FN Thomson Reuters Web of Science™ VR 1.0 PT J AU Fallon, JB Irving, S Pannu, SS Tooker, AC Wise, AK Shepherd, RK Irvine, DRF AF Fallon, James B. Irving, Sam Pannu, Satinderpall S. Tooker, Angela C. Wise, Andrew K. Shepherd, Robert K. Irvine, Dexter R. F. TI Second spatial derivative analysis of cortical surface potentials recorded in cat primary auditory cortex using thin film surface arrays: Comparisons with multi-unit data SO JOURNAL OF NEUROSCIENCE METHODS LA English DT Article DE Local field potential; Cochlear implant; Cortical plasticity; Neural prosthesis; Sensorineural hearing loss ID LOCAL-FIELD POTENTIALS; ORGANIZATION; DEAFNESS; COCHLEA AB Background: Current source density analysis of recordings from penetrating electrode arrays has traditionally been used to examine the layer-specific cortical activation and plastic changes associated with changed afferent input. We report on a related analysis, the second spatial derivative (SSD) of surface local field potentials (LFPs) recorded using custom designed thin-film polyimide substrate arrays. Results: SSD analysis of tone-evoked LFPs generated from the auditory cortex under the recording array demonstrated a stereotypical single local minimum, often flanked by maxima on both the caudal and rostral sides. In contrast, tone-pips at frequencies not represented in the region under the array, but known (on the basis of normal tonotopic organization) to be represented caudal to the recording array, had a more complex pattern of many sources and sinks. Comparison with existing methods: Compared to traditional analysis of LFPs, SSD analysis produced a tonotopic map that was more similar to that obtained with multi-unit recordings in a normal-hearing animal. Additionally, the statistically significant decrease in the number of acoustically responsive cortical locations in partially deafened cats following 6 months of cochlear implant use compared to unstimulated cases observed with multi-unit data (p = 0.04) was also observed with SSD analysis (p = 0.02), but was not apparent using traditional analysis of LFPs (p = 0.6). Conclusions: SSD analysis of surface LFPs from the thin-film array provides a rapid and robust method for examining the spatial distribution of cortical activity with improved spatial resolution compared to more traditional LFP recordings. (C) 2016 Elsevier B.V. All rights reserved. C1 [Fallon, James B.; Irving, Sam; Wise, Andrew K.; Shepherd, Robert K.; Irvine, Dexter R. F.] Bion Inst, Melbourne, Vic, Australia. [Fallon, James B.; Wise, Andrew K.] Univ Melbourne, Dept Otolaryngol, Melbourne, Vic, Australia. [Fallon, James B.; Wise, Andrew K.; Shepherd, Robert K.] Univ Melbourne, Med Bion Dept, Melbourne, Vic, Australia. [Pannu, Satinderpall S.; Tooker, Angela C.] Lawrence Livermore Natl Lab, Livermore, CA USA. RP Fallon, JB (reprint author), Bion Inst, 384-388 Albert St, East Melbourne, Vic 3002, Australia. EM jfallon@bionicsinstitute.org FU NHMRC [GNT1002430]; National Institute of Deafness and Other Communication Disorders [NIH Y1-DC-8002-01]; Lawrence Livermore National Laboratory; Victorian Government through its Operational Infrastructure Support Program FX This work was funded by the NH&MRC (GNT1002430) and National Institute of Deafness and Other Communication Disorders (NIH Y1-DC-8002-01) and Lawrence Livermore National Laboratory. The Bionics Institute acknowledges the support it receives from the Victorian Government through its Operational Infrastructure Support Program. NR 23 TC 1 Z9 1 U1 4 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0165-0270 EI 1872-678X J9 J NEUROSCI METH JI J. Neurosci. Methods PD JUL 15 PY 2016 VL 267 BP 14 EP 20 DI 10.1016/j.jneumeth.2016.04.004 PG 7 WC Biochemical Research Methods; Neurosciences SC Biochemistry & Molecular Biology; Neurosciences & Neurology GA DO6WB UT WOS:000377923100002 PM 27060384 ER PT J AU Saha, D Spurri, A Chen, JH Hensley, DK AF Saha, Dipendu Spurri, Amanda Chen, Jihua Hensley, Dale K. TI Controlled release of alendronate from nitrogen-doped mesoporous carbon SO MICROPOROUS AND MESOPOROUS MATERIALS LA English DT Article DE Nitrogen doping; Mesoporous carbon; Alendronate; Osteoporosis; Controlled release ID CONTROLLED-DELIVERY; ORAL BISPHOSPHONATES; DRUG DELIVERY; IN-VITRO; BONE; SYSTEM; FUNCTIONALIZATION; MICROSPHERES; OSTEOPOROSIS; NANOSPHERES AB We have synthesized a nitrogen doped mesoporous carbon with the BET surface area of 1066 m(2)/g, total pore volume 0.6 cm(3)/g and nitrogen content of 0.5%. Total alendronate adsorption in this carbon was similar to 5%. The release experiments were designed in four different media with sequential pH values of 1.2, 4.5, 6.8 and 7.4 for 3, 1, 3 and 5 h, respectively and at 37 degrees C to imitate the physiological conditions of stomach, duodenum, small intestine and colon, respectively. Release of the drug demonstrated a controlled fashion; only 20% of the drug was released in the media with pH = 1.2, whereas 64% of the drug was released in pH = 7.4. This is in contrary to pure alendronate that was completely dissolved within 30 min in the first release media (pH = 1.2) only. The relatively larger uptake of alendronate in this carbon and its sustained fashion of release can be attributed to the hydrogen bonding between the drug and the nitrogen functionalities on carbon surface. Based on this result, it can be inferred that this formulation may lower the side effects of oral delivery of alendronate. (C) 2016 Elsevier Inc. All rights reserved. C1 [Saha, Dipendu; Spurri, Amanda] Widener Univ, Dept Chem Engn, One Univ Pl, Chester, PA 19013 USA. [Chen, Jihua; Hensley, Dale K.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Saha, D (reprint author), Widener Univ, Dept Chem Engn, One Univ Pl, Chester, PA 19013 USA. EM dsaha@mail.widener.edu RI Chen, Jihua/F-1417-2011 OI Chen, Jihua/0000-0001-6879-5936 FU School of Engineering (SOE) of Widener University; SOE of Widener University FX D.S. acknowledges the faculty development award from School of Engineering (SOE) of Widener University. A.S. acknowledges funding from SOE of Widener University for senior project, which contributed to the part of this study. The authors acknowledge the student undergraduate team members, including Tara Moken, Lauren Benham and Ather Malik for their assistance in the experiment. TEM (J.C.) and SEM (D.K.H.) experiments were conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. NR 43 TC 3 Z9 3 U1 5 U2 15 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 1387-1811 EI 1873-3093 J9 MICROPOR MESOPOR MAT JI Microporous Mesoporous Mat. PD JUL 15 PY 2016 VL 229 BP 8 EP 13 DI 10.1016/j.micromeso.2016.04.014 PG 6 WC Chemistry, Applied; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DO4DX UT WOS:000377733100002 ER PT J AU Liang, JF Yu, L Zhao, S Ying, L Liu, F Yang, W Peng, JB Cao, Y AF Liang, Junfei Yu, Lei Zhao, Sen Ying, Lei Liu, Feng Yang, Wei Peng, Junbiao Cao, Yong TI Improving efficiency and color purity of poly(9,9-dioctylfluorene) through addition of a high boiling-point solvent of 1-chloronaphthalene SO NANOTECHNOLOGY LA English DT Article DE beta-phase; poly(9,9-dioctylfluorene); polymer light-emitting diodes ID LIGHT-EMITTING-DIODES; BETA-PHASE FORMATION; POLYOCTYLFLUORENE THIN-FILM; OPTOELECTRONIC PROPERTIES; OPTICAL-PROPERTIES; IRIDIUM COMPLEX; POLYFLUORENE; POLY(9,9-DI-N-OCTYLFLUORENE); MORPHOLOGY; CARBAZOLE AB In this work, the beta-phase of poly(9,9-dioctylfluorene) (PFO) was used as a probe to study the effects of the addition of a high boiling-point solvent of 1-chloronaphthalene on the nanostructures and electroluminescence of PFO films. Both absorption and photoluminescence spectra showed that the content of the beta-phase in PFO film was obviously enhanced as a result of the addition of a small amount of 1-chloronaphthalene into the processing solvent of p-xylenes. Apparently rougher morphology associated with the effectively enhanced ordering of polymer chains across the entire film was observed for films processed from p-xylene solutions consisting of a certain amount of 1-chloronaphthalene, as revealed by atomic force microscopy and grazing incidence x-ray diffraction measurements. In addition to the effects on the nanostructures of films, of particular interest is that the performance and color purity of polymer light-emitting devices can be noticeably enhanced upon the addition of 1-chloronaphthalene. These observations highlight the importance of controlling the nanostructures of the emissive layer, and demonstrate that the addition of a low volume ratio of high boiling-point additive can be a promising strategy to attain high-performance polymer light-emitting diodes. C1 [Liang, Junfei; Yu, Lei; Zhao, Sen; Ying, Lei; Yang, Wei; Peng, Junbiao; Cao, Yong] S China Univ Technol, State Key Lab Luminescent Mat & Devices, Inst Polymer Optoelect Mat & Devices, Guangzhou 510640, Guangdong, Peoples R China. [Liu, Feng] Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. [Liu, Feng] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Ying, L (reprint author), S China Univ Technol, State Key Lab Luminescent Mat & Devices, Inst Polymer Optoelect Mat & Devices, Guangzhou 510640, Guangdong, Peoples R China. EM msleiying@scut.edu.cn; iamfengliu@gmail.com; psjbpeng@scut.edu.cn RI Ying, Lei/N-1399-2016; Liu, Feng/J-4361-2014 OI Ying, Lei/0000-0003-1137-2355; Liu, Feng/0000-0002-5572-8512 FU Ministry of Science and Technology-China [2015AA033402, 2015CB655004]; National Natural Science Foundation of China [51303056, 51473054, 51273069]; US Office of Naval Research [N00014-15-1-2244]; DOE, Office of Science, and Office of Basic Energy Sciences FX The authors are grateful for financial support from the Ministry of Science and Technology-China (2015AA033402 and 2015CB655004) and the National Natural Science Foundation of China (Grants 51303056, 51473054 and 51273069). FL was supported by the US Office of Naval Research under contract N00014-15-1-2244. Portions of this research were carried out at beamline 7.3.3 at the Advanced Light Source and Molecular Foundry, Lawrence Berkeley National Laboratory, which was supported by the DOE, Office of Science, and Office of Basic Energy Sciences. NR 46 TC 3 Z9 3 U1 8 U2 19 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD JUL 15 PY 2016 VL 27 IS 28 AR 284001 DI 10.1088/0957-4484/27/28/284001 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DO0XU UT WOS:000377503100003 PM 27250786 ER PT J AU Liu, XY McBride, SP Jaeger, HM Nealey, PF AF Liu, Xiaoying McBride, Sean P. Jaeger, Heinrich M. Nealey, Paul F. TI Hybrid nanostructures of well-organized arrays of colloidal quantum dots and a self-assembled monolayer of gold nanoparticles for enhanced fluorescence SO NANOTECHNOLOGY LA English DT Article DE colloidal quantum dots; gold nanoparticles; self-assembled monolayer; directed assembly; fluorescence enhancement ID MECHANICAL-PROPERTIES; MEMBRANES; NANOCRYSTALS; EMISSION; PHOTOLUMINESCENCE; LUMINESCENCE; FABRICATION; BRUSHES; FILMS AB Hybrid nanomaterials comprised of well-organized arrays of colloidal semiconductor quantum dots (QDs) in close proximity to metal nanoparticles (NPs) represent an appealing system for high-performance, spectrum-tunable photon sources with controlled photoluminescence. Experimental realization of such materials requires well-defined QD arrays and precisely controlled QD-metal interspacing. This long-standing challenge is tackled through a strategy that synergistically combines lateral confinement and vertical stacking. Lithographically generated nanoscale patterns with tailored surface chemistry confine the QDs into well-organized arrays with high selectivity through chemical pattern directed assembly, while subsequent coating with a monolayer of close-packed Au NPs introduces the plasmonic component for fluorescence enhancement. The results show uniform fluorescence emission in large-area ordered arrays for the fabricated QD structures and demonstrate five-fold fluorescence amplification for red, yellow, and green QDs in the presence of the Au NP monolayer. Encapsulation of QDs with a silica shell is shown to extend the design space for reliable QD/metal coupling with stronger enhancement of 11 times through the tuning of QD-metal spatial separation. This approach provides new opportunities for designing hybrid nanomaterials with tailored array structures and multiple functionalities for applications such as multiplexed optical coding, color display, and quantum transduction. C1 [Liu, Xiaoying; Nealey, Paul F.] Univ Chicago, Inst Mol Engn, 5747 South Ellis Ave, Chicago, IL 60637 USA. [McBride, Sean P.; Jaeger, Heinrich M.] Univ Chicago, James Franck Inst, 929 East 57th St, Chicago, IL 60637 USA. [McBride, Sean P.] Marshall Univ, Dept Phys & Phys Sci, Huntington, WV 25755 USA. [Jaeger, Heinrich M.] Univ Chicago, Dept Phys, 5720 South Ellis Ave, Chicago, IL 60637 USA. [Nealey, Paul F.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Jaeger, HM (reprint author), Univ Chicago, James Franck Inst, 929 East 57th St, Chicago, IL 60637 USA. EM h-jaeger@uchicago.edu; nealey@uchicago.edu FU US Air Force Office of Scientific Research (AFOSR) [FA8650-090-D-5037]; National Science Foundation (NSF) [DMR-1207204, DMR-1508110]; US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX The authors thank financial support by the US Air Force Office of Scientific Research (AFOSR) under award FA8650-090-D-5037 and National Science Foundation (NSF) through DMR-1207204 and DMR-1508110. Use of the Center for Nanoscale Materials, an Office of Science User Facility, was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 37 TC 0 Z9 0 U1 22 U2 57 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0957-4484 EI 1361-6528 J9 NANOTECHNOLOGY JI Nanotechnology PD JUL 15 PY 2016 VL 27 IS 28 AR 285301 DI 10.1088/0957-4484/27/28/285301 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DO0XU UT WOS:000377503100012 PM 27251019 ER PT J AU Kim, JH Kwon, G Lim, H Zhu, C You, H Kim, YT AF Kim, Jun-Hyuk Kwon, Gihan Lim, Hankwon Zhu, Chenhui You, Hoydoo Kim, Yong-Tae TI Effects of transition metal doping in Pt/M-TiO2 (M = V, Cr, and Nb) on oxygen reduction reaction activity SO JOURNAL OF POWER SOURCES LA English DT Article DE PEMFC; TiO2; Metal-support interaction; EXAFS; ORR; Durability ID MEMBRANE FUEL-CELLS; DOPED TIO2; CATHODE CATALYST; ELECTROCHEMICAL CHARACTERIZATION; HETEROGENEOUS CATALYSIS; ALLOY ELECTROCATALYSTS; ELECTRONIC-PROPERTIES; NANOTUBE ARRAYS; DURABILITY; NANOPARTICLES AB High cost and low durability are unresolved issues that impede the commercialization of proton exchange membrane fuel cells (PEMFCs). To overcome these limitations, Pt/TiO2 is reported as an alternative electrocatalyst for enhancing the oxygen reduction reaction (ORR) activity and/or durability of the system. However, the low electrical conductivity of TiO2 is a drawback that may be addressed by doping. To date, most reports related to Pt/doped-TiO2 focus on changes in the catalyst activity caused by the Pt-TiO2 interaction (metal -support interaction), instead of the effect of doping itself; doping is merely considered to enhance the electrical conductivity of TiO2. In this study, we discuss the variation in the electronic fine structure of Pt caused by the dopant, and its correlation with the ORR activity. More extensive contraction of the Pt lattice in Pt/M-TiO2 (M = V, Cr, and Nb) relative to Pt/TiO2 and Pt/C leads to outstanding ORR specific activity of Pt/M-TiO2. Notably, a fourfold increase of the specific activity is achieved with Pt/V-TiO2 relative to Pt/C. Furthermore, an accelerated durability test (ADT) of Pt/V-TiO2 demonstrates that this system is three times more durable than conventional Pt/C due to the metal support interaction. (C) 2016 Elsevier B.V. All rights reserved. C1 [Kim, Jun-Hyuk; Kim, Yong-Tae] Pusan Natl Univ, Sch Mech Engn, Busan 609735, South Korea. [Kim, Jun-Hyuk] Pusan Natl Univ, Hybrid Mat Solut Natl Core Res Ctr NCRC, Busan 609735, South Korea. [Kwon, Gihan] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Lim, Hankwon] Catholic Univ Daegu, Dept Chem Systemat Engn, Daegu 712702, South Korea. [Zhu, Chenhui; You, Hoydoo] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Zhu, Chenhui] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Kim, YT (reprint author), Pusan Natl Univ, Sch Mech Engn, Busan 609735, South Korea. EM yongtae@pusan.ac.kr FU National Research Foundation (NRF) of Korea [2015M1A2A2056556, 2015R1A2A1A10056156, 2013M1A8A1040703]; Nano-Convergence Foundation [R201500910]; Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant [20153030031510] FX This work was supported by the National Research Foundation (NRF) of Korea grant (2015M1A2A2056556, 2015R1A2A1A10056156, 2013M1A8A1040703), Nano-Convergence Foundation (R201500910), and Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant (20153030031510). NR 59 TC 4 Z9 4 U1 33 U2 87 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-7753 EI 1873-2755 J9 J POWER SOURCES JI J. Power Sources PD JUL 15 PY 2016 VL 320 BP 188 EP 195 DI 10.1016/j.jpowsour.2016.04.019 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Materials Science GA DN1MA UT WOS:000376828900021 ER PT J AU Tang, M Nelson, AT Wood, ES Maloy, SA Jiang, YB AF Tang, Ming Nelson, Andrew T. Wood, Elizabeth S. Maloy, Stuart A. Jiang, Ying-Bing TI Grazing incidence X-ray diffraction and transmission electron microscopy studies on the oxide formation of molybdenum in a water vapor environment SO SCRIPTA MATERIALIA LA English DT Article DE Molybdenum; Oxidation; Water vapor; GIXRD; TEM ID HIGH-TEMPERATURE OXIDATION AB To evaluate the feasibility of molybdenum as light water reactor nuclear fuel cladding, the oxidation behavior was tested in water vapor at elevated temperatures. In this study, we present experimental results on the oxidation and volatilization of molybdenum using various characterization techniques including grazing incidence X-ray diffraction and transmission electron microscopy. After oxidation testing in water vapor at 600 degrees C, experiment results show the formation of both MoO3 and MoO2. With the increasing temperature, MoO2 is the final oxidation product between 800 and 1200 degrees C, and MoO3 is volatile at these temperatures. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Tang, Ming; Nelson, Andrew T.; Wood, Elizabeth S.; Maloy, Stuart A.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Jiang, Ying-Bing] Univ New Mexico, TEM Lab, Albuquerque, NM 87131 USA. RP Tang, M (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. EM mtang@lanl.gov RI Maloy, Stuart/A-8672-2009; OI Maloy, Stuart/0000-0001-8037-1319; Nelson, Andrew/0000-0002-4071-3502 FU U.S. Department of Energy, Office of Nuclear Energy, Fuel Cycle Research and Development program FX This work was supported by the U.S. Department of Energy, Office of Nuclear Energy, Fuel Cycle Research and Development program. NR 15 TC 0 Z9 0 U1 2 U2 10 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-6462 J9 SCRIPTA MATER JI Scr. Mater. PD JUL 15 PY 2016 VL 120 BP 49 EP 53 DI 10.1016/j.scriptamat.2016.04.010 PG 5 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Science & Technology - Other Topics; Materials Science; Metallurgy & Metallurgical Engineering GA DN1DT UT WOS:000376807200012 ER PT J AU Acquaah-Mensah, GK Taylor, RC AF Acquaah-Mensah, George K. Taylor, Ronald C. TI Brain in situ hybridization maps as a source for reverse-engineering transcriptional regulatory networks: Alzheimer's disease insights SO GENE LA English DT Article DE In situ hybridization; Transcriptional regulatory networks; Alzheimer's disease; Sp3; Nfe2l1; Egr1; Usf2 ID OXIDATIVE STRESS; DIABETES-MELLITUS; GENE-EXPRESSION; AMYLOID-BETA; CELL-DEATH; DEMENTIA; RISK; INFERENCE; MEMORY; PROTEINS AB Microarray data have been a valuable resource for identifying transcriptional regulatory relationships among genes. As an example, brain region-specific transcriptional regulatory events have the potential of providing etiological insights into Alzheimer Disease (AD). However, there is often a paucity of suitable brain-region specific expression data obtained via microarrays or other high throughput means. The Allen Brain Atlas in situ hybridization (ISH) data sets (Jones et al., 2009) represent a potentially valuable alternative source of high-throughput brain region-specific gene expression data for such purposes. In this study, Allen Brain Atlas mouse ISH data in the hippocampal fields were extracted, focusing on 508 genes relevant to neurodegeneration. Transcriptional regulatory networks were learned using three high-performing network inference algorithms. Only 17% of regulatory edges from a network reverse-engineered based on brain region-specific ISH data were also found in a network constructed upon gene expression correlations in mouse whole brain microarrays, thus showing the specificity of gene expression within brain sub-regions. Furthermore, the ISH data-based networks were used to identify instructive transcriptional regulatory relationships. Ncor2, Sp3 and Usf2 form a unique three-party regulatory motif, potentially affecting memory formation pathways. Nfe211, Egrl and Usf2 emerge among regulators of genes involved in AD (e.g. Dhcr24, Aplp2, Tial, Pdrx1, Vdacl, and Syn2). Further, Nfe211, Egrl and Usf2 are sensitive to dietary factors and could be among links between dietary influences and genes in the AD etiology. Thus, this approach of harnessing brain region-specific ISH data represents a rare opportunity for gleaning unique etiological insights for diseases such as AD. (C) 2016 Elsevier B.V. All rights reserved. C1 [Acquaah-Mensah, George K.] MCPHS Univ, Massachusetts Coll Pharm & Hlth Sci, Dept Pharmaceut Sci, Worcester, MA USA. [Taylor, Ronald C.] US DOE, Pacific NW Natl Lab, Computat Biol & Bioinformat Grp, Richland, WA USA. RP Acquaah-Mensah, GK (reprint author), MCPHS Univ, Massachusetts Coll Pharm & Hlth Sci, Dept Pharmaceut Sci, Worcester, MA USA. EM george.acquaah-mensah@mcphs.edu OI Taylor, Ronald/0000-0001-9777-9767 NR 89 TC 1 Z9 1 U1 2 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0378-1119 EI 1879-0038 J9 GENE JI Gene PD JUL 15 PY 2016 VL 586 IS 1 BP 77 EP 86 DI 10.1016/j.gene.2016.03.045 PG 10 WC Genetics & Heredity SC Genetics & Heredity GA DM9OQ UT WOS:000376696000011 PM 27050105 ER PT J AU Starr, JM Li, WW Graham, SE Bradham, KD Stout, DM Williams, A Sylva, J AF Starr, James M. Li, Weiwei Graham, Stephen E. Bradham, Karen D. Stout, Daniel M., II Williams, Alan Sylva, Jason TI Using paired soil and house dust samples in an in vitro assay to assess the post ingestion bioaccessibility of sorbed fipronil SO JOURNAL OF HAZARDOUS MATERIALS LA English DT Article DE Fipronil; Bioaccessibility; Ingestion; Soils; House dusts ID DEGRADATION-PRODUCTS; PESTICIDES; FATE; METABOLITES; BEHAVIOR; SORPTION; INDOOR; FIELD; SIZE AB For children, ingestion of soils and house dusts can be an important exposure pathway for regulated organic compounds. Following ingestion, the extent to which compounds desorb and become bioaccessible is a critical determinant of systemic adsorption. We characterized the physicochemical properties of 37 soil and house dust pairs collected during a national survey of United States homes. For each sample, we measured the bioaccessibility of fipronil, a phenylpyrazole insecticide using an in vitro, three- compartment digestive system, then modeled the physicochemical predictors of fipronil bioaccessibility. The properties of the soils and dusts were not correlated and percent carbon was the only significant predictor of bioaccessibility for both soils (p < 0.001) and dusts (p < 0.001). The carbon content of the soils (3.1 +/- 2.4%) was lower than that of the dusts (18.6 +/- 6.9%) Due to the lower carbon content, soil sorbed fipronil was more bioaccessible than dust sorbed fipronil. However, the slope of the bioaccessibility carbon regression line was steeper for the soils than for the house dusts. This suggested that, for soils having carbon percentages greater than those in this study, fipronil bioaccessibility may be less than that of house dusts having equal carbon content. Published by Elsevier B.V. C1 [Starr, James M.; Bradham, Karen D.; Stout, Daniel M., II] US EPA, Natl Exposure Res Lab, Res Triangle Pk, NC 27711 USA. [Li, Weiwei] US EPA, Oak Ridge Inst Sci & Educ, Natl Exposure Res Lab, Res Triangle Pk, NC 27711 USA. [Graham, Stephen E.] US EPA, Off Air Qual Planning & Stand, Res Triangle Pk, NC 27711 USA. [Williams, Alan; Sylva, Jason] US EPA, Natl Exposure Res Lab, Las Vegas, NV 89119 USA. RP Starr, JM (reprint author), US EPA, MD D205-05,109 TW Alexander Dr, Res Triangle Pk, NC 27711 USA. EM starr.james@epa.gov FU United States Environmental Protection Agency through its Office of Research and Development FX This work was supported by The United States Environmental Protection Agency through its Office of Research and Development who funded and managed the research described here. It has been subjected to Agency administrative review and approved for publication. This does not signify that the contents necessarily reflect the views and policies of the Agency, nor does mention of trade names or commercial products constitute endorsement or recommendation for use. NR 32 TC 0 Z9 0 U1 4 U2 12 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0304-3894 EI 1873-3336 J9 J HAZARD MATER JI J. Hazard. Mater. PD JUL 15 PY 2016 VL 312 BP 141 EP 149 DI 10.1016/j.jhazmat.2016.03.053 PG 9 WC Engineering, Environmental; Engineering, Civil; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DN1AU UT WOS:000376799000016 PM 27017400 ER PT J AU Manzini, G Delzanno, GL Vencels, J Markidis, S AF Manzini, G. Delzanno, G. L. Vencels, J. Markidis, S. TI A Legendre-Fourier spectral method with exact conservation laws for the Vlasov-Poisson system SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE Vlasov-Poisson; Legendre-Fourier discretization; Conservation laws stability ID FINITE-DIFFERENCE APPROXIMATIONS; EQUATION; SIMULATIONS; SUMMATION; IMPLICIT; SCHEMES; PARTS; SPACE AB We present the design and implementation of an L-2-stable spectral method for the discretization of the Vlasov-Poisson model of a collisionless plasma in one space and velocity dimension. The velocity and space dependence of the Vlasov equation are resolved through a truncated spectral expansion based on Legendre and Fourier basis functions, respectively. The Poisson equation, which is coupled to the Vlasov equation, is also resolved through a Fourier expansion. The resulting system of ordinary differential equation is discretized by the implicit second-order accurate Crank-Nicolson time discretization. The non-linear dependence between the Vlasov and Poisson equations is iteratively solved at any time cycle by a Jacobian-Free Newton-Krylov method. In this work we analyze the structure of the main conservation laws of the resulting Legendre-Fourier model, e.g., mass, momentum, and energy, and prove that they are exactly satisfied in the semi-discrete and discrete setting. The L-2-stability of the method is ensured by discretizing the boundary conditions of the distribution function at the boundaries of the velocity domain by a suitable penalty term. The impact of the penalty term on the conservation properties is investigated theoretically and numerically. An implementation of the penalty term that does not affect the conservation of mass, momentum and energy, is also proposed and studied. A collisional term is introduced in the discrete model to control the filamentation effect, but does not affect the conservation properties of the system. Numerical results on a set of standard test problems illustrate the performance of the method. Published by Elsevier Inc. C1 [Manzini, G.; Delzanno, G. L.; Vencels, J.] Los Alamos Natl Lab, Appl Math & Plasma Phys Grp T5, POB 1663, Los Alamos, NM 87545 USA. [Markidis, S.] KTH Royal Inst Technol, HPCViz Dept, Stockholm, Sweden. [Manzini, G.] CNR, IMATI, Via Ferrata 1, I-27100 Pavia, Italy. RP Manzini, G (reprint author), Los Alamos Natl Lab, Appl Math & Plasma Phys Grp T5, POB 1663, Los Alamos, NM 87545 USA.; Manzini, G (reprint author), CNR, IMATI, Via Ferrata 1, I-27100 Pavia, Italy. EM gm.manzini@gmail.com FU Laboratory Directed Research and Development program (LDRD), under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy by Los Alamos National Laboratory [DE-AC52-06NA25396] FX This work was partially funded by the Laboratory Directed Research and Development program (LDRD), under the auspices of the National Nuclear Security Administration of the U.S. Department of Energy by Los Alamos National Laboratory, operated by Los Alamos National Security LLC under contract DE-AC52-06NA25396. NR 35 TC 0 Z9 0 U1 4 U2 6 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUL 15 PY 2016 VL 317 BP 82 EP 107 DI 10.1016/j.jcp.2016.03.069 PG 26 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DM1AX UT WOS:000376078600006 ER PT J AU Christon, MA Bakosi, J Nadiga, BT Berndt, M Francois, MM Stagg, AK Xia, YD Luo, H AF Christon, Mark A. Bakosi, Jozsef Nadiga, Balasubramanya T. Berndt, Markus Francois, Marianne M. Stagg, Alan K. Xia, Yidong Luo, Hong TI A hybrid incremental projection method for thermal-hydraulics applications SO JOURNAL OF COMPUTATIONAL PHYSICS LA English DT Article DE FVM; FEM; Incompressible flow; Monotonicity-preserving advection; Projection method; Mixed-topology meshes; Thermal-hydraulics ID NAVIER-STOKES EQUATIONS; FINITE-ELEMENT METHOD; VISCOUS INCOMPRESSIBLE-FLOW; ADVECTION-DIFFUSION EQUATION; GENERALIZED FOURIER ANALYSES; CONSISTENT MASS MATRIX; APPROXIMATE PROJECTION; LAGRANGIAN-MULTIPLIERS; POROUS-MEDIUM; PART I AB A new second-order accurate, hybrid, incremental projection method for time-dependent incompressible viscous flow is introduced in this paper. The hybrid finite-element/finite-volume discretization circumvents the well-known Ladyzhenskaya-Babuska-Brezzi conditions for stability, and does not require special treatment to filter pressure modes by either Rhie-Chow interpolation or by using a Petrov-Galerkin finite element formulation. The use of a co-velocity with a high-resolution advection method and a linearly consistent edge-based treatment of viscous/diffusive terms yields a robust algorithm for a broad spectrum of incompressible flows. The high-resolution advection method is shown to deliver second-order spatial convergence on mixed element topology meshes, and the implicit advective treatment significantly increases the stable time-step size. The algorithm is robust and extensible, permitting the incorporation of features such as porous media flow, RANS and LES turbulence models, and semi-/fully-implicit time stepping. A series of verification and validation problems are used to illustrate the convergence properties of the algorithm. The temporal stability properties are demonstrated on a range of problems with 2 <= CFL <= 100. The new flow solver is built using the Hydra multiphysics toolkit. The Hydra toolkit is written in C++ and provides a rich suite of extensible and fully-parallel components that permit rapid application development, supports multiple discretization techniques, provides I/O interfaces, dynamic run-time load balancing and data migration, and interfaces to scalable popular linear solvers, e.g., in open-source packages such as HYPRE, PETSc, and Trilinos. (C) 2016 Elsevier Inc. All rights reserved. C1 [Christon, Mark A.] Computat Sci Int, Los Alamos, NM 87544 USA. [Christon, Mark A.; Bakosi, Jozsef; Nadiga, Balasubramanya T.; Berndt, Markus] Los Alamos Natl Lab, Computat Phys & Methods Grp CCS 2, POB 1663, Los Alamos, NM 87545 USA. [Francois, Marianne M.] Los Alamos Natl Lab, Methods & Algorithms Grp XCP 4, POB 1663, Los Alamos, NM 87545 USA. [Stagg, Alan K.] Oak Ridge Natl Lab, Modeling & Simulat Grp, Oak Ridge, TN 37831 USA. [Xia, Yidong] Idaho Natl Lab, Dept Energy Resource Recovery & Sustainabil, Idaho Falls, ID 83415 USA. [Luo, Hong] N Carolina State Univ, Dept Mech & Aerosp Engn, Raleigh, NC 27695 USA. RP Berndt, M (reprint author), Los Alamos Natl Lab, Computat Phys & Methods Grp CCS 2, POB 1663, Los Alamos, NM 87545 USA. EM machriston@gmail.com; jbakosi@lanl.gov; balu@lanl.gov; berndt@lanl.gov; mmfran@lanl.gov; staggak@ornl.gov; Yidong_Xia@inl.gov; hluo2@ncsu.edu RI Luo, Hong/A-9133-2011; OI Berndt, Markus/0000-0001-5360-6848; Bakosi, Jozsef/0000-0002-0604-5555; Francois, Marianne/0000-0003-3062-6234; Xia, Yidong/0000-0002-1955-7330 FU Consortium for Advanced Simulation of Light Water Reactors an Energy Innovation Hub for Modeling and Simulation of Nuclear Reactors under U.S. Department of Energy [DE-AC05-00OR22725]; U.S. Department of Energy National Nuclear Security Administration [DE-AC52-06NA25396] FX This research was supported by the Consortium for Advanced Simulation of Light Water Reactors (http://www.casl.gov), an Energy Innovation Hub (http://www.energy.gov/hubs) for Modeling and Simulation of Nuclear Reactors under U.S. Department of Energy Contract No. DE-AC05-00OR22725. This research used resources provided by the Los Alamos National Laboratory Institutional Computing Program, which is supported by the U.S. Department of Energy National Nuclear Security Administration under Contract No. DE-AC52-06NA25396. Los Alamos Report LA-UR-16-22436. NR 50 TC 2 Z9 2 U1 3 U2 7 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0021-9991 EI 1090-2716 J9 J COMPUT PHYS JI J. Comput. Phys. PD JUL 15 PY 2016 VL 317 BP 382 EP 404 DI 10.1016/j.jcp.2016.04.061 PG 23 WC Computer Science, Interdisciplinary Applications; Physics, Mathematical SC Computer Science; Physics GA DM1AX UT WOS:000376078600019 ER PT J AU Yao, K Basnet, P Sessions, H Larsen, GK Murph, SEH Zhao, YP AF Yao, Kun Basnet, Pradip Sessions, Henry Larsen, George K. Murph, Simona E. Hunyadi Zhao, Yiping TI Fe2O3-TiO2 core-shell nanorod arrays for visible light photocatalytic applications SO CATALYSIS TODAY LA English DT Article; Proceedings Paper CT 249th National Meeting and Exposition of the Division-of-Energy-and-Fuels of American-Chemical-Society (ACS) CY MAR 22-26, 2015 CL Denver, CO SP Amer Chem Soc, Div Energy & Fuels DE Glancing angle deposition; Nanorod arrays; Core-shell Fe2O3-TiO2 ID GLANCING ANGLE DEPOSITION; CARBON-DIOXIDE; THIN-FILMS; TIO2; CONVERSION; WATER; CO2; NANOCOMPOSITES; DEGRADATION; IRRADIATION AB By using the glancing angle deposition technique and post-deposition annealing, Fe2O3-TiO2 core-shell nanorod arrays with specific crystalline states can be designed and fabricated. The Fe2O3-TiO2 core-shell samples annealed at temperatures greater than 450 degrees C formed alpha-Fe2O3 and anatase TiO2, and showed higher catalytic efficiency for the degradation of methylene blue (MB) under visible light illumination when compared with pure anatase TiO2 or alpha-Fe2O3 nanorod arrays. Solar conversion of carbon dioxide and water vapor in the presence of Fe2O3-TiO2 core-shell nanorod arrays was also investigated. Carbon monoxide, hydrogen, methane, and methanol along with other hydrocarbons were produced after only several hours' exposure under ambient sunlight. It was determined that the core-shell structure showed greater efficiency for solar CO2 conversion than the pure TiO2 nanorod arrays. Published by Elsevier B.V. C1 [Yao, Kun] Univ Georgia, Coll Engn, Athens, GA 30602 USA. [Yao, Kun; Basnet, Pradip; Zhao, Yiping] Univ Georgia, Nanoscale Sci & Engn Ctr, Athens, GA 30602 USA. [Basnet, Pradip; Zhao, Yiping] Univ Georgia, Dept Phys & Astron, Athens, GA 30602 USA. [Sessions, Henry; Larsen, George K.; Murph, Simona E. Hunyadi] Savannah River Natl Lab, Natl Secur Directorate, Savannah River Site, Aiken, SC USA. [Murph, Simona E. Hunyadi] Georgia Regents Univ, Dept Chem & Phys, Augusta, GA USA. RP Zhao, YP (reprint author), Univ Georgia, Nanoscale Sci & Engn Ctr, Athens, GA 30602 USA.; Murph, SEH (reprint author), Savannah River Natl Lab, Natl Secur Directorate, Savannah River Site, Aiken, SC USA. EM Simona.Murph@srnl.doe.gov; zhaoy@physast.uga.edu RI Basnet, Pradip/N-6649-2015 OI Basnet, Pradip/0000-0002-5619-7581 NR 42 TC 5 Z9 5 U1 31 U2 111 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0920-5861 EI 1873-4308 J9 CATAL TODAY JI Catal. Today PD JUL 15 PY 2016 VL 270 BP 51 EP 58 DI 10.1016/j.cattod.2015.10.026 PG 8 WC Chemistry, Applied; Chemistry, Physical; Engineering, Chemical SC Chemistry; Engineering GA DK7RZ UT WOS:000375124700007 ER PT J AU Franco, JM Cywiak, M Cywiak, D Mourad, I AF Manuel Franco, Juan Cywiak, Moises Cywiak, David Mourad, Idir TI Optimal focusing conditions of lenses using Gaussian beams SO OPTICS COMMUNICATIONS LA English DT Article DE Best focusing plane; Focal length; Focusing lens; Fresnel number ID CONVERGING SPHERICAL WAVES; EFFECTIVE FRESNEL-NUMBER; FOCAL SHIFT; DEPENDENCE AB By using the analytical equations of the propagation of Gaussian beams in which truncation exhibits negligible consequences, we describe a method that uses the value of the focal length of a focusing lens to classify its focusing performance. We show that for different distances between a laser and a focusing lens there are different planes where best focusing conditions can be obtained and we demonstrate how the value of the focal length impacts the lens focusing properties. To perform the classification we introduce the term delimiting focal length. As the value of the focal length used in wave propagation theory is nominal and difficult to measure accurately, we describe an experimental approach to calculate its value matching our analytical description. Finally, we describe possible applications of the results for characterizing Gaussian sources, for measuring focal lengths and/or alternatively for characterizing piston-like movements. (C) 2016 Elsevier B.V. All rights reserved. C1 [Manuel Franco, Juan; Cywiak, Moises] Ctr Invest Opt AC, Loma Del Bosque 115, Leon, Mexico. [Cywiak, David] Ctr Nacl Metrol, Queretaro 76246, Mexico. [Mourad, Idir] Brookhaven Natl Lab, NSLS II 50 Rutherford Dr, Upton, NY 11973 USA. RP Cywiak, M (reprint author), Ctr Invest Opt AC, Loma Del Bosque 115, Leon, Mexico. EM moi@cio.mx FU CONACyT FX We thank CONACyT for partial support. NR 14 TC 0 Z9 0 U1 5 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0030-4018 EI 1873-0310 J9 OPT COMMUN JI Opt. Commun. PD JUL 15 PY 2016 VL 371 BP 226 EP 230 DI 10.1016/j.optcom.2016.03.084 PG 5 WC Optics SC Optics GA DL1WJ UT WOS:000375423300037 ER PT J AU De Baere, B Molins, S Mayer, KU Francois, R AF De Baere, Bart Molins, Sergi Mayer, K. Ulrich Francois, Roger TI Determination of mineral dissolution regimes using flow-through time-resolved analysis (FT-TRA) and numerical simulation SO CHEMICAL GEOLOGY LA English DT Article DE Dissolution regime; Flow-through; Mineral dissolution; Dissolution rates; Forsterite dissolution; Calcite dissolution ID NAVIER-STOKES EQUATIONS; CALCITE DISSOLUTION; FORSTERITE DISSOLUTION; DIFFUSION CONTROL; AQUEOUS-SOLUTIONS; KINETICS; RATES; PH; 25-DEGREES-C; DEPENDENCE AB Flow-through time resolved analysis (FT-TRA) involves subjecting small mineral samples (<10 mg) inserted in a miniature flow-through cell (50 mu L) to controlled flows of eluent analyzed on-line by ICP-MS. In this study, FT-TRA is used to empirically determine the dissolution regimes for the two well-studied minerals forsterite and calcite, representing minerals with relatively slow and fast dissolution kinetics. A proportional increase in steady-state effluent [Mg, Si] concentrations with increasing flow-through cell eluent residence times confirms a dominantly surface-controlled dissolution regime for a powdered forsterite sample at pH 2.3, implying that transport limitations are negligible. In contrast, the relationship between flow rates and dissolution rates for single grain calcite samples at pH 2.3-4 reveals that transport limitations affect the rate of calcite dissolution. To provide a quantitative and process-based assessment of the effect of diffusive transport limitations, simulations of the calcite experiments were performed with a high resolution, pore-scale model that considers the geometry of the calcite grain and the FT-TRA flow-through reactor. The pore-scale model reproduces the observed effluent [Ca] concentrations for all experimental conditions using a single set of surface kinetic parameters, by accounting for the formation of a diffusive boundary layer (DBL) that varies in thickness as a function of flowrates. These results demonstrate that combining FT-TRA with pore-scale modeling makes it possible to obtain unprecedented insights not achievable by either method separately, including quantification of DBL thicknesses and the determination of transport controls as a function of pH, flow velocity and residence times. (C) 2016 Elsevier B.V. All rights reserved. C1 [De Baere, Bart; Mayer, K. Ulrich; Francois, Roger] Univ British Columbia, Dept Earth Ocean & Atmospher Sci, 2020-2207 Main Mall, Vancouver, BC V6T 1Z4, Canada. [Molins, Sergi] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Earth & Environm Sci, 1 Cyclotron Rd,MS 74R316C, Berkeley, CA 94720 USA. RP De Baere, B (reprint author), Univ British Columbia, Dept Earth Ocean & Atmospher Sci, 2020-2207 Main Mall, Vancouver, BC V6T 1Z4, Canada. EM b.debaere@alumni.ubc.ca; smolins@lbl.gov; umayer@eos.ubc.ca; rfrancoi@eos.ubc.ca RI Molins, Sergi/A-9097-2012; OI Molins, Sergi/0000-0001-7675-3218; De Baere, Bart/0000-0002-3136-5497; Mayer, K. Ulrich/0000-0002-4168-781X FU Center for Nanoscale Control of Geologic CO2, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-05CH11231] FX The authors would like to thank 3 anonymous reviewers for constructive criticisms and feedback. S.M. was supported as part of the Center for Nanoscale Control of Geologic CO2, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-AC02-05CH11231. The authors would like to acknowledge Vivian Lai and Marghaleray Amini at the Pacific Centre for Isotopic and Geochemical Research (PCIGR). Method development has been made possible using a NSERC Research Tools and Instrumentation grant. Finally, BDB thanks Derrick Horne for technical SEM assistance and training at the UBC BioImaging Facility. NR 50 TC 2 Z9 2 U1 6 U2 17 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0009-2541 EI 1878-5999 J9 CHEM GEOL JI Chem. Geol. PD JUL 15 PY 2016 VL 430 BP 1 EP 12 DI 10.1016/j.chemgeo.2016.03.014 PG 12 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DK1FS UT WOS:000374658500001 ER PT J AU Sampath, S Rementeria, R Huang, X Poplawsky, JD Garcia-Mateo, C Caballero, FG Janisch, R AF Sampath, S. Rementeria, R. Huang, X. Poplawsky, J. D. Garcia-Mateo, C. Caballero, F. G. Janisch, R. TI The role of silicon, vacancies, and strain in carbon distribution in low temperature bainite SO JOURNAL OF ALLOYS AND COMPOUNDS LA English DT Article DE Metals and alloys; Atomic scale structure; Microstructure; Computer simulations; Atom probe tomography ID TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; CARBIDE PRECIPITATION; ALPHA-IRON; FERRITE; SUPERSATURATION; STEELS; TRANSFORMATION; TETRAGONALITY; MARTENSITES AB We investigated the phenomenon of carbon supersaturation and carbon clustering in bainitic ferrite with atom probe tomography (APT) and ab-initio density functional theory (DFT) calculations. The experimental results show a homogeneous distribution of silicon in the microstructure, which contains both ferrite and retained austenite. This distribution is mimicked well by the computational approach. In addition, an accumulation of C in certain regions of the bainitic ferrite with C concentrations up to 13 at % is observed. Based on the DFT results, these clusters are explained as strained, tetragonal regions in the ferritic bainite, in which the solution enthalpy of C can reach large, negative values. It seems that Si itself only has a minor influence on this phenomenon. (C) 2016 Elsevier B.V. All rights reserved. C1 [Sampath, S.; Huang, X.; Janisch, R.] Ruhr Univ Bochum, ICAMS, D-44780 Bochum, Germany. [Rementeria, R.; Garcia-Mateo, C.; Caballero, F. G.] CSIC, Natl Ctr Met Res CENIM, Dept Met Phys, Avda Gregorio del Amo 8, E-28040 Madrid, Spain. [Poplawsky, J. D.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, 1 Bethel Valley Rd,POB 2008,MS 6064, Oak Ridge, TN 37831 USA. RP Janisch, R (reprint author), Ruhr Univ Bochum, ICAMS, D-44780 Bochum, Germany. EM rebecca.janisch@rub.de RI CABALLERO, FRANCISCA/A-4292-2008; Garcia-Mateo, Carlos/A-7752-2008; OI Garcia-Mateo, Carlos/0000-0002-4773-5077; Rementeria, Rosalia/0000-0003-2364-7344; Janisch, Rebecca/0000-0003-2136-0788 FU Research Fund for Coal and Steel [RFSR-CT-2012-00017] FX APT measurements and analyses were conducted at ORNL's Center for Nanophase Materials Sciences (CNMS), which is a U.S. Department of Energy, Office of Science User Facility. The authors gratefully acknowledge the support of the Research Fund for Coal and Steel for funding this research under the Contract RFSR-CT-2012-00017. NR 35 TC 1 Z9 1 U1 5 U2 29 PU ELSEVIER SCIENCE SA PI LAUSANNE PA PO BOX 564, 1001 LAUSANNE, SWITZERLAND SN 0925-8388 EI 1873-4669 J9 J ALLOY COMPD JI J. Alloy. Compd. PD JUL 15 PY 2016 VL 673 BP 289 EP 294 DI 10.1016/j.jallcom.2016.02.151 PG 6 WC Chemistry, Physical; Materials Science, Multidisciplinary; Metallurgy & Metallurgical Engineering SC Chemistry; Materials Science; Metallurgy & Metallurgical Engineering GA DI4JO UT WOS:000373466400039 ER PT J AU Harrison, AW Ryazanov, M Sullivan, EN Neumark, DM AF Harrison, Aaron W. Ryazanov, Mikhail Sullivan, Erin N. Neumark, Daniel M. TI Photodissociation dynamics of the methyl perthiyl radical at 248 and 193 nm using fast-beam photofragment translational spectroscopy SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID FLIGHT MASS-SPECTROMETER; ISOMERIC CH3S2; SULFUR; CH3SSCH3; CHEMISTRY AB The photodissociation dynamics of the methyl perthiyl radical (CH3SS) have been investigated using fast-beam coincidence translational spectroscopy. Methyl perthiyl radicals were produced by photodetachment of the CH3SS- anion followed by photodissociation at 248 nm ( 5.0 eV) and 193 nm ( 6.4 eV). Photofragment mass distributions and translational energy distributions were measured at each dissociation wavelength. Experimental results show S atom loss as the dominant ( 96%) dissociation channel at 248 nm with a near parallel, anisotropic angular distribution and translational energy peaking near the maximal energy available to ground state CH3S and S fragments, indicating that the dissociation occurs along a repulsive excited state. At 193 nm, S atom loss remains the major fragmentation channel, although S-2 loss becomes more competitive and constitutes 32% of the fragmentation. The translational energy distributions for both channels are very broad at this wavelength, suggesting the formation of the S-2 and S atom products in several excited electronic states. Published by AIP Publishing. C1 [Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Harrison, Aaron W.] Univ New South Wales Kensington, Sch Chem, Sydney, NSW 2052, Australia. [Ryazanov, Mikhail] JILA, 440 Univ Ave, Boulder, CO 80309 USA. RP Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu RI Neumark, Daniel/B-9551-2009 OI Neumark, Daniel/0000-0002-3762-9473 FU Office of Basic Energy Science, Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors would like to thank Dr. Neil-Cole Filipiak and Mark Shapero for their help in completing this work. This research was supported by the Director, Office of Basic Energy Science, Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 39 TC 1 Z9 1 U1 2 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 14 PY 2016 VL 145 IS 2 AR 024305 DI 10.1063/1.4955195 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DT0DS UT WOS:000381153600016 PM 27421403 ER PT J AU Golt, MC Strawhecker, KE Bratcher, MS Shanholtz, ER AF Golt, M. C. Strawhecker, K. E. Bratcher, M. S. Shanholtz, E. R. TI Polycrystalline silicon carbide dopant profiles obtained through a scanning nano-Schottky contact SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID ATOMIC-FORCE MICROSCOPY; THERMIONIC-FIELD EMISSION; BARRIER HEIGHT; GRAIN-BOUNDARIES; CERAMICS; DEPENDENCE; INTERFACES; TRANSPORT; SIC/SIO2; DIODES AB The unique thermo-electro-mechanical properties of polycrystalline silicon carbide (poly-SiC) make it a desirable candidate for structural and electronic materials for operation in extreme environments. Necessitated by the need to understand how processing additives influence poly-SiC structure and electrical properties, the distribution of lattice defects and impurities across a specimen of hot-pressed 6H poly-SiC processed with p-type additives was visualized with high spatial resolution using a conductive atomic force microscopy approach in which a contact forming a nano-Schottky interface is scanned across the sample. The results reveal very intricate structures within poly-SiC, with each grain having a complex core-rim structure. This complexity results from the influence the additives have on the evolution of the microstructure during processing. It was found that the highest conductivities localized at rims as well as at the interface between the rim and the core. The conductivity of the cores is less than the conductivity of the rims due to a lower concentration of dopant. Analysis of the observed conductivities and current-voltage curves is presented in the context of nano-Schottky contact regimes where the conventional understanding of charge transport to diode operation is no longer valid. C1 [Golt, M. C.; Strawhecker, K. E.; Bratcher, M. S.] US Army Res Lab, WMRD, Aberdeen Proving Ground, MD 21005 USA. [Shanholtz, E. R.] ORISE, Belcamp, MD 21017 USA. RP Golt, MC (reprint author), US Army Res Lab, WMRD, Aberdeen Proving Ground, MD 21005 USA. FU U.S. Department of Energy; U.S. Army Research Laboratory FX The authors would like to thank Dr. Thomas Parker for performing XPS analysis of the native oxide thickness and Dr. Kristopher Behler for performing the Raman analysis of the polytype composition. This project was supported in part by an appointment to the Internship/Research Participation Program for the U.S. Army Research Laboratory administered by the Oak Ridge Institute for Science and Education (ORISE) through an agreement between the U.S. Department of Energy and the U.S. Army Research Laboratory. NR 41 TC 0 Z9 0 U1 3 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 14 PY 2016 VL 120 IS 2 AR 024302 DI 10.1063/1.4957177 PG 10 WC Physics, Applied SC Physics GA DT0CW UT WOS:000381151200007 ER PT J AU Cole-Filipiak, NC Shapero, M Haibach-Morris, C Neumark, DM AF Cole-Filipiak, Neil C. Shapero, Mark Haibach-Morris, Courtney Neumark, Daniel M. TI Production and Photodissociation of the Methyl Perthiyl Radical SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID ELECTRON-IMPACT IONIZATION; SULFUR-CONTAINING MOLECULES; 193 NM; DISSOCIATIVE IONIZATION; TROPOSPHERIC CHEMISTRY; DIMETHYL DISULFIDE; ABSORPTION-SPECTRA; ISOMERIC CH3S2; SPECTROSCOPY; DYNAMICS AB The photodissociation dynamics of the methyl perthiyl (CH3SS) radical are investigated via molecular beam photofragment translational spectroscopy, using "soft" electron ionization to detect the radicals and their photofragments. With this new capability, we have shown that CH3SS can be generated from flash pyrolysis of dimethyl trisulfide. Utilizing this source of radicals and the advantages afforded by soft electron ionization, we have reinvestigated the photodissociation dynamics of CH3SS at 248 nm, finding CH3S + S to be the dominant dissociation channel with CH3 + SS as a minor process. These results differ from previous work reported in our laboratory in which we found CH3 + SS and CH2S + SH as the main dissociation channels. The difference in results is discussed in light of our new capabilities for characterization of radical production. C1 [Cole-Filipiak, Neil C.; Shapero, Mark; Neumark, Daniel M.] Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA. [Cole-Filipiak, Neil C.; Shapero, Mark; Haibach-Morris, Courtney; Neumark, Daniel M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Cole-Filipiak, Neil C.] Univ Warwick, Dept Chem, Coventry CV4 7AL, W Midlands, England. RP Neumark, DM (reprint author), Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA.; Neumark, DM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM dneumark@berkeley.edu RI Neumark, Daniel/B-9551-2009 OI Neumark, Daniel/0000-0002-3762-9473 FU Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX The authors thank Narbe Mardirossian and Yuezhi Mao for assistance with Q-Chem, Patrick W. Smith for synthesis of a potential radical precursor, and Drs. Aaron W. Harrison and Mikhail Ryazanov for helpful discussions. This work was supported by the Director, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 66 TC 0 Z9 0 U1 3 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 14 PY 2016 VL 120 IS 27 BP 4818 EP 4826 DI 10.1021/acs.jpca.5b12284 PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DR6CE UT WOS:000379988900025 PM 26859337 ER PT J AU Bandyopadhyay, B Stein, T Fang, YG Kostko, O White, A Head-Gordon, M Ahmed, M AF Bandyopadhyay, Biswajit Stein, Tamar Fang, Yigang Kostko, Oleg White, Alec Head-Gordon, Martin Ahmed, Musahid TI Probing Ionic Complexes of Ethylene and Acetylene with Vacuum-Ultraviolet Radiation SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID POTENTIAL-ENERGY SURFACE; POLYCYCLIC AROMATIC-HYDROCARBONS; CYCLOBUTADIENE RADICAL-CATION; VUV PHOTOIONIZATION; UNSATURATED COMPOUNDS; WATER CLUSTERS; POLYMERIZATION; SPECTROSCOPY; IONIZATION; DYNAMICS AB Mixed complexes of acetylene ethylene are studied using vacuum-ultraviolet (VUV) photoionization mass spectrometry and theoretical calculations. These complexes are produced and ionized at different distances from the exit of a continuous nozzle followed by reflectron time-of-flight mass spectrometry detection. Acetylene, with a higher ionization energy (11.4 eV) than ethylene (10.6 eV), allows for tuning the VUV energy and initializing reactions either from a C2H2+ or a C2H4+ cation. Pure acetylene and ethylene expansions are separately carried out to compare, contrast, and hence identify products from the mixed expansion: these are C3H3+ (m/z = 39), C4H5+ (m/z = 53), and C5H5+ (m/z = 65). Intensity distributions of C2H2, C2H4, their dimers and reactions products are plotted as a function of ionization distance. These distributions suggest that association mechanisms play a crucial role in product formation closer to the nozzle. Photoionization efficiency (PIE) curves of the mixed complexes demonstrate rising edges closer to both ethylene and acetylene ionization energies. We use density functional theory (omega B97X-V/aug-cc-pVTZ) to study the structures of the neutral and ionized dimers, calculate their adiabatic and vertical ionization energies, as well as the energetics of different isomers on the potential energy surface (PES). Upon ionization, vibrationally excited clusters can use the extra energy to access different isomers on the PES. At farther ionization distances from the nozzle, where the number densities are lower, unimolecular decay is expected to be the dominant mechanism. We discuss the possible decay pathways from the different isomers on the PES and examine the ones that are energetically accessible. C1 [Bandyopadhyay, Biswajit; Stein, Tamar; Fang, Yigang; Kostko, Oleg; White, Alec; Head-Gordon, Martin; Ahmed, Musahid] Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Stein, Tamar; White, Alec; Head-Gordon, Martin] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Head-Gordon, M; Ahmed, M (reprint author), Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Head-Gordon, M (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. EM mhg@cchem.berkeley.edu; MAhmed@lbl.gov RI Ahmed, Musahid/A-8733-2009 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; National Aeronautics and Space Administration through the NASA Astrobiology Institute [NNH13ZDA017C] FX This work and the Advanced Light Source are supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. M.H.G. and T.S. acknowledge additional support from The National Aeronautics and Space Administration through the NASA Astrobiology Institute under Cooperative Agreement Notice NNH13ZDA017C. NR 41 TC 0 Z9 0 U1 4 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 14 PY 2016 VL 120 IS 27 BP 5053 EP 5064 DI 10.1021/acs.jpca.6b00107 PG 12 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DR6CE UT WOS:000379988900052 PM 26983013 ER PT J AU Pratt, LR Chaudhari, MI Rempe, SB AF Pratt, Lawrence R. Chaudhari, Mangesh I. Rempe, Susan B. TI Statistical Analyses of Hydrophobic Interactions: A Mini-Review SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Review ID SCALED-PARTICLE THEORY; AQUEOUS-SOLUTION; PRESSURE-DEPENDENCE; MOLECULAR-DYNAMICS; ATTRACTIVE FORCES; HYDROGEN GAS; LOOP-CLOSURE; BULK WATER; HYDRATION; MODELS AB This review focuses on the striking recent progress in solving for hydrophobic interactions between small inert molecules. We discuss several new understandings. First, the inverse temperature phenomenology of hydrophobic interactions, i.e., strengthening of hydrophobic bonds with increasing temperature, is decisively exhibited by hydrophobic interactions between atomic-scale hard sphere solutes in water. Second, inclusion of attractive interactions associated with atomic-size hydrophobic reference cases leads to substantial, nontrivial corrections to reference results for purely repulsive solutes. Hydrophobic bonds are weakened by adding solute dispersion forces to treatment of reference cases. The classic statistical mechanical theory for those corrections is not accurate in this application, but molecular quasi-chemical theory shows promise. Finally, because of the masking roles of excluded volume and attractive interactions, comparisons that do not discriminate the different possibilities face an interpretive danger. C1 [Pratt, Lawrence R.] Tulane Univ, Dept Chem & Biomol Engn, New Orleans, LA 70118 USA. [Chaudhari, Mangesh I.; Rempe, Susan B.] Sandia Natl Labs, Ctr Biol & Engn Sci, Albuquerque, NM 87185 USA. RP Pratt, LR (reprint author), Tulane Univ, Dept Chem & Biomol Engn, New Orleans, LA 70118 USA.; Chaudhari, MI; Rempe, SB (reprint author), Sandia Natl Labs, Ctr Biol & Engn Sci, Albuquerque, NM 87185 USA. EM lpratt@tulane.edu; michaud@sandia.gov; slrempe@sandia.gov FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL8500]; Sandia's LDRD program; Defense Threat Reduction Agency (DTRA); U.S. DOE's Office of Science [DE-AC52-06NA25396] FX Sandia National Laboratories (SNL) is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL8500. The financial support of Sandia's LDRD program and the Defense Threat Reduction Agency (DTRA) is gratefully acknowledged. The work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. DOE's Office of Science by Los Alamos National Laboratory (Contract DE-AC52-06NA25396) and SNL. NR 64 TC 0 Z9 0 U1 9 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUL 14 PY 2016 VL 120 IS 27 BP 6455 EP 6460 DI 10.1021/acs.jpcb.6b04082 PG 6 WC Chemistry, Physical SC Chemistry GA DR6CZ UT WOS:000379991000001 PM 27258151 ER PT J AU Schwierz, N Lam, RK Gamlieli, Z Tills, JJ Leung, A Geissler, PL Saykally, RJ AF Schwierz, Nadine Lam, Royce K. Gamlieli, Zach Tills, Jeremiah J. Leung, Alvin Geissler, Phillip L. Saykally, Richard J. TI Hydrogen and Electric Power Generation from Liquid Microjets: Design Principles for Optimizing Conversion Efficiency SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID AIR-WATER-INTERFACE; ELECTROKINETIC ENERGY-CONVERSION; STREAMING CURRENT MEASUREMENTS; NANOFLUIDIC CHANNELS; HOFMEISTER SERIES; PHOTOELECTRON-SPECTRA; WATER/VAPOR INTERFACE; SURFACE CONDUCTIVITY; HYDROPHILIC SURFACES; SOLVATED ELECTRONS AB Liquid water microjets have been successfully employed for both electrical power generation and gaseous hydrogen production, but the demonstrated efficiencies have been low. Here, we employ a combination of a modified Poisson-Boltzmann description, continuum hydrodynamic equations, and microjet electrokinetic experiments to gain detailed insight into the origin of the streaming currents produced in pure water. We identify the contributions to the streaming current from specific ion adsorption at the solid/liquid interface and from long-ranged electrostatic interactions, finding that the portion originating from the latter dominate at charged surfaces. The detailed understanding afforded by theory and the close agreement with experimental results elucidates design principles for optimizing hydrogen production and power generation. Changing the sign of the surface charge density through targeted use of surface coatings via silanization switches the primary charge carrier between hydronium and hydroxide and therefore switches the corresponding production of molecular hydrogen to oxygen at the target electrode. Moreover, hydrophobic surface coatings reduce dissipation due to fluid/solid friction, thereby increasing the conversion efficiency. C1 [Schwierz, Nadine; Lam, Royce K.; Gamlieli, Zach; Tills, Jeremiah J.; Leung, Alvin; Geissler, Phillip L.; Saykally, Richard J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Lam, Royce K.; Geissler, Phillip L.; Saykally, Richard J.] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Geissler, Phillip L.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Schwierz, N; Saykally, RJ (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Saykally, RJ (reprint author), Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM nschwierz@berkeley.edu; saykally@berkeley.edu OI Lam, Royce/0000-0003-2878-038X FU Alexander von Humboldt Foundation; NSF EAGER Program [CHE-0963844]; Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy (DOE) through the Chemical Sciences Division and Material Sciences Division of the Lawrence Berkeley National Laboratory (LBNL) [DE-AC02-05CH11231] FX N.S. thanks the Alexander von Humboldt Foundation for financial support. The early stages of this work were supported by a grant from the NSF EAGER Program (Grant CHE-0963844). R.K.L. was supported by the Director, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy (DOE) under Contract No. DE-AC02-05CH11231, through the Chemical Sciences Division and Material Sciences Division of the Lawrence Berkeley National Laboratory (LBNL). NR 58 TC 0 Z9 0 U1 4 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 14 PY 2016 VL 120 IS 27 BP 14513 EP 14521 DI 10.1021/acs.jpcc.6b03788 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DR6CT UT WOS:000379990400006 ER PT J AU Assary, RS Zhang, L Huang, JH Curtiss, LA AF Assary, Rajeev S. Zhang, Lu Huang, Jinhua Curtiss, Larry A. TI Molecular Level Understanding of the Factors Affecting the Stability of Dimethoxy Benzene Catholyte Candidates from First-Principles Investigations SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID ELECTRICAL ENERGY-STORAGE; LITHIUM-ION BATTERIES; SOLVATION FREE-ENERGIES; REDOX-FLOW BATTERIES; ORGANIC-MOLECULES; OVERCHARGE PROTECTION; REDUCTION POTENTIALS; CATHODE MATERIALS; SHUTTLE; ELECTROLYTES AB First-principles simulations are performed to gain molecular level insights into the factors affecting the stability of seven 1,4-dimethoxybenzene (DMB) derivatives. These molecules are potential catholyte candidates for nonaqueous redox flow battery systems. Computations are performed to predict oxidation potentials in various dielectric mediums, intrinsic-reorganization energies, and structural changes of these representative catholyte molecules during the redox process. In order to understand the stability of the DMB-based radical cations, the thermodynamic feasibility of the following reactions is computed using density functional theory: (a) deprotonation, (b) dimerization, (c) hydrolysis, and (d) demethylation. The computations indicate that radical cations of the 2,3-dimethyl and 2,5-dimethyl derivatives are the most stable among the DMB derivatives considered in this study. In the presence of solvents with high-proton solvating ability (water, DMSO, acetonitrile), degradation of cation radical occurring via deprotonation is the most likely mechanism. In the presence of solvents such as propylene carbonate (PC), demethylation was found to be the most likely reaction that causes degradation of radical cations. From the computed enthalpy of activation (Delta H-double dagger) for a demethylation reaction in PC, the 2,5-dimethyl DMB cation radical would exhibit better kinetic stability in comparison to the other candidates. This investigation suggests that computational studies of structural properties such as redox potentials, reorganization energies, and the computed reaction energetics (deprotonation and demethylation) of charged species can be used to predict the relative stability of a large set of molecules required for the discovery of novel redox active materials for flow battery applications. C1 [Assary, Rajeev S.; Zhang, Lu; Huang, Jinhua; Curtiss, Larry A.] Argonne Natl Lab, Joint Ctr Energy Storage Res, Argonne, IL 60439 USA. [Assary, Rajeev S.; Curtiss, Larry A.] Argonne Natl Lab, Div Sci Mat, Argonne, IL 60439 USA. [Zhang, Lu; Huang, Jinhua] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. RP Assary, RS (reprint author), Argonne Natl Lab, Joint Ctr Energy Storage Res, Argonne, IL 60439 USA.; Assary, RS (reprint author), Argonne Natl Lab, Div Sci Mat, Argonne, IL 60439 USA. EM assary@anl.gov FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences FX This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. We gratefully acknowledge the computing resources provided on "Blues", a 320-node computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 38 TC 3 Z9 3 U1 9 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 14 PY 2016 VL 120 IS 27 BP 14531 EP 14538 DI 10.1021/acs.jpcc.6b04263 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DR6CT UT WOS:000379990400008 ER PT J AU Kim, C Pilania, G Ramprasad, R AF Kim, Chiho Pilania, Ghanshyam Ramprasad, Rampi TI Machine Learning Assisted Predictions of Intrinsic Dielectric Breakdown Strength of ABX(3) Perovskites SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID THERMAL-OXIDATION; RATIONAL DESIGN; ELECTRON-GAS; SILICON; OXIDES; REDISTRIBUTION; CRYSTALS; EXCHANGE; FIELD AB New and improved dielectric materials with high dielectric breakdown strength are required for both high energy density electric energy storage applications and continued miniaturization of electronic devices. Despite much practical significance, accurate ab initio predictions of dielectric breakdown strength for complex materials are beyond the current state-of-the art. Here we take an alternative data-enabled route to address this design problem. Our informatics-based approach employs a transferable machine learning model, trained and validated on a limited amount of accurate data generated through laborious first-principles computations, to predict intrinsic dielectric breakdown strength of several hundreds of chemical compositions in a highly efficient manner. While the adopted approach is quite general, here we take up a specific example of perovskite materials to demonstrate the efficacy of our method. Starting from several thousands of compounds, we systematically downselect 209 insultors which are dynamically stable in a perovskite crystal structure. After making predictions on these compounds using our machine learning model, the intrinsic dielectric breakdown strength was further cross-validated using first-principles computations. Our analysis reveals that boron-containing compounds are of particular interest, some of which exhibit remarkable intrinsic breakdown strength of almost 2 GV/m. C1 [Kim, Chiho; Ramprasad, Rampi] Univ Connecticut, Dept Mat Sci & Engn, 97 North Eagleville Rd, Storrs, CT 06269 USA. [Kim, Chiho; Ramprasad, Rampi] Univ Connecticut, Inst Mat Sci, 97 North Eagleville Rd, Storrs, CT 06269 USA. [Pilania, Ghanshyam] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. RP Ramprasad, R (reprint author), Univ Connecticut, Dept Mat Sci & Engn, 97 North Eagleville Rd, Storrs, CT 06269 USA.; Ramprasad, R (reprint author), Univ Connecticut, Inst Mat Sci, 97 North Eagleville Rd, Storrs, CT 06269 USA. EM rampi@uconn.edu OI Pilania, Ghanshyam/0000-0003-4460-1572 FU Office of Naval Research [N00014-10-1-0944, N00014-15-1-2665]; Multidisciplinary University Research Initiative (MURI) grant; U.S. Department of Energy through the LANL/LDRD grant [20140679PRD3] FX This paper is based on work supported by the Office of Naval Research through grants N00014-10-1-0944 and N00014-15-1-2665, the former being a Multidisciplinary University Research Initiative (MURI) grant. Computational support was provided by the Extreme Science and Engineering Discovery Environment (XSEDE) and the National Energy Research Scientific Computing Center (NERSC). G.P. acknowledges the support of the U.S. Department of Energy through the LANL/LDRD grant (20140679PRD3) as a Director's postdoctoral fellowship. Ying Sun and Clive Bealing are acknowledged for a prior post Quantum ESPRESSO code development effort to compute the intrinsic dielectric breakdown field. NR 44 TC 2 Z9 2 U1 17 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 14 PY 2016 VL 120 IS 27 BP 14575 EP 14580 DI 10.1021/acs.jpcc.6b05068 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DR6CT UT WOS:000379990400013 ER PT J AU Babar, S Mane, AU Yanguas-Gil, A Mohimi, E Haasch, RT Elam, JW AF Babar, Shaista Mane, Anil U. Yanguas-Gil, Angel Mohimi, Elham Haasch, Richard T. Elam, Jeffrey W. TI W:Al2O3 Nanocomposite Thin Films with Tunable Optical Properties Prepared by Atomic Layer Deposition SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID HIGH-TEMPERATURE; ALLOY-FILMS; ELECTRICAL-PROPERTIES; SELECTIVE ABSORBERS; COATINGS; GROWTH; OXIDE; NANOSTRUCTURES; CERMETS; AL2O3 AB A systematic alteration in the optical properties of W:Al2O3 nanocomposite films is demonstrated by precisely varying the W cycle percentage (W%) from 0 to 100% in Al2O3 during atomic layer deposition. The direct and indirect band energies of the nanocomposite materials decrease from 5.2 to 4.2 eV and from 3.3 to 1.8 eV, respectively, by increasing the W% from 10 to 40. X-ray absorption spectroscopy reveals that, for W% < 50, W is present in both metallic and suboxide states, whereas, for W% >= 50, only metallic W is seen. This transition from dielectric to metallic character at W% similar to 50 is accompanied by an increase in the electrical and thermal conductivity and the disappearance of a dear band gap in the absorption spectrum. The density of the films increases monotonically from 3.1 g/cm(3) for pure Al2O3 to 17.1 g/cm(3) for pure W, whereas the surface roughness is greatest for the W% = 50 films. The W:Al2O3 nanocomposite films are thermally stable and show little change in optical properties upon annealing in air at 500 degrees C. These W:Al2O3 nanocomposite films show promise as selective solar absorption coatings for concentrated solar power applications. C1 [Babar, Shaista; Mane, Anil U.; Yanguas-Gil, Angel; Elam, Jeffrey W.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mohimi, Elham] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61820 USA. [Haasch, Richard T.] Univ Illinois, Mat Res Lab, Urbana, IL 61820 USA. RP Elam, JW (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jelam@anl.gov FU Argonne Laboratory Directed Research and Development (LDRD) [2015-151-N0]; U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, through the SuNLaMP program; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the Argonne Laboratory Directed Research and Development (LDRD) project 2015-151-N0 and the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, through the SuNLaMP program. We wish to acknowledge Prof. David Cahill and Dr. Judith Kimling from the Materials Science and Engineering Department at the University of Illinois Urbana-Champaign for performing the thermal conductivity measurements. Electron microscopy was performed at the Electron Microscopy Center for Materials Research (EMCMR) at Argonne National Laboratory. Use of the EMCMR was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357 operated by UChicago Argonne, LLC. NR 46 TC 1 Z9 1 U1 8 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 14 PY 2016 VL 120 IS 27 BP 14681 EP 14689 DI 10.1021/acs.jpcc.6b03823 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DR6CT UT WOS:000379990400024 ER PT J AU Bradley, L Larsen, G Zhao, YP AF Bradley, Layne Larsen, George Zhao, Yiping TI Designed to Fail: Flexible, Anisotropic Silver Nanorod Sheets for Low-Cost Wireless Activity Monitoring SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID GLANCING ANGLE DEPOSITION; 25TH ANNIVERSARY ARTICLE; TRANSPARENT ELECTRODES; NANOTROUGH NETWORKS; SENSORS; FABRICATION; FILMS; SKIN AB We describe the fabrication and properties of flexible, anisotropic silver nanorod sheets and investigate their potential to function as a sensor. Aligned and tilted silver nanorod (AgNR) arrays are incorporated into polydimethylsiloxane (PDMS) to form flexible conductive sheets. The electrical properties of these sheets are investigated and show large anisotropies, which are related to the alignment direction of the nanorods. Notably, the films show the greatest electrical resistance in the direction perpendicular to the nanorod alignment, and when strain is applied along this direction, the resistance increases monotonically with increasing loading/unloading cycles. In comparison, the resistance along the nanorod alignment direction remains constant over many strain cycles and therefore can serve as an internal reference or as a stable strain gauge. These changes in resistivity are attributed to changes in the internanorod connectivity and can be modeled using an effective medium approximation for anisotropic percolation. Stable piezoresistivity (in one orientation) and surface-enhanced Raman scattering activity of the AgNR sheets make them attractive for flexible electronics applications such as electronic skin or as monitors for human machine interactions. however, the ability to encode a surface's dynamic history into material properties through resistance changes is a considerable simplification over other systems and can enable-wireless activity monitoring where cost or demanding environments prevent more complicated devices from being implemented. C1 [Bradley, Layne; Zhao, Yiping] Univ Georgia, Dept Phys & Astron, Athens, GA 30601 USA. [Larsen, George] Savannah River Natl Lab, Natl Secur Directorate, Aiken, SC 29808 USA. RP Zhao, YP (reprint author), Univ Georgia, Dept Phys & Astron, Athens, GA 30601 USA. EM zhaoy@physast.uga.edu FU National Science Foundation [CBET-1064228] FX This work was supported in part by the National Science Foundation (CBET-1064228). NR 27 TC 0 Z9 0 U1 6 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 14 PY 2016 VL 120 IS 27 BP 14969 EP 14976 DI 10.1021/acs.jpcc.6b04792 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DR6CT UT WOS:000379990400056 ER PT J AU Foster, ME Sohlberg, K Spataru, CD Allendorf, MD AF Foster, Michael E. Sohlberg, Karl Spataru, Catalin D. Allendorf, Mark D. TI Proposed Modification of the Graphene Analogue Ni-3(HITP)(2) To Yield a Semiconducting Material SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID METAL-ORGANIC FRAMEWORK; ELECTRICAL-CONDUCTIVITY; 2-DIMENSIONAL MATERIALS; THIN-FILMS; BAND-GAPS AB The metal organic framework material Ni-3(2,3,6,7,10,11-hexaiminotriphenylene)(2) (Ni-3(HITP)(2)) is composed of layers of extended conjugated planes analogous to graphene. We carried out density functional theory (DFT) calculations to model the electronic structure of monolayer, bilayer, and bulk Ni-3(HITP)(2). These materials have intriguing electronic properties; for example, appreciable band dispersion is predicted not only in plane but also perpendicular to the stacking planes. This suggests that, unlike graphene, the material may have appreciable conductivity in all crystallographic directions. Moreover, the bulk and bilayer structures are predicted to be metallic; in contrast, a 2D monolayer of the material exhibits a band gap. Insight obtained from studies of the transition of the material from semiconducting to metallic as the dimensionality increases from 2D to 3D suggests the possibility of producing a 3D semiconducting material by inserting spacer moieties between the layers. Our calculations suggest that it is not energetically favorable for Ni-3(HITP)(2) to accept a spacer linker (i.e., pyridine); however, changing the coordinating metal to Cr makes spacer insertion energetically favorable. The proposed 3D material is predicted to possess a band gap of similar to 1 eV with electron/hole effective masses similar to that of silicon. C1 [Foster, Michael E.; Spataru, Catalin D.; Allendorf, Mark D.] Sandia Natl Labs, Livermore, CA 94551 USA. [Sohlberg, Karl] Drexel Univ, Dept Chem, Philadelphia, PA 19104 USA. RP Foster, ME (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM mefoste@sandia.gov FU U.S. Department of Energy Office of Energy Efficiency and Renewable Energy SunShot Program [DE-EE0000990-1634]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the U.S. Department of Energy Office of Energy Efficiency and Renewable Energy SunShot Program under Award DE-EE0000990-1634. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 42 TC 0 Z9 0 U1 34 U2 48 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 14 PY 2016 VL 120 IS 27 BP 15001 EP 15008 DI 10.1021/acs.jpcc.6b05746 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DR6CT UT WOS:000379990400060 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Konig, A Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rad, N Rahbaran, B Rohringer, H Schieck, J Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S De Wolf, EA Janssen, X Knutsson, A Lauwers, J Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Lowette, S Moortgat, S Moreels, L Olbrechts, A Python, Q Tavernier, S Van Doninck, W Van Mulders, P Van Parijs, I Brun, H Caillol, C Clerbaux, B De Lentdecker, G Delannoy, H Fasanella, G Favart, L Goldouzian, R Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Luetic, J Maerschalk, T Marinov, A Randle-conde, A Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Cimmino, A Cornelis, T Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Poyraz, D Salva, S Schofbeck, R Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L De Visscher, S Delaere, C Delcourt, M Forthomme, L Francois, B Giammanco, A Jafari, A Jez, P Komm, M Lemaitre, V Magitteri, A Mertens, A Musich, M Nuttens, C Piotrzkowski, K Quertenmont, L Selvaggi, M Marono, MV Wertz, S Beliy, N Alda, WL Alves, FL Alves, GA Brito, L Martins, MC Hensel, C Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Da Silveira, GG Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Herrera, CM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Fang, W Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Chen, Y Cheng, T Du, R Jiang, CH Leggat, D Liu, Z Romeo, F Shaheen, SM Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Zhao, J Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Hernandez, CFG Alvarez, JDR Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Ferencek, D Kadija, K Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Finger, M Finger, M Jarrin, EC Elgammal, S Mohamed, A Mohammed, Y Salama, E Calpas, B Kadastik, M Murumaa, M Perrini, L Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Peltola, T Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Ghosh, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Kucher, I Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Abdulsalam, A Antropov, I Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Davignon, O de Cassagnac, RG Jo, M Lisniak, S Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Pigard, P Regnard, S Salerno, R Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gele, D Goerlach, U Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Bernet, C 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Beernaert, K Behnke, O Behrens, U Bin Anuar, AA Borras, K Campbell, A Connor, P Contreras-Campana, C Costanza, F Pardos, CD Dolinska, G Eckerlin, G Eckstein, D Eichhorn, T Gallo, E Garcia, JG Geiser, A Gizhko, A Luyando, JMG Gunnellini, P Harb, A Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Keaveney, J Kieseler, J Kleinwort, C Korol, I Lange, W Lelek, A Leonard, J Lipka, K Lobanov, A Lohmann, W Mankel, R Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Ntomari, E Pitzl, D Placakyte, R Raspereza, A Roland, B Sahin, MO Saxena, P Schoerner-Sadenius, T Seitz, C Spannagel, S Stefaniuk, N Trippkewitz, KD Van Onsem, GP Walsh, R Wissing, C Blobel, V Vignali, MC Draeger, AR Dreyer, T Erfle, J Garutti, E Goebel, K Gonzalez, D Gorner, M Haller, J Hoffmann, M Hoing, RS Junkes, A Klanner, R Kogler, R Kovalchuk, N Lapsien, T Lenz, T Marchesini, I Marconi, D Meyer, M Niedziela, M Nowatschin, D Ott, J Pantaleo, F Peiffer, T Perieanu, A Pietsch, N Poehlsen, J Sander, C Scharf, C Schleper, P Schlieckau, E Schmidt, A Schumann, S Schwandt, J Stadie, H Steinbruck, G Stober, FM Stover, M Tholen, H Troendle, D Usai, E Vanelderen, L Vanhoefer, A Vormwald, B Barth, C Baus, C Berger, J Butz, E Chwalek, T Colombo, F De Boer, W Dierlamm, A Fink, S Friese, R Giffels, M Gilbert, A Haitz, D Hartmann, F Heindl, SM Husemann, U Katkov, I Kornmayer, A Pardo, PL Maier, B Mildner, H Mozer, MU Muller, T Muller, T Plagge, M Quast, G Rabbertz, K Rocker, S Roscher, F Schroder, M Sieber, G Simonis, HJ Ulrich, R Wagner-Kuhr, J Wayand, S Weber, M Weiler, T Williamson, S Wohrmann, C Wolf, R Anagnostou, G Daskalakis, G Geralis, T Giakoumopoulou, VA Kyriakis, A Loukas, D Topsis-Giotis, I Agapitos, A Kesisoglou, S Panagiotou, A Saoulidou, N Tziaferi, E Evangelou, I Flouris, G Foudas, C Kokkas, P Loukas, N Manthos, N Papadopoulos, I Paradas, E Filipovic, N Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Karancsi, J Molnar, J Szillasi, Z Bartok, M Makovec, A Raics, P Trocsanyi, ZL Ujvari, B Bahinipati, S Choudhury, S Mal, P Mandal, K Nayak, A Sahoo, DK Sahoo, N Swain, SK Bansal, S Beri, SB Bhatnagar, V Chawla, R Gupta, R Bhawandeep, U Kalsi, AK Kaur, A Kaur, M Kumar, R Mehta, A Mittal, M Singh, JB Walia, G Kumar, A Bhardwaj, A Choudhary, BC Garg, RB Keshri, S Kumar, A Malhotra, S Naimuddin, M Nishu, N Ranjan, K Sharma, R Sharma, V Bhattacharya, R Bhattacharya, S Chatterjee, K Dey, S Dutt, S Dutta, S Ghosh, S Majumdar, N Modak, A Mondal, K Mukhopadhyay, S Nandan, S Purohit, A Roy, A Roy, D Chowdhury, SR Sarkar, S Sharan, M Thakur, S Behera, PK Chudasama, R Dutta, D Jha, V Kumar, V Mohanty, AK Netrakanti, PK Pant, LM Shukla, P Topkar, A Aziz, T Dugad, S Kole, G Mahakud, B Mitra, S Mohanty, GB Sur, N Sutar, B Banerjee, S Bhowmik, S Dewanjee, RK Ganguly, S Guchait, M Jain, S Kumar, S Maity, M Majumder, G Mazumdar, K Parida, B Sarkar, T Wickramage, N Chauhan, S Dube, S Kapoor, A Kothekar, K 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CA CMS Collaboration TI Search for Narrow Resonances in Dijet Final States at root s=8 TeV with the Novel CMS Technique of Data Scouting SO PHYSICAL REVIEW LETTERS LA English DT Article ID P(P)OVER-BAR COLLISIONS; MASS-DISTRIBUTION; HADRON COLLIDERS; SPECTRUM; BOSONS; QUARK AB A search for narrow resonances decaying into dijet final states is performed on data from proton-proton collisions at a center-of-mass energy of 8 TeV, corresponding to an integrated luminosity of 18.8 fb(-1). The data were collected with the CMS detector using a novel technique called data scouting, in which the information associated with these selected events is much reduced, permitting collection of larger data samples. This technique enables CMS to record events containing jets at a rate of 1 kHz, by collecting the data from the high-level-trigger system. In this way, the sensitivity to low-mass resonances is increased significantly, allowing previously inaccessible couplings of new resonances to quarks and gluons to be probed. The resulting dijet mass distribution yields no evidence of narrow resonances. Upper limits are presented on the resonance cross sections as a function of mass, and compared with a variety of models predicting narrow resonances. The limits are translated into upper limits on the coupling of a leptophobic resonance Z'(B) to quarks, improving on the results obtained by previous experiments for the mass range from 500 to 800 GeV. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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K.] Indian Inst Technol, Madras, Tamil Nadu, India. [Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Netrakanti, P. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay, Maharashtra, India. [Aziz, T.; Dugad, S.; Kole, G.; Mahakud, B.; Mitra, S.; Mohanty, G. B.; Sur, N.; Sutar, B.] Tata Inst Fundamental Res A, Bombay, Maharashtra, India. [Banerjee, S.; Bhowmik, S.; Dewanjee, R. K.; Ganguly, S.; Guchait, M.; Jain, Sa.; Kumar, S.; Maity, M.; Majumder, G.; Mazumdar, K.; Parida, B.; Sarkar, T.; Wickramage, N.] Tata Inst Fundamental Res B, Bombay, Maharashtra, India. [Chauhan, S.; Dube, S.; Kapoor, A.; Kothekar, K.; Rane, A.; Sharma, S.] IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Chenarani, S.; Tadavani, E. Eskandari; Etesami, S. M.; Fahim, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvagg, G.; Silvestris, L.; Venditti, R.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy. [Calabria, C.; Caputo, C.; Creanza, D.; Cristella, L.; De Palma, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvagg, G.; Venditti, R.] Univ Bari, Bari, Italy. [De Filippis, N.; Iaselli, G.; Maggi, G.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Battilana, C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.] Univ Bologna, Bologna, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Di Mattia, A.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Pigazzini, S.; Ragazzi, S.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; De Nardo, G.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.; Thyssen, F.] Ist Nazl Fis Nucl, Sez Napoli, Rome, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Napoli Federico II, Rome, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, Rome, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Checchia, P.; Dall'Osso, M.; Manzano, P. De Castro; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Trento, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Trento, Italy. Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Magnani, A.; Montagna, P.; Ratti, S. P.; Riccardi, C.; Vai, I.; Vitulo, P.] Univ Pavia, Pavia, Italy. [Solestizi, L. Alunni; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Leonardi, R.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] Ist Nazl Fis Nucl, Sez Perugia, Perugia, Italy. [Solestizi, L. Alunni; Ciangottini, D.; Fano, L.; Lariccia, P.; Leonardi, R.; Mantovani, G.; Santocchia, A.] Univ Perugia, Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Fedi, G.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Cipriani, M.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; Cipriani, M.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.] Univ Roma, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bartosik, N.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Shchelina, K.; Sola, V.; Solano, A.; Staiano, A.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Torino, Novara, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Shchelina, K.; Solano, A.; Traczyk, P.] Univ Turin, Novara, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; La Licata, C.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Lee, S.; Lee, S. W.; Oh, Y. D.; Sekmen, S.; Son, D. C.; Yang, Y. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, H.; Lee, A.] Chonbuk Natl Univ, Jeonju, South Korea. [Cifuentes, J. A. Brochero; Kim, T. J.] Hanyang Univ, Seoul, South Korea. [Cho, S.; Choi, S.; Go, Y.; Gyun, D.; Ha, S.; Hong, B.; Jo, Y.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Lim, J.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Almond, J.; Kim, J.; Oh, S. B.; Seo, S. H.; Yang, U. K.; Yoo, H. D.; Yu, G. B.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Yusli, M. N.; Zolkapli, Z.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Mejia Guisao, J.; Sanchez-Hernandez, A.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.; Uribe Estrada, C.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Toms, M.; Vlasov, E.; Zhokin, A.] Univ Auckland, Auckland, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Qazi, S.; Shoaib, M.; Waqas, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.; Bargassa, P.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Hollar, J.; Leonardo, N.; Lloret Iglesias, L.; Nemallapudi, M. V.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Finger, M.; Finger, M., Jr.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbounov, N.; Gorbunov, I.; Karjavin, V.; Kozlov, G.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Savina, M.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Chtchipounov, L.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Murzin, V.; Oreshkin, V.; Sulimov, V.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Matveev, V.; Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Musienko, Y.] Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Toms, M.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Matveev, V.; Chadeeva, M.; Danilov, M.; Zhemchugov, E.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Rusakov, S. V.; Terkulov, A.] PN Lebedev Phys Inst, Moscow, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Miagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Elumakhov, D.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.; Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. [de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Sanchez Cruz, S.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; Curras, E.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Martinez Rivero, C.; Matorras, F.; Piedra Gomez, J.; Rodrigo, T.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, Santander, Spain. [Merlin, J. A.; Stahl, A.; Pantaleo, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Tosi, N.; Viliani, L.; Primavera, F.; Manzoni, R. A.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Pazzini, J.; Azzurri, P.; D'imperio, G.; Del Re, D.; Arcidiacono, R.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Camporesi, T.; Castello, R.; Cepeda, M.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duggan, D.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Fartoukh, S.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Girone, M.; Glege, F.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Knuenz, V.; Kortelainen, M. J.; Kousouris, K.; Krammer, M.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Sauvan, J. B.; Schaefer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veckalns, V.; Veres, G. I.; Wardle, N.; Zagozdzinska, A.; Zeuner, W. D.; Virdee, T.] European Org Nucl Res, CERN, Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marionneau, M.; Del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meinhard, M. T.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrin, G.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Schoenenberger, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Rauco, G.; Robmann, P.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Pozdnyakov, A.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Kumar, Arun; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Paganis, E.; Psallidas, A.; Tsai, J. F.; Tzeng, Y. M.] NTU, Taipei, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Damarseckin, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Onengut, G.; Ozdemir, K.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle East Tech Univ, Dept Phys, Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Burns, D.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Lucas, R.] Rutherford Appleton Lab, Didcot, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Futyan, D.; Haddad, Y.; Hall, G.; Iles, G.; Lane, R.; Laner, C.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mastrolorenzo, L.; Nash, J.; Nikitenko, A.; Pela, J.; Penning, B.; Pesaresi, M.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Imperial Coll, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Gastler, D.; Rankin, D.; Richardson, C.; Rohlf, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Benelli, G.; Berry, E.; Cutts, D.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Jesus, O.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Spencer, E.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Burns, D.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Flores, C.; Funk, G.; Gardner, M.; Ko, W.; Lander, R.; Mclean, C.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.; Cousins, R.] Univ Calif Davis, Davis, CA 95616 USA. [Everaerts, P.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Malberti, M.; Negrete, M. Olmedo; Paneva, M. I.; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Gerosa, R.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wood, J.; Wurthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bhandari, R.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Heller, R.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Ovcharova, A.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bendavid, J.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chaves, J.; Chu, J.; Dittmer, S.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Sun, W.; Tan, S. M.; Tao, Z.; Thom, J.; Tucker, J.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.; Abdullin, S.] Fairfield Univ, Fairfield, CT 06430 USA. [Albrow, M.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Cremonesi, M.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Ristori, L.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Stoynev, S.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Wang, M.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Kuznetsova, E.; Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Brinkerhoff, A.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Konigsberg, J.; Korytov, A.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Shchutska, L.; Sperka, D.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Diamond, B.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Santra, A.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.; Zhang, J.] UIC, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Blumenfeld, B.; Cocoros, A.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Osherson, M.; Roskes, J.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Al-bataineh, A.; Baringer, P.; Bean, A.; Bowen, J.; Bruner, C.; Castle, J.; Kenny, R. P., III; Kropivnitskaya, A.; Majumder, D.; Mcbrayer, W.; Murray, M.; Sanders, S.; Stringer, R.; Takaki, J. D. Tapia; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.; Apyan, A.; Barbieri, R.] Univ Maryland, College Pk, MD 20742 USA. [Baty, A.; Bi, R.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Hsu, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Krajczar, K.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Tatar, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Benvenuti, A. C.; Chatterjee, R. M.; Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bartek, R.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Siado, J. E.; Snow, G. R.; Stieger, B.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Parker, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wood, D.] Northeastern Univ, Boston, MA 02115 USA. [Bhattacharya, S.; Hahn, K. A.; Kubik, A.; Low, J. F.; Mucia, N.; Odell, N.; Pollack, B.; Schmitt, M. H.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Dev, N.; Hildreth, M.; Anampa, K. Hurtado; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Planer, M.; Reinsvold, A.; Ruchti, R.; Rupprecht, N.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Alimena, J.; Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Francis, B.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Luo, J.; Marlow, D.; Mooney, M.; Olsen, J.; Palmer, C.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barker, A.; Barnes, V. E.; Benedetti, D.; Folgueras, S.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, A. W.; Jung, K.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Duh, Y. T.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Hindrichs, O.; Khukhunaishvili, A.; Lo, K. H.; Tan, P.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Chou, J. P.; Contreras-Campana, E.; Gershtein, Y.; Espinosa, T. A. Gomez; Halkiadakis, E.; Heindl, M.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Kyriacou, S.; Lath, A.; Nash, K.; Saka, H.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Heideman, J.; Riley, G.; Rose, K.; Spanier, S.; Thapa, K.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Celik, A.; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Huang, T.; Juska, E.; Kamon, T.; Krutelyov, V.; Mueller, R.; Pakhotin, Y.; Patel, R.; Perloff, A.; Pernie, L.; Rathjens, D.; Rose, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Avetisyan, A.; Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.; Wang, Z.] Texas Tech Univ, Lubbock, TX 79409 USA. [Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Melo, A.; Ni, H.; Sheldon, P.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Barria, P.; Cox, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Neu, C.; Sinthuprasith, T.; Sun, X.; Wang, Y.; Wolfe, E.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Lamichhane, P.; Sturdy, J.; Belknap, D. A.] Wayne State Univ, Detroit, MI USA. [Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Grothe, M.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Verwilligen, P.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Jeitler, M.; Schieck, J.] Vienna Univ Technol, Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Elgammal, S.; Salama, E.] British Univ Egypt, Cairo, Egypt. [Mohamed, A.] Zewail City Sci & Technol, Zewail, Egypt. [Mohammed, Y.] Fayoum Univ, Al Fayyum, Egypt. [Salama, E.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Lohmann, W.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Choudhury, S.] Indian Inst Sci Educ & Res, Bhopal, India. [Nayak, A.] Inst Phys, Bhubaneswar, Orissa, India. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Chenarani, S.; Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.] Univ Siena, Siena, Italy. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] Agensi Nuklear Malaysia, MOSTI, Kajang, Malaysia. [Heredia-De La Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Adzic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Di Marco, E.] Univ Roma, Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. [Veckalns, V.] Riga Tech Univ, Riga, Latvia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Damarseckin, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, E. A.] Istanbul Bilgi Univ, Istanbul, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Colafranceschi, S.] Univ Roma, Fac Ingn, Rome, Italy. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Bouhali, O.; Hernandez, A. Castaneda] Texas A&M Univ, Doha, Qatar. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan, Armenia. RI Smirnov, Vitaly/B-5001-2017; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; Puljak, Ivica/D-8917-2017; Goh, Junghwan/Q-3720-2016; Varela, Joao/K-4829-2016; TUVE', Cristina/P-3933-2015; Chadeeva, Marina/C-8789-2016; Danilov, Mikhail/C-5380-2014; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Andreev, Vladimir/M-8665-2015; Leonardo, Nuno/M-6940-2016; Dudko, Lev/D-7127-2012; Zhemchugov, Evgeny/C-8885-2016; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Sznajder, Andre/L-1621-2016; Della Ricca, Giuseppe/B-6826-2013; Lokhtin, Igor/D-7004-2012; Da Silveira, Gustavo Gil/N-7279-2014; Stahl, Achim/E-8846-2011; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Manganote, Edmilson/K-8251-2013; Colafranceschi, Stefano/M-1807-2016; VARDARLI, Fuat Ilkehan/B-6360-2013 OI Ogul, Hasan/0000-0002-5121-2893; Goh, Junghwan/0000-0002-1129-2083; Varela, Joao/0000-0003-2613-3146; Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; Ptochos, Fotios/0000-0002-3432-3452; Hurtado Anampa, Kenyi/0000-0002-9779-3566; TUVE', Cristina/0000-0003-0739-3153; Chadeeva, Marina/0000-0003-1814-1218; Danilov, Mikhail/0000-0001-9227-5164; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Leonardo, Nuno/0000-0002-9746-4594; Dudko, Lev/0000-0002-4462-3192; Zhemchugov, Evgeny/0000-0002-0914-9739; Yazgan, Efe/0000-0001-5732-7950; Sznajder, Andre/0000-0001-6998-1108; Della Ricca, Giuseppe/0000-0003-2831-6982; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Stahl, Achim/0000-0002-8369-7506; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); BUAP (Mexico); CINVESTAV (Mexico); CONACYT (Mexico); LNS (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA) FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); BUAP, CINVESTAV, CONACYT, LNS, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA). NR 46 TC 5 Z9 5 U1 59 U2 103 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 14 PY 2016 VL 117 IS 3 AR 031802 DI 10.1103/PhysRevLett.117.031802 PG 17 WC Physics, Multidisciplinary SC Physics GA DR1IP UT WOS:000379659500002 ER PT J AU Doud, DFR Angenent, LT AF Doud, Devin F. R. Angenent, Largus T. TI Single-Genotype Syntrophy by Rhodopseudomonas palustris Is Not a Strategy to Aid Redox Balance during Anaerobic Degradation of Lignin Monomers SO FRONTIERS IN MICROBIOLOGY LA English DT Article DE single-genotype syntrophy; Rhodopseudomonas palustris; microbial electrochemistry; lignin degradation; redox balance ID P-COUMARATE DEGRADATION; GEOBACTER-SULFURREDUCENS; AROMATIC-COMPOUNDS; ELECTROCHEMICAL ACTIVITY; BIODEGRADATION; IDENTIFICATION; BENZOATE; BACTERIA AB Rhodopseudomonas palustris has emerged as a model microbe for the anaerobic metabolism of p-coumarate, which is an aromatic compound and a primary component of lignin. However, under anaerobic conditions, R. palustris must actively eliminate excess reducing equivalents through a number of known strategies (e.g., CO2 fixation, H-2 evolution) to avoid lethal redox imbalance. Others had hypothesized that to ease the burden of this redox imbalance, a clonal population of R. palustris could functionally differentiate into a pseudo-consortium. Within this pseudo-consortium, one sub-population would perform the aromatic moiety degradation into acetate, while the other sub-population would oxidize acetate, resulting in a single-genotype syntrophy through acetate sharing. Here, the objective was to test this hypothesis by utilizing microbial electrochemistry as a research tool with the extracellular-electron-transferring bacterium Geobacter sulfurreducens as a reporter strain replacing the hypothesized acetate-oxidizing sub-population. We used a 2 x 4 experimental design with pure cultures of R. palustris in serum bottles and co-cultures of R. palustris and G. sulfurreducens in bioelectrochemical systems. This experimental design included growth medium with and without bicarbonate to induce non-lethal and lethal redox imbalance conditions, respectively, in R. palustris. Finally, the design also included a mutant strain (NifA*) of R. palustris, which constitutively produces H-2, to serve both as a positive control for metabolite secretion (H-2) to G. sulfurreducens, and as a non-lethal redox control for without bicarbonate conditions. Our results demonstrate that acetate sharing between different sub-populations of R. palustris does not occur while degrading p-coumarate under either non-lethal or lethal redox imbalance conditions. This work highlights the strength of microbial electrochemistry as a tool for studying microbial syntrophy. C1 [Doud, Devin F. R.; Angenent, Largus T.] Cornell Univ, Dept Biol & Environm Engn, Ithaca, NY 14850 USA. [Doud, Devin F. R.] DOE Joint Genome Inst, Walnut Creek, CA USA. RP Angenent, LT (reprint author), Cornell Univ, Dept Biol & Environm Engn, Ithaca, NY 14850 USA. EM la249@cornell.edu FU US DOE Advanced Research Projects Agency - Energy (ARPA-E) [DE-AR0000312] FX We would like to thank Dr. Hanno Richter for helpful discussions and Bahareh Guilvaiee and Prof. Tammo Steenhuis (Cornell University) for use of their digital microscope. This project was funded in part: by the US DOE Advanced Research Projects Agency - Energy (ARPA-E) with project: number DE-AR0000312. NR 25 TC 0 Z9 0 U1 12 U2 15 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-302X J9 FRONT MICROBIOL JI Front. Microbiol. PD JUL 14 PY 2016 VL 7 AR 1082 DI 10.3389/fmicb.2016.01082 PG 10 WC Microbiology SC Microbiology GA DR1CK UT WOS:000379643400001 PM 27471497 ER PT J AU Moll, PJW Nair, NL Helm, T Potter, AC Kimchi, I Vishwanath, A Analytis, JG AF Moll, Philip J. W. Nair, Nityan L. Helm, Toni Potter, Andrew C. Kimchi, Itamar Vishwanath, Ashvin Analytis, James G. TI Transport evidence for Fermi-arc-mediated chirality transfer in the Dirac semimetal Cd3As2 SO NATURE LA English DT Article ID TOPOLOGICAL INSULATOR; SURFACE-STATE; GRAPHENE; MOBILITY; WEYL; OSCILLATIONS; CRYSTAL; WIRES AB The dispersion of charge carriers in a metal is distinctly different from that of free electrons owing to their interactions with the crystal lattice. These interactions may lead to quasiparticles mimicking the massless relativistic dynamics of high-energy particle physics(1-3), and they can twist the quantum phase of electrons into topologically non-trivial knots-producing protected surface states with anomalous electromagnetic properties(4-9). These effects intertwine in materials known as Weyl semimetals, and in their crystal-symmetry-protected analogues, Dirac semimetals(10). The latter show a linear electronic dispersion in three dimensions described by two copies of the Weyl equation (a theoretical description of massless relativistic fermions). At the surface of a crystal, the broken translational symmetry creates topological surface states, so-called Fermi arcs(11), which have no counterparts in high-energy physics or conventional condensed matter systems. Here we present Shubnikov-de Haas oscillations in focused-ion-beam-prepared microstructures of Cd3As2 that are consistent with the theoretically predicted 'Weyl orbits', a kind of cyclotron motion that weaves together Fermi-arc and chiral bulk states(12). In contrast to conventional cyclotron orbits, this motion is driven by the transfer of chirality from one Weyl node to another, rather than momentum transfer of the Lorentz force. Our observations provide evidence for direct access to the topological properties of charge in a transport experiment, a first step towards their potential application. C1 [Moll, Philip J. W.; Nair, Nityan L.; Helm, Toni; Potter, Andrew C.; Kimchi, Itamar; Vishwanath, Ashvin; Analytis, James G.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Moll, Philip J. W.; Nair, Nityan L.] Max Planck Inst Chem Phys Solids, Noethnitzer Str 40, D-01187 Dresden, Germany. [Analytis, James G.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Moll, PJW; Analytis, JG (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Moll, PJW (reprint author), Max Planck Inst Chem Phys Solids, Noethnitzer Str 40, D-01187 Dresden, Germany. EM philip.moll@cpfs.mpg.de; analytis@berkeley.edu FU SCOPE-M centre for electron microscopy at ETH Zurich; Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF4307, GBMF4374]; Office of Science, Office of Basic Energy Sciences, Materials Sciences Division, of the US Department of Energy [DE-AC02-05CH11231]; University of California, Berkeley; Quantum Materials FWP, US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02- 05CH11231]; Office of Science, Office of Basic Energy Sciences, of the US Department of Energy [DE-AC02-05CH11231] FX The FIB work was supported by the SCOPE-M centre for electron microscopy at ETH Zurich. We thank P Gasser, J. Reuteler and B. Batlogg for FIB support, and M. Bachmann for performing magnetoresistance measurements. A.C.P. was supported by the Gordon and Betty Moore Foundation's EPiQS Initiative through grant GBMF4307. We also thank S. Teat and K. Gagnon for their help in conducting X-ray diffraction measurements at the Advanced Light Source (ALS) beam line 11.3.1, and N. Tamura for micro-diffraction on beam line 12.3.2. N.T. and the ALS are supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences Division, of the US Department of Energy under contract no. DE-AC02-05CH11231 at Lawrence Berkeley National Laboratory and the University of California, Berkeley. Transport experiments, material synthesis and FIB microstructuring were supported by the Gordon and Betty Moore Foundation's EPiQS Initiative through grant GBMF4374. Single-crystal X-ray refinements (T.H.) and theoretical support (A.V. and I.K.) were funded by the Quantum Materials FWP, US Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under contract no. DE-AC02- 05CH11231. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the US Department of Energy under contract no. DE-AC02-05CH11231. NR 43 TC 14 Z9 14 U1 51 U2 82 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JUL 14 PY 2016 VL 535 IS 7611 BP 266 EP + DI 10.1038/nature18276 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR4ZN UT WOS:000379912600053 PM 27376477 ER PT J AU Hartl, M Gillis, RC Daemen, L Olds, DP Page, K Carlson, S Cheng, YQ Hugle, T Iverson, EB Ramirez-Cuesta, AJ Lee, Y Muhrer, G AF Hartl, Monika Gillis, Robert Chad Daemen, Luke Olds, Daniel P. Page, Katherine Carlson, Stefan Cheng, Yongqiang Hugle, Thomas Iverson, Erik B. Ramirez-Cuesta, A. J. Lee, Yongjoong Muhrer, Gunter TI Hydrogen adsorption on two catalysts for the ortho- to parahydrogen conversion: Cr-doped silica and ferric oxide gel SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID SPALLATION NEUTRON SOURCES; PARA H2 CONVERSION; LIQUID-HYDROGEN; SURFACE CATALYSIS; CARBON NANOTUBES; SOLID HYDROGEN; SPILLOVER; SCATTERING; STORAGE; SPECTROSCOPY AB Molecular hydrogen exists in two spin-rotation coupled states: parahydrogen and orthohydrogen. Due to the variation of energy with rotational level, the occupation of ortho- and parahydrogen states is temperature dependent, with parahydrogen being the dominant species at low temperatures. The equilibrium at 20 K (99.8% parahydrogen) can be reached by natural conversion only after a lengthy process. With the use of a suitable catalyst, this process can be shortened significantly. Two types of commercial catalysts currently being used for ortho-to parahydrogen conversion are: iron(III) oxide (Fe2O3, IONEX (R)), and chromium(II) oxide doped silica catalyst (CrO center dot SiO2, OXISORB (R)). We investigate the interaction of ortho-and parahydrogen with the surfaces of these ortho-para conversion catalysts using neutron vibrational spectroscopy. The catalytic surfaces have been characterized using X-ray absorption fine structure (XAFS) and X-ray/neutron pair distribution function measurements. C1 [Hartl, Monika; Lee, Yongjoong; Muhrer, Gunter] ESS, Tunavagen 24, S-22363 Lund, Sweden. [Gillis, Robert Chad; Daemen, Luke; Olds, Daniel P.; Page, Katherine; Cheng, Yongqiang; Hugle, Thomas; Iverson, Erik B.; Ramirez-Cuesta, A. J.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Carlson, Stefan] Lund Univ, Max Lab 4, POB 118, S-22100 Lund, Sweden. RP Hartl, M (reprint author), ESS, Tunavagen 24, S-22363 Lund, Sweden. EM monika.hartl@esss.se RI Page, Katharine/C-9726-2009; Hartl, Monika/N-4586-2016; OI Page, Katharine/0000-0002-9071-3383; Hartl, Monika/0000-0002-6601-7273; Huegle, Thomas/0000-0002-7762-1302; Iverson, Erik /0000-0002-7920-705X; Ramirez-Cuesta, Anibal /0000-0003-1231-0068; Olds, Daniel/0000-0002-4611-4113 FU Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC0500OR22725]; UT Battelle, LLC; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; U.S. DOE [DE-AC02-06CH11357]; Swedish Research Council; Knut och Alice Wallenbergs Stiftelse FX M. H. is grateful to P. Karlsson at Bodo Moeller Chemie Sweden for supplying a sample of their IONEX (R) Type O-P catalyst. BET measurements were performed by B. Linden at the Department of Chemical Engineering, Lund University. This research benefited from the use of the VISION and NOMAD beamlines at ORNL's Spallation Neutron Source, which is supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy under Contract No. DE-AC0500OR22725 with UT Battelle, LLC. Work performed at Argonne and use of the Advanced Photon Source were supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. We gratefully acknowledge Hsiu-Wen Wang and Ying Shi for the use of reference silica PDF data. This work was also supported by the use of the Advanced Photon Source at the Argonne National Laboratory supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. Portions of this research were carried out at beamline I811, MAX-lab synchrotron radiation source, Lund University, Sweden. Funding for the beamline I811 project was kindly provided by The Swedish Research Council and The Knut och Alice Wallenbergs Stiftelse. NR 59 TC 0 Z9 0 U1 4 U2 13 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD JUL 14 PY 2016 VL 18 IS 26 BP 17281 EP 17293 DI 10.1039/c6cp01154c PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DQ8ST UT WOS:000379482100018 PM 27149564 ER PT J AU Wan, LWF Wright, J Perdue, BR Fister, TT Kim, S Apblett, CA Prendergast, D AF Wan, Liwen F. Wright, Joshua Perdue, Brian R. Fister, Timothy T. Kim, Soojeong Apblett, Christopher A. Prendergast, David TI Revealing electronic structure changes in Chevrel phase cathodes upon Mg insertion using X-ray absorption spectroscopy SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID BATTERIES AB Following previous work predicting the electronic response of the Chevrel phase Mo6S8 upon Mg insertion (Thole et al., Phys. Chem. Chem. Phys., 2015, 17, 22548), we provide the experimental proof, evident in X-ray absorption spectroscopy, to illustrate the charge compensation mechanism of the Chevrel phase compound during Mg insertion and de-insertion processes. C1 [Wan, Liwen F.; Prendergast, David] Lawrence Berkeley Natl Lab, Mol Foundry, JCESR, Berkeley, CA 94720 USA. [Wright, Joshua] IIT, Chicago, IL 60616 USA. [Perdue, Brian R.; Apblett, Christopher A.] Sandia Natl Labs, JCESR, Albuquerque, NM 87123 USA. [Fister, Timothy T.; Kim, Soojeong] Argonne Natl Lab, JCESR, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Wan, LWF (reprint author), Lawrence Berkeley Natl Lab, Mol Foundry, JCESR, Berkeley, CA 94720 USA. EM LWan@lbl.gov RI ID, MRCAT/G-7586-2011 FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. DOE's NNSA [DE-AC04-94AL85000]; U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. Part of the computations were performed through a User Project at The Molecular Foundry (TMF) using the local cluster (Vulcan), managed by the High Performance Computing Services Group, at Lawrence Berkeley National Laboratory and others used the computing resources of the National Energy Research Scientific Computing (NERSC) center. Both TMF and NERSC are DOE User Facilities supported by the Office of Science of the U.S. Department of Energy under contract No. DE-AC02-05CH11231. The full cell experiments were performed at Sandia National Laboratory, which is a multiprogram laboratory managed and operated by Sandia Corp., a wholly owned subsidiary of Lockheed Martin Co., for the U.S. DOE's NNSA under Contract DE-AC04-94AL85000. The use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 8 TC 1 Z9 1 U1 9 U2 16 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD JUL 14 PY 2016 VL 18 IS 26 BP 17326 EP 17329 DI 10.1039/c6cp02412b PG 4 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DQ8ST UT WOS:000379482100023 PM 27314253 ER PT J AU Wen, H Hou, GL Liu, YR Wang, XB Huang, W AF Wen, Hui Hou, Gao-Lei Liu, Yi-Rong Wang, Xue-Bin Huang, Wei TI Examining the structural evolution of bicarbonate-water clusters: insights from photoelectron spectroscopy, basin-hopping structural search, and comparison with available IR spectral studies SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; MOLECULAR-DYNAMICS SIMULATIONS; DOUBLY-CHARGED ANION; SODIUM-BICARBONATE; GAS-PHASE; INFRARED PHOTODISSOCIATION; THERMOCHEMICAL PROPERTIES; CATALYTIC MECHANISM; EXCITATION-ENERGIES; CARBONIC-ANHYDRASE AB Bicarbonate plays a crucial biochemical role in the physiological pH buffering system and also has important atmospheric implications. In the current study, HCO3- (H2O)(n) (n = 0-13) clusters were successfully produced via electrospray ionization of the corresponding bulk salt solution, and were characterized by negative ion photoelectron spectroscopy and theoretical calculations. Photoelectron spectra reveal that the electron binding energy monotonically increases with the cluster size up to n = 10 and remains largely the same after n 4 > 10. The photo-detaching feature of the solute HCO3- itself, which dominates in the small clusters, diminishes with the increase of water coverage. Based on the charge distribution and molecular orbital analyses, the universal high electron binding energy tail that dominates in the larger clusters can be attributed to the ionization of water. Thus, the transition of ionization from the solute to the solvent at a size larger than n = 10 has been observed. Extensive theoretical structural search based on the basin-hopping unbiased method was carried out, and a plethora of low energy isomers have been obtained for each medium and large-sized cluster. By comparing the simulated photoelectron spectra and calculated electron binding energies with the experiments, as well as by comparing the simulated infrared spectra with previously reported IR spectra, the best fit structures and the structural evolutionary routes are presented. The nature of bicarbonate-water interactions is mainly electrostatic as implied by electron localization function (ELF) analysis. C1 [Wen, Hui; Liu, Yi-Rong; Huang, Wei] Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Lab Atmospher Physicochem, Hefei 230031, Anhui, Peoples R China. [Wen, Hui; Hou, Gao-Lei; Wang, Xue-Bin] Pacific NW Natl Lab, Div Phys Sci, POB 999,MS K8-88, Richland, WA 99352 USA. [Huang, Wei] Univ Sci & Technol China, Sch Environm Sci & Optoelect Technol, Hefei 230026, Anhui, Peoples R China. RP Huang, W (reprint author), Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Lab Atmospher Physicochem, Hefei 230031, Anhui, Peoples R China.; Wang, XB (reprint author), Pacific NW Natl Lab, Div Phys Sci, POB 999,MS K8-88, Richland, WA 99352 USA.; Huang, W (reprint author), Univ Sci & Technol China, Sch Environm Sci & Optoelect Technol, Hefei 230026, Anhui, Peoples R China. EM Xuebin.Wang@pnnl.gov; Huangwei6@ustc.edu.cn FU U. S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences; Division of Chemical Sciences, Geosciences, and Biosciences; DOE's Office of Biological and Environmental Research; National Natural Science Foundation of China [21403244, 21573241, 41527808]; State Key Program of National Natural Science of China [21133008]; National High Technology Research and Development Program of China (863 Program) [2014AA06A501]; "Interdisciplinary and Cooperative Team" of CAS FX The experimental work done at PNNL was supported by the U. S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences, the Division of Chemical Sciences, Geosciences, and Biosciences, and was performed using EMSL, a national scientific user facility sponsored by DOE's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory, which is operated by the Battelle Memorial Institute for the DOE. The theoretical work was supported by the National Natural Science Foundation of China (Grant No. 21403244, 21573241 and 41527808), the State Key Program of National Natural Science of China (Grant No. 21133008), the National High Technology Research and Development Program of China (863 Program No. 2014AA06A501) and the "Interdisciplinary and Cooperative Team" of CAS. Acknowledgement is also made to the "Thousand Youth Talents Plan". Part of the computation was performed by Cascade in EMSL, and part of the computation was performed at the Supercomputing Center of the CAS and Supercomputing Center of USTC. NR 49 TC 1 Z9 1 U1 15 U2 22 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD JUL 14 PY 2016 VL 18 IS 26 BP 17470 EP 17482 DI 10.1039/c6cp01542e PG 13 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DQ8ST UT WOS:000379482100042 PM 27302736 ER PT J AU Veinberg, SL Johnston, KE Jaroszewicz, MJ Kispal, BM Mireault, CR Kobayashi, T Pruski, M Schurko, RW AF Veinberg, Stanislav L. Johnston, Karen E. Jaroszewicz, Michael J. Kispal, Brianna M. Mireault, Christopher R. Kobayashi, Takeshi Pruski, Marek Schurko, Robert W. TI Natural abundance N-14 and N-15 solid-state NMR of pharmaceuticals and their polymorphs SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID DYNAMIC NUCLEAR-POLARIZATION; DENSITY-FUNCTIONAL THEORY; X-RAY-DIFFRACTION; MAGNETIC-RESONANCE-SPECTROSCOPY; 2 LOCAL-ANESTHETICS; 100 KHZ MAS; CHEMICAL-SHIFT; QUADRUPOLE RESONANCE; CROSS-POLARIZATION; CRYSTAL-STRUCTURES AB N-14 ultra-wideline (UW), H-1{N-15} indirectly-detected HETCOR (idHETCOR) and N-15 dynamic nuclear polarization (DNP) solid-state NMR (SSNMR) experiments, in combination with plane-wave density functional theory (DFT) calculations of N-14 EFG tensors, were utilized to characterize a series of nitrogen-containing active pharmaceutical ingredients (APIs), including HCl salts of scopolamine, alprenolol, isoprenaline, acebutolol, dibucaine, nicardipine, and ranitidine. A case study applying these methods for the differentiation of polymorphs of bupivacaine HCl is also presented. All experiments were conducted upon samples with naturally-abundant nitrogen isotopes. For most of the APIs, it was possible to acquire frequency-stepped UW N-14 SSNMR spectra of stationary samples, which display powder patterns corresponding to pseudo-tetrahedral (i.e., RR'R '' NH+ and RR'NH2+) or other (i.e., RNH2 and RNO2) nitrogen environments. Directly-excited N-14 NMR spectra were acquired using the WURST-CPMG pulse sequence, which incorporates WURST (wideband, uniform rate, and smooth truncation) pulses and a CPMG (Carr-Purcell Meiboom-Gill) refocusing protocol. In certain cases, spectra were acquired using H-1 -> N-14 broadband cross-polarization, via the BRAIN-CP (broadband adiabatic inversion-cross polarization) pulse sequence. These spectra provide N-14 electric field gradient (EFG) tensor parameters and orientations that are particularly sensitive to variations in local structure and intermolecular hydrogen-bonding interactions. The H-1{N-15} idHETCOR spectra, acquired under conditions of fast magic-angle spinning (MAS), used CP transfers to provide H-1-N-15 chemical shift correlations for all nitrogen environments, except for two sites in acebutolol and nicardipine. One of these two sites (RR'NH2+ in acebutolol) was successfully detected using the DNP-enhanced N-15{H-1} CP/MAS measurement, and one (RNO2 in nicardipine) remained elusive due to the absence of nearby protons. This exploratory study suggests that this combination of techniques has great potential for the characterization of solid APIs and numerous other organic, biological, and inorganic systems. C1 [Veinberg, Stanislav L.; Jaroszewicz, Michael J.; Kispal, Brianna M.; Mireault, Christopher R.; Schurko, Robert W.] Univ Windsor, Dept Chem & Biochem, Windsor, ON N9B 3P4, Canada. [Johnston, Karen E.] Univ Durham, Dept Chem, Durham DH1 3L3, England. [Kobayashi, Takeshi; Pruski, Marek] Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA. [Pruski, Marek] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Schurko, RW (reprint author), Univ Windsor, Dept Chem & Biochem, Windsor, ON N9B 3P4, Canada.; Pruski, M (reprint author), Iowa State Univ, US DOE, Ames Lab, Ames, IA 50011 USA.; Pruski, M (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA. EM mpruski@iastate.edu; rschurko@uwindsor.ca FU Natural Science and Engineering Research Council (NSERC, Canada) in the form of Discovery, Accelerator, and Research Tools and Instruments (RTI) grants; University of Windsor; Ontario for a Queen Elizabeth II - Graduate Scholarship in Science and Technology; Ontario Graduate Scholarship; Canadian Foundation for Innovation (CFI); Ontario Innovation Trust (OIT); U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences; DOE by Iowa State University [DE-AC02-07CH11358] FX R. W. S. acknowledges the Natural Science and Engineering Research Council (NSERC, Canada) for support in the form of Discovery, Accelerator, and Research Tools and Instruments (RTI) grants. He also acknowledges the University of Windsor for a 50th Golden Jubilee Research Award. S. L. V. thanks the province of Ontario for a Queen Elizabeth II - Graduate Scholarship in Science and Technology as well as an Ontario Graduate Scholarship. We are grateful to the Canadian Foundation for Innovation (CFI), the Ontario Innovation Trust (OIT), and the University of Windsor for supporting our NMR spectroscopy and X-ray facilities. Experiments at 21.1 T were conducted at the Canadian National Ultrahigh-Field NMR facility for Solids (www.nmr900.ca). Drs Victor Terskikh, Eric Ye, Luke O'Dell, Kris Harris, and Bryan Lucier are thanked for their assistance with all experiments at 21.1 T. In addition, Mr Jamie Bennett (NRC, Ottawa) is thanked for construction of the 7 mm double resonance probe used for all experiments at 21.1 T. Computational work described herein was made possible by the facilities of the Shared Hierarchical Academic Research Computing Network (SHARCNET: www.sharcnet.ca). At the Ames Laboratory, this research is supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences. Ames Laboratory is operated for the DOE by Iowa State University under Contract No. DE-AC02-07CH11358. The authors note that the contributions of S.L.V. and K.E.J. to this work are regarded as equal. NR 166 TC 3 Z9 3 U1 19 U2 35 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD JUL 14 PY 2016 VL 18 IS 26 BP 17713 EP 17730 DI 10.1039/c6cp02855a PG 18 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DQ8ST UT WOS:000379482100066 PM 27314503 ER PT J AU Durkin, M Mondragon-Shem, I Eley, S Hughes, TL Mason, N AF Durkin, Malcolm Mondragon-Shem, Ian Eley, Serena Hughes, Taylor L. Mason, Nadya TI History-dependent dissipative vortex dynamics in superconducting arrays SO PHYSICAL REVIEW B LA English DT Article ID JOSEPHSON-JUNCTION ARRAYS; RESISTIVE TRANSITION; 2-DIMENSIONAL ARRAYS; II SUPERCONDUCTORS; MAGNETIC-FIELD; PHASE; LATTICES AB We perform current (I)-voltage (V) measurements on low resistance superconductor-normal-superconductor arrays in finite magnetic fields, focusing on the dilute vortex population regime. We observe significant deviations from predicted behavior, notably the absence of a differential resistance peak near the vortex depinning current, and a broad linear I-V region with an extrapolated I intercept equal to the depinning current. Comparing these results to an overdamped molecular vortex model, we find that this behavior can be explained by the presence of a history-dependent dissipative force. This approach has not been considered previously, to our knowledge, yet it is crucial for obtaining a correct description of the vortex dynamics in superconducting arrays. C1 [Eley, Serena] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. Univ Illinois, Frederick Seitz Mat Res Lab, Urbana, IL 61801 USA. [Eley, Serena] Los Alamos Natl Lab, Condensed Matter & Magnet Sci Grp, Los Alamos, NM 87545 USA. RP Eley, S (reprint author), Univ Illinois, Dept Phys, Urbana, IL 61801 USA.; Eley, S (reprint author), Los Alamos Natl Lab, Condensed Matter & Magnet Sci Grp, Los Alamos, NM 87545 USA. OI Eley, Serena/0000-0002-2928-5316 FU Department of Energy Basic Energy Sciences [DE-SC0012649]; Sloan Foundation [FG-BR2013-044] FX The authors wish to thank S. Gopalakrishnan for useful discussions. This paper was supported by the Department of Energy Basic Energy Sciences under Grant No. DE-SC0012649. I.M.S. acknowledges support from the Sloan Foundation Grant No. FG-BR2013-044. This research was carried out in part at the Center for Microanalysis of Materials, University of Illinois at Urbana-Champaign. NR 25 TC 0 Z9 0 U1 4 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 14 PY 2016 VL 94 IS 2 AR 024510 DI 10.1103/PhysRevB.94.024510 PG 8 WC Physics, Condensed Matter SC Physics GA DR1ER UT WOS:000379649300008 ER PT J AU Galda, A Vinokur, VM AF Galda, Alexey Vinokur, Valerii M. TI Parity-time symmetry breaking in magnetic systems SO PHYSICAL REVIEW B LA English DT Article ID SPIN; TRANSITION; STATES AB The understanding of out-of-equilibrium physics, especially dynamic instabilities and dynamic phase transitions, is one of the major challenges of contemporary science, spanning the broadest wealth of research areas that range from quantum optics to living organisms. Focusing on nonequilibrium dynamics of an open dissipative spin system, we introduce a non-Hermitian Hamiltonian approach, in which non-Hermiticity reflects dissipation and deviation from equilibrium. The imaginary part of the proposed spin Hamiltonian describes the effects of Gilbert damping and applied Slonczewski spin-transfer torque. In the classical limit, our approach reproduces Landau-Lifshitz-Gilbert-Slonczewski dynamics of a large macrospin. We reveal the spin-transfer torque-driven parity-time symmetry-breaking phase transition corresponding to a transition from precessional to exponentially damped spin dynamics. Micromagnetic simulations for nanoscale ferromagnetic disks demonstrate the predicted effect. Our findings can pave the way to a general quantitative description of out-of-equilibrium phase transitions driven by spontaneous parity-time symmetry breaking. C1 [Galda, Alexey; Vinokur, Valerii M.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Galda, A (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. EM agalda@anl.gov FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX We thank Alex Kamenev for critical reading of the manuscript and valuable suggestions. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 34 TC 3 Z9 3 U1 2 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 14 PY 2016 VL 94 IS 2 AR 020408 DI 10.1103/PhysRevB.94.020408 PG 5 WC Physics, Condensed Matter SC Physics GA DR1ER UT WOS:000379649300003 ER PT J AU Nomura, T Harada, Y Niwa, H Ishii, K Ishikado, M Shamoto, S Jarrige, I AF Nomura, T. Harada, Y. Niwa, H. Ishii, K. Ishikado, M. Shamoto, S. Jarrige, I. TI Resonant inelastic x-ray scattering study of entangled spin-orbital excitations in superconducting PrFeAsO0.7 SO PHYSICAL REVIEW B LA English DT Article ID IRON-BASED SUPERCONDUCTORS; MAGNETISM; ORDER AB Low-energy electron excitation spectra were measured on a single crystal of a typical iron-based superconductor PrFeAsO0.7 using resonant inelastic x-ray scattering (RIXS) at the Fe-L-3 edge. Characteristic RIXS features are clearly observed around 0.5, 1-1.5, and 2-3 eV energy losses. These excitations are analyzed microscopically with theoretical calculations using a 22-orbital model derived from first-principles electronic structure calculation. Based on the agreement with the experiment, the RIXS features are assigned to Fe-d orbital excitations which, at low energies, are accompanied by spin flipping and dominated by Fe d(yz) and d(xz) orbital characters. Furthermore, our calculations suggest dispersive momentum dependence of the RIXS excitations below 0.5 eV, and predict remarkable splitting and merging of the lower-energy excitations in momentum space. Those excitations, which were not observed in the present experiment, highlight the potential of RIXS with an improved energy resolution to unravel new details of the electronic structure of the iron-based superconductors. C1 [Nomura, T.; Ishii, K.] SPring 8, Natl Inst Quantum & Radiol Sci & Technol, 1-1-1 Kouto, Sayo, Hyogo 6795148, Japan. [Harada, Y.] Univ Tokyo, ISSP, Kashiwa, Chiba 2778581, Japan. [Niwa, H.] Univ Tsukuba, Fac Pure & Appl Sci, Div Phys, Tsukuba, Ibaraki 3058571, Japan. [Ishikado, M.] Comprehens Res Org Sci & Soc, Res Ctr Neutron Sci & Technol, Tokai, Ibaraki 3191106, Japan. [Shamoto, S.] Japan Atom Energy Agcy, Adv Sci Res Ctr, Tokai, Ibaraki 3191195, Japan. [Jarrige, I.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Upton, NY 11973 USA. RP Nomura, T (reprint author), SPring 8, Natl Inst Quantum & Radiol Sci & Technol, 1-1-1 Kouto, Sayo, Hyogo 6795148, Japan. EM nomurat@spring8.or.jp RI Jarrige, Ignace/M-6371-2016 OI Jarrige, Ignace/0000-0002-1043-5695 NR 42 TC 1 Z9 1 U1 1 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 14 PY 2016 VL 94 IS 3 AR 035134 DI 10.1103/PhysRevB.94.035134 PG 9 WC Physics, Condensed Matter SC Physics GA DR1EZ UT WOS:000379650100004 ER PT J AU Post, KW Goncharov, AF Yin, ZP Simonson, JW Guo, J Sun, LL Zellman, S Goldflam, MD Stinson, HT Chapler, BC McNally, DE Zhao, ZX Kotliar, G Aronson, MC Basov, DN AF Post, K. W. Goncharov, Alexander F. Yin, Z. P. Simonson, J. W. Guo, Jing Sun, Liling Zellman, S. Goldflam, M. D. Stinson, H. T. Chapler, B. C. McNally, D. E. Zhao, Zhongxian Kotliar, G. Aronson, M. C. Basov, D. N. TI Electronic correlations and pressure-induced metallicity in LaMnPO1-xFx revealed via infrared spectroscopy SO PHYSICAL REVIEW B LA English DT Article ID MEAN-FIELD THEORY; IRON PNICTIDES; T-C; INSULATOR; SUPERCONDUCTORS; METAL AB We spectroscopically investigated the energy gap of the correlated antiferromagnetic insulator LaMnPO1-xFx (x = 0.0 and 0.04) as a function of temperature and pressure, separately, in conjunction with many-body electronic structure calculations. These results show that the electronic structure in all measured regimes is well described by a model that includes both Mott-Hubbard interactions and Hund's rule coupling. Moreover, we find that by applying external pressure, thereby reducing the effective Mott-Hubbard interaction and Hund's coupling, the energy gap in LaMnPO1 xFx can be fully closed, yielding a metallic state. C1 [Post, K. W.; Goldflam, M. D.; Stinson, H. T.; Chapler, B. C.; Basov, D. N.] Univ Calif San Diego, Phys Dept, La Jolla, CA 92093 USA. [Goncharov, Alexander F.] Carnegie Inst Sci, Geophys Lab, 5251 Broad Branch Rd NW, Washington, DC 20015 USA. [Yin, Z. P.; Kotliar, G.] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Simonson, J. W.; Zellman, S.; McNally, D. E.; Aronson, M. C.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Guo, Jing; Sun, Liling; Zhao, Zhongxian] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Guo, Jing; Sun, Liling; Zhao, Zhongxian] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Aronson, M. C.] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11937 USA. [Aronson, M. C.] Texas A&M Univ, Dept Phys, College Stn, TX 77843 USA. [Basov, D. N.] Columbia Univ, Dept Phys, New York, NY 10027 USA. RP Post, KW (reprint author), Univ Calif San Diego, Phys Dept, La Jolla, CA 92093 USA. EM kwpost@physics.ucsd.edu FU Office of the Assistant Secretary of Defense; ARO [w911NF-13-1-0210] FX We acknowledge the Office of the Assistant Secretary of Defense for Research and Engineering for providing the NSSEFF funds that supported this research (Z.P.Y, J.W.S., S.Z., D.E.M.). K.W.P. and D.N.B. are supported by ARO w911NF-13-1-0210. D.N.B is the Gordon and Betty Moore Foundation Fellow in Quantum Materials GBMF4533. NR 33 TC 0 Z9 0 U1 9 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 14 PY 2016 VL 94 IS 4 AR 045115 DI 10.1103/PhysRevB.94.045115 PG 7 WC Physics, Condensed Matter SC Physics GA DR1FI UT WOS:000379651000003 ER PT J AU Tamm, A Samolyuk, G Correa, AA Klintenberg, M Aabloo, A Caro, A AF Tamm, A. Samolyuk, G. Correa, A. A. Klintenberg, M. Aabloo, A. Caro, A. TI Electron-phonon interaction within classical molecular dynamics SO PHYSICAL REVIEW B LA English DT Article ID TRANSITION-METALS; PSEUDOPOTENTIALS AB We present a model for nonadiabatic classical molecular dynamics simulations that captures with high accuracy the wave-vector q dependence of the phonon lifetimes, in agreement with quantum mechanics calculations. It is based on a local view of the e-ph interaction where individual atom dynamics couples to electrons via a damping term that is obtained as the low-velocity limit of the stopping power of a moving ion in a host. The model is parameter free, as its components are derived from ab initio-type calculations, is readily extended to the case of alloys, and is adequate for large-scale molecular dynamics computer simulations. We also show how this model removes some oversimplifications of the traditional ionic damped dynamics commonly used to describe situations beyond the Born-Oppenheimer approximation. C1 [Tamm, A.; Caro, A.] Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA. [Tamm, A.; Aabloo, A.] Univ Tartu, Inst Technol, IMS Lab, EE-50411 Tartu, Estonia. [Samolyuk, G.] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN USA. [Correa, A. A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Klintenberg, M.] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden. RP Tamm, A (reprint author), Los Alamos Natl Lab, Div Mat Sci & Technol, Los Alamos, NM 87545 USA.; Tamm, A (reprint author), Univ Tartu, Inst Technol, IMS Lab, EE-50411 Tartu, Estonia. FU US Department of Energy at Los Alamos National Laboratory [2014ORNL1026]; National Nuclear Security Administration of the U.S. DOE [DE-AC52-06NA25396]; US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; US Department of Energy at Oak Ridge National Laboratory [2014ORNL1026] FX Work was performed at the Energy Dissipation to Defect Evolution Center, an Energy Frontier Research Center funded by the US Department of Energy (Award No. 2014ORNL1026) at Los Alamos and Oak Ridge National Laboratories. This research used resources provided by the LANL Institutional Computing Program. LANL, an affirmative action/equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. DOE under Contract No. DE-AC52-06NA25396. Work by A.A.C. was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 24 TC 0 Z9 0 U1 4 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 14 PY 2016 VL 94 IS 2 AR 024305 DI 10.1103/PhysRevB.94.024305 PG 5 WC Physics, Condensed Matter SC Physics GA DR1ER UT WOS:000379649300004 ER PT J AU Marshall, CM Aliaga, L Altinok, O Bellantoni, L Bercellie, A Betancourt, M Bodek, A Bravar, A Budd, H Cai, T Carneiro, MF Chvojka, J da Motta, H Devan, J Dytman, SA Diaz, GA Eberly, B Endress, E Felix, J Fields, L Filkins, A Fine, R Gago, AM Galindo, R Gallagher, H Ghosh, A Golan, T Gran, R Griswold, S Harris, DA Higuera, A Hurtado, K Kiveni, M Kleykamp, J Kordosky, M Le, T Maher, E Majoros, I Manly, S Mann, WA Caicedo, DAM McFarland, KS McGivern, CL McGowan, AM Messerly, B Miller, J Mislivec, A Morfin, JG Mousseau, J Naples, D Nelson, JK Norrick, A Osta, J Paolone, V Park, J Patrick, CE Perdue, GN Rakotondravohitra, L Ramirez, MA Ransome, RD Ray, H Ren, L Rimal, D Rodrigues, PA Rosenberg, M Ruterbories, D Schellman, H Schmitz, DW Shadler, LA Simon, C Salinas, CJS Sanchez, SF Tice, BG Valencia, E Walton, T Wang, Z Watkins, P Wiley, K Wolcott, J Wospakrik, M Zhang, D AF Marshall, C. M. Aliaga, L. Altinok, O. Bellantoni, L. Bercellie, A. Betancourt, M. Bodek, A. Bravar, A. Budd, H. Cai, T. Carneiro, M. F. Chvojka, J. da Motta, H. Devan, J. Dytman, S. A. Diaz, G. A. Eberly, B. Endress, E. Felix, J. Fields, L. Filkins, A. Fine, R. Gago, A. M. Galindo, R. Gallagher, H. Ghosh, A. Golan, T. Gran, R. Griswold, S. Harris, D. A. Higuera, A. Hurtado, K. Kiveni, M. Kleykamp, J. Kordosky, M. Le, T. Maher, E. Majoros, I. Manly, S. Mann, W. A. Caicedo, D. A. Martinez McFarland, K. S. McGivern, C. L. McGowan, A. M. Messerly, B. Miller, J. Mislivec, A. Morfin, J. G. Mousseau, J. Naples, D. Nelson, J. K. Norrick, A. Osta, J. Paolone, V. Park, J. Patrick, C. E. Perdue, G. N. Rakotondravohitra, L. Ramirez, M. A. Ransome, R. D. Ray, H. Ren, L. Rimal, D. Rodrigues, P. A. Rosenberg, M. Ruterbories, D. Schellman, H. Schmitz, D. W. Shadler, L. A. Simon, C. Salinas, C. J. Solano Sanchez, S. F. Tice, B. G. Valencia, E. Walton, T. Wang, Z. Watkins, P. Wiley, K. Wolcott, J. Wospakrik, M. Zhang, D. CA MINERvA Collaboration TI Measurement of K+ production in charged-current nu(mu) interactions SO PHYSICAL REVIEW D LA English DT Article ID STRANGE-PARTICLE-PRODUCTION; TOTAL CROSS-SECTIONS; PROTON-DECAY; NUCLEON-DECAY; NEUTRINO OSCILLATIONS; BEAM; NEON; COLLISIONS; GENERATOR; DETECTOR AB Production of K+ mesons in charged-current nu(mu) interactions on plastic scintillator (CH) is measured using MINERvA exposed to the low-energy NuMI beam at Fermilab. Timing information is used to isolate a sample of 885 charged-current events containing a stopping K+ which decays at rest. The differential cross section in K+ kinetic energy, d sigma/dT(K), is observed to be relatively flat between 0 and 500 MeV. Its shape is in good agreement with the prediction by the GENIE neutrino event generator when final-state interactions are included, however the data rate is lower than the prediction by 15%. C1 [Marshall, C. M.; Bercellie, A.; Bodek, A.; Budd, H.; Cai, T.; Chvojka, J.; Diaz, G. A.; Filkins, A.; Fine, R.; Golan, T.; Griswold, S.; Higuera, A.; Kleykamp, J.; Manly, S.; McFarland, K. S.; McGowan, A. M.; Mislivec, A.; Park, J.; Perdue, G. N.; Rodrigues, P. A.; Ruterbories, D.; Shadler, L. A.; Wang, Z.; Wiley, K.; Wolcott, J.] Univ Rochester, Rochester, NY 14627 USA. [Aliaga, L.; Devan, J.; Kordosky, M.; Nelson, J. K.; Norrick, A.; Zhang, D.] Coll William & Mary, Dept Phys, Williamsburg, VA 23187 USA. [Aliaga, L.; Diaz, G. A.; Endress, E.; Gago, A. M.; Sanchez, S. F.] Pontificia Univ Catolica Peru, Dept Ciencias, Secc Fis, Apartado 1761, Lima, Peru. [Altinok, O.; Gallagher, H.; Le, T.; Mann, W. A.] Tufts Univ, Dept Phys, Medford, MA 02155 USA. [Bellantoni, L.; Betancourt, M.; Fields, L.; Golan, T.; Harris, D. A.; Kiveni, M.; McFarland, K. S.; Morfin, J. G.; Osta, J.; Perdue, G. N.; Rakotondravohitra, L.; Schmitz, D. W.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Bravar, A.] Univ Geneva, CH-1211 Geneva 4, Switzerland. [Carneiro, M. F.; da Motta, H.; Ghosh, A.; Hurtado, K.; Caicedo, D. A. Martinez] Ctr Brasileiro Pesquisas Fis, Rua Dr Xavier Sigaud 150, BR-22290180 Rio De Janeiro, RJ, Brazil. [Dytman, S. A.; Eberly, B.; McGivern, C. L.; Messerly, B.; Naples, D.; Paolone, V.; Ren, L.; Rosenberg, M.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Felix, J.; Higuera, A.; Ramirez, M. A.] Univ Guanajuato, Campus Leon & Campus Guanajuato, Guanajuato 36000, Mexico. [Fields, L.; Patrick, C. E.; Schellman, H.] Northwestern Univ, Evanston, IL 60208 USA. [Galindo, R.; Miller, J.; Norrick, A.] Univ Tecn Federico Santa Maria, Dept Fis, Ave Espana 1680 Casilla 110-V, Valparaiso, Chile. [Gran, R.] Univ Minnesota, Dept Phys, Duluth, MN 55812 USA. [Hurtado, K.; Salinas, C. J. Solano] Univ Nacl Ingn, Apartado 31139, Lima, Peru. [Le, T.; Norrick, A.; Ransome, R. D.; Tice, B. G.] Rutgers State Univ, Piscataway, NJ 08854 USA. [Maher, E.] Massachusetts Coll Liberal Arts, 375 Church St, North Adams, MA 01247 USA. [Majoros, I.] Otterbein Univ, Dept Phys, 1 South Grove St, Westerville, OH 43081 USA. [Mousseau, J.; Ray, H.; Rimal, D.; Wospakrik, M.] Univ Florida, Dept Phys, Gainesville, FL 32611 USA. [Schellman, H.] Oregon State Univ, Dept Phys, Corvallis, OR 97331 USA. [Schmitz, D. W.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Simon, C.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Walton, T.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Eberly, B.] SLAC Natl Accelerator Lab, Stanford, CA 94309 USA. [Higuera, A.] Univ Houston, Houston, TX 77204 USA. [Caicedo, D. A. Martinez] Illinois Inst Technol, Chicago, IL 60616 USA. [McGivern, C. L.] Iowa State Univ, Ames, IA 50011 USA. [Mousseau, J.] Univ Michigan, Ann Arbor, MI 48109 USA. [Rakotondravohitra, L.] Univ Antananarivo, Dept Phys, Antananarivo, Madagascar. [Walton, T.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Wolcott, J.] Tufts Univ, Medford, MA 02155 USA. RP Marshall, CM (reprint author), Univ Rochester, Rochester, NY 14627 USA. OI Bodek, Arie/0000-0003-0409-0341; Schmitz, David/0000-0003-2165-7389 FU Fermi National Accelerator Laboratory under U.S. Department of Energy [DE-AC02-07CH11359]; MINERvA construction project; United States National Science Foundation [PHY-0619727]; NSF (USA); DOE (USA); CAPES (Brazil); CNPq (Brazil); CoNaCyT (Mexico); CONICYT (Chile); CONCYTEC (Peru); DGI-PUCP (Peru); IDI/IGI-UNI (Peru); Latin American Center for Physics (CLAF) FX This work was supported by the Fermi National Accelerator Laboratory under U.S. Department of Energy Contract No. DE-AC02-07CH11359 which included the MINERvA construction project. Construction support was also granted by the United States National Science Foundation under Award No. PHY-0619727 and by the University of Rochester. Support for participating scientists was provided by NSF and DOE (USA), by CAPES and CNPq (Brazil), by CoNaCyT (Mexico), by CONICYT (Chile), by CONCYTEC, DGI-PUCP and IDI/IGI-UNI (Peru), and by Latin American Center for Physics (CLAF). We thank the MINOS Collaboration for use of its near detector data. We acknowledge the dedicated work of the Fermilab staff responsible for the operation and maintenance of the NuMI beamline, MINERvA and MINOS detectors and the physical and software environments that support scientific computing at Fermilab. NR 52 TC 1 Z9 1 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 14 PY 2016 VL 94 IS 1 AR 012002 DI 10.1103/PhysRevD.94.012002 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DR1GB UT WOS:000379652900001 ER PT J AU Mikaelian, KO AF Mikaelian, Karnig O. TI Oscillations of a standing shock wave generated by the Richtmyer-Meshkov instability SO PHYSICAL REVIEW FLUIDS LA English DT Article ID RAYLEIGH-TAYLOR; AIR/SF6 INTERFACE; INITIAL CONDITIONS; STABILITY; SIMULATION; VISCOSITY; FRONTS; FLUIDS; TUBE AB In a typical Richtmyer-Meshkov experiment a fast moving flat shock strikes a stationary perturbed interface between fluids A and B creating a transmitted and a reflected shock, both of which are perturbed. We propose shock tube experiments in which the reflected shock is stationary in the laboratory. Such a standing perturbed shock undergoes well-known damped oscillations. We present the conditions required for producing such a standing shock wave, which greatly facilitates the measurement of the oscillations and their rate of damping. We define a critical density ratio R-critical, in terms of the adiabatic indices of the two fluids, and a critical Mach number M-s(critical) of the incident shock wave, which produces a standing reflected wave. If the initial density ratio R of the two fluids is less than R-critical then a standing shock wave is possible at M-s = M-s(critical) . Otherwise a standing shock is not possible and the reflected wave always moves in the direction opposite the incident shock. Examples are given for present-day operating shock tubes with sinusoidal or inclined interfaces. We consider the effect of viscosity, which affects the damping rate of the oscillations. We point out that nonlinear bubble and spike amplitudes depend relatively weakly on the viscosity of the fluids and that the interface area is a better diagnostic. C1 [Mikaelian, Karnig O.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Mikaelian, KO (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. FU US Department of Energy [DE-AC52-07NA27344] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 65 TC 2 Z9 2 U1 12 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-990X J9 PHYS REV FLUIDS JI Phys. Rev. Fluids PD JUL 13 PY 2016 VL 1 IS 3 AR 033601 DI 10.1103/PhysRevFluids.1.033601 PG 26 WC Physics, Fluids & Plasmas SC Physics GA EF3CO UT WOS:000390202300001 ER PT J AU Li, MT Zhu, WS Zhang, PF Chao, YH He, Q Yang, BL Li, HM Borisevich, A Dai, S AF Li, Mingtao Zhu, Wenshuai Zhang, Pengfei Chao, Yanhong He, Qian Yang, Bolun Li, Huaming Borisevich, Albinab Dai, Sheng TI Graphene-Analogues Boron Nitride Nanosheets Confining Ionic Liquids: A High-Performance Quasi-Liquid Solid Electrolyte SO SMALL LA English DT Article ID LITHIUM-METAL BATTERIES; NANOPARTICLE HYBRID ELECTROLYTES; ROOM-TEMPERATURE; POLYMER ELECTROLYTES; ELECTROCHEMICAL CHARACTERIZATION; SECONDARY BATTERIES; FABRICATION; COMPOSITES; CATIONS; IMIDE AB Solid electrolytes are one of the most promising electrolyte systems for safe lithium batteries, but the low ionic conductivity of these electrolytes seriously hinders the development of efficient lithium batteries. Here, a novel class of graphene-analogues boron nitride (g-BN) nanosheets confining an ultrahigh concentration of ionic liquids (ILs) in an interlayer and out-of-layer chamber to give rise to a quasi-liquid solid electrolyte (QLSE) is reported. The electron-insulated g-BN nanosheet host with a large specific surface area can confine ILs as much as 10 times of the host's weight to afford high ionic conductivity (3.85 x 10(-3) S cm(-1) at 25 degrees C, even 2.32 x 10(-4) S cm(-1) at -20 degrees C), which is close to that of the corresponding bulk IL electrolytes. The high ionic conductivity of QLSE is attributed to the enormous absorption for ILs and the confi ning effect of g-BN to form the ordered lithium ion transport channels in an interlayer and out-of-layer of g-BN. Furthermore, the electrolyte displays outstanding electrochemical properties and battery performance. In principle, this work enables a wider tunability, further opening up a new field for the fabrication of the next-generation QLSE based on layered nanomaterials in energy conversion devices. C1 [Li, Mingtao; Yang, Bolun] Xi An Jiao Tong Univ, Sch Chem Engn & Technol, Xian 710049, Shaanxi, Peoples R China. [Li, Mingtao; Zhu, Wenshuai; Zhang, Pengfei; Chao, Yanhong; Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Zhu, Wenshuai; Chao, Yanhong; Li, Huaming] Jiangsu Univ, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China. [He, Qian; Borisevich, Albinab] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Borisevich, Albinab] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Zhu, WS; Dai, S (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.; Zhu, WS (reprint author), Jiangsu Univ, Sch Chem & Chem Engn, Zhenjiang 212013, Peoples R China. EM zhuws@ujs.edu.cn; dais@ornl.gov RI He, Qian/J-1277-2014 FU National Natural Science Foundation of China [21376111, 21303132, 21576122, 21506083]; Six Big Talent Peak in Jiangsu province [JNHB-004]; US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Science and Engineering; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; ORNL's Center for Nanophase Materials Sciences; Scientific User Facilities Division, Office of Science, Basic Energy Sciences, U.S. Department of Energy FX M.T.L. and W.S.Z. contributed equally to this work. S.D., M.T.L., and W.S.Z. conceived the idea. W.S.Z. and Y.H.C. carried out the BN synthesis and characterization. M.T.L. prepared the quasi-liquid solid electrolytes and performed the electrochemical test. P.F.Z., B.L.Y., and H.M.L. analyzed the physicochemical properties of this new electrolyte. Q.H. and A.B. performed the STEM measurement and data analysis. M.T.L. and W.S.Z. wrote the paper. M.T.Li, W.S.Z., P.F.Z., and S.D. discussed the results and participated in the preparation of the paper. M.T.Li, W.S.Z., and Y.H.C. appreciate the financial support from the National Natural Science Foundation of China (Nos. 21376111, 21303132, 21576122 and 21506083) and Six Big Talent Peak in Jiangsu province (JNHB-004). P.F.Z. and S.D. were supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Materials Science and Engineering. Electron microscopy research (QH and AYB) is supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division and through a user project supported by ORNL's Center for Nanophase Materials Sciences, sponsored by the Scientific User Facilities Division, Office of Science, Basic Energy Sciences, U.S. Department of Energy. NR 56 TC 0 Z9 0 U1 44 U2 47 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1613-6810 EI 1613-6829 J9 SMALL JI Small PD JUL 13 PY 2016 VL 12 IS 26 BP 3535 EP 3542 DI 10.1002/smll.201600358 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DW1AI UT WOS:000383374600007 PM 27225944 ER PT J AU Dichter, BK Bouchard, KE Chang, EF AF Dichter, Benjamin K. Bouchard, Kristofer E. Chang, Edward F. TI Dynamic Structure of Neural Variability in the Cortical Representation of Speech Sounds SO JOURNAL OF NEUROSCIENCE LA English DT Article DE ECoG; encoding; noise correlations; speech; superior temporal gyrus; variability ID SUPERIOR TEMPORAL GYRUS; LOCAL-FIELD POTENTIALS; MONKEY VISUAL-CORTEX; RESPONSE VARIABILITY; AUDITORY-CORTEX; SPIKE TRAINS; LARGE-SCALE; NEURONS; OSCILLATIONS; PERCEPTION AB Accurate sensory discrimination is commonly believed to require precise representations in the nervous system; however, neural stimulus responses can be highly variable, even to identical stimuli. Recent studies suggest that cortical response variability decreases during stimulus processing, but the implications of such effects on stimulus discrimination are unclear. To address this, we examined electrocorticographic cortical field potential recordings from the human nonprimary auditory cortex (superior temporal gyrus) while subjects listened to speech syllables. Compared with a prestimulus baseline, activation variability decreased upon stimulus onset, similar to findings from microelectrode recordings in animal studies. We found that this decrease was simultaneous with encoding and spatially specific for those electrodes that most strongly discriminated speech sounds. We also found that variability was predominantly reduced in a correlated subspace across electrodes. We then compared signal and variability (noise) correlations and found that noise correlations reduce more for electrodes with strong signal correlations. Furthermore, we found that this decrease in variability is strongest in the high gamma band, which correlates with firing rate response. Together, these findings indicate that the structure of single-trial response variability is shaped to enhance discriminability despite non-stimulus-related noise. C1 [Dichter, Benjamin K.; Bouchard, Kristofer E.; Chang, Edward F.] Univ Calif San Francisco, Dept Neurol Surg, San Francisco, CA 94143 USA. [Dichter, Benjamin K.; Bouchard, Kristofer E.; Chang, Edward F.] Univ Calif San Francisco, Dept Physiol, San Francisco, CA 94143 USA. [Dichter, Benjamin K.; Bouchard, Kristofer E.; Chang, Edward F.] Univ Calif San Francisco, Ctr Integrat Neurosci, San Francisco, CA 94158 USA. [Dichter, Benjamin K.; Chang, Edward F.] Univ Calif Berkeley & Univ Calif San Francisco Jo, Berkeley, CA 94720 USA. [Bouchard, Kristofer E.; Chang, Edward F.] Univ Calif San Francisco & Univ Calif Berkeley, Ctr Neural Engn & Prosthesis, Berkeley, CA 94720 USA. [Bouchard, Kristofer E.] Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94720 USA. [Chang, Edward F.] Univ Calif San Francisco, Epilepsy Ctr, San Francisco, CA 94143 USA. RP Chang, EF (reprint author), Univ Calif San Francisco Mission Bay, Sandler Neurosci Bldg,675 Nelson Rising Lane, San Francisco, CA 94143 USA. EM edward.chang@ucsf.edu FU National Science Foundation Graduate Research Fellowship [1144247]; National Institutes of Health [R00-NS065120, DP2-OD00862, R01-DC012379]; Ester A. and Joseph Klingenstein Foundation FX This work was supported by the National Science Foundation Graduate Research Fellowship Grant 1144247, National Institutes of Health Grants R00-NS065120, DP2-OD00862, and R01-DC012379, and the Ester A. and Joseph Klingenstein Foundation. We thank the NVIDIA Corporation for donation of the Tesla K40 GPU used for this research; Connie Cheung for assistance in collecting data; and Matthew Leonard and Joseph Makin for providing helpful feedback on the manuscript. NR 52 TC 0 Z9 0 U1 7 U2 7 PU SOC NEUROSCIENCE PI WASHINGTON PA 11 DUPONT CIRCLE, NW, STE 500, WASHINGTON, DC 20036 USA SN 0270-6474 J9 J NEUROSCI JI J. Neurosci. PD JUL 13 PY 2016 VL 36 IS 28 BP 7453 EP 7463 DI 10.1523/JNEUROSCI.0156-16.2016 PG 11 WC Neurosciences SC Neurosciences & Neurology GA DS1ST UT WOS:000380380500012 PM 27413155 ER PT J AU Mori, H Bhat, R Bruni-Cardoso, A Chen, EI Jorgens, DM Coutinho, K Louie, K Ben Bowen, B Inman, JL Tecca, V Lee, SJ Becker-Weimann, S Northen, T Seiki, M Borowsky, AD Auer, M Bissell, MJ AF Mori, Hidetoshi Bhat, Ramray Bruni-Cardoso, Alexandre Chen, Emily I. Jorgens, Danielle M. Coutinho, Kester Louie, Katherine Ben Bowen, Benjamin Inman, Jamie L. Tecca, Victoria Lee, Sarah J. Becker-Weimann, Sabine Northen, Trent Seiki, Motoharu Borowsky, Alexander D. Auer, Manfred Bissell, Mina J. TI New insight into the role of MMP14 in metabolic balance SO PEERJ LA English DT Article DE Autophagy; Homeostasis; Mammary gland; Glycogen; Mmp14KO mouse; Triglycerides; Lipids; Energy metabolism; Glucose; Matrix metalloproteinase 14 ID MUSCLE PHOSPHOFRUCTOKINASE DEFICIENCY; CONGENITAL GENERALIZED LIPODYSTROPHY; TYPE-1 MATRIX-METALLOPROTEINASE; MAMMARY EPITHELIAL-CELLS; MASS-SPECTROMETRY; BRANCHING MORPHOGENESIS; PROTEIN IDENTIFICATIONS; COLLAGEN TURNOVER; SIGNALING AXIS; TUMOR-CELLS AB Membrane-anchored matrix metalloproteinase 14 (MMP14) is involved broadly in organ development through both its proteolytic and signal-transducing functions. Knockout of Mmp14 (KO) in mice results in a dramatic reduction of body size and wasting followed by premature death, the mechanism of which is poorly understood. Since the mammary gland develops after birth and is thus dependent for its functional progression on systemic and local cues, we chose it as an organ model for understanding why KO mice fail to thrive. A global analysis of the mammary glands' proteome in the wild type (WT) and KO mice provided insight into an unexpected role of MMP14 in maintaining metabolism and homeostasis. We performed mass spectrometry and quantitative proteomics to determine the protein signatures of mammary glands from 7 to 11 days old WT and KO mice and found that KO rudiments had a significantly higher level of rate-limiting enzymes involved in catabolic pathways. Glycogen and lipid levels in KO rudiments were reduced, and the circulating levels of triglycerides and glucose were lower. Analysis of the ultrastructure of mammary glands imaged by electron microscopy revealed a significant increase in autophagy signatures in KO mice. Finally, Mmp14 silenced mammary epithelial cells displayed enhanced autophagy. Applied to a systemic level, these findings indicate that MMP14 is a crucial regulator of tissue homeostasis. If operative on a systemic level, these findings could explain how Mmp14 KO litter fail to thrive due to disorder in metabolism. C1 [Mori, Hidetoshi; Borowsky, Alexander D.] Univ Calif Davis, Ctr Comparat Med, Dept Pathol, Davis, CA 95616 USA. [Mori, Hidetoshi; Bhat, Ramray; Bruni-Cardoso, Alexandre; Inman, Jamie L.; Tecca, Victoria; Lee, Sarah J.; Becker-Weimann, Sabine; Bissell, Mina J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94720 USA. [Bhat, Ramray] Univ Calcutta, Calcutta Med Coll, Kolkata, W Bengal, India. [Bruni-Cardoso, Alexandre] Univ Sao Paulo, Inst Quim, Dept Bioquim, Sao Paulo, Brazil. [Chen, Emily I.] Columbia Univ, Med Ctr, Herbert Irving Comprehens Canc Ctr, Dept Pharmacol, New York, NY USA. [Jorgens, Danielle M.; Coutinho, Kester; Auer, Manfred] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging Div, Berkeley, CA 94720 USA. [Louie, Katherine; Ben Bowen, Benjamin; Northen, Trent] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Environm Genom & Syst Biol, Berkeley, CA 94720 USA. [Seiki, Motoharu] Kanazawa Univ, Inst Med Pharmaceut & Hlth Sci, Kanazawa, Ishikawa, Japan. RP Mori, H (reprint author), Univ Calif Davis, Ctr Comparat Med, Dept Pathol, Davis, CA 95616 USA.; Mori, H; Bissell, MJ (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94720 USA. EM hmori@lbl.gov; MJBissell@lbl.gov RI Bruni-Cardoso, Alexandre/K-6443-2013; OI Northen, Trent/0000-0001-8404-3259 FU US Department of Energy, Office of Biological and Environmental Research and Low Dose Scientific Focus Area [DE-AC02-05CH1123]; National Cancer Institute [R37CA064786, R01CA057621, R01CA140663, U54CA112970, U01CA143233]; US Department of Defense [W81XWH0810736]; NIH/NCRR [1 S10 RR023680-1] FX The work in M.J.B.'s laboratory is supported by grants from the US Department of Energy, Office of Biological and Environmental Research and Low Dose Scientific Focus Area (DE-AC02-05CH1123); by National Cancer Institute (R37CA064786, R01CA057621, R01CA140663, U54CA112970, U01CA143233); by the US Department of Defense (W81XWH0810736). The mass spectrometer used in this study was funded by the shared instrument grant (NIH/NCRR 1 S10 RR023680-1). The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 64 TC 0 Z9 0 U1 7 U2 8 PU PEERJ INC PI LONDON PA 341-345 OLD ST, THIRD FLR, LONDON, EC1V 9LL, ENGLAND SN 2167-8359 J9 PEERJ JI PeerJ PD JUL 13 PY 2016 VL 4 AR e2142 DI 10.7717/peerj.2142 PG 24 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR7GL UT WOS:000380067900002 PM 27478693 ER PT J AU Li, SD Guo, JH Ye, Z Zhao, X Wu, SQ Mi, JX Wang, CZ Gong, ZL McDonald, MJ Zhu, ZZ Ho, KM Yang, Y AF Li, Shouding Guo, Jianghuai Ye, Zhuo Zhao, Xin Wu, Shunqing Mi, Jin-Xiao Wang, Cai-Zhuang Gong, Zhengliang McDonald, Matthew J. Zhu, Zizhong Ho, Kai-Ming Yang, Yong TI Zero-Strain Na2FeSiO4 as Novel Cathode Material for Sodium-Ion Batteries SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE Na2FeSiO4; nanocrystallites; zero-strain; cathode; sodium ion batteries ID ENERGY-STORAGE; HIGH-CAPACITY; LITHIUM; PERFORMANCE; ELECTRODES AB A new cubic polymorph of sodium iron silicate, Na2FeSiO4, is reported for the first time as a cathode material for Na-ion batteries. It adopts an unprecedented cubic rigid tetrahedral open framework structure, i.e., F (4) over bar 3m, leading to a polyanion cathode material without apparent cell volume change during the charge/discharge processes. This cathode shows a reversible capacity of 106 mAh g(-1) and a capacity retention of 96% at 5 mA g(-1) after 20 cycles. C1 [Li, Shouding; Guo, Jianghuai; McDonald, Matthew J.; Yang, Yong] Xiamen Univ, State Key Lab Phys Chem Solid Surface, Collaborat Innovat Ctr Chem Energy Mat, Xiamen 361005, Peoples R China. [Li, Shouding; Guo, Jianghuai; McDonald, Matthew J.; Yang, Yong] Xiamen Univ, Coll Chem & Chem Engn, Dept Chem, Xiamen 361005, Peoples R China. [Wu, Shunqing; Zhu, Zizhong] Xiamen Univ, Dept Phys, Xiamen 361005, Peoples R China. [Wu, Shunqing; Zhu, Zizhong] Xiamen Univ, Collaborat Innovat Ctr Optoelect Semicond & Effic, Xiamen 361005, Peoples R China. [Mi, Jin-Xiao] Xiamen Univ, Dept Mat Sci & Engn, Xiamen 361005, Peoples R China. [Gong, Zhengliang; Yang, Yong] Xiamen Univ, Coll Energy, Xiamen 361005, Peoples R China. [Ye, Zhuo; Zhao, Xin; Wang, Cai-Zhuang; Ho, Kai-Ming] US DOE, Ames Lab, Ames, IA 50011 USA. [Ye, Zhuo; Zhao, Xin; Wang, Cai-Zhuang; Ho, Kai-Ming] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Ho, Kai-Ming] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Int Ctr Quantum Design Funct Mat ICQD, Hefei 230026, Anhui, Peoples R China. RP Yang, Y (reprint author), Xiamen Univ, State Key Lab Phys Chem Solid Surface, Collaborat Innovat Ctr Chem Energy Mat, Xiamen 361005, Peoples R China.; Yang, Y (reprint author), Xiamen Univ, Coll Chem & Chem Engn, Dept Chem, Xiamen 361005, Peoples R China.; Yang, Y (reprint author), Xiamen Univ, Coll Energy, Xiamen 361005, Peoples R China. EM yyang@xmu.edu.cn RI Mi, Jin-Xiao MI/G-4129-2010; Yang, Yong/G-4650-2010; Wu, S.Q./G-3992-2010; OI Mi, Jin-Xiao MI/0000-0002-4316-457X; Wu, S.Q./0000-0002-2545-0054; Zhao, Xin/0000-0002-3580-512X FU National Basic Research Program of China (973 program) [2011CB935903]; National Natural Science Foundation of China [21233004, 21473148, 21021002, 21428303]; Natural Science Foundation of Fujian Province of China [2015J01030]; U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering [DE-AC02-07CH11358] FX This work was supported by financial support from the National Basic Research Program of China (973 program, Grant No. 2011CB935903), the National Natural Science Foundation of China (Grant Nos. 21233004, 21473148, and 21021002 and in part 21428303), and the Natural Science Foundation of Fujian Province of China (Grant No. 2015J01030). Work at Ames Laboratory was supported by the U.S. Department of Energy, Basic Energy Sciences, Division of Materials Science and Engineering, under Contract No. DE-AC02-07CH11358, including a grant of computer time at the National Energy Research Scientific Computing Center (NERSC) in Berkeley, CA. NR 33 TC 5 Z9 5 U1 48 U2 85 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUL 13 PY 2016 VL 8 IS 27 BP 17233 EP 17238 DI 10.1021/acsami.6b03969 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DR3HK UT WOS:000379794100026 PM 27305627 ER PT J AU Ye, CH Nikolov, SV Geryak, RD Calabrese, R Ankner, JF Alexeev, A Kaplan, DL Tsukruk, VV AF Ye, Chunhong Nikolov, Svetoslav V. Geryak, Ren D. Calabrese, Rossella Ankner, John F. Alexeev, Alexander Kaplan, David L. Tsukruk, Vladimir V. TI Bimorph Silk Microsheets with Programmable Actuating Behavior: Experimental Analysis and Computer Simulations SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE microfabricated biopolymers; LbL assembly; silk micro-origami; responsive biomaterials; theoretical simulation; neutron reflectivity ID NEUTRON REFLECTIVITY; IONOMER MICROCAPSULES; SHAPE TRANSFORMATIONS; HYDROGEL SHEETS; BILAYERS; FILMS; PH; ROBUST; MICROSTRUCTURES; ENCAPSULATION AB Microscaled self-rolling construct sheets from silk protein material have been fabricated, containing a silk bimorph composed of silk ionomers as an active layer and cross-linked silk fisheet as the passive layer. The programmable morphology was experimentally explored along with a computational simulation to understand the mechanism of shape reconfiguration. The neutron reflectivity shows that the active silk ionomers layer undergoes remarkable swelling (eight times increase in thickness) after deprotonation while the passive silk fi-sheet retains constant volume under the same conditions and supports the bimorph construct. This selective swelling within the silk-on-silk bimorph microsheets generates strong interfacial stress between layers and out-of-plane forces, which trigger autonomous self -rolling into various 3D constructs such as cylindrical and helical tubules. The experimental observations and computational modeling confirmed the role of interfacial stresses and allow programming the morphology of the 3D constructs with particular design. We demonstrated that the biaxial stress distribution over the 2D planar films depends upon the lateral dimensions, thickness and the aspect ratio of the microsheets. The results allow the fine-tuning of autonomous shape transformations for the further design of complex micro origami constructs and the silk based rolling/unrolling structures provide a promising platform for polymer -based biomimetic devices for implant applications. C1 [Ye, Chunhong; Geryak, Ren D.; Tsukruk, Vladimir V.] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. [Nikolov, Svetoslav V.; Alexeev, Alexander] Georgia Inst Technol, Sch Mech Engn, Atlanta, GA 30332 USA. [Calabrese, Rossella; Kaplan, David L.] Tufts Univ, Dept Biomed Engn, 4 Colby St, Medford, MA 02155 USA. [Ankner, John F.] Oak Ridge Natl Lab, Spallat Neutron Source, Oka Ridge, TN 37831 USA. RP Tsukruk, VV (reprint author), Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA. EM Vladimir@mse.gatech.edu FU Air Force Office for Scientific Research [FA9550-14-1-0269, FA9550-14-1-0015]; Alexander von Humboldt Foundation; [NSF-CBET-1402712]; [DGE-1144591] FX The authors appreciate helpful discussions with Sidney Malak and Kesong Hu. This work is supported by the Air Force Office for Scientific Research FA9550-14-1-0269 and FA9550-14-1-0015, the NSF-CBET-1402712 and DGE-1144591. acknowledges financial support from the Alexander von Humboldt Foundation. NR 57 TC 1 Z9 1 U1 12 U2 24 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUL 13 PY 2016 VL 8 IS 27 BP 17694 EP 17706 DI 10.1021/acsami.6b05156 PG 13 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DR3HK UT WOS:000379794100079 PM 27308946 ER PT J AU Chai, SH Liu, ZM Huang, K Tan, S Dai, S AF Chai, Song-Hai Liu, Zhi-Ming Huang, Kuan Tan, Shuai Dai, Sheng TI Amine Functionalization of Microsized and Nanosized Mesoporous Carbons for Carbon Dioxide Capture SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID CO2 CAPTURE; POROUS CARBON; ADSORBENTS; ACTIVATION; TEMPERATURE; PERFORMANCE; ADSORPTION; SEPARATION; NANOTUBES; SYSTEMS AB Carbonaceous nanomaterials with uniform pore size are potential solid sorbents in various industrial applications, such as gas purification and water treatment, because of their easily tunable pore diameter and morphology. However, the carbon-based sorbents are greatly limited in CO2 capture, because of their weak interaction with CO2 (physical adsorption in nature). This work reports the amino functionalizalion of micronized and nanosized mesoporous carbons for CO2 capture. Two strategies, i.e., physical impregnation with branched polyethylenimine (PEI) and chemical grafting of ethylenediamine, are used to functionalize mesoporous carbon microparticles (MCMs) with a particle size of 100-200 pan. The amine-grafted MCMs (NH2-MCMs) show little advantage over PEI-impregnated MCMs (PEI/MCMs) in CO2 adsorption capacities, because of their similar surface functional groups and textural properties. In addition, mesoporous carbon nanospheres (MCNs) with a sphere size of 850-1000 nm are prepared by a silica-assisted self-assembly method for comparison with MCMs. The PEI-impregnated MCNs (PEI/MCNs) have higher CO2 adsorption capacities and amine efficiencies than PEI/MCMs at the same PEI loading, indicating a more efficient utilization of the incorporated PEI in the nanosized carbon spheres. The best performing PEI/MCNs adsorbent shows a CO2 capacity of 1.97 mmol-CO2 g(-1) at 75 degrees C, which is more than three times that of PEI/MCMs. C1 [Chai, Song-Hai; Liu, Zhi-Ming; Huang, Kuan; Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37966 USA. [Tan, Shuai] Georgia Inst Technol, Sch Chem Biomol Engn, Atlanta, GA 30332 USA. [Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Dai, S (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37966 USA.; Dai, S (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM dais@ornl.gov RI Dai, Sheng/K-8411-2015; Tan, Shuai/D-6737-2011; Huang, Kuan/F-7003-2015 OI Dai, Sheng/0000-0002-8046-3931; Tan, Shuai/0000-0003-3200-7875; Huang, Kuan/0000-0003-1905-3017 FU Center for Understanding and Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME); Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, at Oak Ridge National Laboratory and at Georgia Tech [DE-SC0012577] FX This contribution was identified by Prof. Dr. De-en Jiang (University of California at Riverside) as the Best Presentation in the session "ENFL Porous Materials for Energy & Sustainability from Discovery to Application" of the 2015 ACS Fall National Meeting in Boston, MA. This work was supported as part of the Center for Understanding and Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, at Oak Ridge National Laboratory and at Georgia Tech, under Contract No. DE-SC0012577. NR 27 TC 2 Z9 2 U1 26 U2 43 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD JUL 13 PY 2016 VL 55 IS 27 BP 7355 EP 7361 DI 10.1021/acs.iecr.6b00823 PG 7 WC Engineering, Chemical SC Engineering GA DR3HO UT WOS:000379794500014 ER PT J AU Isenberg, SL Carter, MD Hayes, SR Graham, LA Johnson, D Mathews, TP Harden, LA Takeoka, GR Thomas, JD Pirkle, JL Johnson, RC AF Isenberg, Samantha L. Carter, Melissa D. Hayes, Shelby R. Graham, Leigh Ann Johnson, Darryl Mathews, Thomas P. Harden, Leslie A. Takeoka, Gary R. Thomas, Jerry D. Pirkle, James L. Johnson, Rudolph C. TI Quantification of Toxins in Soapberry (Sapindaceae) Arils: Hypoglycin A and Methylenecyclopropylglycine SO JOURNAL OF AGRICULTURAL AND FOOD CHEMISTRY LA English DT Article DE Litchi; lychee; ackee; methylenecyclopropylglycine; hypoglycin A; soapberry; methylenecyclopropylalanine; Acer; Aceraceae; cyclopropylamino acids; Sapindaceae; Aesculus; rambutan ID BIOLOGICALLY-ACTIVE POLYPEPTIDES; JAMAICAN VOMITING SICKNESS; ACKEE BLIGHIA-SAPIDA; ACUTE ENCEPHALITIS; FRUIT; MUZAFFARPUR; MATURITY; CHILDREN; SEEDS AB Methylenecyclopropylglycine (MCPG) and hypoglycin A (HGA) are naturally occurring amino acids found in some soapberry fruits. Fatalities have been reported worldwide as a result of HGA ingestion, and exposure to MCPG has been implicated recently in the Asian outbreaks of hypoglycemic encephalopathy. In response to an outbreak linked to soapberry ingestion, the authors developed the first method to simultaneously quantify MCPG and HGA in soapberry fruits from 1 to 10 000 ppm of both toxins in dried fruit aril. Further, this is the first report of HGA in litchi, longan, and mamoncillo arils. This method is presented to specifically address the laboratory needs of public-health investigators in the hypoglycemic encephalitis outbreaks linked to soapberry fruit ingestion. C1 [Isenberg, Samantha L.; Graham, Leigh Ann; Mathews, Thomas P.] Ctr Dis Control & Prevent, Battelle Mem Inst, Atlanta, GA 30341 USA. [Carter, Melissa D.; Thomas, Jerry D.; Pirkle, James L.; Johnson, Rudolph C.] Ctr Dis Control & Prevent, Div Sci Lab, Natl Ctr Environm Hlth, Atlanta, GA 30341 USA. [Hayes, Shelby R.; Johnson, Darryl] Ctr Dis Control & Prevent, Oak Ridge Inst Sci & Educ, Atlanta, GA 30341 USA. [Harden, Leslie A.; Takeoka, Gary R.] Agr Res Serv, Western Reg Res Ctr, US Dept Agr Albany, Albany, CA 94710 USA. RP Carter, MD (reprint author), Ctr Dis Control & Prevent, Div Sci Lab, Natl Ctr Environm Hlth, Atlanta, GA 30341 USA. EM melissa.carter@cdc.hhs.gov FU Centers for Disease Control and Prevention; Battelle Memorial Institute; Oak Ridge Institute for Science and Education; U.S. Department of Agriculture FX This work was supported by the Centers for Disease Control and Prevention, the Battelle Memorial Institute, the Oak Ridge Institute for Science and Education, and the U.S. Department of Agriculture. NR 32 TC 2 Z9 2 U1 12 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0021-8561 EI 1520-5118 J9 J AGR FOOD CHEM JI J. Agric. Food Chem. PD JUL 13 PY 2016 VL 64 IS 27 BP 5607 EP 5613 DI 10.1021/acs.jafc.6b02478 PG 7 WC Agriculture, Multidisciplinary; Chemistry, Applied; Food Science & Technology SC Agriculture; Chemistry; Food Science & Technology GA DR3HM UT WOS:000379794300021 PM 27367968 ER PT J AU Barbieri, R Buttazzo, D Hall, LJ Marzocca, D AF Barbieri, Riccardo Buttazzo, Dario Hall, Lawrence J. Marzocca, David TI Higgs mass and unified gauge coupling in the NMSSM with vector matter SO JOURNAL OF HIGH ENERGY PHYSICS LA English DT Article DE Beyond Standard Model; GUT; Higgs Physics; Supersymmetric Standard Model ID UNIFICATION; RESONANCE; MODEL AB We consider the NMSSM extended to include one vector-like family of quarks and leptons. If (some of) these vector-like matter particles, as the Higgs doublets, have Yukawa couplings to the singlet S that exceed unity at about the same scale Lambda less than or similar to 10(3) TeV, this gives the order 40% enhancement of the tree level Higgs boson mass required in the MSSM to reach 125 GeV. It is conceivable that the Yukawa couplings to the singlet S, although naively blowing up close to Lambda, will not spoil gauge coupling unification. In such a case the unified coupling alpha(X) could be interestingly led to a value not far from unity, thus providing a possible explanation for the number of generations. The characteristic signal is an enhanced resonant production of neutral spin zero particles at LHC, that could even explain the putative diphoton resonance hinted by the recent LHC data at 750 GeV. C1 [Barbieri, Riccardo] Swiss Fed Inst Technol, Inst Theoret Studies, Clausiusstr 47, CH-8092 Zurich, Switzerland. [Barbieri, Riccardo] Scuola Normale Super Pisa, Piazza Cavalieri 7, I-56126 Pisa, Italy. [Buttazzo, Dario; Marzocca, David] Univ Zurich, Inst Phys, Winterthurerstr 190, CH-8057 Zurich, Switzerland. [Hall, Lawrence J.] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Theoret Phys, 366 Le Conte Hall, Berkeley, CA 94720 USA. [Hall, Lawrence J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Theoret Phys Grp, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Barbieri, R (reprint author), Swiss Fed Inst Technol, Inst Theoret Studies, Clausiusstr 47, CH-8092 Zurich, Switzerland.; Barbieri, R (reprint author), Scuola Normale Super Pisa, Piazza Cavalieri 7, I-56126 Pisa, Italy. EM riccardo.barbieri@sns.it; buttazzo@physik.uzh.ch; ljhall@lbl.gov; marzocca@physik.uzh.ch FU Office of Science, Office of High Energy and Nuclear Physics, of the US Department of Energy [DE-AC02-05CH11231]; National Science Foundation [PHY-1002399, PHY-1316783]; Walter Haefner Foundation; ETH Zurich Foundation; Swiss National Science Foundation (SNF) [200021-159720] FX L. Hall thanks Keisuke Harigaya and Yasunori Nomura for many useful conversations. R. Barbieri, D. Buttazzo, and D. Marzocca thank Gino Isidori for interesting discussions on various points of this paper. This work was supported in part by the Director, Office of Science, Office of High Energy and Nuclear Physics, of the US Department of Energy under Contract DE-AC02-05CH11231 and by the National Science Foundation under grants PHY-1002399 and PHY-1316783. R. Barbieri wants to thank Dr. Max Rossler, the Walter Haefner Foundation and the ETH Zurich Foundation for support. D. Buttazzo and D. Marzocca are supported in part by the Swiss National Science Foundation (SNF) under contract 200021-159720. NR 36 TC 3 Z9 3 U1 1 U2 2 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1029-8479 J9 J HIGH ENERGY PHYS JI J. High Energy Phys. PD JUL 13 PY 2016 IS 7 AR 067 DI 10.1007/JHEP07(2016)067 PG 15 WC Physics, Particles & Fields SC Physics GA DR4MC UT WOS:000379874700001 ER PT J AU Hu, L Chen, J Sanson, A Wu, H Rodriguez, CG Olivi, L Ren, Y Fan, LL Deng, JX Xing, XR AF Hu, Lei Chen, Jun Sanson, Andrea Wu, Hui Rodriguez, Clara Guglieri Olivi, Luca Ren, Yang Fan, Longlong Deng, Jinxia Xing, Xianran TI New Insights into the Negative Thermal Expansion: Direct Experimental Evidence for the "Guitar-String" Effect in Cubic ScF3 SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID DEBYE-WALLER FACTOR; ZERO AB The understanding of the negative thermal expansion (NTE) mechanism remains challenging but critical for the development of NTE materials. This study sheds light on NTE of ScF3, one of the most outstanding materials with NTE. The local dynamics of ScF3 has been investigated by a combined analysis of synchrotron-based X-ray total scattering, extended X-ray absorption fine structure, and neutron powder diffraction. Very interestingly, we observe that (i) the Sc-F nearest-neighbor distance strongly expands with increasing temperature, while the Sc-Sc next-nearest-neighbor distance contracts, (ii) the thermal ellipsoids of relative vibrations between Sc-F nearest-neighbors are highly elongated in the direction perpendicular to the Sc-F bond, indicating that the Sc-F bond is much softer to bend than to stretch, and (iii) there is mainly dynamically transverse motion of fluorine atoms, rather than static shifts. These results are direct experimental evidence for the NTE mechanism, in which the rigid unit is not necessary for the occurrence of NTE, and the key role is played by the transverse thermal vibrations of fluorine atoms through the "guitar-string" effect. C1 [Hu, Lei; Chen, Jun; Fan, Longlong; Deng, Jinxia; Xing, Xianran] Univ Sci & Technol Beijing, Dept Phys Chem, Beijing 100083, Peoples R China. [Sanson, Andrea] Univ Padua, Dept Phys & Astron, I-35131 Padua, Italy. [Wu, Hui] NIST, NIST Ctr Neutron Res, Gaithersburg, MD 20878 USA. [Rodriguez, Clara Guglieri; Olivi, Luca] Elettra Synchrotron, I-34149 Basovizza, Triestre, Italy. [Ren, Yang] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Chen, J; Xing, XR (reprint author), Univ Sci & Technol Beijing, Dept Phys Chem, Beijing 100083, Peoples R China. EM junchen@ustb.edu.cn; xing@ustb.edu.cn RI Wu, Hui/C-6505-2008; Chen, Jun/M-1669-2015 OI Wu, Hui/0000-0003-0296-5204; FU National Natural Science Foundation of China [21322102, 91422301, 21231001, 21590793]; Changjiang Young Scholars Award; National Program for Support of Top-notch Young Professionals; Fundamental Research Funds for the Central Universities, China [FRF-TP-14-012C1]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; ELETTRA project [20140214] FX This work was supported by the National Natural Science Foundation of China (grant nos. 21322102, 91422301, 21231001, and 21590793), the Changjiang Young Scholars Award. National Program for Support of Top-notch Young Professionals, the Fundamental Research Funds for the Central Universities, China (FRF-TP-14-012C1). The use of the Advanced Photon Source at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences (DE-AC02-06CH11357). We acknowledge the ELETTRA Synchrotron Radiation Facility for provision of synchrotron radiation as well as all the staff of the XAFS beamline. This work has been partially supported by the ELETTRA project no. 20140214. NR 33 TC 8 Z9 8 U1 30 U2 81 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 13 PY 2016 VL 138 IS 27 BP 8320 EP 8323 DI 10.1021/jacs.6b02370 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DR3HN UT WOS:000379794400001 PM 27336200 ER PT J AU Fracaroli, AM Siman, P Nagib, DA Suzuki, M Furukawa, H Toste, FD Yaghi, OM AF Fracaroli, Alejandro M. Siman, Peter Nagib, David A. Suzuki, Mitsuharu Furukawa, Hiroyasu Toste, F. Dean Yaghi, Omar M. TI Seven Post-synthetic Covalent Reactions in Tandem Leading to Enzyme-like Complexity within Metal-Organic Framework Crystals SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID POSTSYNTHETIC MODIFICATION AB The design of enzyme-like complexity within metal-organic frameworks (MOFs) requires multiple reactions to be performed on a MOF crystal without losing access to its interior. Here, we show that seven post-synthetic reactions can be successfully achieved within the pores of a multivariate MOF, MTV-IRMOF-74-III, to covalently incorporate tripeptides that resemble the active sites of enzymes in their spatial arrangement and compositional heterogeneity. These reactions build up H2N-Pro-Gly-Ala-CONHL and H2N-Cys-His-Asp-CONHL (where L = organic struts) amino acid sequences by covalently attaching them to the organic struts in the MOFs, without losing porosity or crystallinity. An enabling feature of this chemistry is that the primary amine functionality (-CH(2)NHBoc) of the original MOF is more reactive than the commonly examined aromatic amines (-NH2), and this allowed for the multi-step reactions to be carried out in tandem within the MOF. Preliminary findings indicate that the complexity thus achieved can affect reactions that were previously accomplished only in the presence of enzymes. C1 [Fracaroli, Alejandro M.; Siman, Peter; Nagib, David A.; Suzuki, Mitsuharu; Furukawa, Hiroyasu; Toste, F. Dean; Yaghi, Omar M.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Fracaroli, Alejandro M.; Siman, Peter; Suzuki, Mitsuharu; Furukawa, Hiroyasu; Yaghi, Omar M.] Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Fracaroli, Alejandro M.; Siman, Peter; Suzuki, Mitsuharu; Furukawa, Hiroyasu; Yaghi, Omar M.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. [Fracaroli, Alejandro M.] Univ Nacl Cordoba, Fac Ciencias Quim, Dept Quim Organ, Inst Invest Fisicoquim Cordoba,INFIQC CONICET, Ciudad Univ,X5000HUA, Cordoba, Argentina. RP Yaghi, OM (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Yaghi, OM (reprint author), Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA.; Yaghi, OM (reprint author), Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. EM yaghi@berkeley.edu RI Nagib, David/B-6618-2014; OI Nagib, David/0000-0002-2275-6381; Yaghi, Omar/0000-0002-5611-3325 FU BASF SE (Ludwigshafen, Germany); U.S. Department of Defense, Defense Threat Reduction Agency [HDTRA 1-12-1-0053]; U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0001015]; National Institutes of Health under a Kirschtein National Service Award [F32GM097956] FX This work was partially supported for synthesis by BASF SE (Ludwigshafen, Germany), catalytic reactions by U.S. Department of Defense, Defense Threat Reduction Agency (HDTRA 1-12-1-0053), and gas adsorption studies by the Center for Gas Separations Relevant to Clean Energy Technologies, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences (DE-SC0001015). D.A.N. was supported by the National Institutes of Health under a Kirschtein National Service Award (F32GM097956). NR 22 TC 11 Z9 11 U1 65 U2 119 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 13 PY 2016 VL 138 IS 27 BP 8352 EP 8355 DI 10.1021/jacs.6b04204 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DR3HN UT WOS:000379794400009 PM 27346625 ER PT J AU Cormary, B Li, T Liakakos, N Peres, L Fazzini, PF Blon, T Respaud, M Kropf, AJ Chaudret, B Miller, JT Mader, EA Soulantica, K AF Cormary, Benoit Li, Tao Liakakos, Nikos Peres, Laurent Fazzini, Pier-Francesco Blon, Thomas Respaud, Marc Kropf, A. Jeremy Chaudret, Bruno Miller, Jeffrey T. Mader, Elizabeth A. Soulantica, Katerina TI Concerted Growth and Ordering of Cobalt Nanorod Arrays as Revealed by Tandem in Situ SAXS-XAS Studies SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID RAY-ABSORPTION SPECTROSCOPY; STRUCTURAL-CHARACTERIZATION; NANOCRYSTAL SUPERLATTICES; COLLOIDAL NANOCRYSTALS; ORIENTED ATTACHMENT; CRYSTAL-STRUCTURES; CDSE NANOCRYSTALS; AU NANOWIRES; MESOCRYSTALS; NANOPARTICLES AB The molecular and ensemble dynamics for the growth of hierarchical supercrystals of cobalt nanorods have been studied by in situ tandem X-ray absorption spectroscopy-small-angle X-ray scattering (XAS-SAXS). The supercrystals were obtained by reducing a Co(II) precursor under H-2 in the presence of a long-chain amine and a long-chain carboxylic acid. Complementary time-dependent ex situ TEM studies were also performed. The experimental data provide critical insights into the nanorod growth mechanism and unequivocal evidence for a concerted growth organization process. Nanorod formation involves cobalt nucleation, a fast atom-by-atom anisotropic growth, and a slower oriented attachment process that continues well after cobalt reduction is complete. Smectic-like ordering of the nanorods appears very early in the process, as soon as nanoparticle elongation appears, and nanorod growth takes place inside organized superlattices, which can be regarded as mesocrystals. C1 [Cormary, Benoit; Liakakos, Nikos; Peres, Laurent; Fazzini, Pier-Francesco; Blon, Thomas; Respaud, Marc; Chaudret, Bruno; Soulantica, Katerina] Univ Toulouse, CNRS, UPS, LPCNO,CNRS UMR5215, 135 Ave Rangueil, F-31077 Toulouse, France. [Li, Tao] Argonne Natl Lab, Xray Sci Div, 9700 South Cass Ave, Chicago, IL 60605 USA. [Kropf, A. Jeremy; Miller, Jeffrey T.; Mader, Elizabeth A.] Argonne Natl Lab, Chem Sci & Engn Div, 9700 South Cass Ave, Chicago, IL 60605 USA. [Miller, Jeffrey T.] Purdue Univ, Sch Chem Engn, 480 Stadium Mall Dr, W Lafayette, IN 47097 USA. RP Soulantica, K (reprint author), Univ Toulouse, CNRS, UPS, LPCNO,CNRS UMR5215, 135 Ave Rangueil, F-31077 Toulouse, France.; Mader, EA (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 South Cass Ave, Chicago, IL 60605 USA. EM elizabeth.mader@yale.edu; ksoulant@insa-toulouse.fr FU ANR for the project BATMAG [ANR-07-BLAN-0296]; European Commission for the FP7 NAMDIATREAM project [EU NMP4-LA-2010-246479]; Region Midi-Pyrenees for the POCTEFA Interreg project [MET-NANO EFA 17/08]; Chemical Sciences and Engineering Division at Argonne National Laboratory; Institute for Atom-efficient Chemical Transformations (TACT), an Energy Frontier Research Center - U.S. DOE, Office of Science, Office of Basic Energy Sciences; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; Department of Energy; MRCAT FX B.C., N.L., B.C., and K.S. thank the ANR for the project BATMAG (ANR-07-BLAN-0296), the European Commission for the FP7 NAMDIATREAM project (EU NMP4-LA-2010-246479), the European Commission and the Region Midi-Pyrenees for the POCTEFA Interreg project (MET-NANO EFA 17/08). E.A.M. and A.J.K. acknowledge financial support from the Chemical Sciences and Engineering Division at Argonne National Laboratory. J.T.M. and T.L. were supported as part of the Institute for Atom-efficient Chemical Transformations (TACT), an Energy Frontier Research Center funded by the U.S. DOE, Office of Science, Office of Basic Energy Sciences. Use of the Advanced Photon Source (APS) is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract DE-AC02-06CH11357. MRCAT operations are supported by the Department of Energy and the MRCAT member institutions. NR 71 TC 1 Z9 1 U1 25 U2 39 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 13 PY 2016 VL 138 IS 27 BP 8422 EP 8431 DI 10.1021/jacs.6b01929 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA DR3HN UT WOS:000379794400025 PM 27300493 ER PT J AU Maughan, AE Ganose, AM Bordelon, MM Miller, EM Scanlon, DO Neilson, JR AF Maughan, Annalise E. Ganose, Alex M. Bordelon, Mitchell M. Miller, Elisa M. Scanlon, David O. Neilson, James R. TI Defect Tolerance to Intolerance in the Vacancy-Ordered Double Perovskite Semiconductors Cs2SnI6 and Cs2TeI6 SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID METHYLAMMONIUM LEAD IODIDE; SENSITIZED SOLAR-CELLS; ORGANOMETAL HALIDE PEROVSKITES; EFFECTIVE IONIC-RADII; PHASE-TRANSITIONS; CRYSTAL-STRUCTURE; HIGH-PERFORMANCE; PHOTOVOLTAIC APPLICATIONS; ORGANOHALIDE PEROVSKITES; CONTROLLED HUMIDITY AB Vacancy-ordered double perovskites of the general formula A(2)BX(6) are a family of perovskite derivatives composed of a face-centered lattice of nearly isolated [BX6] units with A-site cations occupying the cuboctahedral voids. Despite the presence of isolated octahedral units, the close-packed iodide lattice provides significant electronic dispersion, such that Cs2SnI6 has recently been explored for applications in photovoltaic devices. To elucidate the structure property relationships of these materials, we have synthesized solid-solution Cs2Sn1-xTexI6. However, even though tellurium substitution increases electronic dispersion via closer I-I contact distances, the substitution experimentally yields insulating behavior from a significant decrease in carrier concentration and mobility. Density functional calculations of native defects in Cs2SnI6 reveal that iodine vacancies exhibit a low enthalpy of formation, and that the defect energy level is a shallow donor to the conduction band rendering the material tolerant to these defect states. The increased covalency of Te-I bonding renders the formation of iodine vacancy states unfavorable and is responsible for the reduction in conductivity upon Te substitution. Additionally, Cs2TeI6 is intolerant to the formation of these defects, because the defect level occurs deep within the band gap and thus localizes potential mobile charge carriers. In these vacancy-ordered double perovskites, the close-packed lattice of iodine provides significant electronic dispersion, while the interaction of the B- and X-site ions dictates the properties as they pertain to electronic structure and defect tolerance. This simplified perspective based on extensive experimental and theoretical analysis provides a platform from which to understand structure property relationships in functional perovskite halides C1 [Maughan, Annalise E.; Bordelon, Mitchell M.; Neilson, James R.] Colorado State Univ, Dept Chem, Ft Collins, CO 80523 USA. [Ganose, Alex M.; Scanlon, David O.] UCL, Dept Chem, Kathleen Lonsdale Mat Chem, 20 Gordon St, London WC1H 0AJ, England. [Ganose, Alex M.; Scanlon, David O.] Diamond Light Source Ltd, Diamond House,Harwell Sci & Innovat Campus, Didcot OX11 0DE, Oxon, England. [Miller, Elisa M.] Natl Renewable Energy Lab, Chem & Mat Sci Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. RP Neilson, JR (reprint author), Colorado State Univ, Dept Chem, Ft Collins, CO 80523 USA. EM james.neilson@colostate.edu RI Scanlon, David/B-1516-2008; OI Scanlon, David/0000-0001-9174-8601; Neilson, James/0000-0001-9282-5752 FU DOE Office of Science [DE-AC02-06CH11357]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; NSF [CNS-0923386]; Extreme Science and Engineering Discovery Environment (XSEDE); National Science Foundation [ACI-1053575]; EPSRC [EP/L000202, EP/N01572X/1]; SUPERSOLAR Solar Energy Hub [EP/J017361/1]; Diamond Light Source [EP/L015862/1]; NVIDIA Corporation; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences [DE-AC36- 08GO28308] FX We thank M. M. Reynolds for use of her optical spectrometer, Y. Yang for photoluminescence measurements, A. Huq for neutron powder diffraction measurements, and J. A. Kurzman, A. J. Martinolich, and B. C. Melot for useful discussions. Research at the 11-ID-B and 11-BM-B beamlines used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. A portion of this research at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The calculations performed at CSU used the CSU ISTeC Cray HPC System supported by NSF Grant No. CNS-0923386 and the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation grant number ACI-1053575. This work also made use of the ARCHER UK National Supercomputing Service (http://www.archer.ac.uk), via the membership of the UK's HPC Materials Chemistry Consortium, which is funded by EPSRC (EP/L000202). The work at UCL was supported by EPSRC (EP/N01572X/1). D.O.S. acknowledges support from the SUPERSOLAR Solar Energy Hub (EP/J017361/1) for the provision of a flexible funding call award. A.M.G. acknowledges Diamond Light Source for the cosponsorship of a studentship on the EPSRC Centre for Doctoral Training in Molecular Modelling and Materials Science (EP/L015862/1). We gratefully acknowledge the support of NVIDIA Corporation with the donation of the Tesla K40 GPU used for this research. E.M.M. would like to thank U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences (contract DE-AC36- 08GO28308). NR 121 TC 3 Z9 3 U1 37 U2 71 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 13 PY 2016 VL 138 IS 27 BP 8453 EP 8464 DI 10.1021/jacs.6b03207 PG 12 WC Chemistry, Multidisciplinary SC Chemistry GA DR3HN UT WOS:000379794400028 PM 27284638 ER PT J AU Ye, R Yuan, B Zhao, J Ralston, WT Wu, CY Barin, EU Toste, FD Somorjai, GA AF Ye, Rong Yuan, Bing Zhao, Jie Ralston, Walter T. Wu, Chung-Yeh Barin, Ebru Unel Toste, F. Dean Somorjai, Gabor A. TI Metal Nanoparticles Catalyzed Selective Carbon-Carbon Bond Activation in the Liquid Phase SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID HYDROGENATION; HYDROGENOLYSIS; CYCLOPROPANE; PALLADIUM; CLEAVAGE; SIZE; VINYLCYCLOPROPANES; INSERTION; PLATINUM AB Understanding the C-C bond activation mechanism is essential for developing the selective production of hydrocarbons in the petroleum industry and for selective polymer decomposition. In this work, ring-opening reactions of cydopropane derivatives under hydrogen catalyzed by metal nanoparticles (NPs) in the liquid phase were studied. 40-atom rhodium (Rh) NPs, encapsulated by dendrimer molecules and supported in mesoporous silica, catalyzed the ring opening of cydopropylbenzene at room temperature under hydrogen in benzene, and the turnover frequency (TOF) was higher than other metals or the Rh homogeneous catalyst counterparts. Comparison of reactants with various substitution groups showed that electron donation on the three-membered ring boosted the TOF of ring opening. The linear products formed with 100% selectivity for ring opening of all reactants catalyzed by the Rh NP. Surface Rh(0) acted as the active site in the NP. The capping agent played an important role in the ring-opening reaction kinetics. Larger particle size tended to show higher TOF and smaller reaction activation energy for Rh NPs encapsulated in either dendrimer or poly(vinylpyrrolidone). The generation/size of dendrimer and surface group also affected the reaction rate and activation energy. C1 [Ye, Rong; Yuan, Bing; Zhao, Jie; Ralston, Walter T.; Wu, Chung-Yeh; Barin, Ebru Unel; Toste, F. Dean; Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Ye, Rong; Somorjai, Gabor A.] Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Toste, FD; Somorjai, GA (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Somorjai, GA (reprint author), Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM fdtoste@berkeley.edu; somorjai@berkeley.edu OI Ye, Rong/0000-0002-4171-5964 FU Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geological and Biosciences of the US DOE [DE-AC02-05CH11231] FX We acknowledge support from the Director, Office of Science, Office of Basic Energy Sciences, Division of Chemical Sciences, Geological and Biosciences of the US DOE under contract DE-AC02-05CH11231. We thank Dr. Kyungsu Na for the synthesis of mesoporous zeolite, and Dr. Joyce Rodrigues De Araujo for XPS fitting. We thank Profs. A. Paul Alivisatos and Peidong Yang for the use of TEM. We thank the Molecular Fondry of the Lawrance Berkeley National Laboratory (Proposal 3806) for using their facilities. NR 30 TC 3 Z9 3 U1 26 U2 57 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 13 PY 2016 VL 138 IS 27 BP 8533 EP 8537 DI 10.1021/jacs.6b03977 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA DR3HN UT WOS:000379794400037 PM 27322570 ER PT J AU Dembowski, M Olds, TA Pellegrini, KL Hoffmann, C Wang, XP Hickam, S He, JH Oliver, AG Burns, PC AF Dembowski, Mateusz Olds, Travis A. Pellegrini, Kristi L. Hoffmann, Christina Wang, Xiaoping Hickam, Sarah He, Junhong Oliver, Allen G. Burns, Peter C. TI Solution P-31 NMR Study of the Acid-Catalyzed Formation of a Highly Charged {U(24)Pp(12)} Nanocluster, [(UO2)(24)(O-2)(24)(P2O7)(12)](48-), and Its Structural Characterization in the Solid State Using Single-Crystal Neutron Diffraction SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID BOND-VALENCE PARAMETERS; POLYOXOMETALATE DIPHOSPHATE COMPLEXES; URANYL PEROXIDE NANOCLUSTERS; CAGE CLUSTERS; METAL CLUSTER; URANIUM; OXIDE AB The first neutron diffraction study of a single crystal containing uranyl peroxide nanoclusters is reported for pyrophosphate-functionalized Na44K6[(UO2)(24)(O-2)(24)(P2O7)(12)][IO3](2)center dot 140H(2)O (1). Relative to earlier X-ray studies, neutron diffraction provides superior information concerning the positions of H atoms and lighter counterions. Hydrogen positions have been assigned and reveal an extensive network of H-bonds; notably, most O atoms present in the anionic cluster accept H-bonds from surrounding H2O molecules, and none of the surface-bound O atoms are protonated. The D(4)h symmetry of the cage is consistent with the presence of six encapsulated K cations, which appear to stabilize the lower symmetry variant of this cluster. P-31 NMR measurements demonstrate retention of this symmetry in solution, while in situ P-31 NMR studies suggest an acid-catalyzed mechanism for the assembly of 1 across a wide range of pH values. C1 [Dembowski, Mateusz; Oliver, Allen G.; Burns, Peter C.] Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA. [Olds, Travis A.; Pellegrini, Kristi L.; Hickam, Sarah; Burns, Peter C.] Univ Notre Dame, Dept Civil & Environm Engn & Earth Sci, Notre Dame, IN 46556 USA. [Hoffmann, Christina; Wang, Xiaoping] Oak Ridge Natl Lab, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [He, Junhong] Oak Ridge Natl Lab, Instrument & Source Div, Oak Ridge, TN 37831 USA. RP Burns, PC (reprint author), Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA.; Burns, PC (reprint author), Univ Notre Dame, Dept Civil & Environm Engn & Earth Sci, Notre Dame, IN 46556 USA. EM pburns@nd.edu RI Wang, Xiaoping/E-8050-2012; hoffmann, christina/D-2292-2016 OI Wang, Xiaoping/0000-0001-7143-8112; hoffmann, christina/0000-0002-7222-5845 FU Materials Science of Actinides Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001089]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy [DE-AC05-00OR22725]; UT-Battelle, LLC FX This material is based upon work supported as a part of the Materials Science of Actinides Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. DE-SC0001089. NMR measurements were conducted at the Magnetic Resonance Research Center at the University of Notre Dame. Electrospray ionization mass spectra were collected at the Mass Spectrometry and Proteomics Facility at University of Notre Dame. Raman spectroscopy and thermogravimetric analysis measurements were collected at the Materials Characterization Facility of the Center for Sustainable Energy at the University of Notre Dame. Work performed at the ORNL Spallation Neutron Source's TOPAZ single-crystal diffractometer was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy, under Contract No. DE-AC05-00OR22725 with UT-Battelle, LLC. NR 32 TC 1 Z9 1 U1 19 U2 42 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 13 PY 2016 VL 138 IS 27 BP 8547 EP 8553 DI 10.1021/jacs.6b04028 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA DR3HN UT WOS:000379794400039 PM 27322657 ER PT J AU Ke, WJ Xiao, CX Wang, CL Saparov, B Duan, HS Zhao, DW Xiao, ZW Schulz, P Harvey, SP Liao, WQ Meng, WW Yu, Y Cimaroli, AJ Jiang, CS Zhu, K Al-Jassim, M Fang, GJ Mitzi, DB Yan, YF AF Ke, Weijun Xiao, Chuanxiao Wang, Changlei Saparov, Bayrammurad Duan, Hsin-Sheng Zhao, Dewei Xiao, Zewen Schulz, Philip Harvey, Steven P. Liao, Weiqiang Meng, Weiwei Yu, Yue Cimaroli, Alexander J. Jiang, Chun-Sheng Zhu, Kai Al-Jassim, Mowafak Fang, Guojia Mitzi, David B. Yan, Yanfa TI Employing Lead Thiocyanate Additive to Reduce the Hysteresis and Boost the Fill Factor of Planar Perovskite Solar Cells SO ADVANCED MATERIALS LA English DT Article ID ORGANOMETAL HALIDE PEROVSKITES; ELECTRON SELECTIVE LAYERS; AUGMENTED-WAVE METHOD; I-V HYSTERESIS; THIN-FILMS; ANOMALOUS HYSTERESIS; HYBRID MATERIALS; TIN OXIDE; EFFICIENT; PERFORMANCE AB Lead thiocyanate in the perovskite precursor can increase the grain size of a perovskite thin film and reduce the conductivity of the grain boundaries, leading to perovskite solar cells with reduced hysteresis and enhanced fill factor. A planar perovskite solar cell with grain boundary and interface passivation achieves a steady-state efficiency of 18.42%. C1 [Ke, Weijun; Wang, Changlei; Zhao, Dewei; Xiao, Zewen; Liao, Weiqiang; Meng, Weiwei; Yu, Yue; Cimaroli, Alexander J.; Yan, Yanfa] Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA. [Ke, Weijun; Wang, Changlei; Zhao, Dewei; Xiao, Zewen; Liao, Weiqiang; Meng, Weiwei; Yu, Yue; Cimaroli, Alexander J.; Yan, Yanfa] Univ Toledo, Wright Ctr Photovolta Innovat & Commercializat, 2801 W Bancroft St, Toledo, OH 43606 USA. [Ke, Weijun; Fang, Guojia] Wuhan Univ, Sch Phys & Technol, Minist Educ China, Key Lab Artificial Micro & Nanostruct, Wuhan 430072, Peoples R China. [Ke, Weijun; Xiao, Chuanxiao; Zhao, Dewei; Schulz, Philip; Harvey, Steven P.; Jiang, Chun-Sheng; Zhu, Kai; Al-Jassim, Mowafak] Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. [Saparov, Bayrammurad; Duan, Hsin-Sheng; Mitzi, David B.] Duke Univ, Dept Mech Engn & Mat Sci, Durham, NC 27708 USA. [Saparov, Bayrammurad; Mitzi, David B.] Duke Univ, Dept Chem, Durham, NC 27708 USA. RP Yan, YF (reprint author), Univ Toledo, Dept Phys & Astron, Toledo, OH 43606 USA.; Mitzi, DB; Yan, YF (reprint author), Univ Toledo, Wright Ctr Photovolta Innovat & Commercializat, 2801 W Bancroft St, Toledo, OH 43606 USA.; Fang, GJ (reprint author), Wuhan Univ, Sch Phys & Technol, Minist Educ China, Key Lab Artificial Micro & Nanostruct, Wuhan 430072, Peoples R China.; Mitzi, DB (reprint author), Duke Univ, Dept Mech Engn & Mat Sci, Durham, NC 27708 USA.; Mitzi, DB (reprint author), Duke Univ, Dept Chem, Durham, NC 27708 USA. EM gjfang@whu.edu.cn; david.mitzi@duke.edu; yanfa.yan@utoledo.edu RI Xiao, Zewen/B-3674-2015 OI Xiao, Zewen/0000-0002-4911-1399 FU Office of Energy Efficiency and Renewable Energy (EERE), U.S. Department of Energy [DE-EE0006712]; Ohio Research Scholar Program; National High Technology Research and Development Program [2015AA050601]; National Natural Science Foundation of China [61376013, 91433203, J1210061]; Fundamental Research Funds for the Central Universities [2014202020207]; U.S. Department of Energy SunShot Initiative under the Next Generation Photovoltaics 3 program [DE-FOA-0000990, DE-AC36-08-GO28308]; Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) Postdoctoral Research Award; DOE [DE-AC05-06OR23100]; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was funded in part by the Office of Energy Efficiency and Renewable Energy (EERE), U.S. Department of Energy, under Award Number DE-EE0006712 and the Ohio Research Scholar Program. W.J.K. and G.J.F acknowledge the support from the National High Technology Research and Development Program (Grant No. 2015AA050601), the National Natural Science Foundation of China (Grant Nos. 61376013, 91433203, and J1210061), and the Fundamental Research Funds for the Central Universities (Grant No. 2014202020207). The work at the National Renewable Energy Laboratory was supported by the U.S. Department of Energy SunShot Initiative under the Next Generation Photovoltaics 3 program (DE-FOA-0000990) under Contract No. DE-AC36-08-GO28308. B.S. acknowledges support from a Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy (EERE) Postdoctoral Research Award administered by the Oak Ridge Institute for Science and Education (ORISE) for the DOE. ORISE is managed by Oak Ridge Associated Universities (ORAU) under DOE Contract Number DE-AC05-06OR23100. This research used the resources of the Ohio Supercomputer Center and the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 70 TC 23 Z9 23 U1 90 U2 202 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD JUL 13 PY 2016 VL 28 IS 26 BP 5214 EP + DI 10.1002/adma.201600594 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DR5JH UT WOS:000379938800009 PM 27145346 ER PT J AU Xu, BB Luo, ZP Wilson, AJ Chen, K Gao, WX Yuan, GL Chopra, HD Chen, X Willets, KA Dauter, Z Ren, SQ AF Xu, Beibei Luo, Zhipu Wilson, Andrew J. Chen, Ke Gao, Wenxiu Yuan, Guoliang Chopra, Harsh Deep Chen, Xing Willets, Katherine A. Dauter, Zbigniew Ren, Shenqiang TI Multifunctional Charge-Transfer Single Crystals through Supramolecular Assembly SO ADVANCED MATERIALS LA English DT Article ID TETRACYANOQUINODIMETHANE TTF-TCNQ; TRANSFER COMPLEXES; TRANSFER INTERFACES; ELECTRON-TRANSFER; TRANSFER SALT; MULTIFERROICITY; FERROELECTRICITY; SEMICONDUCTOR; CONDUCTIVITY; MAGNETISM AB Centimeter-sized segregated stacking TTF-C-60 single crystals are crystallized by a mass-transport approach combined with solvent-vapor evaporation for the first time. The intermolecular charge-transfer interaction in the long-range ordered superstructure enables the crystals to demonstrate external stimuli-controlled multifunctionalities and angle/electrical-potential-dependent luminescence. C1 [Xu, Beibei; Chopra, Harsh Deep; Ren, Shenqiang] Temple Univ, Dept Mech Engn, Temple Mat Inst, Philadelphia, PA 19122 USA. [Luo, Zhipu; Dauter, Zbigniew] Argonne Natl Lab, Synchrotron Radiat Res Sect, Macromol Crystallog Lab, Natl Canc Inst, 9700 S Cass Ave, Argonne, IL 60439 USA. [Wilson, Andrew J.; Willets, Katherine A.] Temple Univ, Dept Chem, Philadelphia, PA 19122 USA. [Chen, Ke] Temple Univ, Dept Phys, Temple Mat Inst, Philadelphia, PA 19122 USA. [Gao, Wenxiu; Yuan, Guoliang] Nanjing Univ Sci Technol, Sch Mat Sci & Engn, Nanjing 210094, Jiangsu, Peoples R China. [Chen, Xing] Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Ren, SQ (reprint author), Temple Univ, Dept Mech Engn, Temple Mat Inst, Philadelphia, PA 19122 USA. EM shenqiang.ren@temple.edu OI Wilson, Andrew/0000-0003-3427-810X FU Army Research Office, Young Investigator Program [W911NF-15-1-0610]; U.S. Department of Energy, Basic Energy Sciences Award [DE-FG02-13ER46937]; Department of Energy (DOE), Office of Science, Basic Energy Science (BES) [DE-SC0010307]; National Science Foundation DMR , Condensed Matter Physics [1541236]; Temple University's OVPR's Infrastructure Grant; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [W-31-109-Eng-38] FX Work at Temple University (S.R.) was supported by the Army Research Office, Young Investigator Program (W911NF-15-1-0610, material design/self-assembly of carbon photovoltaics), and the U.S. Department of Energy, Basic Energy Sciences Award No. DE-FG02-13ER46937 (organic synthesis and physical property measurement). Work at Temple University (A.J.W. and K.A.W.) was supported by the Department of Energy (DOE), Office of Science, Basic Energy Science (BES) under Award No. DE-SC0010307. H.D.C. gratefully acknowledges support from the National Science Foundation DMR, Condensed Matter Physics under Grant No. 1541236 (previously Grant No. 1309712) and Temple University's OVPR's Infrastructure Grant. Diffraction data were collected at the SER-CAT beamline 22BM at the Advanced Photon Source, Argonne National Laboratory. Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. W-31-109-Eng-38. The authors also thank Temple Materials Institute and Dr. X. Xi for the AFM measurements. NR 48 TC 0 Z9 0 U1 24 U2 61 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD JUL 13 PY 2016 VL 28 IS 26 BP 5322 EP + DI 10.1002/adma.201600383 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DR5JH UT WOS:000379938800024 PM 27146726 ER PT J AU Ceriotti, M Fang, W Kusalik, PG McKenzie, RH Michaelides, A Morales, MA Markland, TE AF Ceriotti, Michele Fang, Wei Kusalik, Peter G. McKenzie, Ross H. Michaelides, Angelos Morales, Miguel A. Markland, Thomas E. TI Nuclear Quantum Effects in Water and Aqueous Systems: Experiment, Theory, and Current Challenges SO CHEMICAL REVIEWS LA English DT Review ID POLYMER MOLECULAR-DYNAMICS; TIME-CORRELATION-FUNCTIONS; PATH-INTEGRAL SIMULATIONS; DENSITY-FUNCTIONAL THEORY; POTENTIAL-ENERGY SURFACE; GRAPHICAL PROCESSING UNITS; THERMAL RATE CONSTANTS; VALENCE-BOND MODEL; LIQUID WATER; HYDROGEN-BOND AB Nuclear quantum effects influence the structure and dynamics of hydrogen-bonded systems, such as water, which impacts their observed properties with widely varying magnitudes. This review highlights the recent significant developments in the experiment, theory, and simulation of nuclear quantum effects in water. Novel experimental techniques, such as deep inelastic neutron scattering, now provide a detailed view of the role of nuclear quantum effects in water's properties. These have been combined with theoretical developments such as the introduction of the principle of competing quantum effects that allows the subtle interplay of water's quantum effects and their manifestation in experimental observables to be explained. We discuss how this principle has recently been used to explain the apparent dichotomy in water's isotope effects, which can range from very large to almost nonexistent depending on the property and conditions. We then review the latest major developments in simulation algorithms and theory that have enabled the efficient inclusion of nuclear quantum effects in molecular simulations, permitting their combination with on-the-fly evaluation of the potential energy surface using electronic structure theory. Finally, we identify current challenges and future opportunities in this area of research. C1 [Ceriotti, Michele] Ecole Polytech Fed Lausanne, Inst Mat, Lab Computat Sci & Modeling, CH-1015 Lausanne, Switzerland. [Fang, Wei; Michaelides, Angelos] UCL, London Ctr Nanotechnol, Thomas Young Ctr, London WC1E 6BT, England. [Fang, Wei; Michaelides, Angelos] UCL, Dept Phys & Astron, London WC1E 6BT, England. [Kusalik, Peter G.] Univ Calgary, Dept Chem, 2500 Univ Dr NW, Calgary, AB T2N 1N4, Canada. [McKenzie, Ross H.] Univ Queensland, Sch Math & Phys, Brisbane, Qld 4072, Australia. [Morales, Miguel A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Markland, Thomas E.] Stanford Univ, Dept Chem, 333 Campus Dr, Stanford, CA 94305 USA. RP Markland, TE (reprint author), Stanford Univ, Dept Chem, 333 Campus Dr, Stanford, CA 94305 USA. EM tmarkland@stanford.edu RI Ceriotti, Michele/C-2393-2009; McKenzie, Ross/D-8900-2013; OI Ceriotti, Michele/0000-0003-2571-2832; Michaelides, Angelos/0000-0002-9169-169X FU Royal Swedish Academy of Sciences through Nobel Institutes for Physics and Chemistry; Swedish Research Council; Department of Physics at Stockholm University; CCMX; Swiss National Science Foundation [200021-159896]; Natural Sciences and Engineering Research Council of Canada; European Research Council under the European Union's Seventh Framework Programme (FP)/ERC Grant [616121]; Royal Society through a Wolfson Research Merit Award; Predictive Theory and Modeling for Materials and Chemical Science program of the U.S. Department of Energy (U.S. DOE), Office of Science, Office of Basic Energy Sciences; U.S. DOE at Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.S. DOE, Office of Science, Office of Basic Energy Sciences [DE-SC0014437]; Cottrell Scholarship from the Research Corporation for Science Advancement; Alfred P. Sloan Research fellowship FX We thank Lars G. M. Pettersson, Lu Wang, and Ondrej Marsalek for providing insightful comments and suggestions for this review. This review was initiated during the Nordita (Nordic Institute for Theoretical Physics) scientific program "Water - the Most Anomalous Liquid". Additional financial support for this program was provided by the Royal Swedish Academy of Sciences through its Nobel Institutes for Physics and Chemistry, the Swedish Research Council, and the Department of Physics at Stockholm University. M.C. acknowledges funding from CCMX and the Swiss National Science Foundation (Project 200021-159896). P.G.K is grateful for the financial support of the Natural Sciences and Engineering Research Council of Canada. A.M. and W.F.'s work was supported by the European Research Council under the European Union's Seventh Framework Programme (FP/2007-2013)/ERC Grant Agreement 616121 (HeteroIce Project). A.M. was also supported by the Royal Society through a Wolfson Research Merit Award. M.A.M was supported by the Predictive Theory and Modeling for Materials and Chemical Science program of the U.S. Department of Energy (U.S. DOE), Office of Science, Office of Basic Energy Sciences, and by the U.S. DOE at Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. T.E.M. was supported by the U.S. DOE, Office of Science, Office of Basic Energy Sciences, under Award DE-SC0014437. T.E.M. also acknowledges support from a Cottrell Scholarship from the Research Corporation for Science Advancement and an Alfred P. Sloan Research fellowship. NR 278 TC 23 Z9 23 U1 24 U2 52 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0009-2665 EI 1520-6890 J9 CHEM REV JI Chem. Rev. PD JUL 13 PY 2016 VL 116 IS 13 BP 7529 EP 7550 DI 10.1021/acs.chemrev.5b00674 PG 22 WC Chemistry, Multidisciplinary SC Chemistry GA DR3HJ UT WOS:000379794000004 PM 27049513 ER PT J AU Bellissent-Funel, MC Hassanali, A Havenith, M Henchman, R Pohl, P Sterpone, F van der Spoel, D Xu, Y Garcia, AE AF Bellissent-Funel, Marie-Claire Hassanali, Ali Havenith, Martina Henchman, Richard Pohl, Peter Sterpone, Fabio van der Spoel, David Xu, Yao Garcia, Angel E. TI Water Determines the Structure and Dynamics of Proteins SO CHEMICAL REVIEWS LA English DT Review ID ANGLE NEUTRON-SCATTERING; TRP-CAGE MINIPROTEIN; FOLDING FREE-ENERGY; HIGH-PRESSURE CRYSTALLOGRAPHY; GREEN FLUORESCENCE PROTEIN; CAVITY-CREATING MUTATIONS; POLARIZABLE FORCE-FIELD; 3-HELIX BUNDLE PROTEIN; HELIX-COIL TRANSITION; MOLAR HEAT-CAPACITY AB Water is an essential participant in the stability, structure, dynamics, and function of proteins and other biomolecules. Thermodynamically, changes in the aqueous environment affect the stability of biomolecules. Structurally, water participates chemically in the catalytic function of proteins and nucleic acids and physically in the collapse of the protein chain during folding through hydrophobic collapse and mediates binding through the hydrogen bond in complex formation. Water is a partner that slaves the dynamics of proteins, and water interaction with proteins affect their dynamics. Here we provide a review of the experimental and computational advances over the past decade in understanding the role of water in the dynamics, structure, and function of proteins. We focus on the combination of X-ray and neutron crystallography, NMR, terahertz spectroscopy, mass spectroscopy, thermodynamics, and computer simulations to reveal how water assist proteins in their function. The recent advances in computer simulations and the enhanced sensitivity of experimental tools promise major advances in the understanding of protein dynamics, and water surely will be a protagonist. C1 [Bellissent-Funel, Marie-Claire] CEA Saclay, CNRS, Lab Leon Brillouin, F-91191 Gif Sur Yvette, France. [Hassanali, Ali] Abdus Salaam Int Ctr Theoret Phys, Condensed Matter & Stat Phys, I-34151 Trieste, Italy. [Havenith, Martina; Xu, Yao] Ruhr Univ Bochum, Fac Chem & Biochem, Univ Str 150 Bldg NC 7-72, D-44780 Bochum, Germany. [Henchman, Richard] Univ Manchester, Manchester Inst Biotechnol, 131 Princess St, Manchester M1 7DN, Lancs, England. [Pohl, Peter] Johannes Kepler Univ Linz, Gruberstr 40, A-4020 Linz, Austria. [Sterpone, Fabio] Inst Biol Physicochim, Lab Biochim Theor, 13 Rue Pierre & Marie Curie, F-75005 Paris, France. [van der Spoel, David] Uppsala Univ, Dept Cell & Mol Biol Computat & Syst Biol, S-75124 Uppsala, Sweden. [Garcia, Angel E.] Los Alamos Natl Lab, Ctr Non Linear Studies, Los Alamos, NM 87545 USA. RP Garcia, AE (reprint author), Los Alamos Natl Lab, Ctr Non Linear Studies, Los Alamos, NM 87545 USA. EM angel@rpi.edu RI Pohl, Peter/A-5361-2008; van der Spoel, David/A-5471-2008 OI Pohl, Peter/0000-0002-1792-2314; van der Spoel, David/0000-0002-7659-8526 FU National Science Foundation in the USA [MCB-1050966]; Austrian Science Fund (FWF) [P23679]; European Research Council (ERC) under the European Community [258748]; Los Alamos National Laboratory LDRD funds; Royal Swedish Academy of Sciences through its Nobel Institutes for Physics and Chemistry; Swedish Research Council; Department of Physics at Stockholm University FX This work was supported by the National Science Foundation in the USA (MCB-1050966 to AEG) and the Austrian Science Fund (FWF, Grant P23679 to P.P.). F.S. acknowledges funding from the European Research Council (ERC) under the European Community's Seventh Framework Programme (FP7/2007-2013), Grant 258748. A.E.G. acknowledges support from Los Alamos National Laboratory LDRD funds. This review was initiated during the NORDITA (Nordic Institute for Theoretical Physics) scientific program "Water - the Most Anomalous Liquid". Additional financial support for this program was provided by the Royal Swedish Academy of Sciences through its Nobel Institutes for Physics and Chemistry, by the Swedish Research Council, and by the Department of Physics at Stockholm University. NR 312 TC 24 Z9 24 U1 86 U2 160 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0009-2665 EI 1520-6890 J9 CHEM REV JI Chem. Rev. PD JUL 13 PY 2016 VL 116 IS 13 BP 7673 EP 7697 DI 10.1021/acs.chemrev.5b00664 PG 25 WC Chemistry, Multidisciplinary SC Chemistry GA DR3HJ UT WOS:000379794000011 PM 27186992 ER PT J AU Bjornehohn, E Hansen, MH Hodgson, A Liu, LM Limmer, DT Michaelides, A Pedevilla, P Rossmeisl, J Shen, H Tocci, G Tyrode, E Walz, MM Werner, J Bluhm, H AF Bjornehohn, E. Hansen, Martin H. Hodgson, Andrew Liu, Li-Min Limmer, David T. Michaelides, Angelos Pedevilla, Philipp Rossmeisl, Jan Shen, Huaze Tocci, Gabriele Tyrode, Eric Walz, Marie-Madeleine Werner, Josephina Bluhm, Hendrik TI Water at Interfaces SO CHEMICAL REVIEWS LA English DT Review ID DENSITY-FUNCTIONAL THEORY; SUM-FREQUENCY SPECTROSCOPY; MOLECULAR-DYNAMICS SIMULATIONS; RAY PHOTOELECTRON-SPECTROSCOPY; NEAR-AMBIENT CONDITIONS; SITU X-RAY; SURFACE-ADSORPTION LAYERS; LIQUID-VAPOR INTERFACE; METAL-SURFACES; AQUEOUS-SOLUTION AB The interfaces of neat water and aqueous solutions play a prominent role in many technological processes and in the environment. Examples of aqueous interfaces are ultrathin water films that cover most hydrophilic surfaces under ambient relative humidities, the liquid/solid interface which drives many electrochemical reactions, and the liquid/vapor interface, which governs the uptake and release of trace gases by the oceans and cloud droplets. In this article we review some of the recent experimental and theoretical advances in our knowledge of the properties of aqueous interfaces and discuss open questions and gaps in our understanding. C1 [Bjornehohn, E.; Walz, Marie-Madeleine; Werner, Josephina] Uppsala Univ, Dept Phys & Astron, BOX 516, S-75120 Uppsala, Sweden. [Hansen, Martin H.] Tech Univ Denmark, DK-2800 Lyngby, Denmark. [Hodgson, Andrew] Univ Liverpool, Dept Chem, Liverpool L69 7ZD, Merseyside, England. [Liu, Li-Min; Michaelides, Angelos; Pedevilla, Philipp; Tocci, Gabriele] UCL, London Ctr Nanotechnol, Thomas Young Ctr, Dept Phys & Astron, London WC1E 6BT, England. [Liu, Li-Min; Michaelides, Angelos; Pedevilla, Philipp; Tocci, Gabriele] UCL, Dept Chem, London WC1E 6BT, England. [Liu, Li-Min] Beijing Computat Sci Res Ctr, Beijing 100193, Peoples R China. [Limmer, David T.] Princeton Univ, Princeton Ctr Theoret Sci, Princeton, NJ 08544 USA. [Hansen, Martin H.; Rossmeisl, Jan] Univ Copenhagen, Dept Chem, Univ Pk 5, DK-2100 Copenhagen, Denmark. [Shen, Huaze] Peking Univ, Int Ctr Quantum Mat, Beijing 100871, Peoples R China. [Shen, Huaze] Peking Univ, Sch Phys, Beijing 100871, Peoples R China. [Tyrode, Eric] KTH Royal Inst Technol, Dept Chem, S-10044 Stockholm, Sweden. [Werner, Josephina] Swedish Univ Agr Sci, Dept Chem & Biotechnol, Box 7015, S-75007 Uppsala, Sweden. [Bluhm, Hendrik] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Tocci, Gabriele] Ecole Polytech Fed Lausanne, Sch Engn, Inst Bioengn & Mat Sci & Engn, Lab Fundamental BioPhoton,Lab Computat Sci & Mode, CH-1015 Lausanne, Switzerland. [Tocci, Gabriele] Ecole Polytech Fed Lausanne, Lausanne Ctr Ultrafast Sci, CH-1015 Lausanne, Switzerland. [Walz, Marie-Madeleine] Uppsala Univ, Dept Cell & Mol Biol, Box 596, SE-75124 Uppsala, Sweden. RP Bluhm, H (reprint author), Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM HBluhm@lbl.gov RI Liu, Li-Min/A-7051-2010; Rossmeisl, Jan/A-5714-2011; OI Liu, Li-Min/0000-0003-3925-5310; Rossmeisl, Jan/0000-0001-7749-6567; Werner, Josephina/0000-0002-1532-9920; Michaelides, Angelos/0000-0002-9169-169X FU Royal Swedish Academy of Sciences through its Nobel Institutes for Physics and Chemistry; Swedish Research Council; Department of Physics at Stockholm University; Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231]; European Research Council under the European Union [616121]; Royal Society through a Wolfson Research Merit Award; Swedish Research Council (VR); Swedish Foundation for Strategic Research (SSF-Future Research Leaders program); Carl Tryggers foundation FX This review was initiated during the Nordita (Nordic Institute for Theoretical Physics) scientific program "Water - the Most Anomalous Liquid". Additional financial support for this program was provided by the Royal Swedish Academy of Sciences through its Nobel Institutes for Physics and Chemistry, by the Swedish Research Council, and by the Department of Physics at Stockholm University. H.B. acknowledges support by the Director, Office of Science, Office of Basic Energy Sciences, and by the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL under Contract No. DE-AC02-05CH11231. A.M. and P.P.'s work is supported by the European Research Council under the European Union's Seventh Framework Programme (FP/2007-2013)/ERC Grant Agreement No. 616121 (Hetero-Ice project). A.M. is also supported by the Royal Society through a Wolfson Research Merit Award. E.T. acknowledges support from the Swedish Research Council (VR) and the Swedish Foundation for Strategic Research (SSF-Future Research Leaders program). Financial support from the Carl Tryggers foundation is gratefully acknowledged (M.-M.W.). NR 298 TC 12 Z9 12 U1 92 U2 155 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0009-2665 EI 1520-6890 J9 CHEM REV JI Chem. Rev. PD JUL 13 PY 2016 VL 116 IS 13 BP 7698 EP 7726 DI 10.1021/acs.chemrev.6b00045 PG 29 WC Chemistry, Multidisciplinary SC Chemistry GA DR3HJ UT WOS:000379794000012 ER PT J AU Tan, GT Song, Y Zhang, CL Lin, LF Xu, Z Hou, TT Tian, W Cao, HB Li, SL Feng, SP Dai, PC AF Tan, Guotai Song, Yu Zhang, Chenglin Lin, Lifang Xu, Zhuang Hou, Tingting Tian, Wei Cao, Huibo Li, Shiliang Feng, Shiping Dai, Pengcheng TI Electron doping evolution of structural and antiferromagnetic phase transitions in NaFe1-xCoxAs iron pnictides SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM CRITICAL-POINT; SUPERCONDUCTIVITY; ORDER AB We use transport and neutron diffraction to study the electronic phase diagram of NaFe1-xCox As. In the undoped state, NaFeAs exhibits a tetragonal-to-orthorhombic structural transition below T-s followed by a collinear antiferromagnetic (AF) order below T-N. Upon codoping to form NaFe1-xCox As, T-s and T-N are gradually suppressed, leading to optimal superconductivity near Co-doping x = 0.025. While transport experiments on these materials reveal an anomalous behavior suggesting the presence of a quantum critical point (QCP) near optimal superconductivity, our neutron diffraction results indicate that commensurate AF order becomes transversely incommensurate with T-N > T-c before vanishing abruptly at optimal superconductivity. These results are remarkably similar to electron-doping and isovalent-doping evolution of the AF order in BaFe2-xNixAs2 and BaFe2(As1-xPx)(2), thus suggesting a universal behavior in the suppression of the magnetic order in iron pnictides as superconductivity is induced. C1 [Tan, Guotai; Lin, Lifang; Xu, Zhuang; Hou, Tingting; Feng, Shiping; Dai, Pengcheng] Beijing Normal Univ, Dept Phys, Beijing 100875, Peoples R China. [Song, Yu; Zhang, Chenglin; Dai, Pengcheng] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. [Tian, Wei; Cao, Huibo] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Li, Shiliang] Chinese Acad Sci, Inst Phys, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Li, Shiliang] Collaborat Innovat Ctr Quantum Matter, Beijing, Peoples R China. RP Dai, PC (reprint author), Beijing Normal Univ, Dept Phys, Beijing 100875, Peoples R China.; Dai, PC (reprint author), Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA. EM pdai@rice.edu RI Dai, Pengcheng /C-9171-2012; Tian, Wei/C-8604-2013; Li, Shiliang/B-9379-2009 OI Dai, Pengcheng /0000-0002-6088-3170; Tian, Wei/0000-0001-7735-3187; FU United States DOE, BES [DE-SC0012311]; Robert A. Welch Foundation [C-1839]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; National Basic Research Program of China (973 Program) [2012CB821401]; National Natural Science Foundation of China [11374011]; Fundamental Research Funds for the Central Universities [2014KJJCB27] FX The single-crystal growth efforts and neutron scattering work at Rice are supported by the United States DOE, BES, through Contract No. DE-SC0012311 (P.D.). Part of the materials work at Rice University is supported by the Robert A. Welch Foundation through Grant No. C-1839 (P.D.). The neutron scattering work at ORNLs HFIR is sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. Transport measurements are supported by the National Basic Research Program of China (973 Program, Grant No. 2012CB821401), the National Natural Science Foundation of China (Grant No. 11374011), and the Fundamental Research Funds for the Central Universities (Grant No. 2014KJJCB27). NR 50 TC 2 Z9 2 U1 11 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 13 PY 2016 VL 94 IS 1 AR 014509 DI 10.1103/PhysRevB.94.014509 PG 6 WC Physics, Condensed Matter SC Physics GA DQ8YR UT WOS:000379498100007 ER PT J AU Briceno, RA Hansen, MT AF Briceno, Raul A. Hansen, Maxwell T. TI Relativistic, model-independent, multichannel 2 -> 2 transition amplitudes in a finite volume SO PHYSICAL REVIEW D LA English DT Article ID PROTON-PROTON-SCATTERING; PARITY VIOLATION; LATTICE QCD; MATRIX-ELEMENTS; FIELD THEORIES; FORM-FACTORS; GAMMA; STATES; NONCONSERVATION; CONSERVATION AB We derive formalism for determining 2 + J -> 2 infinite-volume transition amplitudes from finite-volume matrix elements. Specifically, we present a relativistic, model-independent relation between finite-volume matrix elements of external currents and the physically observable infinite-volume matrix elements involving two-particle asymptotic states. The result presented holds for states composed of two scalar bosons. These can be identical or nonidentical and, in the latter case, can be either degenerate or nondegenerate. We further accommodate any number of strongly coupled two-scalar channels. This formalism will, for example, allow future lattice QCD calculations of the p-meson form factor, in which the unstable nature of the p is rigorously accommodated. C1 [Briceno, Raul A.] Thomas Jefferson Natl Accelerator Facil, 12000 Jefferson Ave, Newport News, VA 23606 USA. [Hansen, Maxwell T.] Johannes Gutenberg Univ Mainz, Inst Kernphys, D-55099 Mainz, Germany. [Hansen, Maxwell T.] Johannes Gutenberg Univ Mainz, Helmholz Inst Mainz, D-55099 Mainz, Germany. RP Briceno, RA (reprint author), Thomas Jefferson Natl Accelerator Facil, 12000 Jefferson Ave, Newport News, VA 23606 USA.; Hansen, MT (reprint author), Johannes Gutenberg Univ Mainz, Inst Kernphys, D-55099 Mainz, Germany.; Hansen, MT (reprint author), Johannes Gutenberg Univ Mainz, Helmholz Inst Mainz, D-55099 Mainz, Germany. EM rbriceno@jlab.org; hansen@kph.uni-mainz.de FU U.S. Department of Energy [DE-AC05-06OR23177] FX R. B. acknowledges support from the U.S. Department of Energy Contract No. DE-AC05-06OR23177, under which Jefferson Science Associates, LLC, manages and operates the Jefferson Lab. The authors would like to thank David Wilson, Christian Shultz and Andre Walker-Loud for useful discussions and Steve Sharpe for very helpful comments on the manuscript. M. T. H. would also like to thank Dalibor Djukanovic, Parikshit Junnarkar, and Harvey Meyer for useful discussions. NR 80 TC 1 Z9 1 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 13 PY 2016 VL 94 IS 1 AR 013008 DI 10.1103/PhysRevD.94.013008 PG 36 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DR0CK UT WOS:000379575400002 ER PT J AU Meinel, S van Dyk, D AF Meinel, Stefan van Dyk, Danny TI Using Lambda(b) -> Lambda mu(+)mu(-) data within a Bayesian analysis of vertical bar Delta B vertical bar = vertical bar Delta S vertical bar=1 decays SO PHYSICAL REVIEW D LA English DT Article ID PHYSICS; RARE AB We study the impact of including the baryonic decay Lambda(b) -> Lambda(-> p pi(-))mu(+)mu(-) in a Bayesian analysis of vertical bar Delta B vertical bar = vertical bar Delta S vertical bar = 1 transitions. We perform fits of the Wilson coefficients C-9, C-9', C-10 and C-10', in addition to the relevant nuisance parameters. Our analysis combines data for the differential branching fraction and three angular observables of Lambda(b) -> Lambda(-> p pi(-))mu(+)mu(-) with data for the branching ratios of B-s -> mu(+)mu(-) and inclusive b -> sl(+)l(-) decays. Newly available precise lattice QCD results for the full set of Lambda(b) -> Lambda form factors are used to evaluate the observables of the baryonic decay. Our fits prefer shifts to C-9 that are opposite in sign compared to those found in global fits of only mesonic decays, and the posterior odds show no evidence of physics beyond the Standard Model. We investigate a possible hadronic origin of the observed tensions between theory and experiment. C1 [Meinel, Stefan] Univ Arizona, Dept Phys, Tucson, AZ 85721 USA. [Meinel, Stefan] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [van Dyk, Danny] Univ Zurich, Inst Phys, Winterthurer Str 190, CH-8057 Zurich, Switzerland. RP Meinel, S (reprint author), Univ Arizona, Dept Phys, Tucson, AZ 85721 USA.; Meinel, S (reprint author), Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA.; van Dyk, D (reprint author), Univ Zurich, Inst Phys, Winterthurer Str 190, CH-8057 Zurich, Switzerland. EM smeinel@email.arizona.edu; dvandyk@physik.uzh.ch FU National Science Foundation [PHY-1520996]; RHIC Physics Fellow Program of the RIKEN BNL Research Center; Swiss National Science Foundation [PP00P2-144674] FX The work of S. M. is supported by National Science Foundation Grant No. PHY-1520996, and by the RHIC Physics Fellow Program of the RIKEN BNL Research Center. The work of D. v. D. is supported by Swiss National Science Foundation Grant No. PP00P2-144674. We thank Christoph Bobeth, Joaquim Matias, Luca Silvestrini, and Roman Zwicky for the useful comments on our preliminary results that were presented during the "4th Workshop on Implications of LHCb Measurements and Future Prospects." NR 46 TC 3 Z9 3 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 13 PY 2016 VL 94 IS 1 AR 013007 DI 10.1103/PhysRevD.94.013007 PG 10 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DR0CK UT WOS:000379575400001 ER PT J AU Taufour, V Kaluarachchi, US Khasanov, R Nguyen, MC Guguchia, Z Biswas, PK Bonfa, P De Renzi, R Lin, X Kim, SK Mun, ED Kim, H Furukawa, Y Wang, CZ Ho, KM Bud'ko, SL Canfield, PC AF Taufour, Valentin Kaluarachchi, Udhara S. Khasanov, Rustem Manh Cuong Nguyen Guguchia, Zurab Biswas, Pabitra Kumar Bonfa, Pietro De Renzi, Roberto Lin, Xiao Kim, Stella K. Mun, Eun Deok Kim, Hyunsoo Furukawa, Yuji Wang, Cai-Zhuang Ho, Kai-Ming Bud'ko, Sergey L. Canfield, Paul C. TI Ferromagnetic Quantum Critical Point Avoided by the Appearance of Another Magnetic Phase in LaCrGe3 under Pressure SO PHYSICAL REVIEW LETTERS LA English DT Article ID SUPERCONDUCTIVITY; GPA; SUSCEPTIBILITY; RESISTIVITY; TRANSITIONS; DEPENDENCE; BEHAVIOR; SYSTEMS; METALS; ENERGY AB The temperature-pressure phase diagram of the ferromagnet LaCrGe3 is determined for the first time from a combination of magnetization, muon-spin-rotation, and electrical resistivity measurements. The ferromagnetic phase is suppressed near 2.1 GPa, but quantum criticality is avoided by the appearance of a magnetic phase, likely modulated, AFM(Q). Our density functional theory total energy calculations suggest a near degeneracy of antiferromagnetic states with small magnetic wave vectors Q allowing for the potential of an ordering wave vector evolving from Q = 0 to finite Q, as expected from the most recent theories on ferromagnetic quantum criticality. Our findings show that LaCrGe3 is a very simple example to study this scenario of avoided ferromagnetic quantum criticality and will inspire further study on this material and other itinerant ferromagnets. C1 [Taufour, Valentin; Kaluarachchi, Udhara S.; Manh Cuong Nguyen; Kim, Stella K.; Furukawa, Yuji; Wang, Cai-Zhuang; Ho, Kai-Ming; Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, US Dept Energy, Ames Lab, Ames, IA 50011 USA. [Kaluarachchi, Udhara S.; Lin, Xiao; Kim, Stella K.; Mun, Eun Deok; Kim, Hyunsoo; Furukawa, Yuji; Ho, Kai-Ming; Bud'ko, Sergey L.; Canfield, Paul C.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Khasanov, Rustem; Guguchia, Zurab] Paul Scherrer Inst, Lab Muon Spin Spect, CH-5232 Villigen, Switzerland. [Biswas, Pabitra Kumar] STFC Rutherford Appleton Lab, ISIS Pulsed Neutron & Muon Source, Harwell Campus, Didcot OX11 0QX, Oxon, England. [Bonfa, Pietro] Dipartimento Fis & Sci Terra, Parco Area Sci 7-A, I-43124 Parma, Italy. RP Taufour, V (reprint author), Iowa State Univ, US Dept Energy, Ames Lab, Ames, IA 50011 USA. EM taufour@ameslab.gov RI Nguyen, Manh Cuong/G-2783-2015; De Renzi, Roberto/F-9182-2011; OI Nguyen, Manh Cuong/0000-0001-8027-9029; De Renzi, Roberto/0000-0002-5015-0061; Khasanov, Rustem/0000-0002-4768-5524 FU Materials Sciences Division of the Office of Basic Energy Sciences of the U.S. Department of Energy; Ames Laboratory, U.S. Department of Energy [DE-AC02-07CH11358]; Ames Laboratory's Laboratory-Directed Research and Development (LDRD) funding; AFOSR-MURI Grant [FA9550-09-1-0603] FX We would like to thank V. G. Kogan, A. Kreyssig, P. Kumar, and D. K. Finnemore for useful discussions, as well as D. Belitz, T. R. Kirkpatrick, F. Kruger, and A. G. Green for their critical reading of the manuscript. This work was supported by the Materials Sciences Division of the Office of Basic Energy Sciences of the U.S. Department of Energy. Part of this work was performed at the Ames Laboratory, U.S. Department of Energy, under Contract No. DE-AC02-07CH11358. Magnetization measurements under pressure (V. T.) were supported by Ames Laboratory's Laboratory-Directed Research and Development (LDRD) funding. X. L., E. D. M., and H. K. were supported by the AFOSR-MURI Grant No. FA9550-09-1-0603. NR 58 TC 0 Z9 0 U1 19 U2 29 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 13 PY 2016 VL 117 IS 3 AR 037207 DI 10.1103/PhysRevLett.117.037207 PG 6 WC Physics, Multidisciplinary SC Physics GA DR0DM UT WOS:000379578200002 PM 27472137 ER PT J AU Greene, AC Henderson, IM Gomez, A Paxton, WF VanDelinder, V Bachand, GD AF Greene, Adrienne C. Henderson, Ian M. Gomez, Andrew Paxton, Walter F. VanDelinder, Virginia Bachand, George D. TI The Role of Membrane Fluidization in the Gel-Assisted Formation of Giant Polymersomes SO PLOS ONE LA English DT Article ID UNILAMELLAR VESICLES; DRUG-DELIVERY; MODEL SYSTEMS; LIPOSOMES; COPOLYMERS; NETWORKS; FILMS AB Polymersomes are being widely explored as synthetic analogs of lipid vesicles based on their enhanced stability and potential uses in a wide variety of applications in (e.g., drug delivery, cell analogs, etc.). Controlled formation of giant polymersomes for use in membrane studies and cell mimetic systems, however, is currently limited by low-yield production methodologies. Here, we describe for the first time, how the size distribution of giant poly(ethylene glycol)-poly(butadiene) (PEO-PBD) polymersomes formed by gel-assisted rehydration may be controlled based on membrane fluidization. We first show that the average diameter and size distribution of PEO-PBD polymersomes may be readily increased by increasing the temperature of the rehydration solution. Further, we describe a correlative relationship between polymersome size and membrane fluidization through the addition of sucrose during rehydration, enabling the formation of PEO-PBD polymersomes with a range of diameters, including giant-sized vesicles (>100 mu m). This correlative relationship suggests that sucrose may function as a small molecule fluidizer during rehydration, enhancing polymer diffusivity during formation and increasing polymersome size. Overall the ability to easily regulate the size of PEO-PBD polymersomes based on membrane fluidity, either through temperature or fluidizers, has broadly applicability in areas including targeted therapeutic delivery and synthetic biology. C1 [Greene, Adrienne C.; Henderson, Ian M.; Paxton, Walter F.; VanDelinder, Virginia; Bachand, George D.] Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. [Gomez, Andrew] Sandia Natl Labs, Ctr Mat Sci & Engn, Albuquerque, NM USA. RP Bachand, GD (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM gdbacha@sandia.gov OI Greene, Adrienne/0000-0003-0270-3351; Bachand, George/0000-0002-3169-9980 FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (BES-MSE); U.S. Department of Energy (DOE) Office of Science [RA2015A0004]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering (BES-MSE). The funder provided support in the form of salaries for authors [ACG, AG, WFP, GDB], but did not have any additional role in the study design, data collection and analysis, decision to publish, or preparation of the manuscript. The specific roles of these authors are articulated in the 'author contributions' section. This work was performed, in part, at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science (user project number RA2015A0004). The funder provided support in the form of salaries for authors [IMH and VV], but did not have any additional role in the study design, data collection and analysis, decision to publish, or preparation of the manuscript. The specific roles of these authors are articulated in the 'author contributions' section. This does not alter the authors' adherence to PLOS ONE policies on sharing data and materials. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 37 TC 1 Z9 1 U1 8 U2 11 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUL 13 PY 2016 VL 11 IS 7 AR e0158729 DI 10.1371/journal.pone.0158729 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DQ9CP UT WOS:000379508300033 PM 27410487 ER PT J AU Iandiorio, MJ Fair, JM Chatzipanagiotou, S Ioannidis, A Trikka-Graphakos, E Charalampaki, N Sereti, C Tegos, GP Hoogesteijn, AL Rivas, AL AF Iandiorio, Michelle J. Fair, Jeanne M. Chatzipanagiotou, Stylianos Ioannidis, Anastasios Trikka-Graphakos, Eleftheria Charalampaki, Nikoletta Sereti, Christina Tegos, George P. Hoogesteijn, Almira L. Rivas, Ariel L. TI Preventing Data Ambiguity in Infectious Diseases with Four-Dimensional and Personalized Evaluations SO PLOS ONE LA English DT Article ID RESISTANT STAPHYLOCOCCUS-AUREUS; SYSTEMS BIOLOGY; IN-VITRO; EMERGENCE; CHALLENGES; IMMUNITY; MODELS; HETEROGENEITY; HOMEOSTASIS; UNFOLDOMICS AB Background Diagnostic errors can occur, in infectious diseases, when anti-microbial immune responses involve several temporal scales. When responses span from nanosecond to week and larger temporal scales, any pre-selected temporal scale is likely to miss some (faster or slower) responses. Hoping to prevent diagnostic errors, a pilot study was conducted to evaluate a four-dimensional (4D) method that captures the complexity and dynamics of infectious diseases. Methods Leukocyte-microbial-temporal data were explored in canine and human (bacterial and/or viral) infections, with: (i) a non-structured approach, which measures leukocytes or microbes in isolation; and (ii) a structured method that assesses numerous combinations of interacting variables. Four alternatives of the structured method were tested: (i) a noise-reduction oriented version, which generates a single (one data point-wide) line of observations; (ii) a version that measures complex, three-dimensional (3D) data interactions; (iii) a non-numerical version that displays temporal data directionality (arrows that connect pairs of consecutive observations); and (iv) a full 4D (single line-, complexity-, directionality-based) version. Results In all studies, the non-structured approach revealed non-interpretable ( ambiguous) data: observations numerically similar expressed different biological conditions, such as recovery and lack of recovery from infections. Ambiguity was also found when the data were structured as single lines. In contrast, two or more data subsets were distinguished and ambiguity was avoided when the data were structured as complex, 3D, single lines and, in addition, temporal data directionality was determined. The 4D method detected, even within one day, changes in immune profiles that occurred after antibiotics were prescribed. Conclusions Infectious disease data may be ambiguous. Four-dimensional methods may prevent ambiguity, providing earlier, in vivo, dynamic, complex, and personalized information that facilitates both diagnostics and selection or evaluation of anti-microbial therapies. C1 [Iandiorio, Michelle J.; Rivas, Ariel L.] Univ New Mexico, Sch Med, Dept Internal Med, Albuquerque, NM 87131 USA. [Fair, Jeanne M.] Los Alamos Natl Lab, Global Secur, Mailstop M888, Los Alamos, NM 87545 USA. [Chatzipanagiotou, Stylianos] Univ Athens, Sch Med, Aeginition Hosp, Dept Biopathol & Clin Microbiol, Athens, Greece. [Ioannidis, Anastasios] Univ Peloponnese, Fac Human Movement & Qual Life Sci, Dept Nursing, Sparta, Greece. [Trikka-Graphakos, Eleftheria; Charalampaki, Nikoletta; Sereti, Christina] Thriasio Gen Hosp, Dept Clin Microbiol, Magoula, Greece. [Tegos, George P.] Torrey Pines Inst Mol Studies, Port St Lucie, FL USA. [Tegos, George P.] Harvard Med Sch, Dept Dermatol, Boston, MA USA. [Tegos, George P.] Massachusetts Gen Hosp, Wellman Ctr Photomed, Boston, MA 02114 USA. [Hoogesteijn, Almira L.] Ctr Invest Avanzadas, Dept Human Ecol, Merida, Mexico. [Rivas, Ariel L.] Univ New Mexico, Sch Med, Ctr Global Hlth, Div Infect Dis, Albuquerque, NM 87131 USA. RP Rivas, AL (reprint author), Univ New Mexico, Sch Med, Dept Internal Med, Albuquerque, NM 87131 USA.; Rivas, AL (reprint author), Univ New Mexico, Sch Med, Ctr Global Hlth, Div Infect Dis, Albuquerque, NM 87131 USA. EM alrivas@unm.edu NR 58 TC 0 Z9 0 U1 4 U2 4 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUL 13 PY 2016 VL 11 IS 7 AR e0159001 DI 10.1371/journal.pone.0159001 PG 19 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DQ9CP UT WOS:000379508300047 PM 27411058 ER PT J AU Zhang, W Liu, Y Jackson, AC Savage, AM Ertem, SP Tsai, TH Seifert, S Beyer, FL Liberatore, MW Herring, AM Coughlin, EB AF Zhang, Wenxu Liu, Ye Jackson, Aaron C. Savage, Alice M. Ertem, S. Piril Tsai, Tsung-Han Seifert, Soenke Beyer, Frederick L. Liberatore, Matthew W. Herring, Andrew M. Coughlin, E. Bryan TI Achieving Continuous Anion Transport Domains Using Block Copolymers Containing Phosphonium Cations SO MACROMOLECULES LA English DT Article ID FUEL-CELL APPLICATIONS; POLYMER ELECTROLYTE MEMBRANES; CHAIN TRANSFER POLYMERIZATION; HYDROXIDE EXCHANGE MEMBRANES; ABA TRIBLOCK COPOLYMERS; PHASE-BEHAVIOR; BUTYL ACRYLATE; IONIC LIQUIDS; FUNCTIONALIZED POLYETHYLENE; RADICAL POLYMERIZATION AB Triblock and diblock copolymers based on isoprene (Ip) and chloromethylstyrene (CMS) were synthesized by sequential polymerization using reversible addition-fragmentation chain transfer radical polymerization (RAFT). The block copolymers were quaternized with tris(2,4,6-trimethoxyphenyl)phosphine (Ar3P) to prepare soluble ionomers. The ionomers were cast from chloroform to form anion exchange membranes (AEMs) with highly ordered morphologies. At low volume fractions of ionic blocks, the ionomers formed lamellar morphologies, while at moderate volume fractions (>= 30% for triblock and >= 22% for diblock copolymers) hexagonal phases with an ionic matrix were observed. Ion conductivities were higher through the hexagonal phase matrix than in the lamellar phases. Promising chloride conductivities (20 mS/cm) were achieved at elevated temperatures and humidified conditions. C1 [Zhang, Wenxu; Ertem, S. Piril; Tsai, Tsung-Han; Coughlin, E. Bryan] Univ Massachusetts, Dept Polymer Sci & Engn, 120 Governors Dr, Amherst, MA 01003 USA. [Liu, Ye; Herring, Andrew M.] Colorado Sch Mines, Dept Chem & Biol Engn, Golden, CO 80401 USA. [Jackson, Aaron C.; Savage, Alice M.; Beyer, Frederick L.] US Army, Res Lab, Aberdeen Proving Ground, MD 21005 USA. [Seifert, Soenke] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Liberatore, Matthew W.] Univ Toledo, Dept Chem & Environm Engn, 2801 W Bancroft St, Toledo, OH 43606 USA. RP Coughlin, EB (reprint author), Univ Massachusetts, Dept Polymer Sci & Engn, 120 Governors Dr, Amherst, MA 01003 USA. EM Coughlin@mail.pse.umass.edu RI Liberatore, Matthew/B-6828-2008; OI Herring, Andrew/0000-0001-7318-5999 FU Army Research Office through MURI award [W911NF-10-1-0520]; NSF; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357]; Postgraduate Research Participation Program at the US Army Research Laboratory [ORISE 1120-1120-99] FX The authors gratefully acknowledge financial support from the Army Research Office through a MURI award, W911NF-10-1-0520, and the central analytical facilities used in these investigations are supported by the NSF-Sponsored MRSEC at UMass Amherst. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract DE-AC02-06CH11357. A.C.J. and A.M.S. were supported by the Postgraduate Research Participation Program at the US Army Research Laboratory, administered by the Oak Ridge Institute of Science and Education through an interagency agreement between the US Department of Energy and Army Research Laboratory (Contract ORISE 1120-1120-99). NR 101 TC 1 Z9 1 U1 6 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD JUL 12 PY 2016 VL 49 IS 13 BP 4714 EP 4722 DI 10.1021/acs.macromol.6b00653 PG 9 WC Polymer Science SC Polymer Science GA DR1ZI UT WOS:000379704000004 ER PT J AU Aaboud, M Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R AbouZeid, OS Abraham, NL Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adachi, S Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aring;kesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Alstaty, M Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Armitage, LJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Aring;sman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barklow, T Barlow, N Barnes, SL Barnett, BM 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Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. Nedden, M. Zur Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for squarks and gluinos in final states with jets and missing transverse momentum at root s=13 TeV with the ATLAS detector SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID PROTON-PROTON COLLISIONS; PARTON DISTRIBUTIONS; HADRON COLLIDERS; SUPERSYMMETRY; EXTENSION; PARTICLE; DECAY; WEAK; LHC AB A search for squarks and gluinos in final states containing hadronic jets, missing transverse momentum but no electrons or muons is presented. The data were recorded in 2015 by the ATLAS experiment in root s = 13 TeV proton-proton collisions at the Large Hadron Collider. No excess above the Standard Model background expectation was observed in 3.2 fb(-1) of analyzed data. Results are interpreted within simplified models that assume R-parity is conserved and the neutralino is the lightest supersymmetric particle. An exclusion limit at the 95 % confidence level on the mass of the gluino is set at 1.51 TeV for a simplified model incorporating only a gluino octet and the lightest neutralino, assuming the lightest neutralino is massless. For a simplified model involving the strong production of mass-degenerate first- and second-generation squarks, squark masses below 1.03 TeV are excluded for a massless lightest neutralino. These limits substantially extend the region of supersymmetric parameter space excluded by previous measurements with the ATLAS detector. C1 [Corriveau, F.; Jackson, P.; Lee, L.; McPherson, R. A.; Petridis, A.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. 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U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch; Ghneimat, M.; Grefe, C.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Mijovic, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Seema, P.; Stillings, J. A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.; Zhang, R.] Univ Bonn, Phys Inst, Bonn, Germany. [Ahlen, S. P.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Coutinho, Y. Amaral; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio De Janeiro COPPE EE IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; de Andrade Filho, L. Manhaes; Peralva, B. S.] Fed Univ Juiz de Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; Navarro, J. L. La Rosa; Leite, M. A. L.; Nepomuceno, A. A.] Univ Sao Paulo, Inst Fis, Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Elmsheuser, J.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lee, C. A.; Liu, H.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M. -A.; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Tricoli, A.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alexa, C.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Dobre, M.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciu, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. Univ Politehn Bucuresti, Bucharest, Romania. [Gravila, P. M.] West Univ Timisoara, Timisoara, Romania. [Sola, J. D. Bossio; Marceca, G.; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.; Sopczak, A.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Brunt, B. H.; Carter, J. R.; Chapman, J. D.; Cottin, G.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Lester, C. G.; Mueller, T.; Parker, M. A.; Potter, C. J.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Gillberg, D.; Koffas, T.; Lacey, J.; Leight, W. A.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Ruiz-Martinez, A.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Amoroso, S.; Anders, G.; Anghinolfi, F.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Burckhart, H.; Camarda, S.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Colombo, T.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Di Nardo, R.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feng, E. J.; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jakobsen, S.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Malyukov, S.; Mandelli, B.; Manousos, A.; Mapelli, L.; Marzin, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Sforza, F.; Sanchez, C. A. Solans; Spigo, G.; Staerz, S.; Stelzer, H. J.; Teischinger, F. A.; Ten Kate, H.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Anderson, K. J.; Bryant, P.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Gardner, R. W.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Okumura, Y.; Oreglia, M. J.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Diaz, M. A.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Salazar Loyola, J. E.; Tapia Araya, S.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costaa, J. Barreiro Guimaraes; Cheng, H. J.; Fang, Y.; Jin, S.; Li, Q.; Liang, Z.; Merino, J. Llorente; Lou, X.; Mansour, J. D.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.; Wang, W.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Wang, C.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Ma, L. L.; Ma, Y.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yange, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yange, H.] PKU CHEP, Shanghai, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Perez, A. Rodriguez; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Madar, R.; Pallin, D.; Perez, A. Rodriguez; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Clark, M. R.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; Del Gaudio, M.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Coll Cosenza, Lab Nazl Frascati, Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; Del Gaudio, M.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Kowalewska, A. B.; Malecki, Pa; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Gaur, B.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] Southern Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75230 USA. [Asbah, N.; Behr, J. K.; Bertsche, C.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Dyndal, M.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Peters, K.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Zakharchuk, N.] DESY, Hamburg, Germany. [Asbah, N.; Behr, J. K.; Bertsche, C.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Dyndal, M.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Peters, K.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 04, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Proissl, M.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Gonella, G.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Nagel, M.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Freiburg, Germany. [Ancu, L. S.; De Mendizabal, J. Bilbao; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; Khoo, T. J.; Lionti, A. E.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Miglioranzi, S.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Miglioranzi, S.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; Gul, U.; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; De Maria, A.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Quadt, A.; Rieger, J.; Rosien, N. -A.; Rzehorz, G. F.; Shabalina, E.; Stolte, P.; Veatch, J.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Berlendis, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Gradin, P. O. J.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E-E; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; de Lima, D. E. Ferreira; Giulini, M.; Kolb, M.; Lisovyi, M.; Radescu, V.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Phys Inst, Heidelberg, Germany. [Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Milic, A.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Abdallah, J.; Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Prell, S.] Iowa State Univ, Dept Phys & Astron, Ames, IA 50011 USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Lyubushkin, V.; Minashvili, I. A.; Mineev, M.; Mueller, R. S. P.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka, Japan. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Argentina. [Verzini, M. J. Alconada; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Argentina. [Barton, A. E.; Beattie, M. D.; Bertram, I. A.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Parker, A. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Aliev, M.; Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Reale, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, Lecce, Italy. [Aliev, M.; Bachas, K.; Gorini, E.; Longo, L.; Reale, M.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lewis, D.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Luzi, P. M.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Luzi, P. M.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Luzi, P. M.; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hedberg, V.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fys Inst, Lund, Sweden. [Barreiro, F.; De la Torre, H.; Del Peso, J.; Glasman, C.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Geisen, M.; Groh, S.; Heck, T.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Webb, S.; Wollstadt, S. J.; Yildirim, E.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Raine, J. A.; Schweiger, H.; Shaw, S. M.; Tomlinson, L.; Watts, S.; Wilk, F.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alstaty, M.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alstaty, M.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Pettersson, N. E.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Le, B.; McDonald, E. F.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Cheng, H. C.; Diehl, E. B.; Feng, H.; Ferretti, C.; Levin, D.; Liu, H.; Marley, D. E.; McCarn, A.; Neal, H. A.; Qian, J.; Zhang, D.; Zhou, B.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Plucinski, P.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Camplani, A.; Carminati, L.; Cavalli, D.; Citterio, M.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Lazzaroni, M.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Camplani, A.; Carminati, L.; Fanti, M.; Lazzaroni, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Ducu, O. A.; Gagnon, L. G.; Gauthier, L.; Leroy, C.; Mochizuki, K.; Manh, T. Nguyen; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Brandt, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Belyaev, N. L.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Roda, C.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Hartmann, N. M.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, B. F.; Ruschke, A.; Schachtner, B. M.; Schaile, D.; Unverdorben, C.; Valderanis, C.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; McCarthy, T. G.; Menke, S.; Mueller, F.; Mueller, R. S. P.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schmidt-Sommerfeld, K. R.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kentaro, K.; Mueller, R. S. P.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Horii, Y.; Kentaro, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Mueller, R. S. P.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Mueller, R. S. P.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Mueller, R. S. P.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Koenig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, Nikhef, Nijmegen, Netherlands. [Aben, R.; Aloisio, A.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelijn, R.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Mueller, R. S. P.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Saha, P.] Univ Illinois, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Maslennikov, A. L.; Maximov, D. A.; Mueller, R. S. P.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Mueller, R. S. P.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Mueller, R. S. P.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama, Japan. [Abbott, B.; Alhroob, M.; Aloisio, A.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Mueller, R. S. P.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Cantero, J.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Aloisio, A.; Alonso, A.; Amorim, A.; Andreazza, A.; Angerami, A.; Annovi, A.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J-F; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Mueller, R. S. P.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.] Univ Paris 11, Univ Paris Saclay, CNRS IN2P3, LAL, Orsay, France. [Endo, M.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Aloisio, A.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Mueller, R. S. P.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Serfon, C.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Aloisio, A.; Alonso, A.; Artoni, G.; Barr, A. J.; Becker, K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Frost, J. A.; Gallas, E. J.; Giuli, F.; Gwenlan, C.; Hays, C. P.; Henderson, J.; Issever, C.; Kalderon, C. W.; Mueller, R. S. P.; Nagai, K.; Petrov, M.; Pickering, M. A.; Tseng, J. C-L.; Viehhauser, G. H. A.; Vigani, L.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Aloisio, A.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Mueller, R. S. P.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Mueller, R. S. P.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Mueller, R. S. P.; Reichert, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Cavasinni, V.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Mueller, R. S. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] Natl Res Ctr, Kurchatov Inst, BP Konstantinov Petersburg Nucl Phys Inst, St Petersburg, Russia. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Mueller, R. S. P.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Mueller, R. S. P.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Mueller, R. S. P.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Aloisio, A.; Dos Santos, S. P. Amor; Amorim, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Mueller, R. S. P.; Seabra, L. F. Oleiro; Onofre, A.; Palma, A.; Pedro, R.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; De Sousa, M. J. Da Cunha Sargedas; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Silva, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Saraiva, J. G.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dep Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Aloisio, A.; Alonso, A.; Amorim, A.; Andreazza, A.; Angerami, A.; Annovi, A.; Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Mueller, R. S. P.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Berta, P.; Carli, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Slovak, R.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Aloisio, A.; Alonso, A.; Amorim, A.; Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Mueller, R. S. P.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Vaniachine, A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Protvino, Russia. [Aloisio, A.; Alonso, A.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Kirk, J.; Middleton, R. P.; Mueller, R. S. P.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Aloisio, A.; Alonso, A.; Amorim, A.; Andreazza, A.; Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Messina, A.; Mueller, R. S. P.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Mueller, R. S. P.; Vanadia, M.; Verducci, M.; Zanello, L.] Sapienza Univ Roma, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Mueller, R. S. P.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Fac Sci Ain Chock, Reseau Univ Phys Hautes Energies, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Aaboud, M.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Aaboud, M.; Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddade, N.; Idrissie, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Besson, N.; Blanchard, J-B; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Meyer, J-P.; Mueller, R. S. P.; Nicolaidou, R.; Ouraou, A.; Perego, M. M.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay Comm Energie Atom & Energie Atom & Ene, DSM IRFU Inst Rech Lois Fondament Univers, Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schier, S.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Aloisio, A.; Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S-C; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Mueller, R. S. P.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.; Whallon, N. L.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC, Canada. [Aloisio, A.; Alonso, A.; Armbruster, A. J.; Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Mueller, R. S. P.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazeka, T.; Dado, T.; Melo, M.; Mueller, R. S. P.; Plazak, L.; Smiesko, J.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Karc, D.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, Stockholm, Sweden. [Aloisio, A.; Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Huo, P.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Mueller, R. S. P.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Huo, P.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Abraham, N. L.; Allbrooke, B. M. M.; Aloisio, A.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Lerner, G.; Miano, F.; Mueller, R. S. P.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.; Winston, O. J.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G-Y; Limosani, A.; Morley, A. K.; Mueller, R. S. P.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW, Australia. [Hou, S.; Hsu, P. J.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Mueller, R. S. P.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Mueller, R. S. P.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Mueller, R. S. P.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Adachi, S.; Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Kozakai, C.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Mueller, R. S. P.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Adachi, S.; Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Kozakai, C.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo, Japan. [Batista, S. J.; Chau, C. C.; Cormier, K. J. R.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Keoshkerian, H.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Mueller, R. S. P.; Orr, R. S.; Pascuzzi, V. R.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Hod, N.; Jovicevic, J.; Codina, E. Perez; Schneider, B.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC, Canada. [Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON, Canada. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Son, H.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] Ist Nazl Fis Nucl, Sez Trieste, Grp Collegato Udine, Udine, Italy. [Acharya, B. S.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, Udine, Italy. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Maddocks, H. J.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Atkinson, M.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Sickles, A. M.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Melini, D.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Melini, D.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Melini, D.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Aloisio, A.; Alonso, A.; Piqueras, D. Alvarez; Amorim, A.; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Melini, D.; Mitsou, V. A.; Mueller, R. S. P.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Piqueras, D. Alvarez; Navarro, L. Barranco; Urban, S. Cabrera; Gimenez, V. Castillo; Alberich, L. Cerda; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Jimenez, Y. Hernandez; Higon-Rodriguez, E.; Pena, J. Jimenez; King, M.; Lacasta, C.; Lacuesta, V. R.; Mamuzic, J.; Marti-Garcia, S.; Melini, D.; Mitsou, V. A.; Mueller, R. S. P.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] CSIC, Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC, Canada. [Albert, J.; David, C.; Elliot, A. A.; Fincke-Keeler, M.; Hamano, K.; Hill, E.; Keeler, R.; Kowalewski, R.; Kuwertz, E. S.; Kwan, T.; LeBlanc, M.; Lefebvre, M.; McPherson, R. A.; Mueller, R. S. P.; Pearce, J.; Seuster, R.; Sobie, R.; Trovatelli, M.; Venturi, M.] Univ Victoria, Dept Phys & Astron, Victoria, BC, Canada. [Beckingham, M.; Ennis, J. S.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Aloisio, A.; Bressler, S.; Citron, Z. H.; Duchovni, E.; Dumancic, M.; Gross, E.; Koehler, M. K.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Mueller, R. S. P.; Pitt, M.; Ravinovich, I.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.; Turgeman, D.] Weizmann Inst Sci, Dept Particle Phys, Rehovot, Israel. [Banerjee, Sw; Guan, W.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, Madison, WI USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Trefzger, T.; Wallangen, V.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, Wurzburg, Germany. [Bannoura, A. A. E.; Boerner, D.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Gabizon, O.; Gilles, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kersten, S.; Kuechler, J. T.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. J.; Sandhoff, M.; Tepel, F.; Vogel, M.; Wagner, W.; Zeitnitz, C.] Berg Univ Wuppertal, Fak Math & Nat Wissensch, Fachgrp Phys, Wuppertal, Germany. [Baker, O. K.; Noccioli, E. Benhar; Cummings, J.; Demers, S.; Ideal, E.; Lagouri, T.; Leister, A. G.; Loginov, A.; Mueller, R. S. P.; Hernandez, D. Paredes; Thomsen, L. A.; Tipton, P.; Vasquez, J. G.; Wang, X.] Yale Univ, Dept Phys, New Haven, CT USA. [Hakobyan, H.; Vardanyan, G.] Yerevan Phys Inst, Yerevan, Armenia. [Rahal, G.] Ctr Calcul, IN2P3, Villeurbanne, France. [Acharya, B. 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A.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Fedin, O. L.] St Petersburg State Polytech Univ, Dept Phys, St Petersburg, Russia. [Geng, C.; Guo, Y.; Li, B.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Govender, N.] Ctr High Performance Comp, CSIR Campus, Cape Town, South Africa. [Greenwood, Z. D.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Grinstein, S.; Juste Rozas, A.; Martinez, M.] ICREA, Inst Catalana Recerca Estudis Avancats, Barcelona, Spain. [Hanagaki, K.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Hsu, P. J.] Natl Tsing Hua Univ, Dept Phys, Taipei, Taiwan. [Igonkina, O.] Radboud Univ Nijmegen, Inst Math Astrophys & Particle Phys, Nikhef, Nijmegen, Netherlands. [Ilchenko, Y.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Jejelava, J.] Ilia State Univ, Inst Theoret Phys, Tbilisi, Rep of Georgia. [Jenni, P.] CERN, Geneva, Switzerland. [Khubua, J.] GTU, Tbilisi, Rep of Georgia. [Kono, T.] Ochanomizu Univ, Ochadai Acad Prod, Tokyo, Japan. [Konoplich, R.] Manhattan Coll, New York, NY USA. [Leisos, A.] Hellen Open Univ, Patras, Greece. [Lin, S. C.] Acad Sinica, Acad Sinica Grid Comp, Inst Phys, Taipei, Taiwan. [Liu, B.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. Moscow Inst Phys, Dolgoprudnyi, Russia. Technol State Univ, Dolgoprudnyi, Russia. Univ Geneva, Sect Phys, Geneva, Switzerland. Eotvos Lorand Univ, Budapest, Hungary. Int Sch Adv Studies SISSA, Trieste, Italy. Univ S Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Guangdong, Peoples R China. Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy INRNE, Sofia, Bulgaria. Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. Acad Sinica, Inst Phys, Taipei, Taiwan. Natl Res Nucl Univ MEPhI, Moscow, Russia. Stanford Univ, Dept Phys, Stanford, CA 94305 USA. Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. Flensburg Univ Appl Sci, Flensburg, Germany. Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. Aix Marseille Univ, CPPM, Marseille, France. CNRS IN2P3, Marseille, France. RP Aaboud, M (reprint author), Univ Mohamed Premier, Fac Sci, Oujda, Morocco.; Aaboud, M (reprint author), LPTPM, Oujda, Morocco. RI Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Gladilin, Leonid/B-5226-2011; Garcia, Jose /H-6339-2015; Mitsou, Vasiliki/D-1967-2009; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Guo, Jun/O-5202-2015; Di Simone, Andrea/K-6609-2013; Villa, Mauro/C-9883-2009; Coccaro, Andrea/P-5261-2016; Brooks, William/C-8636-2013; Staroba, Pavel/G-8850-2014; Lazzaroni, Massimo/N-3675-2015; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Doyle, Anthony/C-5889-2009; Shulga, Evgeny/R-1759-2016; Maleev, Victor/R-4140-2016; Grinstein, Sebastian/N-3988-2014; Zhukov, Konstantin/M-6027-2015; Livan, Michele/D-7531-2012; Tikhomirov, Vladimir/M-6194-2015; Ventura, Andrea/A-9544-2015; Stabile, Alberto/L-3419-2016; Warburton, Andreas/N-8028-2013; Carvalho, Joao/M-4060-2013; Boyko, Igor/J-3659-2013; Prokoshin, Fedor/E-2795-2012 OI Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Gladilin, Leonid/0000-0001-9422-8636; Mitsou, Vasiliki/0000-0002-1533-8886; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Guo, Jun/0000-0001-8125-9433; Di Simone, Andrea/0000-0003-0201-3377; Villa, Mauro/0000-0002-9181-8048; Coccaro, Andrea/0000-0003-2368-4559; Brooks, William/0000-0001-6161-3570; Lazzaroni, Massimo/0000-0002-4094-1273; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; Doyle, Anthony/0000-0001-6322-6195; Shulga, Evgeny/0000-0001-5099-7644; Grinstein, Sebastian/0000-0002-6460-8694; Livan, Michele/0000-0002-5877-0062; Tikhomirov, Vladimir/0000-0002-9634-0581; Ventura, Andrea/0000-0002-3368-3413; Stabile, Alberto/0000-0002-6868-8329; Warburton, Andreas/0000-0002-2298-7315; Carvalho, Joao/0000-0002-3015-7821; Boyko, Igor/0000-0002-3355-4662; Prokoshin, Fedor/0000-0001-6389-5399 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF; Canada Council; CANARIE; CRC; Compute Canada; FQRNT; Ontario InnovationTrust, Canada; EPLANET; ERC; FP7; Horizon; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex; ANR; Region Auvergne; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario InnovationTrust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 88 TC 1 Z9 1 U1 35 U2 46 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 12 PY 2016 VL 76 IS 7 AR 392 DI 10.1140/epjc/s10052-016-4184-8 PG 29 WC Physics, Particles & Fields SC Physics GA DR2SF UT WOS:000379753500003 ER PT J AU Shi, TJ Niepel, M McDermott, JE Gao, YQ Nicora, CD Chrisler, WB Markillie, LM Petyuk, VA Smith, RD Rodland, KD Sorger, PK Qian, WJ Wiley, HS AF Shi, Tujin Niepel, Mario McDermott, Jason E. Gao, Yuqian Nicora, Carrie D. Chrisler, William B. Markillie, Lye M. Petyuk, Vladislav A. Smith, Richard D. Rodland, Karin D. Sorger, Peter K. Qian, Wei-Jun Wiley, H. Steven TI Conservation of protein abundance patterns reveals the regulatory architecture of the EGFR-MAPK pathway SO SCIENCE SIGNALING LA English DT Article ID MAMMARY EPITHELIAL-CELLS; GROWTH-FACTOR RECEPTOR; CYSTEINYL-PEPTIDE ENRICHMENT; SIGNAL-TRANSDUCTION NETWORKS; HUMAN-BREAST-CANCER; QUANTITATIVE-ANALYSIS; MULTIPLE MECHANISMS; SHOTGUN PROTEOMICS; MASS-SPECTROMETRY; NOONAN-SYNDROME AB Various genetic mutations associated with cancer are known to alter cell signaling, but it is not clear whether they dysregulate signaling pathways by altering the abundance of pathway proteins. Using a combination of RNA sequencing and ultrasensitive targeted proteomics, we defined the primary components-16 core proteins and 10 feedback regulators-of the epidermal growth factor receptor (EGFR)-mitogen-activated protein kinase (MAPK) pathway in normal human mammary epithelial cells and then quantified their absolute abundance across a panel of normal and breast cancer cell lines as well as fibroblasts. We found that core pathway proteins were present at very similar concentrations across all cell types, with a variance similar to that of proteins previously shown to display conserved abundances across species. In contrast, EGFR and transcriptionally controlled feedback regulators were present at highly variable concentrations. The absolute abundance of most core proteins was between 50,000 and 70,000 copies per cell, but the adaptors SOS1, SOS2, and GAB1 were found at far lower amounts (2000 to 5000 copies per cell). MAPK signaling showed saturation in all cells between 3000 and 10,000 occupied EGFRs, consistent with the idea that adaptors limit signaling. Our results suggest that the relative stoichiometry of core MAPK pathway proteins is very similar across different cell types, with cell-specific differences mostly restricted to variable amounts of feedback regulators and receptors. The low abundance of adaptors relative to EGFR could be responsible for previous observations that only a fraction of total cell surface EGFR is capable of rapid endocytosis, high-affinity binding, and mitogenic signaling. C1 [Shi, Tujin; McDermott, Jason E.; Gao, Yuqian; Nicora, Carrie D.; Chrisler, William B.; Petyuk, Vladislav A.; Smith, Richard D.; Rodland, Karin D.; Qian, Wei-Jun] Pacific Northwest Natl Lab, Biol Sci Div, Richland, WA 99352 USA. [Niepel, Mario; Sorger, Peter K.] Harvard Med Sch, HMS LINCS Ctr, Boston, MA 02115 USA. [Niepel, Mario; Sorger, Peter K.] Harvard Med Sch, Lab Syst Pharmacol, Dept Syst Biol, Boston, MA 02115 USA. [Markillie, Lye M.; Smith, Richard D.; Wiley, H. Steven] Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. RP Wiley, HS (reprint author), Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. EM steven.wiley@pnnl.gov RI Smith, Richard/J-3664-2012; OI Smith, Richard/0000-0002-2381-2349; Wiley, Steven/0000-0003-0232-6867 FU NIH [DP2OD006668, P41GM103493, U24-CA-16001901, UC4-DK104167, U54-HL127365] FX Portions of the research were supported by NIH grants DP2OD006668, P41GM103493, U24-CA-16001901, UC4-DK104167, and U54-HL127365. NR 84 TC 2 Z9 2 U1 4 U2 5 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 1945-0877 EI 1937-9145 J9 SCI SIGNAL JI Sci. Signal. PD JUL 12 PY 2016 VL 9 IS 436 AR rs6 DI 10.1126/scisignal.aaf0891 PG 13 WC Biochemistry & Molecular Biology; Cell Biology SC Biochemistry & Molecular Biology; Cell Biology GA DS4VD UT WOS:000380778800004 PM 27405981 ER PT J AU Zhang, HH Ma, CX Bonnesen, PV Zhu, JH Sumpter, BG Carrillo, JMY Yin, PC Wang, YY Li, AP Hong, KL AF Zhang, Hong-Hai Ma, Chuanxu Bonnesen, Peter V. Zhu, Jiahua Sumpter, Bobby G. Carrillo, Jan-Michael Y. Yin, Panchao Wang, Yangyang Li, An-Ping Hong, Kunlun TI Helical Poly(5-alkyl-2,3-thiophene)s: Controlled Synthesis and Structure Characterization SO MACROMOLECULES LA English DT Article ID CATALYST-TRANSFER POLYCONDENSATION; CROSS-COUPLING POLYMERIZATION; CHAIN-GROWTH POLYMERIZATION; PI-CONJUGATED POLYMERS; AB-TYPE MONOMERS; ORTHO-PHENYLENES; CONDENSATION POLYMERIZATION; LIQUID-CRYSTALS; CONFORMATION; INITIATOR AB Whereas poly(3-alkyl-2,5-thiophene)s (P3AT), with many potential applications, have been extensively investigated, their ortho-connected isomers, poly(5-alkyl-2,3-thiophene)s (PSAT), have never been reported because of the difficulty in their syntheses. We herein present the first synthesis of regioregular PSAT via controlled Suzuki cross-coupling polymerization with PEPPSI-IPr as catalyst, affording the polymers with tunable molecular weight, narrow polydispersity (PDI), and well-defined functional end groups at the gram scale. The helical geometry of P5AT was studied by a combination of NMR, small-angle X-ray scattering (SAXS), and scanning tunneling microscopy (STM). Particularly, the single polymer chain of poly(5-butyl-2,3-thiophene) (POT) on highly oriented pyrolytic graphite (HOPG) substrates with either M or P helical conformation was directly observed by STM. The comparison of UV-vis absorption between poly(5-hexyl-2,3-thiophene) (PSHT) (lambda = 345 nm) and poly(3-hexyl-2,5-thiophene) (P3HT) (A = 450 nm) indicated that the degree of conjugation of the backbone in P5HT is less than in P3HT, which may be a consequence of the helical geometry of the former compared to the more planar geometry of the latter. Moreover, we found that P5HT can emit green fluorescence under UV (lambda = 360 nm) irradiation. C1 [Zhang, Hong-Hai; Ma, Chuanxu; Bonnesen, Peter V.; Zhu, Jiahua; Sumpter, Bobby G.; Carrillo, Jan-Michael Y.; Wang, Yangyang; Li, An-Ping; Hong, Kunlun] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Sumpter, Bobby G.; Carrillo, Jan-Michael Y.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Yin, Panchao] Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. RP Zhang, HH; Hong, KL (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM zhangh1@ornl.gov; hongkq@ornl.gov RI Yin, Panchao/J-3322-2013; Ma, Chuanxu/Q-2512-2015; Wang, Yangyang/A-5925-2010; Sumpter, Bobby/C-9459-2013; Hong, Kunlun/E-9787-2015; Li, An-Ping/B-3191-2012 OI Yin, Panchao/0000-0003-2902-8376; Ma, Chuanxu/0000-0001-6478-5917; Wang, Yangyang/0000-0001-7042-9804; Sumpter, Bobby/0000-0001-6341-0355; Hong, Kunlun/0000-0002-2852-5111; Li, An-Ping/0000-0003-4400-7493 NR 66 TC 0 Z9 0 U1 9 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0024-9297 EI 1520-5835 J9 MACROMOLECULES JI Macromolecules PD JUL 12 PY 2016 VL 49 IS 13 BP 4691 EP 4698 DI 10.1021/acs.macromol.6b01233 PG 8 WC Polymer Science SC Polymer Science GA DR1ZI UT WOS:000379704000002 ER PT J AU Calvey, JR Hartung, W Makita, J Venturini, M AF Calvey, J. R. Hartung, W. Makita, J. Venturini, M. TI Beam induced electron cloud resonances in dipole magnetic fields SO PHYSICAL REVIEW ACCELERATORS AND BEAMS LA English DT Article ID POSITRON RING; TIN AB The buildup of low energy electrons in an accelerator, known as electron cloud, can be severely detrimental to machine performance. Under certain beam conditions, the beam can become resonant with the cloud dynamics, accelerating the buildup of electrons. This paper will examine two such effects: multipacting resonances, in which the cloud development time is resonant with the bunch spacing, and cyclotron resonances, in which the cyclotron period of electrons in a magnetic field is a multiple of bunch spacing. Both resonances have been studied directly in dipole fields using retarding field analyzers installed in the Cornell Electron Storage Ring. These measurements are supported by both analytical models and computer simulations. C1 [Calvey, J. R.; Hartung, W.; Makita, J.] Cornell Univ, Cornell Lab Accelerator Based Sci & Educ, Ithaca, NY 14853 USA. [Venturini, M.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Calvey, J. R.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Hartung, W.] Michigan State Univ, Facil Rare Isotope Beams, E Lansing, MI 48824 USA. [Makita, J.] Old Domin Univ, Dept Phys, Norfolk, VA 23529 USA. RP Calvey, JR (reprint author), Cornell Univ, Cornell Lab Accelerator Based Sci & Educ, Ithaca, NY 14853 USA.; Calvey, JR (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. FU NSF; DOE [PHY-0734867, PHY-1002467, PHYS-1068662, DE-FC02-08ER41538, DE-SC0006505]; Japan/U.S. Cooperation Program FX This research was supported by NSF and DOE Contracts No. PHY-0734867, No. PHY-1002467, No. PHYS-1068662, No. DE-FC02-08ER41538, No. DE-SC0006505, and the Japan/U.S. Cooperation Program. The authors would like to thank D. Rubin, G. Dugan, J. A. Crittenden, J. Sikora, J. Livesey, M. Palmer, and K. Harkay for their helpful advice and suggestions; R. Schwartz, S. Santos, and S. Roy for assisting with the RFA measurements; and M. Furman at LBNL for his support with the POSINST simulation code. NR 34 TC 0 Z9 0 U1 2 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9888 J9 PHYS REV ACCEL BEAMS JI Phys. Rev. Accel. Beams PD JUL 12 PY 2016 VL 19 IS 7 AR 074401 DI 10.1103/PhysRevAccelBeams.19.074401 PG 12 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DR8CU UT WOS:000380126800002 ER PT J AU Hertzberg, BJ Huang, A Hsieh, A Chamoun, M Davies, G Seo, JK Zhong, Z Croft, M Erdonmez, C Meng, YS Steingart, D AF Hertzberg, Benjamin J. Huang, An Hsieh, Andrew Chamoun, Mylad Davies, Greg Seo, Joon Kyo Zhong, Zhong Croft, Mark Erdonmez, Can Meng, Ying Shirley Steingart, Dan TI Effect of Multiple Cation Electrolyte Mixtures on Rechargeable Zn MnO2 Alkaline Battery SO CHEMISTRY OF MATERIALS LA English DT Article ID MANGANESE-DIOXIDE; BI(NO3)(3) MIXTURES; DISSOLVED KMNO4; GAMMA-MNO2; CATHODE; BI; REDUCTION; CELLS; DECOMPOSITION; COMPOSITES AB A Bi2O3 in beta-MnO2 composite cathode material has been synthesized using a simple hydrothermal method and cycled in a mixed KOH-LiOH electrolyte with a range of concentrations. We show that, at a KOH:LiOH molar ratio of 1:3, both proton insertion and lithium insertion occur, allowing access to a higher fraction of the theoretical capacity of the MnO2 while preventing the formation of ZnMn2O4. This enables a capacity of 360 mAh/g for over 60 cycles, with cycling limited more by anode properties than traditional cathodic failure mechanisms. The structural changes occurring during cycling are characterized using electron microscopy and in situ synchrotron energy-dispersive X-ray diffraction (EDXRD) techniques. This mixed electrolyte shows exceptional cyclability and capacity and can be used as a drop-in replacement for current alkaline batteries, potentially drastically improving their cycle life and creating a wide range of new applications for this energy storage technology. C1 [Hertzberg, Benjamin J.; Hsieh, Andrew; Davies, Greg; Steingart, Dan] Princeton Univ, Dept Mech & Aerosp Engn, Princeton, NJ 08544 USA. [Huang, An; Seo, Joon Kyo] Univ Calif San Diego, Dept Mat Sci & Engn, 9500 Gilman Dr, La Jolla, CA 92093 USA. [Chamoun, Mylad] Stockholm Univ, Dept Mat & Environm Engn, Univ Vagen 10, S-11418 Stockholm, Sweden. [Meng, Ying Shirley] Univ Calif San Diego, Dept NanoEngn, 9500 Gilman Dr, La Jolla, CA 92093 USA. [Erdonmez, Can] Brookhaven Natl Lab, Sustainable Technol Div, 2 Ctr St, Upton, NY 11973 USA. [Zhong, Zhong] Brookhaven Natl Lab, Photon Sci, 2 Ctr St, Upton, NY 11973 USA. [Croft, Mark] Rutgers State Univ, Dept Phys & Astron, 136 Frelinghuysen Rd, Piscataway, NJ 08854 USA. RP Steingart, D (reprint author), Princeton Univ, Dept Mech & Aerosp Engn, Princeton, NJ 08544 USA. EM steingart@princeton.edu FU DOE ARPA-E RANGE Grant [DE-AR000000400] FX This work was supported by DOE ARPA-E RANGE Grant No. DE-AR000000400. NR 39 TC 3 Z9 3 U1 43 U2 62 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 12 PY 2016 VL 28 IS 13 BP 4536 EP 4545 DI 10.1021/acs.chemmater.6b00232 PG 10 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DR1ZJ UT WOS:000379704100004 ER PT J AU Wang, HP Sutter-Fella, CM Lobaccaro, P Hettick, M Zheng, M Lien, DH Miller, DW Warren, CW Roe, ET Lonergan, MC Guthrey, HL Haegel, NM Ager, JW Carraro, C Maboudian, R He, JH Javey, A AF Wang, Hsin-Ping Sutter-Fella, Carolin M. Lobaccaro, Peter Hettick, Mark Zheng, Maxwell Lien, Der-Hsien Miller, D. Westley Warren, Charles W. Roe, Ellis T. Lonergan, Mark C. Guthrey, Harvey L. Haegel, Nancy M. Ager, Joel W. Carraro, Carlo Maboudian, Roya He, Jr-Hau Javey, Ali TI Increased Optoelectronic Quality and Uniformity of Hydrogenated p-InP Thin Films SO CHEMISTRY OF MATERIALS LA English DT Article ID SOLAR-CELLS; INDIUM-PHOSPHIDE; PASSIVATION; PHOTOLUMINESCENCE; SEMICONDUCTORS; SILICON; ZN; ACCEPTORS; DEFECTS; GAAS AB The thin-film vapor-liquid-solid (TF-VLS) growth technique presents a promising route for high quality, scalable, and cost-effective InP thin films for optoelectronic devices. Toward this goal, careful optimization of material properties and device performance is of utmost interest. Here, we show that exposure of polycrystalline Zn-doped TF-VLS InP to a hydrogen plasma (in the following referred to as hydrogenation) results in improved optoelectronic quality as well as lateral optoelectronic uniformity. A combination of low temperature photoluminescence and transient photocurrent spectroscopy was used to analyze the energy position and relative density of defect states before and after hydrogenation. Notably, hydrogenation reduces the relative intragap defect density by 1 order of magnitude. As a metric to monitor lateral optoelectronic uniformity of polycrystalline TF-VLS InP, photoluminescence and electron beam induced current mapping reveal homogenization of the grain versus grain boundary upon hydrogenation. At the device level, we measured more than 260 TF-VLS InP solar cells before and after hydrogenation to verify the improved optoelectronic properties. Hydrogenation increased the average open-circuit voltage (VOC) of individual TF-VLS InP solar cells by up to 130 mV and reduced the variance in VOC for the analyzed devices. C1 [Wang, Hsin-Ping; Sutter-Fella, Carolin M.; Hettick, Mark; Zheng, Maxwell; Lien, Der-Hsien; Javey, Ali] Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Lobaccaro, Peter; Carraro, Carlo; Maboudian, Roya] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Wang, Hsin-Ping; Sutter-Fella, Carolin M.; Hettick, Mark; Zheng, Maxwell; Lien, Der-Hsien; Ager, Joel W.; Javey, Ali] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Lobaccaro, Peter] Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, Berkeley, CA 94720 USA. [Wang, Hsin-Ping; He, Jr-Hau] KAUST, Comp Elect & Math Sci & Engn CEMSE Div, Thuwal 239556900, Saudi Arabia. [Wang, Hsin-Ping; Lien, Der-Hsien] Natl Taiwan Univ, Inst Photon & Optoelect, Taipei 10617, Taiwan. [Wang, Hsin-Ping; Lien, Der-Hsien] Natl Taiwan Univ, Dept Elect Engn, Taipei 10617, Taiwan. [Miller, D. Westley; Warren, Charles W.; Roe, Ellis T.] Univ Oregon, Dept Phys, Eugene, OR 97403 USA. [Lonergan, Mark C.] Univ Oregon, Dept Chem & Biochem, Eugene, OR 97403 USA. [Guthrey, Harvey L.; Haegel, Nancy M.] Natl Renewable Energy Lab, Natl Ctr Photovolta NCPV, Golden, CO 80401 USA. RP Javey, A (reprint author), Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA.; Javey, A (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; He, JH (reprint author), KAUST, Comp Elect & Math Sci & Engn CEMSE Div, Thuwal 239556900, Saudi Arabia. EM jrhau.he@kaust.edu.sa; ajavey@eecs.berkeley.edu OI Sutter-Fella, Carolin/0000-0002-7769-0869 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Department of Energy through the Bay Area Photovoltaic Consortium [DE-EE0004946]; Swiss National Science Foundation [P2EZP2_155586] FX Materials characterization and growth was supported by the Electronic Materials Program funded by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy, under Contract No. DE-AC02-05CH11231. Device fabrication was supported by the Department of Energy through the Bay Area Photovoltaic Consortium under Award Number DE-EE0004946. J.-H.H. acknowledges KAUST and National Science Council of Taiwan (NSC 102-2911-I-002-552). C.M.S.-F. acknowledges financial support from the Swiss National Science Foundation (P2EZP2_155586). NR 41 TC 1 Z9 1 U1 4 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 12 PY 2016 VL 28 IS 13 BP 4602 EP 4607 DI 10.1021/acs.chemmater.6b01257 PG 6 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DR1ZJ UT WOS:000379704100011 ER PT J AU Wahila, MJ Butler, KT Lebens-Higgins, ZW Hendon, CH Nandur, AS Treharne, RE Quackenbush, NF Sallis, S Mason, K Paik, H Schlom, DG Woicik, JC Guo, JH Arena, DA White, BE Watson, GW Walsh, A Piper, LFJ AF Wahila, Matthew J. Butler, Keith T. Lebens-Higgins, Zachary W. Hendon, Christopher H. Nandur, Abhishek S. Treharne, Robert E. Quackenbush, Nicholas F. Sallis, Shawn Mason, Katie Paik, Hanjong Schlom, Darrell G. Woicik, Joseph C. Guo, Jinghua Arena, Dario A. White, Bruce E., Jr. Watson, Graeme W. Walsh, Aron Piper, Louis F. J. TI Lone-Pair Stabilization in Transparent Amorphous Tin Oxides: A Potential Route to p-Type Conduction Pathways SO CHEMISTRY OF MATERIALS LA English DT Article ID ROOM-TEMPERATURE FABRICATION; THIN-FILM TRANSISTORS; AUGMENTED-WAVE METHOD; SEMICONDUCTOR; CUALO2; SNO; MONOXIDE AB The electronic and atomic structures of amorphous transparent tin oxides have been investigated by a combination of X-ray spectroscopy and atomistic calculations. Crystalline SnO is a promising p-type transparent oxide semiconductor due to a complex lone-pair hybridization that affords both optical transparency despite a small electronic band gap and spherical s-orbital character at the valence band edge. We find that both of these desirable properties (transparency and s-orbital valence band character) are retained upon amorphization despite the disruption of the layered lone-pair states by structural disorder. We explain the anomalously large band gap widening necessary to maintain transparency in terms of lone-pair stabilization via atomic clustering. Our understanding of this mechanism suggests that continuous hole conduction pathways along extended lone pair clusters should be possible under certain stoichiometries. Moreover, these findings should be applicable to other lone-pair active semiconductors. C1 [Wahila, Matthew J.; Lebens-Higgins, Zachary W.; Quackenbush, Nicholas F.; Mason, Katie; Piper, Louis F. J.] Binghamton Univ, Dept Phys Appl Phys & Astron, Binghamton, NY 13902 USA. [Butler, Keith T.; Hendon, Christopher H.; Walsh, Aron] Univ Bath, Dept Chem, Bath BA2 7AY, Avon, England. [Nandur, Abhishek S.; Sallis, Shawn; White, Bruce E., Jr.] Binghamton Univ, Mat Sci & Engn, Binghamton, NY 13902 USA. [Treharne, Robert E.] Univ Liverpool, Stephenson Inst Renewable Energy, Liverpool L69 7ZF, Merseyside, England. [Paik, Hanjong; Schlom, Darrell G.] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA. [Paik, Hanjong; Schlom, Darrell G.] Kavli Inst Cornell Nanoscale Sci, Ithaca, NY 14853 USA. [Woicik, Joseph C.] NIST, Mat Sci & Engn Lab, Gaithersburg, MD 20899 USA. [Guo, Jinghua] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Arena, Dario A.] Brookhaven Natl Lab, Natl Synchrotron Light Source 2, Basic Energy Sci Directorate, Upton, NY 11973 USA. [Watson, Graeme W.] Trinity Coll Dublin, Sch Chem, Dublin 2, Ireland. [Watson, Graeme W.] Trinity Coll Dublin, CRANN, Dublin 2, Ireland. [Hendon, Christopher H.] MIT, Dept Chem, Cambridge, MA 02139 USA. [Arena, Dario A.] Univ S Florida, Dept Phys, Tampa, FL 33620 USA. RP Piper, LFJ (reprint author), Binghamton Univ, Dept Phys Appl Phys & Astron, Binghamton, NY 13902 USA.; Butler, KT (reprint author), Univ Bath, Dept Chem, Bath BA2 7AY, Avon, England. EM ktb22@bath.ac.uk; lpiper@binghamton.edu RI Walsh, Aron/A-7843-2008; Watson, Graeme/B-4262-2008 OI Walsh, Aron/0000-0001-5460-7033; Watson, Graeme/0000-0001-6732-9474 FU National Science Foundation [DMR-1409912, ECCS-1542081]; NSF REU [DMR-1263004]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; EPSRC [EP/K016288/1, EP/J017361/1]; SFI Grant [12/IA/1414]; PRACE; Center for Low Energy Systems Technology (LEAST), one of six centers of STARnet, a Semiconductor Research Corporation program - MARCO; Center for Low Energy Systems Technology (LEAST), one of six centers of STARnet, a Semiconductor Research Corporation program - DARPA FX The research at Binghamton was partially supported by the National Science Foundation under Grant No. DMR-1409912. KM. acknowledges support from an NSF REU under Grant No. DMR-1263004. Use of the National Synchrotron Light Source, Brookhaven National Laboratory, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. The research at Bath was supported by EPSRC grants: EP/K016288/1 and EP/J017361/1. The research at Trinity College Dublin was supported by SFI Grant 12/IA/1414. We also acknowledge PRACE for awarding us access to resource ARCHER based in the U.K. We thank Ken Durose for access to his laboratory facilities supported by EPSRC EP/K005901/1. The work of H.P. and D.G.S. was supported by the Center for Low Energy Systems Technology (LEAST), one of six centers of STARnet, a Semiconductor Research Corporation program sponsored by MARCO and DARPA. This work was performed in part at the Cornell NanoScale Facility, a member of the National Nanotechnology Coordinated Infrastructure (NNCI), which is supported by the National Science Foundation (Grant ECCS-1542081). NR 49 TC 1 Z9 1 U1 24 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 12 PY 2016 VL 28 IS 13 BP 4706 EP 4713 DI 10.1021/acs.chemmater.6b01608 PG 8 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DR1ZJ UT WOS:000379704100022 ER PT J AU Youm, SG Hwang, E Chavez, CA Li, X Chatterjee, S Lusker, KL Lu, L Strzalka, J Ankner, JF Losovyj, Y Garno, JC Nesterov, EE AF Youm, Sang Gil Hwang, Euiyong Chavez, Carlos A. Li, Xin Chatterjee, Sourav Lusker, Kathie L. Lu, Lu Strzalka, Joseph Ankner, John F. Losovyj, Yaroslav Garno, Jayne C. Nesterov, Evgueni E. TI Polythiophene Thin Films by Surface-Initiated Polymerization: Mechanistic and Structural Studies SO CHEMISTRY OF MATERIALS LA English DT Article ID CATALYST-TRANSFER POLYCONDENSATION; CHAIN-GROWTH POLYMERIZATION; PI-CONJUGATED POLYMERS; FULLERENE SOLAR-CELLS; LIGHT-EMITTING-DIODES; NANOSPHERE LITHOGRAPHY; REGIOREGULAR POLY(3-ALKYLTHIOPHENES); GRIGNARD METATHESIS; SEXITHIOPHENE FILMS; CRYSTAL-STRUCTURE AB The ability to control nanoscale morphology and molecular organization in organic semiconducting polymer thin films is an important prerequisite for enhancing the efficiency of organic thin-film devices including organic light-emitting and photovoltaic devices. The current "top-down" paradigm for making such devices is based on utilizing solution-based processing (e.g., spin-casting) of soluble semiconducting polymers. This approach typically provides only modest control over nanoscale molecular organization and polymer chain alignment. A promising alternative to using solutions of presynthesized semiconducting polymers pursues instead a "bottom-up' approach to prepare surface-grafted semiconducting polymer thin films by surface-initiated polymerization of small-molecule monomers. Herein, we describe the development of an efficient method to prepare polythiophene thin films utilizing surface-initiated Kumada catalyst transfer polymerization. In this study, we provided evidence that the surface-initiated polymerization occurs by the highly robust controlled (quasi-"living') chain-growth mechanism. Further optimization of this method enabled reliable preparation of polythiophene thin films with thickness up to 100 nm. Extensive structural studies of the resulting thin films using X-ray and neutron scattering methods as well as ultraviolet photoemission spectroscopy revealed detailed information on molecular organization and the bulk morphology of the films, and enabled further optimization of the polymerization protocol. One of the remarkable findings was that surface-initiated polymerization delivers polymer thin films showing complex molecular organization, where polythiophene chains assemble into lateral crystalline domains of about 3.2 nm size, with individual polymer chains folded to form in-plane aligned and densely packed oligomeric segments (7-8 thiophene units per each segment) within each domain. Achieving such a complex mesoscale organization is virtually impossible with traditional methods relying on solution processing of presynthesized polymers. Another significant advantage of surface-confined polymer thin films is their remarkable stability toward organic solvents and other processing conditions. In addition to controlled bulk morphology, uniform molecular organization, and stability, a unique feature of the surface-initiated polymerization is that it can be used for the preparation of large-area uniformly nanopatterned polymer thin films. This was demonstrated using a combination of particle lithography and surface-initiated polymerization. In general, surface-initiated polymerization is not limited to polythiophene but can be also expanded toward other classes of semiconducting polymers and copolymers. C1 [Youm, Sang Gil; Hwang, Euiyong; Chavez, Carlos A.; Li, Xin; Chatterjee, Sourav; Lusker, Kathie L.; Lu, Lu; Garno, Jayne C.; Nesterov, Evgueni E.] Louisiana State Univ, Dept Chem, Baton Rouge, LA 70803 USA. [Strzalka, Joseph] Argonne Natl Lab, Xray Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Ankner, John F.