COLD DARK-MATTER; HALO OCCUPATION DISTRIBUTION; DIGITAL SKY SURVEY; LUMINOUS RED GALAXIES; N-BODY SIMULATIONS; ACOUSTIC-OSCILLATIONS; POWER-SPECTRUM; LAMBDA-CDM; PERTURBATION-THEORY AB We reproduce the galaxy clustering catalogue from the SDSS-III Baryon Oscillation Spectroscopic Survey Final Data Release (BOSS DR11&DR12) with high fidelity on all relevant scales in order to allow a robust analysis of baryon acoustic oscillations and redshift space distortions. We have generated (6000) 12 288 MultiDark PATCHY BOSS (DR11) DR12 light cones corresponding to an effective volume of similar to 192 000 [h(-1) Gpc](3) (the largest ever simulated volume), including cosmic evolution in the redshift range from 0.15 to 0.75. The mocks have been calibrated using a reference galaxy catalogue based on the halo abundance matching modelling of the BOSS DR11&DR12 galaxy clustering data and on the data themselves. The production follows three steps. First, we apply the PATCHY code to generate a dark matter field and an object distribution including non-linear stochastic galaxy bias. Secondly, we run the halo/stellar distribution reconstruction HADRON code to assign masses to the various objects. This step uses the mass distribution as a function of local density and non-local indicators (i.e. tidal field tensor eigenvalues and relative halo exclusion separation for massive objects) from the reference simulation applied to the corresponding patchy dark matter and galaxy distribution. Finally, we apply the SUGAR code to build the light cones. The resulting MultiDarkPATCHY mock light cones reproduce the number density, selection function, survey geometry, and in general within 1 sigma, for arbitrary stellar mass bins, the power spectrum up to k = 0.3 h Mpc(-1), the two-point correlation functions down to a few Mpc scales, and the three-point statistics of the BOSS DR11&DR12 galaxy samples. C1 [Kitaura, Francisco-Shu] Leibniz Inst Astrophys Potsdam AIP, Sternwarte 16, D-14482 Potsdam, Germany. [Rodriguez-Torres, Sergio; Chuang, Chia-Hsun; Prada, Francisco; Comparat, Johan] Univ Autonoma Madrid, UAM CSIC, Inst Fis Teor, E-28049 Madrid, Spain. [Rodriguez-Torres, Sergio; Prada, Francisco] Campus Int Excellence UAM CSIC, E-28049 Madrid, Spain. [Rodriguez-Torres, Sergio] Univ Autonoma Madrid, Dept Fis Teor, E-28049 Madrid, Spain. [Zhao, Cheng] Tsinghua Univ, Tsinghua Ctr Astrophys, Dept Phys, Beijing 100084, Peoples R China. [Prada, Francisco] Inst Astrofis Andalucia CSIC, Glorieta Astron, E-18080 Granada, Spain. [Gil-Marin, Hector; Percival, Will J.; Ross, Ashley] Univ Portsmouth, Inst Cosmol & Gravitat, Dennis Sciama Bldg, Portsmouth PO1 3FX, Hants, England. [Guo, Hong] Chinese Acad Sci, Shanghai Astron Observ, Key Lab Res Galaxies & Cosmol, Shanghai 200030, Peoples R China. [Guo, Hong] Univ Utah, Dept Phys & Astron, Salt Lake City, UT 84112 USA. [Klypin, Anatoly] New Mexico State Univ, Astron Dept, Las Cruces, NM 88003 USA. [Klypin, Anatoly] Inst Fis Teor UAM CSIC, E-28049 Madrid, Spain. [Scoccola, Claudia G.] Inst Astrofis Canarias IAC, C Via Lactea S-N, E-38200 Tenerife, Spain. [Scoccola, Claudia G.] Univ La Laguna, Dept Astrofis, E-38206 Tenerife, Spain. [Tinker, Jeremy] NYU, Ctr Cosmol & Particle Phys, 4 Washington Pl, New York, NY 10003 USA. [McBride, Cameron] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. [Reid, Beth; Beutler, Florian] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, 1 Cyclotron Rd,Berkeley, Berkeley, CA 94720 USA. [Reid, Beth] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Reid, Beth] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Sanchez, Ariel G.; Salazar-Albornoz, Salvador; Grieb, Jan Niklas] Max Planck Inst Extraterr Phys, Postfach 1312,Giessenbachstr, D-85741 Garching, Germany. [Salazar-Albornoz, Salvador; Grieb, Jan Niklas] Univ Sternwarte Munchen, Scheinerstr 1, D-81679 Munich, Germany. [Vargas-Magana, Mariana] Univ Nacl Autonoma Mexico, Inst Fis, Apdo Postal 20-364, Mexico City 01000, DF, Mexico. [Cuesta, Antonio J.; Neyrinck, Mark] Univ Barcelona IEEC UB, Inst Ciencies Cosmos ICCUB, Marti & Franques 1, E-08028 Barcelona, Spain. [Neyrinck, Mark] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. [Ross, Ashley] Ohio State Univ, Ctr Cosmol & AstroParticle Phys, Columbus, OH 43210 USA. RP Kitaura, FS (reprint author), Leibniz Inst Astrophys Potsdam AIP, Sternwarte 16, D-14482 Potsdam, Germany. EM kitaura@aip.de RI Guo, Hong/J-5797-2015; Gil Marin, Hector/B-2013-2017; OI Guo, Hong/0000-0003-4936-8247; Gil Marin, Hector/0000-0003-0265-6217; Beutler, Florian/0000-0003-0467-5438; Cuesta Vazquez, Antonio Jose/0000-0002-4153-9470 FU Spanish MICINNs Consolider-Ingenio Programme under grant MultiDark [CSD2009-00064]; MINECO Centro de Excelencia Severo Ochoa Programme [SEV-2012-0249, AYA2014-60641-C2-1-P]; Spanish MEC 'Salvador de Madariaga' programme [PRX14/00444]; UK Science and Technology Facilities Council [ST/I001204/1]; Chinese Academy of Sciences; MINECO (Spain) [AYA2012-31101, FPA2012-34694]; Transregional Collaborative Research Centre TR33 'The Dark Universe' of the German Research Foundation (DFG); European Research Council under the European Community [FP7-IDEAS-Phys.LSS 240117]; Spanish MINECO of ICCUB (Unidad de Excelencia 'Maria de Maeztu') [MDM-2014-0369]; ICG; SEPNet; University of Portsmouth; Office of Science of the US Department of Energy [DE-AC02-05CH11231]; Alfred P. Sloan Foundation; National Science Foundation; US Department of Energy Office of Science; University of Arizona; Brazilian Participation Group; Brookhaven National Laboratory; University of Cambridge; Carnegie Mellon University; University of Florida; French Participation Group; German Participation Group; Harvard University; Instituto de Astrofisica de Canarias; Michigan State/Notre Dame/JINA Participation Group; Johns Hopkins University; Lawrence Berkeley National Laboratory; Max Planck Institute for Astrophysics; Max Planck Institute for Extraterrestrial Physics; New Mexico State University; New York University; Ohio State University; Pennsylvania State University; Princeton University; Spanish Participation Group; University of Tokyo; University of Utah; Vanderbilt University; University of Virginia; University of Washington; Yale University; [2012060963] FX FSK, SRT, CC, CZ, FP, AK, and CGS acknowledge support from the Spanish MICINNs Consolider-Ingenio 2010 Programme under grant MultiDark CSD2009-00064, MINECO Centro de Excelencia Severo Ochoa Programme under grant SEV-2012-0249, and grant AYA2014-60641-C2-1-P. FSK and CZ also want to thank the Instituto de Fisica Teorica UAM/CSIC for the hospitality and support during several visits, where part of this work was completed. FP wishes to thank the Lawrence Berkeley National Laboratory for the hospitality during the development of this work; he also acknowledges the Spanish MEC 'Salvador de Madariaga' programme, Ref. PRX14/00444. HGM is grateful for support from the UK Science and Technology Facilities Council through the grant ST/I001204/1. HG acknowledges the support of the 100 Talents Program of the Chinese Academy of Sciences. GY wishes to thank MINECO (Spain) for financial support under project grants AYA2012-31101 and FPA2012-34694. He also thanks the Red Espanola de Supercomputacion for granting computing time in the Marenostrum supercomputer, in which part of this work has been done. AGS, SSA, and JNG acknowledge support from the Transregional Collaborative Research Centre TR33 'The Dark Universe' of the German Research Foundation (DFG). AJC is supported by supported by the European Research Council under the European Community's Seventh Framework Programme FP7-IDEAS-Phys.LSS 240117. Funding for this work was partially provided by the Spanish MINECO under project MDM-2014-0369 of ICCUB (Unidad de Excelencia 'Maria de Maeztu').; The BigMultiDark simulations have been performed on the SuperMUC supercomputer at the Leibniz-Rechenzentrum (LRZ) in Munich, using the computing resources awarded to the PRACE project number 2012060963. We want to thank V. Springel for providing us with the optimized version of GADGET-2.; Numerical computations for the power spectrum multipoles and bispectrum were performed on the Sciama High Performance Compute (HPC) cluster which is supported by the ICG, SEPNet, and the University of Portsmouth.; This research also used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231.; Funding for SDSS-III has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, and the US Department of Energy Office of Science. The SDSS-III website is http://www.sdss3.org/.; SDSS-III is managed by the Astrophysical Research Consortium for the Participating Institutions of the SDSS-III Collaboration including the University of Arizona, the Brazilian Participation Group, Brookhaven National Laboratory, University of Cambridge, Carnegie Mellon University, University of Florida, the French Participation Group, the German Participation Group, Harvard University, the Instituto de Astrofisica de Canarias, the Michigan State/Notre Dame/JINA Participation Group, Johns Hopkins University, Lawrence Berkeley National Laboratory, Max Planck Institute for Astrophysics, Max Planck Institute for Extraterrestrial Physics, New Mexico State University, New York University, Ohio State University, Pennsylvania State University, University of Portsmouth, Princeton University, the Spanish Participation Group, University of Tokyo, University of Utah, Vanderbilt University, University of Virginia, University of Washington, and Yale University. NR 146 TC 19 Z9 19 U1 2 U2 7 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD MAR 11 PY 2016 VL 456 IS 4 BP 4156 EP 4173 DI 10.1093/mnras/stv2826 PG 18 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG7LM UT WOS:000372265800058 ER PT J AU Zhang, Q Kumar, CMN Tian, W Dennis, KW Goldman, AI Vaknin, D AF Zhang, Qiang Kumar, C. M. N. Tian, Wei Dennis, Kevin W. Goldman, Alan I. Vaknin, David TI Structure and magnetic properties of LnMnSbO (Ln = La and Ce) SO PHYSICAL REVIEW B LA English DT Article ID ANTIFERROMAGNETISM; SUPERCONDUCTIVITY; DYNAMICS; ORDER; PR; ND AB A neutron powder diffraction (NPD) study of LnMnSbO (Ln = La or Ce) reveals differences between the magnetic ground state of the two compounds due to the strong Ce-Mn coupling compared to La-Mn. The two compounds adopt the P4/nmm space group down to 2 K, and whereas magnetization measurements do not show obvious anomaly at high temperatures, NPD reveals a C-type antiferromagnetic (AFM) order below T-N = 255 K for LaMnSbO and 240 K for CeMnSbO. While the magnetic structure of LaMnSbO is preserved to base temperature, a sharp transition at T-SR = 4.5 K is observed in CeMnSbO due to a spin-reorientation (SR) transition of the Mn2+ magnetic moments from pointing along the c axis to the ab plane. The SR transition in CeMnSbO is accompanied by a simultaneous long-range AFM ordering of the Ce moments, which indicates that the Mn SR transition is driven by the Ce-Mn coupling. The ordered moments are found to be somewhat smaller than those expected for Mn2+ (S = 5/2) in insulators, but large enough to suggest that these compounds belong to the class of local-moment antiferromagnets. The lower TN found in these two compounds compared to the As-based counterparts (T-N = 317 for LaMnAsO, T-N = 347 K for CeMnAsO) indicates that the Mn-Pn (Pn = As or Sb) hybridization that mediates the superexchange Mn-Pn-Mn coupling is weaker for the Sb-based compounds. C1 [Zhang, Qiang; Dennis, Kevin W.; Goldman, Alan I.; Vaknin, David] Ames Lab, Ames, IA 50011 USA. [Zhang, Qiang; Goldman, Alan I.; Vaknin, David] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Kumar, C. M. N.] Forschungszentrum Julich GmbH, Oak Ridge Natl Lab, JCNS, Outstn SNS, Oak Ridge, TN 37831 USA. [Kumar, C. M. N.] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Tian, Wei] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Zhang, Q; Vaknin, D (reprint author), Ames Lab, Ames, IA 50011 USA.; Zhang, Q; Vaknin, D (reprint author), Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. EM qzhangemail@gmail.com; vaknin@ameslab.gov RI Vaknin, David/B-3302-2009; Tian, Wei/C-8604-2013; OI Vaknin, David/0000-0002-0899-9248; Tian, Wei/0000-0001-7735-3187; Zhang, Qiang/0000-0003-0389-7039; Chogondahalli Muniraju, Naveen Kumar/0000-0002-8867-8291 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering [DE-AC02-07CH11358]; U.S. Department of Energy, Office of Basic Energy Sciences, Scientific Users Facilities Division FX Research at Ames Laboratory is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Contract No. DE-AC02-07CH11358. Use of the High Flux Isotope Reactor and the Spallation Neutron Source at the Oak Ridge National Laboratory is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Scientific Users Facilities Division. NR 33 TC 1 Z9 1 U1 6 U2 14 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 11 PY 2016 VL 93 IS 9 AR 094413 DI 10.1103/PhysRevB.93.094413 PG 7 WC Physics, Condensed Matter SC Physics GA DG3HK UT WOS:000371959900004 ER PT J AU Balitsky, I Kazakov, V Sobko, E AF Balitsky, Ian Kazakov, Vladimir Sobko, Evgeny TI Structure constant of twist-2 light-ray operators in the Regge limit SO PHYSICAL REVIEW D LA English DT Article ID SCATTERING; POMERON AB We compute the normalized structure constant of three twist-2 operators in N = 4 SYM in the leading Balitsky-Fadin-Kuraev-Lipatov (BFKL) approximation at any N-c. The result is applicable to other gauge theories including QCD. C1 [Balitsky, Ian] Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA. [Balitsky, Ian] JLAB, Theory Grp, 12000 Jefferson Ave, Newport News, VA 23606 USA. [Kazakov, Vladimir] Ecole Normale Super, LPT, 24 Rue Lhomond, F-75005 Paris, France. [Kazakov, Vladimir] Univ Paris 06, Pl Jussieu, F-75005 Paris, France. [Sobko, Evgeny] DESY, Theory Grp, Notkestr 85, D-22607 Hamburg, Germany. RP Balitsky, I (reprint author), Old Dominion Univ, Dept Phys, Norfolk, VA 23529 USA.; Balitsky, I (reprint author), JLAB, Theory Grp, 12000 Jefferson Ave, Newport News, VA 23606 USA. FU People Programme (Marie Curie Actions) of the European Union's Seventh Framework Programme FP7 under REA Grant Agreement [317089]; European Research Council (Programme Ideas Grant) [ERC-2012-AdG 320769 AdS-CFT-solvable]; ANR grant StrongInt [BLANC- SIMI- 4-2011]; ESF [HOLOGRAV-09- RNP- 092]; DOE [DE-AC050-6OR23177, DE-FG02-97ER41028] FX We thank J. Bartels, S. Caron-Huot, L. Lipatov, and V. Schomerus for discussions. Our special thanks to G. Korchemsky who participated in the initial stage of this work. The work of E. S. and V. K. was supported by the People Programme (Marie Curie Actions) of the European Union's Seventh Framework Programme FP7/2007-2013/ under REA Grant Agreement No. 317089 (GATIS). The work of V. K. has received funding from the European Research Council (Programme Ideas Grant No. ERC-2012-AdG 320769 AdS-CFT-solvable), from the ANR grant StrongInt (Grant No. BLANC- SIMI- 4-2011) and from ESF Grant No. HOLOGRAV-09- RNP-092. The work of I. B. was supported by DOE Contract No. DE-AC050-6OR23177 and by Grant No. DE-FG02-97ER41028. NR 18 TC 2 Z9 2 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD MAR 11 PY 2016 VL 93 IS 6 AR 061701 DI 10.1103/PhysRevD.93.061701 PG 6 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DG3JC UT WOS:000371964400002 ER PT J AU Davidovits, S Fisch, NJ AF Davidovits, Seth Fisch, Nathaniel J. TI Sudden Viscous Dissipation of Compressing Turbulence SO PHYSICAL REVIEW LETTERS LA English DT Article ID HOMOGENEOUS TURBULENCE; ISOTROPIC TURBULENCE AB Compression of turbulent plasma can amplify the turbulent kinetic energy, if the compression is fast compared to the viscous dissipation time of the turbulent eddies. A sudden viscous dissipation mechanism is demonstrated, whereby this amplified turbulent kinetic energy is rapidly converted into thermal energy, suggesting a new paradigm for fast ignition inertial fusion. C1 [Davidovits, Seth; Fisch, Nathaniel J.] Princeton Univ, Princeton, NJ 08540 USA. [Fisch, Nathaniel J.] Princeton Univ, Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. RP Davidovits, S (reprint author), Princeton Univ, Princeton, NJ 08540 USA. FU DOE [DE-AC02-09CH1-1466, NNSA 67350-9960, DOE DE-NA0001836]; DTRA [HDTRA1-11-1-0037]; NSF [PHY-1506122] FX This work was supported by DOE through Contracts No. DE-AC02-09CH1-1466 and NNSA 67350-9960 (Prime No. DOE DE-NA0001836), by DTRA HDTRA1-11-1-0037, and by NSF Contract No. PHY-1506122. For stimulating the ideas presented here, the authors would like to acknowledge the discovery of the dominant effect of TKE in compressing Z-pinch experiments carried out at the Weizmann Institute [1-4]. NR 20 TC 4 Z9 4 U1 5 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 11 PY 2016 VL 116 IS 10 AR 105004 DI 10.1103/PhysRevLett.116.105004 PG 5 WC Physics, Multidisciplinary SC Physics GA DG3GG UT WOS:000371956900004 PM 27015488 ER PT J AU Khuntia, P Bert, F Mendels, P Koteswararao, B Mahajan, AV Baenitz, M Chou, FC Baines, C Amato, A Furukawa, Y AF Khuntia, P. Bert, F. Mendels, P. Koteswararao, B. Mahajan, A. V. Baenitz, M. Chou, F. C. Baines, C. Amato, A. Furukawa, Y. TI Spin Liquid State in the 3D Frustrated Antiferromagnet PbCuTe2O6: NMR and Muon Spin Relaxation Studies SO PHYSICAL REVIEW LETTERS LA English DT Article ID LATTICE ANTIFERROMAGNET AB PbCuTe2O6 is a rare example of a spin liquid candidate featuring a three-dimensional magnetic lattice. Strong geometric frustration arises from the dominant antiferromagnetic interaction that generates a hyperkagome network of Cu2+ ions although additional interactions enhance the magnetic lattice connectivity. Through a combination of magnetization measurements and local probe investigations by NMR and muon spin relaxation down to 20 mK, we provide robust evidence for the absence of magnetic freezing in the ground state. The local spin susceptibility probed by the NMR shift hardly deviates from the macroscopic one down to 1 K pointing to a homogeneous magnetic system with a low defect concentration. The saturation of the NMR shift and the sublinear power law temperature (T) evolution of the 1/T-1 NMR relaxation rate at low T point to a nonsinglet ground state favoring a gapless fermionic description of the magnetic excitations. Below 1 K a pronounced slowing down of the spin dynamics is witnessed, which may signal a reconstruction of spinon Fermi surface. Nonetheless, the compound remains in a fluctuating spin liquid state down to the lowest temperature of the present investigation. C1 [Khuntia, P.; Furukawa, Y.] US DOE, Ames Lab, Ames, IA 50011 USA. [Khuntia, P.; Bert, F.; Mendels, P.] Univ Paris 11, Univ Paris Saclay, CNRS, Phys Solides Lab, F-91405 Orsay, France. [Koteswararao, B.] Univ Hyderabad, Sch Phys, Cent Univ PO, Hyderabad 500046, Andhra Pradesh, India. [Koteswararao, B.; Chou, F. C.] Natl Taiwan Univ, Ctr Condensed Matter Sci, Taipei 10617, Taiwan. [Mahajan, A. V.] Indian Inst Technol, Dept Phys, Bombay 400076, Maharashtra, India. [Baenitz, M.] Max Planck Inst Chem Phys Solids, D-01187 Dresden, Germany. [Baines, C.; Amato, A.] Paul Scherrer Inst, Lab Muon Spin Spect, CH-5232 Villigen, Switzerland. [Furukawa, Y.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. RP Khuntia, P (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA.; Khuntia, P (reprint author), Univ Paris 11, Univ Paris Saclay, CNRS, Phys Solides Lab, F-91405 Orsay, France. EM khuntia@lps.u-psud.fr RI Baenitz, Michael/E-4085-2016; Khuntia, Panchanan /E-4270-2010; Amato, Alex/H-7674-2013 OI Amato, Alex/0000-0001-9963-7498 FU European Commission through Marie Curie International Incoming Fellowship [PIIF-GA-2013-627322]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering; U.S. Department of Energy [DE-AC02-07CH11358]; French Agence Nationale de la Recherche under "SPINLIQ" Grant [ANR-12-BS04-0021]; Universite Paris-Sud Grant MRM PMP; SESAME grant from Region Ile-de-France FX We acknowledge R. R. P. Singh for discussions on the HTSE and P. Wiecki for some T2 measurements. P. K. acknowledges support from the European Commission through Marie Curie International Incoming Fellowship (PIIF-GA-2013-627322). The research was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. B. K. thanks the DST INSPIRE faculty scheme for carrying out the research work. This work was also supported by the French Agence Nationale de la Recherche under "SPINLIQ" Grant No. ANR-12-BS04-0021, by Universite Paris-Sud Grant MRM PMP, and by a SESAME grant from Region Ile-de-France. NR 34 TC 2 Z9 2 U1 6 U2 21 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD MAR 11 PY 2016 VL 116 IS 10 AR 107203 DI 10.1103/PhysRevLett.116.107203 PG 5 WC Physics, Multidisciplinary SC Physics GA DG3GG UT WOS:000371956900005 PM 27015508 ER PT J AU Brunk, E Mih, N Monk, J Zhang, Z O'Brien, EJ Bliven, SE Chen, K Chang, RL Bourne, PE Palsson, BO AF Brunk, Elizabeth Mih, Nathan Monk, Jonathan Zhang, Zhen O'Brien, Edward J. Bliven, Spencer E. Chen, Ke Chang, Roger L. Bourne, Philip E. Palsson, Bernhard O. TI Systems biology of the structural proteome SO BMC SYSTEMS BIOLOGY LA English DT Article ID COMPLETE GENOME SEQUENCE; LATERAL GENE-TRANSFER; ESCHERICHIA-COLI; THERMOTOGA-MARITIMA; FAMILIES DATABASE; I-TASSER; STRUCTURE PREDICTION; METABOLIC NETWORK; PROTEINS; EVOLUTION AB Background: The success of genome-scale models (GEMs) can be attributed to the high-quality, bottom-up reconstructions of metabolic, protein synthesis, and transcriptional regulatory networks on an organism-specific basis. Such reconstructions are biochemically, genetically, and genomically structured knowledge bases that can be converted into a mathematical format to enable a myriad of computational biological studies. In recent years, genome-scale reconstructions have been extended to include protein structural information, which has opened up new vistas in systems biology research and empowered applications in structural systems biology and systems pharmacology. Results: Here, we present the generation, application, and dissemination of genome-scale models with protein structures (GEM-PRO) for Escherichia coli and Thermotoga maritima. We show the utility of integrating molecular scale analyses with systems biology approaches by discussing several comparative analyses on the temperature dependence of growth, the distribution of protein fold families, substrate specificity, and characteristic features of whole cell proteomes. Finally, to aid in the grand challenge of big data to knowledge, we provide several explicit tutorials of how protein-related information can be linked to genome-scale models in a public GitHub repository (https://github.com/SBRG/GEMPro/tree/master/GEMPro_recon/). Conclusions: Translating genome-scale, protein-related information to structured data in the format of a GEM provides a direct mapping of gene to gene-product to protein structure to biochemical reaction to network states to phenotypic function. Integration of molecular-level details of individual proteins, such as their physical, chemical, and structural properties, further expands the description of biochemical network-level properties, and can ultimately influence how to model and predict whole cell phenotypes as well as perform comparative systems biology approaches to study differences between organisms. GEM-PRO offers insight into the physical embodiment of an organism's genotype, and its use in this comparative framework enables exploration of adaptive strategies for these organisms, opening the door to many new lines of research. With these provided tools, tutorials, and background, the reader will be in