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Losovyj, Yaroslav] Indiana Univ, Dept Chem, Bloomington, IN 47401 USA. RP Nesterov, EE (reprint author), Louisiana State Univ, Dept Chem, Baton Rouge, LA 70803 USA. EM een@lsu.edu RI Lu, Lu/J-6646-2016 FU U.S. Department of Energy under EPSCoR [DE-SC0012432]; Louisiana Board of Regents; National Science Foundation [DMR-1006336]; NSF Graduate Research Fellowship Program [DGE-127192]; NSF [DMR MRI-1126394] FX This research was supported by the U.S. Department of Energy under EPSCoR Grant No. DE-SC0012432 with additional support from the Louisiana Board of Regents. The initial experimental studies were supported by the National Science Foundation (grant DMR-1006336). C.A.C. was supported by the NSF Graduate Research Fellowship Program (DGE-127192). Access to XPS at Nanoscale Characterization Facility of Indiana University Nanoscience Center was provided by NSF award DMR MRI-1126394. NR 102 TC 2 Z9 2 U1 18 U2 38 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0897-4756 EI 1520-5002 J9 CHEM MATER JI Chem. Mat. PD JUL 12 PY 2016 VL 28 IS 13 BP 4787 EP 4804 DI 10.1021/acs.chemmater.6b01957 PG 18 WC Chemistry, Physical; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DR1ZJ UT WOS:000379704100031 ER PT J AU Holzmann, M Clay, RC Morales, MA Tubman, NM Ceperley, DM Pierleoni, C AF Holzmann, Markus Clay, Raymond C., III Morales, Miguel A. Tubman, Norm M. Ceperley, David M. Pierleoni, Carlo TI Theory of finite size effects for electronic quantum Monte Carlo calculations of liquids and solids SO PHYSICAL REVIEW B LA English DT Article ID MANY-BODY SIMULATIONS; GROUND-STATE; HYDROGEN; DIMENSIONS; GAS AB Concentrating on zero temperature quantum Monte Carlo calculations of electronic systems, we give a general description of the theory of finite size extrapolations of energies to the thermodynamic limit based on one- and two-body correlation functions. We introduce effective procedures, such as using the potential and wave function split up into long and short range functions to simplify the method, and we discuss how to treat backflow wave functions. Then we explicitly test the accuracy of our method to correct finite size errors on example hydrogen and helium many-body systems and show that the finite size bias can be drastically reduced for even small systems. C1 [Holzmann, Markus] Univ Paris 06, CNRS, UMR 7600, LPTMC, F-75005 Paris, France. [Holzmann, Markus] Univ Grenoble Alpes, UMR 5493, LPMMC, CNRS, F-38042 Grenoble, France. [Holzmann, Markus] Inst Laue Langevin, BP 156, F-38042 Grenoble 9, France. [Clay, Raymond C., III; Tubman, Norm M.; Ceperley, David M.] Univ Illinois, Urbana, IL 61801 USA. [Morales, Miguel A.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Pierleoni, Carlo] Univ Aquila, Dept Phys & Chem Sci, Via Vetoio 10, I-67010 Laquila, Italy. RP Holzmann, M (reprint author), Univ Paris 06, CNRS, UMR 7600, LPTMC, F-75005 Paris, France.; Holzmann, M (reprint author), Univ Grenoble Alpes, UMR 5493, LPMMC, CNRS, F-38042 Grenoble, France.; Holzmann, M (reprint author), Inst Laue Langevin, BP 156, F-38042 Grenoble 9, France. RI Pierleoni, Carlo/D-5519-2016 OI Pierleoni, Carlo/0000-0001-9188-3846 FU Italian Institute of Technology (IIT) under the SEED project [259 SIMBEDD]; U.S. Department of Energy at the Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; Predictive Theory and Modeling for Materials and Chemical Science program by the Basic Energy Science (BES); Scientific Discovery through Advanced Computing (SciDAC) program - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences; DOE [NA DE-NA0001789]; NanoSciences Fondation (Grenoble); PRACE projects [2011050781, 2013091918]; National Science Foundation [OCI 07-25070]; state of Illinois; CNRS-IDRIS [i2014051801] FX C.P. was partially supported by the Italian Institute of Technology (IIT) under the SEED project Grant No. 259 SIMBEDD. M.A.M. was supported by the U.S. Department of Energy at the Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. M.A.M. and R.C. were supported through the Predictive Theory and Modeling for Materials and Chemical Science program by the Basic Energy Science (BES). N.M.T. was supported through the Scientific Discovery through Advanced Computing (SciDAC) program funded by the U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences. D.M.C. and R.C. were supported by DOE Grant No. NA DE-NA0001789 and by the NanoSciences Fondation (Grenoble). M.H. and C.P. thank the Theory Group at ILL Grenoble for hospitality. Computer time was provided by PRACE projects 2011050781 and 2013091918 and by an allocation on the Blue Waters sustained-petascale computing project, supported by the National Science Foundation (award number OCI 07-25070) and the state of Illinois, and by CNRS-IDRIS, Project No. i2014051801. NR 54 TC 3 Z9 3 U1 1 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 12 PY 2016 VL 94 IS 3 AR 035126 DI 10.1103/PhysRevB.94.035126 PG 16 WC Physics, Condensed Matter SC Physics GA DQ9AI UT WOS:000379502400001 ER PT J AU Shamblin, J Calder, S Dun, ZL Lee, M Choi, ES Neuefeind, J Zhou, HD Lang, M AF Shamblin, Jacob Calder, Stuart Dun, Zhiling Lee, Minseong Choi, Eun Sang Neuefeind, Joerg Zhou, Haidong Lang, Maik TI Crystal structure and partial Ising-like magnetic ordering of orthorhombic Dy2TiO5 SO PHYSICAL REVIEW B LA English DT Article ID ZERO-POINT ENTROPY; SPIN-ICE; DYSPROSIUM TITANATE; LN(2)TIO(5) LN; NUCLEAR-WASTE; GD; DY; IMMOBILIZATION; PLUTONIUM; CERAMICS AB The structure andmagnetic properties of orthorhombic Dy2TiO5 have been investigated using x-ray diffraction, neutron diffraction, and alternating current (ac)/direct current (dc) magnetic susceptibility measurements. We report a continuous structural distortion below 100 K characterized by negative thermal expansion in the [0 1 0] direction. Neutron diffraction and magnetic susceptibility measurements revealed that two-dimensional (2D) magnetic ordering begins at 3.1 K, which is followed by a three-dimensional magnetic transition at 1.7 K. The magnetic structure has been solved through a representational analysis approach and can be indexed with the propagation vector k = [0 1/2 0]. The spin structure corresponds to a coplanar model of interwoven 2D "sheets" extending in the [0 1 0] direction. The local crystal field is different for each Dy3+ ion (Dy1 and Dy2), one of which possesses strong uniaxial symmetry indicative of Ising-like magnetic ordering. Consequently, two succeeding transitions under magnetic field are observed in the ac susceptibility, which are associated with flipping each Dy3+ spin independently. C1 [Shamblin, Jacob; Lang, Maik] Univ Tennessee, Dept Nucl Engn, Knoxville, TN 37996 USA. [Shamblin, Jacob; Dun, Zhiling; Zhou, Haidong] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Calder, Stuart] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Lee, Minseong; Choi, Eun Sang] Florida State Univ, Dept Phys, Tallahassee, FL 32306 USA. [Lee, Minseong] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA. [Neuefeind, Joerg] Oak Ridge Natl Lab, Chem & Engn Mat Div, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Zhou, HD (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. EM HZhou10@utk.edu; MLang2@utk.edu RI Zhou, Haidong/O-4373-2016; Lee, Minseong/D-5371-2016; Dun, Zhiling/F-5617-2016; OI Dun, Zhiling/0000-0001-6653-3051; Shamblin, Jacob/0000-0002-1799-5353 FU Organized Research Unit funding through the University of Tennessee Office of Research; National Science Foundation (NSF) [NSF-DMR-1350002]; NSF [DMR-1157490]; State of Florida; Material's Science of Actinides, an Energy Frontier Research Center - US Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0001089] FX J.S. acknowledges support from Organized Research Unit funding through the University of Tennessee Office of Research. Z.L.D. and H.D.Z. acknowledge support from the National Science Foundation (NSF) Contract No. NSF-DMR-1350002. A portion of this research used resources at the High Flux Isotope Reactor and Spallation Neutron Source, a DOE Office of Science User Facility operated by the Oak Ridge National Laboratory. A portion of this work was performed at the National High Magnetic Field Laboratory, which is supported by NSF Cooperative Agreement No. DMR-1157490 and the State of Florida. M.L.'s effort and the sample preparation were supported as a part of the Material's Science of Actinides, an Energy Frontier Research Center funded by the US Department of Energy, Office of Science, Basic Energy Sciences under Award No. DE-SC0001089. NR 26 TC 0 Z9 0 U1 8 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 12 PY 2016 VL 94 IS 2 AR 024413 DI 10.1103/PhysRevB.94.024413 PG 10 WC Physics, Condensed Matter SC Physics GA DQ8ZT UT WOS:000379500900004 ER PT J AU Wakeham, N Rosa, PFS Wang, YQ Kang, M Fisk, Z Ronning, F Thompson, JD AF Wakeham, N. Rosa, P. F. S. Wang, Y. Q. Kang, M. Fisk, Z. Ronning, F. Thompson, J. D. TI Low-temperature conducting state in two candidate topological Kondo insulators: SmB6 and Ce3Bi4Pt3 SO PHYSICAL REVIEW B LA English DT Article ID NEUTRON-IRRADIATION; MAGNETIC-FIELDS; SURFACE-STATES; SPIN TEXTURE; GAP AB We have investigated the low-temperature conducting state of two Kondo insulators, SmB6 and Ce3Bi4Pt3, which have been theoretically predicted to host topological surface states. Through comparison of the specific heat of as-grown and powdered single crystals of SmB6, we show that the residual term that is linear in temperature is not dominated by any surface state contribution, but rather is a bulk property. In Ce3Bi4Pt3, we find that the Hall coefficient is independent of sample thickness, which indicates that conduction at low temperatures is dominated by the bulk of the sample, and not by a surface state. The low-temperature resistivity of Ce3Bi4Pt3 is found to monotonically decrease with low concentrations of disorder introduced through ion irradiation. This is in contrast to SmB6, which is again indicative of the contrasting origins of the low-temperature conduction. In SmB6, we also show that the effect of low concentrations of irradiation damage of the surface with Fe+ ions is qualitatively consistent with damage with nonmagnetic ions. C1 [Wakeham, N.; Rosa, P. F. S.; Wang, Y. Q.; Kang, M.; Ronning, F.; Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Fisk, Z.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. RP Wakeham, N (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. OI Ronning, Filip/0000-0002-2679-7957; Ferrari Silveira Rosa, Priscila/0000-0002-3437-548X; Kang, Min Gu/0000-0001-6991-0481 FU Los Alamos National Laboratory LDRD program; Los Alamos LDRD program; US Department of Energy, Office of Science FX N.W., Y.Q.W., and J.D.T. acknowledge the support of the Los Alamos National Laboratory LDRD program. P.F.S.R. acknowledges a Director's Postdoctoral Fellowship supported through the Los Alamos LDRD program. The work of F.R. was performed under the auspices of the US Department of Energy, Office of Science. The ion implantation facility was partially supported by the Center for Integrated Nanotechnologies (CINT), a DOE nanoscience user facility jointly operated by Los Alamos and Sandia National Laboratories. NR 35 TC 2 Z9 2 U1 17 U2 24 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 12 PY 2016 VL 94 IS 3 AR 035127 DI 10.1103/PhysRevB.94.035127 PG 5 WC Physics, Condensed Matter SC Physics GA DQ9AI UT WOS:000379502400002 ER PT J AU Koeller, J Leichenauer, S AF Koeller, Jason Leichenauer, Stefan TI Holographic proof of the quantum null energy condition SO PHYSICAL REVIEW D LA English DT Article ID ADS/CFT CORRESPONDENCE; ENTANGLEMENT ENTROPY; FIELD-THEORIES; BLACK-HOLES; ANOMALIES; SPACETIME; DENSITY AB We use holography to prove the quantum null energy condition (QNEC) at leading order in large N for CFTs and relevant deformations of CFTs in Minkowski space which have Einstein gravity duals. Given any codimension-two surface Sigma which is locally stationary under a null deformation in the direction k at the point p, the QNEC is a lower bound on the energy-momentum tensor at p in terms of the second variation of the entropy to one side of Sigma: < T-kk > >= S ''/2 pi root h. In a CFT, conformal transformations of this inequality give results which apply when Sigma is not locally stationary. The QNEC was proven previously for free theories, and taken together with our result this provides strong evidence that the QNEC is a true statement about quantum field theory in general. C1 [Koeller, Jason] Univ Calif Berkeley, Ctr Theoret Phys, Berkeley, CA 94720 USA. [Koeller, Jason] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Leichenauer, Stefan] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Koeller, J (reprint author), Univ Calif Berkeley, Ctr Theoret Phys, Berkeley, CA 94720 USA.; Koeller, J (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Leichenauer, S (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM jkoeller@berkeley.edu; sleichen@berkeley.edu FU Berkeley Center for Theoretical Physics; National Science Foundation [1214644, 1316783, 1521446]; fqxi [RFP3-1323]; US Department of Energy [DE-AC02-05CH11231] FX We would like to thank C. Akers, R. Bousso, X. Dong, Z. Fisher, M. Mezei, M. Moosa, and A. Wall for discussions. We would also like to thank N. Curington for help with the figures. The work of J. K. and S. L. is supported in part by the Berkeley Center for Theoretical Physics, by the National Science Foundation (Grants No. 1214644, No. 1316783, and No. 1521446), by fqxi Grant No. RFP3-1323, and by the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 67 TC 6 Z9 6 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 12 PY 2016 VL 94 IS 2 AR 024026 DI 10.1103/PhysRevD.94.024026 PG 14 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DQ9DQ UT WOS:000379511000004 ER PT J AU Buchmann, LF Schreppler, S Kohler, J Spethmann, N Stamper-Kurn, DM AF Buchmann, L. F. Schreppler, S. Kohler, J. Spethmann, N. Stamper-Kurn, D. M. TI Complex Squeezing and Force Measurement Beyond the Standard Quantum Limit SO PHYSICAL REVIEW LETTERS LA English DT Article ID BICHROMATIC LOCAL OSCILLATOR; CAVITY OPTOMECHANICS; RADIATION PRESSURE; NOISE REDUCTION; LIGHT; STATES; RESONATOR; MOTION AB A continuous quantum field, such as a propagating beam of light, may be characterized by a squeezing spectrum that is inhomogeneous in frequency. We point out that homodyne detectors, which are commonly employed to detect quantum squeezing, are blind to squeezing spectra in which the correlation between amplitude and phase fluctuations is complex. We find theoretically that such complex squeezing is a component of ponderomotive squeezing of light through cavity optomechanics. We propose a detection scheme called synodyne detection, which reveals complex squeezing and allows the accounting of measurement backaction. Even with the optomechanical system subject to continuous measurement, such detection allows the measurement of one component of an external force with sensitivity only limited by the mechanical oscillator's thermal occupation. C1 [Buchmann, L. F.] Aarhus Univ, Dept Phys & Astron, Ny Munkegade 120, DK-8000 Aarhus C, Denmark. [Buchmann, L. F.; Schreppler, S.; Kohler, J.; Spethmann, N.; Stamper-Kurn, D. M.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Spethmann, N.] Tech Univ Kaiserslautern, Fachbereich Phys, D-67663 Kaiserslautern, Germany. [Stamper-Kurn, D. M.] Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. RP Buchmann, LF (reprint author), Aarhus Univ, Dept Phys & Astron, Ny Munkegade 120, DK-8000 Aarhus C, Denmark.; Buchmann, LF (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM lbuchmann@phys.au.dk OI Kohler, Jonathan/0000-0003-3881-1514 FU Air Force Office of Scientific Research; Villum Foundation Center of Excellence; National Science Foundation; Marie Curie International Outgoing Fellowship; U.S. Department of Defense through the National Defense Science and Engineering Graduate Fellowship Program; Swiss National Science Foundation FX This work was supported by the Air Force Office of Scientific Research, the Villum Foundation Center of Excellence, and National Science Foundation. N. S. was supported by a Marie Curie International Outgoing Fellowship, J. K. and S. S. by the U.S. Department of Defense through the National Defense Science and Engineering Graduate Fellowship Program, and L. F. B. by the Swiss National Science Foundation. L. F. B. acknowledges helpful discussions with K. Molmer, D. Petrosyan, and N. Kampel. NR 40 TC 4 Z9 4 U1 6 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 12 PY 2016 VL 117 IS 3 AR 030801 DI 10.1103/PhysRevLett.117.030801 PG 6 WC Physics, Multidisciplinary SC Physics GA DQ9EZ UT WOS:000379514500002 PM 27472106 ER PT J AU Weng, YK Lin, LF Dagotto, E Dong, S AF Weng, Yakui Lin, Lingfang Dagotto, Elbio Dong, Shuai TI Inversion of Ferrimagnetic Magnetization by Ferroelectric Switching via a Novel Magnetoelectric Coupling SO PHYSICAL REVIEW LETTERS LA English DT Article ID THIN-FILMS; OXIDE HETEROSTRUCTURES; ELECTRIC-FIELD; BIFEO3; REVERSAL; TRANSITIONS; INTERFACE; MULTIFERROICS; POLARIZATION; CRYSTAL AB Although several multiferroic materials or heterostructures have been extensively studied, finding strong magnetoelectric couplings for the electric field control of the magnetization remains challenging. Here, a novel interfacial magnetoelectric coupling based on three components (ferroelectric dipole, magnetic moment, and antiferromagnetic order) is analytically formulated. As an extension of carrier-mediated magnetoelectricity, the new coupling is shown to induce an electric-magnetic hysteresis loop. Realizations employing BiFeO3 bilayers grown along the [111] axis are proposed. Without involving magnetic phase transitions, the magnetization orientation can be switched by the carrier modulation driven by the field effect, as confirmed using first-principles calculations. C1 [Weng, Yakui; Lin, Lingfang; Dong, Shuai] Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. [Dagotto, Elbio] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Dagotto, Elbio] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA. RP Dong, S (reprint author), Southeast Univ, Dept Phys, Nanjing 211189, Jiangsu, Peoples R China. EM sdong@seu.edu.cn RI Dong (董), Shuai (帅)/A-5513-2008 OI Dong (董), Shuai (帅)/0000-0002-6910-6319 FU National Natural Science Foundation of China [11274060, 51322206]; Fundamental Research Funds for the Central Universities; Scientific Research Foundation of Graduate School of Southeast University [YBJJ1619]; Jiangsu Innovation Projects for Graduate Student [KYLX15_0112]; U.S. DOE, Office of Basic Energy Sciences, Materials Sciences and Engineering Division FX We acknowledge discussions with Hangwen Guo, Pu Yu, Xiaofang Zhai, Jinxing Zhang, and Junling Wang. This work was mainly supported by the National Natural Science Foundation of China (Grants No. 11274060 and No. 51322206), the Fundamental Research Funds for the Central Universities, Scientific Research Foundation of Graduate School of Southeast University (Grant No. YBJJ1619), and Jiangsu Innovation Projects for Graduate Student (Grant No. KYLX15_0112). E. D. was supported by the U.S. DOE, Office of Basic Energy Sciences, Materials Sciences and Engineering Division. NR 62 TC 2 Z9 2 U1 40 U2 77 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 12 PY 2016 VL 117 IS 3 AR 037601 DI 10.1103/PhysRevLett.117.037601 PG 6 WC Physics, Multidisciplinary SC Physics GA DQ9EZ UT WOS:000379514500016 PM 27472140 ER PT J AU Luo, D Wang, F Zhu, JY Cao, F Liu, Y Li, XG Willson, RC Yang, ZZ Chu, CW Ren, ZF AF Luo, Dan Wang, Feng Zhu, Jingyi Cao, Feng Liu, Yuan Li, Xiaogang Willson, Richard C. Yang, Zhaozhong Chu, Ching-Wu Ren, Zhifeng TI Nanofluid of graphene-based amphiphilic Janus nanosheets for tertiary or enhanced oil recovery: High performance at low concentration SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE nanofluid flooding; amphiphilic Janus nanosheets; enhanced oil recovery; climbing film; interfacial film ID WETTABILITY ALTERATION; SOLIDS; OXIDE; NANOPARTICLES; INTERFACES; PARTICLES; MECHANISM; DROPS AB The current simple nanofluid flooding method for tertiary or enhanced oil recovery is inefficient, especially when used with low nanoparticle concentration. We have designed and produced a nanofluid of graphene-based amphiphilic nanosheets that is very effective at low concentration. Our nanosheets spontaneously approached the oil-water interface and reduced the interfacial tension in a saline environment (4 wt % NaCl and 1 wt % CaCl2), regardless of the solid surface wettability. A climbing film appeared and grew at moderate hydrodynamic condition to encapsulate the oil phase. With strong hydrodynamic power input, a solid-like interfacial film formed and was able to return to its original form even after being seriously disturbed. The film rapidly separated oil and water phases for slug-like oil displacement. The unique behavior of our nanosheet nanofluid tripled the best performance of conventional nanofluid flooding methods under similar conditions. C1 [Luo, Dan; Wang, Feng; Cao, Feng; Liu, Yuan; Chu, Ching-Wu; Ren, Zhifeng] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Luo, Dan; Wang, Feng; Cao, Feng; Liu, Yuan; Chu, Ching-Wu; Ren, Zhifeng] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Luo, Dan; Willson, Richard C.] Univ Houston, Dept Chem & Biomol Engn, Houston, TX 77204 USA. [Luo, Dan; Zhu, Jingyi; Li, Xiaogang; Yang, Zhaozhong] Southwest Petr Univ, State Key Lab Oil & Gas Reservoir Geol & Exploita, Chengdu 610500, Sichuan, Peoples R China. [Willson, Richard C.] Tecnol Monterrey, Dept Biotecnol & Ingn Alimentos, Monterrey 64849, Nuevo Leon, Mexico. [Chu, Ching-Wu] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Chu, CW; Ren, ZF (reprint author), Univ Houston, Dept Phys, Houston, TX 77204 USA.; Chu, CW; Ren, ZF (reprint author), Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA.; Yang, ZZ (reprint author), Southwest Petr Univ, State Key Lab Oil & Gas Reservoir Geol & Exploita, Chengdu 610500, Sichuan, Peoples R China.; Chu, CW (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM Yangzhaozhong@swpu.edu.cn; cwchu@uh.edu; zren@uh.edu FU US Department of Energy [DE-FG02-13ER46917/DE-SC0010831]; US Air Force Office of Scientific Research [FA9550-15-1-0236]; T.L.L. Temple Foundation; John J. and Rebecca Moores Endowment; State of Texas through the Texas Center for Superconductivity at the University of Houston FX We thank Ishwar Mishra and Prof. Dong Cai in the Department of Physics, University of Houston, for providing particle size analysis on Malvern NS300. The work performed at University of Houston is supported in part by the US Department of Energy under Contract DE-FG02-13ER46917/DE-SC0010831, US Air Force Office of Scientific Research Grant FA9550-15-1-0236, the T.L.L. Temple Foundation, the John J. and Rebecca Moores Endowment, and the State of Texas through the Texas Center for Superconductivity at the University of Houston. NR 23 TC 0 Z9 0 U1 21 U2 45 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 12 PY 2016 VL 113 IS 28 BP 7711 EP 7716 DI 10.1073/pnas.1608135113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR1VX UT WOS:000379694100028 PM 27354529 ER PT J AU Parazoo, NC Commane, R Wofsy, SC Koven, CD Sweeney, C Lawrence, DM Lindaas, J Chang, RYW Miller, CE AF Parazoo, Nicholas C. Commane, Roisin Wofsy, Steven C. Koven, Charles D. Sweeney, Colm Lawrence, David M. Lindaas, Jakob Chang, Rachel Y. -W. Miller, Charles E. TI Detecting regional patterns of changing CO2 flux in Alaska SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE carbon cycle; permafrost thaw; climate; Earth system models; remote sensing ID NORTHERN ECOSYSTEMS; SATELLITE-OBSERVATIONS; CARBON-DIOXIDE; PERMAFROST; CLIMATE; CYCLE; AIRCRAFT; DYNAMICS; EXCHANGE; FEEDBACK AB With rapid changes in climate and the seasonal amplitude of carbon dioxide (CO2) in the Arctic, it is critical that we detect and quantify the underlying processes controlling the changing amplitude of CO2 to better predict carbon cycle feedbacks in the Arctic climate system. We use satellite and airborne observations of atmospheric CO2 with climatically forced CO2 flux simulations to assess the detectability of Alaskan carbon cycle signals as future warming evolves. We find that current satellite remote sensing technologies can detect changing uptake accurately during the growing season but lack sufficient cold season coverage and near-surface sensitivity to constrain annual carbon balance changes at regional scale. Airborne strategies that target regular vertical profile measurements within continental interiors are more sensitive to regional flux deeper into the cold season but currently lack sufficient spatial coverage throughout the entire cold season. Thus, the current CO2 observing network is unlikely to detect potentially large CO2 sources associated with deep permafrost thaw and cold season respiration expected over the next 50 y. Although continuity of current observations is vital, strategies and technologies focused on cold season measurements (active remote sensing, aircraft, and tall towers) and systematic sampling of vertical profiles across continental interiors over the full annual cycle are required to detect the onset of carbon release from thawing permafrost. C1 [Parazoo, Nicholas C.; Miller, Charles E.] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Parazoo, Nicholas C.] Univ Calif Los Angeles, Joint Inst Reg Earth Syst Sci & Engn, Los Angeles, CA 90095 USA. [Commane, Roisin; Wofsy, Steven C.; Lindaas, Jakob] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA. [Commane, Roisin; Wofsy, Steven C.] Harvard Univ, Harvard Sch Engn & Appl Sci, Cambridge, MA 02138 USA. [Koven, Charles D.] Lawrence Berkeley Natl Lab, Climate & Ecosyst Sci Div, Berkeley, CA 94720 USA. [Sweeney, Colm] NOAA, Earth Syst Res Lab, Boulder, CO 80305 USA. [Sweeney, Colm] Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA. [Lawrence, David M.] Natl Ctr Atmospher Res, Climate & Global Dynam Lab, Boulder, CO 80302 USA. [Lindaas, Jakob] Colorado State Univ, Dept Atmospher Sci, Ft Collins, CO 80523 USA. [Chang, Rachel Y. -W.] Dalhousie Univ, Dept Phys & Atmospher Sci, Halifax, NS B3H 4R2, Canada. RP Parazoo, NC (reprint author), CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA.; Parazoo, NC (reprint author), Univ Calif Los Angeles, Joint Inst Reg Earth Syst Sci & Engn, Los Angeles, CA 90095 USA. EM nicholas.c.parazoo@jpl.nasa.gov RI Koven, Charles/N-8888-2014; OI Koven, Charles/0000-0002-3367-0065; Lindaas, Jakob/0000-0003-1872-3162; Commane, Roisin/0000-0003-1373-1550 FU NASA; Office of Science, Office of Biological and Environmental Research (BER) of the US Department of Energy (DOE) [DE-AC02-05CH11231]; US DOE, BER [DE-FC03-97ER62402/A010]; NSF [PLR-1304220] FX Some of the research described was performed for CARVE, an Earth Ventures (EV-1) investigation, under contract with NASA. A portion of this research was carried out at the Jet Propulsion Laboratory, California Institute of Technology under a contract with NASA. C.D.K. was supported by the Director, Office of Science, Office of Biological and Environmental Research (BER) of the US Department of Energy (DOE) Contract DE-AC02-05CH11231 as part of their Regional and Global Climate Modeling (BGC-Feedbacks SFA) and Terrestrial Ecosystem Science (NGEE-Arctic) Programs. D.M.L. was supported by the US DOE, BER as part of Climate Change Prediction Program Cooperative Agreement DE-FC03-97ER62402/A010 and by NSF Grant PLR-1304220. NR 36 TC 0 Z9 0 U1 13 U2 20 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 12 PY 2016 VL 113 IS 28 BP 7733 EP 7738 DI 10.1073/pnas.1601085113 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR1VX UT WOS:000379694100032 PM 27354511 ER PT J AU Hatzenpichler, R Connon, SA Goudeau, D Malmstrom, RR Woyke, T Orphan, VJ AF Hatzenpichler, Roland Connon, Stephanie A. Goudeau, Danielle Malmstrom, Rex R. Woyke, Tanja Orphan, Victoria J. TI Visualizing in situ translational activity for identifying and sorting slow-growing archaeal-bacterial consortia SO PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA LA English DT Article DE activity-based cell sorting; BONCAT; click chemistry; ecophysiology; single-cell microbiology ID SULFATE-REDUCING BACTERIA; NEWLY SYNTHESIZED PROTEINS; SINGLE-CELL GENOMICS; TARGETED OLIGONUCLEOTIDE PROBES; METHANE-OXIDIZING ARCHAEA; ANAEROBIC OXIDATION; RIBOSOMAL-RNA; METHANOTROPHIC ARCHAEA; MICROBIAL CONSORTIA; MAMMALIAN-CELLS AB To understand the biogeochemical roles of microorganisms in the environment, it is important to determine when and under which conditions they are metabolically active. Bioorthogonal noncanonical amino acid tagging (BONCAT) can reveal active cells by tracking the incorporation of synthetic amino acids into newly synthesized proteins. The phylogenetic identity of translationally active cells can be determined by combining BONCAT with rRNA-targeted fluorescence in situ hybridization (BONCAT-FISH). In theory, BONCAT-labeled cells could be isolated with fluorescence-activated cell sorting (BONCAT-FACS) for subsequent genetic analyses. Here, in the first application, to our knowledge, of BONCAT-FISH and BONCAT-FACS within an environmental context, we probe the translational activity of microbial consortia catalyzing the anaerobic oxidation of methane (AOM), a dominant sink of methane in the ocean. These consortia, which typically are composed of anaerobic methane-oxidizing archaea (ANME) and sulfate-reducing bacteria, have been difficult to study due to their slow in situ growth rates, and fundamental questions remain about their ecology and diversity of interactions occurring between ANME and associated partners. Our activity-correlated analyses of >16,400 microbial aggregates provide the first evidence, to our knowledge, that AOM consortia affiliated with all five major ANME clades are concurrently active under controlled conditions. Surprisingly, sorting of individual BONCAT-labeled consortia followed by whole-genome amplification and 16S rRNA gene sequencing revealed previously unrecognized interactions of ANME with members of the poorly understood phylum Verrucomicrobia. This finding, together with our observation that ANME-associated Verrucomicrobia are found in a variety of geographically distinct methane seep environments, suggests a broader range of symbiotic relationships within AOM consortia than previously thought. C1 [Hatzenpichler, Roland; Connon, Stephanie A.; Orphan, Victoria J.] CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. [Goudeau, Danielle; Malmstrom, Rex R.; Woyke, Tanja] Joint Genome Inst, Dept Energy, Walnut Creek, CA 94598 USA. RP Hatzenpichler, R; Orphan, VJ (reprint author), CALTECH, Div Geol & Planetary Sci, Pasadena, CA 91125 USA. EM hatzenpichler@caltech.edu; vorphan@gps.caltech.edu FU National Science Foundation [OCE-0825791]; Erwin Schrodinger Postdoctoral Fellowship from the Austrian Science Fund (FWF) [J 3162-B20]; Center for Dark Energy Biosphere Investigations (C-DEBI); Gordon and Betty Moore Foundation [GBMF3780]; Department of Energy (DOE) [DE-PS02-09ER09-25]; JGI Director Discretionary Project Award; [DE-AC02-05CH11231] FX We thank Alexis Pasulka and Kat Dawson for shipboard sample processing, Silvan Scheller and Kat Dawson for measurements of AOM rates and methane concentrations, Hang Yu for performing cline assays, Connor Skennerton for help during sampling of sediment incubations, David Case for discussions on tag sequence analyses, and Shawn McGlynn for discussions on storage compounds. David Case, Kat Dawson, and Elizabeth Wilbanks are acknowledged for critical comments on the manuscript. We thank The Biological Imaging Facility of California Institute of Technology for access to their confocal microscope. We thank the crew and pilots of R/V Atlantis Cruises AT-15-68 and AT-18-10 to Hydrate Ridge (supported by National Science Foundation Grant OCE-0825791) and the R/V Western Flyer Cruise to Santa Monica Basin run by the Monterey Bay Aquarium Research Institute. R.H. was supported by an Erwin Schrodinger Postdoctoral Fellowship from the Austrian Science Fund (FWF) (project no. J 3162-B20), and a postdoctoral fellowship from the Center for Dark Energy Biosphere Investigations (C-DEBI). Funding for this project was provided by Gordon and Betty Moore Foundation Grant GBMF3780 (to V.J.O.), Department of Energy (DOE) Grant DE-PS02-09ER09-25 (to V.J.O.), and a JGI Director Discretionary Project Award (to R.H. and V.J.O.). The work conducted by the DOE Joint Genome Institute, a DOE Office of Science User Facility, is supported under Contract DE-AC02-05CH11231. This is C-DEBI Contribution 330. NR 96 TC 2 Z9 2 U1 19 U2 38 PU NATL ACAD SCIENCES PI WASHINGTON PA 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA SN 0027-8424 J9 P NATL ACAD SCI USA JI Proc. Natl. Acad. Sci. U. S. A. PD JUL 12 PY 2016 VL 113 IS 28 BP E4069 EP E4078 DI 10.1073/pnas.1603757113 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR1VX UT WOS:000379694100013 PM 27357680 ER PT J AU Bang, W Albright, BJ Bradley, PA Vold, EL Boettger, JC Fernandez, JC AF Bang, W. Albright, B. J. Bradley, P. A. Vold, E. L. Boettger, J. C. Fernandez, J. C. TI Linear dependence of surface expansion speed on initial plasma temperature in warm dense matter SO SCIENTIFIC REPORTS LA English DT Article ID ION-BEAMS; LASER; SCATTERING; DIAMOND; CARBON; STATE; GOLD AB Recent progress in laser-driven quasi-monoenergetic ion beams enabled the production of uniformly heated warm dense matter. Matter heated rapidly with this technique is under extreme temperatures and pressures, and promptly expands outward. While the expansion speed of an ideal plasma is known to have a square-root dependence on temperature, computer simulations presented here show a linear dependence of expansion speed on initial plasma temperature in the warm dense matter regime. The expansion of uniformly heated 1-100 eV solid density gold foils was modeled with the RAGE radiation-hydrodynamics code, and the average surface expansion speed was found to increase linearly with temperature. The origin of this linear dependence is explained by comparing predictions from the SESAME equation-of-state tables with those from the ideal gas equation-of-state. These simulations offer useful insight into the expansion of warm dense matter and motivate the application of optical shadowgraphy for temperature measurement. C1 [Bang, W.; Albright, B. J.; Bradley, P. A.; Vold, E. L.; Boettger, J. C.; Fernandez, J. C.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Bang, W (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM wbang@lanl.gov RI Bang, Woosuk/E-8135-2015; Fernandez, Juan/H-3268-2011; OI Bang, Woosuk/0000-0002-4259-1342; Fernandez, Juan/0000-0002-1438-1815; Albright, Brian/0000-0002-7789-6525; Bradley, Paul/0000-0001-6229-6677 FU U.S. Department of Energy by the Los Alamos National Security, LLC, Los Alamos National Laboratory [DE-AC52-06NA25396]; LANL LDRD program FX This work was performed under the auspices of the U.S. Department of Energy by the Los Alamos National Security, LLC, Los Alamos National Laboratory under Contract No. DE-AC52-06NA25396 and was supported in part by the LANL LDRD program. NR 35 TC 1 Z9 1 U1 9 U2 17 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 12 PY 2016 VL 6 AR 29441 DI 10.1038/srep29441 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DQ7LP UT WOS:000379389200001 PM 27405664 ER PT J AU Akyol, M Jiang, WJ Yu, GQ Fan, YB Gunes, M Ekicibil, A Amiri, PK Wang, KL AF Akyol, Mustafa Jiang, Wanjun Yu, Guoqiang Fan, Yabin Gunes, Mustafa Ekicibil, Ahmet Amiri, Pedram Khalili Wang, Kang L. TI Effect of heavy metal layer thickness on spin-orbit torque and current-induced switching in Hf broken vertical bar CoFeB broken vertical bar MgO structures SO APPLIED PHYSICS LETTERS LA English DT Article ID EFFECTIVE-FIELD; DOMAIN-WALLS; HETEROSTRUCTURES; DRIVEN AB We study the heavy metal layer thickness dependence of the current-induced spin-orbit torque (SOT) in perpendicularly magnetized Hf broken vertical bar CoFeB broken vertical bar MgO multilayer structures. The damping-like (DL) current-induced SOT is determined by vector anomalous Hall effect measurements. A non-monotonic behavior in the DL-SOT is found as a function of the thickness of the heavy-metal layer. The sign of the DL-SOT changes with increasing the thickness of the Hf layer in the trilayer structure. As a result, in the current-driven magnetization switching, the preferred direction of switching for a given current direction changes when the Hf thickness is increased above similar to 7 nm. Although there might be a couple of reasons for this unexpected behavior in DL-SOT, such as the roughness in the interfaces and/or impurity based electric potential in the heavy metal, one can deduce a roughness dependence sign reversal in DL-SOT in our trilayer structure. Published by AIP Publishing. C1 [Akyol, Mustafa; Yu, Guoqiang; Fan, Yabin; Amiri, Pedram Khalili; Wang, Kang L.] Univ Calif Los Angeles, Dept Elect Engn, Los Angeles, CA 90095 USA. [Akyol, Mustafa; Ekicibil, Ahmet] Cukurova Univ, Dept Phys, TR-01330 Adana, Turkey. [Jiang, Wanjun] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Gunes, Mustafa] Adana Sci & Technol Univ, Dept Mat Engn, TR-01180 Adana, Turkey. RP Akyol, M (reprint author), Univ Calif Los Angeles, Dept Elect Engn, Los Angeles, CA 90095 USA.; Akyol, M (reprint author), Cukurova Univ, Dept Phys, TR-01330 Adana, Turkey. RI Yu, Guoqiang/F-1871-2013 OI Yu, Guoqiang/0000-0002-7439-6920 FU NSF Nanosystems Engineering Research Center for Translational Applications of Nanoscale Multiferroic Systems (TANMS); FAME Center, one of six centers of STARnet, a Semiconductor Research Corporation (SRC) program - MARCO; DARPA; TUBITAK "The Scientific and Technological Research Council of Turkey"; Cukurova University (Adana/Turkey) [FEF2013D31] FX This work was partially supported by the NSF Nanosystems Engineering Research Center for Translational Applications of Nanoscale Multiferroic Systems (TANMS). This work was also supported in part by the FAME Center, one of six centers of STARnet, a Semiconductor Research Corporation (SRC) program sponsored by MARCO and DARPA. We would further like to acknowledge the collaboration of this research with the King Abdul-Aziz City for Science and Technology (KACST) via The Center of Excellence for Green Nanotechnologies (CEGN). M.A. would like to acknowledge TUBITAK "The Scientific and Technological Research Council of Turkey" for his financial support during this work. This work was also partially supported by Cukurova University (Adana/Turkey) under the Project No. of 2013, FEF2013D31. NR 27 TC 0 Z9 0 U1 13 U2 13 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 11 PY 2016 VL 109 IS 2 AR 022403 DI 10.1063/1.4958295 PG 5 WC Physics, Applied SC Physics GA DT0EH UT WOS:000381155200037 ER PT J AU Bates, CR Pies, C Kempf, S Hengstler, D Fleischmann, A Gastaldo, L Enss, C Friedrich, S AF Bates, C. R. Pies, C. Kempf, S. Hengstler, D. Fleischmann, A. Gastaldo, L. Enss, C. Friedrich, S. TI Reproducibility and calibration of MMC-based high-resolution gamma detectors SO APPLIED PHYSICS LETTERS LA English DT Article ID METALLIC MAGNETIC CALORIMETERS; PARTICLE-DETECTION; RAY SPECTROSCOPY; ENERGIES; EMISSION AB We describe a prototype gamma-ray detector based on a metallic magnetic calorimeter with an energy resolution of 46eV at 60 keV and a reproducible response function that follows a simple second-order polynomial. The simple detector calibration allows adding high-resolution spectra from different pixels and different cool-downs without loss in energy resolution to determine c-ray centroids with high accuracy. As an example of an application in nuclear safeguards enabled by such a c-ray detector, we discuss the non-destructive assay of Pu-242 in a mixed-isotope Pu sample. Published by AIP Publishing. C1 [Bates, C. R.; Friedrich, S.] Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. [Pies, C.; Kempf, S.; Hengstler, D.; Fleischmann, A.; Gastaldo, L.; Enss, C.] Heidelberg Univ, Kirchhoff Inst Phys, Neuenheimer Feld 227, D-69120 Heidelberg, Germany. [Bates, C. R.] Los Alamos Natl Lab, POB 1663 F663, Los Alamos, NM 87545 USA. RP Friedrich, S (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave, Livermore, CA 94550 USA. EM friedrich1@llnl.gov RI Kempf, Sebastian/P-7612-2016 OI Kempf, Sebastian/0000-0002-3303-128X FU U.S. Department of Energy, Office on Non-proliferation Research [LL12-MagMicro-PD03]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was supported by the U.S. Department of Energy, Office on Non-proliferation Research under grant LL12-MagMicro-PD03. It was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 28 TC 1 Z9 1 U1 1 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 11 PY 2016 VL 109 IS 2 AR 023513 DI 10.1063/1.4958699 PG 5 WC Physics, Applied SC Physics GA DT0EH UT WOS:000381155200067 ER PT J AU Dong, KC Lou, S Choe, HS Liu, K You, Z Yao, J Wu, JQ AF Dong, Kaichen Lou, Shuai Choe, Hwan Sung Liu, Kai You, Zheng Yao, Jie Wu, Junqiao TI Stress compensation for arbitrary curvature control in vanadium dioxide phase transition actuators SO APPLIED PHYSICS LETTERS LA English DT Article ID RESIDUAL-STRESS; THIN-FILMS; VO2; MICROACTUATORS; ELIMINATION AB Due to its thermally driven structural phase transition, vanadium dioxide (VO2) has emerged as a promising material for micro/nano-actuators with superior volumetric work density, actuation amplitude, and repetition frequency. However, the high initial curvature of VO2 actuators severely obstructs the actuation performance and application. Here, we introduce a "seesaw" method of fabricating tri-layer cantilevers to compensate for the residual stress and realize nearly arbitrary curvature control of VO2 actuators. By simply adjusting the thicknesses of the individual layers, cantilevers with positive, zero, or negative curvatures can be engineered. The actuation amplitude can be decoupled from the curvature and controlled independently as well. Based on the experimentally measured residual stresses, we demonstrate sub-micron thick VO2 actuators with nearly zero final curvature and a high actuation amplitude simultaneously. This "seesaw" method can be further extended to the curvature engineering of other microelectromechanical system multi-layer structures where large stress-mismatch between layers are inevitable. Published by AIP Publishing. C1 [Dong, Kaichen; Lou, Shuai; Choe, Hwan Sung; Yao, Jie; Wu, Junqiao] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Dong, Kaichen; Lou, Shuai; Choe, Hwan Sung; Yao, Jie; Wu, Junqiao] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Dong, Kaichen; You, Zheng] Tsinghua Univ, Dept Precis Instrument, State Key Lab Precis Measurement Technol & Instru, Beijing 100084, Peoples R China. [Liu, Kai] Tsinghua Univ, Sch Mat Sci & Engn, Beijing 100084, Peoples R China. RP Dong, KC; Wu, JQ (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Dong, KC; Wu, JQ (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Dong, KC (reprint author), Tsinghua Univ, Dept Precis Instrument, State Key Lab Precis Measurement Technol & Instru, Beijing 100084, Peoples R China. EM dkc12@mails.tsinghua.edu.cn; wuj@berkeley.edu RI Wu, Junqiao/G-7840-2011; Liu, Kai/A-4754-2012 OI Wu, Junqiao/0000-0002-1498-0148; Liu, Kai/0000-0002-0638-5189 FU U.S. Department of Energy Early Career Award [DE-FG02-11ER46796]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; Tsinghua-Berkeley Funds; China Scholarship Council (CSC) [201406210211] FX This work was supported by the U.S. Department of Energy Early Career Award No. DE-FG02-11ER46796. Some of the measurements and device fabrication used facilities in the Lawrence Berkeley National Laboratory, which was supported by the Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. Partial measurement and fabrication were done in the U.C. Berkeley Marvell Nanolab and Biomolecular Nanotechnology Center. J.W., J.Y. and K.D. acknowledge support from the Tsinghua-Berkeley Funds. K.D. acknowledges the China Scholarship Council (CSC, No. 201406210211) for financial support. The authors would thank K. Wang, C. Ko, X. Wang, Y. Chen, Z. Hou, P. Dong, X. Lei, K. Tom, and Y. Liu for helpful discussions. NR 34 TC 0 Z9 0 U1 13 U2 13 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 11 PY 2016 VL 109 IS 2 AR 023504 DI 10.1063/1.4958692 PG 5 WC Physics, Applied SC Physics GA DT0EH UT WOS:000381155200058 ER PT J AU Lee, JCT Chess, JJ Montoya, SA Shi, X Tamura, N Mishra, SK Fischer, P McMorran, BJ Sinha, SK Fullerton, EE Kevan, SD Roy, S AF Lee, J. C. T. Chess, J. J. Montoya, S. A. Shi, X. Tamura, N. Mishra, S. K. Fischer, P. McMorran, B. J. Sinha, S. K. Fullerton, E. E. Kevan, S. D. Roy, S. TI Synthesizing skyrmion bound pairs in Fe-Gd thin films SO APPLIED PHYSICS LETTERS LA English DT Article ID MAGNETIC SKYRMION; FERROMAGNETS; LATTICE; STATES AB We show that properly engineered amorphous Fe-Gd alloy thin films with perpendicular magnetic anisotropy exhibit bound pairs of like-polarity, opposite helicity skyrmions at room temperature. Magnetic mirror symmetry planes present in the stripe phase, instead of chiral exchange, determine the internal skyrmion structure and the net achirality of the skyrmion phase. Our study shows that stripe domain engineering in amorphous alloy thin films may enable the creation of skyrmion phases with technologically desirable properties. Published by AIP Publishing. C1 [Lee, J. C. T.; Chess, J. J.; Shi, X.; McMorran, B. J.; Kevan, S. D.] Univ Oregon, Dept Phys, Eugene, OR 97401 USA. [Lee, J. C. T.; Tamura, N.; Mishra, S. K.; Kevan, S. D.; Roy, S.] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Lee, J. C. T.; Fischer, P.; Kevan, S. D.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Montoya, S. A.; Fullerton, E. E.] Univ Calif San Diego, Ctr Memory & Recording Res, San Diego, CA 92093 USA. [Fischer, P.] Univ Calif Santa Cruz, Dept Phys, Santa Cruz, CA 94056 USA. [Sinha, S. K.] Univ Calif San Diego, Dept Phys, San Diego, CA 92093 USA. RP Roy, S (reprint author), Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. EM sroy@lbl.gov RI Fischer, Peter/A-3020-2010; Fullerton, Eric/H-8445-2013; McMorran, Benjamin/G-9954-2016; OI Fischer, Peter/0000-0002-9824-9343; Fullerton, Eric/0000-0002-4725-9509; McMorran, Benjamin/0000-0001-7207-1076; Tamura, Nobumichi/0000-0002-3698-2611 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering [DE-FG02-11ER46831]; U.S. Department of Energy (DOE), Office of Basic Energy Sciences [DE-SC0003678]; Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy [DE-AC02-05-CH11231]; Air Force Research Laboratory [FA8650-05-1-5041]; NSF [0923577, 0421086] FX The work at the ALS, LBNL was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy (Contract No. DE-AC02-05CH11231). The work at the University of Oregon was partially supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering under Grant No. DE-FG02-11ER46831. The research at UCSD was supported by the research programs of the U.S. Department of Energy (DOE), Office of Basic Energy Sciences (Award No. DE-SC0003678). S.K. and P.F. were supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, of the U.S. Department of Energy under Contract No. DE-AC02-05-CH11231 within the Non-Equilibrium Magnetic Materials Program at LBNL. B.J.M. and J.J.C. gratefully acknowledge the use of the CAMCOR High Resolution and Analytical Facility at University of Oregon, which is supported by the W.M. Keck Foundation, the M.J. Murdock Charitable Trust, ONAMI, the Air Force Research Laboratory (Agreement No. FA8650-05-1-5041), NSF (Award Nos. 0923577, 0421086), and the University of Oregon. NR 24 TC 1 Z9 1 U1 11 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 11 PY 2016 VL 109 IS 2 AR 022402 DI 10.1063/1.4955462 PG 4 WC Physics, Applied SC Physics GA DT0EH UT WOS:000381155200036 ER PT J AU Olson, BV Kadlec, EA Kim, JK Klem, JF Hawkins, SD Tauke-Pedretti, A Coon, WT Fortune, TR Shaner, EA AF Olson, B. V. Kadlec, E. A. Kim, J. K. Klem, J. F. Hawkins, S. D. Tauke-Pedretti, A. Coon, W. T. Fortune, T. R. Shaner, E. A. TI Contactless measurement of equilibrium electron concentrations in n-type InAs/InAs(1-x)Sb(x)type-II superlattices SO APPLIED PHYSICS LETTERS LA English DT Article AB Measurements of the equilibrium majority carrier electron concentration (n(0)) in narrow-bandgap n-type InAs/InAs1-xSbx type-II superlattices are made using contactless time-resolved microwave reflectance (TMR). By calibrating TMR decays to the number of optically injected electron -hole pairs, direct conversion to carrier lifetimes as a function of excited canier density is made arid allowing for accurate measurement of no. The temperature dependence of both n(0), and the intrinsic carrier density (n(i)) are measured using this method, where no 1 x 10(15) cm(-3) and n(i) = 1.74 x 10(11) at 100 K. These results provide non-destructive insight into critical parameters that directly determine infrared photodetector dark diffusion current. Published by AIP Publishing. C1 [Olson, B. V.; Kadlec, E. A.; Kim, J. K.; Klem, J. F.; Hawkins, S. D.; Tauke-Pedretti, A.; Coon, W. T.; Fortune, T. R.; Shaner, E. A.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Olson, B. V.] Vixar Inc, 2950 Xenium Ave, Plymouth, MN 55441 USA. RP Olson, BV (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA.; Olson, BV (reprint author), Vixar Inc, 2950 Xenium Ave, Plymouth, MN 55441 USA. EM bolson@vixarinc.com; eashane@sandia.gov OI Olson, Benjamin/0000-0003-1421-2541 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; University of Iowa FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division and in part by a subcontract through the University of Iowa. The authors thank Professor Michael Flatte at the University of Iowa for the K . p software. NR 21 TC 0 Z9 0 U1 4 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 11 PY 2016 VL 109 IS 2 AR 022105 DI 10.1063/1.4956351 PG 4 WC Physics, Applied SC Physics GA DT0EH UT WOS:000381155200031 ER PT J AU Yang, Z Albrecht, AR Cederberg, JG Sheik-Bahae, M AF Yang, Z. Albrecht, A. R. Cederberg, J. G. Sheik-Bahae, M. TI 80nm tunable DBR-free semiconductor disk laser SO APPLIED PHYSICS LETTERS LA English DT Article ID SURFACE-EMITTING LASERS; HIGH-POWER; GAIN STRUCTURES; VECSELS; WAVE; OPERATION AB We report a widely tunable optically pumped distributed Bragg reflector (DBR)-free semiconductor disk laser with 6W continuous wave output power near 1055nm when using a 2% output coupler. Using only high reflecting mirrors, the lasing wavelength is centered at 1034 nm and can be tuned up to a record 80 nm by using a birefringent filter. We attribute such wide tunability to the unique broad effective gain bandwidth of DBR-free semiconductor disk lasers achieved by eliminating the active mirror geometry. Published by AIP Publishing. C1 [Yang, Z.; Albrecht, A. R.; Sheik-Bahae, M.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Cederberg, J. G.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Cederberg, J. G.] MIT, Lincoln Lab, Lexington, MA 02420 USA. RP Sheik-Bahae, M (reprint author), Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. EM msb@unm.edu NR 32 TC 0 Z9 0 U1 5 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 11 PY 2016 VL 109 IS 2 AR 022101 DI 10.1063/1.4958164 PG 4 WC Physics, Applied SC Physics GA DT0EH UT WOS:000381155200027 ER PT J AU Zhuo, ZQ Hu, JT Duan, YD Yang, WL Pan, F AF Zhuo, Zengqing Hu, Jiangtao Duan, Yandong Yang, Wanli Pan, Feng TI Transition metal redox and Mn disproportional reaction in LiMn0.5Fe0.5PO4 electrodes cycled with aqueous electrolyte SO APPLIED PHYSICS LETTERS LA English DT Article ID RECHARGEABLE LITHIUM BATTERIES; ION BATTERIES; X-RAY; CATHODE MATERIAL; SPECTROSCOPY; PERFORMANCE; LITHIATION; STATES; SOFT AB We performed soft x-ray absorption spectroscopy (sXAS) and a quantitative analysis of the transition metal redox in the LiMn0.5Fe0.5PO4 electrodes upon electrochemical cycling. In order to circumvent the complication of the surface reactions with organic electrolyte at high potential, the LiMn0.5Fe0.5PO4 electrodes are cycled with aqueous electrolyte. The analysis of the transitional metal L-edge spectra allows a quantitative determination of the redox evolution of Mn and Fe during the electrochemical cycling. The sXAS analysis reveals the evolving Mn oxidation states in LiMn0.5Fe0.5PO4. We found that electrochemically inactive Mn2+ is formed on the electrode surface during cycling. Additionally, the signal indicates about 20% concentration of Mn4+ at the charged state, providing a strong experimental evidence of the disproportional reaction of Mn3+ to Mn2+ and Mn4+ on the surface of the charged LiMn0.5Fe0.5PO4 electrodes. Published by AIP Publishing. C1 [Zhuo, Zengqing; Hu, Jiangtao; Duan, Yandong; Pan, Feng] Peking Univ, Shenzhen Grad Sch, Sch Adv Mat, Shenzhen 518055, Peoples R China. [Zhuo, Zengqing; Yang, Wanli] Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Duan, YD; Pan, F (reprint author), Peking Univ, Shenzhen Grad Sch, Sch Adv Mat, Shenzhen 518055, Peoples R China.; Yang, WL (reprint author), Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM duanyd@pkusz.edu.cn; wlyang@lbl.gov; panfeng@pkusz.edu.cn RI Duan, Yandong/I-4206-2013; Yang, Wanli/D-7183-2011 OI Yang, Wanli/0000-0003-0666-8063 FU Guangdong Innovation Team Project [2013N080]; Shenzhen Science and Technology Research Grant [KYPT20141016105435850]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by Guangdong Innovation Team Project (No. 2013N080) and Shenzhen Science and Technology Research Grant (peacock plan KYPT20141016105435850). Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 26 TC 2 Z9 2 U1 6 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 11 PY 2016 VL 109 IS 2 AR 023901 DI 10.1063/1.4958639 PG 5 WC Physics, Applied SC Physics GA DT0EH UT WOS:000381155200071 ER PT J AU Rinaldi, R Jastrzebski, R Clough, MT Ralph, J Kennema, M Bruijnincx, PCA Weckhuysen, BM AF Rinaldi, Roberto Jastrzebski, Robin Clough, Matthew T. Ralph, John Kennema, Marco Bruijnincx, Pieter C. A. Weckhuysen, Bert M. TI Paving the Way for Lignin Valorisation: Recent Advances in Bioengineering, Biorefining and Catalysis SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Review DE bioengineering; biorefining; catalysis; lignin; lignocellulose ID ACID-O-METHYLTRANSFERASE; CINNAMOYL-COA-REDUCTASE; BOND-DISSOCIATION ENTHALPIES; TANDEM MASS-SPECTROMETRY; CYTOCHROME P450-DEPENDENT MONOOXYGENASE; NONENZYMATIC SUGAR PRODUCTION; WATER-SOLUBLE LIGNOCELLULOSE; IONIC LIQUID PRETREATMENT; FORMALDEHYDE RESOL RESINS; CELL-WALL BIOSYNTHESIS AB Lignin is an abundant biopolymer with a high carbon content and high aromaticity. Despite its potential as a raw material for the fuel and chemical industries, lignin remains the most poorly utilised of the lignocellulosic biopolymers. Effective valorisation of lignin requires careful fine-tuning of multiple "upstream" (i.e., lignin bioengineering, lignin isolation and "early-stage catalytic conversion of lignin") and "downstream" (i.e., lignin depolymerisation and upgrading) process stages, demanding input and understanding from a broad array of scientific disciplines. This review provides a "beginning-to-end" analysis of the recent advances reported in lignin valorisation. Particular emphasis is placed on the improved understanding of lignin's biosynthesis and structure, differences in structure and chemical bonding between native and technical lignins, emerging catalytic valorisation strategies, and the relationships between lignin structure and catalyst performance. C1 [Rinaldi, Roberto] Imperial Coll London, Dept Chem Engn, South Kensington Campus, London SW7 2AZ, England. [Jastrzebski, Robin; Bruijnincx, Pieter C. A.; Weckhuysen, Bert M.] Univ Utrecht, Inorgan Chem & Catalysis, Debye Inst Nanomat Sci, Univ Weg 99, NL-3584 CG Utrecht, Netherlands. [Clough, Matthew T.; Kennema, Marco] Max Planck Inst Kohlenforsch, Kaiser Wilhelm Pl 1, D-45470 Mulheim, Germany. [Ralph, John] Univ Wisconsin, Dept Energy, Great Lakes Bioenergy Res Ctr, Wisconsin Energy Inst, Madison, WI 53726 USA. [Ralph, John] Univ Wisconsin, Dept Biochem, Madison, WI 53726 USA. RP Rinaldi, R (reprint author), Imperial Coll London, Dept Chem Engn, South Kensington Campus, London SW7 2AZ, England.; Bruijnincx, PCA; Weckhuysen, BM (reprint author), Univ Utrecht, Inorgan Chem & Catalysis, Debye Inst Nanomat Sci, Univ Weg 99, NL-3584 CG Utrecht, Netherlands.; Ralph, J (reprint author), Univ Wisconsin, Dept Energy, Great Lakes Bioenergy Res Ctr, Wisconsin Energy Inst, Madison, WI 53726 USA.; Ralph, J (reprint author), Univ Wisconsin, Dept Biochem, Madison, WI 53726 USA. EM rrinaldi@imperial.ac.uk; jralph@wisc.edu; p.c.a.bruijnincx@uu.nl; b.m.weckhuysen@uu.nl RI Weckhuysen, Bert/D-3742-2009; Institute (DINS), Debye/G-7730-2014; Bruijnincx, Pieter/C-7992-2011 OI Weckhuysen, Bert/0000-0001-5245-1426; Bruijnincx, Pieter/0000-0001-8134-0530 FU Alexander von Humboldt Foundation; Cluster of Excellence "Tailor-Made Fuels from Biomass"; Netherlands Organisation for Scientific Research (NWO); European Research Council [321140]; European Commission (SuBi-Cat Initial Training Network) [607044]; CatchBio program - Smart Mix Program of The Netherlands Ministry of Economic Affairs; Netherlands Ministry of Education, Culture, and Science; DOE Great Lakes Bioenergy Research Center (DOE Office of Science) [BER DE-FC02-07ER64494]; Stanford University's Global Climate and Energy Project FX R.R. acknowledges the financial support from the Alexander von Humboldt Foundation (Sofja Kovalevskaja Award 2010) and the Cluster of Excellence "Tailor-Made Fuels from Biomass". R.R. is grateful to Prof. Dr. Patricia Nunes da Silva (Institute of Mathematics and Statistics, State University of Rio de Janeiro, Brazil) for the valuable discussions on the statistics of depolymerisation processes. P.C.A.B. acknowledges the Netherlands Organisation for Scientific Research (NWO) for a Vernieuwingsimpuls Veni Grant. B.M.W. acknowledges the European Research Council (Advanced ERC grant no. 321140). P.C.A.B. and B.M.W. also gratefully acknowledge support from the European Commission (SuBi-Cat Initial Training Network, Call FP7-PEOPLE-2013, ITN, grant no. 607044) and from the CatchBio program, funded by the Smart Mix Program of The Netherlands Ministry of Economic Affairs and The Netherlands Ministry of Education, Culture, and Science. J.R. was funded in part by the DOE Great Lakes Bioenergy Research Center (DOE Office of Science BER DE-FC02-07ER64494), and in part by Stanford University's Global Climate and Energy Project. NR 443 TC 44 Z9 44 U1 115 U2 131 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JUL 11 PY 2016 VL 55 IS 29 BP 8164 EP 8215 DI 10.1002/anie.201510351 PG 52 WC Chemistry, Multidisciplinary SC Chemistry GA DV9IE UT WOS:000383253300001 PM 27311348 ER PT J AU Mohamed, MH Elsaidi, SK Pham, T Forrest, KA Schaef, HT Hogan, A Wojtas, L Xu, WQ Space, B Zaworotko, MJ Thallapally, PK AF Mohamed, Mona H. Elsaidi, Sameh K. Pham, Tony Forrest, Katherine A. Schaef, Herbert T. Hogan, Adam Wojtas, Lukasz Xu, Wenqian Space, Brian Zaworotko, Michael J. Thallapally, Praveen K. TI Hybrid Ultra-Microporous Materials for Selective Xenon Adsorption and Separation SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE chromium; hybrid ultra-microporous materials; metal-organic frameworks; separations; xenon ID METAL-ORGANIC FRAMEWORKS; NOBLE-GAS ADSORPTION; COORDINATION POLYMERS; CO2; KR; XE; REMOVAL; KRYPTON AB The demand for Xe/Kr separation continues to grow due to the industrial significance of high-purity Xe gas. Current separation processes rely on energy intensive cryogenic distillation. Therefore, less energy intensive alternatives, such as physisorptive separation, using porous materials, are required. Herein we show that an underexplored class of porous materials called hybrid ultra-microporous materials (HUMs) affords new benchmark selectivity for Xe separation from Xe/Kr mixtures. The isostructural materials, CROFOUR-1-Ni and CROFOUR-2-Ni, are coordination networks that have coordinatively saturated metal centers and two distinct types of micropores, one of which is lined by CrO42- (CROFOUR) anions and the other is decorated by the functionalized organic linker. These nets offer unprecedented selectivity towards Xe. Modelling indicates that the selectivity of these nets is tailored by synergy between the pore size and the strong electrostatics afforded by the CrO42- anions. C1 [Mohamed, Mona H.; Elsaidi, Sameh K.; Schaef, Herbert T.; Thallapally, Praveen K.] Pacific Northwest Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. [Mohamed, Mona H.; Elsaidi, Sameh K.] Univ Alexandria, Dept Chem, Fac Sci, POB 426, Alexandria 21321, Egypt. [Pham, Tony; Forrest, Katherine A.; Hogan, Adam; Wojtas, Lukasz; Space, Brian] Univ S Florida, Dept Chem, 4202 East Fowler Ave,CHE205, Tampa, FL 33620 USA. [Xu, Wenqian] Argonne Natl Lab, Xray Sci Div, Adv Photon Source, Argonne, IL 60439 USA. [Zaworotko, Michael J.] Univ Limerick, Dept Chem & Environm Sci, Limerick, Ireland. RP Thallapally, PK (reprint author), Pacific Northwest Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. EM praveen.thallapally@pnnl.gov RI zaworotko, michael/A-7448-2009; Pham, Tony/A-3787-2014; OI zaworotko, michael/0000-0002-1360-540X; Thallapally, Praveen Kumar/0000-0001-7814-4467 FU National Science Foundation [CHE-1152362]; Major Research Instrumentation Program [CHE-1531590]; XSEDE Grant [TG-DMR090028]; US Department of Energy [DE-AC05-76RL01830]; Science Foundation Ireland [13/RP/B2549]; DOE Office of Science [DE-AC02-06CH11357] FX B.S. acknowledges the National Science Foundation (Award No. CHE-1152362), including support from the Major Research Instrumentation Program (Award No CHE-1531590), the computational resources that were made available by a XSEDE Grant (No. TG-DMR090028), and the use of the services provided by Research Computing at the University of South Florida. We (P.K.T) thank the US Department of Energy (DOE), Office of Nuclear Energy for adsorption and breakthrough measurements. We (P.K.T) particularly thank J. Bresee, K. Gray, T. Todd (Idaho National Laboratory), John Vienna (PNNL), B. Jubin (Oak Ridge National Laboratory), and D. M. Strachan (Strachan LLC) for providing programmatic support and guidance. Pacific Northwest National Laboratory is a multi-program national laboratory operated for the US Department of Energy by Battelle Memorial Institute under Contract DE-AC05-76RL01830. M.J.Z. gratefully acknowledges Science Foundation Ireland (Award 13/RP/B2549) for support. This research used Beamline 17-BM of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 28 TC 2 Z9 2 U1 25 U2 28 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. 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Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Navarro, LB Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Bassalat, A Basalaev, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Beccherle, R Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bedognetti, M Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Beringer, J Bernard, C Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertsche, C Bertsche, D Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW 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CA ATLAS Collaboration TI A search for an excited muon decaying to a muon and two jets in pp collisions at root s=8 TeV with the ATLAS detector SO NEW JOURNAL OF PHYSICS LA English DT Article DE excited leptons; lepton compositeness; leptoquarks ID PARTON DISTRIBUTIONS; LEPTON PRODUCTION; HADRON COLLIDERS; QUARK; EVENTS; HEAVY; HERA; LHC AB Anew search signature for excited leptons is explored. Excited muons are sought in the channel pp -> mu mu* -> mu mu jet jet, assuming both the production and decay occur via a contact interaction. The analysis is based on 20.3 fb(-1) of pp collision data at a centre-of-mass energy of root s = 8 TeV taken with the ATLAS detector at the large hadron collider. No evidence of excited muons is found, and limits are set at the 95% confidence level on the cross section times branching ratio as a function of the excited-muon mass m(mu)*. For m(mu)* between 1.3 and 3.0 TeV, the upper limit on sigma B(mu* -> mu q (q) over bar) is between 0.6 and 1 fb. Limits on sB are converted to lower bounds on the compositeness scale Lambda. In the limiting case Lambda = m(mu)*, excited muons with a mass below 2.8 TeV are excluded. With the same model assumptions, these limits at larger mu* masses improve upon previous limits from traditional searches based on the gauge-mediated decay mu* -> mu gamma. C1 [Jackson, P.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. 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[Biedermann, D.; Dietrich, J.; Giorgi, F. M.; Grancagnolo, S.; Herbert, G. H.; Hristova, I.; Kind, O. M.; Kolanoski, H.; Lacker, H.; Lohse, T.; Mergelmeyer, S.; Nikiforov, A.; Rehnisch, L.; Rieck, P.; Schulz, H.; Sperlich, D.; Stamm, S.; zur Nedden, M.] Humboldt Univ, Dept Phys, Berlin, Germany. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Beck, H. P.; Cervelli, A.; Ereditato, A.; Haug, S.; Marti, L. F.; Meloni, F.; Mullier, G. A.; Stramaglia, M. E.; Stucci, S. A.; Weber, M. S.] Univ Bern, High Energy Phys Lab, Bern, Switzerland. [Allport, P. P.; Bella, L. Aperio; Baca, M. J.; Bracinik, J.; Charlton, D. G.; Chisholm, A. S.; Hawkes, C. M.; Head, S. J.; Hillier, S. J.; Levy, M.; Mudd, R. D.; Quijada, J. A. Murillo; Newman, P. R.; Nikolopoulos, K.; Owen, R. E.; Slater, M.; Thomas, J. P.; Thompson, P. D.; Watkins, P. M.; Watson, A. T.; Watson, M. F.; Wilson, J. A.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Arik, M.; Istina, S.; Ozcan, V. E.] Bogazici Univ, Dept Phys, Istanbul, Turkey. [Beddall, A. J.; Beddall, A.; Bingul, A.] Gaziantep Univ, Dept Engn Phys, Gaziantep, Turkey. [Cetin, S. A.] Dogus Univ, Dept Phys, Istanbul, Turkey. [Alberghi, G. L.; Bellagamba, L.; Biondi, S.; Boscherini, D.; Bruni, A.; Bruni, G.; Bruschi, M.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Giacobbe, B.; Giorgi, F. M.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Negrini, M.; Piccinini, M.; Polini, A.; Rinaldi, L.; Romano, M.; Sbarraa, C.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Spighi, R.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] INFN Sez Bologna, Bologna, Italy. [Alberghi, G. L.; Biondi, S.; De Castro, S.; Fabbri, L.; Franchini, M.; Gabrielli, A.; Grafstroem, P.; Manghi, F. Lasagni; Massa, I.; Massa, L.; Mengarelli, A.; Piccinini, M.; Romano, M.; Sbrizzi, A.; Semprini-Cesari, N.; Sidoti, A.; Sioli, M.; Tupputi, S. A.; Valentinetti, S.; Villa, M.; Zoccoli, A.] Univ Bologna, Dipartimento Fis & Astron, Bologna, Italy. [Arslan, O.; Bechtle, P.; Bernlochner, F. U.; Brock, I.; Bruscino, N.; Cioara, I. A.; Cristinziani, M.; Davey, W.; Desch, K.; Dingfelder, J.; Gaycken, G.; Geich-Gimbel, Ch; Gonella, L.; Grefe, C.; Haefner, P.; Hageboeck, S.; Hansen, M. C.; Hohn, D.; Huegging, F.; Janssen, J.; Kostyukhin, V. V.; Kraus, J. K.; Kroseberg, J.; Krueger, H.; Lantzsch, K.; Lenz, T.; Leyko, A. M.; Liebal, J.; Limbach, C.; Mijovic, L.; Moles-Valls, R.; Obermann, T.; Pohl, D.; Ricken, O.; Sarrazin, B.; Schaefer, D.; Schaepe, S.; Schopf, E.; Schultens, M. J.; Schwindt, T.; Seema, P.; Stillings, J. A.; von Toerne, E.; Wagner, P.; Wang, T.; Wermes, N.; Wienemann, P.; Wiik-Fuchs, L. A. M.; Winter, B. T.; Wong, K. H. Yau; Yuen, S. P. Y.; Zhang, R.] Univ Bonn, Inst Phys, Bonn, Germany. [Ahlen, S. P.; Bernard, C.; Black, K. M.; Butler, J. M.; Dell'Asta, L.; Helary, L.; Kruskal, M.; Long, B. A.; Shank, J. T.; Yan, Z.; Youssef, S.] Boston Univ, Dept Phys, 590 Commonwealth Ave, Boston, MA 02215 USA. [Amelung, C.; Amundsen, G.; Barone, G.; Bensinger, J. R.; Bianchini, L.; Blocker, C.; Coffey, L.; Dhaliwal, S.; Loew, K. M.; Sciolla, G.; Venturini, A.; Zengel, K.] Brandeis Univ, Dept Phys, Waltham, MA 02254 USA. [Amaral Coutinho, Y.; Caloba, L. P.; Maidantchik, C.; Marroquim, F.; Nepomuceno, A. A.; Seixas, J. M.] Univ Fed Rio de Janeiro, COPPE, EE, IF, Rio De Janeiro, Brazil. [Cerqueira, A. S.; Manhaes de Andrade Filho, L.] Fed Univ Juiz De Fora UFJF, Elect Circuits Dept, Juiz De Fora, Brazil. [do Vale, M. A. B.] Fed Univ Sao Joao Del Rei UFSJ, Sao Joao Del Rei, Brazil. [Donadelli, M.; La Rosa Navarrod, J. L.; Leite, M. A. L.] Univ Sao Paulo, Inst Fis, Sao Paulo, Brazil. [Adams, D. L.; Assamagan, K.; Begel, M.; Buttinger, W.; Chen, H.; Chernyatin, V.; Debbe, R.; Ernst, M.; Gibbard, B.; Gordon, H. A.; Iakovidis, G.; Klimentov, A.; Kouskoura, V.; Kravchenko, A.; Lanni, F.; Lee, C. A.; Lissauer, D.; Liu, H.; Lynn, D.; Ma, H.; Maeno, T.; Mountricha, E.; Nevski, P.; Nilsson, P.; Damazio, D. Oliveira; Paige, F.; Panitkin, S.; Perepelitsa, D. V.; Pleier, M-A; Polychronakos, V.; Protopopescu, S.; Purohit, M.; Radeka, V.; Rajagopalan, S.; Redlinger, G.; Snyder, S.; Steinberg, P.; Takai, H.; Undrus, A.; Wenaus, T.; Xu, L.; Ye, S.] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. Transilvania Univ Brasov, Brasov, Romania. [Alexa, C.; Boldea, V.; Caprini, I.; Caprini, M.; Chitan, A.; Ciubancan, M.; Constantinescu, S.; Dita, P.; Dita, S.; Ducu, O. A.; Jinaru, A.; Martoiu, V. S.; Maurer, J.; Olariu, A.; Pantea, D.; Rotaru, M.; Stoicea, G.; Tudorache, A.; Tudorache, V.] Natl Inst Phys & Nucl Engn, Bucharest, Romania. [Popeneciuc, G. A.] Natl Inst Res & Dev Isotop & Mol Technol, Dept Phys, Cluj Napoca, Romania. [Dobre, M.] Univ Politehn Bucuresti, Bucharest, Romania. West Univ Timisoara, Timisoara, Romania. [Bossio Sola, J. D.; Otero y Garzon, G.; Piegaia, R.; Reisin, H.; Sacerdoti, S.] Univ Buenos Aires, Dept Fis, Buenos Aires, DF, Argentina. [Arratia, M.; Barlow, N.; Batley, J. R.; Brochu, F. M.; Brunt, B. H.; Carter, J. R.; Chapman, J. D.; Cottin, G.; Gillam, T. P. S.; Hill, J. C.; Kaneti, S.; Khoo, T. J.; Lester, C. G.; Mueller, T.; Parker, M. A.; Potter, C. J.; Robinson, D.; Rosten, J. H. N.; Thomson, M.; Ward, C. P.; Yusuff, I.] Univ Cambridge, Cavendish Lab, Cambridge, England. [Bellerive, A.; Cree, G.; Di Valentino, D.; Gillberg, D.; Koffas, T.; Lacey, J.; Leight, W. A.; McCarthy, T. G.; Nomidis, I.; Oakham, F. G.; Pasztor, G.; Ueno, R.; Vincter, M. G.] Carleton Univ, Dept Phys, Ottawa, ON, Canada. [Aleksa, M.; Gonzalez, B. Alvarez; Amoroso, S.; Anders, G.; Anghinolfi, F.; Armbruster, A. J.; Arnaez, O.; Avolio, G.; Baak, M. A.; Backes, M.; Backhaus, M.; Barak, L.; Barnett, B. M.; Beermann, T. A.; Beltramello, O.; Bianco, M.; Bogaerts, J. A.; Boveia, A.; Boyd, J.; Campana, S.; Garrido, M. D. M. Capeans; Carli, T.; Carrillo-Montoya, G. D.; Catinaccio, A.; Cattai, A.; Cerv, M.; Chromek-Burckhart, D.; Conti, G.; Dell'Acqua, A.; Deviveiros, P. O.; Di Girolamo, A.; Di Girolamo, B.; Dittus, F.; Dobos, D.; Dudarev, A.; Duehrssen, M.; Eifert, T.; Ellis, N.; Elsing, M.; Farthouat, P.; Fassnacht, P.; Feng, E. J.; Francis, D.; Fressard-Batraneanu, S. M.; Froidevaux, D.; Gadatsch, S.; Glatzer, J.; Goossens, L.; Gorini, B.; Gray, H. M.; Gumpert, C.; Hawkings, R. J.; Helsens, C.; Correia, A. M. Henriques; Hervas, L.; Hoecker, A.; Huhtinen, M.; Iengo, P.; Jakobsen, S.; Klioutchnikova, T.; Krasznahorkay, A.; Lapoire, C.; Lassnig, M.; Miotto, G. Lehmann; Lenzi, B.; Lichard, P.; Malyukov, S.; Mandelli, B.; Mapelli, L.; Marzin, A.; McFayden, J. A.; Milic, A.; Berlingen, J. Montejo; Mornacchi, G.; Nairz, A. M.; Nakahama, Y.; Nessi, M.; Nicquevert, B.; Nordberg, M.; Oide, H.; Palestini, S.; Pauly, T.; Pernegger, H.; Peters, K.; Petersen, B. A.; Pommes, K.; Poppleton, A.; Poulard, G.; Poveda, J.; Astigarraga, M. E. Pozo; Rammensee, M.; Raymond, M.; Rembser, C.; Ritsch, E.; Roe, S.; Ruiz-Martinez, A.; Ruthmann, N.; Salzburger, A.; Schaefer, D.; Schlenker, S.; Schmieden, K.; Serfon, C.; Sforza, F.; Sanchez, C. A. Solans; Spigo, G.; Staerz, S.; Stelzer, H. J.; Taenzer, J.; Teischinger, F. A.; Ten Kate, H.; Tremblet, L.; Tricoli, A.; Unal, G.; van Woerden, M. C.; Vandelli, W.; Voss, R.; Vuillermet, R.; Wells, P. S.; Wengler, T.; Wenig, S.; Werner, P.; Wilkens, H. G.; Wotschack, J.; Young, C. J. S.; Zhong, J.; Zwalinski, L.] CERN, Geneva, Switzerland. [Alison, J.; Andeen, T.; Anderson, K. J.; Bryant, P.; Toro, R. Camacho; Cheng, Y.; Dandoy, J. R.; Facini, G.; Gardner, R. W.; Ilchenko, Y.; Kapliy, A.; Kim, Y. K.; Krizka, K.; Li, H. L.; Merritt, F. S.; Miller, D. W.; Narayan, R.; Okumura, Y.; Onyisi, P. U. E.; Oreglia, M. J.; Penning, B.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, 5640 S Ellis Ave, Chicago, IL 60637 USA. [Blunier, S.; Carquin, E.; Diaz, M. A.; Ochoa-Ricoux, J. P.; Vogel, M.] Pontificia Univ Catolica Chile, Dept Fis, Santiago, Chile. [Brooks, W. K.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Salazar Loyola, J. E.; Tapia Araya, S.; White, R.] Univ Tecn Federico Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Fang, Y.; Jin, S.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Song, H. Y.; Zhang, G.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Feng, C.; Ma, L. L.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai Key Lab Particle Phys & Cosmol, Shanghai, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph; Liao, H.; Loebinger, F. K.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph; Liao, H.; Loebinger, F. K.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Schaefer, D.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Dubreuil, E.; Gilles, G.; Gris, Ph; Liao, H.; Loebinger, F. K.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] IN2P3, CNRS, Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN Grp Collegato Cosenza, Lab Nazl Frascati, Frascati, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, Arcavacata Di Rende, Italy. [Adamczyk, L.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindura, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] Southern Methodist Univ, Dept Phys, Dallas, TX USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX USA. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmit, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Hamburg, Germany. [Asbah, N.; Bessner, M.; Bloch, I.; Britzger, D.; Camarda, S.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; Peschke, R.; Pirumov, H.; Poley, A.; Radescu, V.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmit, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, Fmgaray; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] INFN Lab Nazl Frascati, Frascati, Italy. [Betancourt, C.; Buehrer, F.; Buescher, D.; Coniavitis, E.; Di Simone, A.; Luedtke, C.; Sammel, D.; Schillo, C.; Ta, D.; Weiser, C.] Albert Ludwigs Univ, Fak Math & Phys, Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; De Mendizabal, J. Bilbao; Calace, N.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] INFN Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Dueren, M.; Kreutzfeldt, K.; Stenzel, H.] Justus Liebig Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Du, Y.; Ferrando, J.; Ferreira de Lima, D. E.; Gul, U.; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; McHedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Schorlemmer, A. L. S.; Shabalina, E.; Stolte, P.; Weingarten, J.; Zinonos, Z.] Georg August Univ, Inst Phys 2, Gottingen, Germany. [Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS, IN2P3, Lab Phys Subat & Cosmol, Grenoble, France. [McFarlane, K. W.; Unno, Y.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Clark, B. L.; Franklin, M.; Frate, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA USA. [Baas, A. E.; Brandt, O.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E-E; Meier, K.; Theenhausen, H. Meyer Zu; Villara, D. I. Narrias; Sahinsoya, M.; Schaefer, D.; Schultz-Coulona, H-C; Stamen, R.; Starovoitov, P.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolbb, M.; Lisovyi, M.; Schaetzel, S.; Schmitt, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Colombo, T.; Kretzc, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Buckley, A. G.; Yagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Annovi, A.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka, Japan. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Chiodini, G.; Gorini, E.; Primavera, M.; Spagnolo, S.; Ventura, A.] INFN Sez Lecce, Lecce, Italy. [Gorini, E.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Faucci Giannelli, M.; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr; Savage, G.; Schaefer, D.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Egham, Surrey, England. [Butterworth, J. M.; Campanelli, M.; Casadei, D.; Chislett, R. T.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Lambourne, L.; Leney, K. J. C.; Martyniuk, A. C.; McFayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Cgrossi, G.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] IN2P3, CNRS, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Inst Fys, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Theck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Kopp, A. K.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Valderanis, C.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Balli, F.; Cox, B. E.; Da Via, C.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Keoshkerian, H.; Masik, J.; Sanchez, F. J. Munoz; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Queitsch-Maitland, M.; Schwanenberger, C.; Schweiger, H.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Webb, S.; Woudstra, M. J.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Alio, L.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Alio, L.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ducu, O. A.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagai, Y.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tiouchichine, E.; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] IN2P3, CNRS, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Lari, T.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Perini, L.; Ragusa, F.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] INFN Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Perini, L.; Ragusa, F.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F; Azuelos, G.; Dallaire, F.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Avakimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; AGorbounov, P.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu; Smirnov, Y.; Soldatov, E. Yu; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Boldyrev, A. S.; Giugni, D.; Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Elmsheuser, J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Walker, R.; Wittkowski, J.] Ludwig Maximilians Univ Munchen, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys Werner Heisenberg Inst, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] INFN Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Napoli, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Gale, C.; Konig, A. C.; Nektarijevic, S.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Karastathis, N.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van den Wollenberg, W.; Van der Deijl, P. C.; van der Geer, R.; van der Graaf, H.; van Vulpen, I.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burdin, S.; Burgard, C. D.; Chakraborty, D.; Cole, S.; Saha, P.] Northern Illinois Univ, Dept Phys, De Kalb, IL 60115 USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Bousson, N.; Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.; Sinev, N. B.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Basalaev, A.; Becot, C.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J-F; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris Saclay, Univ Paris Sud, LAL, CNRS IN2P3, Orsay, France. [Endo, M.; Nomachi, M.; Schaffer, A. C.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, L.; Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramling, J.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Behr, J. K.; Beresford, L.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Dafinca, A.; Davies, E.; Frost, J. A.; Gallas, E. J.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Nagai, K.; Nickerson, R. B.; Pickering, M. A.; Ryder, N. C.; Tseng, J. C-L; Viehhauser, G. H. A.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] INFN Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Bassalat, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Petersburg Nucl Phys Inst, Natl Res Ctr Kurchatov Inst, St Petersburg, Russia. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] INFN Sez Pisa, Pisa, Italy. [Annovi, A.; Beccherle, R.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedraa, J. A.; Amor Dos Santos, S. P.; Amorim, A.; Annovi, A.; Araque, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhaisa, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Lopes, L.; Maio, A.; Maneira, J.; Oleiro Seabra, L. F.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Fiolhaisa, M. C. N.; Galhardo, B.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Amor Dos Santos, S. P.; Carvalho, J.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedraa, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedraa, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dep Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr Inst High Energy Phys Protvino, Moscow, Russia. [Adye, T.; Baines, J. T.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, Cnp; Haywood, S. J.; Hsu, P. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Nisatia, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvo, L.; Rescigno, M.; Rosati, S.; Tehrania, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] INFN Sez Roma, Rome, Italy. [Annovi, A.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.; Zanello, L.] Sapienza Univ Roma, Dipartimento Fis, Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] INFN Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] INFN Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Roma Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummadaa, A.] Reseau Univ Phys Hautes Energies Univ Hassan II, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, Fac Sci Semlalia, LPHEA Marrakech, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [Cherkaoui El Mourslie, R.; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Bauer, F.; Besson, N.; Blanchard, J-B; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Goncalves Pinto Firmino Da Costa, J.; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kozanecki, W.; Kukla, R.; Lancon, E.; Laporte, J. F.; Mansoulie, B.; Meyer, J-P; Nicolaidou, R.; Ouraou, A.; Peyaud, A.; Protopapadaki, E.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph; Schwemling, Ph; Schwindling, J.] CEA Saclay, DSM IRFU, Gif Sur Yvette, France. [Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S-C; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Wallangen, V.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Tylmad, M.; Ughetto, M.; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, Stockholm, Sweden. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY USA. [Balestri, T.; Bee, C. P.; Campoverde, A.; Chen, K.; Hobbs, J.; Jia, J.; Li, H.; Lindquist, B. E.; McCarthy, R. L.; Montalbano, A.; Morvaj, L.; Puldon, D.; Radhakrishnan, S. K.; Rijssenbeek, M.; Schamberger, R. D.; Tsybychev, D.; Zaman, A.; Zhou, M.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G-Y; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW, Australia. [Abdallah, J.; Hou, S.; Lee, S. C.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.] Acad Sinica, Inst Phys, Taipei, Taiwan. [Abreu, H.; Di Mattia, A.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, Tel Aviv, Israel. [Bachas, K.; Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Orlando, N.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Int Ctr Elementary Particle Phys, Tokyo, Japan. [Annovi, A.; Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Albrand, S.; Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo, Japan. [AbouZeid, O. S.; Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsmana, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Schouten, D.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON, Canada. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Hayashi, T.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Losada, M.; Moreno, D.; Navarro, G.; Sandoval, C.] Univ Antonio Narino, Ctr Invest, Bogota, Colombia. [Casper, D. W.; Corso-Radu, A.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Giordani, M. P.; Quayle, W. B.; Serkin, L.; Shaw, K.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Cobal, M.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.; Truong, L.] Univ Udine, Dipartimento Chim Fis & Ambiente, Udine, Italy. [Atkinson, M.; Basye, A.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Maddocks, H. J.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Alvarez Piqueras, D.; Annovi, A.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. 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A.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. J.; Fernandez Martinez, P.; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Garcia Navarro, J. E.; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; Kaci, M.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Microelect Barcelona IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Castillo Gimenez, V.; Cerda Alberich, L.; Costa, M. 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[Liu, B.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Myagkov, A. G.; Nikolaenko, V.; Zaitsev, A. M.] Moscow Inst Phys & Technol, Dolgoprudnyi, Russia. Univ Geneva, Sect Phys, Geneva, Switzerland. [Pinamonti, M.] Int Sch Adv Studies SISSA, Trieste, Italy. [Purohit, M.] Univ South Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Shi, L.; Soh, D. A.] Sun Yat Sen Univ, Sch Phys & Engn, Guangzhou, Guangdong, Peoples R China. [Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, Fac Phys, Moscow, Russia. [Tikhomirov, V. O.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Tompkins, L.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Toth, J.] Wigner Res Ctr Phys, Inst Particle & Nucl Phys, Budapest, Hungary. [Vest, A.] Flensburg Univ Appl Sci, Flensburg, Germany. [Yusuff, I.] Univ Malaya, Dept Phys, Kuala Lumpur, Malaysia. [Zhang, R.] Aix Marseille Univ, CPPM, Marseille, France. [Zhang, R.] IN2P3, CNRS, Marseille, France. RP Aad, G (reprint author), Aix Marseille Univ, CPPM, Marseille, France.; Aad, G (reprint author), IN2P3, CNRS, Marseille, France. RI Villa, Mauro/C-9883-2009; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015; Mitsou, Vasiliki/D-1967-2009; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Guo, Jun/O-5202-2015; Prokoshin, Fedor/E-2795-2012; Coccaro, Andrea/P-5261-2016; Brooks, William/C-8636-2013; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Di Domenico, Antonio/G-6301-2011; Doyle, Anthony/C-5889-2009; Shulga, Evgeny/R-1759-2016; Maleev, Victor/R-4140-2016; Conde Muino, Patricia/F-7696-2011; Gladilin, Leonid/B-5226-2011; Grinstein, Sebastian/N-3988-2014; Zhukov, Konstantin/M-6027-2015; Livan, Michele/D-7531-2012; Tikhomirov, Vladimir/M-6194-2015; Stabile, Alberto/L-3419-2016; Warburton, Andreas/N-8028-2013; Carvalho, Joao/M-4060-2013; Boyko, Igor/J-3659-2013; Ventura, Andrea/A-9544-2015 OI Villa, Mauro/0000-0002-9181-8048; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Haas, Andrew/0000-0002-4832-0455; Mitsou, Vasiliki/0000-0002-1533-8886; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Guo, Jun/0000-0001-8125-9433; Prokoshin, Fedor/0000-0001-6389-5399; Coccaro, Andrea/0000-0003-2368-4559; Brooks, William/0000-0001-6161-3570; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; Di Domenico, Antonio/0000-0001-8078-2759; Doyle, Anthony/0000-0001-6322-6195; Shulga, Evgeny/0000-0001-5099-7644; Conde Muino, Patricia/0000-0002-9187-7478; Gladilin, Leonid/0000-0001-9422-8636; Grinstein, Sebastian/0000-0002-6460-8694; Livan, Michele/0000-0002-5877-0062; Tikhomirov, Vladimir/0000-0002-9634-0581; Stabile, Alberto/0000-0002-6868-8329; Warburton, Andreas/0000-0002-2298-7315; Carvalho, Joao/0000-0002-3015-7821; Boyko, Igor/0000-0002-3355-4662; Ventura, Andrea/0000-0002-3368-3413 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMTCR, Czech Republic; MPOCR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRCKI, Russian Federation; JINR, Serbia; MESTD, Serbia; MSSR, Slovakia; ARRS; MIZS Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; CANARIE, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET, European Union; ERC, European Union; FP7, European Union; Horizon, European Union; Marie Sklodowska-Curie Actions, European Union; Investissement d'Avenir Labex, France; Investissement d'Avenir Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Spain; Generalitat Valenciana, Spain; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom; Thales programme - EU-ESF FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMTCR, MPOCR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRCKI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF(Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 62 TC 0 Z9 0 U1 29 U2 45 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1367-2630 J9 NEW J PHYS JI New J. Phys. PD JUL 11 PY 2016 VL 18 AR 073021 DI 10.1088/1367-2630/18/7/073021 PG 21 WC Physics, Multidisciplinary SC Physics GA DU0DE UT WOS:000381870700003 ER PT J AU Zhivun, E Wickenbrock, A Sudyka, J Patton, B Pustelny, S Budker, D AF Zhivun, Elena Wickenbrock, Arne Sudyka, Julia Patton, Brian Pustelny, Szymon Budker, Dmitry TI Vector light shift averaging in paraffin-coated alkali vapor cells SO OPTICS EXPRESS LA English DT Article ID BEAM FREQUENCY STANDARD; MAGNETIC-RESONANCE; OPTICAL DETECTION; ATOMS; LASER; MAGNETOMETER AB Light shifts are an important source of noise and systematics in optically pumped magnetometers. We demonstrate that the long spin-coherence time in paraffin-coated cells leads to spatial averaging of the vector light shift over the entire cell volume. This renders the averaged vector light shift independent, under certain approximations, of the light-intensity distribution within the sensor cell. Importantly, the demonstrated averaging mechanism can be extended to other spatially varying phenomena in anti-relaxation-coated cells with long coherence times. (C) 2016 Optical Society of America C1 [Zhivun, Elena; Patton, Brian; Budker, Dmitry] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Wickenbrock, Arne; Budker, Dmitry] Johannes Gutenberg Univ Mainz, D-55128 Mainz, Germany. [Sudyka, Julia; Pustelny, Szymon] Marian Smoluchowski Inst Phys, Lojasiewicza 11, PL-30348 Krakow, Poland. [Patton, Brian] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany. [Budker, Dmitry] Helmholtz Inst Mainz, D-55099 Mainz, Germany. [Budker, Dmitry] Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. RP Wickenbrock, A (reprint author), Johannes Gutenberg Univ Mainz, D-55128 Mainz, Germany. EM wickenbr@uni-mainz.de FU National Science Foundation [CHE-1308381]; NGA NURI program; Marie Curie programme, FP7 "Coherent optics sensors for medical applications-COSMA" [PIRSES-GA-2012-295264]; National Centre for Research and Development within the Leader program FX We would like to thank Larry R. Hunter for helpful input and comments. This research was supported in part by the National Science Foundation under award CHE-1308381 and by the NGA NURI program. JS and SP would like to acknowledge support from Marie Curie programme, FP7 "Coherent optics sensors for medical applications-COSMA" (PIRSES-GA-2012-295264), and the National Centre for Research and Development within the Leader program. NR 33 TC 2 Z9 2 U1 7 U2 8 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JUL 11 PY 2016 VL 24 IS 14 BP 15383 EP 15390 DI 10.1364/OE.24.015383 PG 8 WC Optics SC Optics GA DT8UF UT WOS:000381770500036 PM 27410814 ER PT J AU Colombo, AP Carter, TR Borna, A Jau, YY Johnson, CN Dagel, AL Schwindt, PDD AF Colombo, Anthony P. Carter, Tony R. Borna, Amir Jau, Yuan-Yu Johnson, Cort N. Dagel, Amber L. Schwindt, Peter D. D. TI Four-channel optically pumped atomic magnetometer for magnetoencephalography SO OPTICS EXPRESS LA English DT Article ID FETAL MAGNETOCARDIOGRAPHY; ARRAY; FIELDS AB We have developed a four-channel optically pumped atomic magnetometer for magnetoencephalography (MEG) that incorporates a passive diffractive optical element (DOE). The DOE allows us to achieve a long, 18-mm gradiometer baseline in a compact footprint on the head. Using gradiometry, the sensitivities of the channels are < 5 fT/Hz(1/2), and the 3-dB bandwidths are approximately 90 Hz, which are both sufficient to perform MEG. Additionally, the channels are highly uniform, which offers the possibility of employing standard MEG post-processing techniques. This module will serve as a building block of an array for magnetic source localization. (C) 2016 Optical Society of America C1 [Colombo, Anthony P.; Carter, Tony R.; Borna, Amir; Jau, Yuan-Yu; Johnson, Cort N.; Dagel, Amber L.; Schwindt, Peter D. D.