a position to run GEM-PRO for their own purposes. C1 [Brunk, Elizabeth; Monk, Jonathan; Zhang, Zhen; O'Brien, Edward J.; Chen, Ke; Palsson, Bernhard O.] Univ Calif La Jolla, Dept Bioengn, San Diego, CA 92093 USA. [Brunk, Elizabeth] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Mih, Nathan; O'Brien, Edward J.] Univ Calif La Jolla, Bioinformat & Syst Biol Program, San Diego, CA 92093 USA. [O'Brien, Edward J.] NIH, Natl Ctr Biotechnol Informat, Natl Lib Med, Bethesda, MD 20894 USA. [Chang, Roger L.] Harvard Univ, Dept Syst Biol, Sch Med, Boston, MA 02115 USA. [Bourne, Philip E.] NIH, Off Director, Bethesda, MD 20894 USA. RP Palsson, BO (reprint author), Univ Calif La Jolla, Dept Bioengn, San Diego, CA 92093 USA. EM palsson@eng.ucsd.edu OI Bliven, Spencer/0000-0002-1200-1698 FU Swiss National Science Foundation [p2elp2_148961]; Gordon and Betty Moore Foundation [GBMF 2550.04]; National Institutes of Health [GM057089]; Intramural Research Program of the National Center for Biotechnology Information, National Library of Medicine, National Institutes of Health FX The authors acknowledge support from the Swiss National Science Foundation (grant p2elp2_148961 to E.C.B), the Gordon and Betty Moore Foundation GBMF 2550.04 Life Sciences Research Foundation postdoctoral fellowship (to R.L.C.). We also acknowledge funding from the National Institutes of Health (grant GM057089). This research was supported in part by the Intramural Research Program of the National Center for Biotechnology Information, National Library of Medicine, National Institutes of Health (support to S.B. and P.B.). The authors also gratefully acknowledge NERSC supercomputer facilities and Ali Ebrahim for technical support. NR 114 TC 7 Z9 7 U1 3 U2 16 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 1752-0509 J9 BMC SYST BIOL JI BMC Syst. Biol. PD MAR 11 PY 2016 VL 10 AR 26 DI 10.1186/s12918-016-0271-6 PG 16 WC Mathematical & Computational Biology SC Mathematical & Computational Biology GA DG0TU UT WOS:000371779400001 PM 26969117 ER PT J AU Barcellos-Hoff, MH Mao, JH AF Barcellos-Hoff, Mary Helen Mao, Jian-Hua TI HZE Radiation Non-Targeted Effects on the Microenvironment That Mediate Mammary Carcinogenesis SO FRONTIERS IN ONCOLOGY LA English DT Article DE cosmic radiation; cancer risk models; ionizing radiation exposure; carcinogenesis process ID BREAST-CANCER RISK; TRACHEAL EPITHELIAL-CELLS; TUMOR-SUPPRESSOR GENE; IONIZING-RADIATION; STEM-CELLS; NEOPLASTIC PROGRESSION; SKIN CARCINOGENESIS; ADAPTIVE IMMUNITY; MOUSE MODELS; DNA-REPAIR AB Clear mechanistic understanding of the biological processes elicited by radiation that increase cancer risk can be used to inform prediction of health consequences of medical uses, such as radiotherapy, or occupational exposures, such as those of astronauts during deep space travel. Here, we review the current concepts of carcinogenesis as a multicellular process during which transformed cells escape normal tissue controls, including the immune system, and establish a tumor microenvironment. We discuss the contribution of two broad classes of radiation effects that may increase cancer: radiation targeted effects that occur as a result of direct energy deposition, e.g., DNA damage, and non -targeted effects (NTE) that result from changes in cell signaling, e.g., genomic instability. It is unknown whether the potentially greater carcinogenic effect of high Z and energy (HZE) particle radiation is a function of the relative contribution or extent of NTE or due to unique NTE. We addressed this problem using a radiation/genetic mammary chimera mouse model of breast cancer. Our experiments suggest that NTE promote more aggressive cancers, as evidenced by increased growth rate, transcriptomic signatures, and metastasis, and that HZE particle NTE are more effective than reference gamma-radiation. Emerging evidence suggest that HZE irradiation dampens antitumor immunity. These studies raise concern that HZE radiation exposure not only increases the likelihood of developing cancer but also could promote progression to more aggressive cancer with a greater risk of mortality. C1 [Barcellos-Hoff, Mary Helen] Univ Calif San Francisco, Dept Radiat Oncol, San Francisco, CA USA. [Mao, Jian-Hua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Barcellos-Hoff, MH (reprint author), Univ Calif San Francisco, Dept Radiat Oncol, San Francisco, CA USA. EM mary.barcellos-hoff@ucsf.edu OI Barcellos-Hoff, Mary Helen/0000-0002-5994-9558 NR 115 TC 1 Z9 1 U1 3 U2 5 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 2234-943X J9 FRONT ONCOL JI Front. Oncol. PD MAR 11 PY 2016 VL 6 AR 57 DI 10.3389/fonc.2016.00057 PG 10 WC Oncology SC Oncology GA DG0OD UT WOS:000371763600002 PM 27014632 ER PT J AU Chodash, PA Burke, JT Norman, EB Wilks, SC Casperson, RJ Fisher, SE Holliday, KS Jeffries, JR Wakeling, MA AF Chodash, P. A. Burke, J. T. Norman, E. B. Wilks, S. C. Casperson, R. J. Fisher, S. E. Holliday, K. S. Jeffries, J. R. Wakeling, M. A. TI Nuclear excitation by electronic transition of U-235 SO PHYSICAL REVIEW C LA English DT Article ID HALF-LIFE; NEET; MECHANISMS; RADIATION; OS-189; AU-197; PLASMA AB Background: Nuclear excitation by electronic transition (NEET) is a rare nuclear excitation that can occur in isotopes containing a low-lying nuclear excited state. Over the past 40 yr, several experiments have attempted to measure NEET of U-235 and those experiments have yielded conflicting results. Purpose: An experiment was performed to determine whether NEET of U-235 occurs and to determine its excitation rate. Method: A pulsed Nd:YAG laser operating at 1064 nm with a pulse energy of 790 mJ and a pulse width of 9 ns was used to generate a uranium plasma. The plasma was collected on a catcher plate and electrons from the catcher plate were accelerated and focused onto a microchannel plate detector. An observation of a decay with a 26-min half-life would suggest the creation of U-235m and the possibility that NEET of U-235 occurred. Results: A 26-min decay consistent with the decay of U-235m was not observed and there was no evidence that NEET occurred. An upper limit for the NEET rate of U-235 was determined to be lambda(NEET) < 1.8 x 10(-4) s(-1), with a confidence level of 68.3%. Conclusions: The upper limit determined from this experiment is consistent with most of the past measurements. Discrepancies between this experiment and past measurements can be explained by assuming that past experiments misinterpreted the data. C1 [Chodash, P. A.; Norman, E. B.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Burke, J. T.; Casperson, R. J.] Lawrence Livermore Natl Lab, Nucl & Chem Sci Div, Livermore, CA 94550 USA. [Wilks, S. C.] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. [Fisher, S. E.] Lawrence Livermore Natl Lab, Natl Secur Engn Div, Livermore, CA 94550 USA. [Holliday, K. S.; Jeffries, J. R.] Lawrence Livermore Natl Lab, Div Mat Sci, Livermore, CA 94550 USA. [Wakeling, M. A.] US Air Force, Inst Technol, Wright Patterson AFB, OH 45433 USA. RP Chodash, PA (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. RI Chodash, Perry/P-1840-2014 OI Chodash, Perry/0000-0002-4154-7219 FU Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; National Nuclear Security Administration's Next Generation Safeguards Initiative (NGSI); US Department of Homeland Security; Nuclear Science and Security Consortium under DOE [DE-NA-0000979]; UC Berkeley FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. This research was additionally performed under appointment to the Nuclear Nonproliferation International Safeguards Graduate Fellowship Program sponsored by the National Nuclear Security Administration's Next Generation Safeguards Initiative (NGSI). This work was further supported by the US Department of Homeland Security, UC Berkeley, and the Nuclear Science and Security Consortium under DOE Contract No. DE-NA-0000979. NR 31 TC 1 Z9 1 U1 4 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD MAR 11 PY 2016 VL 93 IS 3 AR 034610 DI 10.1103/PhysRevC.93.034610 PG 11 WC Physics, Nuclear SC Physics GA DG3IP UT WOS:000371963000002 ER PT J AU Hihath, S Santala, MK Cen, X Campbell, GH van Benthem, K AF Hihath, Sahar Santala, Melissa K. Cen, Xi Campbell, Geoffrey H. van Benthem, Klaus TI High speed direct imaging of thin metal film ablation by movie-mode dynamic transmission electron microscopy SO SCIENTIFIC REPORTS LA English DT Article ID EXCIMER-LASER RADIATION; GAP SINGLE-CRYSTALS; SILICON; REAL; GENERATION; PLASMA; PULSES; TEM AB Obliteration of matter by pulsed laser beams is not only prevalent in science fiction movies, but finds numerous technological applications ranging from additive manufacturing over machining of micro- and nanostructured features to health care. Pulse lengths ranging from femtoseconds to nanoseconds are utilized at varying laser beam energies and pulse lengths, and enable the removal of nanometric volumes of material. While the mechanisms for removal of material by laser irradiation, i.e., laser ablation, are well understood on the micrometer length scale, it was previously impossible to directly observe obliteration processes on smaller scales due to experimental limitations for the combination of nanometer spatial and nanosecond temporal resolution. Here, we report the direct observation of metal thin film ablation from a solid substrate through dynamic transmission electron microscopy. Quantitative analysis reveals liquid-phase dewetting of the thin-film, followed by hydrodynamic sputtering of nano-to submicron sized metal droplets. We discovered unexpected fracturing of the substrate due to evolving thermal stresses. This study confirms that hydrodynamic sputtering remains a valid mechanism for droplet expulsion on the nanoscale, while irradiation induced stress fields represent limit laser processing of nanostructured materials. Our results allow for improved safety during laser ablation in manufacturing and medical applications. C1 [Hihath, Sahar; Cen, Xi; van Benthem, Klaus] Univ Calif Davis, Dept Chem & Mat Sci, 1 Shields Ave, Davis, CA 95616 USA. [Hihath, Sahar] Univ Calif Davis, Dept Phys, 1 Shields Ave, Davis, CA 95616 USA. [Santala, Melissa K.; Campbell, Geoffrey H.] Lawrence Livermore Natl Lab, Phys & Life Sci Directory, 7000 East Ave, Livermore, CA 94550 USA. RP van Benthem, K (reprint author), Univ Calif Davis, Dept Chem & Mat Sci, 1 Shields Ave, Davis, CA 95616 USA. EM benthem@ucdavis.edu FU University of California Laboratory Fee grant [12-LR-238313]; NSF [DMR-0955638]; US Department of Energy, Office of Basic Energy Sciences [DE-AC52-07NA27344] FX This work was supported by a University of California Laboratory Fee grant (#12-LR-238313) and NSF Early Career Award (DMR-0955638). DTEM experiments at Lawrence Livermore National Laboratory were carried out under the auspices of the US Department of Energy, Office of Basic Energy Sciences under contract DE-AC52-07NA27344. NR 41 TC 1 Z9 1 U1 14 U2 28 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD MAR 11 PY 2016 VL 6 AR 23046 DI 10.1038/srep23046 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG1WM UT WOS:000371858200001 PM 26965073 ER PT J AU Collins, L Belianinov, A Somnath, S Rodriguez, BJ Balke, N Kalinin, SV Jesse, S AF Collins, Liam Belianinov, Alex Somnath, Suhas Rodriguez, Brian J. Balke, Nina Kalinin, Sergei V. Jesse, Stephen TI Multifrequency spectrum analysis using fully digital G Mode-Kelvin probe force microscopy SO NANOTECHNOLOGY LA English DT Article DE Kelvin probe force microscopy; contact potential difference; dual harmonic KPFM; big data; multivariate statistical analysis ID POLYMER SOLAR-CELLS; MODULATION-DETECTION; LABEL-FREE; NANOSCALE; AMPLITUDE; DYNAMICS; INTERFACE; DEVICES AB Since its inception over two decades ago, Kelvin probe force microscopy (KPFM) has become the standard technique for characterizing electrostatic, electrochemical and electronic properties at the nanoscale. In this work, we present a purely digital, software-based approach to KPFM utilizing big data acquisition and analysis methods. General mode (G-Mode) KPFM works by capturing the entire photodetector data stream, typically at the sampling rate limit, followed by subsequent de-noising, analysis and compression of the cantilever response. We demonstrate that the G-Mode approach allows simultaneous multi-harmonic detection, combined with on-the-fly transfer function correction-required for quantitative CPD mapping. The KPFM approach outlined in this work significantly simplifies the technique by avoiding cumbersome instrumentation optimization steps (i. e. lock in parameters, feedback gains etc), while also retaining the flexibility to be implemented on any atomic force microscopy platform. We demonstrate the added advantages of G-Mode KPFM by allowing simultaneous mapping of CPD and capacitance gradient (C') channels as well as increased flexibility in data exploration across frequency, time, space, and noise domains. G-Mode KPFM is particularly suitable for characterizing voltage sensitive materials or for operation in conductive electrolytes, and will be useful for probing electrodynamics in photovoltaics, liquids and ionic conductors. C1 [Collins, Liam; Belianinov, Alex; Somnath, Suhas; Balke, Nina; Kalinin, Sergei V.; Jesse, Stephen] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Collins, Liam; Belianinov, Alex; Somnath, Suhas; Balke, Nina; Kalinin, Sergei V.; Jesse, Stephen] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Rodriguez, Brian J.] Univ Coll Dublin, Sch Phys, Dublin 4, Ireland. [Rodriguez, Brian J.] Univ Coll Dublin, Conway Inst Biomol & Biomed Res, Dublin 4, Ireland. RP Collins, L; Jesse, S (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM collinslf@ornl.gov; sjesse@ornl.gov RI Balke, Nina/Q-2505-2015; OI Balke, Nina/0000-0001-5865-5892; Belianinov, Alex/0000-0002-3975-4112 FU Scientific User Facilities Division, Office of Basic Energy Sciences, US DOE; US DOE, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, US DOE Support was provided by the US DOE, Basic Energy Sciences, Materials Sciences and Engineering Division through the Office of Science Early Career Research Program (NB). NR 56 TC 6 Z9 6 U1 9 U2 38 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD MAR 11 PY 2016 VL 27 IS 10 AR 105706 DI 10.1088/0957-4484/27/10/105706 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DD3US UT WOS:000369849200018 PM 26866505 ER PT J AU Nielsen, J Keasling, JD AF Nielsen, Jens Keasling, Jay D. TI Engineering Cellular Metabolism SO CELL LA English DT Review ID TRANSCRIPTIONAL REGULATORY NETWORKS; ACETYL-COA METABOLISM; HIGH-LEVEL PRODUCTION; GENOME-SCALE MODELS; DE-NOVO PRODUCTION; ESCHERICHIA-COLI; SACCHAROMYCES-CEREVISIAE; SYNTHETIC BIOLOGY; GENE-EXPRESSION; PATHWAY OPTIMIZATION AB Metabolic engineering is the science of rewiring the metabolism of cells to enhance production of native metabolites or to endow cells with the ability to produce new products. The potential applications of such efforts are wide ranging, including the generation of fuels, chemicals, foods, feeds, and pharmaceuticals. However, making cells into efficient factories is challenging because cells have evolved robust metabolic networks with hard-wired, tightly regulated lines of communication between molecular pathways that resist efforts to divert resources. Here, we will review the current status and challenges of metabolic engineering and will discuss how new technologies can enable metabolic engineering to be scaled up to the industrial level, either by cutting off the lines of control for endogenous metabolism or by infiltrating the system with disruptive, heterologous pathways that overcome cellular regulation. C1 [Nielsen, Jens] Chalmers, Dept Biol & Biol Engn, Kemivagen 10, SE-41296 Gothenburg, Sweden. [Nielsen, Jens; Keasling, Jay D.] Tech Univ Denmark, Novo Nordisk Fdn Ctr Biosustainabil, DK-2970 Horsholm, Denmark. [Nielsen, Jens] Royal Inst Technol, Sci Life Lab, SE-17121 Solna, Sweden. [Keasling, Jay D.] Joint Bioenergy Inst, Emeryville, CA 94608 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94720 USA. [Keasling, Jay D.] Synthet Biol Engn Res Ctr Synberc, Berkeley, CA 94720 USA. RP Nielsen, J (reprint author), Chalmers, Dept Biol & Biol Engn, Kemivagen 10, SE-41296 Gothenburg, Sweden.; Nielsen, J; Keasling, JD (reprint author), Tech Univ Denmark, Novo Nordisk Fdn Ctr Biosustainabil, DK-2970 Horsholm, Denmark.; Nielsen, J (reprint author), Royal Inst Technol, Sci Life Lab, SE-17121 Solna, Sweden.; Keasling, JD (reprint author), Joint Bioenergy Inst, Emeryville, CA 94608 USA.; Keasling, JD (reprint author), Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA.; Keasling, JD (reprint author), Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA.; Keasling, JD (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94720 USA.; Keasling, JD (reprint author), Synthet Biol Engn Res Ctr Synberc, Berkeley, CA 94720 USA. EM nielsenj@chalmers.se; keasling@berkeley.edu OI Nielsen, Jens/0000-0002-9955-6003 FU Novo Nordisk Foundation; Knut and Alice Wallenberg Foundation; Vetenskapsradet; FORMAS; Joint Bio-Energy Institute - US Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; Synthetic Biology Engineering Research Center (SynBERC) through National Science Foundation [NSF EEC 0540879] FX We acknowledge funding from the Novo Nordisk Foundation, the Knut and Alice Wallenberg Foundation, Vetenskapsradet, FORMAS, the Joint Bio-Energy Institute (http://www.jbei.org/), which is supported by the US Department of Energy, Office of Science, Office of Biological and Environmental Research through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the US Department of Energy, and by the Synthetic Biology Engineering Research Center (SynBERC) through National Science Foundation grant NSF EEC 0540879. We thank Yun Chen, Victor Chubukov, Nathan Hillson, Mingtao Huang, Dina Petranovic, and Yongjin Zhou for constructive comments. NR 111 TC 22 Z9 22 U1 51 U2 124 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0092-8674 EI 1097-4172 J9 CELL JI Cell PD MAR 10 PY 2016 VL 164 IS 6 BP 1185 EP 1197 DI 10.1016/j.cell.2016.02.004 PG 13 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA DH4VY UT WOS:000372784900016 PM 26967285 ER PT J AU Aartsen, MG Abraham, K Ackermann, M Adams, J Aguilar, JA Ahlers, M Ahrens, M Altmann, D Anderson, T Ansseau, I Archinger, M Arguelles, C Arlen, TC Auffenberg, J Bai, X Barwick, SW Baum, V Bay, R Beatty, JJ Tjus, JB Becker, KH Beiser, E Benabderrahmane, ML Berghaus, P Berley, D Bernardini, E Bernhard, A Besson, DZ Binder, G Bindig, D Bissok, M Blaufuss, E Blumenthal, J Boersma, DJ Bohm, C Borner, M Bos, F Bose, D Boser, S Botner, O Braun, J Brayeur, L Bretz, HP Buzinsky, N Casey, J Casier, M Cheung, E Chirkin, D Christov, A Clark, K Classen, L Coenders, S Cowen, DF Silva, AHC Daughhetee, J Davis, JC Day, M de Andre, JPAM De Clercq, C Rosendo, ED Dembinski, H De Ridder, S Desiati, P de Vries, KD de Wasseige, G de With, M DeYoung, T Diaz-Velez, JC di Lorenzo, V Dumm, JP Dunkman, M Eberhardt, B Ehrhardt, T Eichmann, B Euler, S Evenson, PA Fahey, S Fazely, AR Feintzeig, J Felde, J Filimonov, K Finley, C Fischer-Wasels, T Flis, S Fosig, CC Fuchs, T Gaisser, TK Gaior, R Gallagher, J Gerhardt, L Ghorbani, K Gier, D Gladstone, L Glagla, M Glusenkamp, T Goldschmidt, A Golup, G Gonzalez, JG Gora, D Grant, D Griffith, Z Gross, A Ha, C Haack, C Ismail, AH Hallgren, A Halzen, F Hansen, E Hansmann, B Hanson, K Hebecker, D Heereman, D Helbing, K Hellauer, R Hickford, S Hignight, J Hill, GC Hoffman, KD Hoffmann, R Holzapfel, K Homeier, A Hoshina, K Huang, F Huber, M Huelsnitz, W Hulth, PO Hultqvist, K In, S Ishihara, A Jacobi, E Japaridze, GS Jeong, M Jero, K Jurkovic, M Kappes, A Karg, T Karle, A Kauer, M Keivani, A Kelley, JL Kemp, J Kheirandish, A Kiryluk, J Klas, J Klein, SR Kohnen, G Koirala, R Kolanoski, H Konietz, R Kopke, L Kopper, C Kopper, S Koskinen, DJ Kowalski, M Krings, K Kroll, G Kroll, M Kruckl, G Kunnen, J Kurahashi, N Kuwabara, T Labare, M Lanfranchi, JL Larson, MJ Lesiak-Bzdak, M Leuermann, M Leuner, J Lu, L Lunemann, J Madsen, J Maggi, G Mahn, KBM Mandelartz, M Maruyama, R Mase, K Matis, HS Maunu, R McNally, F Meagher, K Medici, M Meli, A Menne, T Merino, G Meures, T Miarecki, S Middell, E Mohrmann, L Montaruli, T Morse, R Nahnhauer, R Naumann, U Neer, G Niederhausen, H Nowicki, SC Nygren, DR Pollmann, AO Olivas, A Omairat, A O'Murchadha, A Palczewski, T Pandya, H Pankova, DV Paul, L Pepper, JA de los Heros, CP Pfendner, C Pieloth, D Pinat, E Posselt, J Price, PB Przybylski, GT Putz, J Quinnan, M Raab, C Radel, L Rameez, M Rawlins, K Reimann, R Relich, M Resconi, E Rhode, W Richman, M Richter, S Riedel, B Robertson, S Rongen, M Rott, C Ruhe, T Ryckbosch, D Sabbatini, L Sander, HG Sandrock, A Sandroos, J Sarkar, S Schatto, K Scheriau, F Schimp, M Schmidt, T Schmitz, M Schoenen, S Schoneberg, S Schonwald, A Schulte, L Schumacher, L Seckel, D Seunarine, S Soldin, D Song, M Spiczak, GM Spiering, C Stahlberg, M Stamatikos, M Stanev, T Stasik, A Steuer, A Stezelberger, T Stokstad, RG Stossl, A Strom, R Strotjohann, NL Sullivan, GW Sutherland, M Taavola, H Taboada, I Tatar, J Ter-Antonyan, S Terliuk, A Tesic, G Tilav, S Toale, PA Tobin, MN Toscano, S Tosi, D Tselengidou, M Turcati, A Unger, E Usner, M Vallecorsa, S Vandenbroucke, J van Eijndhoven, N Vanheule, S van Santen, J Veenkamp, J Vehring, M Voge, M Vraeghe, M Walck, C Wallace, A Wallraff, M Wandkowsky, N Weaver, C Wendt, C Westerhoff, S Whelan, BJ Wiebe, K Wiebusch, CH Wille, L Williams, DR Wissing, H Wolf, M Wood, TR Woschnagg, K Xu, DL Xu, XW Xu, Y Yanez, JP Yodh, G Yoshida, S Zoll, M AF Aartsen, M. G. Abraham, K. Ackermann, M. Adams, J. Aguilar, J. A. Ahlers, M. Ahrens, M. Altmann, D. Anderson, T. Ansseau, I. Archinger, M. Arguelles, C. Arlen, T. C. Auffenberg, J. Bai, X. Barwick, S. W. Baum, V. Bay, R. Beatty, J. J. Tjus, J. Becker Becker, K. -H. Beiser, E. Benabderrahmane, M. L. Berghaus, P. Berley, D. Bernardini, E. Bernhard, A. Besson, D. Z. Binder, G. Bindig, D. Bissok, M. Blaufuss, E. Blumenthal, J. Boersma, D. J. Bohm, C. Boerner, M. Bos, F. Bose, D. Boeser, S. Botner, O. Braun, J. Brayeur, L. Bretz, H. -P. Buzinsky, N. Casey, J. Casier, M. Cheung, E. Chirkin, D. Christov, A. Clark, K. Classen, L. Coenders, S. Cowen, D. F. Silva, A. H. Cruz Daughhetee, J. Davis, J. C. Day, M. de Andre, J. P. A. M. De Clercq, C. Rosendo, E. del Pino Dembinski, H. De Ridder, S. Desiati, P. de Vries, K. D. de Wasseige, G. de With, M. DeYoung, T. Diaz-Velez, J. C. di Lorenzo, V. Dumm, J. P. Dunkman, M. Eberhardt, B. Ehrhardt, T. Eichmann, B. Euler, S. Evenson, P. A. Fahey, S. Fazely, A. R. Feintzeig, J. Felde, J. Filimonov, K. Finley, C. Fischer-Wasels, T. Flis, S. Foesig, C. -C. Fuchs, T. Gaisser, T. K. Gaior, R. Gallagher, J. Gerhardt, L. Ghorbani, K. Gier, D. Gladstone, L. Glagla, M. Gluesenkamp, T. Goldschmidt, A. Golup, G. Gonzalez, J. G. Gora, D. Grant, D. Griffith, Z. Gross, A. Ha, C. Haack, C. Ismail, A. Haj Hallgren, A. Halzen, F. Hansen, E. Hansmann, B. Hanson, K. Hebecker, D. Heereman, D. Helbing, K. Hellauer, R. Hickford, S. Hignight, J. Hill, G. C. Hoffman, K. D. Hoffmann, R. Holzapfel, K. Homeier, A. Hoshina, K. Huang, F. Huber, M. Huelsnitz, W. Hulth, P. O. Hultqvist, K. In, S. Ishihara, A. Jacobi, E. Japaridze, G. S. Jeong, M. Jero, K. Jurkovic, M. Kappes, A. Karg, T. Karle, A. Kauer, M. Keivani, A. Kelley, J. L. Kemp, J. Kheirandish, A. Kiryluk, J. Klaes, J. Klein, S. R. Kohnen, G. Koirala, R. Kolanoski, H. Konietz, R. Koepke, L. Kopper, C. Kopper, S. Koskinen, D. J. Kowalski, M. Krings, K. Kroll, G. Kroll, M. Krueckl, G. Kunnen, J. Kurahashi, N. Kuwabara, T. Labare, M. Lanfranchi, J. L. Larson, M. J. Lesiak-Bzdak, M. Leuermann, M. Leuner, J. Lu, L. Luenemann, J. Madsen, J. Maggi, G. Mahn, K. B. M. Mandelartz, M. Maruyama, R. Mase, K. Matis, H. S. Maunu, R. McNally, F. Meagher, K. Medici, M. Meli, A. Menne, T. Merino, G. Meures, T. Miarecki, S. Middell, E. Mohrmann, L. Montaruli, T. Morse, R. Nahnhauer, R. Naumann, U. Neer, G. Niederhausen, H. Nowicki, S. C. Nygren, D. R. Pollmann, A. Obertacke Olivas, A. Omairat, A. O'Murchadha, A. Palczewski, T. Pandya, H. Pankova, D. V. Paul, L. Pepper, J. A. de los Heros, C. Perez Pfendner, C. Pieloth, D. Pinat, E. Posselt, J. Price, P. B. Przybylski, G. T. Puetz, J. Quinnan, M. Raab, C. Raedel, L. Rameez, M. Rawlins, K. Reimann, R. Relich, M. Resconi, E. Rhode, W. Richman, M. Richter, S. Riedel, B. Robertson, S. Rongen, M. Rott, C. Ruhe, T. Ryckbosch, D. Sabbatini, L. Sander, H. -G. Sandrock, A. Sandroos, J. Sarkar, S. Schatto, K. Scheriau, F. Schimp, M. Schmidt, T. Schmitz, M. Schoenen, S. Schoeneberg, S. Schoenwald, A. Schulte, L. Schumacher, L. Seckel, D. Seunarine, S. Soldin, D. Song, M. Spiczak, G. M. Spiering, C. Stahlberg, M. Stamatikos, M. Stanev, T. Stasik, A. Steuer, A. Stezelberger, T. Stokstad, R. G. Stoessl, A. Strom, R. Strotjohann, N. L. Sullivan, G. W. Sutherland, M. Taavola, H. Taboada, I. Tatar, J. Ter-Antonyan, S. Terliuk, A. Tesic, G. Tilav, S. Toale, P. A. Tobin, M. N. Toscano, S. Tosi, D. Tselengidou, M. Turcati, A. Unger, E. Usner, M. Vallecorsa, S. Vandenbroucke, J. van Eijndhoven, N. Vanheule, S. van Santen, J. Veenkamp, J. Vehring, M. Voge, M. Vraeghe, M. Walck, C. Wallace, A. Wallraff, M. Wandkowsky, N. Weaver, Ch. Wendt, C. Westerhoff, S. Whelan, B. J. Wiebe, K. Wiebusch, C. H. Wille, L. Williams, D. R. Wissing, H. Wolf, M. Wood, T. R. Woschnagg, K. Xu, D. L. Xu, X. W. Xu, Y. Yanez, J. P. Yodh, G. Yoshida, S. Zoll, M. TI Searches for relativistic magnetic monopoles in IceCube SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID NEUTRINO TELESCOPE; PARTICLE; ICE; PERFORMANCE; SCATTERING; SPECTRUM; FIELD AB Various extensions of the Standard Model motivate the existence of stable magnetic monopoles that could have been created during an early high-energy epoch of the Universe. These primordial magnetic monopoles would be gradually accelerated by cosmic magnetic fields and could reach high velocities that make them visible in Cherenkov detectors such as IceCube. Equivalently to electrically charged particles, magnetic monopoles produce direct and indirect Cherenkov light while traversing through matter at relativistic velocities. This paper describes searches for relativistic (nu >= 0.76 c) and mildly relativistic (nu >= 0.51 c) monopoles, each using one year of data taken in 2008/2009 and 2011/2012, respectively. No monopole candidate was detected. For a velocity above 0.51 c the monopole flux is constrained down to a level of 1.55 x 10(-18) cm(-2) s(-1) sr(-1). This is an improvement of almost two orders of magnitude over previous limits. C1 [Auffenberg, J.; Bissok, M.; Blumenthal, J.; Gier, D.; Glagla, M.; Haack, C.; Hansmann, B.; Kemp, J.; Konietz, R.; Leuermann, M.; Leuner, J.; Paul, L.; Puetz, J.; Raedel, L.; Reimann, R.; Rongen, M.; Schimp, M.; Schoenen, S.; Schumacher, L.; Stahlberg, M.; Vehring, M.; Wallraff, M.; Wiebusch, C. H.] Rhein Westfal TH Aachen, Phys Inst 3, D-52056 Aachen, Germany. [Benabderrahmane, M. L.] New York Univ Abu Dhabi, Abu Dhabi, U Arab Emirates. [Aartsen, M. G.; Hill, G. C.; Robertson, S.; Wallace, A.; Whelan, B. J.] Univ Adelaide, Dept Phys, Adelaide, SA 5005, Australia. [Rawlins, K.] Univ Alaska Anchorage, Dept Phys & Astron, 3211 Providence Dr, Anchorage, AK 99508 USA. [Japaridze, G. S.] Clark Atlanta Univ, CTSPS, Atlanta, GA 30314 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Sch Phys, Atlanta, GA 30332 USA. [Casey, J.; Daughhetee, J.; Taboada, I.] Georgia Inst Technol, Ctr Relativist Astrophys, Atlanta, GA 30332 USA. [Fazely, A. R.; Ter-Antonyan, S.; Xu, X. W.] Southern Univ, Dept Phys, Baton Rouge, LA 70813 USA. [Bay, R.; Binder, G.; Filimonov, K.; Gerhardt, L.; Ha, C.; Klein, S. R.; Miarecki, S.; Price, P. B.; Tatar, J.; Woschnagg, K.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Binder, G.; Gerhardt, L.; Goldschmidt, A.; Ha, C.; Klein, S. R.; Matis, H. S.; Miarecki, S.; Nygren, D. R.; Przybylski, G. T.; Stezelberger, T.; Stokstad, R. G.; Tatar, J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [de With, M.; Hebecker, D.; Kolanoski, H.; Kowalski, M.] Humboldt Univ, Inst Phys, D-12489 Berlin, Germany. [Tjus, J. Becker; Bos, F.; Eichmann, B.; Kroll, M.; Mandelartz, M.; Schoeneberg, S.] Ruhr Univ Bochum, Fak Phys & Astron, D-44780 Bochum, Germany. [Homeier, A.; Schulte, L.; Voge, M.] Univ Bonn, Phys Inst, Nussallee 12, D-53115 Bonn, Germany. [Aguilar, J. A.; Ansseau, I.; Heereman, D.; Meagher, K.; Meures, T.; O'Murchadha, A.; Pinat, E.; Raab, C.] Univ Libre Bruxelles, Sci Fac CP230, B-1050 Brussels, Belgium. [Brayeur, L.; Casier, M.; De Clercq, C.; de Vries, K. D.; de Wasseige, G.; Golup, G.; Kunnen, J.; Luenemann, J.; Maggi, G.; Toscano, S.; van Eijndhoven, N.] Vrije Univ Brussel, Dienst ELEM, B-1050 Brussels, Belgium. [Gaior, R.; Ishihara, A.; Kuwabara, T.; Lu, L.; Mase, K.; Relich, M.; Yoshida, S.] Chiba Univ, Dept Phys, Chiba 2638522, Japan. [Adams, J.] Univ Canterbury, Dept Phys & Astron, Private Bag 4800, Christchurch 1, New Zealand. [Berley, D.; Blaufuss, E.; Cheung, E.; Felde, J.; Hellauer, R.; Hoffman, K. D.; Huelsnitz, W.; Maunu, R.; Olivas, A.; Schmidt, T.; Song, M.; Sullivan, G. W.; Wissing, H.] Univ Maryland, Dept Phys, College Pk, MD 20742 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Stamatikos, M.; Sutherland, M.] Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. [Beatty, J. J.; Davis, J. C.; Pfendner, C.; Stamatikos, M.; Sutherland, M.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, 174 W 18th Ave, Columbus, OH 43210 USA. [Beatty, J. J.] Ohio State Univ, Dept Astron, 174 W 18Th Ave, Columbus, OH 43210 USA. [Hansen, E.; Koskinen, D. J.; Larson, M. J.; Medici, M.; Sarkar, S.] Univ Copenhagen, Niels Bohr Inst, Blegdamsvej 17, DK-2100 Copenhagen, Denmark. [Boerner, M.; Fuchs, T.; Menne, T.; Pieloth, D.; Rhode, W.; Ruhe, T.; Sandrock, A.; Scheriau, F.; Schmitz, M.] TU Dortmund Univ, Dept Phys, D-44221 Dortmund, Germany. [de Andre, J. P. A. M.; DeYoung, T.; Hignight, J.; Mahn, K. B. M.; Neer, G.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Buzinsky, N.; Grant, D.; Kopper, C.; Nowicki, S. C.; Riedel, B.; Weaver, Ch.; Wood, T. R.] Univ Alberta, Dept Phys, Edmonton, AB T6G 2E1, Canada. [Altmann, D.; Classen, L.; Kappes, A.; Tselengidou, M.] Univ Erlangen Nurnberg, Erlangen Ctr Astroparticle Phys, D-91058 Erlangen, Germany. [Christov, A.; Montaruli, T.; Rameez, M.; Vallecorsa, S.] Univ Geneva, Dept Phys Nucl & Corpusculaire, CH-1211 Geneva, Switzerland. [De Ridder, S.; Ismail, A. Haj; Labare, M.; Meli, A.; Ryckbosch, D.; Vanheule, S.; Vraeghe, M.] Univ Ghent, Dept Phys & Astron, B-9000 Ghent, Belgium. [Barwick, S. W.; Yodh, G.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Besson, D. Z.] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. [Gallagher, J.] Univ Wisconsin, Dept Astron, Madison, WI 53706 USA. [Ahlers, M.; Arguelles, C.; Beiser, E.; Braun, J.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Fahey, S.; Feintzeig, J.; Ghorbani, K.; Gladstone, L.; Griffith, Z.; Halzen, F.; Hanson, K.; Hoshina, K.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kheirandish, A.; McNally, F.; Merino, G.; Morse, R.; Richter, S.; Sabbatini, L.; Tobin, M. N.; Tosi, D.; Vandenbroucke, J.; Wandkowsky, N.; Wendt, C.; Westerhoff, S.; Wille, L.; Xu, D. L.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Ahlers, M.; Arguelles, C.; Beiser, E.; Braun, J.; Chirkin, D.; Day, M.; Desiati, P.; Diaz-Velez, J. C.; Fahey, S.; Feintzeig, J.; Ghorbani, K.; Gladstone, L.; Griffith, Z.; Halzen, F.; Hanson, K.; Hoshina, K.; Jero, K.; Karle, A.; Kauer, M.; Kelley, J. L.; Kheirandish, A.; McNally, F.; Merino, G.; Morse, R.; Richter, S.; Sabbatini, L.; Tobin, M. N.; Tosi, D.; Vandenbroucke, J.; Wandkowsky, N.; Wendt, C.; Westerhoff, S.; Wille, L.; Xu, D. L.] Univ Wisconsin, Wisconsin IceCube Particle Astrophys Ctr, 1150 Univ Ave, Madison, WI 53706 USA. [Archinger, M.; Baum, V.; Boeser, S.; Rosendo, E. del Pino; di Lorenzo, V.; Eberhardt, B.; Ehrhardt, T.; Foesig, C. -C.; Koepke, L.; Kroll, G.; Krueckl, G.; Sander, H. -G.; Sandroos, J.; Schatto, K.; Steuer, A.; Wiebe, K.] Johannes Gutenberg Univ Mainz, Inst Phys, Staudinger Weg 7, D-55099 Mainz, Germany. [Kohnen, G.] Univ Mons, B-7000 Mons, Belgium. [Abraham, K.; Bernhard, A.; Coenders, S.; Gross, A.; Holzapfel, K.; Huber, M.; Jurkovic, M.; Krings, K.; Resconi, E.; Turcati, A.; Veenkamp, J.] Tech Univ Munich, D-85748 Garching, Germany. [Dembinski, H.; Evenson, P. A.; Gaisser, T. K.; Gonzalez, J. G.; Koirala, R.; Pandya, H.; Seckel, D.; Stanev, T.; Tilav, S.] Univ Delaware, Bartol Res Inst, Dept Phys & Astron, Newark, DE 19716 USA. [Kauer, M.; Maruyama, R.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Sarkar, S.] Univ Oxford, Dept Phys, 1 Keble Rd, Oxford OX1 3NP, England. [Kurahashi, N.; Richman, M.] Drexel Univ, Dept Phys, 3141 Chestnut St, Philadelphia, PA 19104 USA. [Bai, X.] South Dakota Sch Mines & Technol, Dept Phys, Rapid City, SD 57701 USA. [Madsen, J.; Seunarine, S.; Spiczak, G. M.] Univ Wisconsin, Dept Phys, River Falls, WI 54022 USA. [Ahrens, M.; Bohm, C.; Dumm, J. P.; Finley, C.; Flis, S.; Hulth, P. O.; Hultqvist, K.; Walck, C.; Wolf, M.; Zoll, M.] Stockholm Univ, Oskar Klein Ctr, Dept Phys, S-10691 Stockholm, Sweden. [Kiryluk, J.; Lesiak-Bzdak, M.; Niederhausen, H.; Xu, Y.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Bose, D.; In, S.; Jeong, M.; Rott, C.] Sungkyunkwan Univ, Dept Phys, Suwon 440746, South Korea. [Clark, K.] Univ Toronto, Dept Phys, 60 St George St, Toronto, ON M5S 1A7, Canada. [Palczewski, T.; Pepper, J. A.; Toale, P. A.; Williams, D. R.] Univ Alabama, Dept Phys & Astron, Tuscaloosa, AL 35487 USA. [Cowen, D. F.] Penn State Univ, Dept Astron & Astrophys, 525 Davey Lab, University Pk, PA 16802 USA. [Anderson, T.; Arlen, T. C.; Cowen, D. F.; Dunkman, M.; Huang, F.; Keivani, A.; Lanfranchi, J. L.; Pankova, D. V.; Quinnan, M.; Tesic, G.] Penn State Univ, Dept Phys, 104 Davey Lab, University Pk, PA 16802 USA. [Boersma, D. J.; Botner, O.; Euler, S.; Hallgren, A.; de los Heros, C. Perez; Strom, R.; Taavola, H.; Unger, E.] Uppsala Univ, Dept Phys & Astron, Box 516, S-75120 Uppsala, Sweden. [Becker, K. -H.; Bindig, D.; Fischer-Wasels, T.; Helbing, K.; Hickford, S.; Hoffmann, R.; Klaes, J.; Kopper, S.; Naumann, U.; Pollmann, A. Obertacke; Omairat, A.; Posselt, J.; Soldin, D.] Univ Wuppertal, Dept Phys, D-42119 Wuppertal, Germany. [Ackermann, M.; Berghaus, P.; Bernardini, E.; Bretz, H. -P.; Silva, A. H. Cruz; Gluesenkamp, T.; Gora, D.; Jacobi, E.; Karg, T.; Kowalski, M.; Middell, E.; Mohrmann, L.; Nahnhauer, R.; Schoenwald, A.; Spiering, C.; Stasik, A.; Stoessl, A.; Strotjohann, N. L.; Terliuk, A.; Usner, M.; van Santen, J.; Yanez, J. P.] DESY, D-15735 Zeuthen, Germany. [Hoshina, K.] Univ Tokyo, Earthquake Res Inst, Bunkyo Ku, Tokyo 1130032, Japan. [Stamatikos, M.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Pollmann, AO; Posselt, J (reprint author), Univ Wuppertal, Dept Phys, D-42119 Wuppertal, Germany. EM anna.pollmann@uni-wuppertal.de; jposselt@icecube.wisc.edu RI Tjus, Julia/G-8145-2012; Koskinen, David/G-3236-2014; Maruyama, Reina/A-1064-2013; Beatty, James/D-9310-2011; Wiebusch, Christopher/G-6490-2012; Sarkar, Subir/G-5978-2011 OI Koskinen, David/0000-0002-0514-5917; Perez de los Heros, Carlos/0000-0002-2084-5866; Dembinski, Hans/0000-0003-3337-3850; Arguelles Delgado, Carlos/0000-0003-4186-4182; Maruyama, Reina/0000-0003-2794-512X; Beatty, James/0000-0003-0481-4952; Wiebusch, Christopher/0000-0002-6418-3008; Sarkar, Subir/0000-0002-3542-858X FU U.S. National Science Foundation-Office of Polar Programs; U.S. National Science Foundation-Physics Division; University of Wisconsin Alumni Research Foundation; Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin - Madison; Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy; National Energy Research Scientific Computing Center; Louisiana Optical Network Initiative (LONI); Natural Sciences and Engineering Research Council of Canada; West-Grid and Compute/Calcul Canada; Swedish Research Council; Swedish Polar Research Secretariat; Swedish National Infrastructure for Computing (SNIC); Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF); Deutsche Forschungsgemeinschaft (DFG); Helmholtz Alliance for Astroparticle Physics (HAP); Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO); FWO Odysseus programme; Flanders Institute to encourage scientific and technological research in industry (IWT); Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF) FX We acknowledge the support from the following agencies: U.S. National Science Foundation-Office of Polar Programs, U.S. National Science Foundation-Physics Division, University of Wisconsin Alumni Research Foundation, the Grid Laboratory Of Wisconsin (GLOW) grid infrastructure at the University of Wisconsin - Madison, the Open Science Grid (OSG) grid infrastructure; U.S. Department of Energy, and National Energy Research Scientific Computing Center, the Louisiana Optical Network Initiative (LONI) grid computing resources; Natural Sciences and Engineering Research Council of Canada, West-Grid and Compute/Calcul Canada; Swedish Research Council, Swedish Polar Research Secretariat, Swedish National Infrastructure for Computing (SNIC), and Knut and Alice Wallenberg Foundation, Sweden; German Ministry for Education and Research (BMBF), Deutsche Forschungsgemeinschaft (DFG), Helmholtz Alliance for Astroparticle Physics (HAP), Research Department of Plasmas with Complex Interactions (Bochum), Germany; Fund for Scientific Research (FNRS-FWO), FWO Odysseus programme, Flanders Institute to encourage scientific and technological research in industry (IWT), Belgian Federal Science Policy Office (Belspo); University of Oxford, United Kingdom; Marsden Fund, New Zealand; Australian Research Council; Japan Society for Promotion of Science (JSPS); the Swiss National Science Foundation (SNSF), Switzerland; National Research Foundation of Korea (NRF); Danish National Research Foundation, Denmark (DNRF). NR 58 TC 4 Z9 4 U1 0 U2 5 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD MAR 10 PY 2016 VL 76 IS 3 AR 133 DI 10.1140/epjc/s10052-016-3953-8 PG 16 WC Physics, Particles & Fields SC Physics GA DG7WL UT WOS:000372294300002 ER PT J AU Balokovic, M Paneque, D Madejski, G Furniss, A Chiang, J Ajell, M Alexander, DM Barret, D Blandford, RD Boggs, SE Christensen, FE Craig, WW Forster, K Giommi, P Grefenstette, B Hailey, C Harrison, FA Hornstrup, A Kitaguchi, T Koglin, JE Madsen, KK Mao, PH Miyasaka, H Mori, K Perri, M Pivovaroff, MJ Puccetti, S Rana, V Stern, D Tagliaferri, G Urry, CM Estergaard, NJW Zhang, WW Zoglauer, A Archambault, S Archer, A Barnacka, A Benbow, W Bird, R Buckley, JH Bugaev, V Cerruti, M Chen, X Ciupik, L Connolly, MP Cui, W Dickinson, HJ Dumm, J Eisch, JD Falcone, A Feng, Q Finley, JP Fleischhack, H Fortson, L Griffin, S Griffiths, ST Grube, J Gyuk, G Huetten, M Hakansson, N Holder, J Humensky, TB Johnson, CA Kaaret, P Kertzman, M Khassen, Y Kieda, D Krause, M Krennrich, F Lang, MJ Maier, G McArthur, S Meagher, K Moriarty, P Nelson, T Nieto, D Ong, RA Park, N Poiil, M Popkow, A Pueschel, E Reynolds, PT Richards, GT Roache, E Santander, M Sembroski, GH Shahinyan, K Smith, AW Staszak, D Telezhinsky, I Todd, NW Tucci, JV Tyler, J Vincent, S Weinstein, A Wilhelm, A Williams, DA Zitzer, B Ahnen, ML Ansoldi, S Antonelli, LA Antoranz, P Babic, A Banerjee, B Bangale, P de Almeida, UB Barrio, JA Gonzalez, JB Bednarek, W Bernardini, E Biasuzzi, B Biland, A Blanch, O Bonnefoy, S Bonnoli, G Borracci, F Bretz, T Carmona, E Carosi, A Chatterjee, A Clavero, R Colin, P Colombo, E Contreras, JL Cortina, J Covino, S Da Vela, P Dazzi, F De Angelis, A De Lotto, B Wilhelmi, ED Mendez, CD Di Pierro, E Prester, DD Dorner, D Doro, M Einecke, S Elsaesser, D Fernandez-Barral, A Fidalgo, D Fonseca, MV Font, L Frantzen, K Fruck, C Galindo, D Lopez, JG Garczarczyk, M Terrats, DG Gaug, M Giammaria, P Glawion, D Gouinovic, N Munoz, AG Guberman, D Hahn, A Hanabata, Y Hayashida, M Herrera, J Hose, J Hrupec, D Hughes, G Idec, W Kodani, K Konno, Y Kubo, H Kushida, J La Barbera, A Lelas, D Lindfors, E Lombardi, S Longo, F Lopez, M Lopez-Coto, R Lopez-Oramas, A Lorenz, E Majumdar, P Makariev, M Mallot, K Maneva, G Manganaro, M Mannheim, K Maraschi, L Marcote, B Mariotti, M Martinez, M Mazin, D Menzel, U Miranda, JM Mirzoyan, R Moralejo, A Moretti, E Nakajima, D Neustroev, V Niedzwiecki, A Rosillo, MN Nilsson, K Nishijima, K Noda, K Orito, R Overkemping, A Paiano, S Palacio, J Palatiello, M Paoletti, R Paredes, JM Paredes-Fortuny, X Persic, M Poutanen, J Moroni, PGP Prandini, E Puljak, I Rhode, W Ribo, M Rico, J Garcia, JR Saito, T Satalecka, K Scapin, V Schultz, C Schweizer, T Shore, SN Sillanpaa, A Sitarek, J Snidaric, I Sobczynska, D Stamerra, A Steinbring, T Strzys, M Takalo, L Takami, H Tavecchio, F Temnikov, P Terzic, T Tescaro, D Teshima, M Thaele, J Torres, DF Toyama, T Treves, A Verguilov, V Vovk, I Ward, JE Will, M Wu, MH Zanin, R Perkins, J Verrecchia, F Leto, C Bottcher, M Villata, M Raiteri, CM Acosta-Pulido, JA Bachev, R Berdyugin, A Blinov, DA Carnerero, MI Chen, WP Chinchilla, P Damljanovic, G Eswaraiah, C Grisinna, TS Ibryamov, S Jordan, B Jorstad, SG Joshi, M Kopatskaya, EN Kurtanidze, OM Kurtanidze, SO Larionova, EG Larionova, LV Larionov, VM Latev, G Lin, HC Marscher, AP Mokrushina, AA Morozova, DA Nikolashvili, MG Semkov, E Smith, PS Strigachev, A Troitskaya, YV Troitsky, IS Vince, O Barnes, J Guver, T Moody, JW Sadun, AC Sun, S Hovatta, T Richards, JL Max-Moerbeck, W Readhead, ACR Lahteenmaki, A Tornikoski, M Tammi, J Ramakrishnan, V Reinthal, R Angelakis, E Fuhrmann, L Myserlis, I Karamanavis, V Sievers, A Ungerechts, H Zensus, JA AF Balokovic, M. Paneque, D. Madejski, G. Furniss, A. Chiang, J. Ajell, M. Alexander, D. M. Barret, D. Blandford, R. D. Boggs, S. E. Christensen, F. E. Craig, W. W. Forster, K. Giommi, P. Grefenstette, B. Hailey, C. Harrison, F. A. Hornstrup, A. Kitaguchi, T. Koglin, J. E. Madsen, K. K. Mao, P. H. Miyasaka, H. Mori, K. Perri, M. Pivovaroff, M. J. Puccetti, S. Rana, V. Stern, D. Tagliaferri, G. Urry, C. M. Estergaard, N. J. W. Zhang, W. W. Zoglauer, A. Archambault, S. Archer, A. Barnacka, A. Benbow, W. Bird, R. Buckley, J. H. Bugaev, V. Cerruti, M. Chen, X. Ciupik, L. Connolly, M. P. Cui, W. Dickinson, H. J. Dumm, J. Eisch, J. D. Falcone, A. Feng, Q. Finley, J. P. Fleischhack, H. Fortson, L. Griffin, S. Griffiths, S. T. Grube, J. Gyuk, G. Huetten, M. Hakansson, N. Holder, J. Humensky, T. B. Johnson, C. A. Kaaret, P. Kertzman, M. Khassen, Y. Kieda, D. Krause, M. Krennrich, F. Lang, M. J. Maier, G. McArthur, S. Meagher, K. Moriarty, P. Nelson, T. Nieto, D. Ong, R. A. Park, N. Poiil, M. Popkow, A. Pueschel, E. Reynolds, P. T. Richards, G. T. Roache, E. Santander, M. Sembroski, G. H. Shahinyan, K. Smith, A. W. Staszak, D. Telezhinsky, I. Todd, N. W. Tucci, J. V. Tyler, J. Vincent, S. Weinstein, A. Wilhelm, A. Williams, D. A. Zitzer, B. Ahnen, M. L. Ansoldi, S. Antonelli, L. A. Antoranz, P. Babic, A. Banerjee, B. Bangale, P. Barres de Almeida, U. Barrio, J. A. Becerra Gonzalez, J. Bednarek, W. Bernardini, E. Biasuzzi, B. Biland, A. Blanch, O. Bonnefoy, S. Bonnoli, G. Borracci, F. Bretz, T. Carmona, E. Carosi, A. Chatterjee, A. Clavero, R. Colin, P. Colombo, E. Contreras, J. L. Cortina, J. Covino, S. Da Vela, P. Dazzi, F. De Angelis, A. De Lotto, B. de Ona Wilhelmi, E. Delgado Mendez, C. Di Pierro, E. Prester, D. Dominis Dorner, D. Doro, M. Einecke, S. Elsaesser, D. Fernandez-Barral, A. Fidalgo, D. Fonseca, M. V. Font, L. Frantzen, K. Fruck, C. Galindo, D. Garcia Lopez, J. Garczarczyk, M. Terrats, D. Garrido Gaug, M. Giammaria, P. Glawion (Eisenacher), D. Gouinovic, N. Gonzalez Munoz, A. Guberman, D. Hahn, A. Hanabata, Y. Hayashida, M. Herrera, J. Hose, J. Hrupec, D. Hughes, G. Idec, W. Kodani, K. Konno, Y. Kubo, H. Kushida, J. La Barbera, A. Lelas, D. Lindfors, E. Lombardi, S. Longo, F. Lopez, M. Lopez-Coto, R. Lopez-Oramas, A. Lorenz, E. Majumdar, P. Makariev, M. Mallot, K. Maneva, G. Manganaro, M. Mannheim, K. Maraschi, L. Marcote, B. Mariotti, M. Martinez, M. Mazin, D. Menzel, U. Miranda, J. M. Mirzoyan, R. Moralejo, A. Moretti, E. Nakajima, D. Neustroev, V. Niedzwiecki, A. Rosillo, M. Nievas Nilsson, K. Nishijima, K. Noda, K. Orito, R. Overkemping, A. Paiano, S. Palacio, J. Palatiello, M. Paoletti, R. Paredes, J. M. Paredes-Fortuny, X. Persic, M. Poutanen, J. Moroni, P. G. Prada Prandini, E. Puljak, I. Rhode, W. Ribo, M. Rico, J. Rodriguez Garcia, J. Saito, T. Satalecka, K. Scapin, V. Schultz, C. Schweizer, T. Shore, S. N. Sillanpaa, A. Sitarek, J. Snidaric, I. Sobczynska, D. Stamerra, A. Steinbring, T. Strzys, M. Takalo, L. Takami, H. Tavecchio, F. Temnikov, P. Terzic, T. Tescaro, D. Teshima, M. Thaele, J. Torres, D. F. Toyama, T. Treves, A. Verguilov, V. Vovk, I. Ward, J. E. Will, M. Wu, M. H. Zanin, R. Perkins, J. Verrecchia, F. Leto, C. Boettcher, M. Villata, M. Raiteri, C. M. Acosta-Pulido, J. A. Bachev, R. Berdyugin, A. Blinov, D. A. Carnerero, M. I. Chen, W. P. Chinchilla, P. Damljanovic, G. Eswaraiah, C. Grisinna, T. S. Ibryamov, S. Jordan, B. Jorstad, S. G. Joshi, M. Kopatskaya, E. N. Kurtanidze, O. M. Kurtanidze, S. O. Larionova, E. G. Larionova, L. V. Larionov, V. M. Latev, G. Lin, H. C. Marscher, A. P. Mokrushina, A. A. Morozova, D. A. Nikolashvili, M. G. Semkov, E. Smith, P. S. Strigachev, A. Troitskaya, Yu. V. Troitsky, I. S. Vince, O. Barnes, J. Guever, T. Moody, J. W. Sadun, A. C. Sun, S. Hovatta, T. Richards, J. L. Max-Moerbeck, W. Readhead, A. C. R. Lahteenmaki, A. Tornikoski, M. Tammi, J. Ramakrishnan, V. Reinthal, R. Angelakis, E. Fuhrmann, L. Myserlis, I. Karamanavis, V. Sievers, A. Ungerechts, H. Zensus, J. A. CA NuSTAR Team VERITAS Collaboration MAGIC Collaboration TI MULTIWAVELENGTH STUDY OF QUIESCENT STATES OF Mrk 421 WITH UNPRECEDENTED HARD X-RAY COVERAGE PROVIDED BY NuSTAR IN 2013 SO ASTROPHYSICAL JOURNAL LA English DT Article DE BL Lacertae objects: individual (Markarian 421); galaxies: active; gamma rays: general; radiation mechanisms: nonthermal; X-rays: galaxies ID ACTIVE GALACTIC NUCLEI; LARGE-AREA TELESCOPE; BL LACERTAE OBJECTS; PARTICLE-ACCELERATION; LAC OBJECTS; CORRELATED VARIABILITY; TEV BLAZARS; ELECTRON ACCELERATION; MAGNETIC RECONNECTION; BACKGROUND-RADIATION AB We present coordinated multiwavelength observations of the bright, nearby BL Lacertae object Mrk 421 taken in 2013 January-March, involving GASP-WEBT, Swift, NuSTAR, Fermi-LAT, MAGIC, VERITAS, and other collaborations and instruments, providing data from radio to very high energy. (VHE).