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Johnson, Cort N.] Charles Stark Draper Lab, 555 Technol Sq, Cambridge, MA 02139 USA. RP Schwindt, PDD (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. EM pschwin@sandia.gov FU US Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; National Institute of Biomedical Imaging and Bioengineering, National Institutes of Health (NIH) [R01EB013302] FX Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the US Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. This work was supported by grant number R01EB013302 from the National Institute of Biomedical Imaging and Bioengineering, National Institutes of Health (NIH). Its contents are solely the responsibility of the authors and do not necessarily represent the official view of the NIH. NR 42 TC 1 Z9 1 U1 17 U2 23 PU OPTICAL SOC AMER PI WASHINGTON PA 2010 MASSACHUSETTS AVE NW, WASHINGTON, DC 20036 USA SN 1094-4087 J9 OPT EXPRESS JI Opt. Express PD JUL 11 PY 2016 VL 24 IS 14 BP 15403 EP 15416 DI 10.1364/OE.24.015403 PG 14 WC Optics SC Optics GA DT8UF UT WOS:000381770500038 PM 27410816 ER PT J AU Ma, XC Hopkins, PF Kasen, D Quataert, E Faucher-Giguere, CA Keres, D Murray, N Strom, A AF Ma, Xiangcheng Hopkins, Philip F. Kasen, Daniel Quataert, Eliot Faucher-Giguere, Claude-Andre Keres, Dusan Murray, Norman Strom, Allison TI Binary stars can provide the 'missing photons' needed for reionization SO MONTHLY NOTICES OF THE ROYAL ASTRONOMICAL SOCIETY LA English DT Article DE binaries: general; stars: evolution; galaxies: formation; galaxies: high-redshift; cosmology: theory ID HUBBLE-SPACE-TELESCOPE; FIRE COSMOLOGICAL SIMULATIONS; HIGH-REDSHIFT GALAXIES; INITIAL MASS FUNCTION; COSMIC REIONIZATION; IONIZING PHOTONS; LYMAN CONTINUUM; ESCAPE FRACTION; FORMING GALAXIES; STELLAR FEEDBACK AB Empirical constraints on reionization require galactic ionizing photon escape fractions f(esc) a parts per thousand(3) 20 per cent, but recent high-resolution radiation-hydrodynamic calculations have consistently found much lower values similar to 1-5 per cent. While these models include strong stellar feedback and additional processes such as runaway stars, they almost exclusively consider stellar evolution models based on single (isolated) stars, despite the fact that most massive stars are in binaries. We re-visit these calculations, combining radiative transfer and high-resolution cosmological simulations with detailed models for stellar feedback from the Feedback in Realistic Environments project. For the first time, we use a stellar evolution model that includes a physically and observationally motivated treatment of binaries (the Binary Population and Spectral Synthesis model). Binary mass transfer and mergers enhance the population of massive stars at late times (a parts per thousand(3)3 Myr) after star formation, which in turn strongly enhances the late-time ionizing photon production (especially at low metallicities). These photons are produced after feedback from massive stars has carved escape channels in the interstellar medium, and so efficiently leak out of galaxies. As a result, the time-averaged 'effective' escape fraction (ratio of escaped ionizing photons to observed 1500 angstrom photons) increases by factors similar to 4-10, sufficient to explain reionization. While important uncertainties remain, we conclude that binary evolution may be critical for understanding the ionization of the Universe. C1 [Ma, Xiangcheng; Hopkins, Philip F.] CALTECH, TAPIR, MC 350-17, Pasadena, CA 91125 USA. [Kasen, Daniel; Quataert, Eliot] Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. [Kasen, Daniel; Quataert, Eliot] Univ Calif Berkeley, Theoret Astrophys Ctr, Berkeley, CA 94720 USA. [Kasen, Daniel] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Faucher-Giguere, Claude-Andre] Northwestern Univ, Dept Phys & Astron, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Faucher-Giguere, Claude-Andre] Northwestern Univ, CIERA, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Keres, Dusan] Univ Calif San Diego, Dept Phys, Ctr Astrophys & Space Sci, 9500 Gilman Dr, La Jolla, CA 92093 USA. [Murray, Norman] Univ Toronto, Canadian Inst Theoret Astrophys, 60 St George St, Toronto, ON M5S 3H8, Canada. [Strom, Allison] CALTECH, Dept Astrophys, MC 249-17, Pasadena, CA 91125 USA. RP Ma, XC (reprint author), CALTECH, TAPIR, MC 350-17, Pasadena, CA 91125 USA. EM xchma@caltech.edu FU NSF MRI award [PHY-0960291]; Alfred P. Sloan Research Fellowship; NASA ATP Grant [NNX14AH35G, 12-APT12-0183]; NSF Collaborative Research Grant [1411920]; CAREER grant [1455342]; Department of Energy Office of Nuclear Physics Early Career Award; Office of Energy Research, Office of High Energy and Nuclear Physics, Divisions of Nuclear Physics, of the US Department of Energy [DE-AC02-05CH11231]; NSF [AST-1109896, AST-1412153, AST-1412836, AST-1517491]; University of California, San Diego; NASA [NNX15AB22G]; STScI [HST-AR-14293.001-A]; Simons Foundation; David and Lucile Packard Foundation FX We thank Chuck Steidel for helpful discussions and the referee for useful comments. We also thank John Beacom and Mike Shull for helpful suggestions after the paper was submitted to arXiv. The simulations used in this paper were run on XSEDE computational resources (allocations TG-AST120025, TG-AST130039, and TG-AST140023). The analysis was performed on the Caltech compute cluster 'Zwicky' (NSF MRI award #PHY-0960291). Support for PFH was provided by an Alfred P. Sloan Research Fellowship, NASA ATP Grant NNX14AH35G, and NSF Collaborative Research Grant #1411920 and CAREER grant #1455342. D. Kasen is supported in part by a Department of Energy Office of Nuclear Physics Early Career Award, and by the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Divisions of Nuclear Physics, of the US Department of Energy under Contract No. DE-AC02-05CH11231 and by the NSF through grant AST-1109896. D. Keres was supported by NSF grant AST-1412153 and funds from the University of California, San Diego. CAFG was supported by NSF through grants AST-1412836 and AST-1517491, by NASA through grant NNX15AB22G, and by STScI through grant HST-AR-14293.001-A. EQ was supported by NASA ATP grant 12-APT12-0183, a Simons Investigator award from the Simons Foundation, and the David and Lucile Packard Foundation. NR 52 TC 6 Z9 6 U1 0 U2 0 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0035-8711 EI 1365-2966 J9 MON NOT R ASTRON SOC JI Mon. Not. Roy. Astron. Soc. PD JUL 11 PY 2016 VL 459 IS 4 BP 3614 EP 3619 DI 10.1093/mnras/stw941 PG 6 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DR3VM UT WOS:000379830700018 ER PT J AU Turner, MF Heuberger, AL Kirkwood, JS Collins, CC Wolfrum, EJ Broeckling, C Prenni, JE Jahn, CE AF Turner, Marie F. Heuberger, Adam L. Kirkwood, Jay S. Collins, Carl C. Wolfrum, Edward J. Broeckling, CoreyD. Prenni, Jessica E. Jahn, Courtney E. TI Non-targeted Metabolomics in Diverse Sorghum Breeding Lines Indicates Primary and Secondary Metabolite Profiles Are Associated with Plant Biomass Accumulation and Photosynthesis SO FRONTIERS IN PLANT SCIENCE LA English DT Article DE Sorghumbicolor; GC-MS; LC-MS; biomass; metabolomics; photosynthesis; chlorogenic acid; shikimic acid ID BICOLOR L. MOENCH; QUANTITATIVE TRAIT LOCI; CHLOROGENIC ACID; DROUGHT TOLERANCE; GENETIC-IMPROVEMENT; MAPPING POPULATION; LEAF; REGISTRATION; ARABIDOPSIS; GROWTH AB Metabolomics is an emerging method to improve our understanding of how genetic diversity affects phenotypic variation in plants. Recent studies have demonstrated that genotype has a major influence on biochemical variation in several types of plant tissues, however, the association between metabolic variation and variation in morphological and physiological traits is largely unknown. Sorghum bicolor (L.) is an important food and fuel crop with extensive genetic and phenotypic variation. Sorghum lines have been bred for differing phenotypes beneficial for production of grain (food), stem sugar (food, fuel), and cellulosic biomass (forage, fuel), and these varying phenotypes are the end products of innate metabolic programming which determines how carbon is allocated during plant growth and development. Further, sorghum has been adapted among highly diverse environments. Because of this geographic and phenotypic variation, the sorghum metabolome is expected to be highly divergent; however, metabolite variation in sorghum has not been characterized. Here, we utilize a phenotypically diverse panel of sorghum breeding lines to identify associations between leaf metabolites and morpho-physiological traits. The panel (11 lines) exhibited significant variation for 21 morpho-physiological traits, as well as broader trends in variation by sorghum type (grain vs. biomass types). Variation was also observed for cell wall constituents (glucan, xylan, lignin, ash). Non-targeted metabolomics analysis of leaf tissue showed that 956 of 1181 metabolites varied among the lines (81%, ANOVA, FDR adjusted p < 0.05). Both univariate and multivariate analyses determined relationships between metabolites and morpho-physiological traits, and 384 metabolites correlated with at least one trait (32%, p < 0.05), including many secondary metabolites such as glycosylated flavonoids and chlorogenic acids. The use of metabolomics to explain relationships between two or more morpho-physiological traits was explored and showed chlorogenic and shikimic acid to be associated with photosynthesis, early plant growth and final biomass measures in sorghum. Taken together, this study demonstrates the integration of metabolomics with morpho-physiological datasets to elucidate links between plant metabolism, growth, and architecture. C1 [Turner, Marie F.; Kirkwood, Jay S.; Collins, Carl C.; Jahn, Courtney E.] Colorado State Univ, Dept Bioagr Sci & Pest Management, Ft Collins, CO 80523 USA. [Heuberger, Adam L.] Colorado State Univ, Dept Horticulture & Lansdscape Architecture, Ft Collins, CO USA. [Kirkwood, Jay S.; Broeckling, CoreyD.; Prenni, Jessica E.] Colorado State Univ, Prot & Metab Facil, Ft Collins, CO USA. [Wolfrum, Edward J.] Natl Renewable Energy Lab, Golden, CO USA. RP Jahn, CE (reprint author), Colorado State Univ, Dept Bioagr Sci & Pest Management, Ft Collins, CO 80523 USA. EM courtney.jahn@colostate.edu OI Prenni, Jessica/0000-0002-0337-8450; Wolfrum, Edward/0000-0002-7361-8931 FU Colorado State University Agricultural Experiment Station; Energy Institute at Colorado State University; U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory; US DOE Bioenergy Technologies Office (BETO); Colorado State University Libraries Open Access Research and Scholarship Fund FX The work of MT, JK, CC, and CJ was supported by the Colorado State University Agricultural Experiment Station and the Energy Institute at Colorado State University. The work of EW was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory with funding provided by US DOE Bioenergy Technologies Office (BETO). The content is solely the responsibility of the authors and does not necessarily represent the official views of the Energy Institute at Colorado State University. We would like to acknowledge generous support by the Colorado State University Libraries Open Access Research and Scholarship Fund. The funding bodies did not participate in the design, collection, analysis and interpretation of data; or in preparation of the manuscript. NR 83 TC 0 Z9 0 U1 29 U2 44 PU FRONTIERS MEDIA SA PI LAUSANNE PA PO BOX 110, EPFL INNOVATION PARK, BUILDING I, LAUSANNE, 1015, SWITZERLAND SN 1664-462X J9 FRONT PLANT SCI JI Front. Plant Sci. PD JUL 11 PY 2016 VL 7 AR 953 DI 10.3389/fpls.2016.00953 PG 17 WC Plant Sciences SC Plant Sciences GA DQ6ZW UT WOS:000379357000001 PM 27462319 ER PT J AU Beauvois, K Campbell, CE Dawidowski, J Fak, B Godfrin, H Krotscheck, E Lauter, HJ Lichtenegger, T Ollivier, J Sultan, A AF Beauvois, K. Campbell, C. E. Dawidowski, J. Fak, B. Godfrin, H. Krotscheck, E. Lauter, H. -J. Lichtenegger, T. Ollivier, J. Sultan, A. TI Superfluid He-4 dynamics beyond quasiparticle excitations SO PHYSICAL REVIEW B LA English DT Article ID NEUTRON-SCATTERING EXPERIMENTS; MULTIPLE-SCATTERING; COLLECTIVE EXCITATIONS; LIQUID-HELIUM; SPECTRUM; TEMPERATURE AB The dynamics of superfluid He-4 at and above the Landau quasiparticle regime is investigated by high-precision inelastic neutron scattering measurements of the dynamic structure factor. A highly structured response is observed above the familiar phonon-maxon-roton spectrum, characterized by sharp thresholds for phonon-phonon, maxon-roton, and roton-roton coupling processes. The experimental dynamic structure factor is compared to the calculation of the same physical quantity by a dynamic many-body theory including three-phonon processes self-consistently. The theory is found to provide a quantitative description of the dynamics of the correlated bosons for energies up to about three times that of the Landau quasiparticles. C1 [Beauvois, K.; Fak, B.; Ollivier, J.] Inst Laue Langevin, 6 Rue Jules Horowitz, F-38042 Grenoble, France. [Beauvois, K.; Godfrin, H.; Sultan, A.] Univ Grenoble Alpes, Inst NEEL, F-38000 Grenoble, France. [Beauvois, K.; Godfrin, H.; Sultan, A.] CNRS, Inst NEEL, F-38042 Grenoble, France. [Campbell, C. E.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Dawidowski, J.] Comis Nacl Energia Atom, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Dawidowski, J.] Consejo Nacl Invest Cient & Tecn, Ctr Atom Bariloche, RA-8400 San Carlos De Bariloche, Rio Negro, Argentina. [Fak, B.] Univ Grenoble Alpes, INAC SPSMS, F-38000 Grenoble, France. [Fak, B.; Sultan, A.] CEA, INAC SPSMS, F-38000 Grenoble, France. [Krotscheck, E.; Lichtenegger, T.] SUNY Buffalo, Univ Buffalo, Dept Phys, New York, NY 14260 USA. [Krotscheck, E.; Lichtenegger, T.] Johannes Kepler Univ Linz, Inst Theoret Phys, A-4040 Linz, Austria. [Lauter, H. -J.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. RP Godfrin, H (reprint author), Univ Grenoble Alpes, Inst NEEL, F-38000 Grenoble, France.; Godfrin, H (reprint author), CNRS, Inst NEEL, F-38042 Grenoble, France. EM henri.godfrin@neel.cnrs.fr FU Austrian Science Fund FWF [I602]; French grant [ANR-2010-INTB-403-01]; European Community [228464] FX We are grateful to X. Tonon for his help with the experiment, and to E. Farhi for his help with the program McStas. This work was supported, in part, by the Austrian Science Fund FWF grant I602, the French grant ANR-2010-INTB-403-01 and the European Community Research Infrastructures under the FP7 Capacities Specific Programme, MICROKELVIN Project No. 228464. NR 28 TC 2 Z9 2 U1 2 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 11 PY 2016 VL 94 IS 2 AR 024504 DI 10.1103/PhysRevB.94.024504 PG 5 WC Physics, Condensed Matter SC Physics GA DQ8YW UT WOS:000379498600006 ER PT J AU Gasparov, VA Drigo, L Audouard, A He, X Bozovic, I AF Gasparov, V. A. Drigo, L. Audouard, A. He, Xi Bozovic, I. TI Magnetic field dependence of high-T-c interface superconductivity in La1.55Sr0.45CuO4/La2CuO4 heterostructures SO PHYSICAL REVIEW B LA English DT Article ID LONG-RANGE ORDER; CONTINUOUS SYMMETRY GROUP; 2-DIMENSIONAL SYSTEMS; QUANTUM OSCILLATIONS; ORGANIC CONDUCTOR; PHASE COHERENCE; TEMPERATURE; TRANSITION; FILMS; LA2-XSRXCUO4 AB Heterostructures made of a layer of a cuprate insulator La2CuO4 on the top of a layer of a nonsuperconducting cuprate metal La1.55Sr0.45CuO4 show high-T-c interface superconductivity confined within a single CuO2 plane. Given this extreme quasi-two-dimensional quantum confinement, it is of interest to find out how interface superconductivity behaves when exposed to an external magnetic field. With this motivation, we have performed contactless tunnel-diode-oscillator-based measurements in pulsed magnetic fields up to 56 T as well as measurements of the complex mutual inductance between a spiral coil and the film in static fields up to 3 T. Remarkably, we observe that interface superconductivity survives up to very high perpendicular fields, in excess of 40 T. In addition, the critical magnetic field H-m (T) reveals an upward divergence with decreasing temperature, in line with vortex melting as in bulk superconducting cuprates. C1 [Gasparov, V. A.] RAS, Inst Solid State Phys, Chernogolovka 142432, Russia. [Drigo, L.; Audouard, A.] UPS, UGA, INSA, CNRS UPR 3228,Lab Natl Champs Magnet Intenses, Toulouse, France. [He, Xi; Bozovic, I.] Yale Univ, Dept Appl Phys, New Haven, CT 06520 USA. [Bozovic, I.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Gasparov, VA (reprint author), RAS, Inst Solid State Phys, Chernogolovka 142432, Russia. FU CNRS-Russian Academy of Sciences [EDC26086]; Russian Academy of Sciences Program "Quantum mesoscopic and nonhomogeneous systems"; Russian Foundation for Basic Research [12-02-00171]; European Magnetic Field Laboratory (EMFL); U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division; Gordon and Betty Moore Foundation's EPiQS Initiative [GBMF4410] FX We would like to thank A. Koshelev for valuable discussions. This work has been supported by the CNRS-Russian Academy of Sciences Cooperation Agreement No. EDC26086, the Russian Academy of Sciences Program "Quantum mesoscopic and nonhomogeneous systems," and the Russian Foundation for Basic Research Grant No. 12-02-00171. The support of the European Magnetic Field Laboratory (EMFL) is acknowledged as well. Atomic-layer-by-layer MBE synthesis and sample characterization were done at Brookhaven (I.B.) and supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Sciences and Engineering Division. X.H. is supported by the Gordon and Betty Moore Foundation's EPiQS Initiative through Grant No. GBMF4410. NR 60 TC 0 Z9 0 U1 28 U2 34 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 11 PY 2016 VL 94 IS 1 AR 014507 DI 10.1103/PhysRevB.94.014507 PG 6 WC Physics, Condensed Matter SC Physics GA DQ8YK UT WOS:000379497400008 ER PT J AU Ristivojevic, Z Matveev, KA AF Ristivojevic, Zoran Matveev, K. A. TI Decay of Bogoliubov excitations in one-dimensional Bose gases SO PHYSICAL REVIEW B LA English DT Article ID ULTRACOLD GASES; QUANTUM; SPECTRUM; BOSONS AB We study the decay of Bogoliubov quasiparticles in one-dimensional Bose gases. Starting from the hydrodynamic Hamiltonian, we develop a microscopic theory that enables one to systematically study both the excitations and their decay. At zero temperature, the leading mechanism of decay of a quasiparticle is disintegration into three others. We find that low-energy quasiparticles (phonons) decay with the rate that scales with the seventh power of momentum, whereas the rate of decay of the high-energy quasiparticles does not depend on momentum. In addition, our approach allows us to study analytically the quasiparticle decay in the whole crossover region between the two limiting cases. When applied to integrable models, including the Lieb-Liniger model of bosons with contact repulsion, our theory confirms the absence of the decay of quasiparticle excitations. We account for two types of integrability-breaking perturbations that enable finite decay: three-body interaction between the bosons and two-body interaction of finite range. C1 [Ristivojevic, Zoran] Univ Toulouse, CNRS, UPS, Lab Phys Theor, Toulouse, France. [Matveev, K. A.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Ristivojevic, Z (reprint author), Univ Toulouse, CNRS, UPS, Lab Phys Theor, Toulouse, France. FU U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division FX We acknowledge stimulating discussions with L. I. Glazman and M. Pustilnik. K.A.M. is grateful to Laboratoire de Physique Theorique, Toulouse, where part of the work was performed, for hospitality. Work by K.A.M. was supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division. NR 41 TC 1 Z9 1 U1 0 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 11 PY 2016 VL 94 IS 2 AR 024506 DI 10.1103/PhysRevB.94.024506 PG 15 WC Physics, Condensed Matter SC Physics GA DQ8YW UT WOS:000379498600008 ER PT J AU DeGrand, T Golterman, M Neil, ET Shamir, Y AF DeGrand, Thomas Golterman, Maarten Neil, Ethan T. Shamir, Yigal TI One-loop chiral perturbation theory with two fermion representations SO PHYSICAL REVIEW D LA English DT Article ID ELECTROWEAK SYMMETRY-BREAKING; FINITE BARYON DENSITY; COMPOSITE AXION; SEXTET QUARKS; COLOR; PARTICLES; HADRONS; UPSILON; PHYSICS; MASS AB We develop chiral perturbation theory for chirally broken theories with fermions in two different representations of the gauge group. Any such theory has a nonanomalous singlet U(1)(A) symmetry, yielding an additional Nambu-Goldstone boson when spontaneously broken. We calculate the next-to-leading order corrections for the pseudoscalar masses and decay constants, which include the singlet Nambu-Goldstone boson, as well as for the two condensates. The results can be generalized to more than two representations. C1 [DeGrand, Thomas; Neil, Ethan T.] Univ Colorado, Dept Phys, Boulder, CO 80309 USA. [Golterman, Maarten] San Francisco State Univ, Dept Phys & Astron, San Francisco, CA 94132 USA. [Neil, Ethan T.] Brookhaven Natl Lab, RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Shamir, Yigal] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. RP DeGrand, T (reprint author), Univ Colorado, Dept Phys, Boulder, CO 80309 USA. FU U.S. Department of Energy [DE-SC0010005, DE-FG03-92ER40711, DE-SC0012704]; Israel Science Foundation [449/13] FX M. G. and Y. S. would like to thank the Department of Physics of the University of Colorado, and Y. S. would like to thank the Department of Physics and Astronomy of San Francisco State University, for hospitality. The research of T. D., M. G., and E. N. is supported in part by the U.S. Department of Energy under Grants No. DE-SC0010005 (T. D. and E. N.) and No. DE-FG03-92ER40711 (M. G.). Y. S. is supported by the Israel Science Foundation under Grant No. 449/13. Brookhaven National Laboratory is supported by the U.S. Department of Energy under Contract No. DE-SC0012704. NR 53 TC 1 Z9 1 U1 1 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 11 PY 2016 VL 94 IS 2 AR 025020 DI 10.1103/PhysRevD.94.025020 PG 12 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DQ9DN UT WOS:000379510700008 ER PT J AU Achilleos, V Bishop, AR Diamantidis, S Frantzeskakis, DJ Horikis, TP Karachalios, NI Kevrekidis, PG AF Achilleos, V. Bishop, A. R. Diamantidis, S. Frantzeskakis, D. J. Horikis, T. P. Karachalios, N. I. Kevrekidis, P. G. TI Dynamical playground of a higher-order cubic Ginzburg-Landau equation: From orbital connections and limit cycles to invariant tori and the onset of chaos SO PHYSICAL REVIEW E LA English DT Article ID NONLINEAR SCHRODINGER-EQUATION; SINE-GORDON EQUATION; DARK SOLITONS; MODULATION INSTABILITY; SPATIOTEMPORAL CHAOS; MODE-LOCKING; LASERS; STATIONARY; ATTRACTORS; GEOMETRY AB The dynamical behavior of a higher-order cubic Ginzburg-Landau equation is found to include a wide range of scenarios due to the interplay of higher-order physically relevant terms. We find that the competition between the third-order dispersion and stimulated Raman scattering effects gives rise to rich dynamics: this extends from Poincare-Bendixson-type scenarios, in the sense that bounded solutions may converge either to distinct equilibria via orbital connections or to space-time periodic solutions, to the emergence of almost periodic and chaotic behavior. One of our main results is that third-order dispersion has a dominant role in the development of such complex dynamics, since it can be chiefly responsible (even in the absence of other higher-order effects) for the existence of periodic, quasiperiodic, and chaotic spatiotemporal structures. Suitable low-dimensional phase-space diagnostics are devised and used to illustrate the different possibilities and identify their respective parametric intervals over multiple parameters of the model. C1 [Achilleos, V.] Univ Maine, Acoust Lab, Ave O Messiaen, F-72085 Le Mans, France. [Bishop, A. R.; Kevrekidis, P. G.] Los Alamos Natl Lab, Ctr Nonlinear Studies & Theoret Div, Los Alamos, NM 87545 USA. [Diamantidis, S.; Karachalios, N. I.] Univ Aegean, Dept Math, Karlovassi 83200, Samos, Greece. [Frantzeskakis, D. J.] Univ Athens, Dept Phys, Athens 15784, Greece. [Horikis, T. P.] Univ Ioannina, Dept Math, POB 1186, GR-45110 Ioannina, Greece. [Kevrekidis, P. G.] Univ Massachusetts, Dept Math & Stat, Amherst, MA 01003 USA. RP Frantzeskakis, DJ (reprint author), Univ Athens, Dept Phys, Athens 15784, Greece. EM dfrantz@phys.uoa.gr OI Karachalios, Nikos I./0000-0002-5580-3957 FU QNRF Grant [NPRP8-764-1-160] FX D.J.F., N.I.K., and P.G.K. gratefully acknowledge the support of QNRF Grant No. NPRP8-764-1-160. NR 56 TC 0 Z9 0 U1 6 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD JUL 11 PY 2016 VL 94 IS 1 AR 012210 DI 10.1103/PhysRevE.94.012210 PG 10 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DQ9DW UT WOS:000379511600006 PM 27575126 ER PT J AU Pickworth, LA Hammel, BA Smalyuk, VA MacPhee, AG Scott, HA Robey, HF Landen, OL Barrios, MA Regan, SP Schneider, MB Hoppe, M Kohut, T Holunga, D Walters, C Haid, B Dayton, M AF Pickworth, L. A. Hammel, B. A. Smalyuk, V. A. MacPhee, A. G. Scott, H. A. Robey, H. F. Landen, O. L. Barrios, M. A. Regan, S. P. Schneider, M. B. Hoppe, M., Jr. Kohut, T. Holunga, D. Walters, C. Haid, B. Dayton, M. TI Measurement of Hydrodynamic Growth near Peak Velocity in an Inertial Confinement Fusion Capsule Implosion using a Self-Radiography Technique SO PHYSICAL REVIEW LETTERS LA English DT Article ID RICHTMYER-MESHKOV INSTABILITY; NATIONAL-IGNITION-FACILITY; OMEGA-LASER-SYSTEM; SPHERICAL IMPLOSIONS; PERTURBATION GROWTH; TAYLOR INSTABILITY; DECELERATION PHASE; SHELL MODULATIONS; ABSORPTION-LINES; TARGETS AB First measurements of hydrodynamic growth near peak implosion velocity in an inertial confinement fusion (ICF) implosion at the National Ignition Facility were obtained using a self-radiographing technique and a preimposed Legendre mode 40, lambda = 140 mu m, sinusoidal perturbation. These are the first measurements of the total growth at the most unstable mode from acceleration Rayleigh-Taylor achieved in any ICF experiment to date, showing growth of the areal density perturbation of similar to 7000x. Measurements were made at convergences of similar to 5 to similar to 10x at both the waist and pole of the capsule, demonstrating simultaneous measurements of the growth factors from both lines of sight. The areal density growth factors are an order of magnitude larger than prior experimental measurements and differed by similar to 2x between the waist and the pole, showing asymmetry in the measured growth factors. These new measurements significantly advance our ability to diagnose perturbations detrimental to ICF implosions, uniquely intersecting the change from an accelerating to decelerating shell, with multiple simultaneous angular views. C1 [Pickworth, L. A.; Hammel, B. A.; Smalyuk, V. A.; MacPhee, A. G.; Scott, H. A.; Robey, H. F.; Landen, O. L.; Barrios, M. A.; Schneider, M. B.; Kohut, T.; Holunga, D.; Walters, C.; Haid, B.; Dayton, M.] Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. [Regan, S. P.] Univ Rochester, Laser Energet Lab, Rochester, NY USA. [Hoppe, M., Jr.] Gen Atom Co, San Diego, CA USA. RP Pickworth, LA (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94551 USA. EM pickworth1@llnl.gov OI Pickworth, Louisa/0000-0002-0585-1934 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors thank the engineering, target fabrication, and operations teams at the National Ignition Facility who made these experiments possible. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 71 TC 1 Z9 1 U1 8 U2 10 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 11 PY 2016 VL 117 IS 3 AR 035001 DI 10.1103/PhysRevLett.117.035001 PG 6 WC Physics, Multidisciplinary SC Physics GA DQ9EO UT WOS:000379513400004 PM 27472117 ER PT J AU Zylstra, AB Herrmann, HW Johnson, MG Kim, YH Frenje, JA Hale, G Li, CK Rubery, M Paris, M Bacher, A Brune, CR Forrest, C Glebov, VY Janezic, R McNabb, D Nikroo, A Pino, J Sangster, TC Seguin, FH Seka, W Sio, H Stoeckl, C Petrasso, RD AF Zylstra, A. B. Herrmann, H. W. Johnson, M. Gatu Kim, Y. H. Frenje, J. A. Hale, G. Li, C. K. Rubery, M. Paris, M. Bacher, A. Brune, C. R. Forrest, C. Glebov, V. Yu. Janezic, R. McNabb, D. Nikroo, A. Pino, J. Sangster, T. C. Seguin, F. H. Seka, W. Sio, H. Stoeckl, C. Petrasso, R. D. TI Using Inertial Fusion Implosions to Measure the T + He-3 Fusion Cross Section at Nucleosynthesis-Relevant Energies SO PHYSICAL REVIEW LETTERS LA English DT Article ID BIG-BANG NUCLEOSYNTHESIS; PRIMORDIAL NUCLEOSYNTHESIS; ENERGIES; LI-6; PERFORMANCE; STARS AB Light nuclei were created during big-bang nucleosynthesis (BBN). Standard BBN theory, using rates inferred from accelerator-beam data, cannot explain high levels of Li-6 in low-metallicity stars. Using high-energy-density plasmas we measure the T(He-3, gamma)Li-6 reaction rate, a candidate for anomalously high Li-6 production; we find that the rate is too low to explain the observations, and different than values used in common BBN models. This is the first data directly relevant to BBN, and also the first use of laboratory plasmas, at comparable conditions to astrophysical systems, to address a problem in nuclear astrophysics. C1 [Zylstra, A. B.; Johnson, M. Gatu; Frenje, J. A.; Li, C. K.; Seguin, F. H.; Sio, H.; Petrasso, R. D.] MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Zylstra, A. B.; Herrmann, H. W.; Kim, Y. H.; Hale, G.; Paris, M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Rubery, M.] AWE Plc, Dept Plasma Phys, Reading RG7 4PR, Berks, England. [Bacher, A.] Indiana Univ, Bloomington, IN 47405 USA. [Brune, C. R.] Ohio Univ, Athens, OH 45701 USA. [Forrest, C.; Glebov, V. Yu.; Janezic, R.; Sangster, T. C.; Seka, W.; Stoeckl, C.] Univ Rochester, Laser Energet Lab, Rochester, NY 14623 USA. [McNabb, D.; Pino, J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Nikroo, A.] Gen Atom Co, San Diego, CA 92186 USA. RP Zylstra, AB (reprint author), MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA.; Zylstra, AB (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM zylstra@lanl.gov FU U.S. DOE [DE-NA0001857, DE-FC52-08NA28752, DE-FG02-88ER40387, DE-NA0001837, DE-AC52-06NA25396]; LLNL [B597367]; LLE [415935-G]; Fusion Science Center at the University of Rochester [524431]; National Laser Users Facility [DE-NA0002035]; National Science Foundation Graduate Research Fellowship Program [1122374]; Laboratory Directed Research and Development (LDRD) program at Los Alamos National Laboratory [20150717PRD2] FX We thank the operations crews and engineering staff at OMEGA for supporting these experiments, and E. Doeg and R. Frankel for their work processing the CR-39. This work was supported in part by the U.S. DOE (Grants No. DE-NA0001857, No. DE-FC52-08NA28752, No. DE-FG02-88ER40387, No. DE-NA0001837, No. DE-AC52-06NA25396), LLNL (No. B597367), LLE (No. 415935-G), the Fusion Science Center at the University of Rochester (No. 524431), and the National Laser Users Facility (No. DE-NA0002035). A. B. Z. acknowledges support by the National Science Foundation Graduate Research Fellowship Program under Grant No. 1122374, and gratefully acknowledges the support provided for this work by the Laboratory Directed Research and Development (LDRD) program, Project No. 20150717PRD2, at Los Alamos National Laboratory. NR 35 TC 0 Z9 0 U1 10 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 11 PY 2016 VL 117 IS 3 AR 035002 DI 10.1103/PhysRevLett.117.035002 PG 5 WC Physics, Multidisciplinary SC Physics GA DQ9EO UT WOS:000379513400005 PM 27472118 ER PT J AU Liu, JX Li, HC Zhang, L Rames, M Zhang, M Yu, YD Peng, B Celis, CD Xu, A Zou, Q Yang, X Chen, XF Ren, G AF Liu, Jinxin Li, Hongchang Zhang, Lei Rames, Matthew Zhang, Meng Yu, Yadong Peng, Bo Celis, Cesar Diaz Xu, April Zou, Qin Yang, Xu Chen, Xuefeng Ren, Gang TI Fully Mechanically Controlled Automated Electron Microscopic Tomography SO SCIENTIFIC REPORTS LA English DT Article ID MOLECULAR-DYNAMICS; IMPLEMENTATION AB Knowledge of three-dimensional (3D) structures of each individual particles of asymmetric and flexible proteins is essential in understanding those proteins' functions; but their structures are difficult to determine. Electron tomography (ET) provides a tool for imaging a single and unique biological object from a series of tilted angles, but it is challenging to image a single protein for three-dimensional (3D) reconstruction due to the imperfect mechanical control capability of the specimen goniometer under both a medium to high magnification (approximately 50,000-160,000x) and an optimized beam coherence condition. Here, we report a fully mechanical control method for automating ET data acquisition without using beam tilt/shift processes. This method could reduce the accumulation of beam tilt/shift that used to compensate the error from the mechanical control, but downgraded the beam coherence. Our method was developed by minimizing the error of the target object center during the tilting process through a closed-loop proportional-integral (PI) control algorithm. The validations by both negative staining (NS) and cryo-electron microscopy (cryo-EM) suggest that this method has a comparable capability to other ET methods in tracking target proteins while maintaining optimized beam coherence conditions for imaging. C1 [Liu, Jinxin; Li, Hongchang; Zhang, Lei; Rames, Matthew; Zhang, Meng; Yu, Yadong; Peng, Bo; Ren, Gang] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Liu, Jinxin; Chen, Xuefeng] Xi An Jiao Tong Univ, State Key Lab Mfg Syst Engn, Xian 710049, Peoples R China. [Li, Hongchang; Yang, Xu] Xi An Jiao Tong Univ, Sch Elect Engn, Xian 710049, Peoples R China. [Celis, Cesar Diaz] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Xu, April] Pfizer BioTherapeut Pharmaceut Sci, 401 N Middletown Rd, Pearl River, NY 10956 USA. [Zou, Qin] Pfizer BioTherapeut Pharmaceut Sci, 700 Chesterfield Pkwy West, St Louis, MO 63017 USA. RP Ren, G (reprint author), Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.; Chen, XF (reprint author), Xi An Jiao Tong Univ, State Key Lab Mfg Syst Engn, Xian 710049, Peoples R China.; Yang, X (reprint author), Xi An Jiao Tong Univ, Sch Elect Engn, Xian 710049, Peoples R China. EM yangxu@mail.xjtu.edu.cn; chenxf@mail.xjtu.edu.cn; gren@lbl.gov OI Li, Hongchang/0000-0002-0684-7582 FU Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-AC02-05CH11231]; National Heart, Lung, and Blood Institute of the National Institutes of Health [R01HL115153]; National Institute of General Medical Sciences of the National Institutes of Health [R01GM104427] FX We thank Carlos Bustamante for the nucleosome-DNA sample, Dr. Ron Krauss for the LDL sample. We would also like to thank Shawn Zeng for his discussions and comments. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. G.R. is supported by the National Heart, Lung, and Blood Institute of the National Institutes of Health (no. R01HL115153) and the National Institute of General Medical Sciences of the National Institutes of Health (no. R01GM104427). We also want to thank Dr. Frank Kotch from Pfizer to generate the antibody conjugate sample. NR 22 TC 0 Z9 0 U1 2 U2 5 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 11 PY 2016 VL 6 AR 29231 DI 10.1038/srep29231 PG 12 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DQ6PL UT WOS:000379327200001 PM 27403922 ER PT J AU Liu, QW Zheng, XL He, JL Wang, WP Fu, MM Cao, YY Li, H Wu, YP Chen, T Zhang, CM Chen, XH Yu, BB Li, SP Kang, JY Wu, ZM AF Liu, Qianwen Zheng, Xuanli He, Jialun Wang, Weiping Fu, Mingming Cao, Yiyan Li, Heng Wu, Yaping Chen, Ting Zhang, Chunmiao Chen, Xiaohong Yu, Binbin Li, Shuping Kang, Junyong Wu, Zhiming TI Enhanced magneto-optical effects in composite coaxial nanowires embedded with Ag nanoparticles SO SCIENTIFIC REPORTS LA English DT Article ID FARADAY-ROTATION ENHANCEMENT; SURFACE-PLASMON RESONANCE; IRON-OXIDE NANOCRYSTALS; MAGNETIC-PROPERTIES; OPTICAL ISOLATION; ARRAYS; FILMS AB Nanostructures decorated with noble metal nanoparticles (NPs) exhibit potential for use in highly sensitive optoelectronic devices through the localized surface plasmon resonance (LSPR) effect. In this study, Faraday rotation was significantly enhanced through the structural optimization of ferromagnetic (FM)/semiconductor composite nanostructures. Experimental and theoretical results revealed that the position of noble metal NPs significantly influenced the coupling of the LSPR-enhanced electromagnetic field with FM materials. Furthermore, nanostructures embedded with noble metals demonstrated an improved capability to efficiently use the electromagnetic field compared to other structures. The Faraday rotation of ZnO/Ag(NPs)/Fe was enhanced 58 fold compared to that of the ZnO(film)/Fe. This work provides a basis for the design of nanoarchitectures for miniaturized high-performance magneto-optical devices. C1 [Liu, Qianwen; Zheng, Xuanli; He, Jialun; Wang, Weiping; Fu, Mingming; Cao, Yiyan; Li, Heng; Wu, Yaping; Chen, Ting; Zhang, Chunmiao; Chen, Xiaohong; Yu, Binbin; Li, Shuping; Kang, Junyong; Wu, Zhiming] Xiamen Univ, Fujian Prov Key Lab Semicond & Applicat, Collaborat Innovat Ctr Optoelect Semicond & Effic, Dept Phys, Xiamen 361005, Peoples R China. [Wu, Zhiming] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Li, H; Wu, ZM (reprint author), Xiamen Univ, Fujian Prov Key Lab Semicond & Applicat, Collaborat Innovat Ctr Optoelect Semicond & Effic, Dept Phys, Xiamen 361005, Peoples R China.; Wu, ZM (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM liheng3000@xmu.edu; zmwu@xmu.edu.cn FU "973" Program [2012CB619301]; National Natural Science Foundations of China [61227009, 11304257]; Natural Science Foundation of Fujian Province of China [2015J01028, 2014J01026]; Fundamental Research Funds for the Central Universities [20720150027, 20720160044, 20720150033] FX The work was supported by "973" Program (no. 2012CB619301), the National Natural Science Foundations of China (no. 61227009 and 11304257), Natural Science Foundation of Fujian Province of China (2015J01028 and 2014J01026), and Fundamental Research Funds for the Central Universities (20720150027, 20720160044 and 20720150033). NR 34 TC 0 Z9 0 U1 22 U2 35 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 11 PY 2016 VL 6 AR 29170 DI 10.1038/srep29170 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DQ6PF UT WOS:000379326600001 PM 27403716 ER PT J AU Anderson, D Apresyan, A Bornheim, A Duarte, J Pena, C Spiropulu, M Trevor, J Xie, S Ronzhin, A AF Anderson, Dustin Apresyan, Artur Bornheim, Adolf Duarte, Javier Pena, Cristian Spiropulu, Maria Trevor, Jason Xie, Si Ronzhin, Anatoly TI Precision timing calorimeter for high energy physics SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Time of flight detector; Precision timing; LYSO; MCP; Pico-second timing ID CRYSTALS AB Scintillator based calorimeter technology is studied with the aim to achieve particle detection with a time resolution on the order of a few 10 ps for photons and electrons at energies of a few GeV and above. We present results from a prototype of a 1.4 x 1.4 x 11.4 cm(3) sampling calorimeter cell consisting of tungsten absorber plates and Cerium-doped Lutetium Yttrium Orthosilicate (LYSO) crystal scintillator plates. The LYSO plates are read out with wave lengths shifting fibers which are optically coupled to fast photo detectors on both ends of the fibers. The measurements with electrons were performed at the Fermilab Test Beam Facility (FTBF) and the CERN SPS H2 test beam. In addition to the baseline setup plastic scintillation counter and a MCP-PMT were used as trigger and as a reference for a time of flight measurement (TOF). We also present measurements with a fast laser to further characterize the response of the prototype and the photo sensors. All data were recorded using a DRS4 fast sampling digitizer. These measurements are part of an R&D program whose aim is to demonstrate the feasibility of building a large scale electromagnetic calorimeter with a time resolution on the order of 10 ps, to be used in high energy physics experiments. (C) 2015 Elsevier B.V. All rights reserved. C1 [Anderson, Dustin; Apresyan, Artur; Bornheim, Adolf; Duarte, Javier; Pena, Cristian; Spiropulu, Maria; Trevor, Jason; Xie, Si] CALTECH, Pasadena, CA 91125 USA. [Ronzhin, Anatoly] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RP Bornheim, A (reprint author), CALTECH, Pasadena, CA 91125 USA. EM bornheim@hep.caltech.edu RI Xie, Si/O-6830-2016 OI Xie, Si/0000-0003-2509-5731 FU Fermi Research Alliance, LLC [DE-AC02-07CH11359]; United States Department of Energy; California Institute of Technology High Energy Physics [DE-SC0011925] FX We would like to thank Erik Ramberg, Sergey Los and Aria Soha for their help and support and the FNAL and CERN TBF for the beam delivery and control. We thank Randy Ruchti for providing us with DSB fibers and Eileen Hahn for polishing the fibers. We would also like to thank Ewa Skup, Geoff Savage and Todd Nobel for help with the beam instrumentation, organizing and providing the supporting equipment at FTBF as well as David Bailleux and Tatiana Medvedeva for help at CERN. This work is supported by funding from Fermi Research Alliance, LLC under Contract no. DE-AC02-07CH11359 with the United States Department of Energy and from California Institute of Technology High Energy Physics under Contract DE-SC0011925 with the United States Department of Energy. NR 10 TC 0 Z9 0 U1 1 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2016 VL 824 BP 670 EP 673 DI 10.1016/j.nima.2015.11.129 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DL1RD UT WOS:000375408700224 ER PT J AU Xie, JQ Byrum, K Demarteau, M May, E Wagner, R Walters, D Wang, JB Xia, L Zhao, HY AF Xie, Junqi Byrum, Karen Demarteau, Marcel May, Edward Wagner, Robert Walters, Dean Wang, Jingbo Xia, Lei Zhao, Huyue TI Development of a low-cost fast-timing microchannel plate photodetector SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Microchannel plate; MCP; Photodetector; Time resolution; Spatial resolution; Quantum efficiency AB We report on the design, fabrication and characterization of a prototype 6 x 6 cm(2) microchannel plate photodetector with precise fast-timing measurement capability. The whole assembly is made of low cost glass materials with a bialkali photocathode top window. All components are hermetically sealed in vacuum. The prototype photodetector exhibits time resolution of 65 ps and 16 ps at single-photoelectron and multi-photoelectron levels, respectively. The spatial resolution reaches 0.54 mm for multi photoelectron measurements. The bialkali photocathode exhibits a maximum quantum efficiency exceeding 20% with a uniformity of +/- 40%. (C) 2015 Elsevier B.V. All rights reserved. C1 [Xie, Junqi; Byrum, Karen; Demarteau, Marcel; May, Edward; Wagner, Robert; Walters, Dean; Wang, Jingbo; Xia, Lei; Zhao, Huyue] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Xie, JQ; Byrum, K (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM jxie@anl.gov; byrum@anl.gov FU U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences and Office of High Energy Physics [DE-AC02-06CH11357] FX Work at Argonne National Laboratory was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences and Office of High Energy Physics under Contract DE-AC02-06CH11357. NR 8 TC 1 Z9 1 U1 3 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2016 VL 824 BP 159 EP 161 DI 10.1016/j.nima.2015.11.024 PG 3 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DL1RD UT WOS:000375408700055 ER PT J AU Barzi, E Zlobin, AV AF Barzi, Emanuela Zlobin, Alexander V. TI 15 Years of R&D on high field accelerator magnets at FNAL SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Accelerator magnet; Composite wire; Dipole; Nb3Sn; Quadrupole; Rutherford cable ID CABLE AB The High Field Magnet (HFM) Program at Fermi National Accelerator Laboratory (FNAL) has been developing Nb3Sn superconducting magnets, materials and technologies for present and future particle accelerators since the late 1990s. This paper summarizes the main results of the Nb3Sn accelerator magnet and superconductor R&D at FNAL and outlines the Program next steps. (C) 2015 Elsevier B.V. All rights reserved. C1 [Barzi, Emanuela; Zlobin, Alexander V.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. RP Barzi, E (reprint author), Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. EM barzi@fnal.gov FU Fermi Research Alliance, LLC [DE-AC02-07CH11359]; US Department of Energy FX This work was supported by Fermi Research Alliance, LLC, under Contract no. DE-AC02-07CH11359 with the US Department of Energy. NR 16 TC 0 Z9 0 U1 4 U2 10 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2016 VL 824 BP 168 EP 172 DI 10.1016/j.nima.2015.12.023 PG 5 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DL1RD UT WOS:000375408700058 ER PT J AU Abba, A Bedeschi, F Caponio, F Cenci, R Citterio, M Cusimano, A Fu, J Geraci, A Grizzuti, M Lusardi, N Marino, P Morello, MJ Neri, N Ninci, D Petruzzo, M Piucci, A Punzi, G Ristori, L Spinella, F Stracka, S Tonelli, D Walsh, J AF Abba, A. Bedeschi, F. Caponio, F. Cenci, R. Citterio, M. Cusimano, A. Fu, J. Geraci, A. Grizzuti, M. Lusardi, N. Marino, P. Morello, M. J. Neri, N. Ninci, D. Petruzzo, M. Piucci, A. Punzi, G. Ristori, L. Spinella, F. Stracka, S. Tonelli, D. Walsh, J. TI An "artificial retina" processor for track reconstruction at the full LHC crossing rate SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Pattern recognition; Trigger; Real-time online tracking AB We present the latest results of an R&D study for a specialized processor capable of reconstructing, in a silicon pixel detector, high-quality tracks from high-energy collision events at 40 MHz. The processor applies a highly parallel pattern-recognition algorithm inspired to quick detection of edges in mammals visual cortex. After a detailed study of a real-detector application, demonstrating that online reconstruction of offline-quality tracks is feasible at 40 MHz with sub-microsecond latency, we are implementing a prototype using common high-bandwidth FPGA devices. (C) 2015 Elsevier B.V. All rights reserved. C1 [Bedeschi, F.; Cenci, R.; Marino, P.; Morello, M. J.; Ninci, D.; Piucci, A.; Punzi, G.; Spinella, F.; Stracka, S.; Walsh, J.] Ist Nazl Fis Nucl, Sez Pisa, Lgo Pontecorvo 3, I-56127 Pisa, Italy. [Ninci, D.; Piucci, A.; Punzi, G.; Stracka, S.] Univ Pisa, Pisa, Italy. [Cenci, R.; Marino, P.; Morello, M. J.] Scuola Normale Super Pisa, Pisa, Italy. [Abba, A.; Caponio, F.; Citterio, M.; Cusimano, A.; Fu, J.; Geraci, A.; Grizzuti, M.; Lusardi, N.; Neri, N.; Petruzzo, M.] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Petruzzo, M.] Univ Milan, Milan, Italy. [Abba, A.; Caponio, F.; Cusimano, A.; Geraci, A.; Grizzuti, M.; Lusardi, N.] Politecn Milan, I-20133 Milan, Italy. [Ristori, L.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Tonelli, D.] CERN, CH-1211 Geneva 23, Switzerland. RP Cenci, R (reprint author), Ist Nazl Fis Nucl, Sez Pisa, Lgo Pontecorvo 3, I-56127 Pisa, Italy. EM riccardo.cenci@pi.infn.it RI Marino, Pietro/N-7030-2015; Stracka, Simone/M-3931-2015 OI Marino, Pietro/0000-0003-0554-3066; Stracka, Simone/0000-0003-0013-4714 NR 6 TC 0 Z9 0 U1 5 U2 9 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2016 VL 824 BP 260 EP 262 DI 10.1016/j.nima.2015.10.048 PG 3 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DL1RD UT WOS:000375408700091 ER PT J AU Citterio, M Camplani, A Cannon, M Chen, H Chen, K Deng, B Liu, C Meroni, C Kierstead, J Takai, H Wirthlin, M Ye, J AF Citterio, M. Camplani, A. Cannon, M. Chen, H. Chen, K. Deng, B. Liu, C. Meroni, C. Kierstead, J. Takai, H. Wirthlin, M. Ye, J. TI Radiation testing campaign results for understanding the suitability of FPGAs in detector electronics SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE FPGA; Radiation; High energy physics experiment AB SRAM based Field Programmable Gate Arrays (FPGAs) have been rarely used in High Energy Physics (HEP) due to their sensitivity to radiation. The last generation of commercial FPGAs based on 28 nm feature size and on Silicon On Insulator (SOI) technologies are more tolerant to radiation to the level that their use in front-end electronics is now feasible. FPGAs provide re-programmability, high-speed computation and fast data transmission through the embedded serial transceivers. They could replace custom application specific integrated circuits in front end electronics in locations with moderate radiation field. The use of a FPGA in HEP experiments is only limited by our ability to mitigate single event effects induced by the high energy hadrons present in the radiation field. (C) 2015 Elsevier B.V. All rights reserved. C1 [Citterio, M.; Camplani, A.; Meroni, C.] Ist Nazl Fis Nucl, Via Celoria 16, I-20133 Milan, Italy. [Cannon, M.; Wirthlin, M.] Brigham Young Univ, Provo, UT 84602 USA. [Chen, H.; Chen, K.; Kierstead, J.; Takai, H.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Deng, B.; Liu, C.; Ye, J.] So Methodist Univ, Dallas, TX 75275 USA. RP Citterio, M (reprint author), Ist Nazl Fis Nucl, Via Celoria 16, I-20133 Milan, Italy. EM mauro.citterio@mi.infn.it OI Citterio, Mauro/0000-0002-0842-0654 NR 2 TC 0 Z9 0 U1 1 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2016 VL 824 BP 270 EP 271 DI 10.1016/j.nima.2015.11.033 PG 2 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DL1RD UT WOS:000375408700095 ER PT J AU Atanov, N Baranov, V Budagov, J Carosi, R Cervelli, F Colao, F Cordelli, M Corradi, G Dane, E Davydov, YI Di Falco, S Donati, S Donghia, R Echenard, B Flood, K Giovannella, S Glagolev, V Grancagnolo, F Happacher, F Hitlin, DG Martini, M Miscetti, S Miyashita, T Morescalchi, L Murat, P Pasciuto, D Pezzullo, G Porter, F Saputi, A Sarra, I Soleti, SR Spinella, F Tassielli, G Tereshchenko, V Usubov, Z Zhu, RY AF Atanov, N. Baranov, V. Budagov, J. Carosi, R. Cervelli, F. Colao, F. Cordelli, M. Corradi, G. Dane, E. Davydov, Yu. I. Di Falco, S. Donati, S. Donghia, R. Echenard, B. Flood, K. Giovannella, S. Glagolev, V. Grancagnolo, F. Happacher, F. Hitlin, D. G. Martini, M. Miscetti, S. Miyashita, T. Morescalchi, L. Murat, P. Pasciuto, D. Pezzullo, G. Porter, F. Saputi, A. Sarra, I. Soleti, S. R. Spinella, F. Tassielli, G. Tereshchenko, V. Usubov, Z. Zhu, R. Y. TI Design and status of the Mu2e electromagnetic calorimeter SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Calorimetry; Scintillating crystals; Avalanche photodiodes; Silicon photomultipliers; Lepton flavour violation AB The Mu2e experiment at Fermilab aims at measuring the neutrinoless conversion of a negative muon into an electron and reach a single event sensitivity of 2.5 x 10(-17) after three years of data taking. The monoenergetic electron produced in the final state, is detected by a high precision tracker and a crystal calorimeter, all embedded in a large superconducting solenoid (SD) surrounded by a cosmic ray veto system. The calorimeter is complementary to the tracker, allowing an independent trigger and powerful particle identification, while seeding the track reconstruction and contributing to remove background tracks mimicking the signal. In order to match these requirements, the calorimeter should have an energy resolution of O(5)% and a time resolution better than 500 ps at 100 MeV. The baseline solution is a calorimeter composed of two disks of BaF2 crystals read by UV extended, solar blind, Avalanche Photodiode (APDs), which are under development from a JPL, Caltech, RMD consortium. In this paper, the calorimeter design, the R&D studies carried out so far and the status of engineering are described. A backup alternative setup consisting of a pure CsI crystal matrix read by UV extended Hamamatsu MPPC's is also presented. (C) 2015 Elsevier B.V. All rights reserved. C1 [Atanov, N.; Baranov, V.; Budagov, J.; Davydov, Yu. I.; Glagolev, V.; Tereshchenko, V.; Usubov, Z.] Joint Inst Nucl Res, Dubna, Russia. [Colao, F.; Cordelli, M.; Corradi, G.; Dane, E.; Donghia, R.; Giovannella, S.; Happacher, F.; Martini, M.; Miscetti, S.; Saputi, A.; Sarra, I.; Soleti, S. R.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Echenard, B.; Flood, K.; Hitlin, D. G.; Miyashita, T.; Porter, F.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Martini, M.] Univ Guglielmo Marconi, Rome, Italy. [Carosi, R.; Cervelli, F.; Di Falco, S.; Donati, S.; Morescalchi, L.; Pasciuto, D.; Pezzullo, G.; Spinella, F.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Morescalchi, L.] Univ Siena, Dipartimento Fis, Via Laterina 8, I-53100 Siena, Italy. [Donati, S.; Pasciuto, D.; Pezzullo, G.] Univ Pisa, Dipartimento Fis, Pisa, Italy. [Murat, P.] Fermi Natl Lab, Batavia, IL USA. [Grancagnolo, F.; Tassielli, G.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Donghia, R.] Univ Rome Tre, I-00146 Rome, Italy. RP Miscetti, S (reprint author), Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. EM Stefano.Miscetti@inf.infn.it RI Tassielli, Giovanni Francesco/K-2929-2015; OI Tassielli, Giovanni Francesco/0000-0003-3410-6754; Soleti, Stefano Roberto/0000-0002-5526-1414; Morescalchi, Luca/0000-0002-7819-8139; Giovannella, Simona/0000-0002-6243-1215; Pezzullo, Gianantonio/0000-0002-6653-1555 NR 4 TC 2 Z9 2 U1 1 U2 3 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2016 VL 824 BP 695 EP 698 DI 10.1016/j.nima.2015.09.074 PG 4 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DL1RD UT WOS:000375408700232 ER PT J AU Alonzi, LP Anastasi, A Bjorkquist, R Cauz, D Cantatore, G Dabagov, S Di Sciascio, G Di Stefano, R Fatemi, R Ferrari, C Fienberg, AT Fioretti, A Frankenthal, A Gabbanini, C Gibbons, LK Giovanetti, K Goadhouse, SD Gohn, WP Gorringe, TP Hampai, D Hertzog, DW Iacovacci, M Kammel, P Karuza, M Kaspar, J Kiburg, B Li, L Marignetti, F Mastroianni, S Moricciani, D Pauletta, G Peterson, DA Pocanic, D Santi, L Smith, MW Sweigart, DA Tishchenko, V Van Wechelm, TD Venanzoni, G Wall, KB Winter, P Yai, K AF Alonzi, L. P. Anastasi, A. Bjorkquist, R. Cauz, D. Cantatore, G. Dabagov, S. Di Sciascio, G. Di Stefano, R. Fatemi, R. Ferrari, C. Fienberg, A. T. Fioretti, A. Frankenthal, A. Gabbanini, C. Gibbons, L. K. Giovanetti, K. Goadhouse, S. D. Gohn, W. P. Gorringe, T. P. Hampai, D. Hertzog, D. W. Iacovacci, M. Kammel, P. Karuza, M. Kaspar, J. Kiburg, B. Li, L. Marignetti, F. Mastroianni, S. Moricciani, D. Pauletta, G. Peterson, D. A. Pocanic, D. Santi, L. Smith, M. W. Sweigart, D. A. Tishchenko, V. Van Wechelm, T. D. Venanzoni, G. Wall, K. B. Winter, P. Yai, K. TI The calorimeter system of the new muon g-2 experiment at Fermilab SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Lead-fluoride crystals; Silicon photomultiplier; Electromagnetic calorimeter AB The electromagnetic calorimeter for the new muon (g-2) experiment at Fermilab will consist of arrays of PbF2 Cerenkov crystals read out by large-area silicon photo-multiplier (SiPM) sensors. We report here the requirements for this system, the achieved solution and the results obtained from a test beam using 2.0-4.5 GeV electrons with a 28-element prototype array. (C) 2015 Elsevier B.V. All rights reserved. C1 [Di Stefano, R.; Marignetti, F.] Univ Cassino, I-03043 Cassino, Italy. [Goadhouse, S. D.; Pocanic, D.] Univ Virginia, Charlottesville, VA 22904 USA. [Anastasi, A.; Dabagov, S.; Ferrari, C.; Fioretti, A.; Frankenthal, A.; Gabbanini, C.; Hampai, D.; Venanzoni, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Giovanetti, K.] James Madison Univ, Harrisonburg, VA 22807 USA. [Bjorkquist, R.; Frankenthal, A.; Gibbons, L. K.; Sweigart, D. A.] Cornell Univ, Ithaca, NY 14850 USA. [Fatemi, R.; Gohn, W. P.; Gorringe, T. P.; Tishchenko, V.] Univ Kentucky, Lexington, KY 40506 USA. [Anastasi, A.] Univ Messina, Dipartimento Fis & Sci Terra, Messina, Italy. [Iacovacci, M.] Univ Naples Federico II, Naples, Italy. [Di Stefano, R.; Iacovacci, M.; Marignetti, F.; Mastroianni, S.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Yai, K.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Ferrari, C.; Fioretti, A.; Gabbanini, C.] UOS Pisa, CNR, Ist Nazl Ott, Pisa, Italy. [Di Sciascio, G.; Moricciani, D.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Alonzi, L. P.; Fienberg, A. T.; Hertzog, D. W.; Kammel, P.; Kaspar, J.; Kiburg, B.; Peterson, D. A.; Smith, M. W.; Van Wechelm, T. D.; Wall, K. B.; Winter, P.; Yai, K.] Univ Washington, Box 351560, Seattle, WA 98195 USA. [Li, L.] Shanghai Jiao Tong Univ, Shanghai 200030, Peoples R China. [Li, L.] Shanghai Key Lab Particle Phys & Cosmol, Shanghai, Peoples R China. [Cauz, D.; Pauletta, G.; Santi, L.] Univ Udine, I-33100 Udine, Italy. [Cantatore, G.] Univ Trieste, Trieste, Italy. [Cauz, D.; Cantatore, G.; Karuza, M.; Pauletta, G.; Santi, L.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Cauz, D.; Cantatore, G.; Karuza, M.; Pauletta, G.; Santi, L.] GC Udine, Trieste, Italy. [Karuza, M.] Univ Rijeka, Rijeka, Croatia. [Alonzi, L. P.] Univ Virginia, Charlottesville, VA 22903 USA. [Kiburg, B.] Fermilab Natl Accelerator Lab, Batavia, IL 60510 USA. [Tishchenko, V.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Winter, P.] Argonne Natl Lab, Argonne, IL 60439 USA. RP Venanzoni, G (reprint author), Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. RI Dabagov, Sultan/M-6425-2015 OI Dabagov, Sultan/0000-0003-3087-1205 NR 3 TC 0 Z9 0 U1 8 U2 8 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2016 VL 824 BP 718 EP 720 DI 10.1016/j.nima.2015.11.041 PG 3 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DL1RD UT WOS:000375408700239 ER PT J AU Yang, F Zhang, LY Zhu, RY Kapustinsky, J Nelson, R Wang, ZH AF Yang, Fan Zhang, Liyuan Zhu, Ren-Yuan Kapustinsky, Jon Nelson, Ron Wang, Zhehui TI Proton induced radiation damage in fast crystal scintillators SO NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT LA English DT Article DE Crystal scintillators; LYSO; Proton damage AB This paper reports proton induced radiation damage in fast crystal scintillators. A 20 cm long LYSO crystal, a 15 cm long CeF3 crystal and four liquid scintillator based sealed quartz capillaries were irradiated by 800 MeV protons at Los Alamos up to 3.3 x 10(14) p/cm(2). Four 1.5 mm thick LYSO plates were irradiated by 24 GeV protons at CERN up to 6.9 x 10(15) p/cm(2). The results show an excellent radiation hardness of LYSO crystals against charged hadrons. (C) 2015 Elsevier B.V. All rights reserved. C1 [Yang, Fan; Zhang, Liyuan; Zhu, Ren-Yuan] CALTECH, Pasadena, CA 91125 USA. [Kapustinsky, Jon; Nelson, Ron; Wang, Zhehui] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Zhu, RY (reprint author), CALTECH, Pasadena, CA 91125 USA. FU US Department of Energy [DE-SC0011925] FX This work was supported in part by the US Department of Energy Grant DE-SC0011925. NR 3 TC 0 Z9 0 U1 3 U2 5 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-9002 EI 1872-9576 J9 NUCL INSTRUM METH A JI Nucl. Instrum. Methods Phys. Res. Sect. A-Accel. Spectrom. Dect. Assoc. Equip. PD JUL 11 PY 2016 VL 824 BP 726 EP 728 DI 10.1016/j.nima.2015.11.100 PG 3 WC Instruments & Instrumentation; Nuclear Science & Technology; Physics, Nuclear; Physics, Particles & Fields SC Instruments & Instrumentation; Nuclear Science & Technology; Physics GA DL1RD UT WOS:000375408700241 ER PT J AU Gong, Y Cooray, A Mitchell-Wynne, K Chen, XL Zemcov, M Smidt, J AF Gong, Yan Cooray, Asantha Mitchell-Wynne, Ketron Chen, Xuelei Zemcov, Michael Smidt, Joseph TI AXION DECAY AND ANISOTROPY OF NEAR-IR EXTRAGALACTIC BACKGROUND LIGHT SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmology: theory; diffuse radiation; large-scale structure of universe ID DARK-MATTER; FLUCTUATIONS; REIONIZATION; ULTRAVIOLET; UNIVERSE; DENSITY; EPOCH; CONSTRAINTS; ATTENUATION; OPACITY AB The extragalactic background light (EBL) is composed of the cumulative radiation from all galaxies and active galactic nuclei over cosmic history. In addition to point sources, the EBL also contains information from diffuse sources of radiation. The angular power spectra of the near-infrared intensities could contain additional signals, and a complete understanding of the nature of the infrared (IR) background is still lacking in the literature. Here we explore the constraints that can be placed on particle decays, especially candidate dark matter (DM) models involving axions that trace DM halos of galaxies. Axions with a mass around a few electronvolts will decay via two photons with wavelengths in the near-IR band and will leave a signature in the IR background intensity power spectrum. Using recent power spectra measurements from the Hubble Space Telescope and the Cosmic Infrared Background Experiment, we find that the 0.6-1.6 mu m power spectra can be explained by axions with masses around 4 eV. The total axion abundance Omega(a) similar or equal to 0.05, and it is comparable to the baryon density of the universe. The suggested mean axion mass and abundance are not ruled out by existing cosmological observations. Interestingly, the axion model with a mass distribution is preferred by the data, which cannot be explained by the standard quantum chromodynamics theory and needs further discussion. C1 [Gong, Yan; Chen, Xuelei] Chinese Acad Sci, Natl Astron Observ, Beijing 100012, Peoples R China. [Gong, Yan; Cooray, Asantha; Mitchell-Wynne, Ketron] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Chen, Xuelei] Peking Univ, Ctr High Energy Phys, Beijing 100871, Peoples R China. [Zemcov, Michael] Rochester Inst Technol, Sch Phys & Astron, Ctr Detectors, Rochester, NY 14623 USA. [Smidt, Joseph] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Gong, Y (reprint author), Chinese Acad Sci, Natl Astron Observ, Beijing 100012, Peoples R China.; Gong, Y (reprint author), Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. OI Gong, Yan/0000-0003-0709-0101 FU Bairen program from National Astronomical Observatories, Chinese Academy of Sciences; NSF CAREER [AST-0645427, AST-1313319]; MoST 863 program grant [2012AA121701]; pilot B grant [XDB09020301]; NSFC grant [11373030] FX YG acknowledges the support of the Bairen program from the National Astronomical Observatories, Chinese Academy of Sciences. YG and AC acknowledge the support from NSF CAREER AST-0645427 and AST-1313319. XLC acknowledges the support of the MoST 863 program grant 2012AA121701, pilot B grant XDB09020301, and the NSFC grant 11373030. We thank an anonymous referee for helpful comments. NR 42 TC 0 Z9 0 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 10 PY 2016 VL 825 IS 2 AR 104 DI 10.3847/0004-637X/825/2/104 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DU1BM UT WOS:000381940800022 ER PT J AU Hong, J Mori, K Hailey, CJ Nynka, M Zhang, S Gotthelf, E Fornasini, FM Krivonos, R Bauer, F Perez, K Tomsick, JA Bodaghee, A Chiu, JL Clavel, M Stern, D Grindlay, JE Alexander, DM Aramaki, T Baganoff, FK Barret, D Barriere, N Boggs, SE Canipe, AM Christensen, FE Craig, WW Desai, MA Forster, K Giommi, P Grefenstette, BW Harrison, FA Hong, D Hornstrup, A Kitaguchi, T Koglin, JE Madsen, KK Mao, PH Miyasaka, H Perri, M Pivovaroff, MJ Puccetti, S Rana, V Westergaard, NJ Zhang, WW Zoglauer, A AF Hong, JaeSub Mori, Kaya Hailey, Charles J. Nynka, Melania Zhang, Shuo Gotthelf, Eric Fornasini, Francesca M. Krivonos, Roman Bauer, Franz Perez, Kerstin Tomsick, John A. Bodaghee, Arash Chiu, Jeng-Lun Clavel, Maica Stern, Daniel Grindlay, Jonathan E. Alexander, David M. Aramaki, Tsuguo Baganoff, Frederick K. Barret, Didier Barriere, Nicolas Boggs, Steven E. Canipe, Alicia M. Christensen, Finn E. Craig, William W. Desai, Meera A. Forster, Karl Giommi, Paolo Grefenstette, Brian W. Harrison, Fiona A. Hong, Dooran Hornstrup, Allan Kitaguchi, Takao Koglin, Jason E. Madsen, Kristen K. Mao, Peter H. Miyasaka, Hiromasa Perri, Matteo Pivovaroff, Michael J. Puccetti, Simonetta Rana, Vikram Westergaard, Niels J. Zhang, William W. Zoglauer, Andreas TI NuSTAR HARD X-RAY SURVEY OF THE GALACTIC CENTER REGION. II. X-RAY POINT SOURCES SO ASTROPHYSICAL JOURNAL LA English DT Article DE Galaxy: center; X-rays: binaries; X-rays: diffuse background; X-rays: general ID MAGNETIC CATACLYSMIC VARIABLES; SUPERNOVA-REMNANT SAGITTARIUS; XMM-NEWTON OBSERVATIONS; BURSTING PULSAR; CHANDRA CATALOG; LIMITING WINDOW; GRS 1741.9-2853; NUMBER COUNTS; V404 CYGNI; A-ASTERISK AB We present the first survey results of hard X-ray point sources in the Galactic Center (GC) region by NuSTAR. We have discovered 70 hard (3-79 keV) X-ray point sources in a 0.6 deg(2) region around Sgr A* with a total exposure of 1.7 Ms, and 7 sources in the Sgr B2 field with 300 ks. We identify clear Chandra counterparts for 58 NuSTAR sources and assign candidate counterparts for the remaining 19. The NuSTAR survey reaches X-ray luminosities of similar to 4x and similar to 8 x 10(32) erg s(-1) at the GC (8 kpc) in the 3-10 and 10-40 keV bands, respectively. The source list includes three persistent luminous X-ray binaries (XBs) and the likely run-away pulsar called the Cannonball. New source-detection significance maps reveal a cluster of hard (>10 keV) X-ray sources near the Sgr. A diffuse complex with no clear soft X-ray counterparts. The severe extinction observed in the Chandra spectra indicates that all the NuSTAR sources are in the central bulge or are of extragalactic origin. Spectral analysis of relatively bright NuSTAR sources suggests that magnetic cataclysmic variables constitute a large fraction (>40%-60%). Both spectral analysis and logN-logS distributions of the NuSTAR sources indicate that the X-ray spectra of the NuSTAR sources should have kT > 20 keV on average for a single temperature thermal plasma model or an average photon index of Gamma = 1.5-2 for a power-law model. These findings suggest that the GC X-ray source population may contain a larger fraction of XBs with high plasma temperatures than the field population. C1 [Hong, JaeSub; Grindlay, Jonathan E.] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. [Mori, Kaya; Hailey, Charles J.; Nynka, Melania; Zhang, Shuo; Gotthelf, Eric; Canipe, Alicia M.; Desai, Meera A.; Hong, Dooran] Columbia Univ, Columbia Astrophys Lab, New York, NY 10027 USA. [Gotthelf, Eric] Univ Barcelona, Dept Fis Quant & Astrofis, Inst Ciencies Cosmos, IEEC UB, Marti & Franques 1, Barcelona 08028, Spain. [Fornasini, Francesca M.] Univ Calif Berkeley, Dept Astron, Berkeley, CA 94720 USA. [Krivonos, Roman] Russian Acad Sci, Space Res Inst, Profsoyuznaya 84-32, Moscow 117997, Russia. [Bauer, Franz] Pontificia Univ Catolica Chile, Fac Fis, Inst Astrofis, Santiago 22, Chile. [Bauer, Franz] Millennium Inst Astrophys, Santiago, Chile. [Bauer, Franz] Space Sci Inst, 4750 Walnut St,Suite 205, Boulder, CO 80301 USA. [Perez, Kerstin] Haverford Coll, 370 Lancaster Ave,KINSC L109, Haverford, PA 19041 USA. [Tomsick, John A.; Chiu, Jeng-Lun; Clavel, Maica; Barriere, Nicolas; Boggs, Steven E.; Craig, William W.; Zoglauer, Andreas] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Bodaghee, Arash] Georgia Coll, 231 W Hancock St, Milledgeville, GA 31061 USA. [Stern, Daniel] CALTECH, Jet Prop Lab, Pasadena, CA 91109 USA. [Alexander, David M.] Univ Durham, Dept Phys, Durham DH1 3LE, England. [Aramaki, Tsuguo] Standford Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Baganoff, Frederick K.] MIT, Kavli Inst Astrophys & Space Res, Cambridge, MA 02139 USA. [Barret, Didier; Christensen, Finn E.] Univ Toulouse, UPS OMP, IRAP, Toulouse, France. [Barret, Didier] Inst Rech Astrophys & Planetol, CNRS, 9Av Colonel Roche,BP 44346, F-31028 Toulouse 4, France. [Craig, William W.; Pivovaroff, Michael J.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Forster, Karl; Grefenstette, Brian W.; Harrison, Fiona A.; Madsen, Kristen K.; Mao, Peter H.; Miyasaka, Hiromasa; Rana, Vikram] CALTECH, Cahill Ctr Astron & Astrophys, Pasadena, CA 91125 USA. [Giommi, Paolo; Perri, Matteo; Puccetti, Simonetta] ASI Sci Data Ctr, Via Politecn Snc, I-00133 Rome, Italy. [Hornstrup, Allan; Westergaard, Niels J.] Tech Univ Denmark, DTU Space Natl Space Inst, Elektrovej 327, DK-2800 Lyngby, Denmark. [Kitaguchi, Takao] Hiroshima Univ, Dept Phys Sci, Higashihiroshima, Hiroshima 7398526, Japan. [Kitaguchi, Takao] Hiroshima Univ, Core Res Energet Universe, Higashihiroshima, Hiroshima 7398526, Japan. [Koglin, Jason E.] Kavli Inst Particle Astrophys & Cosmol, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Perri, Matteo; Puccetti, Simonetta] INAF Astron Roma, Via Frascati 33, I-00040 Monte Porzio Catone, Italy. [Zhang, William W.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. RP Hong, J (reprint author), Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. EM jaesub@head.cfa.harvard.edu OI Clavel, Maica/0000-0003-0724-2742; Krivonos, Roman/0000-0003-2737-5673 FU NASA [NASA Contract No. NNG08FD60C]; National Aeronautics and Space Administration; NASA/APRA grant [NNX14AD59G]; Russian Science Foundation [14-22-00271]; CONICYT-Chile (Basal-CATA) [PFB-06/2007]; CONICYT-Chile (FONDECYT) [1141218]; CONICYT-Chile ("EMBIGGEN" Anillo) [ACT1101]; Ministry of Economy, Development, and Tourism's Millennium Science Initiative [IC120009]; NASA Headquarters under the NASA Earth and Space Science Fellowship Program-Grant [NNX13AM31]; French Space Agency (CNES) FX This work was supported under NASA Contract No. NNG08FD60C, and made use of data from the NuSTAR mission, a project led by the California Institute of Technology, managed by the Jet Propulsion Laboratory, and funded by the National Aeronautics and Space Administration. We thank the NuSTAR Operations, Software and Calibration teams for support with the execution and analysis of these observations. We thank G. Ponti for careful reading and suggestions of the manuscript. This research has made use of the NuSTAR Data Analysis Software (NuSTARDAS) jointly developed by the ASI Science Data Center (ASDC, Italy) and the California Institute of Technology (USA). J. Hong acknowledges support from NASA/APRA grant NNX14AD59G. R. Krivonos acknowledges support from Russian Science Foundation through grant 14-22-00271. F.E. Bauer acknowledges support from CONICYT-Chile (Basal-CATA PFB-06/2007, FONDECYT 1141218, "EMBIGGEN" Anillo ACT1101), and the Ministry of Economy, Development, and Tourism's Millennium Science Initiative through grant IC120009, awarded to The Millennium Institute of Astrophysics, MAS. S. Zhang is supported by NASA Headquarters under the NASA Earth and Space Science Fellowship Program-Grant NNX13AM31. D. Barret acknowledges support from the French Space Agency (CNES). NR 89 TC 3 Z9 3 U1 0 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 10 PY 2016 VL 825 IS 2 AR 132 DI 10.3847/0004-637X/825/2/132 PG 31 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DU1BM UT WOS:000381940800050 ER PT J AU Gnedin, NY AF Gnedin, Nickolay Y. TI COSMIC REIONIZATION ON COMPUTERS: THE FAINT END OF THE GALAXY LUMINOSITY FUNCTION SO ASTROPHYSICAL JOURNAL LETTERS LA English DT Article DE cosmology: theory; galaxies: formation; intergalactic medium; large-scale structure of universe; methods: numerical ID SIMILAR-TO 8; STAR-FORMING GALAXIES; DEEP FIELD CAMPAIGN; BRIGHT END; RADIATIVE-TRANSFER; CONSTRAINTS AB Using numerical cosmological simulations completed under the "Cosmic Reionization On Computers" project, I explore theoretical predictions for the faint end of the galaxy UV luminosity functions at z greater than or similar to 6. A commonly used Schechter function approximation with the magnitude cut at M-cut similar to -13 provides a reasonable fit to the actual luminosity function of simulated galaxies. When the Schechter functional form is forced on the luminosity functions from the simulations, the magnitude cut Mcut is found to vary between -12 and -14 with a mild redshift dependence. An analytical model of reionization from Madau et al., as used by Robertson et al., provides a good description of the simulated results, which can be improved even further by adding two physically motivated modifications to the original Madau et al. equation. C1 [Gnedin, Nickolay Y.] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. [Gnedin, Nickolay Y.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Gnedin, Nickolay Y.] Univ Chicago, Dept Astron & Astrophys, 5640 S Ellis Ave, Chicago, IL 60637 USA. RP Gnedin, NY (reprint author), Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA.; Gnedin, NY (reprint author), Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA.; Gnedin, NY (reprint author), Univ Chicago, Dept Astron & Astrophys, 5640 S Ellis Ave, Chicago, IL 60637 USA. EM gnedin@fnal.gov FU United States Department of Energy [DE-AC02-07CH11359]; NSF [AST-1211190]; Munich Institute for Astro- and Particle Physics (MIAPP) of the DFG cluster of excellence "Origin and Structure of the universe"; DOE Office of Science User Facility [DE-AC02-06CH11357] FX Fermilab is operated by Fermi Research Alliance, LLC, under Contract No. DE-AC02-07CH11359 with the United States Department of Energy. This work was also supported in part by the NSF grant AST-1211190 and by the Munich Institute for Astro- and Particle Physics (MIAPP) of the DFG cluster of excellence "Origin and Structure of the universe." CROC simulations have been performed on the University of Chicago Research Computing Center cluster "Midway," on National Energy Research Supercomputing Center (NERSC) supercomputers "Cori" and "Edison," and on the Argonne Leadership Computing Facility supercomputer "Mira." An award of computer time was provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program. This research used resources of the Argonne Leadership Computing Facility, which is a DOE Office of Science User Facility supported under Contract DE-AC02-06CH11357. NR 26 TC 3 Z9 3 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2041-8205 EI 2041-8213 J9 ASTROPHYS J LETT JI Astrophys. J. Lett. PD JUL 10 PY 2016 VL 825 IS 2 AR L17 DI 10.3847/2041-8205/825/2/L17 PG 5 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DS4GG UT WOS:000380738800001 ER PT J AU Moorthy, KK Satheesh, SK Kotamarthi, VR AF Moorthy, K. Krishna Satheesh, S. K. Kotamarthi, V. R. TI Evolution of aerosol research in India and the RAWEX-GVAX: an overview SO CURRENT SCIENCE LA English DT Article DE Aerosols; climate change; ICARB; RAWEX-GVAX ID TROPICAL COASTAL STATION; GANGETIC-HIMALAYAN REGION; ASIAN SUMMER MONSOON; IN-SITU MEASUREMENTS; MASS ABSORPTION EFFICIENCY; SINGLE SCATTERING ALBEDO; RADIATION BUDGET ICARB; BLACK CARBON AEROSOLS; LONG-RANGE TRANSPORT; CHEMICAL-COMPOSITION AB Climate change has great significance in Asia in general, and India in particular; and atmospheric aerosols have a decisive role in this. The climate forcing potential of aerosols is closely linked to their optical, microphysical and chemical properties. Systematic efforts to characterize these properties over the Indian region started about 5 decades ago, and evolved over the years through concerted efforts in the form of long-term scientific programmes as well as concerted fields experiments. All these have resulted in this activity becoming one of the most vibrant fields of climate research in India and have brought several important issues in the national and international foci. The field experiment, RAWEX-GVAX (Regional Aerosol Warming Experiment-Ganges Valley Aerosol Experiment), conducted during 2011-12 jointly by the US Department of Energy, Indian Space Research Organization and Department of Science and Technology, has emerged as a direct outcome of the above efforts. This overview provides a comprehensive account of the development of aerosol-climate research in India and south Asia, and the accomplishment and newer issues that warranted the above field campaign. Details of RAWEX-GVAX, the major outcomes and the subsequent and more recent efforts are presented, followed by the way forward in this field for the next several years to come. C1 [Moorthy, K. Krishna; Satheesh, S. K.] Indian Inst Sci, Ctr Atmospher & Ocean Sci, Bengaluru 560012, India. [Moorthy, K. Krishna] Indian Space Res Org, Bengaluru 560231, India. [Satheesh, S. K.] Indian Inst Sci, Divecha Ctr Climate Change, Bengaluru 560012, India. [Kotamarthi, V. R.] Argonne Natl Lab, Div Environm Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Moorthy, KK (reprint author), Indian Inst Sci, Ctr Atmospher & Ocean Sci, Bengaluru 560012, India.; Moorthy, KK (reprint author), Indian Space Res Org, Bengaluru 560231, India. EM krishnamoorthy@caos.iisc.ernet.in NR 154 TC 0 Z9 0 U1 8 U2 12 PU INDIAN ACAD SCIENCES PI BANGALORE PA C V RAMAN AVENUE, SADASHIVANAGAR, P B #8005, BANGALORE 560 080, INDIA SN 0011-3891 J9 CURR SCI INDIA JI Curr. Sci. PD JUL 10 PY 2016 VL 111 IS 1 BP 53 EP 75 DI 10.18520/cs/v111/i1/53-75 PG 23 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR0TF UT WOS:000379619100028 ER PT J AU Feng, Y Cadeddu, M Kotamarthi, VR Renju, R Raju, CS AF Feng, Yan Cadeddu, M. Kotamarthi, V. R. Renju, R. Raju, C. Suresh TI Humidity bias and effect on simulated aerosol optical properties during the Ganges Valley Experiment SO CURRENT SCIENCE LA English DT Article DE Aerosol optical depth and extinction; relative humidity; regional climate model ID SOLAR ABSORPTION; INDIAN REGION; GOCART MODEL; WRF-CHEM; DUST; ASIA; PARAMETERIZATION; DISTRIBUTIONS; VARIABILITY; SATELLITE AB The radiosonde humidity profiles available during the Ganges Valley Experiment were compared to those simulated from the regional Weather Research and Forecasting (WRF) model coupled with a chemistry module (WRF-Chem) and the global reanalysis datasets. Large biases were revealed. On a monthly mean basis at Nainital, located in northern India, the WRF-Chem model simulates a large moist bias in the free troposphere (up to +20%) as well as a large dry bias in the boundary layer (up to -30%). While the overall pattern of the biases is similar, the magnitude of the biases varies from time to time and from one location to another. At Thiruvananthapuram, the magnitude of the dry bias is smaller, and in contrast to Nainital, the higher-resolution regional WRF-Chem model generates larger moist biases in the upper troposphere than the global reanalysis data. Furthermore, the humidity biases in the upper troposphere, while significant, have little impact on the model estimation of column aerosol optical depth (AOD). The frequent occurrences of the dry boundary-layer bias simulated by the large-scale models tend to lead to the underestimation of AOD. It is thus important to quantify the humidity vertical profiles for aerosol simulations over South Asia. C1 [Feng, Yan; Cadeddu, M.; Kotamarthi, V. R.] Argonne Natl Lab, Div Environm Sci, Argonne, IL 60439 USA. [Renju, R.; Raju, C. Suresh] Vikram Sarabhai Space Ctr, Space Phys Lab, Thiruvananthapuram 695022, Kerala, India. RP Feng, Y (reprint author), Argonne Natl Lab, Div Environm Sci, Argonne, IL 60439 USA. EM yfeng@anl.gov FU US Department of Energy (DOE); Argonne National Laboratory under US DOE [DE-AC02-06CH11357] FX This work was supported by the US Department of Energy (DOE) as part of the Atmospheric System Research Program. Support for this research was provided to Y.F., V.R.K. and M.C. by Argonne National Laboratory under US DOE contract DE-AC02-06CH11357. All the numerical simulations were performed using the computing cluster (Fusion) operated by Argonne's Laboratory Computing Resource Center. R.R. and C.S.R. acknowledge Dr K. Krishnamoorthy and Dr S.K. Satheesh for GVAX data as well as scientific discussions. NR 36 TC 0 Z9 0 U1 6 U2 7 PU INDIAN ACAD SCIENCES PI BANGALORE PA C V RAMAN AVENUE, SADASHIVANAGAR, P B #8005, BANGALORE 560 080, INDIA SN 0011-3891 J9 CURR SCI INDIA JI Curr. Sci. PD JUL 10 PY 2016 VL 111 IS 1 BP 93 EP 100 DI 10.18520/cs/v111/i1/93-100 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR0TF UT WOS:000379619100031 ER PT J AU Phanikumar, DV Shukla, KK Naja, M Singh, N Sahai, S Sagar, R Satheesh, SK Moorthy, KK Kotamarthi, VR Newsom, RK AF Phanikumar, D. V. Shukla, K. K. Naja, M. Singh, N. Sahai, S. Sagar, R. Satheesh, S. K. Moorthy, K. K. Kotamarthi, V. R. Newsom, Rob K. TI Doppler Lidar observations over a high altitude mountainous site Manora Peak in the central Himalayan region SO CURRENT SCIENCE LA English DT Article DE Boundary layer; Doppler Lidar; GVAX ID BACKSCATTER HETERODYNE LIDAR; BOUNDARY-LAYER; ACCUMULATION; PERFORMANCE; CASES-99; AEROSOL; OZONE AB The RAWEX-GVAX field campaign has been carried out from June 2011 to March 2012 over a high altitude site Manora Peak, Nainital (29.4 degrees N; 79.2 degrees E; 1958 m amsl) in the central Himalayas to assess the impacts of absorbing aerosols on atmospheric thermodynamics and clouds. This paper presents the preliminary results of the observations and data analysis of the Doppler Lidar, installed at Nainital. Strong updrafts with vertical winds in the range of similar to 2-4 ms(-1) occurred during the daytime and throughout the season indicating thermally driven convection. On the other hand during nighttime, weak downdrafts persisted during stable conditions. Plan Position Indicator scan of Doppler Lidar showed north-northwesterly winds in the boundary layer. The mixing layer height, derived from the vertical velocity variance, showed diurnal variations, in the range similar to 0.7-1 km above ground level during daytime and very shallow during nighttime. C1 [Phanikumar, D. V.; Shukla, K. K.; Naja, M.; Singh, N.; Sagar, R.] Aryabhatta Res Inst Observat Sci, Naini Tal 263002, India. [Shukla, K. K.] Pt Ravishankar Shukla Univ, Raipur 492010, Madhya Pradesh, India. [Sahai, S.] Amity Univ, Noida 201303, India. [Satheesh, S. K.; Moorthy, K. K.] Indian Inst Sci, Ctr Atmospher & Ocean Sci, Bengaluru 560012, India. [Satheesh, S. K.] Indian Inst Sci, Divecha Ctr Climate Change, Bengaluru 560012, India. [Kotamarthi, V. R.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Newsom, Rob K.] Pacific Northwest Natl Lab, Richland, WA USA. RP Phanikumar, DV (reprint author), Aryabhatta Res Inst Observat Sci, Naini Tal 263002, India. EM phani@aries.res.in NR 27 TC 0 Z9 0 U1 2 U2 4 PU INDIAN ACAD SCIENCES PI BANGALORE PA C V RAMAN AVENUE, SADASHIVANAGAR, P B #8005, BANGALORE 560 080, INDIA SN 0011-3891 J9 CURR SCI INDIA JI Curr. Sci. PD JUL 10 PY 2016 VL 111 IS 1 BP 101 EP 108 DI 10.18520/cs/v111/i1/101-108 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR0TF UT WOS:000379619100032 ER PT J AU Singh, N Solanki, R Ojha, N Naja, M Dumka, UC Phanikumar, DV Sagar, R Satheesh, SK Moorthy, KK Kotamarthi, VR Dhaka, SK AF Singh, Narendra Solanki, Raman Ojha, N. Naja, M. Dumka, U. C. Phanikumar, D. V. Sagar, Ram Satheesh, S. K. Moorthy, K. Krishna Kotamarthi, V. R. Dhaka, S. K. TI Variations in the cloud-base height over the central Himalayas during GVAX: association with the monsoon rainfall SO CURRENT SCIENCE LA English DT Article DE Ceilometer; central Himalaya; cloud-base; GVAX; monsoon ID VERTICAL-DISTRIBUTION; BOUNDARY-LAYER; MIXING HEIGHT; VARIABILITY; AEROSOL; REGION; CEILOMETER; TROPOSPHERE; ENVIRONMENT; ABSORPTION AB We present the measurements of cloud-base height variations over Aryabhatta Research Institute of Observational Science, Nainital (79.45 degrees E, 29.37 degrees N, 1958 m amsl) obtained from Vaisala Ceilometer, during the nearly year-long Ganges Valley Aerosol Experiment (GVAX). The cloud-base measurements are analysed in conjunction with collocated measurements of rainfall, to study the possible contributions from different cloud types to the observed monsoonal rainfall during June to September 2011. The summer monsoon of 2011 was a normal monsoon year with total accumulated rainfall of 1035.8 mm during June-September with a maximum during July (367.0 mm) and minimum during September (222.3 mm). The annual mean monsoon rainfall over Nainital is 1440 +/- 430 mm. The total rainfall measured during other months (October 2011-March 2012) was only 9% of that observed during the summer monsoon. The first cloud-base height varied from about 31 m above ground level (AGL) to a maximum of 7.6 km AGL during the summer monsoon period of 2011. It is found that about 70% of the total rain is observed only when the first cloud-base height varies between surface and 2 km AGL, indicating that most of the rainfall at high altitude stations such as Nainital is associated with stratiform low-level clouds. However, about 25% of the total rainfall is being contributed by clouds between 2 and 6 km. The occurrences of high-altitude cumulus clouds are observed to be only 2-4%. This study is an attempt to fill a major gap of measurements over the topographically complex and observationally sparse northern Indian region providing the evaluation data for atmospheric models and therefore, have implications towards the better predictions of monsoon rainfall and the weather components over this region. C1 [Singh, Narendra; Solanki, Raman; Naja, M.; Dumka, U. C.; Phanikumar, D. V.; Sagar, Ram] Aryabhatta Res Inst Observat Sci, Naini Tal 263002, India. [Ojha, N.] Max Planck Inst Chem, Dept Atmospher Chem, Mainz, Germany. [Satheesh, S. K.] Indian Inst Sci, Ctr Atmospher & Ocean Sci, Bengaluru 560012, India. [Satheesh, S. K.] Indian Inst Sci, Divecha Ctr Climate Change, Bengaluru 560012, India. [Moorthy, K. Krishna] ISRO Head Quarters, Bengaluru 560231, India. [Kotamarthi, V. R.] Argonne Natl Lab, Div Environm Sci, Argonne, IL 60439 USA. [Dhaka, S. K.] Univ Delhi, Rajdhani Coll, Radio & Atmospher Phys Lab, Delhi 110015, India. [Solanki, Raman] Univ Delhi, Dept Phys & Astrophys, New Delhi 110021, India. RP Singh, N (reprint author), Aryabhatta Res Inst Observat Sci, Naini Tal 263002, India. EM narendra@aries.res.in NR 38 TC 2 Z9 2 U1 2 U2 6 PU INDIAN ACAD SCIENCES PI BANGALORE PA C V RAMAN AVENUE, SADASHIVANAGAR, P B #8005, BANGALORE 560 080, INDIA SN 0011-3891 J9 CURR SCI INDIA JI Curr. Sci. PD JUL 10 PY 2016 VL 111 IS 1 BP 109 EP 116 DI 10.18520/cs/v111/i1/109-116 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR0TF UT WOS:000379619100033 ER PT J AU Naja, M Bhardwaj, P Singh, N Kumar, P Kumar, R Ojha, N Sagar, R Satheesh, SK Moorthy, KK Kotamarthi, VR AF Naja, Manish Bhardwaj, Piyush Singh, Narendra Kumar, Phani Kumar, Rajesh Ojha, N. Sagar, Ram Satheesh, S. K. Moorthy, K. Krishna Kotamarthi, V. R. TI High-frequency vertical profiling of meteorological parameters using AMF1 facility during RAWEX-GVAX at ARIES, Nainital SO CURRENT SCIENCE LA English DT Article DE Aerosols; radiosonde; subtropical jet; tropopause folding; vertical profiling ID CENTRAL HIMALAYAS; OZONE; STRATOSPHERE; TROPOSPHERE; TRANSPORT; CHEMISTRY; INDIA; SITE AB An extensive field study, RAWEX-GVAX, was carried out during a 10-month (June 2011-March 2012) campaign at ARIES, Nainital and observations on a wide range of parameters like physical and optical properties of aerosols, meteorological parameters and boundary layer evolution were made. This work presents results obtained from high-frequency (four launches per day), balloon-borne observations of meteorological parameters (pressure, temperature, relative humidity, wind speed and wind direction). These observations show wind speed as high as 84 m/s near the subtropical jet. It is shown that reanalysis wind speeds are in better agreement at 250 hPa (altitude of subtropical jet) than those above or below this value (100 hPa or 500 hPa). These observations also demonstrate that AIRS-derived temperature profiles are negatively biased in the lower altitude region, whereas they are positively biased near the tropopause. WRF simulated results are able to capture variations in temperature, humidity and wind speed profile reasonable well. WRF and AIRS-derived tropopause height, tropopause pressure and tropopause temperature also show agreement with radiosonde estimates. C1 [Naja, Manish; Bhardwaj, Piyush; Singh, Narendra; Kumar, Phani; Ojha, N.] Aryabhatta Res Inst Observat Sci, Naini Tal 263002, India. [Kumar, Rajesh] Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA. [Sagar, Ram] Indian Inst Astrophys, Bengaluru 560034, India. [Satheesh, S. K.] Indian Inst Sci, Ctr Atmospher & Ocean Sci, Bengaluru 560012, India. [Satheesh, S. K.] Indian Inst Sci, Divecha Ctr Climate Change, Bengaluru 560012, India. [Moorthy, K. Krishna] Indian Space Res Org, Bengaluru 560231, India. [Kotamarthi, V. R.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Naja, M (reprint author), Aryabhatta Res Inst Observat Sci, Naini Tal 263002, India. EM manish@aries.res.in FU NASI FX RAWEX-GVAX field campaign was jointly organized by ISRO, IISc, ARIES and DOE. We are grateful to the air traffic control for help in coordinating the balloon launches, four times in a day. We also thank project trainees for their help with balloon launches, particularly at 2330 and 0530 IST from ARIES. Support from NASI is highly acknowledged by R.S. NR 13 TC 1 Z9 1 U1 2 U2 5 PU INDIAN ACAD SCIENCES PI BANGALORE PA C V RAMAN AVENUE, SADASHIVANAGAR, P B #8005, BANGALORE 560 080, INDIA SN 0011-3891 J9 CURR SCI INDIA JI Curr. Sci. PD JUL 10 PY 2016 VL 111 IS 1 BP 132 EP 140 DI 10.18520/cs/v111/i1/132-140 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR0TF UT WOS:000379619100035 ER PT J AU Quarterman, J Skerker, JM Feng, XY Liu, IY Zhao, HM Arkin, AP Jin, YS AF Quarterman, Josh Skerker, Jeffrey M. Feng, Xueyang Liu, Ian Y. Zhao, Huimin Arkin, Adam P. Jin, Yong-Su TI Rapid and efficient galactose fermentation by engineered Saccharomyces cerevisiae SO JOURNAL OF BIOTECHNOLOGY LA English DT Article DE Galactose; Saccharomyces cerevisiae; Ethanol; Evolutionary engineering; Systems biology; Genome sequencing ID YEAST MUTANTS; XYLOSE METABOLISM; LELOIR PATHWAY; FLUX ANALYSIS; GLUCOSE; GENE; RESPIRATION; CARBON; METABOLOMICS; CHEMICALS AB the important industrial yeast Saccharomyces cerevisiae, galactose metabolism requires energy production by respiration; therefore, this yeast cannot metabolize galactose under strict anaerobic conditions. While the respiratory dependence of galactose metabolism provides benefits in terms of cell growth and population stability, it is not advantageous for producing fuels and chemicals since a substantial fraction of consumed galactose is converted to carbon dioxide. In order to force S. cerevisiae to use galactose without respiration, a subunit (COX9) of a respiratory enzyme was deleted, but the resulting deletion mutant (Delta cox9) was impaired in terms of galactose assimilation. Interestingly, after serial sub-cultures on galactose, the mutant evolved rapidly and was able to use galactose via fermentation only. The evolved strain (JQ-G1) produced ethanol from galactose with a 94% increase in yield and 6.9-fold improvement in specific productivity as compared to the wild-type strain. C-13-metabolic flux analysis demonstrated a three-fold reduction in carbon flux through the TCA cycle of the evolved mutant with redirection of flux toward the fermentation pathway. Genome sequencing of the JQ-G1 strain revealed a loss of function mutation in a master negative regulator of the Leloir pathway (Gal80p). The mutation ( Glu348*) in Ga180p was found to act synergistically with deletion of COX9 for efficient galactose fermentation, and thus the double deletion mutant Delta cox9 Delta gal80 produced ethanol 2.4 times faster and with 35% higher yield than a single knockout mutant with deletion of GAL80 alone. When we introduced a functional COX9 cassette back into the JQ-G1 strain, the JQ-G1-COX9 strain showed a 33% reduction in specific galactose uptake rate and a 49% reduction in specific ethanol production rate as compared to JQ-G1. The wild-type strain was also subjected to serial sub-cultures on galactose but we failed to isolate a mutant capable of utilizing galactose without respiration. We concluded that the metabolic "death valley" (i.e. no galactose utilization by the Delta cox9 mutant) is a necessary intermediate phenotype to facilitate galactose utilization without respiration in yeast. The results in this study demonstrate a promising approach for directing adaptive evolution toward fermentative metabolism and for generating evolved yeast strains with improved phenotypes under anaerobic conditions. (c) 2016 Elsevier B.V. All rights reserved. C1 [Quarterman, Josh; Jin, Yong-Su] Univ Illinois, Dept Food Sci & Human Nutr, Urbana, IL 61801 USA. [Quarterman, Josh; Jin, Yong-Su] Univ Illinois, Inst Genom Biol, Urbana, IL 61801 USA. [Skerker, Jeffrey M.; Arkin, Adam P.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Skerker, Jeffrey M.; Arkin, Adam P.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Feng, Xueyang] Virginia Polytech Inst & State Univ, Dept Biol Syst Engn, Blacksburg, VA 24060 USA. [Liu, Ian Y.] Univ Minnesota, Dept Chem Engn, Minneapolis, MN 55455 USA. [Zhao, Huimin] Univ Illinois, Dept Chem & Biomol Engn, Urbana, IL 61801 USA. RP Jin, YS (reprint author), Inst Genom Biol, 1206 W Gregory Dr, Urbana, IL 61801 USA. EM ysjin@illinois.edu OI Arkin, Adam/0000-0002-4999-2931; Feng, Xueyang/0000-0003-4426-5732 FU Energy Biosciences Institute FX This work was supported by funding from the Energy Biosciences Institute. NR 41 TC 0 Z9 0 U1 12 U2 41 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0168-1656 EI 1873-4863 J9 J BIOTECHNOL JI J. Biotechnol. PD JUL 10 PY 2016 VL 229 BP 13 EP 21 DI 10.1016/j.jbiotec.2016.04.041 PG 9 WC Biotechnology & Applied Microbiology SC Biotechnology & Applied Microbiology GA DO7RR UT WOS:000377980900003 PM 27140870 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R Abolins, M AbouZeid, OS Abraham, NL Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedra, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aring;kesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araquea, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arik, M Armbruster, AJ Armitage, LJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Aring;sman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Navarro, LB Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, HP Bechtle, P Beck, P Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bedognetti, M Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, AS Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Belyaev, NL Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Benitez, J Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Berlendis, S Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertram, IA Bertsche, C Bertsche, D Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, J Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bielski, R Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Boerner, D Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Bortfeldt, J Bortoletto, D Bortolotto, V Bos, K Boscherini, D Bosman, M Sola, JDB Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Boutle, SK Boveia, A Boyd, J Boyko, IR Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E HBroughton, J de Renstrom, PAB Bruncko, D Bruneliere, R 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CA ATLAS Collaboration TI Charged-particle distributions in root s=13 TeV pp interactions measured with the ATLAS detector at the LHC SO PHYSICS LETTERS B LA English DT Article ID PARTON DISTRIBUTIONS AB Charged-particle distributions are measured in proton-proton collisions at a centre-of-mass energy of 13 TeV, using a data sample of nearly 9 million events, corresponding to an integrated luminosity of 170 mu b(-1), recorded by the ATLAS detector during a special Large Hadron Collider fill. The charged-particle multiplicity, its dependence on transverse momentum and pseudorapidity and the dependence of the mean transverse momentum on the charged-particle multiplicity are presented. The measurements are performed with charged particles with transverse momentum greater than 500 MeV and absolute pseudorapidity less than 2.5, in events with at least one charged particle satisfying these kinematic requirements. Additional measurements in a reduced phase space with absolute pseudorapidity less than 0.8 are also presented, in order to compare with other experiments. The results are corrected for detector effects, presented as particle-level distributions and are compared to the predictions of various Monte Carlo event generators. (C) 2016 CERN for the benefit of the ATLAS Collaboration. Published by Elsevier B.V. C1 [Jackson, P.; Lee, L.; Petridis, A.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. 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J.; Pilcher, J. E.; Saxon, J.; Shochet, M. J.; Stark, G. H.; Swiatlowski, M.; Vukotic, I.; Wu, M.] Univ Chicago, Enrico Fermi Inst, Chicago, IL 60637 USA. [Blunier, S.; Diaz, M. A.; Ochoa-Ricoux, J. P.] Pontificia Univ Catolica Chile, Fac Fis, Casilla 6177, Santiago 22, Chile. [Brooks, W. K.; Carquin, E.; Kuleshov, S.; Pezoa, R.; Prokoshin, F.; Salazar Loyola, J. E.; Tapia Araya, S.; White, R.] Univ Tecn Feder Santa Maria, Dept Fis, Valparaiso, Chile. [Bai, Y.; da Costa, J. Barreiro Guimaraes; Cheng, H. J.; Fang, Y.; Jin, S.; Li, Q.; Lou, X.; Ouyang, Q.; Peng, C.; Ren, H.; Shan, L. Y.; Sun, X.; Xu, D.; Zhu, H.; Zhuang, X.] Chinese Acad Sci, Inst High Energy Phys, Beijing, Peoples R China. [Gao, J.; Geng, C.; Guo, Y.; Han, L.; Hu, Q.; Jiang, Y.; Li, B.; Liu, J. B.; Liu, M.; Liu, Y. L.; Liu, Y.; Peng, H.; Zhang, R.; Zhao, Z.; Zhu, Y.] Univ Sci & Technol China, Dept Modern Phys, Hefei, Anhui, Peoples R China. [Chen, S.; Zhang, H.] Nanjing Univ, Dept Phys, Nanjing, Jiangsu, Peoples R China. [Du, Y.; Feng, C.; Liu, B.; Ma, L. L.; Ma, Y.; Wang, C.; Zaidan, R.; Zhang, X.; Zhao, Y.; Zhu, C. G.] Shandong Univ, Sch Phys, Jinan, Shandong, Peoples R China. [Bret, M. Cano; Guo, J.; Li, L.; Yang, H.] Shanghai Jiao Tong Univ, Shanghai Key Lab Particle Phys & Cosmol, Dept Phys & Astron, Shanghai 200030, Peoples R China. [Chen, X.; Zhou, N.] Tsinghua Univ, Dept Phys, Beijing 100084, Peoples R China. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Clermont Univ, Lab Phys Corpusculaire, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Univ Clermont Ferrand, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Chomont, A. R.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Clark, M. R.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. C.; Pingel, A.; Wiglesworth, C.; Xella, S.] Univ Copenhagen, Niels Bohr Inst, Copenhagen, Denmark. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] INFN, Grp Collegato Cosenza, Lab Nazl Frascati, Arcavacata Di Rende, Italy. [Cairo, V. M.; Capua, M.; Crosetti, G.; La Rotonda, L.; Mastroberardino, A.; Policicchio, A.; Salvatore, D.; Scarfone, V.; Schioppa, M.; Susinno, G.; Tassi, E.] Univ Calabria, Dipartimento Fis, I-87036 Arcavacata Di Rende, Italy. [Adamczyk, L.; Bold, T.; Dabrowski, W.; Dyndal, M.; Gach, G. P.; Grabowska-Bold, I.; Kisielewska, D.; Koperny, S.; Kowalski, T. Z.; Mindur, B.; Przybycien, M.; Zemla, A.] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. [Palka, M.; Richter-Was, E.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Krakow, Poland. [Banas, E.; de Renstrom, P. A. Bruckman; Burka, K.; Chwastowski, J. J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Kowalewska, A. B.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Asbah, N.; Behr, J. K.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Notkestr 85, Hamburg, Germany. [Asbah, N.; Behr, J. K.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.; Schorlemmer, A. L. S.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, D-01062 Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, Sch Phys & Astron, SUPA, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Ancu, L. S.; Bell, W. H.; De Mendizabal, J. Bilbao; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Guido, E.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; St Denis, R. D.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, Sch Phys & Astron, SUPA, Glasgow, Lanark, Scotland. [Agricola, J.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; shabalina, E.; Stolte, P.; Veatch, J.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Berlendis, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Radescu, V.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kretz, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, NT, Peoples R China. [Bortolotto, V.; Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofiev, K.] Hong Kong Univ Sci & Technol, Dept Phys, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Lyubushkin, V.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] High Energy Accelerator Res Org, KEK, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch, Kobe, Hyogo 657, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto 612, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka 812, Japan. [Alconada Verzini, M. J.; Aloisio, A.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, RA-1900 La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Aloisio, A.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.; Beattie, M. D.; Bertram, I. A.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Parker, A. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Aliev, M.; Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Aliev, M.; Bachas, K.; Gorini, E.; Longo, L.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; Cindro, V.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. [Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kanjir, L.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, J.; Bona, M.; Cerrito, L.; Fletcher, G.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjoernmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fysiska Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Llorente Merino, J.; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Huelsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schaefer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Webb, S.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Raine, J. A.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Wilk, F.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] Aix Marseille Univ, CPPM, Marseille, France. [Aad, G.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] CNRS IN2P3, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Moyse, E. J. W.; Pais, P.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Heelan, L.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Stradling, A. R.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic 3010, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Geng, C.; Goldfarb, S.; Guan, L.; Guo, Y.; Levin, D.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Lazzaroni, M.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Resconi, S.; Shojaii, S.; Stabile, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Via Celoria 16, I-20133 Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Lazzaroni, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J-F.; Azuelos, G.; Dallaire, F.; Gagnon, L. G.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] ITEP, Moscow, Russia. [Antonov, A.; Belotskiy, K.; Belyaev, N. L.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Valderanis, C.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; La Rosa, A.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Werner Heisenberg Inst, Max Planck Inst Phys, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Maskawa Inst, Grad Sch Sci & Kobayashi, Nagoya, Aichi 4648601, Japan. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen Nikhef, Inst Math Astrophys & Particle Phys, NL-6525 ED Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; Van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Aben, R.; Aloisio, A.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; van der Geer, R.; Van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Univ Amsterdam, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.] No Illinois Univ, Dept Phys, De Kalb, IL USA. [Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama 700, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Haley, J.; jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.; Terashi, K.] Palacky Univ, RCPTM, CR-77147 Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris Saclay, Univ Paris 11, CNRS IN2P3, LAL, Orsay, France. [Endo, M.; Hanagaki, K.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Serfon, C.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Fawcett, W. J.; Frost, J. A.; Gallas, E. J.; Giuli, F.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Nagai, K.; Nickerson, R. B.; Norjoharuddeen, N.; Petrov, M.; Pickering, M. A.; Tseng, J. C-L.; Viehhauser, G. H. A.; Vigani, L.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Via Palestro 3, I-27100 Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Miguens, J. Machado; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov, A.; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. M.; Solovyev, V.] BP Konstantinov Nucl Phys Inst, Kurchatov Inst, Natl Res Ctr, St Petersburg, Russia. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Ist Nazl Fis Nucl, I-56100 Pisa, Italy. [Annovi, A.; Bertolucci, F.; Biesuz, N. V.; Cavasinni, V.; Chiarelli, G.; Del Prete, T.; Dell'Orso, M.; Donati, S.; Giannetti, P.; Leone, S.; Roda, C.; Scuri, F.; Sotiropoulou, C. L.; Spalla, M.; Volpi, G.; White, S.] Univ Pisa, Dipartimento Fis E Fermi, Pisa, Italy. [Bianchi, R. M.; Boudreau, J.; Escobar, C.; Farina, C.; Hong, T. M.; Mueller, J.; Sapp, K.; Su, J.] Univ Pittsburgh, Dept Phys & Astron, Pittsburgh, PA 15260 USA. [Aguilar-Saavedra, J. A.; Dos Santos, S. P. Amor; Amorim, A.; Annovi, A.; Araquea, J. P.; Cantrill, R.; Carvalho, J.; Castro, N. F.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Fiolhais, M. C. N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Oleiro Seabra, L. F.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Tavares Delgado, A.; Veloso, F.; Wolters, H.] Lab Instrumentacao & Fis Expt Particulas LIP, Lisbon, Portugal. [Amorim, A.; Muino, P. Conde; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Miguens, J. Machado; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Tavares Delgado, A.] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Dos Santos, S. P. Amor; Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, P-1699 Lisbon, Portugal. [Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedra, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedra, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Fac Ciencias & Tecnol, Dept Fis, Caparica, Portugal. Univ Nova Lisboa, Fac Ciencias & Tecnol, CEFITEC, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nechansky, F.