-ray bands. NuSTAR yielded previously unattainable sensitivity in the 3-79. keV range, revealing that the spectrum softens when the source is dimmer until the X-ray spectral shape saturates into a steep Gamma approximate to 3 power law, with no evidence for an exponential cutoff or additional hard components up to similar to 80. keV. For the first time, we observed both the synchrotron and the inverse-Compton peaks of the spectral energy distribution (SED) simultaneously shifted to frequencies below the typical quiescent state by an order of magnitude. The fractional variability as a function of photon energy shows a double-bump structure that relates to the two bumps of the broadband SED. In each bump, the variability increases with energy, which, in the framework of the synchrotron self-Compton model, implies that the electrons with higher energies are more variable. The measured multi band variability, the significant X-ray-to-VHE correlation down to some of the lowest fluxes ever observed in both bands, the lack of correlation between optical/UV and X-ray flux, the low degree of polarization and its significant (random) variations, the short estimated electron cooling time, and the significantly longer variability timescale observed in the NuSTAR light curves point toward in situ electron acceleration and suggest that there are multiple compact regions contributing to the broadband emission of Mrk 421 during low-activity states. C1 [Balokovic, M.; Forster, K.; Grefenstette, B.; Harrison, F. A.; Madsen, K. K.; Mao, P. H.; Miyasaka, H.; Rana, V.; Hovatta, T.; Readhead, A. C. R.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. 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RP Balokovic, M (reprint author), CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA.; Paneque, D (reprint author), Max Planck Inst Phys & Astrophys, D-80805 Munich, Germany.; Madejski, G; Chiang, J (reprint author), Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, WW Hansen Expt Phys Lab, Dept Phys, Stanford, CA 94305 USA.; Madejski, G; Chiang, J (reprint author), Stanford Univ, SLAC Natl Accelerator Lab, Stanford, CA 94305 USA.; Furniss, A (reprint author), Stanford Univ, Dept Phys, Stanford, CA 94305 USA. EM mislavb@astro.caltech.edu; dpaneque@mppmu.mpg.de; madejski@stanford.edu; amy.furniss@gmail.com; jchiang@slac.stanford.edu RI Troitskiy, Ivan/K-7979-2013; Jorstad, Svetlana/H-6913-2013; Larionov, Valeri/H-1349-2013; Grishina, Tatiana/H-6873-2013; Miranda, Jose Miguel/F-2913-2013; Blinov, Dmitry/G-9925-2013; Delgado, Carlos/K-7587-2014; Torres, Diego/O-9422-2016; Barrio, Juan/L-3227-2014; GAug, Markus/L-2340-2014; Cortina, Juan/C-2783-2017; Morozova, Daria/H-1298-2013; Larionova, Elena/H-7287-2013; Lahteenmaki, Anne/L-5987-2013; Font, Lluis/L-4197-2014; Nieto, Daniel/J-7250-2015; Poutanen, Juri/H-6651-2016; Contreras Gonzalez, Jose Luis/K-7255-2014; Manganaro, Marina/B-7657-2011; Boggs, Steven/E-4170-2015; Lopez Moya, Marcos/L-2304-2014; Temnikov, Petar/L-6999-2016; Maneva, Galina/L-7120-2016; Makariev, Martin/M-2122-2016; Ramakrishnan, Venkatessh/C-8628-2017; Puljak, Ivica/D-8917-2017; OI Karamanavis, Vassilis/0000-0003-3133-2617; Angelakis, Emmanouil/0000-0001-7327-5441; Urry, Meg/0000-0002-0745-9792; de Ona Wilhelmi, Emma/0000-0002-5401-0744; Bonnoli, Giacomo/0000-0003-2464-9077; Prandini, Elisa/0000-0003-4502-9053; Becerra Gonzalez, Josefa/0000-0002-6729-9022; Troitskiy, Ivan/0000-0002-4218-0148; Jorstad, Svetlana/0000-0001-9522-5453; Larionov, Valeri/0000-0002-4640-4356; Grishina, Tatiana/0000-0002-3953-6676; Miranda, Jose Miguel/0000-0002-1472-9690; Blinov, Dmitry/0000-0003-0611-5784; Delgado, Carlos/0000-0002-7014-4101; Torres, Diego/0000-0002-1522-9065; Barrio, Juan/0000-0002-0965-0259; GAug, Markus/0000-0001-8442-7877; Cortina, Juan/0000-0003-4576-0452; Morozova, Daria/0000-0002-9407-7804; Larionova, Elena/0000-0002-2471-6500; Font, Lluis/0000-0003-2109-5961; Nieto, Daniel/0000-0003-3343-0755; Poutanen, Juri/0000-0002-0983-0049; Contreras Gonzalez, Jose Luis/0000-0001-7282-2394; Manganaro, Marina/0000-0003-1530-3031; Boggs, Steven/0000-0001-9567-4224; Lopez Moya, Marcos/0000-0002-8791-7908; Temnikov, Petar/0000-0002-9559-3384; Ramakrishnan, Venkatessh/0000-0002-9248-086X; Villata, Massimo/0000-0003-1743-6946; Pueschel, Elisa/0000-0002-0529-1973; Rana, Vikram/0000-0003-1703-8796; Krause, Maria/0000-0001-7595-0914; Bird, Ralph/0000-0002-4596-8563 FU International Fulbright Science and Technology Award; NASA Headquarters under the NASA Earth and Space Science Fellowship Program [NNX14AQ07H]; Department of Energy [DE-AC02-765F00515]; NASA [NNX13AO97G, NNG08FD60C, NNX12AO90G, NNX14AQ58G]; French Space Agency (CNES); National Aeronautics and Space Administration; U.S. Department of Energy Office of Science; U.S. National Science Foundation; Smithsonian Institution; NSERC in Canada; STFC in the U.K.; German BMBF; MPG; Italian INFN; INAF; Swiss National Fund SNF; ERDF under the Spanish MINECO; Japanese JSPS; MEXT; Centro de Excelencia Severo Ochoa [SEV-2012-0234, CPAN CSD2007-00042]; Spanish Consolider-Ingenio programme [CSD2009-00064]; Academy of Finland [268740, 212656, 210338, 121148]; Croatian Science Foundation (HrZZ) Project [09/176]; University of Rijeka [13.12.1.3.02]; DFG Collaborative Research Centers [SH3823/C4, SH3876/C3]; Polish MNiSzW grant [745/N-HESS-MAGIC/2010/0]; Russian RFBR [15-02-00949]; St. Petersburg University [6.38.335.2015]; South African Research Chairs Initiative (SARChI) of the Department of Science and Technology; National Research Foundation of South Africa; Institute of Astronomy and Rozhen National Astronomical Observatory, Bulgaria Academy of Sciences; Ministry of Education, Science, and Technological Development of the Republic of Serbia [176011, 176004, 176021]; Scientific Research Fund of the Bulgarian Ministry of Education and Sciences [DO 02-137 (BIn-13/09)]; Shota Rustaveli National Science Foundation [FR/638/6-320/12, 31/77]; Istanbul University [49429, 48285]; Bilim Akademisi (BAGEP program); TUBITAK [13AT100-431, 13AT100-466, 13AT60-430]; NASA grants [NNX08AW31G, NNX11A043G]; NSF grants [AST-0808050, AST-1109911] FX M.B. acknowledges support from the International Fulbright Science and Technology Award, and from NASA Headquarters under the NASA Earth and Space Science Fellowship Program, grant NNX14AQ07H. This research was supported in part by the Department of Energy Contract DE-ACO2-765F00515 to the SLAC National Accelerator Center. G.M. and A.F. acknowledge the support via NASA grant NNX13AO97G. D.B. acknowledges support from the French Space Agency (CNES) for financial support.; This work was supported under NASA Contract No. NNG08FD60C and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA).; VERITAS is supported by grants from the U.S. Department of Energy Office of Science, the U.S. National Science Foundation, and the Smithsonian Institution, by NSERC in Canada, and by STFC in the U.K. We acknowledge the excellent work of the technical support staff at the Fred Lawrence Whipple Observatory and at the collaborating institutions in the construction and operation of the instrument. The VERITAS Collaboration is grateful to Trevor Weekes for his seminal contributions and leadership in the field of VHE gamma-ray astrophysics, which made this study possible.; The MAGIC Collaboration would like to thank the Institute de Astrofisica de Canarias for the excellent working conditions at the Observatorio del Roque de los Muchachos in La Palma. The financial support of the German BMBF and MPG, the Italian INFN and INAF, the Swiss National Fund SNF, the ERDF under the Spanish MINECO, and the Japanese JSPS and MEXT is gratefully acknowledged. This work was also supported by the Centro de Excelencia Severo Ochoa SEV-2012-0234, CPAN CSD2007-00042, and MultiDark CSD2009-00064 projects of the Spanish Consolider-Ingenio 2010 programme, by grant 268740 of the Academy of Finland, by the Croatian Science Foundation (HrZZ) Project 09/176 and the University of Rijeka Project 13.12.1.3.02, by the DFG Collaborative Research Centers SH3823/C4 and SH3876/C3, and by the Polish MNiSzW grant 745/N-HESS-MAGIC/2010/0.; The St. Petersburg University team acknowledges support from Russian RFBR grant 15-02-00949 and St. Petersburg University research grant 6.38.335.2015.; The work of M.B. is supported by the South African Research Chairs Initiative (SARChI) of the Department of Science and Technology and the National Research Foundation of South Africa. Any opinion, finding, and conclusion or recommendation expressed in this material is that of the authors and the NRF does not accept any liability in this regard.; G.D. and O.V. gratefully acknowledge the observing grant support from the Institute of Astronomy and Rozhen National Astronomical Observatory, Bulgaria Academy of Sciences. This work is a part of the Projects No. 176011 (Dynamics and kinematics of celestial bodies and systems), No. 176004 (Stellar physics), and No. 176021 (Visible and invisible matter in nearby galaxies: theory and observations) supported by the Ministry of Education, Science, and Technological Development of the Republic of Serbia.; This research was partially supported by the Scientific Research Fund of the Bulgarian Ministry of Education and Sciences under grant DO 02-137 (BIn-13/09).; The Abastumani team acknowledges financial support of the project FR/638/6-320/12 by the Shota Rustaveli National Science Foundation under contract 31/77.; T.G. acknowledges support from Istanbul University (Project numbers 49429 and 48285), Bilim Akademisi (BAGEP program), and TUBITAK (project numbers 13AT100-431, 13AT100-466, and 13AT60-430).; The Boston University effort was supported in part by NASA grants NNX12AO90G and NNX14AQ58G.; The OVRO 40 m monitoring program is supported in part by NASA grants NNX08AW31G and NNX11A043G and NSF grants AST-0808050 and AST-1109911.; The Metsahovi team acknowledges the support from the Academy of Finland to our observing projects (numbers 212656, 210338, 121148, and others). NR 120 TC 9 Z9 9 U1 7 U2 20 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 10 PY 2016 VL 819 IS 2 AR 156 DI 10.3847/0004-637X/819/2/156 PG 30 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG8AV UT WOS:000372305700068 ER PT J AU Bard, D Kratochvil, JM Dawson, W AF Bard, D. Kratochvil, J. M. Dawson, W. TI MASKED AREAS IN SHEAR PEAK STATISTICS: A FORWARD MODELING APPROACH SO ASTROPHYSICAL JOURNAL LA English DT Article DE dark energy; gravitational lensing: weak ID PRIMORDIAL NON-GAUSSIANITY; WEAK LENSING SURVEYS; COSMIC SHEAR; SIMULATION; COSMOLOGY; CLUSTERS AB The statistics of shear peaks have been shown to provide valuable cosmological information beyond the power spectrum, and will be an important constraint of models of cosmology in forthcoming astronomical surveys. Surveys include masked areas due to bright stars, bad pixels etc., which must be accounted for in producing constraints on cosmology from shear maps. We advocate a forward-modeling approach, where the impacts of masking and other survey artifacts are accounted for in the theoretical prediction of cosmological parameters, rather than correcting survey data to remove them. We use masks based on the Deep Lens Survey, and explore the impact of up to 37% of the survey area being masked on LSST and DES-scale surveys. By reconstructing maps of aperture mass the masking effect is smoothed out, resulting in up to 14% smaller statistical uncertainties compared to simply reducing the survey area by the masked area. We show that, even in the presence of large survey masks, the bias in cosmological parameter estimation produced in the forward-modeling process is approximate to 1%, dominated by bias caused by limited simulation volume. We also explore how this potential bias scales with survey area and evaluate how much small survey areas are impacted by the differences in cosmological structure in the data and simulated volumes, due to cosmic variance. C1 [Bard, D.] SLAC Natl Accelerator Lab, KIPAC, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Kratochvil, J. M.] Univ KwaZulu Natal, Astrophys & Cosmol Res Unit, ZA-4000 Durban, South Africa. [Dawson, W.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. RP Bard, D (reprint author), SLAC Natl Accelerator Lab, KIPAC, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. EM djbard@slac.stanford.edu FU NSF [AST-1108893]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors would like to thank Tony Tyson and Rachel Mandelbaum for their careful review of this paper on behalf of the LSST collaboration, and the anonymous journal referee for their excellent and productive feedback. The authors would also like to thank Michael Schneider for very helpful discussions, particularly related to aspects concerning the simulations and inferred cosmological constraints. We also thank the Deep Lens Survey for the survey masks used in this analysis, in particular Perry Gee who generated the bulk of the masks. WD was supported in part by the NSF under Grant No. AST-1108893. This work performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. NR 42 TC 0 Z9 0 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 10 PY 2016 VL 819 IS 2 AR 158 DI 10.3847/0004-637X/819/2/158 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG8AV UT WOS:000372305700070 ER PT J AU Belczynski, K Repetto, S Holz, DE O'Shaughnessy, R Bulik, T Berti, E Fryer, C Dominik, M AF Belczynski, Krzysztof Repetto, Serena Holz, Daniel E. O'Shaughnessy, Richard Bulik, Tomasz Berti, Emanuele Fryer, Christopher Dominik, Michal TI COMPACT BINARY MERGER RATES: COMPARISON WITH LIGO/VIRGO UPPER LIMITS SO ASTROPHYSICAL JOURNAL LA English DT Article DE binaries: close; gravitation; stars: evolution; stars: neutron ID MASS BLACK-HOLE; SUPERNOVA EXPLOSION MECHANISM; GRAVITATIONAL-WAVE DETECTION; NOVA-OPHIUCHI 1977; X-RAY BINARIES; NEUTRINO-DRIVEN EXPLOSIONS; COMMON ENVELOPE EVOLUTION; RADIAL-VELOCITY SURVEY; IC 10 X-1; OBJECT FORMATION AB We compare evolutionary predictions of double compact object merger rate densities with initial and forthcoming LIGO/Virgo upper limits. We find that: (i) Due to the cosmological reach of advanced detectors, current conversion methods of population synthesis predictions into merger rate densities are insufficient. (ii) Our optimistic models are a factor of 18 below the initial LIGO/Virgo upper limits for BH-BH systems, indicating that a modest increase in observational sensitivity (by a factor of similar to 2.5) may bring the first detections or first gravitational wave constraints on binary evolution. (iii) Stellar-origin massive BH-BH mergers should dominate event rates in advanced LIGO/Virgo and can be detected out to redshift z similar or equal to 2 with templates including inspiral, merger, and ringdown. Normal stars (< 150 M-circle dot) can produce such mergers with total redshifted mass up to M-tot,M-z similar or equal to 400M(circle dot). (iv) High black hole (BH) natal kicks can severely limit the formation of massive BH-BH systems (both in isolated binary and in dynamical dense cluster evolution), and thus would eliminate detection of these systems even at full advanced LIGO/Virgo sensitivity. We find that low and high BH natal kicks are allowed by current observational electromagnetic constraints. (v) The majority of our models yield detections of all types of mergers (NS-NS, BH-NS, BH-BH) with advanced detectors. Numerous massive BH-BH merger detections will indicate small (if any) natal kicks for massive BHs. C1 [Belczynski, Krzysztof; Bulik, Tomasz; Dominik, Michal] Warsaw Univ, Astron Observ, Al Ujazdowskie 4, PL-00478 Warsaw, Poland. [Repetto, Serena] Radboud Univ Nijmegen, Dept Astrophys, IMAPP, POB 9010, NL-6500 GL Nijmegen, Netherlands. [Holz, Daniel E.] Univ Chicago, Enrico Fermi Inst, Dept Phys, Chicago, IL 60637 USA. [Holz, Daniel E.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [O'Shaughnessy, Richard] Rochester Inst Technol, Ctr Computat Relat & Gravitat, Rochester, NY 14623 USA. [Berti, Emanuele] Univ Mississippi, Dept Phys & Astron, University, MS 38677 USA. [Berti, Emanuele] Univ Lisbon, CENTRA, Dept Fis, Inst Super Tecn, Ave Rovisco Pais 1, P-1049 Lisbon, Portugal. [Fryer, Christopher] Los Alamos Natl Lab, CCS 2,MSD409, Los Alamos, NM 87545 USA. RP Belczynski, K (reprint author), Warsaw Univ, Astron Observ, Al Ujazdowskie 4, PL-00478 Warsaw, Poland. RI Berti, Emanuele/C-9331-2016; OI Berti, Emanuele/0000-0003-0751-5130; O'Shaughnessy, Richard/0000-0001-5832-8517 FU NCN [DEC-2012/07/E/ST9/01360, UMO-2014/14/M/ST9/00707, UMO-2014/15/Z/ST9/00038]; FNP professorial subsidy MASTER; National Science Foundation [PHYS-1066293]; Simons Foundation; NSF [PHY-1505629, PHY-1055103]; NSF CAREER grant [PHY-1151836]; Kavli Institute for Cosmological Physics at the University of Chicago through NSF [PHY-1125897]; FCT [IF/00797/2014/CP1214/CT0012]; National Nuclear Security Administration of the U.S. Department of Energy; Los Alamos National Laboratory [DEAC52-06NA25396] FX We would like to thank a number of colleagues who have helped us to improve our project over the past several years. We want to name not only those who have given us information and positive feedback, but also those who have provided critiques. The full list includes Ilya Mandel, Gijs Nelemans, Selma de Mink, Felix Mirabel, Tsvi Piran, Patric Brady, Alessandra Buonanno, David Reitze, Vicky Kalogera, Tassos Fragos, Megan Morscher, Carl Rodriguez, Scott Hughes, Tom Maccarone, Yizhong Fan, and Dany Vanbeveren. KB and MD acknowledge support from the NCN grant Sonata Bis 2 (DEC-2012/07/E/ST9/01360) and FNP professorial subsidy MASTER 2013. TB and KB acknowledge support from the NCN grant Harmonia 6 (UMO-2014/14/M/ST9/00707). This work was supported in part by National Science Foundation Grant No. PHYS-1066293 and the hospitality of the Aspen Center for Physics (KB, DH). This work was partially supported by a grant from the Simons Foundation (KB). ROS was supported by NSF grant PHY-1505629. DEH was supported by NSF CAREER grant PHY-1151836. He also acknowledges support from the Kavli Institute for Cosmological Physics at the University of Chicago through NSF grant PHY-1125897 as well as an endowment from the Kavli Foundation. EB is supported by NSF CAREER grant PHY-1055103 and by FCT Contract IF/00797/2014/CP1214/CT0012 under the IF2014 Programme. The work of CF was done under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy, and supported by its contract DEAC52-06NA25396 at Los Alamos National Laboratory. TB was supported by the NCN grant UMO-2014/15/Z/ST9/00038. NR 157 TC 30 Z9 30 U1 1 U2 5 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 10 PY 2016 VL 819 IS 2 AR 108 DI 10.3847/0004-637X/819/2/108 PG 27 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG8AV UT WOS:000372305700020 ER PT J AU Beresnyak, A Li, H AF Beresnyak, Andrey Li, Hui TI FIRST-ORDER PARTICLE ACCELERATION IN MAGNETICALLY DRIVEN FLOWS SO ASTROPHYSICAL JOURNAL LA English DT Article DE acceleration of particles; magnetohydrodynamics (MHD) ID GAMMA-RAY FLARES; RELATIVISTIC RECONNECTION; ELECTRON ACCELERATION; NONTHERMAL PARTICLES; CRAB-NEBULA; TURBULENCE AB We demonstrate that particles are regularly accelerated while experiencing curvature drift in flows driven by magnetic tension. Some examples of such flows include spontaneous turbulent reconnection and decaying magnetohydrodynamic turbulence, where a magnetic field relaxes to a lower-energy configuration and transfers part of its energy to kinetic motions of the fluid. We show that this energy transfer, which normally causes turbulent cascade and heating of the fluid, also results in a first-order acceleration of non-thermal particles. Since it is generic, this acceleration mechanism is likely to play a role in the production of non-thermal particle distribution in magnetically dominant environments such as the solar chromosphere, pulsar magnetospheres, jets from supermassive black holes, and gamma-ray bursts. C1 [Beresnyak, Andrey] Naval Res Lab, Washington, DC 20375 USA. [Li, Hui] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Beresnyak, A (reprint author), Naval Res Lab, Washington, DC 20375 USA. FU LANL/LDRD program; DoE/Office of Fusion Energy Sciences through CMSO; XSEDE [TG-AST110057] FX We are grateful to Fan Guo for sharing his results during a preliminary stage. The work is supported by the LANL/LDRD program and the DoE/Office of Fusion Energy Sciences through CMSO. Computing resources at LANL were provided through the Institutional Computing Program. We also acknowledge support from XSEDE computational grant TG-AST110057. NR 36 TC 3 Z9 3 U1 1 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 10 PY 2016 VL 819 IS 2 AR 90 DI 10.3847/0004-637X/819/2/90 PG 5 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG8AV UT WOS:000372305700002 ER PT J AU Furst, F Muller, C Madsen, KK Lanz, L Rivers, E Brightman, M Arevalo, P Balokovic, M Beuchert, T Boggs, SE Christensen, FE Craig, WW Dauser, T Farrah, D Graefe, C Hailey, CJ Harrison, FA Kadler, M King, A Krauss, F Madejski, G Matt, G Marinucci, A Markowitz, A Ogle, P Ojha, R Rothschild, R Stern, D Walton, DJ Wilms, J Zhang, W AF Fuerst, F. Mueller, C. Madsen, K. K. Lanz, L. Rivers, E. Brightman, M. Arevalo, P. Balokovic, M. Beuchert, T. Boggs, S. E. Christensen, F. E. Craig, W. W. Dauser, T. Farrah, D. Graefe, C. Hailey, C. J. Harrison, F. A. Kadler, M. King, A. Krauss, F. Madejski, G. Matt, G. Marinucci, A. Markowitz, A. Ogle, P. Ojha, R. Rothschild, R. Stern, D. Walton, D. J. Wilms, J. Zhang, W. TI NuSTAR AND XMM-NEWTON OBSERVATIONS OF THE HARD X- RAY SPECTRUM OF CENTAURUS A SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: active; galaxies: individual (Centaurus A); X-rays: galaxies ID ACTIVE GALACTIC NUCLEI; RADIO GALAXY CENTAURUS; PHOTON IMAGING CAMERA; CLUMPY-TORUS MODELS; COMPTON-THICK; 3C 273; BEPPOSAX OBSERVATIONS; INTERSTELLAR-MEDIUM; CORONAL PROPERTIES; SEYFERT-GALAXIES AB We present simultaneous XMM-Newton and Nuclear Spectroscopic Telescope Array (NuSTAR) observations spanning 3-78 keV of the nearest radio galaxy, Centaurus. A (Cen A). The accretion geometry around the central engine in Cen. A is still debated, and we investigate possible configurations using detailed X-ray spectral modeling. NuSTAR imaged the central region of Cen. A with subarcminute resolution at X-ray energies above 10 keV for the first time, but found no evidence for an extended source or other off-nuclear point sources. The XMM-Newton and NuSTAR spectra agree well and can be described with an absorbed power law with a photon index Gamma = 1.815 +/- 0.005 and a fluorescent Fe K alpha line in good agreement with literature values. The spectrum does not require a high-energy exponential rollover, with a constraint of E-fold > 1 MeV. A thermal Comptonization continuum describes the data well, with parameters that agree with values measured by INTEGRAL, in particular an electron temperature kT(e) between approximate to 100-300 keV and seed photon input temperatures between 5 and 50 eV. We do not find evidence for reflection or a broad iron line and put stringent upper limits of R < 0.01 on the reflection fraction and accretion disk illumination. We use archival Chandra data to estimate the contribution from diffuse emission, extra-nuclear point sources, and the outer X-ray jet to the observed NuSTAR and XMM-Newton X-ray spectra and find the contribution to be negligible. We discuss different scenarios for the physical origin of the observed hard X-ray spectrum and conclude that the inner disk is replaced by an advection-dominated accretion flow or that the X-rays are dominated by synchrotron self-Compton emission from the inner regions of the radio jet or a combination thereof. C1 [Fuerst, F.; Madsen, K. K.; Rivers, E.; Brightman, M.; Balokovic, M.; Harrison, F. A.; Walton, D. J.] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Mueller, C.] Radboud Univ Nijmegen, Dept Astrophys, IMAPP, NL-6500 GL Nijmegen, Netherlands. [Mueller, C.; Beuchert, T.; Graefe, C.; Kadler, M.; Krauss, F.] Univ Wurzburg, Lehrstuhl Astron, D-97074 Wurzburg, Germany. [Mueller, C.; Beuchert, T.; Dauser, T.; Graefe, C.; Krauss, F.; Wilms, J.] Dr Karl Remeis Sternwarte, D-96049 Bamberg, Germany. [Mueller, C.; Beuchert, T.; Dauser, T.; Graefe, C.; Krauss, F.; Wilms, J.] ECAP, D-96049 Bamberg, Germany. [Lanz, L.; Ogle, P.] CALTECH, Ctr Infrared Proc & Anal, Pasadena, CA 91125 USA. [Arevalo, P.] Univ Valparaiso, Fac Ciencias, Inst Fis & Astron, Valparaiso, Chile. [Boggs, S. E.; Craig, W. W.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Christensen, F. E.] Tech Univ Denmark, Natl Space Inst, DTU Space, DK-2800 Lyngby, Denmark. [Craig, W. W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Farrah, D.] Virginia Tech, Dept Phys, Blacksburg, VA 24061 USA. [Hailey, C. J.] Columbia Univ, Columbia Astrophys Lab, 538 W 120th St, New York, NY 10027 USA. [King, A.; Madejski, G.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Menlo Pk, CA 94025 USA. [Matt, G.; Marinucci, A.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Markowitz, A.; Rothschild, R.] Univ Calif San Diego, CASS, La Jolla, CA 92093 USA. [Ojha, R.; Zhang, W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Ojha, R.] Univ Maryland Baltimore Cty, Baltimore, MD 21250 USA. [Ojha, R.] Catholic Univ Amer, Washington, DC 20064 USA. [Stern, D.; Walton, D. J.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. RP Furst, F (reprint author), CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. RI Wilms, Joern/C-8116-2013; Boggs, Steven/E-4170-2015; OI Wilms, Joern/0000-0003-2065-5410; Boggs, Steven/0000-0001-9567-4224; Krauss, Felicia/0000-0001-6191-1244; Kadler, Matthias/0000-0001-5606-6154 FU NASA [NNG08FD60C]; National Aeronautics and Space Administration; ESA Member States; Bundesministerium fur Wirtschaft und Technologie (BMWi) through Deutsches Zentrum fur Luft- und Raumfahrt (DLR) [50OR1404]; Deutsche Forschungsgemeinschaft (DFG) [Wi 1860 10-1]; NASA through Fermi Guest Investigator grants [NNH09ZDA001N, NNH10ZDA001N, NNH12ZDA001N, NNH13ZDA001N-FERMI]; NASA Headquarters under the NASA Earth and Space Science Fellowship Program [NNX14AQ07H] FX We thank the anonymous referee for comments that helped to improve this work. This work was supported under NASA Contract No. NNG08FD60C and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software, and Calibration teams for support with the execution and analysis of these observations. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS), jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). Based on observations obtained with XMM-Newton, an ESA science mission with instruments and contributions directly funded by ESA Member States and NASA. This research has made use of a collection of ISIS scripts provided by the Dr. Karl Remeis Observatory, Bamberg, Germany at http://www.sternwarte.uni-erlangen.de/isis/. C.M. acknowledges the support of the Bundesministerium fur Wirtschaft und Technologie (BMWi) through Deutsches Zentrum fur Luft- und Raumfahrt (DLR) grant 50OR1404. We acknowledge support of the Deutsche Forschungsgemeinschaft (DFG) through grant Wi 1860 10-1. This research was funded in part by NASA through Fermi Guest Investigator grants NNH09ZDA001N, NNH10ZDA001N, NNH12ZDA001N, NNH13ZDA001N-FERMI. This research was supported by an appointment to the NASA Postdoctoral Program at the Goddard Space Flight Center, administered by Oak Ridge Associated Universities through a contract with NASA. M.B. acknowledges support from NASA Headquarters under the NASA Earth and Space Science Fellowship Program, grant NNX14AQ07H. We would like to thank John E. Davis for the slxfig module, which was used to produce all figures in this work. NR 83 TC 4 Z9 4 U1 0 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 10 PY 2016 VL 819 IS 2 AR 150 DI 10.3847/0004-637X/819/2/150 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG8AV UT WOS:000372305700062 ER PT J AU Katz, MP Zingale, M Calder, AC Swesty, FD Almgren, AS Zhang, WQ AF Katz, Max P. Zingale, Michael Calder, Alan C. Swesty, F. Douglas Almgren, Ann S. Zhang, Weiqun TI WHITE DWARF MERGERS ON ADAPTIVE MESHES. I. METHODOLOGY AND CODE VERIFICATION SO ASTROPHYSICAL JOURNAL LA English DT Article DE hydrodynamics; methods: numerical; supernovae: general; white dwarfs ID PARTICLE HYDRODYNAMICS SIMULATIONS; PIECEWISE PARABOLIC METHOD; DYNAMICAL MASS-TRANSFER; IA SUPERNOVAE; NEUTRON-STAR; SURFACE DETONATIONS; NUMERICAL-METHODS; VIOLENT MERGERS; SELF-GRAVITY; BINARIES AB The Type Ia supernova (SN Ia) progenitor problem is one of the most perplexing and exciting problems in astrophysics, requiring detailed numerical modeling to complement observations of these explosions. One possible progenitor that has merited recent theoretical attention is the white dwarf (WD) merger scenario, which has the potential to naturally explain many of the observed characteristics of SNe Ia. To date there have been relatively few self-consistent simulations of merging WD systems using mesh-based hydrodynamics. This is the first paper in a series describing simulations of these systems using a hydrodynamics code with adaptive mesh refinement. In this paper we describe our numerical methodology and discuss our implementation in the compressible hydrodynamics code CASTRO, which solves the Euler equations, and the Poisson equation for self-gravity, and couples the gravitational and rotation forces to the hydrodynamics. Standard techniques for coupling gravitation and rotation forces to the hydrodynamics do not adequately conserve the total energy of the system for our problem, but recent advances in the literature allow progress and we discuss our implementation here. We present a set of test problems demonstrating the extent to which our software sufficiently models a system where large amounts of mass are advected on the computational domain over long timescales. Future papers in this series will describe our treatment of the initial conditions of these systems and will examine the early phases of the merger to determine its viability for triggering a thermonuclear detonation. C1 [Katz, Max P.; Zingale, Michael; Calder, Alan C.; Swesty, F. Douglas] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Calder, Alan C.] SUNY Stony Brook, Inst Adv Computat Sci, Stony Brook, NY 11794 USA. [Almgren, Ann S.; Zhang, Weiqun] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Ctr Computat Sci & Engn, Berkeley, CA 94720 USA. RP Katz, MP (reprint author), SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. OI Zingale, Michael/0000-0001-8401-030X; Katz, Maximilian/0000-0003-0439-4556 FU NSF [PHY-1151197, AST-1211563]; Sherman Fairchild Foundation; LIGO Laboratory at Caltech; Caltech; Office of Science of the Department of Energy [DE-AC05-00OR22725]; National Science Foundation [OCI-0725070, ACI-1238993, ACI-1053575]; state of Illinois; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; Empire State Development grant [NYS #28451]; [AST006]; [AST106]; [AST100037] FX The authors thank John Bell, Volker Springel, and Dominic Marcello for helpful discussions on gravity and hydrodynamics issues. We also thank Noel Scudder and Platon Karpov for their help with this project, especially related to visualization of the results, and Adam Jacobs for his advice on and assistance with running on supercomputing resources. Special thanks are given to the organizers of the 2015 Caltech Gravitational Wave Astrophysics School, and their supporters: the NSF under CAREER award PHY-1151197, the Sherman Fairchild Foundation, the LIGO Laboratory at Caltech, and Caltech.; This research was supported by NSF award AST-1211563. An award of computer time was provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program. This research used resources of the Oak Ridge Leadership Computing Facility located in the Oak Ridge National Laboratory, which is supported by the Office of Science of the Department of Energy under Contract DE-AC05-00OR22725. Projects AST006 and AST106 supported use of the ORNL/Titan resource. This research is part of the Blue Waters sustained-petascale computing project, which is supported by the National Science Foundation (awards OCI-0725070 and ACI-1238993) and the state of Illinois. Blue Waters is a joint effort of the University of Illinois at Urbana-Champaign and its National Center for Supercomputing Applications. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Results in this paper were obtained using the high-performance LIred computing system at the Institute for Advanced Computational Science at Stony Brook University, which was obtained through the Empire State Development grant NYS #28451. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation grant number ACI-1053575. Project AST100037 supported use of the resources NICS/Kraken and NICS/Darter. NR 80 TC 1 Z9 1 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 10 PY 2016 VL 819 IS 2 AR 94 DI 10.3847/0004-637X/819/2/94 PG 28 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG8AV UT WOS:000372305700006 ER PT J AU Ogrean, GA van Weeren, RJ Jones, C Forman, W Dawson, WA Golovich, N Andrade-Santos, F Murray, SS Nulsen, P Roediger, E Zitrin, A Bulbul, E Kraft, R Goulding, A Umetsu, K Mroczkowski, T Bonafede, A Randall, S Sayers, J Churazov, E David, L Merten, J Donahue, M Mason, B Rosati, P Vikhlinin, A Ebeling, H AF Ogrean, G. A. van Weeren, R. J. Jones, C. Forman, W. Dawson, W. A. Golovich, N. Andrade-Santos, F. Murray, S. S. Nulsen, P. Roediger, E. Zitrin, A. Bulbul, E. Kraft, R. Goulding, A. Umetsu, K. Mroczkowski, T. Bonafede, A. Randall, S. Sayers, J. Churazov, E. David, L. Merten, J. Donahue, M. Mason, B. Rosati, P. Vikhlinin, A. Ebeling, H. TI FRONTIER FIELDS CLUSTERS: DEEP CHANDRA OBSERVATIONS OF THE COMPLEX MERGER MACS J1149.6+2223 SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: clusters: general; galaxies: clusters: individual (MACS J1149.6+2223); galaxies: clusters: intracluster medium ID MASSIVE GALAXY CLUSTERS; X-RAY SPECTROSCOPY; COLD FRONTS; PARAMETER-ESTIMATION; TRANSPORT PROCESSES; RADIO-EMISSION; ATOMIC DATA; ABELL 2146; IMAGES; SAMPLE AB The Hubble Space Telescope Frontier Fields cluster MACS. J1149.6+2223 is one of the most complex merging clusters, believed to consist of four dark matter halos. We present results from deep (365 ks) Chandra observations of the cluster, which reveal the most distant cold front (z = 0.544) discovered to date. In the cluster outskirts, we also detect hints of a surface brightness edge that could be the bow shock preceding the cold front. The substructure analysis of the cluster identified several components with large relative radial velocities, thus indicating that at least some collisions occur almost along the line of sight. The inclination of the mergers with respect to the plane of the sky poses significant observational challenges at X-ray wavelengths. MACS. J1149.6+2223 possibly hosts a steep-spectrum radio halo. If the steepness of the radio halo is confirmed, then the radio spectrum, combined with the relatively regular ICM morphology, could indicate that MACS. J1149.6+2223 is an old merging cluster. C1 [Ogrean, G. A.; van Weeren, R. J.; Jones, C.; Forman, W.; Andrade-Santos, F.; Murray, S. S.; Nulsen, P.; Bulbul, E.; Kraft, R.; Randall, S.; David, L.; Vikhlinin, A.] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. [Dawson, W. A.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. [Golovich, N.] Univ Calif Davis, One Shields Ave, Davis, CA 95616 USA. [Murray, S. S.] Johns Hopkins Univ, Dept Phys & Astron, 3400 N Charles St, Baltimore, MD 21218 USA. [Nulsen, P.] Univ Western Australia, ICRAR, 35 Stirling Hwy, Crawley, WA 6009, Australia. [Roediger, E.] Dublin Inst Adv Studies, Astron & Astrophys Sect, 31 Fitzwilliam Pl, Dublin 2, Ireland. [Roediger, E.] Univ Hull, Dept Math & Phys, EA Milne Ctr Astrophys, Kingston Upon Hull HU6 7RX, N Humberside, England. [Zitrin, A.; Sayers, J.] CALTECH, Cahill Ctr Astron & Astrophys, MC 249-17, Pasadena, CA 91125 USA. [Goulding, A.] Princeton Univ, Dept Astrophys Sci, Princeton, NJ 08544 USA. [Umetsu, K.] Acad Sinica, Inst Astron & Astrophys, POB 23-141, Taipei 10617, Taiwan. [Mroczkowski, T.] US Naval Res Lab, 4555 Overlook Ave SW, Washington, DC 20375 USA. [Bonafede, A.] Univ Hamburg, Hamburger Sternwarte, Gojenbergsweg 112, D-21029 Hamburg, Germany. [Churazov, E.] Max Planck Inst Astrophys, Karl Schwarzschild Str 1, D-85741 Garching, Germany. [Churazov, E.] Space Res Inst, Profsoyuznaya 84-32, Moscow 117997, Russia. [Merten, J.] Univ Oxford, Dept Phys, Keble Rd, Oxford OX1 3RH, England. [Donahue, M.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Mason, B.] Natl Radio Astron Observ, 520 Edgemont Rd, Charlottesville, VA 22903 USA. [Rosati, P.] Univ Ferrara, Dept Phys & Earth Sci, Via G Saragat 1, I-44122 Ferrara, Italy. [Ebeling, H.] Univ Hawaii, Inst Astron, 2680 Woodlawn Dr, Honolulu, HI 96822 USA. RP Ogrean, GA (reprint author), Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. EM gogrean@cfa.harvard.edu RI Churazov, Eugene/A-7783-2013; OI Mroczkowski, Tony/0000-0003-3816-5372; Umetsu, Keiichi/0000-0002-7196-4822; Nulsen, Paul/0000-0003-0297-4493; van Weeren, Reinout/0000-0002-0587-1660 FU NASA - Space Telescope Science Institute under NASA [HST-HF2-51345.001-A, NAS5-26555, HST-HF2-51334.001-A]; NASA - Chandra X-ray Center [NAS8-03060, PF2-130104]; Clay Fellowship - Harvard-Smithsonian Center for Astrophysics; National Research Council Research Associateship Award at the Naval Research Laboratory (NRL); Chandra grant [G03-14131X]; U.S. DOE by LLNL [DE-AC52-07NA27344] FX G.A.O. acknowledges support by NASA through a Hubble Fellowship grant HST-HF2-51345.001-A awarded by the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Incorporated, under NASA contract NAS5-26555. R.J.v.W. was supported by NASA through the Einstein Postdoctoral grant number PF2-130104 awarded by the Chandra X-ray Center, which is operated by the Smithsonian Astrophysical Observatory for NASA, under contract NAS8-03060. R.J.v.W. is supported by a Clay Fellowship awarded by the Harvard-Smithsonian Center for Astrophysics. A.Z. acknowledges support by NASA through a Hubble Fellowship grant HST-HF2-51334.001-A awarded by the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Incorporated, under NASA contract NAS5-26555. This research was performed while T.M. held a National Research Council Research Associateship Award at the Naval Research Laboratory (NRL). F.A.S. acknowledges support from Chandra grant G03-14131X. Part of this work was performed under the auspices of the U.S. DOE by LLNL under contract DE-AC52-07NA27344. NR 44 TC 2 Z9 2 U1 1 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 10 PY 2016 VL 819 IS 2 AR 113 DI 10.3847/0004-637X/819/2/113 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG8AV UT WOS:000372305700025 ER PT J AU Palaversa, L Gezari, S Sesar, B Stuart, JS Wozniak, P Holl, B Ivezic, Z AF Palaversa, Lovro Gezari, Suvi Sesar, Branimir Stuart, J. Scott Wozniak, Przemyslaw Holl, Berry Ivezic, Zeljko TI REVEALING THE NATURE OF EXTREME CORONAL-LINE EMITTER SDSS J095209.56+214313.3 SO ASTROPHYSICAL JOURNAL LA English DT Article DE black hole physics; circumstellar matter; galaxies: individual (SDSS J095209.56+214313.3); galaxies: nuclei; supernovae: general; ultraviolet: galaxies ID TIDAL DISRUPTION CANDIDATES; DIGITAL SKY SURVEY; IIN SUPERNOVA; GALAXY; FLARE; SUPERSTRONG; DISCOVERY; TELESCOPE; EVOLUTION; EMISSION AB Extreme coronal-line emitter (ECLE) SDSS J095209.56+214313.3, known by its strong, fading, high-ionization lines, has been a long-standing candidate for a tidal disruption event;. however, a supernova (SN). origin has not yet been ruled out. Here we add several new pieces of information to the puzzle of the nature of the transient that powered its variable coronal lines: (1) an optical light curve from the Lincoln Near Earth Asteroid Research (LINEAR) survey that serendipitously catches the optical flare, and (2) late-time observations of the host galaxy with the Swift Ultraviolet and Optical Telescope (UVOT) and X-ray telescope (XRT) and the ground-based Mercator telescope. The well-sampled, similar to 10 yr long, unfiltered LINEAR light curve constrains the onset of the flare to a precision of +/- 5 days and enables us to place a lower limit on the peak optical magnitude. Difference imaging allows us to estimate the location of the flare in proximity of the host galaxy core. Comparison of the GALEX data (early 2006) with the recently acquired Swift UVOT (2015 June) and Mercator observations (2015 April) demonstrates. a decrease in the UV flux over a similar to 10 yr period, confirming that the flare was UV-bright. The long-lived UV-bright emission, detected 1.8 rest-frame years after the start of the flare, strongly disfavors an SN origin. These new data allow us to conclude that the flare was indeed powered by the tidal disruption of a star by a supermassive black hole and that tidal disruption events are in fact capable of powering the enigmatic class of ECLEs. C1 [Palaversa, Lovro; Holl, Berry] Univ Geneva, Astron Observ, 51 Chemin Maillettes, CH-1290 Sauverny, Switzerland. [Gezari, Suvi] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Sesar, Branimir] Max Planck Inst Astron, Konigstuhl 17, D-69117 Heidelberg, Germany. [Stuart, J. Scott] MIT, Lincoln Lab, 244 Wood St, Lexington, MA 02420 USA. [Wozniak, Przemyslaw] Los Alamos Natl Lab, 30 Bikini Atoll Rd, Los Alamos, NM 87545 USA. [Ivezic, Zeljko] Univ Washington, Dept Astron, POB 351580, Seattle, WA 98195 USA. RP Palaversa, L (reprint author), Univ Geneva, Astron Observ, 51 Chemin Maillettes, CH-1290 Sauverny, Switzerland. EM lovro.palaversa@unige.ch OI Wozniak, Przemyslaw/0000-0002-9919-3310 FU Gaia Research for European Astronomy Training (GREAT-ITN) Marie Curie network - European Union [264895]; NASA Swift grant [NNX15AR46G]; NSF CAREER grant [1454816]; National Aeronautics and Space Administration Near Earth Object Observations Program [FA8721-05-C-0002]; European Research Council under the European Community [227224]; Fund for Scientific Research of Flanders (FWO) [G.0410.09]; National Aeronautics and Space Administration [NNG05GF22G]; Alfred P. Sloan Foundation; National Science Foundation; U.S. Department of Energy; Japanese Monbukagakusho; Max Planck Society; Higher Education Funding Council for England; American Museum of Natural History; Astrophysical Institute Potsdam; University of Basel; University of Cambridge; Case Western Reserve University; University of Chicago; Drexel University; Fermilab; Institute for Advanced Study; Japan Participation Group; Johns Hopkins University; Joint Institute for Nuclear Astrophysics; Kavli Institute for Particle Astrophysics and Cosmology; Korean Scientist Group; Chinese Academy of Sciences (LAMOST); Los Alamos National Laboratory; Max-Planck-Institute for Astronomy (MPIA); Max-Planck-Institute for Astrophysics (MPA); New Mexico State University; Ohio State University; University of Pittsburgh; University of Portsmouth; Princeton University; United States Naval Observatory; University of Washington; U.S. National Science Foundation [AST-0909182] FX L.P. acknowledges support by the Gaia Research for European Astronomy Training (GREAT-ITN) Marie Curie network, funded through the European Union Seventh Framework Programme (FP7/2007-2013) under grant agreement no 264895 and valuable conversations with Laurent Eyer. S.G. was supported in part by NASA Swift grant NNX15AR46G and by NSF CAREER grant 1454816. The authors would also like to thank the anonymous referee for the useful comments.; The LINEAR program at MIT Lincoln Laboratory is funded by the National Aeronautics and Space Administration Near Earth Object Observations Program via an interagency agreement under Air Force Contract #FA8721-05-C-0002. Opinions, interpretations, conclusions, and recommendations are those of the authors and are not necessarily endorsed by the United States Government. Mercator Telescope is operated on the island of La Palma by the Flemish Community, at the Spanish Observatorio del Roque de los Muchachos of the Instituto de Astrofisica de Canarias. The MAIA camera was built by the Institute of Astronomy of KU Leuven, Belgium, thanks to funding from the European Research Council under the European Community's Seventh Framework Programme (FP7/2007-2013)/ERC grant agreement no. 227224 (PROSPERITY, PI: Conny Aerts) and from the Fund for Scientific Research of Flanders (FWO) grant agreement G.0410.09. The CCDs of MAIA were developed by e2v in the framework of the ESA Eddington space mission project; they were offered by ESA on permanent loan to KU Leuven. Photometric calibrations for the MAIA instrument were obtained using the Cambridge Photometric Calibration Server (CPCS), designed and maintained by Sergey Koposov and Lukasz Wyrzykowski. This publication makes use of data products from the Wide-field Infrared Survey Explorer, which is a joint project of the University of California, Los Angeles, and the Jet Propulsion Laboratory/California Institute of Technology, funded by the National Aeronautics and Space Administration. Funding for the SDSS and SDSS-II has been provided by the Alfred P. Sloan Foundation, the Participating Institutions, the National Science Foundation, the U.S. Department of Energy, the National Aeronautics and Space Administration, the Japanese Monbukagakusho, the Max Planck Society, and the Higher Education Funding Council for England. The SDSS Web site is http://www.sdss.org/. The SDSS is managed by the Astrophysical Research Consortium for the Participating Institutions. The Participating Institutions are the American Museum of Natural History, Astrophysical Institute Potsdam, University of Basel, University of Cambridge, Case Western Reserve University, University of Chicago, Drexel University, Fermilab, the Institute for Advanced Study, the Japan Participation Group, Johns Hopkins University, the Joint Institute for Nuclear Astrophysics, the Kavli Institute for Particle Astrophysics and Cosmology, the Korean Scientist Group, the Chinese Academy of Sciences (LAMOST), Los Alamos National Laboratory, the Max-Planck-Institute for Astronomy (MPIA), the Max-Planck-Institute for Astrophysics (MPA), New Mexico State University, Ohio State University, University of Pittsburgh, University of Portsmouth, Princeton University, the United States Naval Observatory, and the University of Washington. The CSS survey is funded by the National Aeronautics and Space Administration under Grant No. NNG05GF22G issued through the Science Mission Directorate Near-Earth Objects Observations Program. The CRTS survey is supported by the U.S. National Science Foundation under grants AST-0909182. NR 41 TC 3 Z9 3 U1 1 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 10 PY 2016 VL 819 IS 2 AR 151 DI 10.3847/0004-637X/819/2/151 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG8AV UT WOS:000372305700063 ER PT J AU Roebber, E Holder, G Holz, DE Warren, M AF Roebber, Elinore Holder, Gilbert Holz, Daniel E. Warren, Michael TI COSMIC VARIANCE IN THE NANOHERTZ GRAVITATIONAL WAVE BACKGROUND SO ASTROPHYSICAL JOURNAL LA English DT Article DE black hole physics; gravitational waves; large-scale structure of universe ID BLACK-HOLE BINARIES; PULSAR TIMING ARRAYS; DARK-MATTER HALOS; BRIGHTEST CLUSTER GALAXIES; DYNAMICAL FRICTION; EVOLUTION; RADIATION; LIMITS; MASSES; SYSTEMS AB We use large N-body simulations and empirical scaling relations between dark matter halos, galaxies, and supermassive black holes (SMBBHs) to estimate the formation rates of SMBBH binaries and the resulting lowfrequency stochastic gravitational wave background (GWB). We find this GWB to be relatively insensitive (less than or similar to 10%) to cosmological parameters, with only slight variation between WMAP5 and Planck cosmologies. We find that uncertainty in the astrophysical scaling relations changes the amplitude of the GWB by a factor of similar to 2. Current observational limits are already constraining this predicted range of models. We investigate the Poisson variance in the amplitude of the GWB for randomly generated populations of SMBBHs, finding a scatter of order unity per frequency bin below 10. nHz, and increasing to a factor of similar to 10 near 100. nHz. This variance is a result of the rarity of the most massive binaries, which dominate the signal, and acts as a fundamental uncertainty on the amplitude of the underlying power law spectrum. This Poisson uncertainty dominates at greater than or similar to 20 nHz, while at lower frequencies the dominant uncertainty is related to our poor understanding of the astrophysical scaling relations, although very low frequencies may be dominated by uncertainties related to the final parsec problem and the processes which drive binaries to the gravitational wave dominated regime. Cosmological effects are negligible at all frequencies. C1 [Roebber, Elinore; Holder, Gilbert] McGill Univ, Dept Phys, 3600 Univ St, Montreal, PQ H3A 2T8, Canada. [Holz, Daniel E.] Univ Chicago, Enrico Fermi Inst, Dept Phys, Chicago, IL 60637 USA. [Holz, Daniel E.