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, CR-16635 Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Slovak, R.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, Inst High Energy Phys Protvino, State Res Ctr, Moscow, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. J.; Wielers, M.] Rutherford Appleton Lab, Particle Phys Dept, Didcot OX11 0QX, Oxon, England. [Anulli, F.; Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; De Pedis, D.; De Salvo, A.; Di Domenico, A.; Di Donato, C.; Falciano, S.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Luminari, L.; Marzano, F.; Messina, A.; Nisati, A.; Pasqualucci, E.; Petrolo, E.; Pontecorvoa, L.; Rescigno, M.; Rosati, S.; Tehrani, F. Safai; Vanadia, M.; Vari, R.; Veneziano, S.; Verducci, M.; Zanello, L.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Bagiacchi, P.; Bagnaia, P.; Bauce, M.; Bini, C.; Ciapetti, G.; Corradi, M.; Di Domenico, A.; Di Donato, C.; Gentile, S.; Giagu, S.; Gustavino, G.; Kuna, M.; Lacava, F.; Luci, C.; Messina, A.; Vanadia, M.; Verducci, M.; Zanello, L.] Univ Roma La Sapienza, Dipartimento Fis, Piazzale Aldo Moro 5, I-00185 Rome, Italy. [Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Via E Carnevale, I-00173 Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziani, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, I-00146 Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. [El Kacimi, M.; Goujdami, D.] Univ Cadi Ayyad, LPHEA, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; Fassi, F.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Basye, A.; Bauer, F.; Besson, N.; Blanchard, J. -B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Giraud, P. F.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Hanna, R.; Hassani, S.; Jeanneau, F.; Kivernyk, O.; Kukla, R.; Lancon, E.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Meyer, J-P.; Nicolaidou, R.; Ouraou, A.; Perego, M. M.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schune, Ph.; Schwemling, Ph.; Schwindling, J.] CEA Saclay, Commissariat Energie Atom & Energies Alternat, Inst Rech Lois Fondament Univers, DSM IRFU, F-91191 Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.; Whallon, N. L.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, D-57068 Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC V5A 1S6, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice 04353, Slovakia. [Castaneda-Miranda, E.; Hamiltona, A.; Yacoob, S.] Univ Cape Town, Dept Phys, ZA-7925 Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Garciac, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Stockholm Univ, Dept Phys, S-10691 Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Cheplakov, A.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Sjolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Oskar Klein Ctr, Stockholm, Sweden. [Lund-Jensen, B.; Sidebo, P. E.; Strandberg, J.] Royal Inst Technol, Dept Phys, S-10044 Stockholm, Sweden. [Abraham, N. L.; Allbrooke, B. M. M.; Asquith, L.; Cerri, A.; Barajas, C. A. Chavez; De Sanctis, U.; De Santo, A.; Grout, Z. J.; Lerner, G.; Salvatore, F.; Castillo, I. Santoyo; Shehu, C. Y.; Suruliz, K.; Sutton, M. R.; Vivarelli, I.; Winston, O. J.] Univ Sussex, Dept Phys & Astron, Brighton, E Sussex, England. [Black, C. W.; Cuthbert, C.; Finelli, K. D.; Jeng, G. -Y.; Limosani, A.; Morley, A. K.; Patel, N. D.; Saavedra, A. F.; Scarcella, M.; Varvell, K. E.; Wang, J.; Watson, I. J.; Yabsley, B.] Univ Sydney, Sch Phys, Sydney, NSW 2006, Australia. [Abdallah, J.; Hou, S.; Hsu, P. J.; Lee, S. C.; Li, B.; Lin, S. C.; Liu, B.; Liu, D.; Lo Sterzo, F.; Mazini, R.; Shi, L.; Soh, D. A.; Song, H. Y.; Teng, P. K.; Wang, C.; Wang, S. M.; Yang, Y.; Zhang, G.] Acad Sinica, Inst Phys, Taipei 115, Taiwan. [Abreu, H.; Di Mattia, A.; Gozani, E.; Rozen, Y.; Tarem, S.; van Eldik, N.] Technion Israel Inst Technol, Dept Phys, IL-32000 Haifa, Israel. [Abramowicz, H.; Alexander, G.; Amram, N.; Ashkenazi, A.; Bella, G.; Benary, O.; Benhammou, Y.; Davies, M.; Duarte-Campderros, J.; Etzion, E.; Gershon, A.; Gueta, O.; Oren, Y.; Soffer, A.; Taiblum, N.] Tel Aviv Univ, Raymond & Beverly Sackler Sch Phys & Astron, IL-69978 Tel Aviv, Israel. [Gkaitatzis, S.; Gkialas, I.; Iliadis, D.; Kimura, N.; Kordas, K.; Kourkoumeli-Charalampidi, A.; Leisos, A.; Papageorgiou, K.; Petridou, C.; Sampsonidis, D.] Aristotle Univ Thessaloniki, Dept Phys, GR-54006 Thessaloniki, Greece. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Grad Sch Sci & Technol, Tokyo, Japan. [Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo 158, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Oh Okayama, Tokyo 152, Japan. [Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Aloisio, A.; Azuelos, G.; Canepa, A.; Chekulaev, S. V.; Gingrich, D. M.; Jovicevic, J.; Oakham, F. G.; Oram, C. J.; Codina, E. Perez; Savard, P.; Schneider, B.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.; Vetterli, M. C.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON M3J 2R7, Canada. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, H. P.; Meoni, E.; Sliwa, K.; Son, H.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. O.; Taffard, A.; Unel, G.; Whiteson, D.] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA USA. [Acharya, B. S.; Barisonzi, M.; Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Soualah, R.; Truong, L.] INFN, Grp Collegato Udine, Sez Trieste, Udine, Italy. [Acharya, B. S.; Barisonzi, M.; Quayle, W. B.; Serkin, L.; Shaw, K.; Truong, L.] Abdus Salaam Int Ctr Theoret Phys, Trieste, Italy. [Boldyrev, A. S.; Cobal, M.; Giordani, M. P.; Miglioranzi, S.; Pinamonti, M.; Soualah, R.] Univ Udine, Dipartimento Chim Fis & Ambiente, I-33100 Udine, Italy. [Kuutmann, E. Bergeaas; Brenner, R.; Ekelof, T.; Ellert, M.; Ferrari, A.; Gradin, P. O. J.; Isaksson, C.; Maddocks, H. J.; Ohman, H.; Pelikan, D.; Rangel-Smith, C.] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden. [Atkinson, M.; Armadans, R. Caminal; Cavaliere, V.; Chang, P.; Errede, S.; Hooberman, B. H.; Lie, K.; Liss, T. M.; Liu, L.; Long, J. D.; Neubauer, M. S.; Rybar, M.; Shang, R.; Vichou, I.; Zeng, J. C.] Univ Illinois, Dept Phys, Urbana, IL 61801 USA. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Gimenez, V. Castillo; Cerda Alberich, L.; Cheplakov, A.; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Inst Fis Corpuscular IFIC, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Gimenez, V. Castillo; Cerda Alberich, L.; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Fis Atom Mol & Nucl, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Gimenez, V. Castillo; Cerda Alberich, L.; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, Dept Ingn Elect, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Gimenez, V. Castillo; Cerda Alberich, L.; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] Univ Valencia, IMB CNM, Valencia, Spain. [Alvarez Piqueras, D.; Barranco Navarro, L.; Cabrera Urban, S.; Gimenez, V. Castillo; Cerda Alberich, L.; Costa, M. J.; Martinez, P. Fernandez; Ferrer, A.; Fiorini, L.; Fuster, J.; Garcia, C.; Navarro, J. E. Garcia; Gonzalez de la Hoz, S.; Hernandez Jimenez, Y.; Higon-Rodriguez, E.; Irles Quiles, A.; Jimenez Pena, J.; King, M.; Lacasta, C.; Lacuesta, V. R.; Marti-Garcia, S.; Mitsou, V. A.; Pedraza Lopez, S.; Rodriguez Rodriguez, D.; Romero Adam, E.; Ros, E.; Salt, J.; Sanchez, J.; Sanchez Martinez, V.; Soldevila, U.; Valero, A.; Valls Ferrer, J. A.; Vos, M.] CSIC, Inst Agroquim & Tecnol Alimentos, Jaime Roig 11, E-46010 Valencia, Spain. [Danninger, M.; Fedorko, W.; Gay, C.; Gecse, Z.; Gignac, M.; Henkelmann, S.; King, S. B.; Lister, A.] Univ British Columbia, Dept Phys, Vancouver, BC V5Z 1M9, Canada. [Beckingham, M.; Ennis, J. S.; Farrington, S. M.; Harrison, P. F.; Jeske, C.; Jones, G.; Martin, T. A.; Murray, W. J.; Pianori, E.; Spangenberg, M.] Univ Warwick, Dept Phys, Coventry CV4 7AL, W Midlands, England. [Iizawa, T.; Mitani, T.; Sakurai, Y.; Yorita, K.] Waseda Univ, Tokyo, Japan. [Bressler, S.; Citron, Z. H.; Duchovni, E.; Gross, E.; Koehler, M. K.; Lellouch, D.; Levinson, L. J.; Mikenberg, G.; Milov, A.; Pitt, M.; Roth, I.; Schaarschmidt, J.; Smakhtin, V.; Turgeman, D.] Weizmann Inst Sci, Dept Particle Phys, IL-76100 Rehovot, Israel. [Banerjee, Sw.; Guan, W.; Hard, A. S.; Heng, Y.; Ji, H.; Ju, X.; Kaplan, L. S.; Kashif, L.; Kruse, A.; Ming, Y.; Wang, F.; Wiedenmann, W.; Wu, S. L.; Yang, H.; Zhang, F.; Zobernig, G.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Kuger, F.; Redelbach, A.; Schreyer, M.; Sidiropoulou, O.; Siragusa, G.; Stroehmer, R.; Tam, J. Y. C.; Trefzger, T.; Weber, S. W.; Zibell, A.] Univ Wurzburg, Fak Phys & Astron, D-97070 Wurzburg, Germany. [Bannoura, A. A. E.; Boerner, D.; Braun, H. M.; Cornelissen, T.; Ellinghaus, F.; Ernis, G.; Fischer, J.; Flick, T.; Gabizon, O.; Gilles, G.; Hamacher, K.; Harenberg, T.; Hirschbuehl, D.; Kersten, S.; Kuechler, J. T.; Maettig, P.; Neumann, M.; Pataraia, S.; Riegel, C. 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RI Gladilin, Leonid/B-5226-2011; Ippolito, Valerio/L-1435-2016; Guo, Jun/O-5202-2015; Livan, Michele/D-7531-2012; Carvalho, Joao/M-4060-2013; BESSON, NATHALIE/L-6250-2015; Lazzaroni, Massimo/N-3675-2015; Warburton, Andreas/N-8028-2013; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Seixas, Joao/F-5441-2013; Tikhomirov, Vladimir/M-6194-2015; Zhukov, Konstantin/M-6027-2015; Stabile, Alberto/L-3419-2016; Boyko, Igor/J-3659-2013; Villa, Mauro/C-9883-2009; Coccaro, Andrea/P-5261-2016; Staroba, Pavel/G-8850-2014; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Di Domenico, Antonio/G-6301-2011; Shulga, Evgeny/R-1759-2016; Maleev, Victor/R-4140-2016; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Mitsou, Vasiliki/D-1967-2009; White, Ryan/E-2979-2015; Smirnova, Oxana/A-4401-2013; Di Nardo, Roberto/J-4993-2012; Ventura, Andrea/A-9544-2015; Maneira, Jose/D-8486-2011; messina, andrea/C-2753-2013; Prokoshin, Fedor/E-2795-2012; Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Grinstein, Sebastian/N-3988-2014 OI Gladilin, Leonid/0000-0001-9422-8636; Ippolito, Valerio/0000-0001-5126-1620; Guo, Jun/0000-0001-8125-9433; Livan, Michele/0000-0002-5877-0062; Carvalho, Joao/0000-0002-3015-7821; Lazzaroni, Massimo/0000-0002-4094-1273; Warburton, Andreas/0000-0002-2298-7315; Vanadia, Marco/0000-0003-2684-276X; Seixas, Joao/0000-0002-7531-0842; Tikhomirov, Vladimir/0000-0002-9634-0581; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Villa, Mauro/0000-0002-9181-8048; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; Di Domenico, Antonio/0000-0001-8078-2759; Shulga, Evgeny/0000-0001-5099-7644; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Pina, Joao /0000-0001-8959-5044; Veneziano, Stefano/0000-0002-2598-2659; Belanger-Champagne, Camille/0000-0003-2368-2617; Belyaev, Nikita/0000-0002-1131-7121; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Mitsou, Vasiliki/0000-0002-1533-8886; White, Ryan/0000-0003-3589-5900; Smirnova, Oxana/0000-0003-2517-531X; Ventura, Andrea/0000-0002-3368-3413; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Grinstein, Sebastian/0000-0002-6460-8694 FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; Lundbeck Foundation, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Canton of Bern, Switzerland; Canton of Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; Canarie, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET; ERC; FP7; Horizon 2020; Marie Sklodowska-Curie Actions; European Union; Investissements d'Avenir Labex and Idex, France; ANR, France; Region Auvergne, France; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; Herakleitos programme - EU-ESF; Thales programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; BSF, Israel; GIF, Israel; Minerva, Israel; BRF, Norway; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF, DNSRC and Lundbeck Foundation, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, Canarie, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. NR 32 TC 4 Z9 4 U1 21 U2 94 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JUL 10 PY 2016 VL 758 BP 67 EP 88 DI 10.1016/j.physletb.2016.04.050 PG 22 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DN8LM UT WOS:000377330500012 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Konig, A Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rad, N Rahbaran, B Rohringer, H Schieck, J Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Lowette, S Moortgat, S Moreels, L Olbrechts, A Python, Q Tavernier, S Van Doninck, W Van Mulders, P Van Parijs, I Brun, H Caillol, C Clerbaux, B De Lentdecker, G Delannoy, H Fasanella, G Favart, L Goldouzian, R Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Randle-Conde, A Seva, T Velde, CV Vanlaer, P Yonamine, R Zenoni, F Zhang, F Cimmino, A Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Poyraz, D Salva, S Schofbeck, R Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L De Visscher, S Delaere, C Delcourt, M Forthomme, L Francois, B Giammanco, A Jafari, A Jez, P Komm, M Lemaitre, V Magitteri, A Mertens, A Musich, M Nuttens, C Piotrzkowski, K Quertenmont, L Selvaggi, M Marono, MV Wertz, S Beliy, N Alda, WL Alves, FL Alves, GA Brito, L Martins, MC Hensel, C Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Da Silveira, GG Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Herrera, CM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Fang, W Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Chen, Y Cheng, T Du, R Jiang, CH Leggat, D Liu, Z Romeo, F Shaheen, SM Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Zhao, J Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Alvarez, JDR Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Ferencek, D Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Finger, M Finger, M Jarrin, EC Abdelalim, AA El-Khateeb, E Mahmoud, MA Radi, A Calpas, B Kadastik, M Murumaa, M Perrini, L Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Peltola, T Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Ghosh, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Abdulsalam, A Antropov, I Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Davignon, O de Cassagnac, RG Jo, M Lisniak, S Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Pigard, P Regnard, S Salerno, R Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gele, D Goerlach, U Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Bernet, C Boudoul, G Bouvier, E Montoya, CAC Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Grenier, G Ille, B Lagarde, F Laktineh, IB Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Popov, A Sabes, D Sordini, V Donckt, MV Verdier, P Viret, S Khvedelidze, A Tsamalaidze, Z Autermann, C Beranek, S Feld, L Heister, A Kiesel, MK Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Schael, S Schomakers, C Schulte, JF Schulz, J Verlage, T Weber, H Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Knutzen, S Merschmeyer, M Meyer, A Millet, P Mukherjee, S Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Scheuch, F Sonnenschein, L Teyssier, D Thuer, S Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Hoehle, F Kargoll, B Kress, T Kunsken, A Lingemann, J Nehrkorn, A Nowack, A Nugent, IM Pistone, C Pooth, O Stahl, A Martin, MA Asin, I Beernaert, K Behnke, O Behrens, U Bin Anuar, AA Borras, K Campbell, A Connor, P Contreras-Campana, C Costanza, F Pardos, CD Dolinska, G Eckerlin, G Eckstein, D Eichhorn, T Gallo, E Garcia, JG Geiser, A Gizhko, A Luyando, JMG Gunnellini, P Harb, A Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Kieseler, J Kleinwort, C Korol, I Lange, W Lelek, A Leonard, J Lipka, K Lobanov, A Lohmann, W Mankel, R Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Ntomari, E Pitzl, D Placakyte, R Raspereza, A Roland, B Sahin, MO Saxena, P Schoerner-Sadenius, T Seitz, C Spannagel, S Stefaniuk, N Trippkewitz, KD Van Onsem, GP Walsh, R Wissing, C Blobel, V Vignali, MC Draeger, AR Dreyer, T Erfle, J Garutti, E Goebel, K Gonzalez, D Gorner, M Haller, J Hoffmann, M Hoing, RS Junkes, A Klanner, R Kogler, R Kovalchuk, N Kurz, S Lapsien, T Lenz, T Marchesini, I Marconi, D Meyer, M Niedziela, M Nowatschin, D Ott, J Pantaleo, F Peiffer, T Perieanu, A Pietsch, N Poehlsen, J Sander, C Scharf, C Schleper, P Schlieckau, E Schmidt, A Schumann, S Schwandt, J Stadie, H Steinbruck, G Stober, FM Stover, M Tholen, H Troendle, D Usai, E Vanelderen, L Vanhoefer, A Vormwald, B Barth, C Baus, C Berger, J Butz, E Chwalek, T Colombo, F De Boer, W Dierlamm, A Fink, S Friese, R Giffels, M Gilbert, A Haitz, D Hartmann, F Heindl, SM Husemann, U Katkov, I Kornmayer, A Pardo, PL Maier, B Mildner, H Mozer, MU Muller, T Muller, T Plagge, M Quast, G Rabbertz, K Rocker, S Roscher, F Schroder, M Sieber, G Simonis, HJ Ulrich, R Wagner-Kuhr, J Wayand, S Weber, M Weiler, T Williamson, S Wohrmann, C Wolf, R Anagnostou, G Daskalakis, G Geralis, T Giakoumopoulou, VA Kyriakis, A Loukas, D Topsis-Giotis, I Agapitos, A Kesisoglou, S Panagiotou, A Saoulidou, N Tziaferi, E Evangelou, I Flouris, G Foudas, C Kokkas, P Loukas, N Manthos, N Papadopoulos, I Paradas, E Filipovic, N Bencze, G Hajdu, C Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Karancsi, J Molnar, J Szillasi, Z Bartok, M Makovec, A Raics, P 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CA CMS Collaboration TI Search for supersymmetry in the multijet and missing transverse momentum final state in pp collisions at 13 TeV SO PHYSICS LETTERS B LA English DT Article DE CMS; Physics; Supersymmetry; Multijets ID SUPERGAUGE TRANSFORMATIONS; GLUINO PRODUCTION; HADRON COLLIDERS; PAIR PRODUCTION; SQUARK; MODEL; RESUMMATION; EXTENSION; INVARIANT; NEUTRINO AB A search for new physics is performed based on all-hadronic events with large missing transverse momentum produced in proton-proton collisions at root s = 13 TeV. The data sample, corresponding to an integrated luminosity of 2.3 fb(-1), was collected with the CMS detector at the CERN LHC in 2015. The data are examined in search regions of jet multiplicity, tagged bottom quark jet multiplicity, missing transverse momentum, and the scalar sum of jet transverse momenta. The observed numbers of events in all search regions are found to be consistent with the expectations from standard model processes. Exclusion limits are presented for simplified supersymmetric models of gluino pair production. Depending on the assumed gluino decay mechanism, and for a massless, weakly interacting, lightest neutralino, lower limits on the gluino mass from 1440 to 1600 GeV are obtained, significantly extending previous limits. (C) 2016 The Author. Published by Elsevier B.V. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.; Abdulsalam, A.; Byszuk, A.] Yerevan Phys Inst, Yerevan, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Koenig, A.; Kraetschmer, I.; Liko, D.; Matsushita, T.; Mikulec, I.; Rabady, D.; Rad, N.; Rahbaran, B.; Rohringer, H.; Schieck, J.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C-E.] OeAW, Inst Hochenergiephys, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. 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[Cimmino, A.; Dobur, D.; Fagot, A.; Garcia, G.; Gul, M.; Mccartin, J.; Poyraz, D.; Salva, S.; Schoefbeck, R.; Tytgat, M.; Van Driessche, W.; Yazgan, E.; Zaganidis, N.] Univ Ghent, B-9000 Ghent, Belgium. [Beluffi, C.; Bondu, O.; Brochet, S.; Bruno, G.; Caudron, A.; Ceard, L.; De Visscher, S.; Delaere, C.; Delcourt, M.; Forthomme, L.; Francois, B.; Giammanco, A.; Jafari, A.; Jez, P.; Komm, M.; Lemaitre, V.; Magitteri, A.; Mertens, A.; Musich, M.; Nuttens, C.; Piotrzkowski, K.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal; Wertz, S.] Catholic Univ Louvain, Louvain La Neuve, Belgium. [Beliy, N.] Univ Mons, B-7000 Mons, Belgium. [Alda Junior, W. L.; Alves, F. L.; Alves, G. A.; Brito, L.; Correa Martins Junior, M.; Hensel, C.; Moraes, A.; Pol, M. E.; Rebello Teles, P.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Belchior Batista Das Chagas, E.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; Da Silveira, G. G.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Huertas Guativa, L. M.; Malbouisson, H.; Matos Figueiredo, D.; Mora Herrera, C.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Ahuja, S.; Dogra, S.; Fernandez Perez Tomei, T. R.; Moon, C. S.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; Gregores, E. M.; Mercadante, P. G.; Romero Abad, D.] Univ Fed ABC, Sao Paulo, Brazil. [Aleksandrov, A.; Hadjiiska, R.; Iaydjiev, P.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Fang, W.] Beihang Univ, Beijing 100191, Peoples R China. [Ahmad, M.; Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Chen, Y.; Cheng, T.; Du, R.; Jiang, C. H.; Leggat, D.; Liu, Z.; Romeo, F.; Shaheen, S. M.; Spiezia, A.; Tao, J.; Wang, C.; Wang, Z.; Zhang, H.; Zhao, J.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Li, Q.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Xu, Z.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Cabrera, A.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Ruiz Alvarez, J. D.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Puljak, I.; Cipriano, P. M. Ribeiro] Univ Split, Fac Elect Engn, Mech Engn & Naval Architecture, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Fac Sci, Split, Croatia. [Brigljevic, V.; Ferencek, D.; Kadija, K.; Luetic, J.; Micanovic, S.; Sudic, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Rykaczewski, H.] Univ Cyprus, CY-1678 Nicosia, Cyprus. [Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Carrera Jarrin, E.] Univ San Francisco Quito, Quito, Ecuador. [Abdelalim, A. A.; El-khateeb, E.; Mahmoud, M. A.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Calpas, B.; Kadastik, M.; Murumaa, M.; Perrini, L.; Raidal, M.; Tiko, A.; Veelken, C.] NICPB, Tallinn, Estonia. [Eerola, P.; Pekkanen, J.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Peltola, T.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Ghosh, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Machet, M.; Malcles, J.; Rander, J.; Rosowsky, A.; Titov, M.; Zghiche, A.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Abdulsalam, A.; Antropov, I.; Baffioni, S.; Beaudette, F.; Busson, P.; Cadamuro, L.; Chapon, E.; Charlot, C.; Davignon, O.; de Cassagnac, R. Granier; Jo, M.; Lisniak, S.; Mine, P.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Ortona, G.; Paganini, P.; Pigard, P.; Regnard, S.; Salerno, R.; Sirois, Y.; Strebler, T.; Yilmaz, Y.; Zabi, A.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, Palaiseau, France. [Agram, J-L.; Andrea, J.; Aubin, A.; Bloch, D.; Brom, J-M.; Buttignol, M.; Chabert, E. C.; Chanon, N.; Collard, C.; Conte, E.; Coubez, X.; Fontaine, J-C.; Gele, D.; Goerlach, U.; Le Bihan, A-C.; Merlin, J. A.; Skovpen, K.; Van Hove, P.] Univ Strasbourg, Univ Haute Alsace Mulhouse, CNRS, IN2P3,Inst Pluridisciplinaire Hubert Curien, Strasbourg, France. [Gadrat, S.] CNRS, IN2P3, Ctr Calcul, Villeurbanne, France. [Beauceron, S.; Bernet, C.; Boudoul, G.; Bouvier, E.; Montoya, C. A. Carrillo; Chierici, R.; Contardo, D.; Courbon, B.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Grenier, G.; Ille, B.; Lagarde, F.; Laktineh, I. B.; Lethuillier, M.; Mirabito, L.; Pequegnot, A. L.; Perries, S.; Popov, A.; Sabes, D.; Sordini, V.; Donckt, M. Vander; Verdier, P.; Viret, S.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Khvedelidze, A.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Tsamalaidze, Z.] Tbilisi State Univ, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Feld, L.; Heister, A.; Kiesel, M. K.; Klein, K.; Lipinski, M.; Ostapchuk, A.; Preuten, M.; Raupach, F.; Schael, S.; Schomakers, C.; Schulte, J. F.; Schulz, J.; Verlage, T.; Weber, H.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Knutzen, S.; Merschmeyer, M.; Meyer, A.; Millet, P.; Mukherjee, S.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Scheuch, F.; Sonnenschein, L.; Teyssier, D.; Thueer, S.] Rhein Westfal TH Aachen, Inst Phys A3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Hoehle, F.; Kargoll, B.; Kress, T.; Kuensken, A.; Lingemann, J.; Nehrkorn, A.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Inst Phys B3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Beernaert, K.; Behnke, O.; Behrens, U.; Bin Anuar, A. A.; Borras, K.; Campbell, A.; Connor, P.; Contreras-Campana, C.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Gallo, E.; Garcia, J. Garay; Geiser, A.; Gizhko, A.; Luyando, J. M. Grados; Gunnellini, P.; Harb, A.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Karacheban, O.; Kasemann, M.; Kieseler, J.; Kleinwort, C.; Korol, I.; Lange, W.; Lelek, A.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Mankel, R.; Melzer-Pellmann, I-A.; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Ntomari, E.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Roland, B.; Sahin, M. Oe; Saxena, P.; Schoerner-Sadenius, T.; Seitz, C.; Spannagel, S.; Stefaniuk, N.; Trippkewitz, K. D.; Van Onsem, G. P.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Dreyer, T.; Erfle, J.; Garutti, E.; Goebel, K.; Gonzalez, D.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Klanner, R.; Kogler, R.; Kovalchuk, N.; Kurz, S.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Meyer, M.; Niedziela, M.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Sander, C.; Scharf, C.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schumann, S.; Schwandt, J.; Stadie, H.; Steinbrueck, G.; Stober, F. M.; Stoever, M.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.; Vormwald, B.] Univ Hamburg, Hamburg, Germany. [Barth, C.; Baus, C.; Berger, J.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Dierlamm, A.; Fink, S.; Friese, R.; Giffels, M.; Gilbert, A.; Haitz, D.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Schroeder, M.; Sieber, G.; Simonis, H. J.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Williamson, S.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.] Univ Athens, Athens 11528, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.] Univ Ioannina, GR-45110 Ioannina, Greece. [Filipovic, N.] Eotvos Lorand Univ, MTA ELTE Lendulet CMS Particle & Nucl Phys Grp, H-1364 Budapest, Hungary. [Bencze, G.; Hajdu, C.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Bahinipati, S.; Choudhury, S.; Mal, P.; Mandal, K.; Nayak, A.; Sahoo, D. K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Keshri, S.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Bhattacharya, R.; Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutt, S.; Dutta, S.; Ghosh, S.; Majumdar, N.; Modak, A.; Mondal, K.; Mukhopadhyay, S.; Nandan, S.; Purohit, A.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.; Thakur, S.] Saha Inst Nucl Phys, Kolkata, India. [Behera, P. K.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Netrakanti, P. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Indian Inst Technol, Madras 600036, Tamil Nadu, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Guchait, M.; Gurtu, A.; Jain, Sa.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Chauhan, S.; Dube, S.; Kapoor, A.; Kothekar, K.; Rane, A.; Sharma, S.] Indian Inst Sci Educ & Res IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Chenarani, S.; Tadavani, E. Eskandari; Etesami, S. M.; Fahim, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.] INFN Sez Bari, Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Battilana, C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.] Univ Bologna, Bologna, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Di Mattia, A.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sez Catania, Catania, Italy. [Albergo, S.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Viliani, L.] INFN Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] INFN Sez Genova, Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.] INFN Sez Napoli, Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Checchia, P.; Dall'Osso, M.; Manzano, P. De Castro; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; De Oliveira, A. Carvalho Antunes; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] INFN Sez Pavia, Pavia, Italy. [Magnani, A.; Montagna, P.; Ratti, S. P.; Riccardi, C.; Vai, I.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Leonardi, R.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] INFN Sez Perugia, Perugia, Italy. [Solestizi, L. Alunni; Ciangottini, D.; Fano, L.; Lariccia, P.; Leonardi, R.; Mantovani, G.; Santocchia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] INFN Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; Cipriani, M.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.] INFN Sez Roma, Rome, Italy. [Barone, L.; Cipriani, M.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bartosik, N.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Sola, V.; Solano, A.; Staiano, A.; Traczyk, P.] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.; Traczyk, P.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; La Licata, C.; Schizzi, A.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Lee, S.; Lee, S. W.; Oh, Y. D.; Sekmen, S.; Son, D. C.; Yang, Y. C.] Kyungpook Natl Univ, Daegu, South Korea. [Kim, H.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Cifuentes, J. A. Brochero; Kim, T. J.] Hanyang Univ, Seoul 133791, South Korea. [Cho, S.; Choi, S.; Go, Y.; Gyun, D.; Ha, S.; Hong, B.; Jo, Y.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Lim, J.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Almond, J.; Kim, J.; Seo, S. H.; Yang, U.; Yoo, H. D.; Yu, G. B.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius State Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.; Zolkapli, Z.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Mejia Guisao, J.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.; Uribe Estrada, C.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.; Waqas, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Hollar, J.; Leonardo, N.; Lloret Iglesias, L.; Nemallapudi, M. V.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Voytishin, N.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Chtchipounov, L.; Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Murzin, V.; Oreshkin, V.; Sulimov, V.; Vorobyev, A.] Petersburg Nucl Phys Inst, Gatchina, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Toms, M.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Chadeeva, M.; Markin, O.; Tarkovskii, E.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Rusakov, S. V.; Terkulov, A.] PN Lebedev Phys Inst, Leninsky Prospect 53, Moscow 117924, Russia. [Baskakov, A.; Belyaev, A.; Boos, E.; Dubinin, M.; Dudko, L.; Ershov, A.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Miagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Elumakhov, D.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] Inst High Energy Phys, State Res Ctr Russian Federat, Protvino, Russia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Sanchez Cruz, S.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; Curras, E.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Martinez Rivero, C.; Matorras, F.; Piedra Gomez, J.; Rodrigo, T.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Camporesi, T.; Castello, R.; Cepeda, M.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duggan, D.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Fartoukh, S.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Girone, M.; Glege, F.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Knuenz, V.; Kortelainen, M. J.; Kousouris, K.; Krammer, M.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Sauvan, J. B.; Schaefer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veckalns, V.; Veres, G. I.; Wardle, N.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meinhard, M. T.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrin, G.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Schoenenberger, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Rauco, G.; Robmann, P.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Pozdnyakov, A.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Paganis, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Damarseckin, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Cerci, D. Sunar; Tali, B.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Phys & Technol Inst, Natl Sci Ctr, UA-310108 Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Burns, D.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Abdulsalam, A.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Futyan, D.; Haddad, Y.; Hall, G.; Iles, G.; Lane, R.; Laner, C.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Mastrolorenzo, L.; Nash, J.; Nikitenko, A.; Pela, J.; Penning, B.; Pesaresi, M.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Gastler, D.; Rankin, D.; Richardson, C.; Rohlf, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Benelli, G.; Berry, E.; Cutts, D.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Jesus, O.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Spencer, E.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Burns, D.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Flores, C.; Funk, G.; Gardner, M.; Ko, W.; Lander, R.; Mclean, C.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Malberti, M.; Negrete, M. Olmedo; Paneva, M. I.; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Gerosa, R.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wood, J.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bhandari, R.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Heller, R.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Ovcharova, A.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bendavid, J.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Sun, W.; Tan, S. M.; Tao, Z.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Winn, D.] Fairfield Univ, Fairfield, CT 06430 USA. [Abdullin, S.; Albrow, M.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Cremonesi, M.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Ristori, L.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Stoynev, S.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Wang, M.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Brinkerhoff, A.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Konigsberg, J.; Korytov, A.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Shchutska, L.; Sperka, D.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Diamond, B.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Santra, A.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.; Zhang, J.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Blumenfeld, B.; Cocoros, A.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Osherson, M.; Roskes, J.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Al-bataineh, A.; Baringer, P.; Bean, A.; Bruner, C.; Castle, J.; Kenny, R. P., III; Kropivnitskaya, A.; Majumder, D.; Malek, M.; Mcbrayer, W.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bi, R.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Hsu, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Krajczar, K.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Tatar, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Benvenuti, A. C.; Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bartek, R.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Siado, J. E.; Snow, G. R.; Stieger, B.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Parker, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY 14260 USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.] Northeastern Univ, Boston, MA 02115 USA. [Bhattacharya, S.; Hahn, K. A.; Kubik, A.; Low, J. F.; Mucia, N.; Odell, N.; Pollack, B.; Schmitt, M. H.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Dev, N.; Hildreth, M.; Anampa, K. Hurtado; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Planer, M.; Reinsvold, A.; Ruchti, R.; Rupprecht, N.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Alimena, J.; Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Francis, B.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Barker, A.; Barnes, V. E.; Benedetti, D.; Folgueras, S.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, A. W.; Jung, K.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Duh, Y. T.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Hindrichs, O.; Khukhunaishvili, A.; Lo, K. 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A.; Stahl, A.; Ott, J.; Hartmann, F.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Zhukov, V.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Borras, K.] Rhein Westfal TH Aachen, Phy Inst A 3, Aachen, Germany. [Gallo, E.] Univ Hamburg, Hamburg, Germany. [Hempel, M.; Karacheban, O.; Lohmann, W.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Abdulsalam, A.; Vesztergombi, G.; Bartok, M.; Veres, G. I.; Brinkerhoff, A.] Eotvos Lorand Univ, MTA ELTE Lendulet CMS Particle & Nucl Phys Grp, Budapest, Hungary. [Karancsi, J.] Univ Debrecen, Debrecen, Hungary. [Choudhury, S.] Indian Inst Sci Educ & Res, Bhopal, India. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Savoy-Navarro, A.] Purdue Univ, W Lafayette, IN 47907 USA. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] MOSTI, Malaysian Nucl Agcy, Kajang, Malaysia. [Heredia-De La Cruz, I.] Consejo Nacl Invest Cient & Tecn, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Matveev, V.; Musienko, Y.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Matveev, V.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Kuznetsova, E.] Univ Florida, Gainesville, FL USA. [Dubinin, M.] CALTECH, Pasadena, CA 91125 USA. [Adzic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Di Marco, E.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens 11528, Greece. [Veckalns, V.] Riga Tech Univ, Riga, Latvia. [Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cerci, S.; Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, E. A.] Istanbul Bilgi Univ, Istanbul, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Newbold, D. M.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Milenovic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Milenovic, P.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Bouhali, O.; Hernandez, A. Castaneda] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [CMS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan, Armenia. RI Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Terkulov, Adel/M-8581-2015; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; TUVE', Cristina/P-3933-2015; Chadeeva, Marina/C-8789-2016; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Sznajder, Andre/L-1621-2016; Della Ricca, Giuseppe/B-6826-2013; Da Silveira, Gustavo Gil/N-7279-2014; Stahl, Achim/E-8846-2011; Mora Herrera, Maria Clemencia/L-3893-2016; Manganote, Edmilson/K-8251-2013; Lokhtin, Igor/D-7004-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; OI Brianza, Luca/0000-0001-5770-6037; Viliani, Lorenzo/0000-0002-1909-6343; ROMERO ABAD, DAVID/0000-0001-5088-9301; ORTONA, Giacomo/0000-0001-8411-2971; Gallinaro, Michele/0000-0003-1261-2277; Chapon, Emilien/0000-0001-6968-9828; Hurtado Anampa, Kenyi/0000-0002-9779-3566; ciocci, maria agnese /0000-0003-0002-5462; HSIUNG, YEE/0000-0003-4801-1238; Khvedelidze, Arsen/0000-0002-5953-0140; Androsov, Konstantin/0000-0003-2694-6542; Saka, Halil/0000-0001-7616-2573; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; Mundim, Luiz/0000-0001-9964-7805; TUVE', Cristina/0000-0003-0739-3153; Chadeeva, Marina/0000-0003-1814-1218; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Sznajder, Andre/0000-0001-6998-1108; Della Ricca, Giuseppe/0000-0003-2831-6982; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Stahl, Achim/0000-0002-8369-7506; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Reis, Thomas/0000-0003-3703-6624; Luukka, Panja/0000-0003-2340-4641; Jacob, Jeson/0000-0001-6895-5493 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MOST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie program; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science; European Union; Regional Development Fund; OPUS program of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR project (Italy) [20108T4XTM]; Thalis programme - EU-ESF; Aristeia programme - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MOST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS program of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); the Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); and the Welch Foundation, contract C-1845. NR 74 TC 16 Z9 16 U1 36 U2 86 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JUL 10 PY 2016 VL 758 BP 152 EP 180 DI 10.1016/j.physletb.2016.05.002 PG 29 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DN8LM UT WOS:000377330500025 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R Abolins, M AbouZeid, OS Abramowicz, H Abreu, H Abreu, R Abulaitia, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedraa, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Aring;kesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S AlconadaVerzini, MJ Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Alimonti, G Alio, L Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, 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K. Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wu, M. Wu, M. Wu, S. L. Wu, X. Wu, Y. Wyatt, T. R. Wynne, B. M. Xella, S. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yakabe, R. Yamaguchi, D. Yamaguchi, Y. Yamamoto, A. Yamamoto, S. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yang, H. Yang, H. Yang, Y. Yang, Z. Yao, W-M. Yap, Y. C. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yeletskikh, I. Yen, A. L. Yildirim, E. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. M. Yu, J. Yuan, L. Yuen, S. P. Y. Yusuff, I. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zakharchuk, N. Zalieckas, J. Zaman, A. Zambito, S. Zanello, L. Zanzi, D. Zeitnitz, C. Zeman, M. Zemla, A. Zeng, J. C. Zeng, Q. Zengel, K. Zenin, O. Zenis, T. Zerwas, D. Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhaod, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhub, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Search for single production of a vector-like quark via a heavy gluon in the 4b final state with the ATLAS detector in pp collisions at root s=8 TeV SO PHYSICS LETTERS B LA English DT Article ID COMPOSITE HIGGS-MODEL; BOSON; PLUS AB A search is performed for the process pp -> G* -> B-H(b) over bar/(B) over bar (H)b -> Hb (b) over bar -> b (b) over barb (b) over bar, predicted in composite Higgs scenarios, where G* is a heavy colour octet vector resonance and B-H a vector-like quark of charge -1/3. The data were obtained from pp collisions at a centre-of-mass energy of 8 TeV corresponding to an integrated luminosity of 19.5 fb(-1), recorded by the ATLAS detector at the LHC. The largest background, multijet production, is estimated using a data-driven method. No significant excess of events with respect to Standard Model predictions is observed, and upper limits on the production cross section times branching ratio are set. Comparisons to the predictions from a specific benchmark model are made, resulting in lower mass limits in the two-dimensional mass plane of m(G*) vs. m(BH). (C) 2016 The Author. Published by Elsevier B.V. C1 [Jackson, P.; Khalil-Zada, F.; Lee, L.; Petridis, A.; Soni, N.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakir, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, TR-06100 Ankara, Turkey. 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[Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] Clermont Univ, Phys Corpusculaire Lab, Clermont Ferrand, France. Univ Blaise Pascal, Clermont Ferrand, France. [Boumediene, D.; Busato, E.; Calvet, D.; Calvet, S.; Donini, J.; Gris, Ph.; Liao, H.; Madar, R.; Pallin, D.; Saez, S. M. Romano; Santoni, C.; Simon, D.; Vazeille, F.] CNRS IN2P3, Clermont Ferrand, France. [Alkire, S. P.; Angerami, A.; Brooijmans, G.; Carbone, R. M.; Cole, B.; Hu, D.; Hughes, E. W.; Iordanidou, K.; Klein, M. H.; Mohapatra, S.; Ochoa, I.; Parsons, J. A.; Smith, M. N. K.; Smith, R. W.; Thompson, E. N.; Tuts, P. M.; Wang, T.; Zhou, L.] Columbia Univ, Nevis Lab, Irvington, NY USA. [Alonso, A.; Besjes, G. J.; Dam, M.; Galster, G.; Hansen, J. B.; Hansen, J. D.; Hansen, P. H.; Loevschall-Jensen, A. E.; Monk, J.; Mortensen, S. S.; Pedersen, L. E.; Petersen, T. 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J.; Derendarz, D.; Godlewski, J.; Gornicki, E.; Hajduk, Z.; Iwanski, W.; Kaczmarska, A.; Knapik, J.; Korcyl, K.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hiller, K. H.; Howarth, J.; Katzy, J.; Keller, J. S.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; O'Rourke, A. A.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Rubinskiy, I.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.] DESY, Notkestr 85, Hamburg, Germany. DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Goessling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.; Schorlemmer, A. L. S.] Tech Univ Dortmund, Inst Expt Phys 4, D-44221 Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kotwal, A.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Clark, P. J.; Dias, F. A.; Edwards, N. C.; Walls, F. M. Garay; Glaysher, P. C. F.; Leonidopoulos, C.; Mills, C.; Proissl, M.; Smart, B. H.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Antonelli, M.; Bilokon, H.; Esposito, B.; Gatti, C.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruehr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Hugstetter Str 55, D-79106 Freiburg, Germany. [Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Katre, A.; Miucci, A.; Ristic, B.; Sfyrla, A.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gaudiello, A.; Guido, E.; Osculati, B.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, GE-380086 Tbilisi, Rep of Georgia. [Dueren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, D-35390 Giessen, Germany. [Britton, D.; Buckley, A. G.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Knue, A.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Robson, A.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Kawamura, G.; Lemmer, B.; Magradze, E.; Mchedlidze, G.; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Shabalina, E.; Weingarten, J.] Univ Gottingen, Inst Phys 2, D-37073 Gottingen, Germany. [Albrand, S.; Berlendis, S.; Buzatu, A.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Durglishvili, A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, CNRS IN2P3, Lab Phys Subatom & Cosmol, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. 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Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Barton, A. E.] Univ Lancaster, Dept Phys, Lancaster, England. [Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, I-73100 Lecce, Italy. [Aloisio, A.; Gorini, E.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Gwilliam, C. B.; Hayward, H. S.; King, B. T.; Kretzschmar, J.; Lehan, A.; Mehta, A.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool L69 3BX, Merseyside, England. Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Filipcic, A.] Univ Ljubljana, Ljubljana, Slovenia. [Bevan, A. J.; Cerrito, L.; Fletcher, G.; Hays, J. M.; Morris, J. D.; Piccaro, E.; Rizvi, E.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Blanco, J. E.; Connelly, I. A.; Cowan, G.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. 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Doyle, Anthony/C-5889-2009; Conde Muino, Patricia/F-7696-2011; Brooks, William/C-8636-2013; Grinstein, Sebastian/N-3988-2014; Zhukov, Konstantin/M-6027-2015; Warburton, Andreas/N-8028-2013; La Rosa Navarro, Jose Luis/K-4221-2016; Vanadia, Marco/K-5870-2016; Seixas, Joao/F-5441-2013; Tikhomirov, Vladimir/M-6194-2015; Ippolito, Valerio/L-1435-2016; Mitsou, Vasiliki/D-1967-2009; Gladilin, Leonid/B-5226-2011; Guo, Jun/O-5202-2015; Livan, Michele/D-7531-2012; Carvalho, Joao/M-4060-2013; BESSON, NATHALIE/L-6250-2015 OI Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; Pina, Joao /0000-0001-8959-5044; Veneziano, Stefano/0000-0002-2598-2659; Lacasta, Carlos/0000-0002-2623-6252; Belanger-Champagne, Camille/0000-0003-2368-2617; Belyaev, Nikita/0000-0002-1131-7121; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Stabile, Alberto/0000-0002-6868-8329; Boyko, Igor/0000-0002-3355-4662; Villa, Mauro/0000-0002-9181-8048; Coccaro, Andrea/0000-0003-2368-4559; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; Di Domenico, Antonio/0000-0001-8078-2759; Shulga, Evgeny/0000-0001-5099-7644; Camarri, Paolo/0000-0002-5732-5645; White, Ryan/0000-0003-3589-5900; Smirnova, Oxana/0000-0003-2517-531X; Ventura, Andrea/0000-0002-3368-3413; Maneira, Jose/0000-0002-3222-2738; Prokoshin, Fedor/0000-0001-6389-5399; Doyle, Anthony/0000-0001-6322-6195; Conde Muino, Patricia/0000-0002-9187-7478; Brooks, William/0000-0001-6161-3570; Grinstein, Sebastian/0000-0002-6460-8694; Warburton, Andreas/0000-0002-2298-7315; Vanadia, Marco/0000-0003-2684-276X; Seixas, Joao/0000-0002-7531-0842; Tikhomirov, Vladimir/0000-0002-9634-0581; Ippolito, Valerio/0000-0001-5126-1620; Mitsou, Vasiliki/0000-0002-1533-8886; Gladilin, Leonid/0000-0001-9422-8636; Guo, Jun/0000-0001-8125-9433; Livan, Michele/0000-0002-5877-0062; Carvalho, Joao/0000-0002-3015-7821; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia, Russian Federation; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF, Canada; Canada Council, Canada; Canarie, Canada; CRC, Canada; Compute Canada, Canada; FQRNT, Canada; Ontario Innovation Trust, Canada; EPLANET; ERC; FP7; Horizon 2020; Marie Sklodowska-Curie Actions; European Union; Investissements d'Avenir Labex and Idex; ANR; Region Auvergne; Fondation Partager le Savoir, France; DFG; AvH Foundation, Germany; Herakleitos, Thales and Aristeia programme; EU-ESF; Greek NSRF; BSF; GIF; Minerva, Israel; BRF, Norway; Royal Society; Leverhulme Trust, United Kingdom FX We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, Canarie, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; the Royal Society and Leverhulme Trust, United Kingdom. NR 55 TC 2 Z9 2 U1 21 U2 70 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JUL 10 PY 2016 VL 758 BP 249 EP 268 DI 10.1016/j.physletb.2016.04.061 PG 20 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DN8LM UT WOS:000377330500038 ER PT J AU Esposito, A Pilloni, A Polosa, AD AF Esposito, A. Pilloni, A. Polosa, A. D. TI Hybridized tetraquarks SO PHYSICS LETTERS B LA English DT Article DE Tetraquarks; Exotic hadrons; Feshbach resonances ID STATES AB We propose a new interpretation of the neutral and charged X, Z exotic hadron resonances. Hybridized-tetraquarks are neither purely compact tetraquark states nor bound or loosely bound molecules but rather a manifestation of the interplay between the two. While meson molecules need a negative or zero binding energy, its counterpart for h-tetraquarks is required to be positive. The formation mechanism of this new class of hadrons is inspired by that of Feshbach metastable states in atomic physics. The recent claim of an exotic resonance in the B-s(0)pi(+/-) channel by the DO Collaboration and the negative result presented subsequently by the LHCb Collaboration are understood in this scheme, together with a considerable portion of available data on X, Z particles. Considerations on a state with the same quantum numbers as the X(5568) are also made. (C) 2016 The Author(s). Published by Elsevier B.V. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/). C1 [Esposito, A.] Columbia Univ, Dept Phys, 538W 120th St, New York, NY 10027 USA. [Pilloni, A.] Thomas Jefferson Natl Accelerator Facil, Ctr Theory, 12000 Jefferson Ave, Newport News, VA 23606 USA. [Pilloni, A.; Polosa, A. D.] Ist Nazl Fis Nucl, Sez Roma, Ple Aldo Moro 5, I-00185 Rome, Italy. [Polosa, A. D.] Univ Roma La Sapienza, Dipartimento Fis, Ple A Moro 2, I-00185 Rome, Italy. [Polosa, A. D.] CERN, Div Theory, CH-1211 Geneva, Switzerland. RP Polosa, AD (reprint author), Ist Nazl Fis Nucl, Sez Roma, Ple Aldo Moro 5, I-00185 Rome, Italy.; Polosa, AD (reprint author), Univ Roma La Sapienza, Dipartimento Fis, Ple A Moro 2, I-00185 Rome, Italy.; Polosa, AD (reprint author), CERN, Div Theory, CH-1211 Geneva, Switzerland. EM antonio.polosa@cern.ch OI Polosa, Antonio Davide/0000-0002-0684-4082 FU U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC05-06OR23177] FX We wish to thank L. Maiani, V. Riquer, A. Ali, F. Piccinini and A.L. Guerrieri for useful and fruitful discussions. We also thank Z.G. Wang for the comments on the manuscript. This material is based upon work supported in part by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under contract DE-AC05-06OR23177. NR 46 TC 16 Z9 16 U1 1 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JUL 10 PY 2016 VL 758 BP 292 EP 295 DI 10.1016/j.physletb.2016.05.028 PG 4 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DN8LM UT WOS:000377330500043 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Rougny, R De Klundert, MV Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D 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Damiao, DD Martins, CD DeSouza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Abad, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Zou, W Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M Abdelalim, AA Awad, A Mahrous, A 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Thomassen, P. Walker, M. Foerster, M. Riley, G. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dalchenko, M. De Mattia, M. Delgado, A. Dildick, S. Eusebi, R. Flanagan, W. Gilmore, J. Kamon, T. Krutelyov, V. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Ni, H. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Boutle, S. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Sun, X. Wang, Y. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Christian, A. Dasu, S. Dodd, L. Duric, S. Friis, E. Gomber, B. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Search for a low-mass pseudoscalar Higgs boson produced in association with a b(b)over-bar pair in pp collisions at root s=8 TeV SO PHYSICS LETTERS B LA English DT Article DE CMS; Physics; Higgs ID LHC; PARTICLE; MODEL; WEAK AB A search is reported for a light pseudoscalar Higgs boson decaying to a pair of tau leptons, produced in association with a b (b) over bar pair, in the context of two-Higgs-doublet models. The results are based on pp collision data at a centre-of-mass energy of 8 TeV collected by the CMS experiment at the LHC and corresponding to an integrated luminosity of 19.7 fb(-1). Pseudoscalar boson masses between 25 and 80 GeV are probed. No evidence for a pseudoscalar boson is found and upper limits are set on the product of cross section and branching fraction to tau pairs between 7 and 39 pb at the 95% confidence level. This excludes pseudoscalar A bosons with masses between 25 and 80 GeV, with SM-like Higgs boson negative couplings to down-type fermions, produced in association with bb pairs, in Type II, two-Higgs-doublet models. (C) 2016 The Author(s). Published by Elsevier B.V. This is an open access article under the CC BY license (http://creativecommonnorg/licensesiby/4.01). C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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G.; Delaere, C.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jafari, A.; Jez, P.; Komm, M.; Lemaitre, V.; Mertens, A.; Nuttens, C.; Perrini, L.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Vidal Marono, M.] Catholic Univ Louvain, Louvain La Neuve, Belgium. [Beliy, N.; Hammad, G. H.] Univ Mons, B-7000 Mons, Belgium. [Caudron, A.; Alda Junior, W. L.; Alves, G. A.; Brito, L.; Correa Martins Junior, M.; Hamer, M.; Hensel, C.; Mora Herrera, C.; Moraes, A.; Pol, M. E.; Rebello Teles, P.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Belchior Batista Das Chagas, E.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Huertas Guativa, L. M.; Malbouisson, H.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Ahuja, S.; Dogra, S.; Fernandez Perez Tomei, T. R.; Moon, C. S.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; De Souza Santos, A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Aleksandrov, A.; Hadjiiska, R.; Iaydjiev, P.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Vutova, M.] Bulgarian Acad Sci, Inst Nucl Res & Nucl Energy, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, BU-1126 Sofia, Bulgaria. [Aleksandrov, A.; Ahmad, M.; Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Cheng, T.; Du, R.; Jiang, C. H.; Plestina, R.; Romeo, F.; Shaheen, S. M.; Tao, J.; Wang, C.; Wang, Z.; Zhang, H.] Inst High Energy Phys, Beijing 100039, Peoples R China. [Zhang, F.; Asawatangtrakuldee, C.; Ban, Y.; Li, Q.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Xu, Z.; Zou, W.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing 100871, Peoples R China. [Avila, C.; Cabrera, A.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Puljak, I.; Cipriano, P. M. Ribeiro] Univ Split, Fac Elect Engn Mech Engn & Naval Architecture, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Fac Sci, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Micanovic, S.; Sudic, L.] Inst Rudjer Boskov, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Rykaczewski, H.] Univ Cyprus, CY-1678 Nicosia, Cyprus. [Bodlak, M.; Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [Abdelalim, A. A.; Awad, A.; Mahrous, A.; Radi, A.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Giammanco, A.; Calpas, B.; Kadastik, M.; Murumaa, M.; Raidal, M.; Tiko, A.; Veelken, C.] NICPB, Tallinn, Estonia. [Eerola, P.; Pekkanen, J.; Voutilainen, M.] Univ Helsinki, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Machet, M.; Malcles, J.; Rander, J.; Rosowsky, A.; Titov, M.; Zghiche, A.] CEA Saclay, DSM IRFU, F-91191 Gif Sur Yvette, France. [Plestina, R.; Antropov, I.; Baffioni, S.; Beaudette, F.; Busson, P.; Cadamuro, L.; Chapon, E.; Charlot, C.; Dahms, T.; Davignon, O.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Lisniak, S.; Mastrolorenzo, L.; Mine, P.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Ortona, G.; Paganini, P.; Pigard, P.; Regnard, S.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Strebler, T.; Yilmaz, Y.; Zabi, A.] Ecole Polytech, CNRS, IN2P3, Lab Leprince Ringuet, F-91128 Palaiseau, France. [Beluffi, C.; Agram, J. -L.; Andrea, J.; Aubin, A.; Bloch, D.; Brom, J. -M.; Buttignol, M.; Chabert, E. C.; Chanon, N.; Collard, C.; Conte, E.; Coubez, X.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Le Bihan, A. -C.; Merlin, J. A.; Skovpen, K.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS IN2P3, Strasbourg, France. [Gadrat, S.] CNRS IN2P3, Inst Natl Phys Nucl & Phys Particules, Ctr Calcul, Villeurbanne, France. [Beauceron, S.; Bernet, C.; Boudoul, G.; Bouvier, E.; Montoya, C. A. Carrillo; Chierici, R.; Contardo, D.; Courbon, B.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Lagarde, F.; Laktineh, I. B.; Lethuillier, M.; Mirabito, L.; Pequegnot, A. L.; Perries, S.; Alvarez, J. D. Ruiz; Sabes, D.; Sgandurra, L.; Sordini, V.; Vander Donckt, M.; Verdier, P.; Viret, S.] Univ Lyon 1, CNRS IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Toriashvili, T.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Toriashvili, T.; Tsamalaidze, Z.] Tbilisi State Univ, GE-380086 Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Edelhoff, M.; Feld, L.; Heister, A.; Kiesel, M. K.; Klein, K.; Lipinski, M.; Ostapchuk, A.; Preuten, M.; Raupach, F.; Schael, S.; Schulte, J. F.; Verlage, T.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Scheuch, F.; Sonnenschein, L.; Teyssier, D.; Thueer, S.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kuensken, A.; Lingemann, J.; Nehrkorn, A.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B 3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behnke, O.; Behrens, U.; Bell, A. J.; Borras, K.; Burgmeier, A.; Cakir, A.; Calligaris, L.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Gallo, E.; Garcia, J. Garay; Geiser, A.; Gizhko, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Karacheban, O.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Korol, I.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Roland, B.; Sahin, M. Oe.; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Trippkewitz, K. D.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Gallo, E.; Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Gonzalez, D.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Klanner, R.; Kogler, R.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Meyer, M.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schwandt, J.; Seidel, M.; Sola, V.; Stadie, H.; Steinbruck, G.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.; Vormwald, B.] Univ Hamburg, Hamburg, Germany. [Akbiyik, M.; Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Giffels, M.; Gilbert, A.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Woehrmann, C.; Wolf, R.] Univ Karlsruhe, Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.; Sphicas, P.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, GR-45110 Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.; Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Karancsi, J.; Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, D. K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh 160014, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi 110007, India. [Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Jain, Sa.; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Bombay 400085, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sudhakar, K.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. [Chauhan, S.; Dube, S.; Sharma, S.] IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin 2, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iasellia, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Puglies, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iasellia, G.; Maggi, G.; My, S.; Puglies, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Catania, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] Ist Nazl Fis Nucl, Sez Milano Bicocca, Via Celoria 16, I-20133 Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.] Ist Nazl Fis Nucl, Sez Napoli, I-80125 Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, I-85100 Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Bellato, M.; Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Checchi, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Ventura, S.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.; Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.; Ryu, M. S.] Chonbuk Natl Univ, Jeonju 561756, South Korea. [Song, S.] Chonnam Natl Univ, Inst Univ & Elementary Particles, Kwangju, South Korea. [Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, H.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lee, S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, H.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Linares, E. Casimiro; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch 1, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentac & Fis Expt Particulas, Lisbon, Portugal. [Finger, M.; Finger, M., Jr.; Tsamalaidze, Z.; Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Russian Acad Sci, Inst Nucl Res, Moscow 117312, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.; Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow 117259, Russia. [Bylinkin, A.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.; Vinogradov, A.] PN Lebedev Phys Inst, Moscow, Russia. [Popov, A.; Zhukov, V.; Katkov, I.; Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Gribushin, A.; Klyukhin, V.; Kodolova, O.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.] Moscow MV Lomonosov State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, POB 550, Belgrade 11001, Serbia. [Adzic, P.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Lopez Virto, A.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Peris, A. Delgado; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Lopez, S. Goy; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-CaleroYzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Duarte Campderros, J.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, Inst Fis Cantabria IFCA, CSIC, E-39005 Santander, Spain. [Rabady, D.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Silvestris, L.; Battilana, C.; Marzocchi, B.; Paolucci, P.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; Colafranceschi, S.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Woehri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Baeni, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Bakirci, M. N.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Eskut, E.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Kangal, I. Hos E. E.; Onengut, G.; Ozdemir, K.; Polatoz, A.; Cerci, D. Sunar; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Newbold, D. M.; Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Sinthuprasith, T.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Gunion, J.; Jiang, Y.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, San Diego, CA 92103 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] UIC, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tan, P.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Barnett, B. A.; Blumenfeld, B.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; DiMatteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Saka, Quan H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Demortier, L.] Rockefeller Univ, 1230 York Ave, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Kunnawalkam Elayavalli, R.; Lath, A.; Nash, K.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Kamon, T.; Mueller, R.; Osipenkov, I.; Patel, R.; Perloff, A.; Rose, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Ni, H.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Christian, A.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Gomber, B.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Jeitler, M.; Kraemmer, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [Moon, C. S.] CNRS, IN2P3, Paris, France. [Abdelalim, A. A.; Awad, A.] Helwan Univ, Cairo, Egypt. [Abdelalim, A. A.] Zewail City Sci & Technol, Zewail, Egypt. [Mahrous, A.; Radi, A.] British Univ Egypt, Cairo, Egypt. [Mahrous, A.; Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Plasma Phys Res Ctr, Sci & Res Branch, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. Agensi Nuklear Malaysia, MOSTI, Kajang, Malaysia. [Heredia-de La Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Bakirci, M. N.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Kangal, I. Hos E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Cerci, D. Sunar] Adiyaman Univ, Adiyaman, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.; Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Boletti, A.; Branca, A.; Gozzelino, A.; Bouhali, O.; Hernandez, A. Castaneda] Texas A&M Univ, Doha, Qatar. [CMS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Petkov, Peicho/M-2080-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Mora Herrera, Maria Clemencia/L-3893-2016; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; TUVE', Cristina/P-3933-2015; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; Della Ricca, Giuseppe/B-6826-2013; Manganote, Edmilson/K-8251-2013; Lokhtin, Igor/D-7004-2012; VARDARLI, Fuat Ilkehan/B-6360-2013; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Verwilligen, Piet/M-2968-2014; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Stahl, Achim/E-8846-2011 OI Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Petkov, Peicho/0000-0002-0420-9480; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Mundim, Luiz/0000-0001-9964-7805; TUVE', Cristina/0000-0003-0739-3153; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; ciocci, maria agnese /0000-0003-0002-5462; Della Ricca, Giuseppe/0000-0003-2831-6982; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Stahl, Achim/0000-0002-8369-7506 FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES, (Brazil); FAPERJ, (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS, (China); MOST, (China); NSFC, (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC, (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG, (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science; European Union; Regional Development Fund; OPUS programme of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR project (Italy) [20108T4XTM]; Thalis and Aristeia programmes - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MOST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, contract C-1845. NR 67 TC 5 Z9 5 U1 24 U2 61 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JUL 10 PY 2016 VL 758 BP 296 EP 320 DI 10.1016/j.physletb.2016.05.003 PG 25 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DN8LM UT WOS:000377330500044 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Rougny, R Van De Klundert, M Van Haevermaet, H Van Mechelen, R Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D 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Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, R. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Measurement of spin correlations in tf production using the matrix element method in the muon plus jets final state in pp collisions at root S=8 TeV SO PHYSICS LETTERS B LA English DT Article DE CMS; LHC; Top quark; Matrix element method; Spin ID T(T)OVER-BAR PRODUCTION; LIKELIHOOD METHOD; MISSING MOMENTUM; EVENTS; DECAY; RECONSTRUCTION; TAUOLA; MASS AB The consistency of the spin correlation strength in top quark pair production with the standard model (SM) prediction is tested in the muon+jets final state. The events are selected from pp collisions, collected by the CMS detector, at a centre-of-mass energy of 8 TeV, corresponding to an integrated luminosity of 19.7 fb(-1). The data are compared with the expectation for the spin correlation predicted by the SM and with the expectation of no correlation. Using a template fit method, the fraction of events that show SM spin correlations is measured to be 0.72 0.08 (stat)(-013)(+015) (syst), representing the most precise measurement of this quantity in the muon+jets final state to date. (C) 2016 The Author. Published by Elsevier B.V. This is an open access article under the CC BY license (http://creativecommons.orglicenses/by/4.01). C1 [CMS Collaboration] CERN, CH-1211 Geneva 23, Switzerland. [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan 375036, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. 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[Aleksandrov, A.; Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Laselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, R.] Ist Nazl Fis Nucl, Sez Bari, I-70126 Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Silvestris, L.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Laselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, R.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Siroli, G. P.; Tosi, N.; Travaglini, R.; Bonato, A.] Ist Nazl Fis Nucl, Sez Bologna, I-40126 Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, R.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Ist Nazl Fis Nucl, Sez Catania, I-95129 Catania, Italy. [Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, R.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, R.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Benussi, L.; Bianco, S.; Fabbri, F.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, POB 13, I-00044 Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Ist Nazl Fis Nucl, Sez Genova, Via Dodecaneso 33, I-16146 Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, R.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. 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N.; Ronchese, R.; Simonetto, F.; Torassa, E.; Tosi, M.; Zotto, R.; Zucchetta, A.; Zumerle, G.] Ist Nazl Fis Nucl, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, A. N.; Ronchese, R.; Simonetto, F.; Tosi, M.; Zotto, R.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, R.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, R.; Vai, I.; Vitulo, R.] Ist Nazl Fis Nucl, Sez Pavia, I-27100 Pavia, Italy. [Montagna, R.; Ratti, S. P.; Riccardi, C.; Vitulo, R.] Univ Pavia, Via Palestro 3, I-27100 Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, R.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.; Spiezia, A.] Ist Nazl Fis Nucl, Sez Perugia, I-06100 Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, R.; Mantovani, G.; Santocchia, A.; Spiezia, A.] Univ Perugia, I-06100 Perugia, Italy. [Androsov, K.; Azzurri, R.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Broccolo, G.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Squillacioti, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Broccolo, G.; Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, R.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, R.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, R.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Dellacasa, G.; Demaria, N.; Finco, L.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Musich, M.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, I-10125 Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. 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[Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-de la Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City 07738, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland 1, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch, New Zealand. [Ahmad, A.; Ahmad, M.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. 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[Adzic, R.; Ekmedzic, M.; Milosevic, J.; Rekovic, V.; Milenovic, R.] Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, R.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, R.; Duarte Campderros, J.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, E-39005 Santander, Spain. [Rabady, D.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, R.; Azzi, R.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, R.; Arcidiacono, R.; Finco, L.; Candelise, V.; Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, R.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, R.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; Colafranceschi, S.; D'Alfons, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Duenser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, R.; Hegeman, J.; Innocente, V.; Janot, R.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, R.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schafer, C.; Schwick, C.; Sharma, A.; Silva, R.; Simon, M.; Sphicas, R.; Spiga, D.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Wohri, H. K.; Zagozdzinska, A.; Zeuner, W. D.; Ulmer, K. A.] CERN, European Org Nucl Res, CH-1211 Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Buchmann, M. A.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, R.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, R.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] ETH, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, R.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli 32054, Taiwan. [Kumar, Arun; Bartek, R.; Chang, R.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W-S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei 10764, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, TR-06531 Ankara, Turkey. [Albayrak, E. A.; Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, TR-80626 Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, R.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.; Lucas, R.] Rutherford Appleton Lab, Didcot OX11 0QX, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, R.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, R.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, R.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, R.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge UB8 3PH, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Kasmi, A.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, R.] Univ Alabama, Tuscaloosa, AL USA. [Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, R.; Rankin, D.; Richardson, C.; Rohlf, J.; John, J. St.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Berry, E.; Bhattacharya, S.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Sinthuprasith, T.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chauhan, S.; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Cousins, R.; Everaerts, R.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.; Weber, M.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, R.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Sharma, V.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wurthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Barge, D.; Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, R.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Justus, C.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; To, W.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Dubinin, M.; Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, R.] Cornell Univ, Ithaca, NY USA. [Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Banerjee, S.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hirschauer, J.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, R.; Merkel, R.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, R.; Bortignon, R.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Furic, I. K.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, R.; Matchev, K.; Mei, H.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.; Hewamanage, S.; Linn, S.; Markowitz, R.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, R.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Veeraraghavan, V.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, R.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, R.; Varelas, N.; Wu, Z.; Zakaria, M.] UIC, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -R; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tan, R.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, R.; Martin, C.; Osherson, M.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, R.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y-J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, R.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Lazo-Flores, J.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA 02115 USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, R.; Hardenbrook, J.; Hebda, R.; Koay, S. A.; Lujan, R.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, R.; Quan, X.; Saka, H.; Stickland, D.; Tully, C.; Werner, J. S.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Savoy-Navarro, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, K.; Kress, M.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, R.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Demortier, L.] Rockefeller Univ, 1230 York Ave, New York, NY 10021 USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, R.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Bouhali, O.; Hernandez, A. Castaneda; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Flanagan, W.; Gilmore, J.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Rose, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Mao, Y.; Melo, A.; Ni, H.; Sheldon, R.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Boutle, S.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, R.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Christian, A.; Dasu, S.; Dodd, L.; Duric, S.; Friis, E.; Gomber, B.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, R.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Sharma, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C-E.] Vienna Univ Technol, A-1040 Vienna, Austria. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, Brazil. [El Sawy, M.] Beni Suef Univ, Bani Suwayf, Egypt. [El Sawy, M.; Salama, E.] British Univ Egypt, Cairo, Egypt. [El-Khateeb, E.; Elkafrawy, T.; Salama, E.] Ain Shams Univ, Cairo, Egypt. [Mohamed, A.] Zewail City Sci & Technol, Zewail, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Hempel, M.; Karacheban, O.; Lohmann, W.; Marfin, I.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Veszpremi, V.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Bhowmik, S.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.; Maity, M.] King Abdulaziz Univ, Jeddah 21413, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Androsov, K.; Ciocci, M. A.; Grippo, M. T.; Squillacioti, P.] Univ Siena, Via Laterina 8, I-53100 Siena, Italy. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] Agensi Nuklear Malaysia, MOSTI, Kajang, Malaysia. [Heredia-de la Cruz, I.] Consejo Nacl Invest Cient & Tecn, Mexico City, DF, Mexico. [Byszuk, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Colafranceschi, S.] Univ Rome, Fac Ingn, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Ist Nazl Fis Nucl, Scuola Normale & Sez, Pisa, Italy. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Cerci, S.; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Albayrak, E. A.; Ozok, F.] Mimar Sinan Univ, Istanbul, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, T.] Yildiz Tekn Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Belyaev, A.] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez] Inst Astrofis Canarias, E-38200 San Cristobal la Laguna, Spain. [Wasserbaech, S.] Utah Valley Univ, Orem, UT USA. [Bilki, B.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.] Erzincan Univ, Erzincan, Turkey. [Bouhali, O.] Texas A&M Univ, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. [Moon, C. S.] CNRS, IN2P3, Paris, France. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan 375036, Armenia. RI Azarkin, Maxim/N-2578-2015; ciocci, maria agnese /I-2153-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Mundim, Luiz/A-1291-2012; Colafranceschi, Stefano/M-1807-2016; TUVE', Cristina/P-3933-2015; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Goh, Junghwan/Q-3720-2016; Varela, Joao/K-4829-2016; Seixas, Joao/F-5441-2013; Vilela Pereira, Antonio/L-4142-2016; Sznajder, Andre/L-1621-2016; Da Silveira, Gustavo Gil/N-7279-2014; Stahl, Achim/E-8846-2011; Mora Herrera, Maria Clemencia/L-3893-2016; Della Ricca, Giuseppe/B-6826-2013; Manganote, Edmilson/K-8251-2013; Lokhtin, Igor/D-7004-2012; VARDARLI, Fuat Ilkehan/B-6360-2013 OI ciocci, maria agnese /0000-0003-0002-5462; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Ogul, Hasan/0000-0002-5121-2893; Mundim, Luiz/0000-0001-9964-7805; TUVE', Cristina/0000-0003-0739-3153; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Goh, Junghwan/0000-0002-1129-2083; Varela, Joao/0000-0003-2613-3146; Seixas, Joao/0000-0002-7531-0842; Vilela Pereira, Antonio/0000-0003-3177-4626; Sznajder, Andre/0000-0001-6998-1108; Da Silveira, Gustavo Gil/0000-0003-3514-7056; Stahl, Achim/0000-0002-8369-7506; Mora Herrera, Maria Clemencia/0000-0003-3915-3170; Della Ricca, Giuseppe/0000-0003-2831-6982; FU BMWFW (Austria); FWF (Austria); FNRS (Belgium); FWO (Belgium); CNPq (Brazil); CAPES (Brazil); FAPERJ (Brazil); FAPESP (Brazil); MES (Bulgaria); CERN; CAS (China); MoST (China); NSFC (China); COLCIENCIAS (Colombia); MSES (Croatia); CSF (Croatia); RPF (Cyprus); MoER (Estonia); ERC IUT (Estonia); ERDF (Estonia); Academy of Finland (Finland); MEC (Finland); HIP (Finland); CEA (France); CNRS/IN2P3 (France); BMBF (Germany); DFG (Germany); HGF (Germany); GSRT (Greece); OTKA (Hungary); NIH (Hungary); DAE (India); DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP (Republic of Korea); NRF (Republic of Korea); LAS (Lithuania); MOE (Malaysia); UM (Malaysia); CINVESTAV (Mexico); CONACYT (Mexico); SEP (Mexico); UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE (Poland); NSC (Poland); FCT (Portugal); JINR (Dubna); MON (Russia); RosAtom (Russia); RAS (Russia); RFBR (Russia); MESTD (Serbia); SEIDI (Spain); CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter (Thailand); IPST (Thailand); STAR (Thailand); NSTDA (Thailand); TUBITAK (Turkey); TAEK (Turkey); NASU (Ukraine); SFFR (Ukraine); STFC (United Kingdom); DOE (USA); NSF (USA); Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A.P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Scientific and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science; European Union; Regional Development Fund; OPUS programme of the National Science Centre (Poland); Compagnia di San Paolo (Torino); MIUR project (Italy) [20108T4XTM]; Thalis and Aristeia programmes - EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses. Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: BMWFW and FWF (Austria); FNRS and FWO (Belgium); CNPq, CAPES, FAPERJ, and FAPESP (Brazil); MES (Bulgaria); CERN; CAS, MoST, and NSFC (China); COLCIENCIAS (Colombia); MSES and CSF (Croatia); RPF (Cyprus); MoER, ERC IUT and ERDF (Estonia); Academy of Finland, MEC, and HIP (Finland); CEA and CNRS/IN2P3 (France); BMBF, DFG, and HGF (Germany); GSRT (Greece); OTKA and NIH (Hungary); DAE and DST (India); IPM (Iran); SFI (Ireland); INFN (Italy); MSIP and NRF (Republic of Korea); LAS (Lithuania); MOE and UM (Malaysia); CINVESTAV, CONACYT, SEP, and UASLP-FAI (Mexico); MBIE (New Zealand); PAEC (Pakistan); MSHE and NSC (Poland); FCT (Portugal); JINR (Dubna); MON, RosAtom, RAS and RFBR (Russia); MESTD (Serbia); SEIDI and CPAN (Spain); Swiss Funding Agencies (Switzerland); MST (Taipei); ThEPCenter, IPST, STAR and NSTDA (Thailand); TUBITAK and TAEK (Turkey); NASU and SFFR (Ukraine); STFC (United Kingdom); DOE and NSF (USA).; Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A.P. Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Scientific and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Centre (Poland); the Compagnia di San Paolo (Torino); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, contract C-1845. NR 52 TC 1 Z9 1 U1 20 U2 49 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JUL 10 PY 2016 VL 758 BP 321 EP 346 DI 10.1016/j.physletb.2016.05.005 PG 26 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DN8LM UT WOS:000377330500045 ER PT J AU Adam, J Adamova, D Aggarwal, MM Rinella, GA Agnello, M Agrawal, N Ahammed, Z Ahmad, S Ahn, SU Aiola, S Akindinov, A Alam, SN Aleksandrov, D Alessandro, B Alexandre, D Molina, RA Alici, A Alkin, A Almaraz, JRM Alme, J Alt, T Altinpinar, S Altsybeev, I Prado, CAG Andrei, C Andronic, A Anguelov, V Anielski, J Anticic, T Antinori, F Antonioli, P Aphecetche, L Appelshauser, H Arcelli, S Arnaldi, R Arnold, OW Arsene, IC Arslandok, M Audurier, B Augustinus, A Averbeck, R Azmi, MD Badala, A Baek, YW Bagnasco, S Bailhache, R Bala, R Balasubramanian, S Baldisseri, A Baral, RC Barbano, AM Barbera, R Barile, F Barnafoldi, GG Barnby, LS Barret, V Bartalini, P Barth, K Bartke, J Bartsch, E Basile, M Bastid, N Basu, S Bathen, B Batigne, G Camejo, AB Batyunya, B 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CA ALICE Collaboration TI Multi-strange baryon production in p-Pb collisions at root(NN)-N-S=5.02 TeV SO PHYSICS LETTERS B LA English DT Article ID PROTON-PROTON COLLISIONS; QUARK-GLUON PLASMA; ENERGY-DEPENDENCE; ROOT-S=7 TEV; MID-RAPIDITY; ENHANCEMENT; ALICE; GEV/C; KAON; PION AB The multi-strange baryon yields in Pb-Pb collisions have been shown to exhibit an enhancement relative to pp reactions. In this work, Xi and Omega production rates have been measured with the ALICE experiment as a function of transverse momentum, p(T), in p-Pb collisions at a centre-of-mass energy of,/sNN = 5.02 TeV. The results cover the kinematic ranges 0.6 GeV/c < p(T) < 7.2 GeV/c and 0.8 GeV/c < p(T) < 5 GeV/c, for E and S-2 respectively, in the common rapidity interval 0.5 < ycms < 0. Multi -strange baryons have been identified by reconstructing their weak decays into charged particles. The p(T) spectra are analysed as a function of event charged -particle multiplicity, which in p-Pb collisions ranges over one order of magnitude and lies between those observed in pp and Pb-Pb collisions. The measured p -r distributions are compared to the expectations from a Blast -Wave model. The parameters which describe the production of lighter hadron species also describe the hyperon spectra in high multiplicity p-Pb collisions. The yield of hyperons relative to charged pions is studied and compared with results from pp and Pb-Pb collisions. A continuous increase in the yield ratios as a function of multiplicity is observed in p-Pb data, the values of which range from those measured in minimum bias pp to the ones in Pb-Pb collisions. A statistical model qualitatively describes this multiplicity dependence using a canonical suppression mechanism, in which the small volume causes a relative reduction of hadron production dependent on the strangeness content of the hyperon. 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Villalobos; Zardoshti, N.] Univ Birmingham, Sch Phys & Astron, Birmingham, W Midlands, England. [Villar, E. Calvo; Endress, E.; Gago, A. M.] Pontificia Univ Catolica Peru, Dept Ciencias, Secc Fis, Lima, Peru. [de cataldo, G.; Elia, D.; Lenti, V.; Manzari, V.; Minervini, L. M.; Nappi, E.; Paticchio, V.] Sezione Ist Nazl Fis Nucl, Bari, Italy. [Alici, A.; Antonioli, P.; Cindolo, F.; Hatzifotiadou, D.; Margotti, A.; Nania, R.; Noferini, F.; Pinazza, O.; Preghenella, R.; Scapparone, E.; Williams, M. C. S.; Zampolli, C.] Sezione Ist Nazl Fis Nucl, Bologna, Italy. [Cicalo, C.; Masoni, A.; Siddhanta, S.] Sezione Ist Nazl Fis Nucl, Cagliari, Italy. [Badala, A.; Pappalardo, G. S.] Sezione Ist Nazl Fis Nucl, Catania, Italy. [Antinori, F.; Dainese, A.; Fabris, D.; Turrisi, R.] Sezione Ist Nazl Fis Nucl, Padua, Italy. [Mazzoni, M. A.] Sezione Ist Nazl Fis Nucl, Rome, Italy. [Fragiacomo, E.; Grion, N.; Piano, S.; Rachevski, A.] Sezione Ist Nazl Fis Nucl, Trieste, Italy. [Agnello, M.; Alessandro, B.; Arnaldi, R.; Bagnasco, S.; Bedda, C.; Bruna, E.; Cerello, P.; Morales, Y. Corrales; de Marco, N.; Feliciello, A.; Giubellino, P.; La Pointe, S. L.; Oppedisano, C.; Prino, F.; Scomparin, E.] Sezione Ist Nazl Fis Nucl, Turin, Italy. [Evdokimov, S.; Izucheev, V.; Kharlov, Y.; Kondratyuk, E.; Petrov, V.; Polichtchouk, B.; Sadovsky, S.; Shangaraev, A.] SSC IHEP NRC Kurchatov Inst, Protvino, Russia. [Weber, M.] Stefan Meyer Inst Subatomare Phys SMI, Vienna, Austria. [Aphecetche, L.; Audurier, B.; Batigne, G.; Erazmus, B.; Estienne, M.; Germain, M.; Blanco, J. Martin; Garcia, G. Martinez; Massacrier, L.; Molnar, L.; De Godoy, D. A. Moreira; Morreale, A.; Pillot, P.; Ronflette, L.; Schutz, Y.; Shabetai, A.; Stocco, D.; Wang, M.; Zhu, J.] Univ Nantes, CNRS IN2P3, Ecole Mines Nantes, SUBATECH, Nantes, France. [Kobdaj, C.; Poonsawat, W.] Suranaree Univ Technol, Nakhon Ratchasima, Thailand. [Cerkala, J.; Jadlovska, S.; Jadlovsky, J.; Kopcik, M.; Papcun, P.] Tech Univ, Kosice, Slovakia. [Gotovac, S.; Mudnic, E.; Vickovic, L.] Tech Univ Split FESB, Split, Croatia. [Bartke, J.; Figiel, J.; Gladysz-Dziadus, E.; Goerlich, L.; Kowalski, M.; Matyja, A.; Mayer, C.; Otwinowski, J.; Rybicki, A.; Sputowska, I.] Polish Acad Sci, Henryk Niewodniczanski Inst Nucl Phys, Krakow, Poland. [Blair, J. T.; Gauger, E. F.; Knospe, A. G.; Markert, C.; Thomas, D.] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA. [Almaraz, J. R. M.; Monzon, I. Leon; Podesta-Lerma, P. L. M.] Univ Autonoma Sinaloa, Culiacan, Mexico. [Prado, C. Alves Garcia; Bregant, M.; Cosentino, M. R.; De, S.; de Conti, C.; Gimenez, D. Domenicis; Figueredo, M. A. S.; Jahnke, C.; Fernandes, C. Lagana; Mas, A.; Munhoz, M. G.; da Luz, H. Natal; Da Silva, A. C. Oliveira; Suaide, A. A. P.; de Toledo, A. Szanto; Zanoli, H. J. C.] Univ Sao Paulo, Sao Paulo, Brazil. [Chinellato, D. D.; Dash, A.; de Souza, R. D.; Takahashi, J.] Univ Estadual Campinas UNICAMP, Campinas, Brazil. [Bellwied, R.; Bianchi, L.; Jayarathna, P. H. S. Y.; Jena, S.; Mcdonald, D.; Ng, F.; Pinsky, L.; Piyarathna, D. B.; Timmins, A. R.] Univ Houston, Houston, TX USA. [Chang, B.; Kim, D. J.; Rak, J.; Slupecki, M.; Snellman, T. W.; Trzaska, W. H.; Vargyas, M.; Viinikainen, J.] Univ Jyvaskyla, Jyvaskyla, Finland. [Borri, M.; Chartier, M.; Figueredo, M. A. S.; Norman, J.; Romita, R.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Castro, A. J.; Mazer, J.; Nattrass, C.; Read, K. F.; Roy, C.; Scott, R.; Sharma, N.; Sorensen, S.] Univ Tennessee, Knoxville, TN USA. [Marchisone, M.; Vilakazi, Z.] Univ Witwatersrand, Johannesburg, South Africa. [Gunji, T.; Hamagaki, H.; Hayashi, S.; Murakami, H.; Sekiguchi, Y.; Terasaki, K.; Tsuji, T.; Watanabe, Y.] Univ Tokyo, Tokyo, Japan. [Bhom, J.; Busch, O.; Chujo, T.; Esumi, S.; Hosokawa, R.; Inaba, M.; Miake, Y.; Sano, M.; Tanaka, N.; Watanabe, D.; Yokoyama, H.] Univ Tsukuba, Tsukuba, Ibaraki, Japan. [Erhardt, F.; Planinic, M.; Poljak, N.; Simatovic, G.; Utrobicic, A.] Univ Zagreb, Zagreb, Croatia. [Cheshkov, C.; Cheynis, B.; Ducroux, L.; Grossiord, J. -Y.; Teyssier, B.; Tieulent, R.; Uras, A.] Univ Lyon 1, IPN Lyon, CNRS IN2P3, Villeurbanne, France. [Altsybeev, I.; Feofilov, G.; Kolojvari, A.; Kondratiev, V.; Kovalenko, V.; Vechernin, V.; Vinogradov, L.; Zarochentsev, A.] St Petersburg State Univ, V Fock Inst Phys, St Petersburg 199034, Russia. [Ahammed, Z.; Alam, S. N.; Basu, S.; Chattopadhyay, S.; Choudhury, S.; Dubey, A. K.; Ghosh, P.; Kar, S.; Khan, S. A.; Mitra, J.; Mohanty, B.; Muhuri, S.; Mukherjee, M.; Nayak, T. K.; Pal, S. K.; Patra, R. N.; Saini, J.; Sarkar, D.; Singaraju, R.; Singha, S.; Singhal, V.; Sinha, B. C.; Viyogi, Y. P.] Variable Energy Cyclotron Ctr, Kolkata, India. [Graczykowski, L. K.; Jakubowska, M. J.; Janik, M. A.; Kisiel, A.; Oleniacz, J.; Pluta, J.; Szymanski, M.; Zaborowska, A.; Zbroszczyk, H.] Warsaw Univ Technol, Warsaw, Poland. [Belmont, R.; Bianchin, C.; Pan, J.; Pruneau, C. A.; Pujahari, P.; Putschke, J.; Reed, R. J.; Saleh, M. A.; Verweij, M.; Voloshin, S. A.; Yaldo, C. G.] Wayne State Univ, Detroit, MI USA. [Barnafoeldi, G. G.; Bencedi, G.; Berenyi, D.; Biro, G.; Boldizsar, L.; Denes, E.; Hamar, G.; Kiss, G.; Levai, P.; Lowe, A.; Olah, L.; Pochybova, S.; Varga, D.; Volpe, G.] Hungarian Acad Sci, Wigner Res Ctr Phys, Budapest, Hungary. [Aiola, S.; Balasubramanian, S.; Caines, H.; Connors, M. E.; Ehlers, R. J.; Epple, E.; Grachov, O. A.; Harris, J. W.; Lutz, T. H.; Majka, R. D.; Mulligan, J. D.; Oh, S.; Oliver, M. H.; Schuster, T.; Smirnov, N.] Yale Univ, New Haven, CT USA. [Kang, J. H.; Kim, D.; Kim, H.; Kim, M.; Kim, T.; Kwon, Y.; Lee, S.; Song, M.] Yonsei Univ, Seoul 120749, South Korea. [Keidel, R.] Fachhochschule Worms, ZTT, Worms, Germany. [Connors, M. E.] Georgia State Univ, Atlanta, GA USA. [Khan, M. Mohisin] Aligarh Muslim Univ, Dept Appl Phys, Aligarh, Uttar Pradesh, India. [Malinina, L.