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Warren, Michael] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Roebber, E (reprint author), McGill Univ, Dept Phys, 3600 Univ St, Montreal, PQ H3A 2T8, Canada. EM roebbere@physics.mcgill.ca FU Canada Foundation for Innovation (CFI); NanoQuebec; RMGA; Fonds de recherche du Quebec-Nature et technologies (FRQ-NT); NSERC Discovery program; Canadian Institute for Advanced Research; Canada Research Chairs program; NSF CAREER grant [PHY-1151836]; Kavli Institute for Cosmological Physics at the University of Chicago through NSF [PHY-1125897]; Kavli Foundation FX We thank Alberto Sesana for insightful comments and Peter Behroozi for the use of a portion of the MCMC chain used to fit parameters in the stellar mass halo mass relation. Computations were made on the Guillimin supercomputer from McGill University, managed by Calcul Quebec and Compute Canada. The operation of this supercomputer is funded by the Canada Foundation for Innovation (CFI), NanoQuebec, RMGA, and the Fonds de recherche du Quebec-Nature et technologies (FRQ-NT). GPH acknowledges support from the NSERC Discovery program, the Canadian Institute for Advanced Research, and the Canada Research Chairs program. DEH was supported by NSF CAREER grant PHY-1151836. He also acknowledges support from the Kavli Institute for Cosmological Physics at the University of Chicago through NSF grant PHY-1125897 as well as an endowment from the Kavli Foundation. NR 69 TC 3 Z9 3 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD MAR 10 PY 2016 VL 819 IS 2 AR 163 DI 10.3847/0004-637X/819/2/163 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DG8AV UT WOS:000372305700075 ER PT J AU Liu, Y Zhu, L Zhan, LW Gracia, JR King, TJ Liu, YL AF Liu, Yong Zhu, Lin Zhan, Lingwei Gracia, Jose R. King, Thomas Jr. Liu, Yilu TI Active power control of solar PV generation for large interconnection frequency regulation and oscillation damping SO INTERNATIONAL JOURNAL OF ENERGY RESEARCH LA English DT Article DE eastern interconnection (EI); frequency regulation; oscillation damping; renewable generation integration; solar photovoltaic (PV) ID PHOTOVOLTAIC GENERATION; INCREASED PENETRATION; STABILITY; SYSTEMS; IMPACT AB Because of zero greenhouse gas emission and decreased manufacture cost, solar photovoltaic (PV) generation is expected to account for a significant portion of future power grid generation portfolio. Because it is indirectly connected to the power grid via power electronic devices, solar PV generation system is fully decoupled from the power grid, which will influence the interconnected power grid dynamic characteristics as a result. In this paper, the impact of solar PV penetration on large interconnected power system frequency response and inter-area oscillation is evaluated, taking the United States Eastern Interconnection (EI) as an example. Furthermore, based on the constructed solar PV electrical control model with additional active power control loops, the potential contributions of solar PV generation to power system frequency regulation and oscillation damping are examined. The advantages of solar PV frequency support over that of wind generator are also discussed. Simulation results demonstrate that solar PV generations can effectively work as 'actuators' in alleviating the negative impacts they bring about. Copyright (C) 2015 John Wiley & Sons, Ltd. C1 [Liu, Yong; Zhu, Lin; Zhan, Lingwei; Liu, Yilu] Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37909 USA. [Gracia, Jose R.; King, Thomas Jr.; Liu, Yilu] Oak Ridge Natl Lab, Elect & Elect Syst Res Div, Oak Ridge, TN 37831 USA. RP Liu, YL (reprint author), Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37909 USA. EM yliu66@utk.edu OI Zhan, Lingwei/0000-0003-0021-6234 NR 25 TC 0 Z9 0 U1 3 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0363-907X EI 1099-114X J9 INT J ENERG RES JI Int. J. Energy Res. PD MAR 10 PY 2016 VL 40 IS 3 SI SI BP 353 EP 361 DI 10.1002/er.3362 PG 9 WC Energy & Fuels; Nuclear Science & Technology SC Energy & Fuels; Nuclear Science & Technology GA DG2HL UT WOS:000371887800007 ER PT J AU Damalanka, VC Kim, Y Alliston, KR Weerawarna, PM Kankanamalage, ACG Lushington, GH Mehzabeen, N Battaile, KP Lovell, S Chang, KO Groutas, WC AF Damalanka, Vishnu C. Kim, Yunjeong Alliston, Kevin R. Weerawarna, Pathum M. Kankanamalage, Anushka C. Galasiti Lushington, Gerald H. Mehzabeen, Nurjahan Battaile, Kevin P. Lovell, Scott Chang, Kyeong-Ok Groutas, William C. TI Oxadiazole-Based Cell Permeable Macrocyclic Transition State Inhibitors of Norovirus 3CL Protease SO JOURNAL OF MEDICINAL CHEMISTRY LA English DT Article ID RECOGNIZE BETA-STRANDS; NORWALK-VIRUS; SUBSTRATE-SPECIFICITY; DATA QUALITY; MACROMOLECULAR CRYSTALLOGRAPHY; MEMBRANE-PERMEABILITY; POTENT INHIBITION; 3C-LIKE PROTEASES; DRUG DISCOVERY; ACTIVE-SITES AB Human noroviruses are the primary causative agents of acute gastroenteritis and a pressing public health burden worldwide. There are currently no vaccines or small molecule therapeutics available for the treatment or prophylaxis of norovirus infections. Norovirus 3CL protease plays a vital role in viral replication by generating structural and nonstructural proteins via the cleavage of the viral polyprotein. Thus, molecules that inhibit the viral protease may have potential therapeutic value. We describe herein the structure-based design, synthesis, and in vitro and cell-based evaluation of the first class of oxadiazole-based, permeable macrocyclic inhibitors of norovirus 3CL protease. C1 [Damalanka, Vishnu C.; Alliston, Kevin R.; Weerawarna, Pathum M.; Kankanamalage, Anushka C. Galasiti; Groutas, William C.] Wichita State Univ, Dept Chem, Wichita, KS 67260 USA. [Kim, Yunjeong; Chang, Kyeong-Ok] Kansas State Univ, Dept Diagnost Med & Pathobiol, Coll Vet Med, Manhattan, KS 66506 USA. [Mehzabeen, Nurjahan; Lovell, Scott] Univ Kansas, Prot Struct Lab, Lawrence, KS 66047 USA. [Lushington, Gerald H.] LiS Consulting, Lawrence, KS 66046 USA. [Battaile, Kevin P.] APS Argonne Natl Lab, Hauptman Woodward Med Res Inst, IMCA CAT, Argonne, IL 60439 USA. RP Groutas, WC (reprint author), Wichita State Univ, Dept Chem, Wichita, KS 67260 USA.; Chang, KO (reprint author), Kansas State Univ, Dept Diagnost Med & Pathobiol, Coll Vet Med, Manhattan, KS 66506 USA. EM kchang@vet.ksu.edu; bill.groutas@wichita.edu RI Damalanka, Vishnu/S-3147-2016; OI Damalanka, Vishnu/0000-0002-1946-1320; Battaile, Kevin/0000-0003-0833-3259 FU National Institutes of Health [R01 AI109039]; National Center for Research Resources [5P20RR017708-10]; National Institute of General Medical Sciences [8P20GM103420-10]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The generous financial support of this work by the National Institutes of Health (Grant R01 AI109039) is gratefully acknowledged. Use of the University of Kansas Protein Structure Laboratory was supported by grants from the National Center for Research Resources (Grant 5P20RR017708-10) and the National Institute of General Medical Sciences (Grant 8P20GM103420-10). Use of the IMCA-CAT beamline 17-ID at the Advanced Photon Source was supported by the companies of the Industrial Macro molecular Crystallography Association through a contract with Hauptman-Woodward Medical Research Institute. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract DE-AC02-06CH11357. NR 56 TC 3 Z9 3 U1 1 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0022-2623 EI 1520-4804 J9 J MED CHEM JI J. Med. Chem. PD MAR 10 PY 2016 VL 59 IS 5 BP 1899 EP 1913 DI 10.1021/acs.jmedchem.5b01464 PG 15 WC Chemistry, Medicinal SC Pharmacology & Pharmacy GA DG4LJ UT WOS:000372043400018 PM 26823007 ER PT J AU Donahue, NM Dubey, MK Wennberg, PO Brune, WH AF Donahue, Neil M. Dubey, Manvendra K. Wennberg, Paul O. Brune, William H. TI James G. Anderson Tribute SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Biographical-Item C1 [Donahue, Neil M.] Carnegie Mellon Univ, Ctr Atmospher Particle Studies, Pittsburgh, PA 15213 USA. [Dubey, Manvendra K.] Los Alamos Natl Lab, Div Earth & Environm Sci, Los Alamos, NM USA. [Wennberg, Paul O.] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. [Wennberg, Paul O.] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. [Brune, William H.] Penn State Univ, Dept Meteorol, University Pk, PA 16802 USA. RP Donahue, NM (reprint author), Carnegie Mellon Univ, Ctr Atmospher Particle Studies, Pittsburgh, PA 15213 USA. EM nmd@cmu.edu RI Donahue, Neil/A-2329-2008; Dubey, Manvendra/E-3949-2010 OI Donahue, Neil/0000-0003-3054-2364; Dubey, Manvendra/0000-0002-3492-790X NR 1 TC 0 Z9 0 U1 0 U2 4 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAR 10 PY 2016 VL 120 IS 9 BP 1317 EP 1319 DI 10.1021/acs.jpca.5b11957 PG 3 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG4KX UT WOS:000372042200001 PM 26960593 ER PT J AU Louie, MK Francisco, JS Verdicchio, M Klippenstein, SJ Sinha, A AF Louie, Matthew K. Francisco, Joseph S. Verdicchio, Marco Klippenstein, Stephen J. Sinha, Amitabha TI Dimethylamine Addition to Formaldehyde Catalyzed by a Single Water Molecule: A Facile Route for Atmospheric Carbinolamine Formation and Potential Promoter of Aerosol Growth SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID INTERSTELLAR ICE ANALOGS; FORMIC-ACID CATALYSIS; GAS-PHASE REACTION; SULFURIC-ACID; AB-INITIO; ASTROPHYSICAL ICES; PARTICLE FORMATION; H2CO/NH3/H2O ICES; ALIPHATIC-AMINES; LOW-TEMPERATURE AB We use ab initio calculations to investigate the energetics and kinetics associated with carbinolamine formation resulting from the addition of dimethylamine formaldehyde catalyzed by a single water molecule. Further, we compare the energetics for this reaction with that for the analogous reactions involving methylamine and ammonia separately. We find that the reaction barrier for the addition of these nitrogen-containing molecules onto formaldehyde decreases along the series ammonia, methylamine, and dimethylamine. Hence, starting with ammonia, the reaction barrier can be "tuned" by the substitution of an alkyl group in place of a hydrogen atom. The reaction involving dimethylamine has the lowest barrier with the transition state being 5.4 kcal/mol below the (CH3)(2)NH + H2CO + H2O separated reactants. This activation energy is significantly lower than that for the bare reaction occurring without water, H2CO + (CH3)(2)NH, which has a barrier of 20.1 kcal/mol. The negative barrier associated with the single-water molecule catalyzed reaction of dimethylamine with H2CO to form the carbinolamine (CH3)(2)NCH2OH suggests that this reaction should be energetically feasible under atmospheric conditions. This is confirmed by rate calculations which suggest that the reaction will be facile even in the gas phase. As amines and oxidized organics containing carbonyl functional groups are common components of secondary organic aerosols, the present finding has important implications for understanding how larger, less volatile organic compounds can be generated in the atmosphere by combining readily available smaller components as required for promoting aerosol growth. C1 [Louie, Matthew K.; Sinha, Amitabha] Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA. [Francisco, Joseph S.] Purdue Univ, Dept Chem, W Lafayette, IN 47907 USA. [Verdicchio, Marco; Klippenstein, Stephen J.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Sinha, A (reprint author), Univ Calif San Diego, Dept Chem & Biochem, La Jolla, CA 92093 USA.; Klippenstein, SJ (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. EM sjk@anl.gov; asinha@ucsd.edu FU U.C. San Diego Academic Senate; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC02-06CH11357] FX A.S. thanks the U.C. San Diego Academic Senate for partial support of this research. The contribution from Argonne National Laboratory is based on work supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences under Contract DE-AC02-06CH11357. We thank Brian Finney for help with the NBO calculations and also acknowledge Yuri Georgievskii for helpful discussions. NR 78 TC 5 Z9 5 U1 13 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAR 10 PY 2016 VL 120 IS 9 BP 1358 EP 1368 DI 10.1021/acs.jpca.5b04887 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG4KX UT WOS:000372042200004 PM 26406105 ER PT J AU Nault, BA Garland, C Wooldridge, PJ Brune, WH Campuzano-Jost, P Crounse, JD Day, DA Dibb, J Hall, SR Huey, LG Jimenez, JL Liu, XX Mao, JQ Mikoviny, T Peischl, J Pollack, IB Ren, XR Ryerson, TB Scheuer, E Ullmann, K Wennberg, PO Wisthaler, A Zhang, L Cohen, RC AF Nault, Benjamin. A. Garland, Charity Wooldridge, Paul J. Brune, William H. Campuzano-Jost, Pedro Crounse, John D. Day, Douglas A. Dibb, Jack Hall, Samuel R. Huey, L. Gregory Jimenez, Jose L. Liu, Xiaoxi Mao, Jingqiu Mikoviny, Tomas Peischl, Jeff Pollack, Ilana B. Ren, Xinrong Ryerson, Thomas B. Scheuer, Eric Ullmann, Kirk Wennberg, Paul O. Wisthaler, Armin Zhang, Li Cohen, Ronald C. TI Observational Constraints on the Oxidation of NOx in the Upper Troposphere SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID INDUCED FLUORESCENCE INSTRUMENT; IONIZATION MASS-SPECTROMETRY; GAS-PHASE REACTIONS; IN-SITU DETECTION; ORGANIC-COMPOUNDS; DIODE-LASER; AIRCRAFT OBSERVATIONS; HNO3-FORMING CHANNEL; TROPICAL TROPOSPHERE; NITRATE FORMATION AB NOx (NxO NO + NO2) regulates O-3 and HOx (HOx OH + HO2) concentrations in the upper troposphere. In the laboratory, it is difficult to measure rates and branching ratios of the chemical reactions affecting NOx at the low temperatures and pressures characteristic of the upper troposphere, making direct measurements in the atmosphere especially useful. We report quasi-Lagrangian observations of the chemical evolution of an air parcel following a lightning event that results in high NOx concentrations. These quasi-Lagrangian measurements obtained during the Deep Convective Clouds and Chemistry experiment are used to characterize the daytime rates for conversion of NOx to different peroxy nitrates, the sum of alkyl and multifunctional nitrates, and HNO3. We infer the following production rate constants [in (cm(3)/molecule)/s] at 225 K and 230 hPa: 7.2(+/- 5.7) X 10(-12) (CH3O2NO2), 5.1(+/- 3.1) X 10(-13) (HO2NO2), 1.3(+/- 0.8) X 10(-11) (PAN), 7.3(+/- 3.4) X 10(-12) (PPN), and 6.2(+/- 2.9) X 10(-12) (HNO3). The HNO3 and HO2NO2 rates are similar to 30-50% lower than currently recommended whereas the other rates are consistent with current recommendations to within +/- 30%. The analysis indicates that HNO3 production from the HO2 and NO reaction (if any) must be accompanied by a slower rate for the reaction of OH with NO2, keeping the total combined rate for the two processes at the rate reported for HNO3 production above. C1 [Nault, Benjamin. A.; Cohen, Ronald C.] Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94709 USA. [Garland, Charity; Wooldridge, Paul J.; Cohen, Ronald C.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94709 USA. [Brune, William H.; Zhang, Li] Penn State Univ, Dept Meteorol, University Pk, PA 16802 USA. [Campuzano-Jost, Pedro; Day, Douglas A.; Jimenez, Jose L.] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Campuzano-Jost, Pedro; Jimenez, Jose L.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80309 USA. [Crounse, John D.; Wennberg, Paul O.] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. [Wennberg, Paul O.] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA. [Dibb, Jack; Scheuer, Eric] Univ New Hampshire, Inst Study Earth Oceans & Space, Earth Syst Res Ctr, Durham, NH 03824 USA. [Hall, Samuel R.; Ullmann, Kirk] Natl Ctr Atmospher Res, Div Atmospher Chem, Boulder, CO 80307 USA. [Huey, L. Gregory; Liu, Xiaoxi] Georgia Inst Technol, Sch Earth & Atmospher Sci, Atlanta, GA 30332 USA. [Mao, Jingqiu] NOAA, Geophys Fluid Dynam Lab, Princeton, NJ 08540 USA. [Mikoviny, Tomas] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. [Peischl, Jeff; Pollack, Ilana B.; Ryerson, Thomas B.] NOAA, Earth Syst Res Lab, Div Chem Sci, Boulder, CO 80305 USA. [Ren, Xinrong] NOAA, Air Resources Lab, College Pk, MD 20740 USA. [Wisthaler, Armin] Univ Innsbruck, Inst Ion Phys & Appl Phys, A-6020 Innsbruck, Austria. [Pollack, Ilana B.] Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA. RP Cohen, RC (reprint author), Univ Calif Berkeley, Dept Earth & Planetary Sci, Berkeley, CA 94709 USA.; Cohen, RC (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94709 USA. EM rccohen@berkeley.edu RI Mao, Jingqiu/F-2511-2010; Crounse, John/C-3700-2014; Peischl, Jeff/E-7454-2010; Pollack, Ilana/F-9875-2012; Cohen, Ronald/A-8842-2011; Ren, Xinrong/E-7838-2015; Jimenez, Jose/A-5294-2008; Manager, CSD Publications/B-2789-2015 OI Mao, Jingqiu/0000-0002-4774-9751; Crounse, John/0000-0001-5443-729X; Peischl, Jeff/0000-0002-9320-7101; Cohen, Ronald/0000-0001-6617-7691; Ren, Xinrong/0000-0001-9974-1666; Jimenez, Jose/0000-0001-6203-1847; FU National Science Foundation Graduate Research Fellowship [DGE 1106400]; NASA [NNX12AB79G, NNX12AC06G, NNX14AP46G, NNX12AC03G, NNX15A-H33A, NNX12AB80G] FX BAN was supported by the National Science Foundation Graduate Research Fellowship under grant no. DGE 1106400. BAN, CG, PWJ, and RCC acknowledge funding support from NASA (NNX12AB79G). PTR-MS measurements aboard the NASA DC-8 were supported by the Austrian Federal Ministry for Transport, Innovation and Technology (bmvit) through the Austrian Space Applications Programme (ASAP) of the Austrian Research Promotion Agency (FFG). TM was supported by an appointment to the NASA Postdoctoral Program at the Langley Research Center, administered by Oak Ridge Associated Universities through a contract with NASA. JDC and POW acknowledge funding support from NASA (NNX12AC06G and NNX14AP46G). PCJ and JLJ acknowledge funding form NASA (NNX12AC03G and NNX15A-H33A). JD and ES acknowledge funding from NASA (NNX12AB80G). BAN would like to thank Joshua L. Laughner in his assistance in setting up and running the GEOS-Chem model. The authors also want to thank the ground and flight crews of the DC-8 and the DC3 science team. Finally, the authors want to thank Donald Blake for the use of the whole air sampler measurements, Glenn Diskin for the use of the CH4 observations, and the reviewers for their constructive and thoughtful comments. NR 63 TC 0 Z9 0 U1 9 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAR 10 PY 2016 VL 120 IS 9 BP 1468 EP 1478 DI 10.1021/acs.jpca.5b07824 PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG4KX UT WOS:000372042200015 PM 26575342 ER PT J AU Arata, C Rahn, T Dubey, MK AF Arata, Caleb Rahn, Thom Dubey, Manvendra K. TI Methane Isotope Instrument Validation and Source Identification at Four Corners, New Mexico, United States SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID ATMOSPHERIC METHANE; CARBON DIOXIDE; ICE CORES; ABUNDANCES; EMISSIONS; FOSSIL; BUDGET; AREAS; URBAN; AIR AB Measurements of delta(CH4)-C-13 and CH4 concentration were made at a field site in Four Corners, New Mexico (FC), where we observed large sustained CH4 enhancements (2-8 ppm peaks for hours) during nocturnal inversions. Potential sources of this large CH4 signal at FC include (1) fugitive emissions from coal mining and gas processing that are thermogenic and isotopically C-13 enriched relative to background atmosphere and (2) emissions from agriculture, ruminants, landfills, and coalbed biogenic methane that are C-13 depleted relative to background atmosphere. We analyze our measurements of methane concentration and delta C-13 during spring and summer of 2012 to identify fugitive methane sources. We find CH4 plumes that are both enriched and depleted in C-13 relative to CH4 in background air. Keeling plots show a continuum of delta C-13 source compositions between -40 parts per thousand and -60 parts per thousand that are consistent with thermogenic and biogenic sources. The Picarro Mobile Methane Investigator (PMMI), a mobile delta(CH4)-C-13 instrument platform, was deployed in the spring of 2013 and used to verify the isotopic enrichment of coal bed methane in the region. We combine our results with meteorological data to spatially separate these sources in the Four Corners regions. Using CO and CO2 data, along with meteorological data, we propose that the high methane concentration events ([CH4] > 3.5 ppm) are from both thermogenic and biogenic methane released from coal beds. C1 [Arata, Caleb; Rahn, Thom; Dubey, Manvendra K.] Los Alamos Natl Lab, Earth Syst Observat, POB 1663, Los Alamos, NM 87545 USA. [Arata, Caleb] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Dubey, MK (reprint author), Los Alamos Natl Lab, Earth Syst Observat, POB 1663, Los Alamos, NM 87545 USA. EM dubey@lanl.gov RI Dubey, Manvendra/E-3949-2010; OI Dubey, Manvendra/0000-0002-3492-790X; Rahn, Thomas/0000-0001-8634-1348 FU LANL's Laboratory Directed Research and Development (LDRD) project [20110081DR] FX This work was supported by LANL's Laboratory Directed Research and Development (LDRD) project 20110081DR (PI MKD). NR 28 TC 2 Z9 2 U1 0 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD MAR 10 PY 2016 VL 120 IS 9 BP 1488 EP 1494 DI 10.1021/acs.jpca.5b12737 PG 7 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DG4KX UT WOS:000372042200017 PM 26840278 ER PT J AU Daily, MD Baer, MD Mundy, CJ AF Daily, Michael D. Baer, Marcel D. Mundy, Christopher J. TI Divalent Ion Parameterization Strongly Affects Conformation and Interactions of an Anionic Biomimetic Polymer SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID INITIO MOLECULAR-DYNAMICS; DENSITY-FUNCTIONAL THEORY; RESIDUE-SPECIFIC RESOLUTION; AIR-WATER-INTERFACE; HYDRATION STRUCTURE; AQUEOUS-SOLUTIONS; IR SPECTROSCOPY; FORCE-FIELD; MECHANICAL CALCULATIONS; EFFICIENT GENERATION AB The description of peptides and the use of molecular dynamics simulations to refine structures and investigate the dynamics on an atomistic scale are well developed. Through a consensus in this community over multiple decades, parameters were developed for molecular interactions that only require the sequence of amino-acids and an initial guess for the three-dimensional structure. The recent discovery of peptoids will require a retooling of the currently available interaction potentials in order to have the same level of confidence in the predicted structures and pathways as there is presently in the peptide counterparts. Here we present modeling of peptoids using a combination of ab initio molecular dynamics (AIMD) and atomistic resolution classical force field (FF) to span the relevant time and length scales. To properly account for the dominant forces that stabilize ordered structures of peptoids, namely steric-, electrostatic, and hydrophobic interactions mediated through side chain-side chain interactions in the FF model, those have to be first mapped out using high fidelity atomistic representations. A key feature here is not only to use gas phase quantum chemistry tools, but also account for solvation effects in the condensed phase AIMD. One major challenge is to elucidate ion binding to charged or polar regions of the peptoid and its concomitant role in the creation of local order. Here, similar to proteins, a specific ion effect is observed suggesting that both the net charge and the precise chemical nature of the ion will need to be described. C1 [Daily, Michael D.; Baer, Marcel D.; Mundy, Christopher J.] Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. [Daily, Michael D.] Univ Texas Med Branch, Dept Biochem & Mol Biol, Galveston, TX 77555 USA. RP Baer, MD (reprint author), Pacific NW Natl Lab, Div Phys Sci, Richland, WA 99352 USA. EM marcel.baer@pnnl.gov FU MS3 (Materials Synthesis and Simulation Across Scales) Initiative at Pacific Northwest National Laboratory; Laboratory Directed Research and Development program at Pacific Northwest National Laboratory; U.S. Department of Energy; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Material Sciences Engineering; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences Biosciences FX M.D.D. was supported by MS3 (Materials Synthesis and Simulation Across Scales) Initiative at Pacific Northwest National Laboratory. Research was funded by the Laboratory Directed Research and Development program at Pacific Northwest National Laboratory. PNNL is a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy. M.D.B. acknowledges support from U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Material Sciences & Engineering. C.J.M. acknowledges support from U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences & Biosciences. NR 93 TC 2 Z9 2 U1 6 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 10 PY 2016 VL 120 IS 9 BP 2198 EP 2208 DI 10.1021/acs.jpcb.5b12277 PG 11 WC Chemistry, Physical SC Chemistry GA DG4KV UT WOS:000372042000014 PM 26882842 ER PT J AU Mayer, BP Kennedy, DJ Lau, EY Valdez, CA AF Mayer, Brian P. Kennedy, Daniel J. Lau, Edmond Y. Valdez, Carlos A. TI Solution-State Structure and Affinities of Cyclodextrin:Fentanyl Complexes by Nuclear Magnetic Resonance Spectroscopy and Molecular Dynamics Simulation SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID INCLUSION COMPLEXES; WATER SUPPRESSION; BETA-CYCLODEXTRIN; FORCE-FIELD; THERMODYNAMICS; ANALGESIA; MODEL; PAIN AB Cyclodextrins (CDs) ate investigated for their ability to form inclusion complexes with the analgesic fentanyl and three similar molecules: acetylfentanyl, thiofentanyl, and acetylthiofentanyl. Stoichiometry, binding strength, and complex structure are revealed through nuclear magnetic resonance (NMR) techniques and discussed in terms of molecular dynamics (MID) simulations. It was found that beta-cyclodextrin is generally capable of forming the strongest complexes with the fentanyl panel. Two-dimensional NMR data and computational chemical calculations are used to derive solution-state structures of the complexes. Binding of the fentanyls to the CDs occurs at the amide phenyl ring, leaving the majority of the molecule solvated by water, an observation common to all four fentanyls. This finding suggests a universal binding behavior, as the vast majority of previously synthesized fentanyl analogues contain this structural moiety. This baseline study serves as the most complete work on CD:fentanyl complexes to date and provides the insights into strategies for producing future generations of designer cyclodextrins capable of stronger and more selective complexation of fentanyl and its analogues. C1 [Mayer, Brian P.; Kennedy, Daniel J.; Valdez, Carlos A.] Lawrence Livermore Natl Lab, Forens Sci Ctr, Livermore, CA 94550 USA. [Lau, Edmond Y.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Biosci & Biotechnol Div, Livermore, CA 94550 USA. RP Valdez, CA (reprint author), Lawrence Livermore Natl Lab, Forens Sci Ctr, Livermore, CA 94550 USA. EM valdez11@llnl.gov FU LLNL's Laboratory Directed Research and Development Program [14-ERD-048]; U.S. Department of Energy, National Nuclear Security Administration [DE-AC52-07NA27344] FX This work was funded by LLNL's Laboratory Directed Research and Development Program (14-ERD-048). Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the U.S. Department of Energy, National Nuclear Security Administration, under Contract DE-AC52-07NA27344. NR 43 TC 0 Z9 0 U1 2 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 10 PY 2016 VL 120 IS 9 BP 2423 EP 2433 DI 10.1021/acs.jpcb.5b12333 PG 11 WC Chemistry, Physical SC Chemistry GA DG4KV UT WOS:000372042000039 PM 26842886 ER PT J AU Santra, K Zhan, JC Song, XY Smith, EA Vaswani, N Petrich, JW AF Santra, Kalyan Zhan, Jinchun Song, Xueyu Smith, Emily A. Vaswani, Namrata Petrich, Jacob W. TI What Is the Best Method to Fit Time-Resolved Data? A Comparison of the Residual Minimization and the Maximum Likelihood Techniques As Applied to Experimental Time-Correlated, Single-Photon Counting Data SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID SHOT NOISE LIMIT; FLUORESCENCE DECAY; LEAST-SQUARES; STATISTICAL-INFERENCE; WAVELENGTH DEPENDENCE; EXPONENTIAL DECAYS; TEST CRITERIA; CHI-SQUARE; MOLECULES; SPECTROSCOPY AB The need for measuring fluorescence lifetimes of species in subdiffraction-limited volumes in, for example, stimulated emission depletion (STED) microscopy, entails the dual challenge of probing a small number of fluorophores and fitting the concomitant sparse data set to the appropriate excited-state decay function. This need has stimulated a further investigation into the relative merits of two fitting techniques commonly referred to as "residual minimization" (RM) and "maximum likelihood" (ML). Fluorescence decays of the well-characterized standard, rose bengal in methanol at room temperature (530 +/- 10 ps), were acquired in a set of five experiments in which the total number of "photon counts" was approximately 20, 200, 1000, 3000, and 6000 and there were about 2-200 counts at the maxima of the respective decays. Each set of experiments was repeated 50 times to generate the appropriate statistics. Each of the 250 data sets was analyzed by ML and two different RM methods (differing in the weighting of residuals) using in-house routines and compared with a frequently used commercial RM routine. Convolution with a real instrument response function was always included in the fitting. While RM using Pearson's weighting of residuals can recover the correct mean result with a total number of counts of 1000 or more, ML distinguishes itself by yielding, in all cases, the same mean lifetime within 2% of the accepted value. For 200 total counts and greater, ML always provides a standard deviation of <10% of the mean lifetime, and even at 20 total counts there is only 20% error in the mean lifetime. The robustness of ML advocates its use for sparse data sets such as those acquired in some subdiffraction-limited microscopies, such as STED, and, more importantly, provides greater motivation for exploiting the time resolved capacities of this technique to acquire and analyze fluorescence lifetime data. C1 [Santra, Kalyan; Song, Xueyu; Smith, Emily A.; Petrich, Jacob W.] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. [Santra, Kalyan; Song, Xueyu; Smith, Emily A.; Petrich, Jacob W.] Iowa State Univ Sci & Technol, Ames Lab, US DOE, Ames, IA 50011 USA. [Zhan, Jinchun; Vaswani, Namrata] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. RP Petrich, JW (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA.; Petrich, JW (reprint author), Iowa State Univ Sci & Technol, Ames Lab, US DOE, Ames, IA 50011 USA. EM jwp@iastate.edu RI Petrich, Jacob/L-1005-2015; OI Smith, Emily/0000-0001-7438-7808 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory; U.S. Department of Energy [DE-AC02-07CH11358]; Division of Material Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy [W-7405-430 ENG-82]; Iowa State University; National Science Foundation [CCF-1117125] FX We thank Mr. Ujjal Bhattacharjee for assistance in the early stages of this work. The work performed by K.S., E.A.S., and J.W.P. was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory. The Ames Laboratory is operated for the U.S. Department of Energy by Iowa State University under Contract No. DE-AC02-07CH11358. X.S. was supported by The Division of Material Sciences and Engineering, Office of Basic Energy Sciences, U.S. Department of Energy, under Contact No. W-7405-430 ENG-82 with Iowa State University. The work of J.Z. and N.V. was partly supported by grant CCF-1117125 from the National Science Foundation. NR 42 TC 2 Z9 2 U1 5 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 10 PY 2016 VL 120 IS 9 BP 2484 EP 2490 DI 10.1021/acs.jpcb.6b00154 PG 7 WC Chemistry, Physical SC Chemistry GA DG4KV UT WOS:000372042000045 PM 26865463 ER PT J AU Olatinwo, MB Ham, K McCarney, J Marathe, S Ge, JH Knapp, G Butler, LG AF Olatinwo, Mutairu B. Ham, Kyungmin McCarney, Jonathan Marathe, Shashidhara Ge, Jinghua Knapp, Gerry Butler, Leslie G. TI Analysis of Flame Retardancy in Polymer Blends by Synchrotron X-ray K-edge Tomography and Interferometric Phase Contrast Movies SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID 3-DIMENSIONAL CHEMICAL-ANALYSIS; POLYPROPYLENE SYSTEM; ANTIMONY TRIOXIDE; METAL-OXIDE; NANOCOMPOSITES; POLYSTYRENE; COMPOSITES; FLAMMABILITY; RELEASE AB Underwriters Laboratories 94 test bars have been imaged with X-ray Kedge tomography between 12 and 32 keV to assess the bromine and antimony concentration gradient across char layers of partially burnt samples. Phase contrast tomography on partially burnt samples showed gas bubbles and dark-field scattering ascribed to residual blend inhomogeneity. In addition, single-shot grating interferometry was used to record X-ray movies of test samples during heating (IR and flame) intended to mimic the UL 94 plastics flammability test. The UL 94 test bars were formulated with varying concentrations of a brominated flame retardant, 3 Saytex 8010, and a synergist, Sb2O3, blended into high-impact polystyrene (HIPS). Depending on the sample composition, samples will pass or fail the UL 94 plastics flammability test. Tomography and interferometry imaging show differences that correlate with UL 94 performance. Key features such as char layer, gas bubble formation, microcracks, and dissolution of the flame retardant in the char layer regions are used in understanding the efficiency of the flame retardant and synergist. The samples that pass the UL 94 test have a thick, highly visible char layer as well as an interior rich in gas bubbles. Growth of gas bubbles from flame-retardant thermal decomposition is noted in the X-ray phase contrast movies. Also noteworthy is an absence of bubbles near the burning surface of the polymer; dark-field images after burning suggest a microcrack structure between interior bubbles and the surface. The accepted mechanism for flame retardant activity includes free radical quenching in the flame by bromine and antimony species. The imaging supports this as well as provides a fast inspection of other parameters, such as viscosity and surface tension. C1 [Olatinwo, Mutairu B.; Butler, Leslie G.] Louisiana State Univ, Dept Chem, 232 Choppin Hall, Baton Rouge, LA 70803 USA. [Ham, Kyungmin] Louisiana State Univ, Ctr Adv Microstruct & Devices, 6980 Jefferson Highway, Baton Rouge, LA 70806 USA. [McCarney, Jonathan] Albemarle Corp, Proc Dev Ctr, POB 341, Baton Rouge, LA 70821 USA. [Marathe, Shashidhara] Argonne Natl Lab, Adv Photon Source, Bldg 401,9700 South Cass Ave, Argonne, IL 60439 USA. [Ge, Jinghua] Louisiana State Univ, Ctr Computat & Technol, 340 East Parker Blvd, Baton Rouge, LA 70808 USA. [Knapp, Gerry] Louisiana State Univ, Dept Mech & Ind Engn, Baton Rouge, LA 70803 USA. [Marathe, Shashidhara] Diamond Light Source Ltd, Div Sci, Didcot, Oxon, England. RP Butler, LG (reprint author), Louisiana State Univ, Dept Chem, 232 Choppin Hall, Baton Rouge, LA 70803 USA. EM lbutler@lsu.edu FU U.S. DOE [DE-AC02-06CH11357]; National Science Foundation (NSF) [CHE-0910937]; National Science Foundation under the NSF EPSCoR [EPS-1003897]; Louisiana Board of Regents; A.G. Leventis Foundation FX Use of the Advanced Photon Source and Center for Nanoscale Materials, Office of Science User Facilities, operated for the U.S. Department of Energy (DOE), Office of Science, by Argonne National Laboratory, was supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. The support of National Science Foundation (NSF) CHE-0910937 is gratefully acknowledged. This material is based upon work supported by the National Science Foundation under the NSF EPSCoR Cooperative Agreement No. EPS-1003897 with additional support from the Louisiana Board of Regents. MBO thanks the A.G. Leventis Foundation for additional research support. NR 50 TC 2 Z9 2 U1 5 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD MAR 10 PY 2016 VL 120 IS 9 BP 2612 EP 2624 DI 10.1021/acs.jpcb.5b12775 PG 13 WC Chemistry, Physical SC Chemistry GA DG4KV UT WOS:000372042000059 PM 26846254 ER PT J AU Patankar, S Gautam, S Rother, G Podlesnyak, A Ehlers, G Liu, TL Cole, DR Tomasko, DL AF Patankar, Sumant Gautam, Siddharth Rother, Gernot Podlesnyak, Andrey Ehlers, Georg Liu, Tingling Cole, David R. Tomasko, David L. TI Role of Confinement on Adsorption and Dynamics of Ethane and an Ethane-CO2 Mixture in Mesoporous CPG Silica SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ELASTIC NEUTRON-SCATTERING; METAL-ORGANIC FRAMEWORKS; MONTE-CARLO-SIMULATION; CONTROLLED-PORE GLASS; CARBON-DIOXIDE; TRANSITION TEMPERATURE; SUPERCRITICAL CO2; SELF-DIFFUSION; CRITICAL-POINT; HIGH-PRESSURE AB Ethane is found confined to mineral and organic pores in certain shale formations. Effects of confinement on structural and dynamic properties of ethane in mesoporous controlled pore glass (CPG) were studied by gravimetric adsorption and quasi-elastic neutron scattering (QENS) measurements. The obtained isotherms and scattering data complement each other by quantifying the relative strength of the solid fluid interactions and the transport properties of the fluid under confinement, respectively. A magnetic suspension balance was used to measure the adsorption isotherms at two temperatures and over a range of pressures corresponding to a bulk density range of 0.01-0.35 g/cm(3). Key confinement effects were highlighted through differences between isotherms for the two pore sizes. A comparison was made with previously published isotherms for CO2 on the same CPG materials. Behavior of ethane in the smaller pore size was probed further using quasi-elastic neutron scattering. By extracting the self-diffusivity and residence time, we were able to study the effect of pressure and transition from gaseous to supercritical densities on the dynamics of confined ethane. A temperature variation QENS study was also completed with pure ethane and a CO2 ethane mixture. Activation energies extracted from the Arrhenius plots show the effects of CO2 addition on ethane mobility. C1 [Patankar, Sumant; Tomasko, David L.] Ohio State Univ, William G Lowrie Dept Chem & Biomol Engn, 151 West Woodruff Ave, Columbus, OH 43210 USA. [Gautam, Siddharth; Liu, Tingling; Cole, David R.] Ohio State Univ, Sch Earth Sci, 125 South Oval Mall, Columbus, OH 43210 USA. [Rother, Gernot] Oak Ridge Natl Lab, Div Chem Sci, Geochem & Interfacial Sci Grp, Oak Ridge, TN 37831 USA. [Podlesnyak, Andrey; Ehlers, Georg] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Tomasko, DL (reprint author), Ohio State Univ, William G Lowrie Dept Chem & Biomol Engn, 151 West Woodruff Ave, Columbus, OH 43210 USA. EM tomasko.1@osu.edu RI Podlesnyak, Andrey/A-5593-2013; Gautam, Siddharth/F-5835-2014; Rother, Gernot/B-7281-2008; Ehlers, Georg/B-5412-2008; OI Podlesnyak, Andrey/0000-0001-9366-6319; Gautam, Siddharth/0000-0003-1443-5382; Rother, Gernot/0000-0003-4921-6294; Ehlers, Georg/0000-0003-3513-508X; patankar, sumant/0000-0002-6937-4241 FU U.S. Department of Energy, Office of Basic Energy Sciences, Geoscience Program [DE-SC0006878]; A. P. Sloan Foundation Deep Carbon Observatory; Division of Chemical Sciences, Geosciences and Bio-sciences, Office of Basic Energy Sciences, U.S. Department of Energy; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX S.P., S.G., and T.L. are grateful for the support from the U.S. Department of Energy, Office of Basic Energy Sciences, Geoscience Program under Contract DE-SC0006878. D.R.C. acknowledges support from the A. P. Sloan Foundation Deep Carbon Observatory. The research of G.R. was sponsored by the Division of Chemical Sciences, Geosciences and Bio-sciences, Office of Basic Energy Sciences, U.S. Department of Energy. SEM images were acquired by Julie Sheets at the Subsurface Energy Materials Characterization and Analysis Laboratory (SEMCAL), School of Earth Sciences, The Ohio State University. Research at Oak Ridge National Laboratory's Spanation Neutron Source was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 55 TC 0 Z9 0 U1 5 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 10 PY 2016 VL 120 IS 9 BP 4843 EP 4853 DI 10.1021/acs.jpcc.5b09984 PG 11 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DG4LB UT WOS:000372042600015 ER PT J AU Hocker, J Duchon, T Veltruska, K Matolin, V Falta, J Senanayake, SD Flege, JI AF Hoecker, Jan Duchon, Tomas Veltruska, Katerina Matolin, Vladimir Falta, Jens Senanayake, Sanjaya D. Flege, J. Ingo TI Controlling Heteroepitaxy by Oxygen Chemical Potential: Exclusive Growth of (100) Oriented Ceria Nanostructures on Cu(111) SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID THIN-FILMS; SURFACE; OXIDE; MORPHOLOGY; ADSORPTION; STABILITY; NANORODS; METHANOL; DEFECTS; CEO2 AB A novel and simple method is presented for the preparation of a well-defined CeO2(100) model system on Cu(111) based on the adjustment of the Ce/O ratio during growth. The method yields micrometer-sized, several nanometers high, single-phase CeO2(100) islands with controllable size and surface termination that can be benchmarked against the known (111) nanostructured islands on Cu(111). Furthermore, we demonstrate the ability to adjust the Ce to O stoichiometry from CeO2(100) (100% Ce4+) to c-Ce2O3(100) (100% Ce3+), which can be readily recognized by characteristic surface reconstructions observed by low-energy electron diffraction. The discovery of the highly stable CeOx(100) phase on a hexagonally close packed metal surface represents an unexpected growth mechanism of ceria on Cu(111), and it provides novel opportunities to prepare more elaborate models, benchmark surface chemical reactivity, and thus gain valuable insights into the redox chemistry of ceria in catalytic processes. C1 [Hoecker, Jan; Falta, Jens; Flege, J. Ingo] Univ Bremen, Inst Solid State Phys, Otto Hahn Allee 1, D-28359 Bremen, Germany. [Duchon, Tomas; Veltruska, Katerina; Matolin, Vladimir] Charles Univ Prague, Fac Math & Phys, Dept Surface & Plasma Sci, V Holesovickach 2, CR-18000 Prague 8, Czech Republic. [Falta, Jens] Univ Bremen, MAPEX Ctr Mat & Proc, D-28359 Bremen, Germany. [Senanayake, Sanjaya D.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Flege, JI (reprint author), Univ Bremen, Inst Solid State Phys, Otto Hahn Allee 1, D-28359 Bremen, Germany.; Senanayake, SD (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM ssenanay@bnl.gov; flege@ifp.uni-bremen.de RI Flege, Jan Ingo/J-6354-2012; COST, CM1104/I-8057-2015; Senanayake, Sanjaya/D-4769-2009; OI Flege, Jan Ingo/0000-0002-8346-6863; Senanayake, Sanjaya/0000-0003-3991-4232; Falta, Jens/0000-0002-4154-822X; Duchon, Tomas/0000-0002-3035-012X FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, and Catalysis Science Program [DE-SC0012704]; European COST Action [CM1104]; Czech Science Foundation [GACR 15-06759S]; Ministry of Education of the Czech Republic [LD13054]; Grant Agency of Charles University in Prague [GAUK 794313] FX This work was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, and Catalysis Science Program under contract No. DE-SC0012704. This work was also supported by the European COST Action CM1104, the Czech Science Foundation (GACR 15-06759S), the Ministry of Education of the Czech Republic (LD13054), and the Grant Agency of Charles University in Prague (GAUK 794313). NR 30 TC 3 Z9 3 U1 10 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 10 PY 2016 VL 120 IS 9 BP 4895 EP 4901 DI 10.1021/acs.jpcc.5b11066 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DG4LB UT WOS:000372042600020 ER PT J AU Zhao, ZY Rossi, VAV Baltrus, JP Ohodnicki, PR Carpenter, MA AF Zhao, Zhouying Rossi, V. A. Vulcano Baltrus, John P. Ohodnicki, Paul R. Carpenter, Michael A. TI Ag Nanoparticles Supported on Yttria-Stabilized Zirconia: A Synergistic System within Redox Environments SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID SURFACE-PLASMON RESONANCE; TEMPERATURE-PROGRAMMED DESORPTION; ELECTROCHEMICAL MEMBRANE REACTOR; SILVER NANOPARTICLES; METAL NANOPARTICLES; PARTIAL OXIDATION; CO OXIDATION; GOLD NANOPARTICLES; OPTICAL-PROPERTIES; CATALYTIC-ACTIVITY AB In this work, we report a distinctive dynamic sintering-free redox behavior of Ag nanoparticles (AgNPs) on 30 nm thick yttria-stabilized zirconia (YSZ) films. The material system demonstrates reversible 200 nm shifts in the plasmonic spectra with an unprecedented particle phase/size/morphology oscillation during cyclic redox reactions in air and hydrogen/air at 300-400 degrees C. This is in significant contrast to the minor changes more commonly observed for AgNPs on quartz. It was found that the ionically active YSZ has a strong tendency to drive AgNPs to oxidize under oxidizing conditions, and upon surface oxidation a large differential surface energy is built up, forcing the core/shell particles to migrate and coalesce toward a lower system free energy. Most strikingly, once switched to a mixture of H-2 and air, the previously formed large dewetted metal-core/thick oxide-shell particles collapse, and new small Ag nanoparticles quickly form and remain in a highly dispersed and sintering-free state on YSZ. This is found to likely be due to catalytic production of water over the material system, which plays a key role in the dynamic redox activities. It is hypothesized that the small metallic particle regeneration and sinter-free behavior take place through a four step process resulting from the synergistic behavior of AgNPs supported on YSZ within a redox environment: (I) production of a local humid environment via catalytic reactions of H2 and 02 mostly at the triple-phase boundary, (II) dissolution of Ag+ from both reduced Ag and the AgOx shell, (III) collapse and spillover of the AgOx shell/water layer with Ag ions onto the hydrous YSZ surface, and (IV) reduction, diffusion, nucleation, and growth to new small metallic AgNPs with a dynamic equilibrium quickly reached. The findings behind this novel system could set up an avenue for a new concept of catalysts operating in a self-controlled dynamic regime for governing chemical reactions via metal and ceramic synergized catalysis with high activities and stabilities. C1 [Zhao, Zhouying; Rossi, V. A. Vulcano; Carpenter, Michael A.] SUNY Polytech Inst, Coll Nanoscale Sci, Albany, NY 12203 USA. [Zhao, Zhouying; Rossi, V. A. Vulcano; Carpenter, Michael A.] SUNY Polytech Inst, Coll Engn, Albany, NY 12203 USA. [Baltrus, John P.; Ohodnicki, Paul R.] US DOE, Natl Energy Technol Lab, Pittsburgh, PA 15236 USA. RP Carpenter, MA (reprint author), SUNY Polytech Inst, Coll Nanoscale Sci, Albany, NY 12203 USA.; Carpenter, MA (reprint author), SUNY Polytech Inst, Coll Engn, Albany, NY 12203 USA. EM mcarpenter@sunycnse.com FU United States Department of Energy National Energy Technology Laboratory [DE-FE0007190]; National Science Foundation [PN 1006399] FX This work was supported by the United States Department of Energy National Energy Technology Laboratory under contract number DE-FE0007190. Any opinions, findings, and conclusions or recommendations expressed in this publication are those of the authors and do not necessarily reflect the views of the United States Department of Energy National Energy Technology Laboratory. This work was also supported by the National Science Foundation research project PN 1006399 NR 82 TC 3 Z9 3 U1 9 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 10 PY 2016 VL 120 IS 9 BP 5020 EP 5032 DI 10.1021/acs.jpcc.6b00189 PG 13 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DG4LB UT WOS:000372042600033 ER PT J AU Mattox, TM Chockkalingam, S Roh, I Urban, JJ AF Mattox, Tracy M. Chockkalingam, Shruthi Roh, Inwhan Urban, Jeffrey J. TI Evolution of Vibrational Properties in Lanthanum Hexaboride Nanocrystals SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID RARE-EARTH HEXABORIDE; RAMAN-SCATTERING; PARTICLE-SIZE; SPECTROSCOPY; NANOPARTICLES; SPECTRA; LAB6; CRYSTALS; SILICON; MICROCRYSTALS AB Lanthanum hexaboride (LaB6) is known for its hardness, mechanical strength, thermionic emission, and strong plasmonic properties. However, given the lack of colloidal synthetic methods to access this material, very little is understood about its physical properties on the nanoscale. Recently, a new moderate-temperature synthetic technique was developed to directly synthesize LaB6 nanoparticles [Mattox et al. Chem. Mater. 2015, 27, 6620]. We report the influence of nanoparticle size on the structural and vibrational properties of LaB6 using a combination of Raman and Fourier transform infrared spectroscopies. Our studies indicate that the size of the lanthanum salt anion has a larger influence on LaB6 vibrational energies than particle size. Surprisingly, our work finds that the LaB6 lattice readily expands to accommodate larger ions and contracts with their removal, while ligand incorporation significantly amplifies and shifts the Raman stretching modes. C1 [Mattox, Tracy M.; Chockkalingam, Shruthi; Roh, Inwhan; Urban, Jeffrey J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Mol Foundry, One Cyclotron Rd, Berkeley, CA 94720 USA. RP Mattox, TM; Urban, JJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Mol Foundry, One Cyclotron Rd, Berkeley, CA 94720 USA. EM tmmattox@lbl.gov; jjurban@lbl.gov FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231] FX This work was completed at The Molecular Foundry, Lawrence Berkeley National Laboratory, a user facility supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231. We would like to give a special thanks to Shaul Aloni for discussions on ion analysis and to Wendy Queen for her discussions on X-ray diffraction. NR 55 TC 0 Z9 0 U1 3 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 10 PY 2016 VL 120 IS 9 BP 5188 EP 5195 DI 10.1021/acs.jpcc.5b12680 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DG4LB UT WOS:000372042600050 ER PT J AU Leach, ADP Shen, X Faust, A Cleveland, MC La Croix, AD Banin, U Pantelides, ST Macdonald, JE AF Leach, Alice D. P. Shen, Xiao Faust, Adam Cleveland, Matthew C. La Croix, Andrew D. Banin, Uri Pantelides, Sokrates T. Macdonald, Janet E. TI Defect Luminescence from Wurtzite CuInS2 Nanocrystals: Combined Experimental and Theoretical Analysis SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID PARTIAL CATION-EXCHANGE; SINGLE-SOURCE PRECURSOR; EXCITED-STATE DYNAMICS; ZN-S NANOCRYSTALS; CU-IN-S; QUANTUM DOTS; SEMICONDUCTOR NANOCRYSTALS; SOLAR-CELLS; TERNARY; PHOTOLUMINESCENCE AB CuInS2 nanocrystals with the wurtzite structure show promise for applications requiring efficient energy transport due to their anisotropic crystal structure. We investigate the source of photoluminescence in the near-infrared spectral region recently observed from these nanocrystals. Spectroscopic studies of both wurtzite CuInS2 itself and samples alloyed with Cd or Zn allow the assignment of this emission to a radiative point defect within the nanocrystal. structure. Further, by varying the organic passivation layer on the material, we are able to determine that the atomic species responsible for nonradiative decay paths on the nanocrystal surface are Cu- or S-based. Density functional theory calculations of defect states within the material allow identification of the likely radiative species. Understanding both the electronic structure and optical properties of wurtzite CuInS2, nanocrystals is necessary for their efficient integration into potential biological, photovoltaic, and photo catalytic applications. C1 [Leach, Alice D. P.; Cleveland, Matthew C.; La Croix, Andrew D.; Macdonald, Janet E.] Vanderbilt Univ, Dept Chem, Box 1583, Nashville, TN 37235 USA. [Shen, Xiao; Pantelides, Sokrates T.] Vanderbilt Univ, Dept Phys & Astron, Nashville, TN 37235 USA. [Pantelides, Sokrates T.] Vanderbilt Univ, Dept Elect Engn & Comp Sci, 221 Kirkland Hall, Nashville, TN 37235 USA. [Shen, Xiao] Univ Memphis, Dept Phys, Memphis, TN 38152 USA. [Faust, Adam; Banin, Uri] Hebrew Univ Jerusalem, Inst Chem, IL-91904 Jerusalem, Israel. [Faust, Adam; Banin, Uri] Hebrew Univ Jerusalem, Ctr Nanosci & Nanotechnol, IL-91904 Jerusalem, Israel. [Pantelides, Sokrates T.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Macdonald, JE (reprint author), Vanderbilt Univ, Dept Chem, Box 1583, Nashville, TN 37235 USA. EM janet.macdonald@vanderbilt.edu FU U.S.-Israel Binational Science Foundation [2012276]; Bergmann Memorial Award; Vanderbilt Institute of Nanoscale Science and Engineering; National Science Foundation (NSF) [Sus-ChEM-1253105]; U.S. Department of Energy [DE-FG02-09ER46554]; McMinn Endowment at Vanderbilt University; TN-SCORE [DMR 0907619]; NSF [EPS-1004083]; National Science Foundation [TG-CHE150005, TG-DMR130121] FX ADPL, JEM, and UB thank the U.S.-Israel Binational Science Foundation, grant number 2012276. JEM thanks the Bergmann Memorial Award. Additional funding from Vanderbilt Institute of Nanoscale Science and Engineering and National Science Foundation (NSF) Sus-ChEM-1253105. XS and SP would like to thank support from U.S. Department of Energy grant DE-FG02-09ER46554, by the McMinn Endowment at Vanderbilt University. Portions of this work were performed at Vanderbilt Institute of Nanoscale Science and Engineering, using facilities renovated and support from TN-SCORE (DMR 0907619) and NSF EPS-1004083. Computational resources were provided by the National Science Foundation through XSEDE resources under grant numbers TG-CHE150005 and TG-DMR130121. NR 49 TC 3 Z9 3 U1 8 U2 28 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 10 PY 2016 VL 120 IS 9 BP 5207 EP 5212 DI 10.1021/acs.jpcc.6b00156 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DG4LB UT WOS:000372042600052 ER PT J AU Milleville, CC Pelcher, KE Sfeir, MY Banerjee, S Watson, DF AF Milleville, Christopher C. Pelcher, Kate E. Sfeir, Matthew Y. Banerjee, Sarbajit Watson, David F. TI Directional Charge Transfer Mediated by Mid-Gap States: A Transient Absorption Spectroscopy Study of CdSe Quantum Dot/beta-Pb0.33V2O5 Heterostructures SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CONDUCTION-BAND ELECTRONS; OXIDE-SEMICONDUCTOR ELECTRODE; SENSITIZED SOLAR-CELLS; OPTICAL ELECTROCHEMISTRY; NANOSCALE HETEROSTRUCTURES; THIN-FILMS; DOTS; V2O5; NANOPARTICLES; NANOWIRES AB For solar energy conversion, not only must a, semiconductor absorb incident solar radiation efficiently- but also its photoexcited electron-hole pairs must further be separated and transported across interfaces. Charge transfer across interfaces requires consideration of both thermodynamic driving forces as well as the;competing kinetics of multiple possible transfer, cooling, and recombination pathways. In this work, we demonstrate a novel strategy for extracting holes from photoexcited CdSe quantum dots (QDs) based on interfacing with beta-Pb0.33V2O5 nanowires that have strategically positioned midgap states derived from the intercalating Pb2+ ions. Unlike midgap states derived from defects or dopants, the states utilized here are derived from the intrinsic crystal structure and are thus homogeneously distributed across the material. CdSe//beta-Pb0.33V2O5 heterostructures were assembled using two distinct methods: successive ionic layer adsorption and reaction (SILAR) and linker -assisted assembly (LAA). Transient absorption spectroscopy measurements indicate that, for both types of heterostructures, photoexcitation of CdSe QDs was followed by the transfer of electrons to the conduction band of beta-Pb0.33V2O5 nanowires and holes to the midgap states of beta-Pb0.33V2O5 nanowires. Holes were transferred on time scales less than 1 ps, whereas electrons were transferred more slowly on time scales of similar to 2 ps. In contrast, for analogous heterostructures consisting of CdSe QDs interfaced with V2O5 nanowires (wherein midgap states are absent), only electron transfer was observed. Interestingly, electron transfer was readily achieved for CdSe QDs interfaced with V2O5 nanowires by the SILAR method; however, for interfaces incorporating molecular linkers, electron transfer was observed only upon excitation at energies substantially greater than the bandgap absorption threshold of CdSe. Transient absorbance decay traces reveal longer excited state lifetimes (1-3 mu s) for CdSe/beta-Pb0.33V2O5 heterostructures relative to bare beta-Pb0.33V2O5 nanowires (0.2 to 0.6 us); the difference is attributed to surface passivation of intrinsic surface defects in beta-Pb0.33V2O5 upon interfacing with CdSe. C1 [Milleville, Christopher C.; Watson, David F.] SUNY Buffalo, Dept Chem, Buffalo, NY 14260 USA. [Pelcher, Kate E.; Banerjee, Sarbajit] Texas A&M Univ, Dept Chem, College Stn, TX 77842 USA. [Pelcher, Kate E.; Banerjee, Sarbajit] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77842 USA. [Sfeir, Matthew Y.] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Watson, DF (reprint author), SUNY Buffalo, Dept Chem, Buffalo, NY 14260 USA.; Banerjee, S (reprint author), Texas A&M Univ, Dept Chem, College Stn, TX 77842 USA.; Banerjee, S (reprint author), Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77842 USA. EM banerjee@chem.tamu.edu; dwatson3@buffalo.edu OI Watson, David/0000-0003-1203-2811 FU Research Corporation for Science Advancement through a Scialog Award; National Science Foundation [DMR 1504702]; Center for Functional Nanomaterials, a U.S. DOE Office of Science Facility [DE-SC0012704] FX This work was funded by the Research Corporation for Science Advancement through a Scialog Award. K.E.P. and S.B. also acknowledge partial support from the National Science Foundation under DMR 1504702. This research used resources of the Center for Functional Nanomaterials, which is a U.S. DOE Office of Science Facility, at Brookhaven National Laboratory under Contract No. DE-SC0012704. NR 47 TC 2 Z9 2 U1 3 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD MAR 10 PY 2016 VL 120 IS 9 BP 5221 EP 5232 DI 10.1021/acs.jpcc.6b00231 PG 12 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DG4LB UT WOS:000372042600054 ER PT J AU Piche-Choquette, S Tremblay, J Tringe, SG Constant, P AF Piche-Choquette, Sarah Tremblay, Julien Tringe, Susannah G. Constant, Philippe TI H-2-saturation of high affinity H-2-oxidizing bacteria alters the ecological niche of soil microorganisms unevenly among taxonomic groups SO PEERJ LA English DT Article DE Soil; Microbial ecology; Correlation network ID DIFFERENTIAL EXPRESSION ANALYSIS; STREPTOMYCES SP PCB7; ATMOSPHERIC HYDROGEN; NIFE HYDROGENASES; TROPOSPHERIC H-2; LEGUME NODULES; CO2 FIXATION; NITROGENASE; OXIDATION; FLEXIBILITY AB Soil microbial communities are continuously exposed to H-2 diffusing into the soil from the atmosphere. N-2-fixing nodules represent a peculiar microniche in soil where H-2 can reach concentrations up to 20,000 fold higher than in the global atmosphere (0.530 ppmv). In this study, we investigated the impact of H-2 exposure on soil bacterial community structure using dynamic microcosm chambers simulating soil H-2 exposure from the atmosphere and N-2-fixing nodules. Biphasic kinetic parameters governing H-2 oxidation activity in soil changed drastically upon elevated H-2 exposure, corresponding to a slight but significant decay of high affinity H-2-oxidizing bacteria population, accompanied by an enrichment or activation of microorganisms displaying low-affinity for H-2. In contrast to previous studies that unveiled limited response by a few species, the relative abundance of 958 bacterial ribotypes distributed among various taxonomic groups, rather than a few distinct taxa, was influenced by H-2 exposure. Furthermore, correlation networks showed important alterations of ribotype covariation in response to H-2 exposure, suggesting that H-2 affects microbe-microbe interactions in soil. Taken together, our results demonstrate that H-2-rich environments exert a direct influence on soil H-2-oxidizing bacteria in addition to indirect effects on other members of the bacterial communities. C1 [Piche-Choquette, Sarah; Constant, Philippe] Univ Quebec, Inst Armand Frappier, INRS, Laval, PQ, Canada. [Tremblay, Julien] Natl Res Council Canada, Biomonitoring, Montreal, PQ, Canada. [Tringe, Susannah G.] US DOE, Joint Genome Inst, Walnut Creek, CA USA. RP Constant, P (reprint author), Univ Quebec, Inst Armand Frappier, INRS, Laval, PQ, Canada. EM philippe.constant@iaf.inrs.ca FU Natural Sciences and Engineering Research Council of Canada; Community Sequencing Program of the Joint Genome Institute (US Department of Energy); Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX This work has been supported by a Natural Sciences and Engineering Research Council of Canada Discovery grant to PC and by the Community Sequencing Program of the Joint Genome Institute (US Department of Energy) to PC, JT and SGT. The work conducted by the US Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 52 TC 2 Z9 2 U1 5 U2 12 PU PEERJ INC PI LONDON PA 341-345 OLD ST, THIRD FLR, LONDON, EC1V 9LL, ENGLAND SN 2167-8359 J9 PEERJ JI PeerJ PD MAR 10 PY 2016 VL 4 AR e1782 DI 10.7717/peerj.1782 PG 19 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DG5TR UT WOS:000372142200004 PM 26989620 ER PT J AU Tian, HQ Lu, CQ Ciais, P Michalak, AM Canadell, JG Saikawa, E Huntzinger, DN Gurney, KR Sitch, S Zhang, BW Yang, J Bousquet, P Bruhwiler, L Chen, GS Dlugokencky, E Friedlingstein, P Melillo, J Pan, SF Poulter, B Prinn, R Saunois, M Schwalm, CR Wofsy, SC AF Tian, Hanqin Lu, Chaoqun Ciais, Philippe Michalak, Anna M. Canadell, Josep G. Saikawa, Eri Huntzinger, Deborah N. Gurney, Kevin R. Sitch, Stephen Zhang, Bowen Yang, Jia Bousquet, Philippe Bruhwiler, Lori Chen, Guangsheng Dlugokencky, Edward Friedlingstein, Pierre Melillo, Jerry Pan, Shufen Poulter, Benjamin Prinn, Ronald Saunois, Marielle Schwalm, Christopher R. Wofsy, Steven C. TI The terrestrial biosphere as a net source of greenhouse gases to the atmosphere SO NATURE LA English DT Article ID CARBON-NITROGEN INTERACTIONS; LAND-USE; ENVIRONMENTAL-CHANGES; CLIMATE EXTREMES; OXIDE EMISSIONS; METHANE; BUDGET; CO2; MODEL; ECOSYSTEMS AB The terrestrial biosphere can release or absorb the greenhouse gases, carbon dioxide (CO2), methane (CH4) and nitrous oxide (N2O), and therefore has an important role in regulating atmospheric composition and climate1. Anthropogenic activities such as land-use change, agriculture and waste management have altered terrestrial biogenic greenhouse gas fluxes, and the resulting increases in methane and nitrous oxide emissions in particular can contribute to climate change(2,3). The terrestrial biogenic fluxes of individual greenhouse gases have been studied extensively(4-6), but the net biogenic greenhouse gas balance resulting from anthropogenic activities and its effect on the climate system remains uncertain. Here we use bottom-up (inventory, statistical extrapolation of local flux measurements, and process-based modelling) and top-down (atmospheric inversions) approaches to quantify the global net biogenic greenhouse gas balance between 1981 and 2010 resulting from anthropogenic activities and its effect on the climate system. We find that the cumulative warming capacity of concurrent biogenic methane and nitrous oxide emissions is a factor of about two larger than the cooling effect resulting from the global land carbon dioxide uptake from 2001 to 2010. This results in a net positive cumulative impact of the three greenhouse gases on the planetary energy budget, with a best estimate (in petagrams of CO2 equivalent per year) of 3.9 +/- 3.8 (top down) and 5.4 +/- 4.8 (bottom up) based on the GWP100 metric (global warming potential on a 100-year time horizon). Our findings suggest that a reduction in agricultural methane and nitrous oxide emissions, particularly in Southern Asia, may help mitigate climate change. C1 [Tian, Hanqin; Lu, Chaoqun; Zhang, Bowen; Yang, Jia; Pan, Shufen] Auburn Univ, Sch Forestry & Wildlife Sci, Int Ctr Climate & Global Change Res, Auburn, AL 36849 USA. [Lu, Chaoqun] Iowa State Univ, Dept Ecol Evolut & Organismal Biol, Ames, IA 50011 USA. [Ciais, Philippe; Bousquet, Philippe; Saunois, Marielle] Lab Sci Climat & Environm, F-91191 Gif Sur Yvette, France. [Michalak, Anna M.] Carnegie Inst Sci, Dept Global Ecol, Stanford, CA 94305 USA. [Canadell, Josep G.] CSIRO Oceans & Atmosphere Res, Global Carbon Project, GPO Box 3023, Canberra, ACT 2601, Australia. [Saikawa, Eri] Emory Univ, Dept Environm Sci, Atlanta, GA 30322 USA. [Huntzinger, Deborah N.; Schwalm, Christopher R.] No Arizona Univ, Sch Earth Sci & Environm Sustainabil, Flagstaff, AZ 86011 USA. [Gurney, Kevin R.] Arizona State Univ, Sch Life Sci, Tempe, AZ 85287 USA. [Sitch, Stephen] Univ Exeter, Coll Life & Environm Sci, Exeter EX4 4RJ, Devon, England. [Bruhwiler, Lori; Dlugokencky, Edward] NOAA, Earth Syst Res Lab, Global Monitoring Div, Boulder, CO 80305 USA. [Chen, Guangsheng] Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. [Friedlingstein, Pierre] Univ Exeter, Coll Engn Math & Phys Sci, Exeter EX4 4QF, Devon, England. [Melillo, Jerry] Marine Biol Lab, Ctr Ecosyst, Woods Hole, MA 02543 USA. [Poulter, Benjamin] Montana State Univ, Inst Ecosyst, Bozeman, MT 59717 USA. [Poulter, Benjamin] Montana State Univ, Dept Ecol, Bozeman, MT 59717 USA. [Prinn, Ronald] MIT, Ctr Global Change Sci, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Schwalm, Christopher R.] Woods Hole Res Ctr, Falmouth, MA 02540 USA. [Wofsy, Steven C.] Harvard Univ, Dept Earth & Planetary Sci, 29 Oxford St, Cambridge, MA 02138 USA. RP Tian, HQ (reprint author), Auburn Univ, Sch Forestry & Wildlife Sci, Int Ctr Climate & Global Change Res, Auburn, AL 36849 USA. EM tianhan@auburn.edu RI Canadell, Josep/E-9419-2010; Friedlingstein, Pierre/H-2700-2014; Yang, Jia/A-6483-2012; OI Canadell, Josep/0000-0002-8788-3218; Yang, Jia/0000-0003-2019-9603; Zhang, Bowen/0000-0002-8370-0509 FU NASA [NNX08AL73G, NNX14AO73G, NNX10AU06G, NNX11AD47G, NNG04GM39C, NNX12AP74G, NNX10AG01A, NNX11AO08A]; NSF [AGS 1243232, AGS-1243220, CNH1210360]; Australian Climate Change Science Program; NOAA Climate Program Office [NA13OAR4310059]; NSF CAREER [AGS-0846358]; NASA Upper Atmosphere Research Program AGAGE grant [NNX11AF17G] FX This research was supported partially by NASA grants (NNX08AL73G, NNX14AO73G, NNX10AU06G, NNX11AD47G, NNG04GM39C) and NSF grants (AGS 1243232, AGS-1243220, CNH1210360). J. G. C. was supported by the Australian Climate Change Science Program. E. S. was supported by the NOAA Climate Program Office (award NA13OAR4310059). C. R. S. was supported by NASA grants (NNX12AP74G, NNX10AG01A, NNX11AO08A). K. R. G. was supported by NSF CAREER (AGS-0846358). R. G. P. was supported by a NASA Upper Atmosphere Research Program AGAGE grant (NNX11AF17G to MIT). This study contributes to the Non-CO2 Greenhouse Gases Synthesis of NACP (North American Carbon Program), and the Global Carbon Project (a joint project of IGBP, IHDP, WCRP and Diversitas). NR 77 TC 20 Z9 22 U1 77 U2 196 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD MAR 10 PY 2016 VL 531 IS 7593 BP 225 EP + DI 10.1038/nature16946 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DF9EZ UT WOS:000371665100039 PM 26961656 ER PT J AU Brahlek, MJ Koirala, N Liu, JP Yusufaly, TI Salehi, M Han, MG Zhu, YM Vanderbilt, D Oh, S AF Brahlek, Matthew J. Koirala, Nikesh Liu, Jianpeng Yusufaly, Tahir I. Salehi, Maryam Han, Myung-Geun Zhu, Yimei Vanderbilt, David Oh, Seongshik TI Tunable inverse topological heterostructure utilizing (Bi1-xInx)(2)Se-3 and multichannel weak-antilocalization effect SO PHYSICAL REVIEW B LA English DT Article ID SURFACE-STATE; INSULATOR; TRANSPORT; BI2SE3; PHASE; CONDUCTION AB In typical topological insulator (TI) systems the TI is bordered by a non-TI insulator, and the surrounding conventional insulators, including vacuum, are not generally treated as part of the TI system. Here, we implement a material system where the roles are reversed, and the topological surface states form around the non-TI (instead of the TI) layers. This is realized by growing a layer of the tunable non-TI (Bi1-xInx)(2)Se-3 in between two layers of the TI Bi2Se3 using the atomically precise molecular beam epitaxy technique. On this tunable inverse topological platform, we systematically vary the thickness and the composition of the (Bi1-xInx)(2)Se-3 layer and show that this tunes the coupling between the TI layers from strongly coupled metallic to weakly coupled, and finally to a fully decoupled insulating regime. This system can be used to probe the fundamental nature of coupling in TI materials and provides a tunable insulating layer for TI devices. C1 [Brahlek, Matthew J.; Koirala, Nikesh; Liu, Jianpeng; Yusufaly, Tahir I.; Vanderbilt, David; Oh, Seongshik] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Salehi, Maryam] Rutgers State Univ, Dept Mat Sci & Engn, Piscataway, NJ 08854 USA. [Han, Myung-Geun; Zhu, Yimei] Brookhaven Natl Lab, Condensed Matter & Phys Mat Sci Dept, Upton, NY 11973 USA. RP Brahlek, MJ (reprint author), Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. EM ohsean@physics.rutgers.edu OI Vanderbilt, David/0000-0002-2465-9091 FU NSF [DMR-1308142, DMR-1005838, DMREF-1233349]; Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF4418]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-98CH10886] FX This work is supported by the NSF (DMR-1308142, DMR-1005838, and DMREF-1233349), and by the Gordon and Betty Moore Foundation's EPiQS Initiative (GBMF4418). The work at Brookhaven National Laboratory is supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering, under Contract No. DE-AC02-98CH10886. We acknowledge J. Garlow for TEM sample preparation using the focused-ion beam at the Center for Functional Nanomaterials, Brookhaven National Laboratory. NR 30 TC 3 Z9 3 U1 6 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD MAR 10 PY 2016 VL 93 IS 12 AR 125416 DI 10.1103/PhysRevB.93.125416 PG 5 WC Physics, Condensed Matter SC Physics GA DG0FK UT WOS:000371739900004 ER EF