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. RI Nattrass, Christine/J-6752-2016; Usai, Gianluca/E-9604-2015; Chinellato, David/D-3092-2012; Cosentino, Mauro/L-2418-2014; Suaide, Alexandre/L-6239-2016; Takahashi, Jun/B-2946-2012; Barnby, Lee/G-2135-2010; Bregant, Marco/I-7663-2012; Peitzmann, Thomas/K-2206-2012; Kondratiev, Valery/J-8574-2013; Vinogradov, Leonid/K-3047-2013; Vechernin, Vladimir/J-5832-2013; Pshenichnov, Igor/A-4063-2008; Castillo Castellanos, Javier/G-8915-2013; Ferreiro, Elena/C-3797-2017; Natal da Luz, Hugo/F-6460-2013; Martinez Hernandez, Mario Ivan/F-4083-2010; Ferretti, Alessandro/F-4856-2013; Derradi de Souza, Rafael/M-4791-2013; Kovalenko, Vladimir/C-5709-2013; Altsybeev, Igor/K-6687-2013; Vickovic, Linda/F-3517-2017; Fernandez Tellez, Arturo/E-9700-2017; OI Nattrass, Christine/0000-0002-8768-6468; Usai, Gianluca/0000-0002-8659-8378; Chinellato, David/0000-0002-9982-9577; Cosentino, Mauro/0000-0002-7880-8611; Suaide, Alexandre/0000-0003-2847-6556; Takahashi, Jun/0000-0002-4091-1779; Barnby, Lee/0000-0001-7357-9904; Peitzmann, Thomas/0000-0002-7116-899X; Kondratiev, Valery/0000-0002-0031-0741; Vinogradov, Leonid/0000-0001-9247-6230; Vechernin, Vladimir/0000-0003-1458-8055; Pshenichnov, Igor/0000-0003-1752-4524; Castillo Castellanos, Javier/0000-0002-5187-2779; Ferreiro, Elena/0000-0002-4449-2356; Natal da Luz, Hugo/0000-0003-1177-870X; Martinez Hernandez, Mario Ivan/0000-0002-8503-3009; Ferretti, Alessandro/0000-0001-9084-5784; Derradi de Souza, Rafael/0000-0002-2084-7001; Kovalenko, Vladimir/0000-0001-6012-6615; Altsybeev, Igor/0000-0002-8079-7026; Vickovic, Linda/0000-0002-9820-7960; Fernandez Tellez, Arturo/0000-0003-0152-4220; Riggi, Francesco/0000-0002-0030-8377; Melikyan, Yury/0000-0002-4165-505X; Giubilato, Piero/0000-0003-4358-5355; Fernandez Tellez, Arturo/0000-0001-5092-9748 FU Grid centres; Worldwide LHC Computing Grid (WLCG); State Committee of Science; World Federation of Scientists (WFS); Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq); Financiadora de Estudos e Projetos (FINEP); Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC); Chinese Ministry of Education (CMOE); Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council; Carlsberg Foundation; Danish National Research Foundation; European Research Council under the European Community; Helsinki Institute of Physics; Academy of Finland; French CNRS-IN2P3; Region Pays de Loire; Region Alsace; Region Auvergne; CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung and Technologie (BMBF); Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; National Research, Development and Innovation Office (NKFIH), Hungary; Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN); Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; Japan Society for the Promotion of Science (JSPS) KAKENHI; MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT); Direction General de Asuntos del Personal Academico (DGAPA), Mexico; Amerique Latine Formation academique - European Commission (ALFA-EC); EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM); Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics; National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation; Russian Academy of Sciences; Russian Federal Agency of Atomic Energy; Russian Federal Agency for Science and Innovation; Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, Republic of South Africa, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT); E-Infrastructure shared between Europe and Latin America (EELA); Ministerio de Economia y Competitividad (MINECO) of Spain; Xunta de Galicia (Conselleria de Education); Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN); Cubaenergia; Cuba; IAEA (International Atomic Energy Agency); Swedish Research Council (VR); Knut AMP; Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); United States Department of Energy; United States National Science Foundation; State of Texas; State of Ohio; Ministry of Science, Education and Sports of Croatia; Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru FX The ALICE Collaboration would like to thank all its engineers and technicians for their invaluable contributions to the construction of the experiment and the CERN accelerator teams for the outstanding performance of the LHC complex. The ALICE Collaboration gratefully acknowledges the resources and support provided by all Grid centres and the Worldwide LHC Computing Grid (WLCG) collaboration.; r The ALICE Collaboration acknowledges the following funding agencies for their support in building and running the ALICE detector: State Committee of Science, World Federation of Scientists (WFS) and Swiss Fonds Kidagan, Armenia; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico (CNPq), Financiadora de Estudos e Projetos (FINEP), Fundacao de Amparo a Pesquisa do Estado de Sao Paulo (FAPESP); National Natural Science Foundation of China (NSFC), the Chinese Ministry of Education (CMOE) and the Ministry of Science and Technology of China (MSTC); Ministry of Education and Youth of the Czech Republic; Danish Natural Science Research Council, the Carlsberg Foundation and the Danish National Research Foundation; The European Research Council under the European Community's Seventh Framework Programme; Helsinki Institute of Physics and the Academy of Finland; French CNRS-IN2P3, the 'Region Pays de Loire', 'Region Alsace', 'Region Auvergne' and CEA, France; German Bundesministerium fur Bildung, Wissenschaft, Forschung and Technologie (BMBF) and the Helmholtz Association; General Secretariat for Research and Technology, Ministry of Development, Greece; National Research, Development and Innovation Office (NKFIH), Hungary; Department of Atomic Energy and Department of Science and Technology of the Government of India; Istituto Nazionale di Fisica Nucleare (INFN) and Centro Fermi - Museo Storico della Fisica e Centro Studi e Ricerche "Enrico Fermi", Italy; Japan Society for the Promotion of Science (JSPS) KAKENHI and MEXT, Japan; Joint Institute for Nuclear Research, Dubna; National Research Foundation of Korea (NRF); Consejo Nacional de Cienca y Tecnologia (CONACYT), Direction General de Asuntos del Personal Academico (DGAPA), Mexico, Amerique Latine Formation academique - European Commission (ALFA-EC) and the EPLANET Program (European Particle Physics Latin American Network); Stichting voor Fundamenteel Onderzoek der Materie (FOM) and the Nederlandse Organisatie voor Wetenschappelijk Onderzoek (NWO), Netherlands; Research Council of Norway (NFR); National Science Centre, Poland; Ministry of National Education/Institute for Atomic Physics and National Council of Scientific Research in Higher Education (CNCSI-UEFISCDI), Romania; Ministry of Education and Science of Russian Federation, Russian Academy of Sciences, Russian Federal Agency of Atomic Energy, Russian Federal Agency for Science and Innovation and The Russian Foundation for Basic Research; Ministry of Education of Slovakia; Department of Science and Technology, Republic of South Africa, South Africa; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), E-Infrastructure shared between Europe and Latin America (EELA), Ministerio de Economia y Competitividad (MINECO) of Spain, Xunta de Galicia (Conselleria de Education), Centro de Aplicaciones Tecnologicas y Desarrollo Nuclear (CEADEN), Cubaenergia, Cuba, and IAEA (International Atomic Energy Agency); Swedish Research Council (VR) and Knut & Alice Wallenberg Foundation (KAW); Ukraine Ministry of Education and Science; United Kingdom Science and Technology Facilities Council (STFC); The United States Department of Energy, the United States National Science Foundation, the State of Texas, and the State of Ohio; Ministry of Science, Education and Sports of Croatia and Unity through Knowledge Fund, Croatia; Council of Scientific and Industrial Research (CSIR), New Delhi, India; Pontificia Universidad Catolica del Peru. NR 39 TC 1 Z9 1 U1 13 U2 50 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0370-2693 EI 1873-2445 J9 PHYS LETT B JI Phys. Lett. B PD JUL 10 PY 2016 VL 758 BP 389 EP 401 DI 10.1016/j.physletb.2016.05.027 PG 13 WC Astronomy & Astrophysics; Physics, Nuclear; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DN8LM UT WOS:000377330500053 ER PT J AU Somerville, L Bareno, J Jennings, P McGordon, A Lyness, C Bloom, I AF Somerville, L. Bareno, J. Jennings, P. McGordon, A. Lyness, C. Bloom, I. TI The Effect of Pre-Analysis Washing on the Surface Film of Graphite Electrodes SO ELECTROCHIMICA ACTA LA English DT Article DE Lithium-ion; XPS; post-test analysis; SEM; battery lifetime prediction; infra-red spectroscopy ID LITHIUM-ION BATTERIES; VINYLENE CARBONATE VC; PERFORMANCE; INTERPHASE; CHEMISTRY; CAPACITY; CELLS; ANODE; SEI AB Electrodes are routinely washed to remove electrolyte deposits, salt, and high boiling point solvents prior to analysis with surface-sensitive techniques. The effect of washing on the surface films of graphite electrodes from LiCoO2/graphite cells, which contained varying amounts of vinylene carbonate (VC), was investigated by comparing the microstructure and chemical composition. We confirmed that there are two different kinds of films on the surface of the electrodes: one at low and one at high VC content concentration. Far from being limited to remove extraneous salt deposits from the surface of the sample, DMC washing was found to completely remove one and to affect the composition of deeper strata in the other. (C) 2016 The Authors. Published by Elsevier Ltd. C1 [Somerville, L.; Bareno, J.; Bloom, I.] Argonne Natl Lab, 9700 S Cass Ave, Lemont, IL 60561 USA. [Somerville, L.; Jennings, P.; McGordon, A.] Univ Warwick, WMG, Coventry CV4 7AL, W Midlands, England. [Lyness, C.] Jaguar Land Rover, Banbury Rd, Warwick CV35 0XJ, England. RP Bloom, I (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Lemont, IL 60561 USA. EM ira.bloom@anl.gov FU Engineering and Physical Sciences Research Council (EPSRC); WMG centre HVM Catapult; Jaguar Land Rover Automotive PLC; U.S. Department of Energy (DOE), Office of Vehicle Technologies (VTO) [DE-AC02-06CH11357]; U.S. Department of Energy [W-31-109-Eng-38] FX We acknowledge support from the Engineering and Physical Sciences Research Council (EPSRC) and the WMG centre HVM Catapult. We also acknowledge support from Jaguar Land Rover Automotive PLC.; The work at Argonne National Laboratory was performed under the auspices of the U.S. Department of Energy (DOE), Office of Vehicle Technologies (VTO), under Contract No. DE-AC02-06CH11357.; The submitted issue has been created by the University of Chicago as Operator of Argonne National Laboratory ("Argonne") under Contract No. W-31-109-Eng-38 with the U.S. Department of Energy. The U.S. Government retains for itself, and others acting on its behalf, a paid-up, non-exclusive, irrevocable, worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the Government. NR 20 TC 1 Z9 1 U1 3 U2 20 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0013-4686 EI 1873-3859 J9 ELECTROCHIM ACTA JI Electrochim. Acta PD JUL 10 PY 2016 VL 206 BP 70 EP 76 DI 10.1016/j.electacta.2016.04.133 PG 7 WC Electrochemistry SC Electrochemistry GA DM7IY UT WOS:000376535100009 ER PT J AU Robinson, JW Zhou, Y Qu, J Erck, R Cosimbescu, L AF Robinson, Joshua W. Zhou, Yan Qu, Jun Erck, Robert Cosimbescu, Lelia TI Effects of star-shaped poly(alkyl methacrylate) arm uniformity on lubricant properties SO JOURNAL OF APPLIED POLYMER SCIENCE LA English DT Article DE friction; polyolefins; viscosity and viscoelasticity; wear and lubrication ID VISCOSITY-INDEX IMPROVERS; RADICAL POLYMERIZATION; MODIFIERS; POLYMERS AB Star-shaped poly(alkyl methacrylate)s (PAMAs) were prepared and blended into an additive-free engine oil to assess the structure-property relationship between macromolecular structure and lubricant performance. These additives were designed with a comparable number of repeating units per arm and the number of arms was varied between 3 and 6. Well-defined star-shaped PAMAs were synthesized by atom transfer radical polymerization (ATRP) via a core-first strategy from multi-functional head-groups. Observations of the polymer-oil blends suggest that stars with less than four arms are favorable as a viscosity index improver (VII), and molecular weight dominates viscosity-related effects over other structural features. Star-shaped PAMAs, as oil additives, effectively reduce the friction coefficient in both mixed and boundary lubrication regime. Several analogs outperformed commercial VIIs in both viscosity and friction performance. Increased wear rates were observed for these star-shaped PAMAs in the boundary lubrication regime suggesting pressure-sensitive conformations may exist. (c) 2016 Wiley Periodicals, Inc. J. Appl. Polym. Sci. 2016, 133, 43611. C1 [Robinson, Joshua W.; Cosimbescu, Lelia] Pacific NW Natl Lab, Richland, WA 99352 USA. [Zhou, Yan; Qu, Jun] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Erck, Robert] Argonne Natl Lab, Lemont, IL USA. RP Cosimbescu, L (reprint author), Pacific NW Natl Lab, Richland, WA 99352 USA. EM lelia.cosimbescu@pnnl.gov OI Qu, Jun/0000-0001-9466-3179 FU Office of Vehicle Technology (VT) of the U.S. Department of Energy (US DOE) [27573]; Department of Energy's Office of Biological and Environmental Research; U.S. DOE [DE_AC06-76RLO 1830] FX This project was funded by the Office of Vehicle Technology (VT) of the U.S. Department of Energy (US DOE), (under contract No. 27573). A portion of this research was performed using EMSL, a national scientific user facility sponsored by the Department of Energy's Office of Biological and Environmental Research and located at Pacific Northwest National Laboratory. PNNL is proudly operated by Battelle for the U.S. DOE (under Contract DE_AC06-76RLO 1830). The authors cordially acknowledge contributions from Anil K. Shukla (PNNL) for performing time-of-flight mass spectrometry and helpful discussions with Ewa Bardasz (Energetics). The authors would like to express their gratitude to David Gray (Evonik) and JoRuetta Ellington (Evonik) for their technical assistance and guidance throughout the project. Authors thank Afton Chemical for generously donating base oils for screening purposes. Author Contributions: J.W.R. synthesized and characterized the materials as well as measured viscosity. Y.Z. conducted friction measurements and analyzed results. R.E. conducted high temperature high shear experiments and analyzed results. J.Q. analyzed friction results. L.C. proposed the original concept, original material design, structured collaborations, and analyzed results. All authors reviewed this manuscript. NR 39 TC 1 Z9 1 U1 6 U2 29 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0021-8995 EI 1097-4628 J9 J APPL POLYM SCI JI J. Appl. Polym. Sci. PD JUL 10 PY 2016 VL 133 IS 26 AR 43611 DI 10.1002/app.43611 PG 11 WC Polymer Science SC Polymer Science GA DJ4KD UT WOS:000374172900024 ER PT J AU Gu, YB Cai, QX Chen, XL Zhuang, ZZ Zhou, H Zhuang, GL Zhong, X Mei, DH Wang, JG AF Gu Yong-Bing Cai Qiu-Xia Chen Xian-Lang Zhuang Zhen-Zhan Zhou Hu Zhuang Gui-Lin Zhong Xing Mei Dong-Hai Wang Jian-Guo TI Theoretical Insights into Role of Interface for CO Oxidation on Inverse Al2O3/Au(111) Catalysts SO ACTA PHYSICO-CHIMICA SINICA LA English DT Article DE Inverse catalyst; Au catalyst; CO oxidation; Density functional theory; Interfacial site ID SUPPORTED AU CATALYSTS; MINIMUM ENERGY PATHS; ELASTIC BAND METHOD; GOLD CATALYSTS; SELECTIVE HYDROGENATION; OXYGEN REDUCTION; SADDLE-POINTS; NANOPARTICLES; SURFACE; CROTONALDEHYDE AB Au catalysts supported on an oxide show excellent activity in CO oxidation under moderate conditions. Many experiments and theoretical calculations have shown the important role of the interface between Au and the oxide support during CO oxidation. Inverse catalysts provide an alternative way to probe the role of the interface. We used Al2O3/Au(111) as a model inverse catalyst in this study, and used density functional theory to investigate the properties of Al2O3/Au(111), the interface between Al2O3 and Au(111), the adsorption of O-2, and CO oxidation over Al2O3/Au(111). Our theoretical calculations show that small Al2O3 clusters are strongly bound on the Au(111) surface as a result of charge transfer. The results for O-2 adsorption on different sites indicate that the interfacial site is the most stable one because of simultaneous bonding of O-2 with Au and Al atoms. The full catalytic cycles for CO oxidation by O-2 by either an association or dissociation pathway were investigated. Oxidation in the association pathway is significantly easier than that in the dissociation one; the participation of CO makes dissociation of the adsorbed O-2 easier. This study reveals not only the origin of inverse catalysts for CO oxidation but also the role of the interface in CO oxidation on Au catalysts. C1 [Gu Yong-Bing; Cai Qiu-Xia; Chen Xian-Lang; Zhuang Zhen-Zhan; Zhou Hu; Zhuang Gui-Lin; Zhong Xing; Wang Jian-Guo] Zhejiang Univ Technol, Coll Chem Engn, Hangzhou 310032, Zhejiang, Peoples R China. [Mei Dong-Hai] Pacific Northwest Natl Lab, Inst Integrated Catalysis, Richland, WA 99352 USA. [Gu Yong-Bing] Lishui Univ, Dept Chem & Chem Engn, Lishui 323000, Zhejiang, Peoples R China. RP Wang, JG (reprint author), Zhejiang Univ Technol, Coll Chem Engn, Hangzhou 310032, Zhejiang, Peoples R China. EM jgw@zjut.edu.cn RI Mei, Donghai/A-2115-2012; Mei, Donghai/D-3251-2011 OI Mei, Donghai/0000-0002-0286-4182; FU National Key Basic Research Program of China (973) [2013CB733501]; National Natural Science Foundation of China [21176221, 21136001, 21101137, 21306169, 91334013] FX The project was supported by the National Key Basic Research Program of China (973) (2013CB733501) and National Natural Science Foundation of China (21176221, 21136001, 21101137, 21306169, 91334013). NR 53 TC 0 Z9 0 U1 7 U2 7 PU PEKING UNIV PRESS PI BEIJING PA PEKING UNIV, CHEMISTRY BUILDING, BEIJING 100871, PEOPLES R CHINA SN 1000-6818 J9 ACTA PHYS-CHIM SIN JI Acta Phys.-Chim. Sin. PD JUL 8 PY 2016 VL 32 IS 7 BP 1674 EP 1680 DI 10.3866/PKU.WHXB2016032806 PG 7 WC Chemistry, Physical SC Chemistry GA DX0UP UT WOS:000384081400013 ER PT J AU Daughton, AR Velappan, N Abeyta, E Priedhorsky, R Deshpande, A AF Daughton, Ashlynn R. Velappan, Nileena Abeyta, Esteban Priedhorsky, Reid Deshpande, Alina TI Novel Use of Flu Surveillance Data: Evaluating Potential of Sentinel Populations for Early Detection of Influenza Outbreaks SO PLOS ONE LA English DT Article ID UNITED-STATES; ADENOVIRUSES; ILLNESS; VIRUS AB Influenza causes significant morbidity and mortality each year, with 2-8% of weekly outpatient visits around the United States for influenza-like-illness (ILI) during the peak of the season. Effective use of existing flu surveillance data allows officials to understand and predict current flu outbreaks and can contribute to reductions in influenza morbidity and mortality. Previous work used the 2009-2010 influenza season to investigate the possibility of using existing military and civilian surveillance systems to improve early detection of flu outbreaks. Results suggested that civilian surveillance could help predict outbreak trajectory in local military installations. To further test that hypothesis, we compare pairs of civilian and military outbreaks in seven locations between 2000 and 2013. We find no predictive relationship between outbreak peaks or time series of paired outbreaks. This larger study does not find evidence to support the hypothesis that civilian data can be used as sentinel surveillance for military installations. We additionally investigate the effect of modifying the ILI case definition between the standard Department of Defense definition, a more specific definition proposed in literature, and confirmed Influenza A. We find that case definition heavily impacts results. This study thus highlights the importance of careful selection of case definition, and appropriate consideration of case definition in the interpretation of results. C1 [Daughton, Ashlynn R.; Abeyta, Esteban; Deshpande, Alina] Los Alamos Natl Lab, Analyt Intelligence & Technol Div, Los Alamos, NM USA. [Velappan, Nileena] Los Alamos Natl Lab, Biosci Div, Los Alamos, NM USA. [Priedhorsky, Reid] Los Alamos Natl Lab, High Performance Comp Div, Los Alamos, NM USA. RP Daughton, AR; Deshpande, A (reprint author), Los Alamos Natl Lab, Analyt Intelligence & Technol Div, Los Alamos, NM USA. EM adaughton@lanl.gov; deshpande_a@lanl.gov OI Velappan, Nileena/0000-0002-4488-9126 FU Defense Threat Reduction Agency - Joint Science and Technology Office [CB10092, DTRA10027-19082]; DTRA FX This project was funded by the Defense Threat Reduction Agency - Joint Science and Technology Office (Grant # CB10092, DTRA10027-19082) (http://www.dtra.mil/).; AFHSC provided data and technical assistance in interpreting it. We would like to specifically acknowledge Aaron Kite-Powell, Jean Chretien, Vivek Khatri and Angela Eick-Cost for assistance understanding data, and ideas about effective ways to analyze in R. We also would like to thank DTRA for funding this work. NR 37 TC 0 Z9 0 U1 1 U2 1 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1932-6203 J9 PLOS ONE JI PLoS One PD JUL 8 PY 2016 VL 11 IS 7 AR e0158330 DI 10.1371/journal.pone.0158330 PG 14 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR6IK UT WOS:000380005400042 PM 27391232 ER PT J AU Wu, GP Liu, XY Chen, XX Suh, HS Li, X Ren, JX Arges, CG Li, FX Jiang, Z Nealey, PF AF Wu, Guang-Peng Liu, Xiaoying Chen, Xuanxuan Suh, Hyo Seon Li, Xiao Ren, Jiaxing Arges, Christopher G. Li, Faxue Jiang, Zhang Nealey, Paul F. TI Directed Self-Assembly of Hierarchical Supramolecular Block Copolymer Thin Films on Chemical Patterns SO ADVANCED MATERIALS INTERFACES LA English DT Article ID DEVICE-ORIENTED STRUCTURES; DENSITY MULTIPLICATION; NANOPARTICLE ASSEMBLIES; DIBLOCK COPOLYMERS; LENGTH SCALES; LITHOGRAPHY; FABRICATION; NANOSTRUCTURES; NANOCOMPOSITES; GRAPHOEPITAXY C1 [Wu, Guang-Peng] Zhejiang Univ, Dept Polymer Sci & Engn, MOE Lab Macromol Synth & Funct, Hangzhou 310027, Zhejiang, Peoples R China. [Liu, Xiaoying; Chen, Xuanxuan; Li, Xiao; Ren, Jiaxing; Li, Faxue; Nealey, Paul F.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Suh, Hyo Seon; Arges, Christopher G.; Nealey, Paul F.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Jiang, Zhang] Argonne Natl Lab, Adv Photon Source, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Wu, GP (reprint author), Zhejiang Univ, Dept Polymer Sci & Engn, MOE Lab Macromol Synth & Funct, Hangzhou 310027, Zhejiang, Peoples R China.; Nealey, PF (reprint author), Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. EM gpwu@zju.edu.cn; nealey@uchicago.edu RI Arges, Christopher/G-9165-2014 OI Arges, Christopher/0000-0003-1703-8323 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, at the Materials Science Division, at the Center for Nanoscale Materials; "Hundred Talents Program" of Zhejiang University from China FX This work was supported in part by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, at the Materials Science Division, at the Center for Nanoscale Materials; and at the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science, all in Argonne National Laboratory under Contract No. DE-AC02-06CH11357. G.-P. Wu gratefully acknowledges the support of "Hundred Talents Program" of Zhejiang University from China. The authors thank Dr. S. McBride and Prof. H. M. Jaeger from the Department of Physics and James Franck Institute at the University of Chicago for helpful discussions. NR 39 TC 1 Z9 1 U1 14 U2 34 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2196-7350 J9 ADV MATER INTERFACES JI Adv. Mater. Interfaces PD JUL 8 PY 2016 VL 3 IS 13 AR 1600048 DI 10.1002/admi.201600048 PG 6 WC Chemistry, Multidisciplinary; Materials Science, Multidisciplinary SC Chemistry; Materials Science GA DR7BG UT WOS:000380054400018 ER PT J AU Schneidman-Duhovny, D Hammel, M Tainer, JA Sali, A AF Schneidman-Duhovny, Dina Hammel, Michal Tainer, John A. Sali, Andrej TI FoXS, FoXSDock and MultiFoXS: Single-state and multi-state structural modeling of proteins and their complexes based on SAXS profiles SO NUCLEIC ACIDS RESEARCH LA English DT Article ID X-RAY-SCATTERING; SMALL-ANGLE SCATTERING; DNA-REPAIR ENZYME; BIOLOGICAL MACROMOLECULES; POLYNUCLEOTIDE KINASE; DOCKING; COMPUTATION; RESOLUTION; CONFORMATIONS; BIOMOLECULES AB Small Angle X-ray Scattering (SAXS) is an increasingly common and useful technique for structural characterization of molecules in solution. A SAXS experiment determines the scattering intensity of a molecule as a function of spatial frequency, termed SAXS profile. Here, we describe three web servers for modeling atomic structures based on SAXS profiles. FoXS (Fast X-Ray Scattering) rapidly computes a SAXS profile of a given atomistic model and fits it to an experimental profile. FoXSDock docks two rigid protein structures based on a SAXS profile of their complex. MultiFoXS computes a population-weighted ensemble starting from a single input structure by fitting to a SAXS profile of the protein in solution. We describe the interfaces and capabilities of the servers (salilab.org/foxs), followed by demonstrating their application on Interleukin-33 (IL-33) and its primary receptor ST2. C1 [Schneidman-Duhovny, Dina; Sali, Andrej] Univ Calif San Francisco, Dept Pharmaceut Chem, Dept Bioengn & Therapeut Sci, San Francisco, CA 94143 USA. [Schneidman-Duhovny, Dina; Sali, Andrej] Univ Calif San Francisco, Calif Inst Quantitat Biosci QB3, San Francisco, CA 94143 USA. [Hammel, Michal; Tainer, John A.] Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging, Berkeley, CA 94720 USA. [Tainer, John A.] Univ Texas MD Anderson Canc Ctr, Dept Mol & Cellular Oncol, Houston, TX 77030 USA. RP Schneidman-Duhovny, D; Sali, A (reprint author), Univ Calif San Francisco, Dept Pharmaceut Chem, Dept Bioengn & Therapeut Sci, San Francisco, CA 94143 USA.; Schneidman-Duhovny, D; Sali, A (reprint author), Univ Calif San Francisco, Calif Inst Quantitat Biosci QB3, San Francisco, CA 94143 USA. EM dina.schneidman@mail.huji.ac.il; sali@salilab.org FU National Institutes of Health (NIH) [CA92584, MINOS GM105404]; United States Department of Energy program IDAT; Biogen and Janssen Pharmaceutica; NIH [R01 GM083960, P41 GM109824] FX SAXS at the Advanced Light Source SIBLYS beamline in supported by National Institutes of Health (NIH) grants CA92584 and MINOS GM105404, United States Department of Energy program IDAT, plus industrial partners Biogen and Janssen Pharmaceutica. This work was supported by grants from the NIH R01 GM083960 and NIH P41 GM109824. NR 37 TC 6 Z9 6 U1 5 U2 7 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JUL 8 PY 2016 VL 44 IS W1 BP W424 EP W429 DI 10.1093/nar/gkw389 PG 6 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DR3FA UT WOS:000379786800070 PM 27151198 ER PT J AU Veltri, D Wight, MM Crouch, JA AF Veltri, Daniel Wight, Martha Malapi Crouch, Jo Anne TI SimpleSynteny: a web-based tool for visualization of microsynteny across multiple species SO NUCLEIC ACIDS RESEARCH LA English DT Article ID PLANT GENOMES; SYNTENY; HOMOLOGY; FUNGI AB Defining syntenic relationships among orthologous gene clusters is a frequent undertaking of biologists studying organismal evolution through comparative genomic approaches. With the increasing availability of genome data made possible through next-generation sequencing technology, there is a growing need for user-friendly tools capable of assessing synteny. Here we present SimpleSynteny, a new web-based platform capable of directly interrogating collinearity of local genomic neighbors across multiple species in a targeted manner. SimpleSynteny provides a pipeline for evaluating the synteny of a preselected set of gene targets across multiple organismal genomes. An emphasis has been placed on ease-of-use, and users are only required to submit FASTA files for their genomes and genes of interest. SimpleSynteny then guides the user through an iterative process of exploring and customizing genomes individually before combining them into a final high-resolution figure. Because the process is iterative, it allows the user to customize the organization of multiple contigs and incorporate knowledge from additional sources, rather than forcing complete dependence on the computational predictions. Additional tools are provided to help the user identify which contigs in a genome assembly contain gene targets and to optimize analyses of circular genomes. C1 [Veltri, Daniel; Wight, Martha Malapi; Crouch, Jo Anne] ARS, Systemat Mycol & Microbiol Lab, USDA, 10300 Baltimore Ave,Bldg 10A, Beltsville, MD 20705 USA. [Veltri, Daniel] Oak Ridge Inst Sci & Educ, ARS Res Program, MC-100-44 POB 117, Oak Ridge, TN 37831 USA. [Wight, Martha Malapi] Anim & Plant Hlth Inspect Serv, Plant Germplasm Quarantine Program, USDA, 9901 Powder Mill Rd,Bldg 580, Beltsville, MD 20705 USA. RP Crouch, JA (reprint author), ARS, Systemat Mycol & Microbiol Lab, USDA, 10300 Baltimore Ave,Bldg 10A, Beltsville, MD 20705 USA. EM joanne.crouch@ars.usda.gov OI Crouch, Jo Anne/0000-0001-6886-8090; Veltri, Daniel/0000-0002-6101-6693 FU United States Department of Agriculture (USDA)-Animal and Plant Health Inspection Service Farm Bill Program [10201, 10007]; USDA-Agricultural Research Service (ARS) [8042-22000-279-00D]; USDA-ARS Floriculture and Nursery Research Initiative [0500-00059-001]; United States Department of Energy (DOE); USDA through the Oak Ridge Institute for Science and Education ARS Research Participation Program [DOE] [DE-AC05-06OR23100]; Class of USDA-ARS Headquarters Research Associate Award; U.S. Department of Agriculture, Agricultural Research Service FX 2013-2015 United States Department of Agriculture (USDA)-Animal and Plant Health Inspection Service Farm Bill 10201 and 10007 Program funds (to J.A.C.); USDA-Agricultural Research Service (ARS) [project 8042-22000-279-00D]; USDA-ARS Floriculture and Nursery Research Initiative [project 0500-00059-001 to J.A.C.]. Inter-agency fellowship agreement between the United States Department of Energy (DOE) and the USDA through the Oak Ridge Institute for Science and Education ARS Research Participation Program Fellowship [DOE contract DE-AC05-06OR23100]; Class of 2013 USDA-ARS Headquarters Research Associate Award (to J.A.C.). Funding for open access charge: U.S. Department of Agriculture, Agricultural Research Service. NR 16 TC 2 Z9 2 U1 2 U2 6 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-1048 EI 1362-4962 J9 NUCLEIC ACIDS RES JI Nucleic Acids Res. PD JUL 8 PY 2016 VL 44 IS W1 BP W41 EP W45 DI 10.1093/nar/gkw330 PG 5 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DR3FA UT WOS:000379786800008 PM 27141960 ER PT J AU Das, SD Dhochak, K Tripathi, V AF Das, S. D. Dhochak, K. Tripathi, V. TI Kondo route to spin inhomogeneities in the honeycomb Kitaev model SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC-IMPURITIES AB Paramagnetic impurities in a quantum spin liquid give rise to Kondo effects with highly unusual properties. We have studied the effect of locally coupling a paramagnetic impurity with the spin-1/2 honeycomb Kitaev model in its gapless spin-liquid phase. The ( impurity) scaling equations are found to be insensitive to the sign of the coupling. The weak and strong coupling fixed points are stable, with the latter corresponding to a noninteracting vacancy and an interacting, spin-1 defect for the antiferromagnetic and ferromagnetic cases, respectively. The ground state in the strong coupling limit in both cases has a nontrivial topology associated with a finite Z(2) flux at the impurity site. For the antiferromagnetic case, this result has been obtained straightforwardly owing to the integrability of the Kitaev model with a vacancy. The strong-coupling limit of the ferromagnetic case is, however, nonintegrable, and we address this problem through exact-diagonalization calculations with finite Kitaev fragments. Our exact diagonalization calculations indicate that the weak-to-strong coupling transition and the topological phase transition occur rather close to each other and are possibly coincident. We also find an intriguing similarity between the magnetic response of the defect and the impurity susceptibility in the two-channel Kondo problem. C1 [Das, S. D.] Univ Bristol, Sch Phys, HH Wills Phys Lab, Tyndall Ave, Bristol BS8 1TL, Avon, England. [Dhochak, K.] Weizmann Inst Sci, Dept Condensed Matter Phys, IL-76100 Rehovot, Israel. [Tripathi, V.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Lemont, IL 60439 USA. [Tripathi, V.] Tata Inst Fundamental Res, Dept Theoret Phys, Homi Bhabha Rd, Bombay 400005, Maharashtra, India. RP Das, SD (reprint author), Univ Bristol, Sch Phys, HH Wills Phys Lab, Tyndall Ave, Bristol BS8 1TL, Avon, England. FU Argonne National Laboratory; University of Chicago Center in Delhi; DST (India) Swarnajayanti [DST/SJF/PSA-0212012-13]; Cambridge Commonwealth Trust (CCT) FX We are grateful for useful discussions with K. Damle and M. Vojta. V.T. acknowledges financial support from Argonne National Laboratory, the University of Chicago Center in Delhi, and DST (India) Swarnajayanti (Grant No. DST/SJF/PSA-0212012-13). S.D.D. acknowledges the financial support provided by Cambridge Commonwealth Trust (CCT) and hospitality provided by DTP (TIFR). NR 29 TC 0 Z9 0 U1 1 U2 2 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 8 PY 2016 VL 94 IS 2 AR 024411 DI 10.1103/PhysRevB.94.024411 PG 9 WC Physics, Condensed Matter SC Physics GA DR2DR UT WOS:000379715700003 ER PT J AU Reyes-Lillo, SE Rangel, T Bruneval, F Neaton, JB AF Reyes-Lillo, Sebastian E. Rangel, Tonatiuh Bruneval, Fabien Neaton, Jeffrey B. TI Effects of quantum confinement on excited state properties of SrTiO3 from ab initio many-body perturbation theory SO PHYSICAL REVIEW B LA English DT Article ID OPTICAL-PROPERTIES; QUASI-PARTICLE; ELECTRONIC-STRUCTURE; HYDROGEN-PRODUCTION; GREENS-FUNCTION; BAND-STRUCTURE; WATER; SEMICONDUCTORS; EXCITATIONS; INSULATORS AB The Ruddlesden-Popper (RP) homologous series Srn+1TinO3n+1 provides a useful template for the study and control of the effects of dimensionality and quantum confinement on the excited state properties of the complex oxide SrTiO3. We use ab initio many-body perturbation theory within the GW approximation and the Bethe-Salpeter equation approach to calculate quasiparticle energies and absorption spectra of Srn+1TinO3n+1 for n = 1-5 and infinity. Our computed direct and indirect optical gaps are in excellent agreement with spectroscopic measurements. The calculated optical spectra reproduce the main experimental features and reveal excitonic structure near the gap edge. We find that electron-hole interactions are important across the series, leading to significant exciton binding energies that increase for small n and reach a value of 330 meV for n = 1, a trend attributed to increased quantum confinement. We find that the lowest-energy singlet exciton of Sr2TiO4 (n = 1) localizes in the two-dimensional plane defined by the TiO2 layer, and we explain the origin of its localization. C1 [Reyes-Lillo, Sebastian E.; Rangel, Tonatiuh; Bruneval, Fabien; Neaton, Jeffrey B.] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Reyes-Lillo, Sebastian E.; Rangel, Tonatiuh; Bruneval, Fabien; Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bruneval, Fabien] CEA, DEN, Serv Rech Met Phys, F-91191 Gif Sur Yvette, France. [Neaton, Jeffrey B.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. RP Reyes-Lillo, SE (reprint author), Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.; Reyes-Lillo, SE (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RI Bruneval, Fabien/C-6923-2009 OI Bruneval, Fabien/0000-0003-0885-8960 FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy; Laboratory Directed Research and Development Program at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231]; SciDAC Program on Excited State Phenomena in Energy Materials; Office of Science of the U.S. Department of Energy FX S.E.R.-L. thanks R. F. Berger and T. Birol for valuable discussions. Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy, and Laboratory Directed Research and Development Program at the Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231. T.R. acknowledges support from the SciDAC Program on Excited State Phenomena in Energy Materials. F.B. acknowledges the Enhanced Eurotalent program and the France Berkeley Fund for supporting his sabbatical leave in UC Berkeley. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy. NR 53 TC 0 Z9 0 U1 4 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 8 PY 2016 VL 94 IS 4 AR 041107 DI 10.1103/PhysRevB.94.041107 PG 6 WC Physics, Condensed Matter SC Physics GA DR2FF UT WOS:000379719700002 ER PT J AU Vujanovic, G Paquet, JF Denicol, GS Luzum, M Jeon, S Gale, C AF Vujanovic, Gojko Paquet, Jean-Francois Denicol, Gabriel S. Luzum, Matthew Jeon, Sangyong Gale, Charles TI Electromagnetic radiation as a probe of the initial state and of viscous dynamics in relativistic nuclear collisions SO PHYSICAL REVIEW C LA English DT Article ID HEAVY-ION COLLISIONS; HADRONIC GAS; THERMODYNAMICS; DILEPTON; FLOW AB The penetrating nature of electromagnetic signals makes them suitable probes to explore the properties of the strongly interacting medium created in relativistic nuclear collisions. We examine the effects of the initial conditions and shear relaxation time on the spectra and flow coefficients of electromagnetic probes, using an event-by-event 3+1-dimensional viscous hydrodynamic simulation (MUSIC). C1 [Vujanovic, Gojko; Paquet, Jean-Francois; Denicol, Gabriel S.; Jeon, Sangyong; Gale, Charles] McGill Univ, Dept Phys, 3600 Rue Univ, Montreal, PQ H3A 2T8, Canada. [Vujanovic, Gojko] Ohio State Univ, Dept Phys, 191 West Woodruff Ave, Columbus, OH 43210 USA. [Paquet, Jean-Francois] SUNY Stony Brook, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Denicol, Gabriel S.] Brookhaven Natl Lab, Dept Phys, Bldg 510A, Upton, NY 11973 USA. [Luzum, Matthew] Univ Santiago de Compostela, Dept Fis Particulas, E-15706 Santiago De Compostela, Galicia, Spain. [Luzum, Matthew] Univ Santiago de Compostela, IGFAE, E-15706 Santiago De Compostela, Galicia, Spain. [Luzum, Matthew] Univ Sao Paulo, Inst Fis, Rua Matao Travessa R 187, BR-05508090 Sao Paulo, Brazil. RP Vujanovic, G (reprint author), McGill Univ, Dept Phys, 3600 Rue Univ, Montreal, PQ H3A 2T8, Canada. RI Silveira Denicol, Gabriel/L-5048-2016; Luzum, Matthew/C-4986-2015 OI Luzum, Matthew/0000-0002-0367-7055 FU Natural Sciences and Engineering Research Council of Canada; Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, of the U.S. Department of Energy [DE-AC02-98CH10886, DE-AC02-05CH11231, DE-SC0004286]; Fonds de Recherche du Quebec-Nature et les Technologies (FRQNT); Canadian Institute for Nuclear Physics; Seymour Schulich Scholarship; Banting Fellowship from the Government of Canada; Calcul Quebec; Compute Canada; Canada Foundation for Innovation (CFI); National Science and Engineering Research Council (NSERC); NanoQuebec FX We are happy to acknowledge helpful discussions with C. Shen and B. Schenke. This work was supported in part by the Natural Sciences and Engineering Research Council of Canada, and in part by the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Division of Nuclear Physics, of the U.S. Department of Energy under Contracts No. DE-AC02-98CH10886, DE-AC02-05CH11231, and DE-SC0004286. G.V. acknowledges support by the Fonds de Recherche du Quebec-Nature et les Technologies (FRQNT), the Canadian Institute for Nuclear Physics, and by the Seymour Schulich Scholarship, while G.S.D. acknowledges support through a Banting Fellowship from the Government of Canada. Computations were performed on the Guillimin supercomputer at McGill University under the auspices of Calcul Quebec and Compute Canada. The operation of Guillimin is funded by the Canada Foundation for Innovation (CFI), the National Science and Engineering Research Council (NSERC), NanoQuebec, and the Fonds de Recherche du Quebec-Nature et les Technologies (FRQNT). NR 47 TC 4 Z9 4 U1 6 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUL 8 PY 2016 VL 94 IS 1 AR 014904 DI 10.1103/PhysRevC.94.014904 PG 11 WC Physics, Nuclear SC Physics GA DR2FY UT WOS:000379721600002 ER PT J AU Suzuki, M AF Suzuki, Mahiko TI Composite gauge-bosons made of fermions SO PHYSICAL REVIEW D LA English DT Article ID INTERMEDIATE VECTOR BOSON; CHIRAL-SYMMETRY-BREAKING; MASSLESS PARTICLES; PHASE-TRANSITION; HIGGS THEORY; FIELDS; MODEL; COLLIDER; EQUIVALENCE; CONFINEMENT AB We construct a class of Abelian and non-Abelian local gauge theories that consist only of matter fields of fermions. The Lagrangian is local and does not contain an auxiliary vector field nor a subsidiary condition on the matter fields. It does not involve an extra dimension nor supersymmetry. This Lagrangian can be extended to non-Abelian gauge symmetry only in the case of SU(2) doublet matter fields. We carry out an explicit diagrammatic computation in the leading 1/N order to show that massless spin-one bound states appear with the correct gauge coupling. Our diagram calculation exposes the dynamical features that cannot be seen in the formal auxiliary vector-field method. For instance, it shows that the s-wave fermion-antifermion interaction in the S-3(1) channel ((psi) over bar gamma(mu)psi) alone cannot form the bound gauge bosons; the fermion-antifermion pairs must couple to the d-wave state too. One feature common to our class of Lagrangian is that the Noether current does not exist. Therefore it evades possible conflict with the no-go theorem of Weinberg and Witten on the formation of the non-Abelian gauge bosons. C1 [Suzuki, Mahiko] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Suzuki, Mahiko] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Suzuki, M (reprint author), Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA.; Suzuki, M (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. FU Office of Science, Division of High Energy Physics, of the U.S. Department of Energy [DE-AC02-05CH11231] FX I am thankful to Professor Pei-Ming Ho for bringing my attention to the possible relevance or irrelevance of the auxiliary vector-field trick to compositeness of a gauge boson at an early stage. During the course of this work, I have benefited from the useful conversation with Professor Korkut Bardakci. After I proceeded substantially in this research, I learned from Professor Eliezer Rabinovic about some aspects of the subject which I had not been familiar with. Thanks is also due to Professor E. Kh. Akhmedov for useful communications that directed me to many early works. This work was supported by the Office of Science, Division of High Energy Physics, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 47 TC 1 Z9 1 U1 0 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 8 PY 2016 VL 94 IS 2 AR 025010 DI 10.1103/PhysRevD.94.025010 PG 21 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DR2GV UT WOS:000379723900006 ER PT J AU Bavishi, K Laursen, T Martinez, KL Moller, BL Della Pia, EA AF Bavishi, Krutika Laursen, Tomas Martinez, Karen L. Moller, Birger Lindberg Della Pia, Eduardo Antonio TI Application of nanodisc technology for direct electrochemical investigation of plant cytochrome P450s and their NADPH P450 oxidoreductase SO SCIENTIFIC REPORTS LA English DT Article ID CYANOGENIC GLUCOSIDE; MICROFLUIDIC PLATFORM; DYNAMIC METABOLONS; CHEMICAL-SYNTHESIS; MEMBRANE-PROTEINS; DRUG-METABOLISM; REDUCTASE; FILMS; BIOSYNTHESIS; EXPRESSION AB Direct electrochemistry of cytochrome P450 containing systems has primarily focused on investigating enzymes from microbes and animals for bio-sensing applications. Plant P450s receive electrons from NADPH P450 oxidoreductase (POR) to orchestrate the bio-synthesis of a plethora of commercially valuable compounds. In this report, full length CYP79A1, CYP71E1 and POR of the dhurrin pathway in Sorghum bicolor were reconstituted individually in nanoscale lipid patches, "nanodiscs", and directly immobilized on unmodified gold electrodes. Cyclic voltammograms of CYP79A1 and CYP71E1 revealed reversible redox peaks with average midpoint potentials of 80 +/- 5 mV and 72 +/- 5 mV vs. Ag/AgCl, respectively. POR yielded two pairs of redox peaks with midpoint potentials of 90 +/- 5 mV and -300 +/- 10 mV, respectively. The average heterogeneous electron transfer rate constant was calculated to be similar to 1.5 s(-1). POR was electro-catalytically active while the P450s generated hydrogen peroxide (H2O2). These nanodisc-based investigations lay the prospects and guidelines for construction of a simplified platform to perform mediator-free, direct electrochemistry of non-engineered cytochromes P450 under native-like conditions. It is also a prelude for driving plant P450 systems electronically for simplified and cost-effective screening of potential substrates/inhibitors and fabrication of nano-bioreactors for synthesis of high value natural products. C1 [Bavishi, Krutika; Laursen, Tomas; Moller, Birger Lindberg] Univ Copenhagen, Dept Plant & Environm Sci, Plant Biochem Lab, Thorvaldsensvej 40, DK-1871 Frederiksberg C, Denmark. [Bavishi, Krutika; Laursen, Tomas; Moller, Birger Lindberg] Univ Copenhagen, VILLUM Res Ctr Plant Plast, Thorvaldsensvej 40, DK-1871 Frederiksberg C, Denmark. [Bavishi, Krutika; Laursen, Tomas; Martinez, Karen L.; Moller, Birger Lindberg] Univ Copenhagen, Ctr Synthet Biol BioSYNergy, Thorvaldsensvej 40, DK-1871 Frederiksberg C, Denmark. [Laursen, Tomas] Joint BioEnergy Inst, Feedstocks Div, Emeryville, CA 94608 USA. [Martinez, Karen L.; Della Pia, Eduardo Antonio] Univ Copenhagen, Dept Chem, Bionanotechnol Lab, Univ Pk 5, DK-2100 Copenhagen, Denmark. [Martinez, Karen L.; Della Pia, Eduardo Antonio] Univ Copenhagen, Nanosci Ctr, Univ Pk 5, DK-2100 Copenhagen, Denmark. RP Moller, BL (reprint author), Univ Copenhagen, Dept Plant & Environm Sci, Plant Biochem Lab, Thorvaldsensvej 40, DK-1871 Frederiksberg C, Denmark.; Moller, BL (reprint author), Univ Copenhagen, VILLUM Res Ctr Plant Plast, Thorvaldsensvej 40, DK-1871 Frederiksberg C, Denmark.; Moller, BL (reprint author), Univ Copenhagen, Ctr Synthet Biol BioSYNergy, Thorvaldsensvej 40, DK-1871 Frederiksberg C, Denmark. EM blm@plen.ku.dk RI martinez, karen/J-5933-2013; Moller, Birger Lindberg/H-2657-2014; bagheri, amir/C-3274-2017; OI martinez, karen/0000-0003-0932-8080; Moller, Birger Lindberg/0000-0002-3252-3119; Laursen, Tomas/0000-0002-6493-2259; Bavishi, Krutika/0000-0002-8638-3887 FU People Programme (Marie Curie Actions) of the European Union's seventh framework programme (FP7) under REA [289217]; VILLUM foundation [95-300-73023]; Danish Research Council [FTP-12-132506]; Center for Synthetic Biology "bioSYNergy" by the UCPH Excellence Program for Interdisciplinary Research; ERC Advanced Grant [ERC-2012-ADG_20120314, 323034] FX K.B. was supported by the People Programme (Marie Curie Actions) of the European Union's seventh framework programme FP7/2007-2013/under REA grant agreement number 289217. T.L. is the recipient of a fellowship awarded by the VILLUM foundation (Project No: 95-300-73023). E.D.A.P. acknowledges a fellowship awarded by the Danish Research Council (FTP-12-132506). This work was supported by a grant from the VILLUM Foundation to the research center of excellence 'Plant Plasticity' (to B.L.M.), by the Center for Synthetic Biology "bioSYNergy" supported by the UCPH Excellence Program for Interdisciplinary Research (to B.L.M.), and by an ERC Advanced Grant to B.L.M. (ERC-2012-ADG_20120314, Project No: 323034). We thank Prof. Gianfranco Gilardi (University of Turin) and Aditi Das (University of Illinois at Urbana-Champaign) for their valuable feedback on the cyclic voltammetry experiments. NR 57 TC 1 Z9 1 U1 19 U2 27 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 8 PY 2016 VL 6 AR 29459 DI 10.1038/srep29459 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR0UT UT WOS:000379623100001 PM 27386958 ER PT J AU Devanathan, R Chase-Woods, D Shin, Y Gotthold, DW AF Devanathan, Ram Chase-Woods, Dylan Shin, Yongsoon Gotthold, David W. TI Molecular Dynamics Simulations Reveal that Water Diffusion between Graphene Oxide Layers is Slow SO SCIENTIFIC REPORTS LA English DT Article ID GRAPHITE OXIDE; ATOMISTIC SIMULATION; NAFION MEMBRANE; DESALINATION; TECHNOLOGY; PERMEATION; SEPARATION; REDUCTION; HYDRATION; INSIGHTS AB Membranes made of stacked layers of graphene oxide (GO) hold the tantalizing promise of revolutionizing desalination and water filtration if selective transport of molecules can be controlled. We present the findings of an integrated study that combines experiment and molecular dynamics simulation of water intercalated between GO layers. We simulated a range of hydration levels from 1 wt.% to 23.3 wt.% water. The interlayer spacing increased upon hydration from 0.8 nm to 1.1 nm. We also synthesized GO membranes that showed an increase in layer spacing from about 0.7 nm to 0.8 nm and an increase in mass of about 15% on hydration. Water diffusion through GO layers is an order of magnitude slower than that in bulk water, because of strong hydrogen bonded interactions. Most of the water molecules are bound to OH groups even at the highest hydration level. We observed large water clusters that could span graphitic regions, oxidized regions and holes that have been experimentally observed in GO. Slow interlayer diffusion can be consistent with experimentally observed water transport in GO if holes lead to a shorter path length than previously assumed and sorption serves as a key rate-limiting step. C1 [Devanathan, Ram; Chase-Woods, Dylan; Shin, Yongsoon; Gotthold, David W.] Pacific Northwest Natl Lab, Richland, WA 99352 USA. RP Devanathan, R (reprint author), Pacific Northwest Natl Lab, Richland, WA 99352 USA. EM ram.devanathan@pnnl.gov FU Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX The research described in this paper is part of the Materials Synthesis and Simulation across Scales (MS3) Initiative at Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program at PNNL, a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy. This work was performed using the resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 46 TC 3 Z9 3 U1 31 U2 73 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 8 PY 2016 VL 6 AR 29484 DI 10.1038/srep29484 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR2YD UT WOS:000379768900001 PM 27388562 ER PT J AU Jones, J Xiong, HF Delariva, AT Peterson, EJ Pham, H Challa, SR Qi, GS Oh, S Wiebenga, MH Hernandez, XIP Wang, Y Datye, AK AF Jones, John Xiong, Haifeng DeLaRiva, Andrew T. Peterson, Eric J. Hien Pham Challa, Sivakumar R. Qi, Gongshin Oh, Se Wiebenga, Michelle H. Hernandez, Xavier Isidro Pereira Wang, Yong Datye, Abhaya K. TI Thermally stable single-atom platinum-on-ceria catalysts via atom trapping SO SCIENCE LA English DT Article ID DIESEL OXIDATION CATALYSTS; WATER-GAS SHIFT; CO OXIDATION; OXIDIZING CONDITIONS; METAL-CATALYSTS; NANOPARTICLES; SURFACE; PD; ATMOSPHERES; DISPERSION AB Catalysts based on single atoms of scarce precious metals can lead to more efficient use through enhanced reactivity and selectivity. However, single atoms on catalyst supports can be mobile and aggregate into nanoparticles when heated at elevated temperatures. High temperatures are detrimental to catalyst performance unless these mobile atoms can be trapped. We used ceria powders having similar surface areas but different exposed surface facets. When mixed with a platinum/aluminum oxide catalyst and aged in air at 800 degrees C, the platinum transferred to the ceria and was trapped. Polyhedral ceria and nanorods were more effective than ceria cubes at anchoring the platinum. Performing synthesis at high temperatures ensures that only the most stable binding sites are occupied, yielding a sinter-resistant, atomically dispersed catalyst. C1 [Jones, John; Xiong, Haifeng; DeLaRiva, Andrew T.; Peterson, Eric J.; Hien Pham; Challa, Sivakumar R.; Datye, Abhaya K.] Univ New Mexico, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA. [Jones, John; Xiong, Haifeng; DeLaRiva, Andrew T.; Peterson, Eric J.; Hien Pham; Challa, Sivakumar R.; Datye, Abhaya K.] Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA. [Qi, Gongshin; Oh, Se; Wiebenga, Michelle H.] Gen Motors Global R&D, 30500 Mound Rd, Warren, MI 48090 USA. [Hernandez, Xavier Isidro Pereira; Wang, Yong] Washington State Univ, Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. [Wang, Yong] Pacific NW Natl Lab, Ins Integrated Catalysis, Richland, WA 99354 USA. RP Datye, AK (reprint author), Univ New Mexico, Dept Chem & Biol Engn, Albuquerque, NM 87131 USA.; Datye, AK (reprint author), Univ New Mexico, Ctr Microengn Mat, Albuquerque, NM 87131 USA. EM datye@unm.edu RI Pereira Hernandez, Xavier Isidro/E-2356-2017 OI Pereira Hernandez, Xavier Isidro/0000-0002-7020-0011 FU NSF GOALI grant [CBET-1438765]; General Motors Global RD; U.S. Department of Energy [DE-FG02-05ER15712]; Center for Biorenewable Chemicals - NSF [EEC-0813570] FX Supported by NSF GOALI grant CBET-1438765 (J.J., H.X., S.R.C., A.K.D.), General Motors Global R&D (G.Q., S.O., and M.H.W.), U.S. Department of Energy grant DE-FG02-05ER15712 (A.T.D., E.J.P., A.K.D., X.I.P.H., and Y.W.), and the Center for Biorenewable Chemicals funded by NSF grant EEC-0813570 (H.X., H.P., and A.K.D.). This work made use of the JEOL JEM-ARM200CF at the University of Illinois at Chicago. We thank A. Nicholls for recording the AC-STEM images and D. Kunwar for assistance in catalyst preparation. NR 29 TC 21 Z9 21 U1 176 U2 286 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 0036-8075 EI 1095-9203 J9 SCIENCE JI Science PD JUL 8 PY 2016 VL 353 IS 6295 BP 150 EP 154 DI 10.1126/science.aaf8800 PG 5 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DQ4XP UT WOS:000379208400034 PM 27387946 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van Parijs, I Barria, P Brun, H Caillol, C Clerbaux, B De Lentdecker, G Fasanella, G Favart, L Grebenyuk, A Karapostoli, G Lenzi, T Leonard, A Maerschalk, T Marinov, A Pernie, L Randle-Conde, A Reis, T Seva, T Vander Velde, C Vanlaer, P Yonamine, R Zenoni, F Zhang, F Beernaert, K Benucci, L Cimmino, A Crucy, S Dobur, D Fagot, A Garcia, G Gul, M Mccartin, J Rios, AAO Poyraz, D Ryckbosch, D Salva, S Sigamani, M Strobbe, N Tytgat, M Van Driessche, W Yazgan, E Zaganidis, N Basegmez, S Beluffi, C Bondu, O Brochet, S Bruno, G Caudron, A Ceard, L Da Silveira, GG Delaere, C Favart, D Forthomme, L Giammanco, A Hollar, J Jafari, A Jez, P Komm, M Lemaitre, V Mertens, A Musich, M Nuttens, C Perrini, L Pin, A Piotrzkowski, K Popov, A Quertenmont, L Selvaggi, M Marono, MV Beliy, N Hammad, GH Alda, WL Alves, FL Alves, GA Brito, L Martins, MC Hamer, M Hensel, C Herrera, CM Moraes, A Pol, ME Teles, PR Das Chagas, EBB Carvalho, W Chinellato, J Custodio, A Da Costa, EM Damiao, DD Martins, CD De Souza, SF Guativa, LMH Malbouisson, H Figueiredo, DM Mundim, L Nogima, H Da Silva, WLP Santoro, A Sznajder, A Manganote, EJT Pereira, AV Ahuja, S Bernardes, CA Santos, AD Dogra, S Tomei, TRFP Gregores, EM Mercadante, PG Moon, CS Novaes, SF Padula, SS Aba, DR Vargas, JCR Aleksandrov, A Hadjiiska, R Iaydjiev, P Rodozov, M Stoykova, S Sultanov, G Vutova, M Dimitrov, A Glushkov, I Litov, L Pavlov, B Petkov, P Ahmad, M Bian, JG Chen, GM Chen, HS Chen, M Cheng, T Du, R Jiang, CH Plestina, R Romeo, F Shaheen, SM Spiezia, A Tao, J Wang, C Wang, Z Zhang, H Asawatangtrakuldee, C Ban, Y Li, Q Liu, S Mao, Y Qian, SJ Wang, D Xu, Z Avila, C Cabrera, A Sierra, LFC Florez, C Gomez, JP Moreno, BG Sanabria, JC Godinovic, N Lelas, D Puljak, I Cipriano, PMR Antunovic, Z Kovac, M Brigljevic, V Kadija, K Luetic, J Micanovic, S Sudic, L Attikis, A Mavromanolakis, G Mousa, J Nicolaou, C Ptochos, F Razis, PA Rykaczewski, H Bodlak, M Finger, M Finger, M El Sawy, M El-Khateeb, E Elkafrawy, T Mohamed, A Salama, E Calpas, B Kadastik, M Murumaa, M Raidal, M Tiko, A Veelken, C Eerola, P Pekkanen, J Voutilainen, M Harkonen, J Karimaki, V Kinnunen, R Lampen, T Lassila-Perini, K Lehti, S Linden, T Luukka, P Maenpaa, T Peltola, T Tuominen, E Tuominiemi, J Tuovinen, E Wendland, L Talvitie, J Tuuva, T Besancon, M Couderc, F Dejardin, M Denegri, D Fabbro, B Faure, JL Favaro, C Ferri, F Ganjour, S Givernaud, A Gras, P de Monchenault, GH Jarry, P Locci, E Machet, M Malcles, J Rander, J Rosowsky, A Titov, M Zghiche, A Antropov, I Baffioni, S Beaudette, F Busson, P Cadamuro, L Chapon, E Charlot, C Dahms, T Davignon, O Filipovic, N Florent, A de Cassagnac, RG Lisniak, S Mastrolorenzo, L Mine, P Naranjo, IN Nguyen, M Ochando, C Ortona, G Paganini, P Pigard, P Regnard, S Salerno, R Sauvan, JB Sirois, Y Strebler, T Yilmaz, Y Zabi, A Agram, JL Andrea, J Aubin, A Bloch, D Brom, JM Buttignol, M Chabert, EC Chanon, N Collard, C Conte, E Coubez, X Fontaine, JC Gele, D Goerlach, U Goetzmann, C Le Bihan, AC Merlin, JA Skovpen, K Van Hove, P Gadrat, S Beauceron, S Bernet, C Boudoul, G Bouvier, E Montoya, CAC Chierici, R Contardo, D Courbon, B Depasse, P El Mamouni, H Fan, J Fay, J Gascon, S Gouzevitch, M Ille, B Lagarde, F Laktineh, IB Lethuillier, M Mirabito, L Pequegnot, AL Perries, S Alvarez, JDR Sabes, D Sgandurra, L Sordini, V Vander Donckt, M Verdier, P Viret, S Toriashvili, T Lomidze, D Autermann, C Beranek, S Edelhoff, M Feld, L Heister, A Kiesel, MK Klein, K Lipinski, M Ostapchuk, A Preuten, M Raupach, F Schael, S Schulte, JF Verlage, T Weber, H Wittmer, B Zhukov, V Ata, M Brodski, M Dietz-Laursonn, E Duchardt, D Endres, M Erdmann, M Erdweg, S Esch, T Fischer, R Guth, A Hebbeker, T Heidemann, C Hoepfner, K Klingebiel, D Knutzen, S Kreuzer, P Merschmeyer, M Meyer, A Millet, P Olschewski, M Padeken, K Papacz, P Pook, T Radziej, M Reithler, H Rieger, M Scheuch, F Sonnenschein, L Teyssier, D Thuer, S Cherepanov, V Erdogan, Y Flugge, G Geenen, H Geisler, M Hoehle, F Kargoll, B Kress, T Kuessel, Y Kunsken, A Lingemann, J Nehrkorn, A Nowack, A Nugent, IM Pistone, C Pooth, O Stahl, A Martin, MA Asin, I Bartosik, N Behnke, O Behrens, U Bell, AJ Borras, K Burgmeier, A Campbell, A Choudhury, S Costanza, F Pardos, CD Dolinska, G Dooling, S Dorland, T Eckerlin, G Eckstein, D Eichhorn, T Flucke, G Gallo, E Garcia, JG Geiser, A Gizhko, A Gunnellini, P Hauk, J Hempel, M Jung, H Kalogeropoulos, A Karacheban, O Kasemann, M Katsas, P Kieseler, J Kleinwort, C Korol, I Lange, W Leonard, J Lipka, K Lobanov, A Lohmann, W Mankel, R Marfin, I Melzer-Pellmann, IA Meyer, AB Mittag, G Mnich, J Mussgiller, A Naumann-Emme, S Nayak, A Ntomari, E Perrey, H Pitzl, D Placakyte, R Raspereza, A Roland, B Sahin, MO Saxena, P Schoerner-Sadenius, T Schroder, M Seitz, C Spannagel, S Trippkewitz, KD Walsh, R Wissing, C Blobel, V Vignali, MC Draeger, AR Erfle, J Garutti, E Goebel, K Gonzalez, D Gorner, M Haller, J Hoffmann, M Hoing, RS Junkes, A Klanner, R Kogler, R Lapsien, T Lenz, T Marchesini, I Marconi, D Meyer, M Nowatschin, D Ott, J Pantaleo, F Peiffer, T Perieanu, A Pietsch, N Poehlsen, J Rathjens, D Sander, C Schettler, H Schleper, P Schlieckau, E Schmidt, A Schwandt, J Sola, V Stadie, H Steinbruck, G Tholen, H Troendle, D Usai, E Vanelderen, L Vanhoefer, A Vormwald, B Akbiyik, M Barth, C Baus, C Berger, J Boser, C Butz, E Chwalek, T Colombo, F De Boer, W Descroix, A Dierlamm, A Fink, S Frensch, F Friese, R Giffels, M Gilbert, A Haitz, D Hartmann, F Heindl, SM Husemann, U Katkov, I Kornmayer, A Pardo, PL Maier, B Mildner, H Mozer, MU Muller, T Muller, T Plagge, M Quast, G Rabbertz, K Rocker, S Roscher, F Sieber, G Simonis, HJ Stober, FM Ulrich, R Wagner-Kuhr, J Wayand, S Weber, M Weiler, T Wohrmann, C Wolf, R Anagnostou, G Daskalakis, G Geralis, T Giakoumopoulou, VA Kyriakis, A Loukas, D Psallidas, A Topsis-Giotis, I Agapitos, A Kesisoglou, S Panagiotou, A Saoulidou, N Tziaferi, E Evangelou, I Flouris, G Foudas, C Kokkas, P Loukas, N Manthos, N Papadopoulos, I Paradas, E Strologas, J Bencze, G Hajdu, C Hazi, A Hidas, P Horvath, D Sikler, F Veszpremi, V Vesztergombi, G Zsigmond, AJ Beni, N Czellar, S Karancsi, J Molnar, J Szillasi, Z Bartok, M Makovec, A Raics, P Trocsanyi, ZL Ujvari, B Mal, P Mandal, K Sahoo, DK Sahoo, N Swain, SK Bansal, S Beri, SB Bhatnagar, V Chawla, R Gupta, R Bhawandeep, U Kalsi, AK Kaur, A Kaur, M Kumar, R Mehta, A Mittal, M Singh, JB Walia, G Kumar, A Bhardwaj, A Choudhary, BC Garg, RB Kumar, A Malhotra, S Naimuddin, M Nishu, N Ranjan, K Sharma, R Sharma, V Bhattacharya, S Chatterjee, K Dey, S Dutta, S Jain, S Majumdar, N Modak, A Mondal, K Mukherjee, S Mukhopadhyay, S Roy, A Roy, D Chowdhury, SR Sarkar, S Sharan, M Abdulsalam, A Chudasama, R Dutta, D Jha, V Kumar, V Mohanty, AK Pant, LM Shukla, P Topkar, A Aziz, T Banerjee, S Bhowmik, S Chatterjee, RM 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Riley, G. Rose, K. Spanier, S. York, A. Bouhali, O. Hernandez, A. Castaneda Dalchenko, M. De Mattia, M. Delgado, A. Dildick, S. Eusebi, R. Gilmore, J. Kamon, T. Krutelyov, V. Mueller, R. Osipenkov, I. Pakhotin, Y. Patel, R. Perloff, A. Rose, A. Safonov, A. Tatarinov, A. Ulmer, K. A. Akchurin, N. Cowden, C. Damgov, J. Dragoiu, C. Dudero, P. R. Faulkner, J. Kunori, S. Lamichhane, K. Lee, S. W. Libeiro, T. Undleeb, S. Volobouev, I. Appelt, E. Delannoy, A. G. Greene, S. Gurrola, A. Janjam, R. Johns, W. Maguire, C. Mao, Y. Melo, A. Ni, H. Sheldon, P. Snook, B. Tuo, S. Velkovska, J. Xu, Q. Arenton, M. W. Cox, B. Francis, B. Goodell, J. Hirosky, R. Ledovskoy, A. Li, H. Lin, C. Neu, C. Sinthuprasith, T. Sun, X. Wang, Y. Wolfe, E. Wood, J. Xia, F. Clarke, C. Harr, R. Karchin, P. E. Don, C. Kottachchi Kankanamge Lamichhane, P. Sturdy, J. Belknap, D. A. Carlsmith, D. Cepeda, M. Dasu, S. Dodd, L. Duric, S. Gomber, B. Grothe, M. Hall-Wilton, R. Herndon, M. Herve, A. Klabbers, P. Lanaro, A. Levine, A. Long, K. Loveless, R. Mohapatra, A. Ojalvo, I. Perry, T. Pierro, G. A. Polese, G. Ruggles, T. Sarangi, T. Savin, A. Sharma, A. Smith, N. Smith, W. H. Taylor, D. Woods, N. CA CMS Collaboration TI Measurement of t(t)over-bar production with additional jet activity, including b quark jets, in the dilepton decay channel using pp collisions at root s=8TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID CROSS-SECTION; LHC AB Jet multiplicity distributions in top quark pair (t (t) over bar) events are measured in pp collisions at a centre-of-mass energy of 8 TeV with the CMS detector at the LHC using a data set corresponding to an integrated luminosity of 19.7 fb(-1). The measurement is performed in the dilepton decay channels (e(+)e(-), mu(+)mu(-), and e(+/-)mu(+/-)). The absolute and normalized differential cross sections for t (t) over bar production are measured as a function of the jet multiplicity in the event for different jet transverse momentum thresholds and the kinematic properties of the leading additional jets. The differential t (t) over barb and t (t) over barb (b) over bar cross sections are presented for the first time as a function of the kinematic properties of the leading additional b jets. Furthermore, the fraction of events without additional jets above a threshold is measured as a function of the transverse momenta of the leading additional jets and the scalar sum of the transverse momenta of all additional jets. The data are compared and found to be consistent with predictions from several perturbative quantum chromodynamics event generators and a next-to-leading order calculation. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Knuenz, V.; Koenig, A.; Krammer, M.; Kraetschmer, I.; Liko, D.; Matsushita, T.; Mikulec, I.; Rabady, D.; Rahbaran, B.; Rohringer, H.; Schieck, J.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C-E] OeAW, Inst Hochenergiephys, Vienna, Austria. [Mossolov, V.; Shumeiko, N.; Gonzalez, J. Suarez] Natl Ctr Particle & High Energy Phys, Minsk, Byelarus. [Alderweireldt, S.; Cornelis, T.; De Wolf, E. A.; Janssen, X.; Knutsson, A.; Lauwers, J.; Luyckx, S.; Van De Klundert, M.; Van Haevermaet, H.; Van Mechelen, P.; Van Remortel, N.; Van Spilbeeck, A.] Univ Antwerp, Antwerp, Belgium. [Abu Zeid, S.; Blekman, F.; D'Hondt, J.; Daci, N.; De Bruyn, I.; Deroover, K.; Heracleous, N.; Keaveney, J.; Lowette, S.; Moreels, L.; Olbrechts, A.; Python, Q.; Strom, D.; Tavernier, S.; Van Doninck, W.; Van Mulders, P.; Van Onsem, G. P.; Van Parijs, I.] Vrije Univ Brussel, Brussels, Belgium. [Barria, P.; Brun, H.; Caillol, C.; Clerbaux, B.; De Lentdecker, G.; Fasanella, G.; Favart, L.; Grebenyuk, A.; Karapostoli, G.; Lenzi, T.; Leonard, A.; Maerschalk, T.; Marinov, A.; Pernie, L.; Randle-Conde, A.; Reis, T.; Seva, T.; Vander Velde, C.; Vanlaer, P.; Yonamine, R.; Zenoni, F.; Zhang, F.] Univ Libre Bruxelles, Brussels, Belgium. [Beernaert, K.; Benucci, L.; Cimmino, A.; Crucy, S.; Dobur, D.; Fagot, A.; Garcia, G.; Gul, M.; Mccartin, J.; Rios, A. A. Ocampo; Poyraz, D.; Ryckbosch, D.; Salva, S.; Sigamani, M.; Strobbe, N.; Tytgat, M.; Van Driessche, W.; Yazgan, E.; Zaganidis, N.] Univ Ghent, Ghent, Belgium. [Basegmez, S.; Beluffi, C.; Bondu, O.; Brochet, S.; Bruno, G.; Caudron, A.; Ceard, L.; Da Silveira, G. G.; Delaere, C.; Favart, D.; Forthomme, L.; Giammanco, A.; Hollar, J.; Jafari, A.; Jez, P.; Komm, M.; Lemaitre, V.; Mertens, A.; Musich, M.; Nuttens, C.; Perrini, L.; Pin, A.; Piotrzkowski, K.; Popov, A.; Quertenmont, L.; Selvaggi, M.; Marono, M. Vidal] Catholic Univ Louvain, Louvain La Neuve, Belgium. [Beliy, N.; Hammad, G. H.] Univ Mons, Mons, Belgium. [Alda, W. L., Jr.; Alves, F. L.; Alves, G. A.; Brito, L.; Correa Martins, M., Jr.; Hamer, M.; Hensel, C.; Mora Herrera, C.; Moraes, A.; Pol, M. E.; Rebello Teles, P.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Belchior Batista Das Chagas, E.; Carvalho, W.; Chinellato, J.; Custodio, A.; Da Costa, E. M.; De Jesus Damiao, D.; De Oliveira Martins, C.; Fonseca De Souza, S.; Huertas Guativa, L. M.; Malbouisson, H.; Matos Figueiredo, D.; Mundim, L.; Nogima, H.; Prado Da Silva, W. L.; Santoro, A.; Sznajder, A.; Tonelli Manganote, E. J.; Vilela Pereira, A.] Univ Estado Rio de Janeiro, BR-20550011 Rio De Janeiro, Brazil. [Ahuja, S.; Dogra, S.; Fernandez Perez Tomei, T. R.; Moon, C. S.; Novaes, S. F.; Padula, Sandra S.] Univ Estadual Paulista, Sao Paulo, Brazil. [Bernardes, C. A.; De Souza Santos, A.; Gregores, E. M.; Mercadante, P. G.] Univ Fed ABC, Sao Paulo, Brazil. [Aleksandrov, A.; Hadjiiska, R.; Iaydjiev, P.; Rodozov, M.; Stoykova, S.; Sultanov, G.; Vutova, M.] Inst Nucl Energy Res, Sofia, Bulgaria. [Dimitrov, A.; Glushkov, I.; Litov, L.; Pavlov, B.; Petkov, P.] Univ Sofia, Sofia, Bulgaria. [Ahmad, M.; Bian, J. G.; Chen, G. M.; Chen, H. S.; Chen, M.; Cheng, T.; Du, R.; Jiang, C. H.; Plestina, R.; Romeo, F.; Shaheen, S. M.; Spiezia, A.; Tao, J.; Wang, C.; Wang, Z.; Zhang, H.] Inst High Energy Phys, Beijing, Peoples R China. [Asawatangtrakuldee, C.; Ban, Y.; Li, Q.; Liu, S.; Mao, Y.; Qian, S. J.; Wang, D.; Xu, Z.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing, Peoples R China. [Avila, C.; Cabrera, A.; Chaparro Sierra, L. F.; Florez, C.; Gomez, J. P.; Gomez Moreno, B.; Sanabria, J. C.] Univ Los Andes, Bogota, Colombia. [Godinovic, N.; Lelas, D.; Puljak, I.; Ribeiro Cipriano, P. M.] Univ Split, Fac Elect Engn Mech Engn & Naval Architecture, Split, Croatia. [Antunovic, Z.; Kovac, M.] Univ Split, Fac Sci, Split, Croatia. [Brigljevic, V.; Kadija, K.; Luetic, J.; Micanovic, S.; Sudic, L.] Rudjer Boskovic Inst, Zagreb, Croatia. [Attikis, A.; Mavromanolakis, G.; Mousa, J.; Nicolaou, C.; Ptochos, F.; Razis, P. A.; Rykaczewski, H.] Univ Cyprus, Nicosia, Cyprus. [Bodlak, M.; Finger, M.; Finger, M., Jr.] Charles Univ Prague, Prague, Czech Republic. [El Sawy, M.; El-Khateeb, E.; Elkafrawy, T.; Mohamed, A.; Salama, E.] Acad Sci Res & Technol Arab Republ Egypt, Egyptian Network High Energy Phys, Cairo, Egypt. [Calpas, B.; Kadastik, M.; Murumaa, M.; Raidal, M.; Tiko, A.; Veelken, C.] NICPB, Tallinn, Estonia. [Eerola, P.; Pekkanen, J.; Voutilainen, M.] Univ Helsinki, Dept Phys, Helsinki, Finland. [Harkonen, J.; Karimaki, V.; Kinnunen, R.; Lampen, T.; Lassila-Perini, K.; Lehti, S.; Linden, T.; Luukka, P.; Maenpaa, T.; Peltola, T.; Tuominen, E.; Tuominiemi, J.; Tuovinen, E.; Wendland, L.] Helsinki Inst Phys, Helsinki, Finland. [Talvitie, J.; Tuuva, T.] Lappeenranta Univ Technol, Lappeenranta, Finland. [Besancon, M.; Couderc, F.; Dejardin, M.; Denegri, D.; Fabbro, B.; Faure, J. L.; Favaro, C.; Ferri, F.; Ganjour, S.; Givernaud, A.; Gras, P.; de Monchenault, G. Hamel; Jarry, P.; Locci, E.; Machet, M.; Malcles, J.; Rander, J.; Rosowsky, A.; Titov, M.; Zghiche, A.] CEA Saclay, DSM, IRFU, Gif Sur Yvette, France. [Antropov, I.; Baffioni, S.; Beaudette, F.; Busson, P.; Cadamuro, L.; Chapon, E.; Charlot, C.; Dahms, T.; Davignon, O.; Filipovic, N.; Florent, A.; de Cassagnac, R. Granier; Lisniak, S.; Mastrolorenzo, L.; Mine, P.; Naranjo, I. N.; Nguyen, M.; Ochando, C.; Ortona, G.; Paganini, P.; Pigard, P.; Regnard, S.; Salerno, R.; Sauvan, J. B.; Sirois, Y.; Strebler, T.; Yilmaz, Y.; Zabi, A.] CNRS, Ecole Polytech, Lab Leprince Ringuet, IN2P3, Palaiseau, France. [Agram, J. -L.; Andrea, J.; Aubin, A.; Bloch, D.; Brom, J. -M.; Buttignol, M.; Chabert, E. C.; Chanon, N.; Collard, C.; Conte, E.; Coubez, X.; Fontaine, J. -C.; Gele, D.; Goerlach, U.; Goetzmann, C.; Le Bihan, A. -C.; Merlin, J. A.; Skovpen, K.; Van Hove, P.] Univ Haute Alsace Mulhouse, Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS,IN2P3, Strasbourg, France. [Gadrat, S.] CNRS, IN2P3, Ctr Calcul, Villeurbanne, France. [Beauceron, S.; Bernet, C.; Boudoul, G.; Bouvier, E.; Montoya, C. A. Carrillo; Chierici, R.; Contardo, D.; Courbon, B.; Depasse, P.; El Mamouni, H.; Fan, J.; Fay, J.; Gascon, S.; Gouzevitch, M.; Ille, B.; Lagarde, F.; Laktineh, I. B.; Lethuillier, M.; Mirabito, L.; Pequegnot, A. L.; Perries, S.; Alvarez, J. D. Ruiz; Sabes, D.; Sgandurra, L.; Sordini, V.; Vander Donckt, M.; Verdier, P.; Viret, S.] Univ Lyon 1, CNRS, IN2P3, Inst Phys Nucl Lyon, F-69622 Villeurbanne, France. [Toriashvili, T.] Georgian Tech Univ, Tbilisi, Rep of Georgia. [Lomidze, D.] Tbilisi State Univ, Tbilisi, Rep of Georgia. [Autermann, C.; Beranek, S.; Edelhoff, M.; Feld, L.; Heister, A.; Kiesel, M. K.; Klein, K.; Lipinski, M.; Ostapchuk, A.; Preuten, M.; Raupach, F.; Schael, S.; Schulte, J. F.; Verlage, T.; Weber, H.; Wittmer, B.; Zhukov, V.] Rhein Westfal TH Aachen, Inst Phys 1, Aachen, Germany. [Ata, M.; Brodski, M.; Dietz-Laursonn, E.; Duchardt, D.; Endres, M.; Erdmann, M.; Erdweg, S.; Esch, T.; Fischer, R.; Gueth, A.; Hebbeker, T.; Heidemann, C.; Hoepfner, K.; Klingebiel, D.; Knutzen, S.; Kreuzer, P.; Merschmeyer, M.; Meyer, A.; Millet, P.; Olschewski, M.; Padeken, K.; Papacz, P.; Pook, T.; Radziej, M.; Reithler, H.; Rieger, M.; Scheuch, F.; Sonnenschein, L.; Teyssier, D.; Thueer, S.] Rhein Westfal TH Aachen, Phys Inst A3, Aachen, Germany. [Cherepanov, V.; Erdogan, Y.; Fluegge, G.; Geenen, H.; Geisler, M.; Hoehle, F.; Kargoll, B.; Kress, T.; Kuessel, Y.; Kuensken, A.; Lingemann, J.; Nehrkorn, A.; Nowack, A.; Nugent, I. M.; Pistone, C.; Pooth, O.; Stahl, A.] Rhein Westfal TH Aachen, Phys Inst B3, Aachen, Germany. [Martin, M. Aldaya; Asin, I.; Bartosik, N.; Behnke, O.; Behrens, U.; Bell, A. J.; Borras, K.; Burgmeier, A.; Campbell, A.; Choudhury, S.; Costanza, F.; Pardos, C. Diez; Dolinska, G.; Dooling, S.; Dorland, T.; Eckerlin, G.; Eckstein, D.; Eichhorn, T.; Flucke, G.; Gallo, E.; Garcia, J. Garay; Geiser, A.; Gizhko, A.; Gunnellini, P.; Hauk, J.; Hempel, M.; Jung, H.; Kalogeropoulos, A.; Karacheban, O.; Kasemann, M.; Katsas, P.; Kieseler, J.; Kleinwort, C.; Korol, I.; Lange, W.; Leonard, J.; Lipka, K.; Lobanov, A.; Lohmann, W.; Mankel, R.; Marfin, I.; Melzer-Pellmann, I. -A.; Meyer, A. B.; Mittag, G.; Mnich, J.; Mussgiller, A.; Naumann-Emme, S.; Nayak, A.; Ntomari, E.; Perrey, H.; Pitzl, D.; Placakyte, R.; Raspereza, A.; Roland, B.; Sahin, M. Oe; Saxena, P.; Schoerner-Sadenius, T.; Schroeder, M.; Seitz, C.; Spannagel, S.; Trippkewitz, K. D.; Walsh, R.; Wissing, C.] DESY, Hamburg, Germany. [Blobel, V.; Vignali, M. Centis; Draeger, A. R.; Erfle, J.; Garutti, E.; Goebel, K.; Gonzalez, D.; Goerner, M.; Haller, J.; Hoffmann, M.; Hoeing, R. S.; Junkes, A.; Klanner, R.; Kogler, R.; Lapsien, T.; Lenz, T.; Marchesini, I.; Marconi, D.; Meyer, M.; Nowatschin, D.; Ott, J.; Pantaleo, F.; Peiffer, T.; Perieanu, A.; Pietsch, N.; Poehlsen, J.; Rathjens, D.; Sander, C.; Schettler, H.; Schleper, P.; Schlieckau, E.; Schmidt, A.; Schwandt, J.; Sola, V.; Stadie, H.; Steinbrueck, G.; Tholen, H.; Troendle, D.; Usai, E.; Vanelderen, L.; Vanhoefer, A.; Vormwald, B.] Univ Hamburg, Hamburg, Germany. [Akbiyik, M.; Barth, C.; Baus, C.; Berger, J.; Boeser, C.; Butz, E.; Chwalek, T.; Colombo, F.; De Boer, W.; Descroix, A.; Dierlamm, A.; Fink, S.; Frensch, F.; Friese, R.; Giffels, M.; Gilbert, A.; Haitz, D.; Hartmann, F.; Heindl, S. M.; Husemann, U.; Katkov, I.; Kornmayer, A.; Pardo, P. Lobelle; Maier, B.; Mildner, H.; Mozer, M. U.; Mueller, T.; Mueller, Th.; Plagge, M.; Quast, G.; Rabbertz, K.; Roecker, S.; Roscher, F.; Sieber, G.; Simonis, H. J.; Stober, F. M.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Woehrmann, C.; Wolf, R.] Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Mal, P.; Mandal, K.; Sahoo, D. K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Kumar, A.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi, India. [Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Jain, Sa.; Majumdar, N.; Modak, A.; Mondal, K.; Mukherjee, S.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Abdulsalam, A.; Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Mumbai, Maharashtra, India. [Chauhan, S.; Dube, S.; Sharma, S.] IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Goldouzian, R.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggia, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.; Verwilligen, P.] Ist Nazl Fis Nucl, Sez Bari, Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggia, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Benvenuti, A. C.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Ist Nazl Fis Nucl, Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.; Travaglini, R.] Univ Bologna, Bologna, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Di Mattia, A.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN, Sez Catania, Catania, Italy. [Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Tropiano, A.; Viliani, L.] INFN, Sez Firenze, Florence, Italy. [Ciulli, V.; D'Alessandro, R.; Focardi, E.; Gonzi, S.; Gori, V.; Lenzi, P.; Tropiano, A.; Viliani, L.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.; Primavera, F.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] INFN, Sez Genova, Genoa, Italy. [Calvelli, V.; Lo Vetere, M.; Monge, M. R.; Tosi, S.] Univ Genoa, Genoa, Italy. [Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN, Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, N.; Fabozzi, F.] Univ Basilicata, Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Bellato, M.; Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Gasparini, F.; Gasparini, U.; Gonella, F.; Gozzelino, A.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN, Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Carlin, R.; Dall'Osso, M.; Fanzago, F.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] INFN, Sez Pavia, Pavia, Italy. [Montagna, P.; Ratti, S. P.; Riccardi, C.; Vitulo, P.] Univ Pavia, Pavia, Italy. [Solestizi, L. Alunni; Biasini, M.; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] INFN, Sez Perugia, Perugia, Italy. [Solestizi, L. Alunni; Biasini, M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.] Univ Perugia, Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] Ist Nazl Fis Nucl, Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] Ist Nazl Fis Nucl, Sez Roma, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.; Tamponi, U.] Ist Nazl Fis Nucl, Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] Ist Nazl Fis Nucl, Sez Trieste, Trieste, Italy. [Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Jeonju, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Kim, H.; Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Jo, M.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Sanchez-Hernandez, A.] IPN, Ctr Invest & Estudios Avanzados, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, H. A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch, New Zealand. [Ahmad, M.; Ahmad, A.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Fac Phys, Inst Expt Phys, Warsaw, Poland. [Bargassa, P.; Beirao Da Cruz E Silva, C.; Di Francesco, A.; Faccioli, P.; Ferreira Parracho, P. G.; Gallinaro, M.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Konoplyanikov, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Bylinkin, A.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Moscow, Russia. [Baskakov, A.; Belyaev, A.; Boos, E.; Bunichev, V.; Dubinin, M.; Dudko, L.; Klyukhin, V.; Kodolova, O.; Korneeva, N.; Lokhtin, I.; Myagkov, I.; Obraztsov, S.; Perfilov, M.; Petrushanko, S.; Savrin, V.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Dominguez Vazquez, D.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Santaolalla, J.; Soares, M. S.] CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; De Castro Manzano, P.; Duarte Campderros, J.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Munoz Sanchez, F. J.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Benitez, J. F.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; du Pree, T.; Dunser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Piparo, D.; Racz, A.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schaefer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Wohri, H. K.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Renker, D.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Robmann, P.; Ronga, F. J.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Cardaci, M.; Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Kumar, Arun; Bartek, R.; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ, Taipei, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Fac Sci, Dept Phys, Bangkok, Thailand. [Adiguzel, A.; Cerci, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Tali, B.; Topakli, H.; Vergili, M.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Akin, I. V.; Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle East Tech Univ, Dept Phys, Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-Storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Bell, K. W.; Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Womersley, W. J.; Worm, S. D.] Rutherford Appleton Lab, Didcot, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Cripps, N.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Ferguson, W.; Fulcher, J.; Futyan, D.; Hall, G.; Iles, G.; Kenzie, M.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Petridis, K.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Univ London Imperial Coll Sci Technol & Med, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leggat, D.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Fantasia, C.; Gastler, D.; Lawson, P.; Rankin, D.; Richardson, C.; Rohlf, J.; St John, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA USA. [Bhattacharya, S.; Alimena, J.; Berry, E.; Cutts, D.; Dhingra, N.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI USA. [Chauhan, S.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De La Barca; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Gardner, M.; Ko, W.; Lander, R.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA USA. [Weber, M.; Cousins, R.; Everaerts, P.; Farrell, C.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Luthra, A.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wuerthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Pierini, M.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado Boulder, Boulder, CO USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Banerjee, S.; Abdullin, S.; Albrow, M.; Anderson, J.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Gruenendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jindariani, S.; Johnson, M.; Joshi, U.; Jung, A. W.; Klima, B.; Kreis, B.; Kwan, S.; Lammel, S.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Outschoorn, V. I. Martinez; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mishra, K.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Weber, H. A.; Whitbeck, A.; Yang, F.] Fermilab Natl Accelerator Lab, Batavia, IL USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Di Giovanni, G. P.; Field, R. D.; Furic, I. K.; Gleyzer, S. V.; Hugon, J.; Konigsberg, J.; Korytov, A.; Low, J. F.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Silkworth, C.; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Martin, C.; Osherson, M.; Roskes, J.; Sady, A.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Benelli, G.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD USA. [Wang, J.; Apyan, A.; Barbieri, R.; Baty, A.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Ralph, D.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA USA. [Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Keller, J.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Kumar, A.; Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY USA. [Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.; Zhang, J.] Northeastern Univ, Boston, MA USA. [Hahn, K. A.; Kubik, A.; Mucia, N.; Odell, N.; Pollack, B.; Pozdnyakov, A.; Schmitt, M.; Stoynev, S.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Brinkerhoff, A.; Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Lynch, S.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Pearson, T.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Kotov, K.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Saka, H.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Harel, A.; Hindrichs, O.; Khukhunaishvili, A.; Petrillo, G.; Tan, P.; Verzetti, M.] Univ Rochester, Rochester, NY USA. [Arora, S.; Barker, A.; Chou, J. P.; Contreras-Campana, C.; Contreras-Campana, E.; Duggan, D.; Ferencek, D.; Gershtein, Y.; Gray, R.; Halkiadakis, E.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Panwalkar, S.; Park, M.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Hernandez, A. Castaneda; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Melo, A.; Ni, H.; Sheldon, P.; Snook, B.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, Nashville, TN USA. [Arenton, M. W.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sinthuprasith, T.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Sharma, A.; Belknap, D. A.; Carlsmith, D.; Cepeda, M.; Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Grothe, M.; Hall-Wilton, R.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Smith, N.; Smith, W. H.; Taylor, D.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Jeitler, M.; Krammer, M.; Schieck, J.; Wulz, C-E] Vienna Univ Technol, Vienna, Austria. [Rabady, D.; Merlin, J. A.; Lingemann, J.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Viliani, L.; Marzocchi, B.; Di Guida, S.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Zucchetta, A.; Ciangottini, D.; Donato, S.; D'imperio, G.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Candelise, V.; Ulmer, K. A.] CERN, European Org Nucl Res, Geneva, Switzerland. [Zhang, F.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing, Peoples R China. [Beluffi, C.] Univ Strasbourg, Inst Pluridisciplinaire Hubert Curien, CNRS, IN2P3, Strasbourg, France. [Giammanco, A.] NICPB, Tallinn, Estonia. [Popov, A.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. CNRS, IN2P3, Paris, France. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan, Armenia. RI Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017; Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Nguyen, Federico/Q-8994-2016; Ruiz, Alberto/E-4473-2011; Petrushanko, Sergey/D-6880-2012; Dudko, Lev/D-7127-2012; Govoni, Pietro/K-9619-2016; Tuominen, Eija/A-5288-2017; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Della Ricca, Giuseppe/B-6826-2013; TUVE', Cristina/P-3933-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Calderon, Alicia/K-3658-2014; Manganote, Edmilson/K-8251-2013; Lokhtin, Igor/D-7004-2012; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015 OI Ogul, Hasan/0000-0002-5121-2893; Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Nguyen, Federico/0000-0002-6713-1596; Ruiz, Alberto/0000-0002-3639-0368; Dudko, Lev/0000-0002-4462-3192; Govoni, Pietro/0000-0002-0227-1301; Tuominen, Eija/0000-0002-7073-7767; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Della Ricca, Giuseppe/0000-0003-2831-6982; TUVE', Cristina/0000-0003-0739-3153; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research; Estonian Research Council [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation; National Innovation Office, Hungary; Department of Atomic Energy; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education; University of Malaya (Malaysia); CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie programme; European Research Council; EPLANET (European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS programme of the Foundation for Polish Science; European Union, Regional Development Fund; OPUS programme of the National Science Center (Poland); Compagnia di San Paolo (Torino); Consorzio per la Fisica (Trieste); MIUR (Italy) [20108T4XTM]; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Welch Foundation [C-1845] FX We thank M. V. Garzelli for providing the theoretical predictions from POWHEL+PYTHIA6. We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centres and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation. Individuals have received support from the Marie-Curie programme and the European Research Council and EPLANET (European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS programme of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS programme of the National Science Center (Poland); the Compagnia di San Paolo (Torino); the Consorzio per la Fisica (Trieste); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programmes cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); and the Welch Foundation, contract C-1845. NR 71 TC 0 Z9 0 U1 21 U2 25 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 7 PY 2016 VL 76 IS 7 AR 379 DI 10.1140/epjc/s10052-016-4105-x PG 56 WC Physics, Particles & Fields SC Physics GA DR2BC UT WOS:000379709000001 PM 28280447 ER PT J AU Share, K Carter, RE Nikolaev, P Hooper, D Oakes, L Cohn, AP Rao, R Puretzky, AA Geohegan, DB Maruyama, B Pint, CL AF Share, Keith Carter, Rachel E. Nikolaev, Pavel Hooper, Daylond Oakes, Landon Cohn, Adam P. Rao, Rahul Puretzky, Alexander A. Geohegan, David B. Maruyama, Benji Pint, Cary L. TI Nanoscale Silicon as a Catalyst for Graphene Growth: Mechanistic Insight from in Situ Raman Spectroscopy SO JOURNAL OF PHYSICAL CHEMISTRY C LA English DT Article ID CHEMICAL-VAPOR-DEPOSITION; EMITTING POROUS SILICON; CARBON NANOTUBE GROWTH; HIGH-QUALITY; SURFACE; PHOTOLUMINESCENCE; PYROLYSIS; ACETYLENE; OXIDATION; FILMS AB Nanoscale carbons are typically synthesized by thermal decomposition of a hydrocarbon at the surface of a metal catalyst. Whereas the use of silicon as an alternative to metal catalysts could unlock new techniques to seamlessly couple carbon nanostructures and semiconductor materials, stable carbide formation renders bulk silicon incapable of the precipitation and growth of graphitic structures. Here, we provide evidence supported by comprehensive in situ Raman experiments that indicates nanoscale grains of silicon in porous silicon (PSi) scaffolds act as catalysts for hydrocarbon decomposition and growth of few layered graphene at temperatures as low as 700 K. Self-limiting growth kinetics of graphene with activation energies measured between 0.32-0.37 eV elucidates the formation of highly reactive surface-bound Si radicals that aid in the decomposition of hydrocarbons. Nucleation and growth of graphitic layers on PSi exhibits striking similarity to catalytic growth on nickel surfaces, involving temperature dependent surface and subsurface diffusion of carbon. This work elucidates how the nanoscale properties of silicon can be exploited to yield catalytic properties distinguished from bulk silicon, opening an important avenue to engineer catalytic interfaces combining the two most technologically important materials for modern applications-silicon and nanoscale carbons. C1 [Share, Keith; Oakes, Landon; Pint, Cary L.] Vanderbilt Univ, Interdisciplinary Mat Sci Program, 221 Kirkland Hall, Nashville, TN 37235 USA. [Share, Keith; Carter, Rachel E.; Oakes, Landon; Cohn, Adam P.; Pint, Cary L.] Vanderbilt Univ, Dept Mech Engn, Nashville, TN 37235 USA. [Nikolaev, Pavel; Hooper, Daylond; Rao, Rahul; Maruyama, Benji] US Air Force, Res Lab, Mat & Mfg Directorate, Wright Patterson AFB, OH 45433 USA. [Puretzky, Alexander A.; Geohegan, David B.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Hooper, Daylond] US Air Force, Res Lab, Airman Syst Directorate, Wright Patterson AFB, OH 45433 USA. RP Pint, CL (reprint author), Vanderbilt Univ, Interdisciplinary Mat Sci Program, 221 Kirkland Hall, Nashville, TN 37235 USA.; Pint, CL (reprint author), Vanderbilt Univ, Dept Mech Engn, Nashville, TN 37235 USA. EM Cary.L.Pint@vanderbilt.edu RI Geohegan, David/D-3599-2013 OI Geohegan, David/0000-0003-0273-3139 FU NSF [CMMI 1334269]; ASEE Summer Faculty Fellowship; NSF GFRP fellowships grant [1445197]; Materials Sciences and Engineering (MSE) Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported by NSF award CMMI 1334269 and an ASEE Summer Faculty Fellowship carried out at AFRL/RXBN. K.S. and A.P.C. are supported by NSF GFRP fellowships grant # 1445197. Characterization science for this work was in part sponsored by the Materials Sciences and Engineering (MSE) Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 47 TC 0 Z9 0 U1 9 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1932-7447 J9 J PHYS CHEM C JI J. Phys. Chem. C PD JUL 7 PY 2016 VL 120 IS 26 BP 14180 EP 14186 DI 10.1021/acs.jpcc.6b03880 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DQ8JL UT WOS:000379457000035 ER PT J AU Feng, ZX Chen, X Fister, TT Bedzyk, MJ Fenter, P AF Feng, Zhenxing Chen, Xiao Fister, Timothy T. Bedzyk, Michael J. Fenter, Paul TI Phase control of Mn-based spinel films via pulsed laser deposition SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID X-RAY-DIFFRACTION; THIN-FILMS; MGMN2O4; TEMPERATURE; BATTERIES; EVOLUTION AB Phase transformations in battery cathode materials during electrochemical-insertion reactions lead to capacity fading and low cycle life. One solution is to keep the same phase of cathode materials during cation insertion-extraction processes. Here, we demonstrate a novel strategy to control the phase and composition of Mn-based spinel oxides for magnesium-ion battery applications through the growth of thin films on lattice-matched substrates using pulsed laser deposition. Materials at two extreme conditions are considered: fully discharged cathode MgMn2O4 and fully charged cathode Mn2O4. The tetragonal MgMn2O4 (MMO) phase is obtained on MgAl2O4 substrates, while the cubic MMO phase is obtained on MgO substrates. Similarly, growth of the empty Mn2O4 spinel in the cubic phase is obtained on an MgO substrate. These results demonstrate the ability to control separately the phase of spinel thin films (e.g., tetragonal vs. cubic MMO) at nominally fixed composition, and to maintain a fixed (cubic) phase while varying its composition (MgxMn2O4, for x = 0, 1). This capability provides a novel route to gain insights into the operation of battery electrodes for energy storage applications. Published by AIP Publishing. C1 [Feng, Zhenxing; Fister, Timothy T.; Fenter, Paul] Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA. [Feng, Zhenxing; Fister, Timothy T.; Fenter, Paul] Argonne Natl Lab, Joint Ctr Energy Storage Res, Lemont, IL 60439 USA. [Chen, Xiao; Bedzyk, Michael J.] Northwestern Univ, Appl Phys Program, Evanston, IL 60208 USA. [Bedzyk, Michael J.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. RP Feng, ZX; Fenter, P (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Lemont, IL 60439 USA.; Feng, ZX; Fenter, P (reprint author), Argonne Natl Lab, Joint Ctr Energy Storage Res, Lemont, IL 60439 USA. EM fengz@anl.gov; fenter@anl.gov RI Bedzyk, Michael/B-7503-2009; OI Fenter, Paul/0000-0002-6672-9748 FU Joint Center for Energy Storage Research, an Energy Innovation Hub - U.S. Department of Energy, Office of Science, Basic Energy Sciences; DOE [DE-AC02-06CH11357]; Materials Research Science and Engineering Center (MRSEC) through National Science Foundation (NSF) [DMR-1121262]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX This work was supported as part of the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences. The Advanced Photon Source is supported by the DOE under Contract No. DE-AC02-06CH11357. This work made use of the Northwestern University Central Facilities supported by the Materials Research Science and Engineering Center (MRSEC) through National Science Foundation (NSF) under Contract No. DMR-1121262. The authors thank the beamline technical support from Christian M. Schlepuetz and Jenia Karapetrova at Sector-33, of APS. Authors thank Chunjoong Kim, Tanhong Yi, and Jordi Cabana from the University of Illinois at Chicago for helping synthesizing PLD target materials, Michael D. Biegalski for PLD growth support at Oak Ridge National Laboratory. The PLD preparation and characterization was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 27 TC 0 Z9 0 U1 14 U2 21 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 7 PY 2016 VL 120 IS 1 AR 015307 DI 10.1063/1.4955135 PG 7 WC Physics, Applied SC Physics GA DR0FR UT WOS:000379583900029 ER PT J AU Sun, Y Zhang, Y Zhang, F Ye, Z Ding, ZJ Wang, CZ Ho, KM AF Sun, Yang Zhang, Yue Zhang, Feng Ye, Zhuo Ding, Zejun Wang, Cai-Zhuang Ho, Kai-Ming TI Cooling rate dependence of structural order in Al90Sm10 metallic glass SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID AL-SM; SUPERCOOLED LIQUID; ALLOYS; TRANSITION; MODEL; CRYSTALLINE; PACKING; PHASES; SYSTEM AB The atomic structure of Al90Sm10 metallic glass is studied using molecular dynamics simulations. By performing a long sub-T-g annealing, we developed a glass model closer to the experiments than the models prepared by continuous cooling. Using the cluster alignment method, we found that "3661" cluster is the dominating short-range order in the glass samples. The connection and arrangement of "3661" clusters, which define the medium-range order in the system, are enhanced significantly in the sub-T-g annealed sample as compared with the fast cooled glass samples. Unlike some strong binary glass formers such as Cu64.5Zr35.5, the clusters representing the short-range order do not form an interconnected interpenetrating network in Al90Sm10, which has only marginal glass formability. Published by AIP Publishing. C1 [Sun, Yang; Ding, Zejun; Ho, Kai-Ming] Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei 230026, Anhui, Peoples R China. [Sun, Yang; Ding, Zejun; Ho, Kai-Ming] Univ Sci & Technol China, Dept Phys, Hefei 230026, Anhui, Peoples R China. [Sun, Yang; Zhang, Yue; Zhang, Feng; Ye, Zhuo; Wang, Cai-Zhuang; Ho, Kai-Ming] US DOE, Ames Lab, Ames, IA 50011 USA. [Wang, Cai-Zhuang; Ho, Kai-Ming] Iowa State Univ, Dept Phys, Ames, IA 50011 USA. [Ho, Kai-Ming] Univ Sci & Technol China, Int Ctr Quantum Design Funct Mat ICQD, Hefei 230026, Anhui, Peoples R China. [Ho, Kai-Ming] Univ Sci & Technol China, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China. RP Zhang, F (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM fzhang@ameslab.gov OI Sun, Yang/0000-0002-4344-2920 FU U.S. Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division [DE-AC02-07CH11358]; China Scholarship Council [201406340015]; National Natural Science Foundation of China [11274288, 11574289]; National Basic Research Program of China [2012CB933702]; USTC Qian-Ren B (1000-Talents Program B) fund FX Work at Ames Laboratory was supported by the U.S. Department of Energy, Basic Energy Sciences, Materials Science and Engineering Division, under Contract No. DE-AC02-07CH11358, including a grant of computer time at the National Energy Research Supercomputing Center (NERSC) in Berkeley, CA. Y.S. acknowledges the support from China Scholarship Council (File No. 201406340015). Z.J.D. acknowledges support from the National Natural Science Foundation of China (Nos. 11274288 and 11574289) and the National Basic Research Program of China (No. 2012CB933702). K.-M.H. acknowledges support from USTC Qian-Ren B (1000-Talents Program B) fund. NR 44 TC 1 Z9 1 U1 14 U2 23 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 7 PY 2016 VL 120 IS 1 AR 015901 DI 10.1063/1.4955223 PG 6 WC Physics, Applied SC Physics GA DR0FR UT WOS:000379583900035 ER PT J AU Tilka, JA Park, J Ahn, Y Pateras, A Sampson, KC Savage, DE Prance, JR Simmons, CB Coppersmith, SN Eriksson, MA Lagally, MG Holt, MV Evans, PG AF Tilka, J. A. Park, J. Ahn, Y. Pateras, A. Sampson, K. C. Savage, D. E. Prance, J. R. Simmons, C. B. Coppersmith, S. N. Eriksson, M. A. Lagally, M. G. Holt, M. V. Evans, P. G. TI Combining experiment and optical simulation in coherent X-ray nanobeam characterization of Si/ SiGe semiconductor heterostructures SO JOURNAL OF APPLIED PHYSICS LA English DT Article ID MISFIT DISLOCATIONS; CMOS APPLICATIONS; DIFFRACTION; SUPERLATTICES; DISTORTIONS; PTYCHOGRAPHY; MICROSCOPY; INTERFACES; STRAIN AB The highly coherent and tightly focused x-ray beams produced by hard x-ray light sources enable the nanoscale characterization of the structure of electronic materials but are accompanied by significant challenges in the interpretation of diffraction and scattering patterns. X-ray nanobeams exhibit optical coherence combined with a large angular divergence introduced by the x-ray focusing optics. The scattering of nanofocused x-ray beams from intricate semiconductor heterostructures produces a complex distribution of scattered intensity. We report here an extension of coherent x-ray optical simulations of convergent x-ray beam diffraction patterns to arbitrary x-ray incident angles to allow the nanobeam diffraction patterns of complex heterostructures to be simulated faithfully. These methods are used to extract the misorientation of lattice planes and the strain of individual layers from synchrotron x-ray nanobeam diffraction patterns of Si/SiGe heterostructures relevant to applications in quantum electronic devices. The systematic interpretation of nanobeam diffraction patterns from semiconductor heterostructures presents a new opportunity in characterizing and ultimately designing electronic materials. Published by AIP Publishing. C1 [Tilka, J. A.; Park, J.; Ahn, Y.; Pateras, A.; Sampson, K. C.; Savage, D. E.; Lagally, M. G.; Evans, P. G.] Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. [Prance, J. R.; Simmons, C. B.; Coppersmith, S. N.; Eriksson, M. A.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Holt, M. V.] Argonne Natl Lab, Ctr Nanoscale Mat, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Evans, PG (reprint author), Univ Wisconsin, Dept Mat Sci & Engn, 1509 Univ Ave, Madison, WI 53706 USA. EM pgevans@wisc.edu RI Prance, Jonathan/B-3536-2013; Evans, Paul/A-9260-2009 OI Prance, Jonathan/0000-0001-5009-383X; Evans, Paul/0000-0003-0421-6792 FU U.S. DOE, Basic Energy Sciences, Materials Sciences and Engineering [DE-FG02-04ER46147]; National Science Foundation Graduate Research Fellowship Program [DGE-1256259]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357]; ARO [W911NF-08-1-0482, W911NF-12-1-0607]; NSF [DMR-1206915]; University of Wisconsin Materials Research Science and Engineering Center [DMR-1121288] FX J.P., Y.A., A.P., and P.G.E. were supported by the U.S. DOE, Basic Energy Sciences, Materials Sciences and Engineering, under Contract No. DE-FG02-04ER46147 for the x-ray scattering studies and analysis. J.A.T. acknowledges support from the National Science Foundation Graduate Research Fellowship Program under Grant No. DGE-1256259. Use of the Center for Nanoscale Materials and the Advanced Photon Source, both Office of Science user facilities, was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. Development and maintenance of the growth facilities used for fabricating samples are supported by the Department of Energy (DE-FG02-03ER46028). The other authors acknowledge support from ARO (W911NF-08-1-0482, W911NF-12-1-0607) and NSF (DMR-1206915). This research used NSF-supported shared facilities supported by the University of Wisconsin Materials Research Science and Engineering Center (DMR-1121288). The authors would like to thank Eli Mueller for carefully reviewing the simulation. NR 38 TC 1 Z9 1 U1 10 U2 22 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-8979 EI 1089-7550 J9 J APPL PHYS JI J. Appl. Phys. PD JUL 7 PY 2016 VL 120 IS 1 AR 015304 DI 10.1063/1.4955043 PG 7 WC Physics, Applied SC Physics GA DR0FR UT WOS:000379583900026 ER PT J AU Buckingham, GT Porterfield, JP Kostko, O Troy, TP Ahmed, M Robichaud, DJ Nimlos, MR Daily, JW Ellison, GB AF Buckingham, Grant T. Porterfield, Jessica P. Kostko, Oleg Troy, Tyler P. Ahmed, Musahid Robichaud, David J. Nimlos, Mark R. Daily, John W. Ellison, G. Barney TI The thermal decomposition of the benzyl radical in a heated micro-reactor. II. Pyrolysis of the tropyl radical SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID THRESHOLD PHOTOELECTRON-SPECTRUM; SHOCK-WAVES; TOLUENE; SPECTROSCOPY; PHOTOIONIZATION; ACETYLENE; ISOMERIZATION; COMBUSTION; KINETICS; CYCLOHEPTATRIENE AB Cycloheptatrienyl (tropyl) radical, C7H7, was cleanly produced in the gas-phase, entrained in He or Ne carrier gas, and subjected to a set of flash-pyrolysis micro-reactors. The pyrolysis products resulting from C7H7 were detected and identified by vacuum ultraviolet photoionization mass spectrometry. Complementary product identification was provided by infrared absorption spectroscopy. Pyrolysis pressures in the micro-reactor were roughly 200 Torr and residence times were approximately 100 mu s. Thermal cracking of tropyl radical begins at 1100 K and the products from pyrolysis of C7H7 are only acetylene and cyclopentadienyl radicals. Tropyl radicals do not isomerize to benzyl radicals at reactor temperatures up to 1600 K. Heating samples of either cycloheptatriene or norbornadiene never produced tropyl (C7H7) radicals but rather only benzyl (C6H5CH2). The thermal decomposition of benzyl radicals has been reconsidered without participation of tropyl radicals. There are at least three distinct pathways for pyrolysis of benzyl radical: the Benson fragmentation, the methyl-phenyl radical, and the bridgehead norbornadienyl radical. These three pathways account for the majority of the products detected following pyrolysis of all of the isotopomers: C6H5CH2, C6H5CD2, C6D5CH2, and (C6H5CH2)-C-13. Analysis of the temperature dependence for the pyrolysis of the isotopic species (C6H5CD2, C6D5CH2, and (C6H5CH2)-C-13) suggests the Benson fragmentation and the norbornadienyl pathways open at reactor temperatures of 1300 K while the methyl-phenyl radical channel becomes active at slightly higher temperatures (1500 K). Published by AIP Publishing. C1 [Buckingham, Grant T.; Porterfield, Jessica P.; Ellison, G. Barney] Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA. [Buckingham, Grant T.; Robichaud, David J.; Nimlos, Mark R.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. [Kostko, Oleg; Troy, Tyler P.; Ahmed, Musahid] Lawrence Berkeley Natl Lab, Chem Sci Div, Berkeley, CA 94720 USA. [Daily, John W.] Univ Colorado, Ctr Combust & Environm Res, Dept Mech Engn, Boulder, CO 80309 USA. RP Buckingham, GT (reprint author), Univ Colorado, Dept Chem & Biochem, Campus Box 215, Boulder, CO 80309 USA.; Buckingham, GT (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. RI Ahmed, Musahid/A-8733-2009; OI Kostko, Oleg/0000-0003-2068-4991 FU National Science Foundation [CHE-1112466, CBET-1403979]; Marion L. Sharrah Memorial Fund at the University of Colorado; Office of Energy Research, Office of Basic Energy Sciences, and Chemical Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231]; United States Department of Energy's Bioenergy Technology Office [DE-AC36-99GO10337]; Sciences Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX We congratulate Professor Dr. Jurgen Troe on his appointment as the Benson Lecturer at the 24th International Symposium on Gas Kinetics and Related Phenomena, July 2016. The authors gratefully acknowledge the extensive helpful discussions with Nicole Labbe, Raghu Sivaramakrishnan, Hans-Heinrich Carstensen, John D. Savee, Veronica M. Bierbaum, and John F. Stanton. We are also in the debt of an anonymous referee for several useful suggestions. We acknowledge support from the National Science Foundation (Grant Nos. CHE-1112466 and CBET-1403979) to J.P.P., G.T.B., J.W.D., and G.B.E. G.T.B. was also funded by the Marion L. Sharrah Memorial Fund at the University of Colorado. M.A., O.K., and T.P.T. and the Advanced Light Source are supported by the Director, Office of Energy Research, Office of Basic Energy Sciences, and Chemical Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. D.J.R. and M.R.N. are supported by United States Department of Energy's Bioenergy Technology Office, under Contract No. DE-AC36-99GO10337 with the Sciences Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 81 TC 1 Z9 1 U1 16 U2 20 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 7 PY 2016 VL 145 IS 1 AR 014305 DI 10.1063/1.4954895 PG 14 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DR0FZ UT WOS:000379584700016 PM 27394106 ER PT J AU Hong, SY Xu, P Camillone, NR White, MG Camillone, N AF Hong, Sung-Young Xu, Pan Camillone, Nina R. White, Michael G. Camillone, Nicholas, III TI Adlayer structure dependent ultrafast desorption dynamics in carbon monoxide adsorbed on Pd (111) SO JOURNAL OF CHEMICAL PHYSICS LA English DT Article ID FEMTOSECOND LASER-PULSES; DENSITY-FUNCTIONAL THEORY; METAL-SURFACES; PT(111) SURFACE; CO ADSORPTION; PHOTOINDUCED DESORPTION; INFRARED-SPECTROSCOPY; VIBRATIONAL DYNAMICS; ORDERED STRUCTURES; CHEMICAL-DYNAMICS AB We report our ultrafast photoinduced desorption investigation of the coverage dependence of substrate-adsorbate energy transfer in carbon monoxide adlayers on the (111) surface of palladium. As the CO coverage is increased, the adsorption site population shifts from all threefold hollows (up to 0.33 ML), to bridge and near bridge (> 0.5 to 0.6 ML) and finally to mixed threefold hollow plus top site (at saturation at 0.75 ML). We show that between 0.24 and 0.75 ML this progression of binding site motifs is accompanied by two remarkable features in the ultrafast photoinduced desorption of the adsorbates: (i) the desorption probability increases roughly two orders magnitude, and (ii) the adsorbate-substrate energy transfer rate observed in two-pulse correlation experiments varies non-monotonically, having a minimum at intermediate coverages. Simulations using a phenomenological model to describe the adsorbate-substrate energy transfer in terms of frictional coupling indicate that these features are consistent with an adsorption-site dependent electron-mediated energy coupling strength, eta(el), that decreases with binding site in the order: three-fold hollow > bridge and near bridge > top site. This weakening of eta(el) largely counterbalances the decrease in the desorption activation energy that accompanies this progression of adsorption site motifs, moderating what would otherwise be a rise of several orders of magnitude in the desorption probability. Within this framework, the observed energy transfer rate enhancement at saturation coverage is due to interadsorbate energy transfer from the copopulation of molecules bound in three-fold hollows to their top-site neighbors. Published by AIP Publishing. C1 [Hong, Sung-Young; Camillone, Nina R.; White, Michael G.; Camillone, Nicholas, III] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Xu, Pan; White, Michael G.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. RP Camillone, N (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM nicholas@bnl.gov OI XU, PAN/0000-0002-5995-8710 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, & Biosciences (CSGB) Division, Condensed Phase and Interfacial Molecular Science (CPIMS) Program [DE-SC0012704] FX The authors would like to acknowledge Maite Alducin for helpful conversations. This article is based upon work supported in its entirety by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, & Biosciences (CSGB) Division, Condensed Phase and Interfacial Molecular Science (CPIMS) Program, under Contract No. DE-SC0012704. NR 88 TC 1 Z9 1 U1 8 U2 15 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0021-9606 EI 1089-7690 J9 J CHEM PHYS JI J. Chem. Phys. PD JUL 7 PY 2016 VL 145 IS 1 AR 014704 DI 10.1063/1.4954408 PG 15 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DR0FZ UT WOS:000379584700028 PM 27394118 ER PT J AU Poutsma, ML AF Poutsma, Marvin L. TI Extension of Structure-Reactivity Correlations for the Hydrogen Abstraction Reaction to the Methyl Radical and Comparison to the Chlorine Atom, Bromine Atom, and Hydroxyl Radical SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID CHEMICAL KINETIC DATABASE; COMBUSTION CHEMISTRY; THEORETICAL PROCEDURES; SUBSTITUTED ALKENES; REACTION-MECHANISM; RATE CONSTANTS; TRIFLUOROMETHYL RADICALS; GAS-PHASE; DATA-BASE; METHANOL AB Recently, we presented structure-reactivity correlations for the gas-phase rate constants for hydrogen abstraction from sp(3)-hybridized carbon by three electrophihc radicals (X-center dot + HCR3 -> XH + (CR3)-C-center dot; X = Cl-center dot, HO center dot, and Br-center dot); the reaction enthalpy effect was represented by the independent variable Delta H-r and the "polar effect" by the independent variables F and R, the Hammett-Taft constants for field/inductive and resonance effects. Here we present a parallel treatment for the less electronegative CH3 center dot. In spite of a limited and scattered database, the resulting least-squares fit [log k(437)(CH3 center dot) = -0.0251 (Delta H-r) + 0.96(Sigma F) - 0.56(Sigma R) - 19.15] was modestly successful and useful for initial predictions. As expected, the polar effect appears to be minor and its directionality, i.e., the "philicity" of CH3 center dot, may depend on the nature of the substituents. C1 [Poutsma, Marvin L.] Oak Ridge Natl Lab, Div Chem Sci, POB 2008, Oak Ridge, TN 37831 USA. RP Poutsma, ML (reprint author), Oak Ridge Natl Lab, Div Chem Sci, POB 2008, Oak Ridge, TN 37831 USA. EM poutsmaml@ornl.gov FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division FX This research was sponsored by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Chemical Sciences, Geosciences and Biosciences Division. NR 67 TC 0 Z9 0 U1 6 U2 10 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 7 PY 2016 VL 120 IS 26 BP 4447 EP 4454 DI 10.1021/acs.jpca.6b04357 PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DQ8JM UT WOS:000379457100003 PM 27266850 ER PT J AU Bjorgaard, JA Sifain, AE Nelson, T Myers, TW Veauthier, JM Chavez, DE Scharff, RJ Tretiak, S AF Bjorgaard, Josiah A. Sifain, Andrew E. Nelson, Tammie Myers, Thomas W. Veauthier, Jacqueline M. Chavez, David E. Scharff, R. Jason Tretiak, Sergei TI Two-Photon Absorption in Conjugated Energetic Molecules SO JOURNAL OF PHYSICAL CHEMISTRY A LA English DT Article ID DENSITY-FUNCTIONAL THEORY; RESONANCE ENHANCEMENT; LASER INITIATION; PORPHYRIN DIMERS; CROSS-SECTION; CHROMOPHORES; DYNAMICS; PETN; DENDRIMERS; OLIGOMERS AB Time-dependent density functional theory (TD-DFT) was used to investigate the relationship between molecular structure and the one- and two-photon absorption (OPA and TPA, respectively) properties of novel and recently synthesized conjugated energetic molecules (CEMs). The molecular structures of CEMs can be strategically altered to influence the heat of formation and oxygen balance, two factors that can contribute to the sensitivity and strength of an explosive material. OPA and TPA are sensitive to changes in molecular structure as well, influencing the optical range of excitation. We found calculated vertical excitation energies to be in good agreement with experiment for most molecules. Peak TPA intensities were found to be significant and on the order of 102 GM. Natural transition orbitals for essential electronic states defining TPA peaks of relatively large intensity were used to examine the character of relevant transitions. Modification of molecular substituents, such as additional oxygen or other functional groups, produces significant changes in electronic structure, OPA, and TPA and improves oxygen balance. The results show that certain molecules are apt to undergo nonlinear absorption, opening the possibility for controlled, direct optical initiation of CEMs through photochemical pathways. C1 [Bjorgaard, Josiah A.; Tretiak, Sergei] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Bjorgaard, Josiah A.; Nelson, Tammie; Tretiak, Sergei] Los Alamos Natl Lab, Div Theoret, Phys & Chem Mat T1, Los Alamos, NM 87545 USA. [Myers, Thomas W.; Veauthier, Jacqueline M.; Chavez, David E.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. [Scharff, R. Jason] Los Alamos Natl Lab, Explos Sci & Shock Phys Div, Shock & Detonat Phys M9, Los Alamos, NM 87545 USA. [Tretiak, Sergei] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Sifain, Andrew E.] Univ So Calif, Dept Phys & Astron, Los Angeles, CA 90089 USA. RP Tretiak, S (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA.; Tretiak, S (reprint author), Los Alamos Natl Lab, Div Theoret, Phys & Chem Mat T1, Los Alamos, NM 87545 USA.; Scharff, RJ (reprint author), Los Alamos Natl Lab, Explos Sci & Shock Phys Div, Shock & Detonat Phys M9, Los Alamos, NM 87545 USA.; Tretiak, S (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. EM scharff@lanl.gov; serg@lanl.gov RI Tretiak, Sergei/B-5556-2009; OI Tretiak, Sergei/0000-0001-5547-3647; Scharff, Robert/0000-0002-1708-8964; Veauthier, Jacqueline/0000-0003-2206-7786 FU U.S. Department of Energy through Los Alamos National Laboratory (LANL) LDRD Program; U.S. Department of Energy [DE-AC52- 06NA25396] FX The authors acknowledge support of the U.S. Department of Energy through the Los Alamos National Laboratory (LANL) LDRD Program. LANL is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract DE-AC52- 06NA25396. This work was done in part at the Center for Nonlinear Studies (CNLS) and the Center for Integrated Nanotechnology (CINT) at LANL. We also acknowledge the LANL Institutional Computing (IC) program for providing computational resources. NR 45 TC 3 Z9 3 U1 10 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1089-5639 J9 J PHYS CHEM A JI J. Phys. Chem. A PD JUL 7 PY 2016 VL 120 IS 26 BP 4455 EP 4464 DI 10.1021/acs.jpca.6b03136 PG 10 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DQ8JM UT WOS:000379457100004 PM 27257984 ER PT J AU Soriaga, AB Sangwan, S Macdonald, R Sawaya, MR Eisenberg, D AF Soriaga, Angela B. Sangwan, Smriti Macdonald, Ramsay Sawaya, Michael R. Eisenberg, David TI Crystal Structures of IAPP Amyloidogenic Segments Reveal a Novel Packing Motif of Out-of-Register Beta Sheets SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID SOLID-STATE NMR; NEURODEGENERATIVE DISEASES; PROTEIN; FIBRILS; PEPTIDE; OLIGOMERS; AMYLIN; MODEL; POLYMORPHISM; DIFFRACTION AB Structural studies of amyloidogenic segments by X-ray crystallography have revealed a novel packing motif, consisting of out-of-register beta sheets, which may constitute one of the toxic species in aggregation related diseases. Here we sought to determine the presence of such a motif in islet amyloid polypeptide (IAPP), whose amyloidogenic properties are associated with type 2 diabetes. We determined four new crystal structures of segments within IAPP, all forming steric zippers. Most interestingly, one of the segments in the fibril core of IAPP forms an out-of-register steric zipper. Analysis of this structure reveals several commonalities with previously solved out-of-register fibrils. Our results provide additional evidence of out of-register beta sheets as a common structural motif in amyloid aggregates. C1 [Soriaga, Angela B.; Sangwan, Smriti; Sawaya, Michael R.; Eisenberg, David] Univ Calif Los Angeles, Howard Hughes Med Inst, Los Angeles, CA 90095 USA. [Soriaga, Angela B.; Sangwan, Smriti; Macdonald, Ramsay; Sawaya, Michael R.; Eisenberg, David] Univ Calif Los Angeles, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA. [Soriaga, Angela B.; Sangwan, Smriti; Sawaya, Michael R.; Eisenberg, David] Univ Calif Los Angeles, Dept Biol Chem, Los Angeles, CA 90095 USA. [Soriaga, Angela B.; Sangwan, Smriti; Macdonald, Ramsay; Sawaya, Michael R.; Eisenberg, David] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. RP Eisenberg, D (reprint author), Univ Calif Los Angeles, Howard Hughes Med Inst, Los Angeles, CA 90095 USA.; Eisenberg, D (reprint author), Univ Calif Los Angeles, UCLA DOE Inst Genom & Prote, Los Angeles, CA 90095 USA.; Eisenberg, D (reprint author), Univ Calif Los Angeles, Dept Biol Chem, Los Angeles, CA 90095 USA.; Eisenberg, D (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. EM david@mbi.ucla.edu OI Sawaya, Michael/0000-0003-0874-9043 FU National Institute of General Medical Sciences [P41 GM103403]; U.S. Department of Energy (DOE) Office of Science [DE-AC02-06CH11357]; HHMI; DOE; NIH [AG 029430]; UCLA; Whitcome predoctoral fellowship FX We thank Michael Collazo and beamline staff at the Advanced Photon Source (APS) Northeastern Collaborative Access Team beamline 24-ID-E for help with experiments. The beamline is funded by the National Institute of General Medical Sciences (P41 GM103403) and U.S. Department of Energy (DOE) Office of Science under Contract No. DE-AC02-06CH11357. We thank HHMI, DOE, and NIH AG 029430 for funding. A.B.S. was supported by the UCLA Dissertation Year fellowship and S.S. was supported by the Whitcome predoctoral fellowship. Atomic coordinates and structure factors have been deposited in the Protein Data Bank as 5E5V for NFGAILS, 5E5Z for LVHSSN, 5E61 for FGAILSS, and 5E5X for ANFLVH. We thank Pascal Krotee for valuable comments on the manuscript. NR 44 TC 3 Z9 3 U1 6 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUL 7 PY 2016 VL 120 IS 26 BP 5810 EP 5816 DI 10.1021/acs.jpcb.5b09981 PG 7 WC Chemistry, Physical SC Chemistry GA DQ8JN UT WOS:000379457200004 PM 26629790 ER PT J AU Salerno, KM Frischknecht, AL Stevens, MJ AF Salerno, K. Michael Frischknecht, Amalie L. Stevens, Mark J. TI Charged Nanoparticle Attraction in Multivalent Salt Solution: A Classical-Fluids Density Functional Theory and Molecular Dynamics Study SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID MONTE-CARLO-SIMULATION; ELECTRIC DOUBLE-LAYERS; STRONG-COUPLING THEORY; COLLOIDAL PARTICLES; ELECTROLYTE-SOLUTIONS; GOLD NANOPARTICLES; POISSON-BOLTZMANN; DNA CONDENSATION; MACROIONS; POLYELECTROLYTES AB Negatively charged nanopartides (NPs) in 1:1, 1:2, and 1:3 electrolyte solutions are studied in a primitive ion model using molecular dynamics (MD) simulations and classical density functional theory (DFT). We determine the conditions for attractive interactions between the like-charged NPs. Ion density profiles and NP NP interaction free energies are compared between the two methods and are found to be in qualitative agreement. The NP interaction free energy is purely repulsive for monovalent counterions, but can be attractive for divalent and trivalent counterions. Using DFT, the NP interaction free energy for different NP diameters and charges is calculated. The depth and location of the minimum in the interaction depend strongly on the NPs' charge. For certain parameters, the depth of the attractive well can reach 8-10 k(B)T, indicating that kinetic arrest and aggregation of the NPs due to electrostatic interactions is possible. Rich behavior arises from the geometric constraints of counterion packing at the NP surface. Layering of counterions around the NPs is observed and, as secondary counterion layers form the minimum of the NP NP interaction free energy shifts to larger separation, and the depth of the free energy minimum varies dramatically. We find that attractive interactions occur with and without NP overcharging. C1 [Salerno, K. Michael; Frischknecht, Amalie L.; Stevens, Mark J.] Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. RP Stevens, MJ (reprint author), Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. EM msteve@sandia.gov RI Frischknecht, Amalie/N-1020-2014 OI Frischknecht, Amalie/0000-0003-2112-2587 FU U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was performed at the Center for Integrated Nanotechnologies, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. NR 68 TC 1 Z9 1 U1 8 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUL 7 PY 2016 VL 120 IS 26 BP 5927 EP 5937 DI 10.1021/acs.jpcb.6b01392 PG 11 WC Chemistry, Physical SC Chemistry GA DQ8JN UT WOS:000379457200016 PM 27057763 ER PT J AU Huber, RC Ferreira, AS Aguirre, JC Kilbride, D Toso, DB Mayoral, K Zhou, ZH Kopidakis, N Rubin, Y Schwartz, BJ Mason, TG Tolbert, SH AF Huber, Rachel C. Ferreira, Amy S. Aguirre, Jordan C. Kilbride, Daniel Toso, Daniel B. Mayoral, Kenny Zhou, Z. Hong Kopidakis, Nikos Rubin, Yves Schwartz, Benjamin J. Mason, Thomas G. Tolbert, Sarah H. TI Structure and Conductivity of Semiconducting Polymer Hydrogels SO JOURNAL OF PHYSICAL CHEMISTRY B LA English DT Article ID RESOLVED MICROWAVE CONDUCTIVITY; SMALL-ANGLE SCATTERING; CONJUGATED POLYELECTROLYTES; SOLAR-CELLS; BIOLOGICAL MACROMOLECULES; HYALURONIC-ACID; DRUG-DELIVERY; POLY(3-HEXYLTHIOPHENE); EFFICIENCY; BILAYERS AB Poly(fluorene-alt-thiophene) (PFT) is a conjugated polyelectrolyte that self-assembles into rod-like micelles in water, with the conjugated polymer backbone running along the length of the micelle. At modest concentrations (similar to 10 mg/mL in aqueous solutions), PFT forms hydrogels, and this work focuses on understanding the structure and intermolecular interactions in those gel networks. The network structure can be directly visualized using cryo electron microscopy. Oscillatory rheology studies further tell us about connectivity within the gel network, and the data are consistent with a picture where polymer chains bridge between micelles to hold the network together. Addition of tetrahydrofuran (THF) to the gels breaks those connections, but once the THF is removed, the gel becomes stronger than it was before, presumably due to the creation of a more interconnected nanoscale architecture. Small polymer oligomers can also passivate the bridging polymer chains, breaking connections between micelles and dramatically weakening the hydrogel network. Fits to solution-phase small-angle X-ray scattering data using a Dammin bead model support the hypothesis of a bridging connection between PFT micelles, even in dilute aqueous solutions. Finally, time-resolved microwave conductivity measurements on dried samples show an increase in carrier mobility after THF annealing of the PFT gel, likely due to increased connectivity within the polymer network. C1 [Huber, Rachel C.; Ferreira, Amy S.; Aguirre, Jordan C.; Kilbride, Daniel; Mayoral, Kenny; Rubin, Yves; Schwartz, Benjamin J.; Mason, Thomas G.; Tolbert, Sarah H.] Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA. [Toso, Daniel B.; Zhou, Z. Hong] Univ Calif Los Angeles, Dept Microbiol Immunol & Mol Genet, 609 Charles E Young Dr South, Los Angeles, CA 90095 USA. [Toso, Daniel B.; Zhou, Z. Hong] Univ Calif Los Angeles, Biomed Engn Program, 609 Charles E Young Dr South, Los Angeles, CA 90095 USA. [Zhou, Z. Hong; Schwartz, Benjamin J.; Tolbert, Sarah H.] Univ Calif Los Angeles, Calif NanoSyst Inst, 570 Westwood Plaza, Los Angeles, CA 90095 USA. [Kopidakis, Nikos] Natl Renewable Energy Lab, Chem & Nanosci Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. Univ Calif Los Angeles, Dept Mat Sci & Engn, Los Angeles, CA 90095 USA. RP Tolbert, SH (reprint author), Univ Calif Los Angeles, Dept Chem & Biochem, Los Angeles, CA 90095 USA.; Tolbert, SH (reprint author), Univ Calif Los Angeles, Calif NanoSyst Inst, 570 Westwood Plaza, Los Angeles, CA 90095 USA. EM tolbert@chem.ucla.edu FU National Science Foundation [CHE-1112569]; Center for Molecularly Engineered Energy Materials (MEEM), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0001342]; NSF IGERT: Materials Creation Training Program (MCTP) [DGE-0654431]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-76SF00515]; DOE Office of Biological and Environmental Research; National Institutes of Health, National Institute of General Medical Sciences [P41GM103393]; NIH [1S10RR23057]; CNSI at UCLA FX This work was supported by the National Science Foundation under Grant Number CHE-1112569 (synthesis, rheology, TEM, and SAXS Monte Carlo fitting) and by the Center for Molecularly Engineered Energy Materials (MEEM), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Award Number DE-SC0001342 (TRMC, SAXS data collection). J.C.A. acknowledges the NSF IGERT: Materials Creation Training Program (MCTP), Grant Number DGE-0654431, and the California NanoSystems Institute. This manuscript contains data collected at the Stanford Synchrotron Radiation Lightsource (SSRL). SSRL and the SLAC National Accelerator Laboratory are supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. The SSRL Structural Molecular Biology Program is supported by the DOE Office of Biological and Environmental Research and by the National Institutes of Health, National Institute of General Medical Sciences (including P41GM103393). The contents of this publication are solely the responsibility of the authors and do not necessarily represent the official views of NIGMS or NIH. The authors acknowledge the use of instruments at the Electron Imaging Center for NanoMachines supported by NIH (1S10RR23057 to ZHZ) and CNSI at UCLA. NR 50 TC 1 Z9 1 U1 12 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1520-6106 J9 J PHYS CHEM B JI J. Phys. Chem. B PD JUL 7 PY 2016 VL 120 IS 26 BP 6215 EP 6224 DI 10.1021/acs.jpcb.6b02202 PG 10 WC Chemistry, Physical SC Chemistry GA DQ8JN UT WOS:000379457200048 PM 27079171 ER PT J AU Kobayashi, T Perras, FA Goh, TW Metz, TL Huang, WY Pruski, M AF Kobayashi, Takeshi Perras, Frederic A. Goh, Tian Wei Metz, Tanner L. Huang, Wenyu Pruski, Marek TI DNP-Enhanced Ultrawideline Solid-State NMR Spectroscopy: Studies of Platinum in Metal-Organic Frameworks SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID DYNAMIC NUCLEAR-POLARIZATION; OXIDATION CATALYSIS; MAGNETIC-RESONANCE; MAGIC-ANGLE; IONS; REDUCTION; COMPLEXES; PULSES; SITES AB Ultrawideline dynamic nuclear polarization (DNP)-enhanced Pt-195 solid-state NMR (SSNMR) spectroscopy and theoretical calculations are used to determine the coordination of atomic Pt species supported within the pores of metal-organic frameworks (MOFs). The Pt-195 SSNMR spectra, with breadths reaching 10 000 ppm, were obtained by combining DNP with broadbanded cross-polarization and CPMG acquisition. Although the DNP enhancements in static samples are lower than those typically observed under magic-angle spinning conditions, the presented measurements would be very challenging using the conventional SSNMR methods. The DNP-enhanced ultrawideline NMR spectra served to separate signals from cis- and trans-coordinated atomic Pt2+ species supported on the UiO-66-NH2 MOF. Additionally, the data revealed a dominance of kinetic effects in the formation of Pt2+ complexes and the thermodynamic effects in their reduction to nanoparticles. A single cis-coordinated Pt2+ complex was confirmed in MOF-253. C1 [Kobayashi, Takeshi; Perras, Frederic A.; Huang, Wenyu; Pruski, Marek] US DOE, Ames Lab, Ames, IA 50011 USA. [Goh, Tian Wei; Metz, Tanner L.; Huang, Wenyu; Pruski, Marek] Iowa State Univ, Dept Chem, Ames, IA 50011 USA. RP Huang, WY; Pruski, M (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA.; Huang, WY; Pruski, M (reprint author), Iowa State Univ, Dept Chem, Ames, IA 50011 USA. EM whuang@iastate.edu; mpruski@iastate.edu RI Huang, Wenyu/L-3784-2014 OI Huang, Wenyu/0000-0003-2327-7259 FU U.S. Department of Energy, Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory; Ames Laboratory (Royalty Account); Iowa State University; Laboratory Directed Research and Development (LDRD) program at the Ames Laboratory; DOE [DE-AC02-07CH11358] FX This research is supported by the U.S. Department of Energy, Basic Energy Sciences, Division of Chemical Sciences, Geosciences, and Biosciences through the Ames Laboratory. W.H. gratefully acknowledges the startup funds support from the Ames Laboratory (Royalty Account) and Iowa State University. Support for F.P. is through a Spedding Fellowship funded by the Laboratory Directed Research and Development (LDRD) program at the Ames Laboratory. Ames Laboratory is operated for the DOE by Iowa State University under Contract No. DE-AC02-07CH11358. We thank Dr. Levi Stanley for his help with the synthesis of the linkers for MOF-253. NR 44 TC 5 Z9 5 U1 29 U2 59 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 7 PY 2016 VL 7 IS 13 BP 2322 EP 2327 DI 10.1021/acs.jpclett.6b00860 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DQ8JP UT WOS:000379457400005 PM 27266444 ER PT J AU Sharma, VK Marnontov, E Tyagi, M Qian, S Rai, DK Urban, VS AF Sharma, V. K. Marnontov, E. Tyagi, M. Qian, S. Rai, D. K. Urban, V. S. TI Dynamical and Phase Behavior of a Phospholipid Membrane Altered by an Antimicrobial Peptide at Low Concentration SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID ELASTIC NEUTRON-SCATTERING; CHOLESTEROL LIPID-BILAYERS; X-RAY-DIFFRACTION; LATERAL DIFFUSION; MOLECULAR-MECHANISM; MODEL MEMBRANES; MELITTIN; ALAMETHICIN; MICELLES; DIMYRISTOYLPHOSPHATIDYLCHOLINE AB The mechanism of action of antimicrobial peptides is traditionally attributed to the formation of pores in the lipid cell membranes of pathogens, which requires a substantial peptide to lipid ratio. However, using incoherent neutron scattering, we show that even at a concentration too low for pore formation, an archetypal antimicrobial peptide, melittin, disrupts the regular phase behavior of the microscopic dynamics in a phospholipid membrane, dimyristoylphosphatidylcholine (DMPC). At the same time, another antimicrobial peptide, alamethicin, does not exert a similar effect on the DMPC microscopic dynamics. The melittin-altered lateral motion of DMPC at physiological temperature no longer resembles the fluid-phase behavior characteristic of functional membranes of the living cells. The disruptive effect demonstrated by melittin even at low concentrations reveals a new mechanism of antimicrobial action relevant in more realistic scenarios, when peptide concentration is not as high as would be required for pore formation, which may facilitate treatment with antimicrobial peptides. C1 [Sharma, V. K.; Qian, S.; Rai, D. K.; Urban, V. S.] Oak Ridge Natl Lab, Neutron Sci Directorate, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA. [Sharma, V. K.] Bhabha Atom Res Ctr, Div Solid State Phys, Bombay 400085, Maharashtra, India. [Marnontov, E.] Oak Ridge Natl Lab, Neutron Sci Directorate, Chem & Engn Mat Div, Oak Ridge, TN 37831 USA. [Tyagi, M.] Natl Inst Stand & Technol, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Tyagi, M.] Univ Maryland, Dept Mat Sci & Engn, College Pk, MD 20742 USA. RP Sharma, VK (reprint author), Oak Ridge Natl Lab, Neutron Sci Directorate, Biol & Soft Matter Div, Oak Ridge, TN 37831 USA.; Sharma, VK (reprint author), Bhabha Atom Res Ctr, Div Solid State Phys, Bombay 400085, Maharashtra, India. EM sharmavk@ornl.gov RI Mamontov, Eugene/Q-1003-2015; OI Mamontov, Eugene/0000-0002-5684-2675; Rai, Durgesh/0000-0001-7257-7210 FU National Science Foundation [DMR-1508249]; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Biological and Environmental Research of the U.S. Department of Energy [FWP ERKP291]; U.S. Department of Energy (DOE) [DE-AC05-00OR22725] FX The neutron scattering experiments on HFBS at NCNR were supported in part by the National Science Foundation under Agreement No. DMR-1508249. The neutron scattering experiments on BASIS at the Spallation Neutron Source were supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. The Bio-SANS of the Center for Structural Molecular Biology (FWP ERKP291) at the High Flux Isotope Reactoris is supported by the Office of Biological and Environmental Research of the U.S. Department of Energy. ORNL is managed by UT-Battelle, LLC, for the U.S. Department of Energy (DOE) under contract no. DE-AC05-00OR22725. NR 56 TC 1 Z9 1 U1 5 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 7 PY 2016 VL 7 IS 13 BP 2394 EP 2401 DI 10.1021/acs.jpclett.6b01006 PG 8 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DQ8JP UT WOS:000379457400018 PM 27232190 ER PT J AU Saha, A Shetty, A Pavan, AR Chattopadhyay, S Shibata, T Viswanatha, R AF Saha, Avijit Shetty, Amitha Pavan, A. R. Chattopadhyay, Soma Shibata, Tomohiro Viswanatha, Ranjani TI Uniform Doping in Quantum-Dots-Based Dilute Magnetic Semiconductor SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID NANOCRYSTAL HETEROSTRUCTURES; ZEEMAN SPLITTINGS; TRANSITION; SURFACE; OXIDES; XAFS; SIZE; FE; FERROMAGNETISM; NANOPARTICLES AB Effective manipulation of magnetic spin within a semiconductor leading to a search for ferromagnets with semiconducting properties has evolved into an important field of dilute magnetic semiconductors (DMS). Although a lot of research is focused on understanding the still controversial origin of magnetism, efforts are also underway to develop new materials with higher magnetic temperatures for spintronics applications. However, so far, efforts toward quantum-dots(QDs)-based DMS materials are plagued with problems of phase separation, leading to nonuniform distribution of dopant ions. In this work, we have developed a strategy to synthesize highly crystalline, single-domain DMS system starting from a small magnetic core and allowing it to diffuse uniformly inside a thick CdS semiconductor matrix and achieve DMS QDs. X-ray absorption fine structure (XAFS) spectroscopy and energy-dispersive X-ray spectroscopy scanning transmission electron microscopy (STEM-EDX) indicates the homogeneous distribution of magnetic impurities inside the semiconductor QDs leading to superior magnetic property. Further, the versatility of this technique was demonstrated by obtaining ultra large particles (similar to 60 nm) with uniform doping concentration as well as demonstrating the high quality magnetic response. C1 [Saha, Avijit; Viswanatha, Ranjani] Jawaharlal Nehru Ctr Adv Sci Res, New Chem Unit, Bangalore 560064, Karnataka, India. [Shetty, Amitha; Pavan, A. R.; Viswanatha, Ranjani] Jawaharlal Nehru Ctr Adv Sci Res, Int Ctr Mat Sci, Bangalore 560064, Karnataka, India. [Chattopadhyay, Soma] CSRRI IIT, Sect ID 10, Adv Photon Source, 9700 South Cass Ave, Lemont, IL 60439 USA. [Shibata, Tomohiro] Argonne Natl Lab, MRCAT, Argonne, IL 60439 USA. [Chattopadhyay, Soma; Shibata, Tomohiro] Illinois Inst Technol, Dept Phys, Adv Mat Grp, Chicago, IL 60616 USA. [Chattopadhyay, Soma] Elgin Community Coll, Dept Phys Sci, 1700 Spartan Dr, Elgin, IL 60123 USA. [Shibata, Tomohiro] Kennametal Inc, Mat Sci, 1600 Technol Way, Latrobe, PA 15650 USA. RP Viswanatha, R (reprint author), Jawaharlal Nehru Ctr Adv Sci Res, New Chem Unit, Bangalore 560064, Karnataka, India.; Viswanatha, R (reprint author), Jawaharlal Nehru Ctr Adv Sci Res, Int Ctr Mat Sci, Bangalore 560064, Karnataka, India. EM rv@jncasr.ac.in RI ID, MRCAT/G-7586-2011 FU JNCASR, Sheikh Saqr Laboratory; Department of Science and Technology, Government of India; CSIR; Sheikh Saqr Career Award Fellowship; MRCAT host institutions; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX A.S. and R.V. thank JNCASR, Sheikh Saqr Laboratory and Department of Science and Technology, Government of India for financial support. A.S. thanks CSIR for research fellowship. RV. is grateful for the Sheikh Saqr Career Award Fellowship. We thank Rana Saha and Somnath Ghara for magnetic measurement and Dr. Jay Ghatak and Kannan Dhandapani for TEM imaging. Authors (S.C. and T.S.) would like to thank Dr. Vladislav Zyryanov for his help with experimental setup during XAFS measurement. MRCAT is funded by MRCAT host institutions. APS is funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under contract number DE-AC02-06CH11357. NR 56 TC 3 Z9 3 U1 18 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 7 PY 2016 VL 7 IS 13 BP 2420 EP 2428 DI 10.1021/acs.jpclett.6b01099 PG 9 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DQ8JP UT WOS:000379457400022 PM 27295453 ER PT J AU Ding, TNX Hou, L van der Meer, H Alivisatos, AP Orrit, M AF Ding, Tina X. Hou, Lei van der Meer, Harmen Alivisatos, A. Paul Orrit, Michel TI Hundreds-fold Sensitivity Enhancement of Photothermal Microscopy in Near-Critical Xenon SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID ROOM-TEMPERATURE; OPTICAL-ABSORPTION; SINGLE MOLECULES; SEMICONDUCTOR NANOCRYSTALS; CRITICAL POINT; SPECTROSCOPY; LUMINESCENCE; LIQUID AB Photothermal absorption microscopy of single Au nanoparticles was conducted at temperatures and pressures near the critical point of Xenon (T-c = 16.583 degrees C, P-c = 5.842 MPa). The divergence of the thermal expansion coefficient at the critical point makes the refractive index highly sensitive to changes in temperature, which directly translates to a large enhancement of the photothermal signal. We find that measurements taken near the critical point of Xe give a signal enhancement factor of up to 440 +/- 130 over those taken in glycerol. The highest sensitivity recorded here corresponds to power dissipation of 64 pW, achieving a signal-to-noise ratio of 9.4 for 5 nm Au nanoparticles with an integration time of 50 ms, making this the most sensitive of any absorption microscopy technique reported to date. Enhancing the sensitivity of absorption microscopy lowers the operating heating power, allowing the technique to be more compatible with absorbers with absorption coefficient and photochemical stability lower than that of Au. C1 [Ding, Tina X.; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Alivisatos, A. Paul] Univ Calif Berkeley, Dept Mat Sci, Berkeley, CA 94720 USA. [Ding, Tina X.; Alivisatos, A. Paul] Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Alivisatos, A. Paul] Kavli Energy NanoSci Inst, Berkeley, CA 94720 USA. [Hou, Lei; van der Meer, Harmen; Orrit, Michel] Leiden Inst Phys, Huygens Kamerlingh Onnes Lab, Postbus 9504, NL-2300 RA Leiden, Netherlands. RP Orrit, M (reprint author), Leiden Inst Phys, Huygens Kamerlingh Onnes Lab, Postbus 9504, NL-2300 RA Leiden, Netherlands. EM orrit@physics.leidenuniv.nl RI Alivisatos , Paul /N-8863-2015; OI Alivisatos , Paul /0000-0001-6895-9048; HOU, Lei /0000-0003-1077-6147 FU National Science Foundation (NSF) [DGE 1106400]; joint NSF-NWO program under the Global Research Opportunities Worldwide (GROW) Fellowship; Chinese Scholarship Council FX T.X.D. acknowledges the National Science Foundation (NSF) Research Fellowship under Grant DGE 1106400 as well as the joint NSF-NWO program under the Global Research Opportunities Worldwide (GROW) Fellowship. L.H. benefitted from a grant from the Chinese Scholarship Council. We thank Dr. Alexander Gaiduk and Dr. Paul Ruijgrok for pointing out the large enhancement of photothermal coefficients in near critical fluids. NR 32 TC 3 Z9 3 U1 4 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 7 PY 2016 VL 7 IS 13 BP 2524 EP 2529 DI 10.1021/acs.jpclett.6b00964 PG 6 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DQ8JP UT WOS:000379457400040 PM 27295542 ER PT J AU Yang, D Xu, PH Browning, ND Gates, BC AF Yang, Dong Xu, Pinghong Browning, Nigel D. Gates, Bruce C. TI Tracking Rh Atoms in Zeolite HY: First Steps of Metal Cluster Formation and Influence of Metal Nuclearity on Catalysis of Ethylene Hydrogenation and Ethylene Dimerization SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID CARBONYL HYDRIDE COMPLEXES; DEALUMINATED Y-ZEOLITE; GAS SHIFT REACTION; SUPPORTED RHODIUM; CO OXIDATION; STRUCTURAL-CHARACTERIZATION; SI/AL RATIO; SITE; SURFACE; ETHENE AB The initial steps of rhodium cluster formation from zeolite-supported mononuclear Rh(C2H4)(2) complexes in H-2 at 373 K and 1 bar were investigated by infrared and extended X-ray absorption fine structure spectroscopies and scanning transmission electron microscopy (STEM). The data show that ethylene ligands on the rhodium react with H-2 to give supported rhodium hydrides and trigger the formation of rhodium clusters. STEM provided the first images of the smallest rhodium clusters (Rh-2) and their further conversion into larger clusters. The samples were investigated in a plug-flow reactor as catalysts for the conversion of ethylene + H-2 in a molar ratio of 4:1 at 1 bar and 298 K, with the results showing how the changes in catalyst structure affect the activity and selectivity; the rhodium clusters are more active for hydrogenation of ethylene than the single-site complexes, which are more selective for dimerization of ethylene to give butenes. C1 [Yang, Dong; Xu, Pinghong; Gates, Bruce C.] Univ Calif Davis, Dept Chem Engn, Davis, CA 95616 USA. [Browning, Nigel D.] Pacific Northwest Natl Lab, Phys & Computat Sci, 902 Battelle Blvd, Richland, WA 99352 USA. RP Gates, BC (reprint author), Univ Calif Davis, Dept Chem Engn, Davis, CA 95616 USA. EM bcgates@ucdavis.edu FU U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences [DE-FG02-04ER15513]; DOE [DE-AC05-76RL01830]; DOE's Office of Biological and Environmental Research FX This work was supported by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences, Grant DE-FG02-04ER15513. A portion of this work was done as part of the Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL) (under Contract DE-AC05-76RL01830), operated for DOE by Battelle. It was conducted under the Laboratory Directed Research and Development Program at PNNL. A portion of the research was performed using EMSL, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research and located at PNNL. We acknowledge beam time at beamline 4-1 at the Stanford Synchrotron Radiation Lightsource supported by the DOE Division of Materials Sciences. We thank the beamline staff for valuable support. NR 40 TC 0 Z9 0 U1 15 U2 33 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 7 PY 2016 VL 7 IS 13 BP 2537 EP 2543 DI 10.1021/acs.jpclett.6b01153 PG 7 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DQ8JP UT WOS:000379457400042 PM 27315020 ER PT J AU Tian, ZQ Dai, S Jiang, DE AF Tian, Ziqi Dai, Sheng Jiang, De-en TI Site Partition: Turning One Site into Two for Adsorbing CO2 SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID METAL-ORGANIC FRAMEWORKS; CARBON-DIOXIDE CAPTURE; PORE-SPACE PARTITION; 2-DIMENSIONAL POLYMER; ADSORPTION; COORDINATION; SEPARATION; CLUSTERS; DEFECTS; MOF AB We propose the concept of site partition to explain the role of guest molecules in increasing CO2 uptake in metal organic frameworks and to design new covalent porous materials for CO2 capture. From grand canonical Monte Carlo simulations of CO2 sorption in the recently synthesized CPM-33 MOFs, we show that guest insertion divides one open metal site into two relatively strong binding sites, hence dramatically increasing CO2 uptake. Further, we extend the site partition concept to covalent organic frameworks with large free volume. After insertion of a designed geometry-matching guest, we show that the volumetric uptake of CO2 doubles. Therefore, the concept of site partition can be used to engineer the pore space of nanoporous materials for higher gas uptake. C1 [Tian, Ziqi; Jiang, De-en] Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. [Dai, Sheng] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Dai, Sheng] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. RP Jiang, DE (reprint author), Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. EM de-en.jiang@ucr.edu RI Dai, Sheng/K-8411-2015; Jiang, De-en/D-9529-2011 OI Dai, Sheng/0000-0002-8046-3931; Jiang, De-en/0000-0001-5167-0731 FU Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. We thank Dr. Xianhui Bu and Dr. Pingyun Feng for very helpful discussions. This research used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 39 TC 1 Z9 1 U1 13 U2 34 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 7 PY 2016 VL 7 IS 13 BP 2568 EP 2572 DI 10.1021/acs.jpclett.6b01141 PG 5 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DQ8JP UT WOS:000379457400047 PM 27320252 ER PT J AU Rodriguez, JA Liu, P Graciani, J Senanayake, SD Grinter, DC Stacchiola, D Hrbek, J Fernandez-Sanz, J AF Rodriguez, Jose A. Liu, Ping Graciani, Jesus Senanayake, Sanjaya D. Grinter, David C. Stacchiola, Dario Hrbek, Jan Fernandez-Sanz, Javier TI Inverse Oxide/Metal Catalysts in Fundamental Studies and Practical Applications: A Perspective of Recent Developments SO JOURNAL OF PHYSICAL CHEMISTRY LETTERS LA English DT Article ID GAS SHIFT REACTION; METAL-SUPPORT INTERACTIONS; SCANNING-TUNNELING-MICROSCOPY; ACTIVE EDGE SITES; CO OXIDATION; IN-SITU; OXIDE INTERFACE; MODEL CATALYST; METHANOL SYNTHESIS; DEFECT STRUCTURE AB Inverse oxide/metal catalysts have shown to be excellent systems for studying the role of the oxide and oxide-metal interface in catalytic reactions. These systems can have special structural and catalytic properties due to strong oxide-metal interactions difficult to attain when depositing a metal on a regular oxide support. Oxide phases that are not seen or are metastable in a bulk oxide can become stable in an oxide/metal system opening the possibility for new chemical properties. Using these systems, it has been possible to explore fundamental properties of the metal-oxide interface (composition, structure, electronic state), which determine catalytic performance in the oxidation of CO, the water-gas shift and the hydrogenation of CO2 to methanol. Recently, there has been a significant advance in the preparation of oxide/metal catalysts for technical or industrial applications. One goal is to identify methods able to control in a precise way the size of the deposited oxide particles and their structure on the metal substrate. C1 [Rodriguez, Jose A.; Liu, Ping; Senanayake, Sanjaya D.; Grinter, David C.; Stacchiola, Dario; Hrbek, Jan] Brookhaven Natl Lab, Dept Chem, Upton 11776, NY USA. [Rodriguez, Jose A.; Liu, Ping] SUNY Stony Brook, Dept Chem, Stony Brook 11749, NY USA. [Graciani, Jesus; Fernandez-Sanz, Javier] Univ Seville, Dept Quim Fis, E-41012 Seville, Spain. RP Rodriguez, JA (reprint author), Brookhaven Natl Lab, Dept Chem, Upton 11776, NY USA.; Rodriguez, JA (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook 11749, NY USA. EM rodrigez@bnl.gov RI Stacchiola, Dario/B-1918-2009; Senanayake, Sanjaya/D-4769-2009; OI Stacchiola, Dario/0000-0001-5494-3205; Senanayake, Sanjaya/0000-0003-3991-4232; Grinter, David/0000-0001-6089-119X FU U.S. Department of Energy (Chemical Sciences Division) [DE-SC0012704]; U.S. Department of Energy FX Many of the studies described above were done in collaboration with members of the Catalysis Group at Brookhaven National Laboratory and collaborators from the Universidad Central de Venezuela and the Institute of Catalysis-Madrid: A Baber, S. Agnoli, L. Barrio, M. Estrella, J. Evans, M. Fernandez-Garcia, J. Hanson, A. Homes, S. Kundu, S. Ma, A. Martinez-Arias, K. Mudiyanselage, J.-B. Park, P.J. Ramirez, A Vidal, F. Yang, and X. Zhao. Many thanks to all of them. The work carried out at Brookhaven National Laboratory was supported by the U.S. Department of Energy (Chemical Sciences Division, DE-SC0012704). Part of these studies was done at the National Synchrotron Light Source and at the Center for Functional Nanomaterials of BNL, which are supported by the U.S. Department of Energy. NR 80 TC 7 Z9 7 U1 32 U2 51 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1948-7185 J9 J PHYS CHEM LETT JI J. Phys. Chem. Lett. PD JUL 7 PY 2016 VL 7 IS 13 BP 2627 EP 2639 DI 10.1021/acs.jpclett.6b00499 PG 13 WC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Atomic, Molecular & Chemical SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DQ8JP UT WOS:000379457400057 PM 27327114 ER PT J AU Stygar, WA Reisman, DB Stoltzfus, BS Austin, KN Ao, T Benage, JF Breden, EW Cooper, RA Cuneo, ME Davis, JP Ennis, JB Gard, PD Greiser, GW Gruner, FR Haill, TA Hutsel, BT Jones, PA LeChien, KR Leckbee, JJ Lewis, SA Lucero, DJ McKee, GR Moore, JK Mulville, TD Muron, DJ Root, S Savage, ME Sceiford, ME Spielman, RB Waisman, EM Wisher, ML AF Stygar, W. A. Reisman, D. B. Stoltzfus, B. S. Austin, K. N. Ao, T. Benage, J. F. Breden, E. W. Cooper, R. A. Cuneo, M. E. Davis, J. -P. Ennis, J. B. Gard, P. D. Greiser, G. W. Gruner, F. R. Haill, T. A. Hutsel, B. T. Jones, P. A. LeChien, K. R. Leckbee, J. J. Lewis, S. A. Lucero, D. J. McKee, G. R. Moore, J. K. Mulville, T. D. Muron, D. J. Root, S. Savage, M. E. Sceiford, M. E. Spielman, R. B. Waisman, E. M. Wisher, M. L. TI Conceptual design of a 10(13)-W pulsed-power accelerator for megajoule-class dynamic-material-physics experiments SO PHYSICAL REVIEW ACCELERATORS AND BEAMS LA English DT Article ID ISENTROPIC COMPRESSION EXPERIMENTS; GENESIS; DRIVER AB We have developed a conceptual design of a next-generation pulsed-power accelerator that is optimized for megajoule-class dynamic-material-physics experiments. Sufficient electrical energy is delivered by the accelerator to a physics load to achieve-within centimeter-scale samples-material pressures as high as 1 TPa. The accelerator design is based on an architecture that is founded on three concepts: single-stage electrical-pulse compression, impedance matching, and transit-time-isolated drive circuits. The prime power source of the accelerator consists of 600 independent impedance-matched Marx generators. Each Marx comprises eight 5.8-GW bricks connected electrically in series, and generates a 100-ns 46-GW electrical-power pulse. A 450-ns-long water-insulated coaxial-transmission-line impedance transformer transports the power generated by each Marx to a system of twelve 2.5-m-radius water-insulated conical transmission lines. The conical lines are connected electrically in parallel at a 66-cm radius by a water-insulated 45-post sextuple-post-hole convolute. The convolute sums the electrical currents at the outputs of the conical lines, and delivers the combined current to a single solid-dielectric-insulated radial transmission line. The radial line in turn transmits the combined current to the load. Since much of the accelerator is water insulated, we refer to it as Neptune. Neptune is 40 m in diameter, stores 4.8 MJ of electrical energy in its Marx capacitors, and generates 28 TW of peak electrical power. Since the Marxes are transit-time isolated from each other for 900 ns, they can be triggered at different times to construct-over an interval as long as 1 mu s-the specific load-current time history required for a given experiment. Neptune delivers 1 MJ and 20MA in a 380-ns current pulse to an 18-m Omega load; hence Neptune is a megajoule-class 20-MA arbitrary waveform generator. Neptune will allow the international scientific community to conduct dynamic equation-of-state, phase-transition, mechanical-property, and other material-physics experiments with a wide variety of drive-pressure time histories. C1 [Stygar, W. A.; Reisman, D. B.; Stoltzfus, B. S.; Austin, K. N.; Ao, T.; Benage, J. F.; Breden, E. W.; Cuneo, M. E.; Davis, J. -P.; Gard, P. D.; Haill, T. A.; Hutsel, B. T.; Jones, P. A.; Leckbee, J. J.; Lewis, S. A.; Lucero, D. J.; McKee, G. R.; Moore, J. K.; Mulville, T. D.; Muron, D. J.; Root, S.; Savage, M. E.; Sceiford, M. E.; Waisman, E. M.; Wisher, M. L.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. [Cooper, R. A.] Gen Atom Co, San Diego, CA 92186 USA. [Ennis, J. B.] NWL Capacitor Div, Snow Hill, NC 28580 USA. [Greiser, G. W.] CSI Technol, Vista, CA 92081 USA. [Gruner, F. R.] Kinetech Corp, Cedar Crest, NM 87008 USA. [LeChien, K. R.] Natl Nucl Secur Adm, Washington, DC 20585 USA. [Spielman, R. B.] Idaho State Univ, Pocatello, ID 83209 USA. RP Stygar, WA (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. FU National Nuclear Security Administration; Laboratory Directed Research and Development Program at Sandia National Laboratories; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors gratefully acknowledge the following for invaluable contributions: Farhat Beg, Mike Campbell, Christine Coverdale, David Fehl, Dawn Flicker, Doug Fulton, Ron Gilgenbach, Mark Gilmore, Clint Hall, David Hammer, Mark Herrmann, Robert Hohlfelder, Dan Jobe, Michael Jones, Kirk Kielholtz, Joel Lash, Jane Lehr, Ray Leeper, Finis Long, John Maenchen, Keith Matzen, Mike Mazarakis, Bob McCrory, John Porter, David Sandoval, Ray Scarpetti, Edl Schamiloglu, Ralph Schneider, Jens Schwarz, Dan Sinars, Pete Wakeland, and JoeWoodworth. We are also extremely indebted to our many other colleagues at the following organizations for their gracious and sustained scientific support: Sandia National Laboratories, ASR Corporation, Barth Electronics, C-Lec Plastics, Cornell University, CSI Technologies, EG&G, General Atomics, Idaho State University, Kinetech Corporation, L-3 Communications, Laboratory for Laser Energetics at the University of Rochester, Lawrence Livermore National Laboratory, Los Alamos National Laboratory, National Nuclear Security Administration, National Security Technologies, Naval Research Laboratory, NWL Capacitor Division, Raytheon-Ktech Corporation, Tech Source Consulting, Texas Tech University, University of California at San Diego, University of Michigan at Ann Arbor, University of Missouri at Columbia, University of Nevada at Reno, University of New Mexico, University of Texas at Austin, Voss Scientific, Votaw Precision Technologies, and Weizmann Institute. This work was supported by the National Nuclear Security Administration, and the Laboratory Directed Research and Development Program at Sandia National Laboratories. Sandia is a multiprogram laboratory operated by Sandia Corporation, a Lockheed Martin Company, for the United States Department of Energy's National Nuclear Security Administration under Contract No. DE-AC04-94AL85000. NR 40 TC 1 Z9 1 U1 5 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9888 J9 PHYS REV ACCEL BEAMS JI Phys. Rev. Accel. Beams PD JUL 7 PY 2016 VL 19 IS 7 AR 070401 DI 10.1103/PhysRevAccelBeams.19.070401 PG 14 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DQ6YP UT WOS:000379353400001 ER PT J AU Choquette, AK Smith, CR Sichel-Tissot, RJ Moon, EJ Scafetta, MD Di Gennaro, E Granozio, FM Karapetrova, E May, SJ AF Choquette, A. K. Smith, C. R. Sichel-Tissot, R. J. Moon, E. J. Scafetta, M. D. Di Gennaro, E. Granozio, F. Miletto Karapetrova, E. May, S. J. TI Octahedral rotation patterns in strained EuFeO3 and other Pbnm perovskite films: Implications for hybrid improper ferroelectricity SO PHYSICAL REVIEW B LA English DT Article ID SRRUO3 THIN-FILMS; OXIDE HETEROSTRUCTURES; CRYSTAL-STRUCTURE; MULTIFUNCTIONAL MATERIALS; PROPERTY RELATIONSHIPS; SOLID-SOLUTIONS; SUPERLATTICES; DIFFRACTION; TRANSITION; TEMPERATURES AB We report the relationship between epitaxial strain and the crystallographic orientation of the in-phase rotation axis and A-site displacements in Pbnm-type perovskite films. Synchrotron diffraction measurements of EuFeO3 films under strain states ranging from 2% compressive to 0.9% tensile on cubic or rhombohedral substrates exhibit a combination of a(-)a(+)c(-) and a(+)a(-)c(-) rotational patterns. We compare the EuFeO3 behavior with previously reported experimental and theoretical work on strained Pbnm-type films on nonorthorhombic substrates, as well as additional measurements from LaGaO3, LaFeO3, and Eu0.7Sr0.3MnO3 films on SrTiO3. Compiling the results from various material systems reveals a general strain dependence in which compressive strain strongly favors a(-)a(+)c(-) and a(+)a(-)c(-) rotation patterns and tensile strain weakly favors a(-)a(-)c(+) structures. In contrast, EuFeO3 films grown on Pbnm-type GdScO3 under 2.3% tensile strain take on a uniform a(-)a(+)c(-) rotation pattern imprinted from the substrate, despite strain considerations that favor the a(-)a(-)c(+) pattern. These results point to the use of substrate imprinting as a more robust route than strain for tuning the crystallographic orientations of the octahedral rotations and A-site displacements needed to realize rotation-induced hybrid improper ferroelectricity in oxide heterostructures. C1 [Choquette, A. K.; Smith, C. R.; Sichel-Tissot, R. J.; Moon, E. J.; Scafetta, M. D.; May, S. J.] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Sichel-Tissot, R. J.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Di Gennaro, E.; Granozio, F. Miletto] Univ Naples Federico II, CNR SPIN, I-80126 Naples, Italy. [Di Gennaro, E.; Granozio, F. Miletto] Univ Naples Federico II, Dipartimento Fis, I-80126 Naples, Italy. [Karapetrova, E.] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60439 USA. RP May, SJ (reprint author), Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. EM smay@coe.drexel.edu RI May, Steven/D-8563-2011; Di Gennaro, Emiliano/G-6311-2010 OI May, Steven/0000-0002-8097-1549; Di Gennaro, Emiliano/0000-0003-4231-9776 FU National Science Foundation [DMR-1151649]; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX We thank Christian Schleputz for assistance with the diffraction measurements. We are grateful to James Rondinelli and Craig Fennie for useful discussions. Work at Drexel was supported by the National Science Foundation (DMR-1151649). This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. NR 73 TC 2 Z9 2 U1 15 U2 35 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 7 PY 2016 VL 94 IS 2 AR 024105 DI 10.1103/PhysRevB.94.024105 PG 8 WC Physics, Condensed Matter SC Physics GA DR1ZB UT WOS:000379702300003 ER PT J AU Kogoj, J Vidmar, L Mierzejewski, M Trugman, SA Bonca, J AF Kogoj, Jan Vidmar, Lev Mierzejewski, Marcin Trugman, Stuart A. Bonca, Janez TI Thermalization after photoexcitation from the perspective of optical spectroscopy SO PHYSICAL REVIEW B LA English DT Article ID QUANTUM-SYSTEMS; RELAXATION; ELECTRONS; POLARON AB We analyze the thermalization of a photoexcited charge carrier coupled to a single branch of quantum phonons within the Holstein model. To this end, we calculate the far-from-equilibrium time evolution of a pure many-body state and compare it with predictions of the thermal Gibbs ensemble. We show that at strong enough carrier excitation, the nonequilibrium system evolves towards a thermal steady state. Our analysis is based on two classes of observables. First, the occupations of fermionic momenta, which are the eigenvalues of the one-particle density matrix, match in the steady state the values in the corresponding Gibbs ensemble. This indicates thermalization of static fermionic correlations on the entire lattice. Second, the dynamic current-current correlations, including the time-resolved optical conductivity, also take the form of their thermal counterparts. Remarkably, both static and dynamic fermionic correlations thermalize with identical temperatures. Our results suggest that the subsequent relaxation processes, observed in time-resolved ultrafast spectroscopy, may be efficiently described by applying quasithermal approaches, e.g., multitemperature models. C1 [Kogoj, Jan; Vidmar, Lev; Bonca, Janez] J Stefan Inst, Ljubljana 1000, Slovenia. [Vidmar, Lev] Univ Munich, Dept Phys, D-80333 Munich, Germany. [Vidmar, Lev] Univ Munich, Arnold Sommerfeld Ctr Theoret Phys, D-80333 Munich, Germany. [Mierzejewski, Marcin] Univ Silesia, Inst Phys, PL-40007 Katowice, Poland. [Trugman, Stuart A.] Los Alamos Natl Lab, Ctr Integrated Nanotechol, Los Alamos, NM USA. [Bonca, Janez] Univ Ljubljana, Fac Math & Phys, Ljubljana 1000, Slovenia. RP Kogoj, J (reprint author), J Stefan Inst, Ljubljana 1000, Slovenia. RI Vidmar, Lev/J-2464-2014; OI Trugman, Stuart/0000-0002-6688-7228 FU ARRS, Slovenia [P1-0044]; Polish National Science Center [DEC-2013/11/B/ST3/00824] FX We acknowledge stimulating discussions with U. Bowensiepen, M. Eckstein, C. Giannetti, and L. Perfetti. J.B. acknowledges discussions with A. Polkovnikov and M. Rigol as well as the support by the P1-0044 of ARRS, Slovenia. L.V. acknowledges discussions with F. Heidrich-Meisner, F. Dorfner, and E. Jeckelmann. M.M. acknowledges support from the DEC-2013/11/B/ST3/00824 project of the Polish National Science Center. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. NR 71 TC 3 Z9 3 U1 5 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 7 PY 2016 VL 94 IS 1 AR 014304 DI 10.1103/PhysRevB.94.014304 PG 10 WC Physics, Condensed Matter SC Physics GA DR1YJ UT WOS:000379700500002 ER PT J AU Kamano, H Nakamura, SX Lee, TSH Sato, T AF Kamano, H. Nakamura, S. X. Lee, T. -S. H. Sato, T. TI Isospin decomposition of gamma N -> N* transitions within a dynamical coupled-channels model SO PHYSICAL REVIEW C LA English DT Article ID NUCLEON RESONANCE REGION; PION-PHOTOPRODUCTION; MESON PRODUCTION; ENERGY-RANGE; NEUTRONS AB By extending the dynamical coupled-channels analysis performed in our previous work [Phys. Rev. C 88, 035209 (2013)] to include the available data of photoproduction of pi mesons off neutrons, the transition amplitudes for the photoexcitation of the neutron-to-nucleon resonances, gamma n -> N*, at the resonance pole positions are determined. The combined fits to the data for both the proton- and neutron-target reactions also revise our results for the resonance pole positions and the gamma p -> N* transition amplitudes. Our results allow an isospin decomposition of the gamma N -> N* transition amplitudes for the isospin I = 1/2 N* resonances, which is necessary for testing hadron structure models and gives crucial inputs for constructing models of neutrino-induced reactions in the nucleon resonance region. C1 [Kamano, H.] High Energy Accelerator Res Org KEK, Inst Particle & Nucl Studies, KEK Theory Ctr, Tsukuba, Ibaraki 3050801, Japan. [Kamano, H.] KEK, IPNS, KEK Theory Ctr, J PARC Branch, Tokai, Ibaraki 3191106, Japan. [Nakamura, S. X.; Sato, T.] Osaka Univ, Dept Phys, Toyonaka, Osaka 5600043, Japan. [Lee, T. -S. H.] Argonne Natl Lab, Div Phys, Argonne, IL 60439 USA. RP Kamano, H (reprint author), High Energy Accelerator Res Org KEK, Inst Particle & Nucl Studies, KEK Theory Ctr, Tsukuba, Ibaraki 3050801, Japan.; Kamano, H (reprint author), KEK, IPNS, KEK Theory Ctr, J PARC Branch, Tokai, Ibaraki 3191106, Japan. EM kamano@post.kek.jp RI Nakamura, Satoshi/M-9097-2016 OI Nakamura, Satoshi/0000-0002-7542-8859 FU Japan Society for the Promotion of Science (JSPS) KAKENHI [25800149, 16K05354]; MEXT KAKENH [25105010]; US Department of Energy, Office of Nuclear Physics Division [DE-AC02-06CH11357]; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Japan Society for the Promotion of Science (JSPS) KAKENHI Grants No. 25800149 (H.K.) and No. 16K05354 (T.S.), the MEXT KAKENHI Grant No. 25105010 (T.S.), and by the US Department of Energy, Office of Nuclear Physics Division, under Contract No. DE-AC02-06CH11357. This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231, and resources provided on Blues and/or Fusion, high-performance computing cluster operated by the Laboratory Computing Resource Center at Argonne National Laboratory. NR 43 TC 2 Z9 2 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUL 7 PY 2016 VL 94 IS 1 AR 015201 DI 10.1103/PhysRevC.94.015201 PG 14 WC Physics, Nuclear SC Physics GA DR2FR UT WOS:000379720900001 ER PT J AU Bose, A Woo, KM Betti, R Campbell, EM Mangino, D Christopherson, AR McCrory, RL Nora, R Regan, SP Goncharov, VN Sangster, TC Forrest, CJ Frenje, J Johnson, MG Glebov, VY Knauer, JP Marshall, FJ Stoeckl, C Theobald, W AF Bose, A. Woo, K. M. Betti, R. Campbell, E. M. Mangino, D. Christopherson, A. R. McCrory, R. L. Nora, R. Regan, S. P. Goncharov, V. N. Sangster, T. C. Forrest, C. J. Frenje, J. Johnson, M. Gatu Glebov, V. Yu Knauer, J. P. Marshall, F. J. Stoeckl, C. Theobald, W. TI Core conditions for alpha heating attained in direct-drive inertial confinement fusion SO PHYSICAL REVIEW E LA English DT Article AB It is shown that direct-drive implosions on the OMEGA laser have achieved core conditions that would lead to significant alpha heating at incident energies available on the National Ignition Facility (NIF) scale. The extrapolation of the experimental results from OMEGA to NIF energy assumes only that the implosion hydrodynamic efficiency is unchanged at higher energies. This approach is independent of the uncertainties in the physical mechanism that degrade implosions on OMEGA, and relies solely on a volumetric scaling of the experimentally observed core conditions. It is estimated that the current best-performing OMEGA implosion [Regan et al., Phys. Rev. Lett. 117, 025001 (2016)] extrapolated to a 1.9 MJ laser driver with the same illumination configuration and laser-target coupling would produce 125 kJ of fusion energy with similar levels of alpha heating observed in current highest performing indirect-drive NIF implosions. C1 [Bose, A.; Woo, K. M.; Betti, R.; Christopherson, A. R.; Theobald, W.] Univ Rochester, Fus Sci Ctr, Rochester, NY 14623 USA. [Bose, A.; Woo, K. M.; Betti, R.; Campbell, E. M.; Mangino, D.; Christopherson, A. R.; McCrory, R. L.; Regan, S. P.; Goncharov, V. N.; Sangster, T. C.; Glebov, V. Yu; Knauer, J. P.; Marshall, F. J.; Stoeckl, C.; Theobald, W.] Univ Rochester, Laser Energet Lab, 250 E River Rd, Rochester, NY 14623 USA. [Nora, R.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Frenje, J.; Johnson, M. Gatu] MIT, Plasma Sci & Fus Ctr, 77 Massachusetts Ave, Cambridge, MA 02139 USA. RP Bose, A (reprint author), Univ Rochester, Fus Sci Ctr, Rochester, NY 14623 USA.; Bose, A (reprint author), Univ Rochester, Laser Energet Lab, 250 E River Rd, Rochester, NY 14623 USA. FU U.S. Department of Energy [DE-FC02-04ER54789, DE-NA0001944]; NYSERDA FX The authors thank D. Shvarts for many useful discussions. This work has been supported by the U.S. Department of Energy under Cooperative Agreements DE-FC02-04ER54789 (Office of Fusion Energy Sciences) and DE-NA0001944 (National Nuclear Security Administration), and by the NYSERDA. NR 30 TC 2 Z9 2 U1 7 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD JUL 7 PY 2016 VL 94 IS 1 AR 011201 DI 10.1103/PhysRevE.94.011201 PG 5 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DR2HM UT WOS:000379725600002 PM 27575069 ER PT J AU Deffner, S Paz, JP Zurek, WH AF Deffner, Sebastian Paz, Juan Pablo Zurek, Wojciech H. TI Quantum work and the thermodynamic cost of quantum measurements SO PHYSICAL REVIEW E LA English DT Article ID DECOHERENCE; INFORMATION AB Quantum work is usually determined from two projective measurements of the energy at the beginning and at the end of a thermodynamic process. However, this paradigm cannot be considered thermodynamically consistent as it does not account for the thermodynamic cost of these measurements. To remedy this conceptual inconsistency we introduce a paradigm that relies only on the expected change of the average energy given the initial energy eigenbasis. In particular, we completely omit quantum measurements in the definition of quantum work, and hence quantum work is identified as a thermodynamic quantity of only the system. As main results we derive a modified quantum Jarzynski equality and a sharpened maximum work theorem in terms of the information free energy. A comparison of our results with the standard approach allows one to quantify the informational cost of projective measurements. C1 [Deffner, Sebastian; Zurek, Wojciech H.] Los Alamos Natl Lab, Theoret Div, Los Alamos, NM 87545 USA. [Deffner, Sebastian] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Paz, Juan Pablo] UBA, FCEyN, Dept Fis, Ciudad Univ Pabellon 1, RA-1428 Buenos Aires, DF, Argentina. [Paz, Juan Pablo] UBA, FCEyN, IFIBA CONICET, Ciudad Univ Pabellon 1, RA-1428 Buenos Aires, DF, Argentina. RP Deffner, S (reprint author), Los Alamos Natl Lab, Theoret Div, Los Alamos, NM 87545 USA.; Deffner, S (reprint author), Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RI Deffner, Sebastian/C-5170-2008 OI Deffner, Sebastian/0000-0003-0504-6932 FU U.S. Department of Energy through a LANL Director's Funded Fellowship; Foundational Questions Institute [2015-144057] FX It is a pleasure to thank Jordan M. Horowitz, Christopher Jarzynski, Jim Crutchfield, and Gavin Crooks for interesting and insightful discussions. S.D. acknowledges financial support by the U.S. Department of Energy through a LANL Director's Funded Fellowship, and W.H.Z. acknowledges partial support by the Foundational Questions Institute Grant No. 2015-144057 on "Physics of What Happens". NR 57 TC 2 Z9 2 U1 5 U2 8 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD JUL 7 PY 2016 VL 94 IS 1 AR 010103 DI 10.1103/PhysRevE.94.010103 PG 5 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DR2HM UT WOS:000379725600001 PM 27575061 ER PT J AU Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Agnew, JP Alexeev, GD Alkhazov, G Alton, A Askew, A Atkins, S Augsten, K Aushev, V Aushev, Y Avila, C Badaud, F Bagby, L Baldin, B Bandurin, DV Banerjee, S Barberis, E Baringer, P Bartlett, JF Bassler, U Bazterra, V Bean, A Begalli, M Bellantoni, L Beri, SB Bernardi, G Bernhard, R Bertram, I Besancon, M Beuselinck, R Bhat, PC Bhatia, S Bhatnagar, V Blazey, G Blessing, S Bloom, K Boehnlein, A Boline, D Boos, EE Borissov, G Borysova, M Brandt, A Brandt, O Brochmann, M Brock, R Bross, A Brown, D Bu, XB Buehler, M Buescher, V Bunichev, V Burdin, S Buszello, CP Camacho-Perez, E Casey, BCK Castilla-Valdez, H Caughron, S Chakrabarti, S Chan, KM Chandra, A Chapon, E Chen, G Cho, SW Choi, S Choudhary, B Cihangir, S Claes, D Clutter, J Cooke, M Cooper, WE Corcoran, M Couderc, F Cousinou, MC Cuth, J Cutts, D Das, A Davies, G de Jong, SJ De La Cruz-Burelo, E Deliot, F Demina, R Denisov, D Denisov, SP Desai, S Deterre, C DeVaughan, K Diehl, HT Diesburg, M Ding, PF Dominguez, A Drutskoy, A Dubey, A Dudko, LV Duperrin, A Dutt, S Eads, M Edmunds, D Ellison, J Elvira, VD Enari, Y Evans, H Evdokimov, A Evdokimov, VN Faure, A Feng, L Ferbel, T Fiedler, F Filthaut, F Fisher, W Fisk, HE Fortner, M Fox, H Franc, J Fuess, S Garbincius, PH Garcia-Bellido, A Garcia-Gonzalez, JA Gavrilov, V Geng, W Gerber, CE Gershtein, Y Ginther, G Gogota, O Golovanov, G Grannis, PD Greder, S Greenlee, H Grenier, G Gris, P Grivaz, JF Grohsjean, A Grunendahl, S Grunewald, MW Guillemin, T Gutierrez, G Gutierrez, P Haley, J Han, L Harder, K Harel, A Hauptman, JM Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinson, AP Heintz, U Hensel, C Heredia-De La Cruz, I Herner, K Hesketh, G Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hoeneisen, B Hogan, J Hohlfeld, M Holzbauer, JL Howley, I Hubacek, Z Hynek, V Iashvili, I Ilchenko, Y Illingworth, R Ito, AS Jabeen, S Jaffre, M Jayasinghe, A Jeong, MS Jesik, R Jiang, P Johns, K Johnson, E Johnson, M Jonckheere, A Jonsson, P Joshi, J Jung, AW Juste, A Kajfasz, E Karmanov, D Katsanos, I Kaur, M Kehoe, R Kermiche, S Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Kiselevich, I Kohli, JM Kozelov, AV Kraus, J Kumar, A Kupco, A Kurca, T Kuzmin, VA Lammers, S Lebrun, P Lee, HS Lee, SW Lee, WM Lei, X Lellouch, J Li, D Li, H Li, L Li, QZ Lim, JK Lincoln, D Linnemann, J Lipaev, VV Lipton, R Liu, H Liu, Y Lobodenko, A Lokajicek, M de Sa, RL Luna-Garcia, R Lyon, AL Maciel, AKA Madar, R Magana-Villalba, R Malik, S Malyshev, VL Mansour, J Martinez-Ortega, J McCarthy, R McGivern, CL Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Meyer, A Meyer, J Miconi, F Mondal, NK Mulhearn, M Nagy, E Narain, M Nayyar, R Neal, HA Negret, JP Neustroev, P Nguyen, HT Nunnemann, T Orduna, J Osman, N Pal, A Parashar, N Parihar, V Park, SK Partridge, R Parua, N Patwa, A Penning, B Perfilov, M Peters, Y Petridis, K Petrillo, G Petroff, P Pleier, MA Podstavkov, VM Popov, AV Prewitt, M Price, D Prokopenko, N Qian, J Quadt, A Quinn, B Ratoff, PN Razumov, I Ripp-Baudot, I Rizatdinova, F Rominsky, M Ross, A Royon, C Rubinov, P Ruchti, R Sajot, G Sanchez-Hernandez, A Sanders, MP Santos, AS Savage, G Savitskyi, M Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schott, M Schwanenberger, C Schwienhorst, R Sekaric, J Severini, H Shabalina, E Shary, V Shaw, S Shchukin, AA Simak, V Skubic, P Slattery, P Snow, GR Snow, J Snyder, S Soldner-Rembold, S Sonnenschein, L Soustruznik, K Stark, J Stefaniuk, N Stoyanova, DA Strauss, M Suter, L Svoisky, P Titov, M Tokmenin, VV Tsai, YT Tsybychev, D Tuchming, B Tully, C Uvarov, L Uvarov, S Uzunyan, S Van Kooten, R van Leeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Verkheev, AY Vertogradov, LS Verzocchi, M Vesterinen, M Vilanova, D Vokac, P Wahl, HD Wang, MHLS Warchol, J Watts, G Wayne, M Weichert, J Welty-Rieger, L Williams, MRJ Wilson, GW Wobisch, M Wood, DR Wyatt, TR Xie, Y Yamada, R Yang, S Yasuda, T Yatsunenko, YA Ye, W Ye, Z Yin, H Yip, K Youn, SW Yu, JM Zennamo, J Zhao, TG Zhou, B Zhu, J Zielinski, M Zieminska, D Zivkovic, L AF Abazov, V. M. Abbott, B. Acharya, B. S. Adams, M. Adams, T. Agnew, J. P. Alexeev, G. D. Alkhazov, G. Alton, A. Askew, A. Atkins, S. Augsten, K. Aushev, V. Aushev, Y. Avila, C. Badaud, F. Bagby, L. Baldin, B. Bandurin, D. V. Banerjee, S. Barberis, E. Baringer, P. Bartlett, J. F. Bassler, U. Bazterra, V. Bean, A. Begalli, M. Bellantoni, L. Beri, S. B. Bernardi, G. Bernhard, R. Bertram, I. Besancon, M. Beuselinck, R. Bhat, P. C. Bhatia, S. Bhatnagar, V. Blazey, G. Blessing, S. Bloom, K. Boehnlein, A. Boline, D. Boos, E. E. Borissov, G. Borysova, M. Brandt, A. Brandt, O. Brochmann, M. Brock, R. Bross, A. Brown, D. Bu, X. B. Buehler, M. Buescher, V. Bunichev, V. Burdin, S. Buszello, C. P. Camacho-Perez, E. Casey, B. C. K. Castilla-Valdez, H. Caughron, S. Chakrabarti, S. Chan, K. M. Chandra, A. Chapon, E. Chen, G. Cho, S. W. Choi, S. Choudhary, B. Cihangir, S. Claes, D. Clutter, J. Cooke, M. Cooper, W. E. Corcoran, M. Couderc, F. Cousinou, M. -C. Cuth, J. Cutts, D. Das, A. Davies, G. de Jong, S. J. De La Cruz-Burelo, E. Deliot, F. Demina, R. Denisov, D. Denisov, S. P. Desai, S. Deterre, C. DeVaughan, K. Diehl, H. T. Diesburg, M. Ding, P. F. Dominguez, A. Drutskoy, A. Dubey, A. Dudko, L. V. Duperrin, A. Dutt, S. Eads, M. Edmunds, D. Ellison, J. Elvira, V. D. Enari, Y. Evans, H. Evdokimov, A. Evdokimov, V. N. Faure, A. Feng, L. Ferbel, T. Fiedler, F. Filthaut, F. Fisher, W. Fisk, H. E. Fortner, M. Fox, H. Franc, J. Fuess, S. Garbincius, P. H. Garcia-Bellido, A. Garcia-Gonzalez, J. A. Gavrilov, V. Geng, W. Gerber, C. E. Gershtein, Y. Ginther, G. Gogota, O. Golovanov, G. Grannis, P. D. Greder, S. Greenlee, H. Grenier, G. Gris, Ph. Grivaz, J. -F. Grohsjean, A. Grunendahl, S. Grunewald, M. W. Guillemin, T. Gutierrez, G. Gutierrez, P. Haley, J. Han, L. Harder, K. Harel, A. Hauptman, J. M. Hays, J. Head, T. Hebbeker, T. Hedin, D. Hegab, H. Heinson, A. P. Heintz, U. Hensel, C. Heredia-De La Cruz, I. Herner, K. Hesketh, G. Hildreth, M. D. Hirosky, R. Hoang, T. Hobbs, J. D. Hoeneisen, B. Hogan, J. Hohlfeld, M. Holzbauer, J. L. Howley, I. Hubacek, Z. Hynek, V. Iashvili, I. Ilchenko, Y. Illingworth, R. Ito, A. S. Jabeen, S. Jaffre, M. Jayasinghe, A. Jeong, M. S. Jesik, R. Jiang, P. Johns, K. Johnson, E. Johnson, M. Jonckheere, A. Jonsson, P. Joshi, J. Jung, A. W. Juste, A. Kajfasz, E. Karmanov, D. Katsanos, I. Kaur, M. Kehoe, R. Kermiche, S. Khalatyan, N. Khanov, A. Kharchilava, A. Kharzheev, Y. N. Kiselevich, I. Kohli, J. M. Kozelov, A. V. Kraus, J. Kumar, A. Kupco, A. Kurca, T. Kuzmin, V. A. Lammers, S. Lebrun, P. Lee, H. S. Lee, S. W. Lee, W. M. Lei, X. Lellouch, J. Li, D. Li, H. Li, L. Li, Q. Z. Lim, J. K. Lincoln, D. Linnemann, J. Lipaev, V. V. Lipton, R. Liu, H. Liu, Y. Lobodenko, A. Lokajicek, M. de Sa, R. Lopes Luna-Garcia, R. Lyon, A. L. Maciel, A. K. A. Madar, R. Magana-Villalba, R. Malik, S. Malyshev, V. L. Mansour, J. Martinez-Ortega, J. McCarthy, R. McGivern, C. L. Meijer, M. M. Melnitchouk, A. Menezes, D. Mercadante, P. G. Merkin, M. Meyer, A. Meyer, J. Miconi, F. Mondal, N. K. Mulhearn, M. Nagy, E. Narain, M. Nayyar, R. Neal, H. A. Negret, J. P. Neustroev, P. Nguyen, H. T. Nunnemann, T. Orduna, J. Osman, N. Pal, A. Parashar, N. Parihar, V. Park, S. K. Partridge, R. Parua, N. Patwa, A. Penning, B. Perfilov, M. Peters, Y. Petridis, K. Petrillo, G. Petroff, P. Pleier, M. -A. Podstavkov, V. M. Popov, A. V. Prewitt, M. Price, D. Prokopenko, N. Qian, J. Quadt, A. Quinn, B. Ratoff, P. N. Razumov, I. Ripp-Baudot, I. Rizatdinova, F. Rominsky, M. Ross, A. Royon, C. Rubinov, P. Ruchti, R. Sajot, G. Sanchez-Hernandez, A. Sanders, M. P. Santos, A. S. Savage, G. Savitskyi, M. Sawyer, L. Scanlon, T. Schamberger, R. D. Scheglov, Y. Schellman, H. Schott, M. Schwanenberger, C. Schwienhorst, R. Sekaric, J. Severini, H. Shabalina, E. Shary, V. Shaw, S. Shchukin, A. A. Simak, V. Skubic, P. Slattery, P. Snow, G. R. Snow, J. Snyder, S. Soldner-Rembold, S. Sonnenschein, L. Soustruznik, K. Stark, J. Stefaniuk, N. Stoyanova, D. A. Strauss, M. Suter, L. Svoisky, P. Titov, M. Tokmenin, V. V. Tsai, Y. -T. Tsybychev, D. Tuchming, B. Tully, C. Uvarov, L. Uvarov, S. Uzunyan, S. Van Kooten, R. van Leeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verkheev, A. Y. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vokac, P. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weichert, J. Welty-Rieger, L. Williams, M. R. J. Wilson, G. W. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Yamada, R. Yang, S. Yasuda, T. Yatsunenko, Y. A. Ye, W. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. M. Zennamo, J. Zhao, T. G. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. TI Evidence for a B-s(0)pi(+/-) State SO PHYSICAL REVIEW LETTERS LA English DT Article ID DETECTOR AB We report evidence for a narrow structure, X(5568), in the decay sequence X(5568) -> B-s(0)pi(+/-), B-s(0) -> J/psi phi, J/psi -> mu(+)mu(-), phi -> K+K-. This is evidence for the first instance of a hadronic state with valence quarks of four different flavors. The mass and natural width of this state are measured to be m = 5567.8 +/- 2.9(stat)(-1.9)(+0.9) (syst) MeV/c(2) and Gamma = 21.9 +/- 6.4(stat)(-2.5)(+5.0) (syst) MeV/c(2). If the decay is X(5568) -> B-s*pi(+/-). B-s(0)gamma pi(+/-) with an unseen gamma, m(X(5568)) will be shifted up by m(B-s*) - m(B-s(0)) similar to 49 MeV/c(2). This measurement is based on 10.4 fb(-1) of p (p) over bar collision data at root s = 1.96 TeV collected by the D0 experiment at the Fermilab Tevatron collider. C1 [Borysova, M.; Hensel, C.; Maciel, A. K. A.; Santos, A. S.] Ctr Brasileiro Pesquisas Fis, LAFEX, BR-22290 Rio De Janeiro, RJ, Brazil. [Begalli, M.] Univ Estado Rio de Janeiro, BR-20550 Rio De Janeiro, RJ, Brazil. [Mercadante, P. G.] Univ Fed ABC, BR-09210 Santo Andre, SP, Brazil. [Han, L.; Jiang, P.; Liu, Y.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Avila, C.; Negret, J. 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V.; Hirosky, R.; Li, H.; Mulhearn, M.; Nguyen, H. T.; Svoisky, P.] Univ Virginia, Charlottesville, VA 22904 USA. [Brochmann, M.; Watts, G.] Univ Washington, Seattle, WA 98195 USA. [Alton, A.] Augustana Coll, Sioux Falls, SD 57197 USA. [Burdin, S.] Univ Liverpool, Liverpool L69 3BX, Merseyside, England. [Deterre, C.; Grohsjean, A.] Deutshes Elektronen Synchrotron DESY, Notkestr 85, Hamburg, Germany. [Heredia-De La Cruz, I.] CONACyT, M-03940 Mexico City, DF, Mexico. [Partridge, R.] SLAC, Menlo Pk, CA 94025 USA. [Hesketh, G.] UCL, London WC1E 6BT, England. [Luna-Garcia, R.] IPN, Ctr Invest Computac, Mexico City 07738, DF, Mexico. Univ Estadual Paulista, BR-01140 Sao Paulo, SP, Brazil. [Meyer, J.] KIT, SCC, D-76128 Karlsruhe, Germany. [Patwa, A.] US DOE, Off Sci, Washington, DC 20585 USA. [Cooke, M.] Amer Assoc Advancement Sci, Washington, DC 20005 USA. KINR, UA-03680 Kiev, Ukraine. [Jabeen, S.] Univ Maryland, College Pk, MD 20742 USA. [Williams, M. R. J.] European Org Nucl Res CERN, CH-1211 Geneva, Switzerland. [Jung, A. W.] Purdue Univ, W Lafayette, IN 47907 USA. [Drutskoy, A.] Russian Acad Sci, Lebedev Phys Inst, Moscow 119991, Russia. RP Abazov, VM (reprint author), Joint Inst Nucl Res, Dubna 141980, Russia. RI Dudko, Lev/D-7127-2012; Drutskoy, Alexey/C-8833-2016; Gutierrez, Phillip/C-1161-2011 OI Dudko, Lev/0000-0002-4462-3192; Drutskoy, Alexey/0000-0003-4524-0422; FU Department of Energy (United States of America); National Science Foundation (United States of America); Alternative Energies and Atomic Energy Commission (France); National Center for Scientific Research/National Institute of Nuclear and Particle Physics (France); Ministry of Education and Science of the Russian Federation (Russia); National Research Center "Kurchatov Institute" of the Russian Federation (Russia); Russian Foundation for Basic Research (Russia); National Council for the Development of Science and Technology; Carlos Chagas Filho Foundation; Department of Atomic Energy (India); Department of Science and Technology (India); Administrative Department of Science, Technology and Innovation (Colombia); National Council of Science and Technology (Mexico); National Research Foundation of Korea (Korea); Foundation for Fundamental Research on Matter (Netherlands); Science and Technology Facilities Council (United Kingdom); Royal Society (United Kingdom); Ministry of Education, Youth and Sports (Czech Republic); Bundesministerium fur Bildung und Forschung (Federal Ministry of Education and Research) (Germany); Deutsche Forschungsgemeinschaft (German Research Foundation) (Germany); Science Foundation Ireland (Ireland); Swedish Research Council (Sweden); China Academy of Sciences (China); National Natural Science Foundation of China (China); Ministry of Education and Science of Ukraine (Ukraine) FX We thank E. Gross and O. Vittels for useful discussions. We thank the staff at Fermilab and collaborating institutions, and acknowledge support from the Department of Energy and National Science Foundation (United States of America); Alternative Energies and Atomic Energy Commission and National Center for Scientific Research/National Institute of Nuclear and Particle Physics (France); Ministry of Education and Science of the Russian Federation, National Research Center "Kurchatov Institute" of the Russian Federation, and Russian Foundation for Basic Research (Russia); National Council for the Development of Science and Technology and Carlos Chagas Filho Foundation for the Support of Research in the State of Rio de Janeiro (Brazil); Department of Atomic Energy and Department of Science and Technology (India); Administrative Department of Science, Technology and Innovation (Colombia); National Council of Science and Technology (Mexico); National Research Foundation of Korea (Korea); Foundation for Fundamental Research on Matter (Netherlands); Science and Technology Facilities Council and The Royal Society (United Kingdom); Ministry of Education, Youth and Sports (Czech Republic); Bundesministerium fur Bildung und Forschung (Federal Ministry of Education and Research) and Deutsche Forschungsgemeinschaft (German Research Foundation) (Germany); Science Foundation Ireland (Ireland); Swedish Research Council (Sweden); China Academy of Sciences and National Natural Science Foundation of China (China); and Ministry of Education and Science of Ukraine (Ukraine). NR 17 TC 27 Z9 27 U1 5 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 7 PY 2016 VL 117 IS 2 AR 022003 DI 10.1103/PhysRevLett.117.022003 PG 8 WC Physics, Multidisciplinary SC Physics GA DR2IR UT WOS:000379728700003 PM 27447502 ER PT J AU Regan, SP Goncharov, VN Igumenshchev, IV Sangster, TC Betti, R Bose, A Boehly, TR Bonino, MJ Campbell, EM Cao, D Collins, TJB Craxton, RS Davis, AK Delettrez, JA Edgell, DH Epstein, R Forrest, CJ Frenje, JA Froula, DH Johnson, MG Glebov, VY Harding, DR Hohenberger, M Hu, SX Jacobs-Perkins, D Janezic, R Karasik, M Keck, RL Kelly, JH Kessler, TJ Knauer, JP Kosc, TZ Loucks, SJ Marozas, JA Marshall, FJ McCrory, RL McKenty, PW Meyerhofer, DD Michel, DT Myatt, JF Obenschain, SP Petrasso, RD Radha, PB Rice, B Rosenberg, MJ Schmitt, AJ Schmitt, MJ Seka, W Shmayda, WT Shoup, MJ Shvydky, A Skupsky, S Solodov, AA Stoeckl, C Theobald, W Ulreich, J Wittman, MD Woo, KM Yaakobi, B Zuegel, JD AF Regan, S. P. Goncharov, V. N. Igumenshchev, I. V. Sangster, T. C. Betti, R. Bose, A. Boehly, T. R. Bonino, M. J. Campbell, E. M. Cao, D. Collins, T. J. B. Craxton, R. S. Davis, A. K. Delettrez, J. A. Edgell, D. H. Epstein, R. Forrest, C. J. Frenje, J. A. Froula, D. H. Johnson, M. Gatu Glebov, V. Yu. Harding, D. R. Hohenberger, M. Hu, S. X. Jacobs-Perkins, D. Janezic, R. Karasik, M. Keck, R. L. Kelly, J. H. Kessler, T. J. Knauer, J. P. Kosc, T. Z. Loucks, S. J. Marozas, J. A. Marshall, F. J. McCrory, R. L. McKenty, P. W. Meyerhofer, D. D. Michel, D. T. Myatt, J. F. Obenschain, S. P. Petrasso, R. D. Radha, P. B. Rice, B. Rosenberg, M. J. Schmitt, A. J. Schmitt, M. J. Seka, W. Shmayda, W. T. Shoup, M. J., III Shvydky, A. Skupsky, S. Solodov, A. A. Stoeckl, C. Theobald, W. Ulreich, J. Wittman, M. D. Woo, K. M. Yaakobi, B. Zuegel, J. D. TI Demonstration of Fuel Hot-Spot Pressure in Excess of 50 Gbar for Direct-Drive, Layered Deuterium-Tritium Implosions on OMEGA SO PHYSICAL REVIEW LETTERS LA English DT Article ID NATIONAL IGNITION FACILITY; LASER; PERFORMANCE; DISPERSION; LIGHT AB A record fuel hot-spot pressure P-hs = 56 +/- 7 Gbar was inferred from x-ray and nuclear diagnostics for direct-drive inertial confinement fusion cryogenic, layered deuterium-tritium implosions on the 60-beam, 30-kJ, 351-nm OMEGA Laser System. When hydrodynamically scaled to the energy of the National Ignition Facility, these implosions achieved a Lawson parameter similar to 60% of the value required for ignition [A. Bose et al., Phys. Rev. E 93, LM15119ER (2016)], similar to indirect-drive implosions [R. Betti et al., Phys. Rev. Lett. 114, 255003 (2015)], and nearly half of the direct-drive ignition-threshold pressure. Relative to symmetric, one-dimensional simulations, the inferred hot-spot pressure is approximately 40% lower. Three-dimensional simulations suggest that low-mode distortion of the hot spot seeded by laser-drive nonuniformity and target-positioning error reduces target performance. C1 [Regan, S. P.; Goncharov, V. N.; Igumenshchev, I. V.; Sangster, T. C.; Betti, R.; Bose, A.; Boehly, T. R.; Bonino, M. J.; Campbell, E. M.; Cao, D.; Collins, T. J. B.; Craxton, R. S.; Davis, A. K.; Delettrez, J. A.; Edgell, D. H.; Epstein, R.; Forrest, C. J.; Froula, D. H.; Glebov, V. Yu.; Harding, D. R.; Hohenberger, M.; Hu, S. X.; Jacobs-Perkins, D.; Janezic, R.; Keck, R. L.; Kelly, J. H.; Kessler, T. J.; Knauer, J. P.; Kosc, T. Z.; Loucks, S. J.; Marozas, J. A.; Marshall, F. J.; McCrory, R. L.; McKenty, P. W.; Michel, D. T.; Myatt, J. F.; Radha, P. B.; Rice, B.; Rosenberg, M. J.; Seka, W.; Shmayda, W. T.; Shoup, M. J., III; Shvydky, A.; Skupsky, S.; Solodov, A. A.; Stoeckl, C.; Theobald, W.; Ulreich, J.; Wittman, M. D.; Woo, K. M.; Yaakobi, B.; Zuegel, J. D.] Univ Rochester, Lab Laser Energet, Rochester, NY 14623 USA. [Betti, R.; Bose, A.; Woo, K. M.] Univ Rochester, Fus Sci Ctr, Rochester, NY 14623 USA. [Frenje, J. A.; Johnson, M. Gatu; Petrasso, R. D.] MIT, Plasma Sci & Fus Ctr, Cambridge, MA 02139 USA. [Karasik, M.; Petrasso, R. D.; Schmitt, A. J.] Naval Res Lab, Washington, DC 20375 USA. [Meyerhofer, D. D.; Schmitt, M. J.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Betti, R.; Bose, A.; McCrory, R. L.; Woo, K. M.] Univ Rochester, Dept Mech Engn, Rochester, NY 14623 USA. [Betti, R.; Bose, A.; McCrory, R. L.; Woo, K. M.] Univ Rochester, Dept Phys & Astron, Rochester, NY 14623 USA. RP Regan, SP (reprint author), Univ Rochester, Lab Laser Energet, Rochester, NY 14623 USA. EM sreg@lle.rochester.edu RI Hu, Suxing/A-1265-2007; OI Hu, Suxing/0000-0003-2465-3818; Schmitt, Mark/0000-0002-0197-9180 FU DOE NNSA [DE-NA0001944]; University of Rochester; New York State Energy Research and Development Authority FX The authors acknowledge the excellent operation of the OMEGA laser system. This material is based on work supported by the DOE NNSA under Award No. DE-NA0001944, the University of Rochester, and the New York State Energy Research and Development Authority. The support of DOE does not constitute an endorsement by the DOE of the views expressed in this Letter. NR 36 TC 7 Z9 7 U1 11 U2 20 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 7 PY 2016 VL 117 IS 2 AR 025001 DI 10.1103/PhysRevLett.117.025001 PG 5 WC Physics, Multidisciplinary SC Physics GA DR2IR UT WOS:000379728700007 PM 27447511 ER PT J AU Chandler, DW AF Chandler, David W. TI CHEMICAL PHYSICS Quantum control of light-induced reactions SO NATURE LA English DT Editorial Material ID PHOTODISSOCIATION; DYNAMICS C1 [Chandler, David W.] Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. RP Chandler, DW (reprint author), Sandia Natl Labs, Combust Res Facil, Livermore, CA 94550 USA. EM chand@sandia.gov NR 9 TC 0 Z9 0 U1 9 U2 19 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JUL 7 PY 2016 VL 535 IS 7610 BP 42 EP 44 PG 3 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DQ2EU UT WOS:000379015600023 PM 27383977 ER PT J AU Gilbert, JA Quinn, RA Debelius, J Xu, ZJZ Morton, J Garg, N Jansson, JK Dorrestein, PC Knight, R AF Gilbert, Jack A. Quinn, Robert A. Debelius, Justine Xu, Zhenjiang Z. Morton, James Garg, Neha Jansson, Janet K. Dorrestein, Pieter C. Knight, Rob TI Microbiome-wide association studies link dynamic microbial consortia to disease SO NATURE LA English DT Review ID HUMAN GUT MICROBIOME; TRIMETHYLAMINE-N-OXIDE; CLOSTRIDIUM-DIFFICILE INFECTION; BIOSYNTHETIC GENE CLUSTERS; FECAL MICROBIOTA; ORAL MICROBIOTA; CROHNS-DISEASE; BACTERIAL COMMUNITIES; RHEUMATOID-ARTHRITIS; DRUG-METABOLISM AB Rapid advances in DNA sequencing, metabolomics, proteomics and computational tools are dramatically increasing access to the microbiome and identification of its links with disease. In particular, time-series studies and multiple molecular perspectives are facilitating microbiome-wide association studies, which are analogous to genome-wide association studies. Early findings point to actionable outcomes of microbiome-wide association studies, although their clinical application has yet to be approved. An appreciation of the complexity of interactions among the microbiome and the host's diet, chemistry and health, as well as determining the frequency of observations that are needed to capture and integrate this dynamic interface, is paramount for developing precision diagnostics and therapies that are based on the microbiome. C1 [Gilbert, Jack A.] Univ Chicago, Dept Surg, 5841 S Maryland Ave, Chicago, IL 60637 USA. [Quinn, Robert A.; Garg, Neha; Dorrestein, Pieter C.] Univ Calif San Diego, Dept Pharmacol, La Jolla, CA 92093 USA. [Quinn, Robert A.; Garg, Neha; Dorrestein, Pieter C.] Univ Calif San Diego, Skaggs Sch Pharm & Pharmaceut Sci, Collaborat Mass Spectrometry Innovat Ctr, La Jolla, CA 92093 USA. [Gilbert, Jack A.; Dorrestein, Pieter C.; Knight, Rob] Univ Calif San Diego, Jacobs Sch Engn, Ctr Microbiome Innovat, La Jolla, CA 92093 USA. [Debelius, Justine; Xu, Zhenjiang Z.; Dorrestein, Pieter C.; Knight, Rob] Univ Calif San Diego, Dept Pediat, Sch Med, La Jolla, CA 92093 USA. [Morton, James; Knight, Rob] Univ Calif San Diego, Jacobs Sch Engn, Dept Comp Sci & Engn, La Jolla, CA 92093 USA. [Jansson, Janet K.] Pacific NW Natl Lab, Earth & Biol Sci Directorate, Richland, WA 99354 USA. RP Knight, R (reprint author), Univ Calif San Diego, Jacobs Sch Engn, Ctr Microbiome Innovat, La Jolla, CA 92093 USA.; Knight, R (reprint author), Univ Calif San Diego, Dept Pediat, Sch Med, La Jolla, CA 92093 USA.; Knight, R (reprint author), Univ Calif San Diego, Jacobs Sch Engn, Dept Comp Sci & Engn, La Jolla, CA 92093 USA. EM robknight@ucsd.edu FU US National Institutes of Health; US Department of Energy; US National Science Foundation; Alfred P. Sloan Foundation; Crohn's and Colitis Foundation of America; US Office of Naval Research FX This work and the work in the authors' laboratories that it describes was supported in part by awards from the US National Institutes of Health, the US Department of Energy, the US National Science Foundation, the Alfred P. Sloan Foundation, the Crohn's and Colitis Foundation of America and the US Office of Naval Research. NR 123 TC 21 Z9 21 U1 66 U2 129 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JUL 7 PY 2016 VL 535 IS 7610 BP 94 EP 103 DI 10.1038/nature18850 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DQ2EU UT WOS:000379015600032 PM 27383984 ER PT J AU Aharonian, F Akamatsu, H Akimoto, F Allen, SW Anabuki, N Angelini, L Arnaud, K Audard, M Awaki, H Axelsson, M Bamba, A Bautz, M Blandford, R Brenneman, L Brown, GV Bulbul, E Cackett, E Chernyakova, M Chiao, M Coppi, P Costantini, E de Plaa, J den Herder, JW Done, C Dotani, T Ebisawa, K Eckart, M Enoto, T Ezoe, Y Fabian, AC Ferrigno, C Foster, A Fujimoto, R Fukazawa, Y Furuzawa, A Galeazzi, M Gallo, L Gandhi, P Giustini, M Goldwurm, A Gu, L Guainazzi, M Haba, Y Hagino, K Hamaguchi, K Harrus, I Hatsukade, I Hayashi, K Hayashi, T Hayashida, K Hiraga, J Hornschemeier, A Hoshino, A Hughes, J Iizuka, R Inoue, H Inoue, Y Ishibashi, K Ishida, M Ishikawa, K Ishisaki, Y Itoh, M Iyomoto, N Kaastra, J Kallman, T Kamae, T Kara, E Kataoka, J Katsuda, S Katsuta, J Kawaharada, M Kawai, N Kelley, R Khangulyan, D Kilbourne, C King, A Kitaguchi, T Kitamoto, S Kitayama, T Kohmura, T Kokubun, M Koyama, S Koyama, K Kretschmar, P Krimm, H Kubota, A Kunieda, H Laurent, P Lebrun, F Lee, SH Leutenegger, M Limousin, O Loewenstein, M Long, KS Lumb, D Madejski, G Maeda, Y Maier, D Makishima, K Markevitch, M Matsumoto, H Matsushita, K McCammon, D McNamara, B Mehdipour, M Miller, E Miller, J Mineshige, S Mitsuda, K Mitsuishi, I Miyazawa, T Mizuno, T Mori, H Mori, K Moseley, H Mukai, K Murakami, H Murakami, T Mushotzky, R Nagino, R Nakagawa, T Nakajima, H Nakamori, T Nakano, T Nakashima, S Nakazawa, K Nobukawa, M Noda, H Nomachi, M O'Dell, S Odaka, H Ohashi, T Ohno, M Okajima, T Ota, N Ozaki, M Paerels, F Paltani, S Parmar, A Petre, R Pinto, C Pohl, M Porter, FS Pottschmidt, K Ramsey, B Reynolds, C Russell, H Safi-Harb, S Saito, S Sakai, K Sameshima, H Sato, G Sato, K Sato, R Sawada, M Schartel, N Serlemitsos, P Seta, H Shidatsu, M Simionescu, A Smith, R Soong, Y Stawarz, L Sugawara, Y Sugita, S Szymkowiak, A Tajima, H Takahashi, H Takahashi, T Takeda, S Takei, Y Tamagawa, T Tamura, K Tamura, T Tanaka, T Tanaka, Y Tanaka, Y Tashiro, M Tawara, Y Terada, Y Terashima, Y Tombesi, F Tomida, H Tsuboi, Y Tsujimoto, M Tsunemi, H Tsuru, T Uchida, H Uchiyama, H Uchiyama, Y Ueda, S Ueda, Y Ueno, S Uno, S Urry, M Ursino, E De Vries, C Watanabe, S Werner, N Wik, D Wilkins, D Williams, B Yamada, S Yamaguchi, H Yamaoka, K Yamasaki, NY Yamauchi, M Yamauchi, S Yaqoob, T Yatsu, Y Yonetoku, D Yoshida, A Yuasa, T Zhuravleva, I Zoghbi, A AF Aharonian, Felix Akamatsu, Hiroki Akimoto, Fumie Allen, Steven W. 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Lumb, David Madejski, Grzegorz Maeda, Yoshitomo Maier, Daniel Makishima, Kazuo Markevitch, Maxim Matsumoto, Hironori Matsushita, Kyoko McCammon, Dan McNamara, Brian Mehdipour, Missagh Miller, Eric Miller, Jon Mineshige, Shin Mitsuda, Kazuhisa Mitsuishi, Ikuyuki Miyazawa, Takuya Mizuno, Tsunefumi Mori, Hideyuki Mori, Koji Moseley, Harvey Mukai, Koji Murakami, Hiroshi Murakami, Toshio Mushotzky, Richard Nagino, Ryo Nakagawa, Takao Nakajima, Hiroshi Nakamori, Takeshi Nakano, Toshio Nakashima, Shinya Nakazawa, Kazuhiro Nobukawa, Masayoshi Noda, Hirofumi Nomachi, Masaharu O'Dell, Steve Odaka, Hirokazu Ohashi, Takaya Ohno, Masanori Okajima, Takashi Ota, Naomi Ozaki, Masanobu Paerels, Frits Paltani, Stephane Parmar, Arvind Petre, Robert Pinto, Ciro Pohl, Martin Porter, F. Scott Pottschmidt, Katja Ramsey, Brian Reynolds, Christopher Russell, Helen Safi-Harb, Samar Saito, Shinya Sakai, Kazuhiro Sameshima, Hiroaki Sato, Goro Sato, Kosuke Sato, Rie Sawada, Makoto Schartel, Norbert Serlemitsos, Peter Seta, Hiromi Shidatsu, Megumi Simionescu, Aurora Smith, Randall Soong, Yang Stawarz, Lukasz Sugawara, Yasuharu Sugita, Satoshi Szymkowiak, Andrew Tajima, Hiroyasu Takahashi, Hiromitsu Takahashi, Tadayuki Takeda, Shin'ichiro Takei, Yoh Tamagawa, Toru Tamura, Keisuke Tamura, Takayuki Tanaka, Takaaki Tanaka, Yasuo Tanaka, Yasuyuki Tashiro, Makoto Tawara, Yuzuru Terada, Yukikatsu Terashima, Yuichi Tombesi, Francesco Tomida, Hiroshi Tsuboi, Yohko Tsujimoto, Masahiro Tsunemi, Hiroshi Tsuru, Takeshi Uchida, Hiroyuki Uchiyama, Hideki Uchiyama, Yasunobu Ueda, Shutaro Ueda, Yoshihiro Ueno, Shiro Uno, Shin'ichiro Urry, Meg Ursino, Eugenio De Vries, Cor Watanabe, Shin Werner, Norbert Wik, Daniel Wilkins, Dan Williams, Brian Yamada, Shinya Yamaguchi, Hiroya Yamaoka, Kazutaka Yamasaki, Noriko Y. Yamauchi, Makoto Yamauchi, Shigeo Yaqoob, Tahir Yatsu, Yoichi Yonetoku, Daisuke Yoshida, Atsumasa Yuasa, Takayuki Zhuravleva, Irina Zoghbi, Abderahmen CA Hitomi Collaboration TI The quiescent intracluster medium in the core of the Perseus cluster SO NATURE LA English DT Article ID X-RAY SPECTROSCOPY; GALAXY CLUSTERS; XMM-NEWTON; TURBULENT VELOCITY; NGC 1275; NGC-1275; LINE; CONSTRAINTS; FEEDBACK; PLASMAS AB Clusters of galaxies are the most massive gravitationally bound objects in the Universe and are still forming. They are thus important probes(1) of cosmological parameters and many astrophysical processes. However, knowledge of the dynamics of the pervasive hot gas, the mass of which is much larger than the combined mass of all the stars in the cluster, is lacking. Such knowledge would enable insights into the injection of mechanical energy by the central supermassive black hole and the use of hydrostatic equilibrium for determining cluster masses. X-rays from the core of the Perseus cluster are emitted by the 50-million-kelvin diffuse hot plasma filling its gravitational potential well. The active galactic nucleus of the central galaxy NGC 1275 is pumping jetted energy into the surrounding intracluster medium, creating buoyant bubbles filled with relativistic plasma. These bubbles probably induce motions in the intracluster medium and heat the inner gas, preventing runaway radiative cooling-a process known as active galactic nucleus feedback(2-6). Here we report X-ray observations of the core of the Perseus cluster, which reveal a remarkably quiescent atmosphere in which the gas has a line-of-sight velocity dispersion of 164 +/- 10 kilometres per second in the region 30-60 kiloparsecs from the central nucleus. A gradient in the line-of-sight velocity of 150 +/- 70 kilometres per second is found across the 60-kiloparsec image of the cluster core. Turbulent pressure support in the gas is four per cent of the thermodynamic pressure, with large-scale shear at most doubling this estimate. We infer that a total cluster mass determined from hydrostatic equilibrium in a central region would require little correction for turbulent pressure. C1 [Aharonian, Felix; Chernyakova, Maria] Dublin Inst Adv Studies, Astron & Astrophys Sect, Dublin 2, Ireland. [Aharonian, Felix] Natl Res Nucl Univ MEPHI, Moscow 115409, Russia. [Akamatsu, Hiroki; Costantini, Elisa; de Plaa, Jelle; den Herder, Jan-Willem; Giustini, Margherita; Gu, Liyi; Kaastra, Jelle; Mehdipour, Missagh; De Vries, Cor] SRON Netherlands Inst Space Res, Utrecht, Netherlands. [Akimoto, Fumie; Furuzawa, Akihiro; Hayashi, Takayuki; Ishibashi, Kazunori; Kunieda, Hideyo; Mitsuishi, Ikuyuki; Miyazawa, Takuya; Tamura, Keisuke; Tawara, Yuzuru; Yamaoka, Kazutaka] Nagoya Univ, Dept Phys, Nagoya, Aichi 4648602, Japan. [Allen, Steven W.; Blandford, Roger; Kamae, Tuneyoshi; King, Ashley; Madejski, Grzegorz; Werner, Norbert; Zhuravleva, Irina] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, Stanford, CA 94305 USA. [Allen, Steven W.; Blandford, Roger; King, Ashley; Werner, Norbert; Zhuravleva, Irina] Stanford Univ, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94305 USA. [Allen, Steven W.; Blandford, Roger; Madejski, Grzegorz] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Anabuki, Naohisa; Hayashida, Kiyoshi; Nagino, Ryo; Nakajima, Hiroshi; Tsunemi, Hiroshi] Osaka Univ, Dept Earth & Space Sci, Osaka 5600043, Japan. [Angelini, Lorella; Arnaud, Keith; Chiao, Meng; Eckart, Megan; Hamaguchi, Kenji; Harrus, Ilana; Hornschemeier, Ann; Kallman, Timothy; Kelley, Richard; Kilbourne, Caroline; Krimm, Hans; Leutenegger, Maurice; Loewenstein, Michael; Markevitch, Maxim; Mori, Hideyuki; Moseley, Harvey; Mukai, Koji; Okajima, Takashi; Petre, Robert; Porter, F. Scott; Pottschmidt, Katja; Sakai, Kazuhiro; Serlemitsos, Peter; Soong, Yang; Tombesi, Francesco; Wik, Daniel; Williams, Brian; Yamaguchi, Hiroya; Yaqoob, Tahir] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Arnaud, Keith; Kara, Erin; Loewenstein, Michael; Mushotzky, Richard; Reynolds, Christopher] Univ Maryland, Dept Astron, College Pk, MD 20742 USA. [Audard, Marc; Ferrigno, Carlo; Paltani, Stephane; Pohl, Martin] Univ Geneva, CH-1211 Geneva 4, Switzerland. [Awaki, Hisamitsu; Terashima, Yuichi] Ehime Univ, Dept Phys, Matsuyama, Ehime 7908577, Japan. [Axelsson, Magnus; Ezoe, Yuichiro; Ishisaki, Yoshitaka; Ohashi, Takaya; Seta, Hiromi; Yamada, Shinya] Tokyo Metropolitan Univ, Dept Phys, Tokyo 1920397, Japan. [Bamba, Aya; Nakazawa, Kazuhiro] Univ Tokyo, Dept Phys, Tokyo 1130033, Japan. [Bautz, Marshall; Bulbul, Esra; Miller, Eric] MIT, Kavli Inst Astrophys & Space Res, Cambridge, MA 02139 USA. [Brenneman, Laura; Foster, Adam; Smith, Randall] Smithsonian Astrophys Observ, 60 Garden St,MS-4, Cambridge, MA 02138 USA. [Brown, Gregory V.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Cackett, Edward; Fabian, Andrew C.; Pinto, Ciro; Russell, Helen] Univ Cambridge, Inst Astron, Madingley Rd, Cambridge CB3 0HA, England. [Coppi, Paolo; Szymkowiak, Andrew; Urry, Meg] Yale Univ, Yale Ctr Astron & Astrophys, New Haven, CT 06520 USA. [Done, Chris] Univ Durham, Dept Phys, Durham DH1 3LE, England. [Dotani, Tadayasu; Ebisawa, Ken; Guainazzi, Matteo; Hagino, Kouichi; Hayashi, Katsuhiro; Iizuka, Ryo; Inoue, Hajime; Inoue, Yoshiyuki; Ishida, Manabu; Kokubun, Motohide; Koyama, Shu; Lee, Shiu-Hang; Maeda, Yoshitomo; Mitsuda, Kazuhisa; Nakagawa, Takao; Nakashima, Shinya; Odaka, Hirokazu; Ozaki, Masanobu; Sameshima, Hiroaki; Sato, Goro; Sato, Rie; Simionescu, Aurora; Takahashi, Tadayuki; Takei, Yoh; Tamura, Takayuki; Tanaka, Yasuo; Tomida, Hiroshi; Tsujimoto, Masahiro; Ueda, Shutaro; Ueno, Shiro; Watanabe, Shin; Yamasaki, Noriko Y.] Japan Aerosp Explorat Agcy JAXA, ISAS, Sagamihara, Kanagawa 2525210, Japan. [Enoto, Teruaki; Mineshige, Shin; Ueda, Yoshihiro] Kyoto Univ, Dept Astron, Kyoto 6068502, Japan. [Enoto, Teruaki] Kyoto Univ, Hakubi Ctr Adv Res, Kyoto 6068302, Japan. [Fujimoto, Ryuichi; Murakami, Toshio; Yonetoku, Daisuke] Kanazawa Univ, Fac Math & Phys, Kanazawa, Ishikawa 9201192, Japan. [Fukazawa, Yasushi; Katsuta, Junichiro; Kitaguchi, Takao; Mizuno, Tsunefumi; Ohno, Masanori; Takahashi, Hiromitsu; Tanaka, Yasuyuki] Hiroshima Univ, Dept Phys Sci, Hiroshima 7398526, Japan. [Galeazzi, Massimiliano; Ursino, Eugenio] Univ Miami, Dept Phys, Miami, FL 33124 USA. [Gallo, Luigi; Wilkins, Dan] St Marys Univ, Dept Phys & Astron, Halifax, NS B3H 3C3, Canada. [Gandhi, Poshak] Univ Southampton, Dept Phys & Astron, Southampton SO17 1BJ, Hants, England. [Goldwurm, Andrea; Laurent, Philippe; Lebrun, Francois; Limousin, Olivier; Maier, Daniel] CEA Saclay, IRFU Serv Astrophys, F-91191 Gif Sur Yvette, France. [Guainazzi, Matteo; Kretschmar, Peter; Schartel, Norbert] ESAC, ESA, Madrid, Spain. [Haba, Yoshito] Aichi Univ Educ, Dept Phys & Astron, Kariya, Aichi 4488543, Japan. [Hamaguchi, Kenji; Harrus, Ilana; Mukai, Koji; Pottschmidt, Katja; Yaqoob, Tahir] Univ Maryland Baltimore Cty, Dept Phys, 1000 Hilltop Circle, Baltimore, MD 21250 USA. [Hatsukade, Isamu; Mori, Koji; Yamauchi, Makoto] Miyazaki Univ, Dept Appl Phys & Elect Engn, Miyazaki 8892192, Japan. [Hiraga, Junko] Kwansei Gakuin Univ, Sch Sci & Technol, Dept Phys, Nishinomiya, Hyogo 6691337, Japan. [Hoshino, Akio; Khangulyan, Dmitry; Kitamoto, Shunji; Saito, Shinya; Uchiyama, Yasunobu] Rikkyo Univ, Dept Phys, Tokyo 1718501, Japan. [Hughes, John] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA. [Ishikawa, Kumi; Nakano, Toshio; Noda, Hirofumi; Tamagawa, Toru; Yuasa, Takayuki] RIKEN, Nishina Ctr, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. [Itoh, Masayuki] Kobe Univ, Fac Human Dev, Kobe, Hyogo 6578501, Japan. [Iyomoto, Naoko] Kyushu Univ, Fukuoka 8190395, Japan. [Kataoka, Jun] Waseda Univ, Res Inst Sci & Engn, Tokyo 1698555, Japan. [Katsuda, Satoru; Sugawara, Yasuharu; Tsuboi, Yohko] Chuo Univ, Dept Phys, Tokyo 1128551, Japan. [Kawaharada, Madoka] Japan Aerosp Explorat Agcy JAXA, Tsukuba Space Ctr TKSC, Tsukuba, Ibaraki 3058505, Japan. [Kawai, Nobuyuki; Sugita, Satoshi; Yatsu, Yoichi] Tokyo Inst Technol, Dept Phys, Tokyo 1528551, Japan. [Kitayama, Tetsu] Toho Univ, Dept Phys, Chiba 2748510, Japan. [Kohmura, Takayoshi] Tokyo Univ Sci, Dept Phys, Chiba 2788510, Japan. [Koyama, Katsuji; Tanaka, Takaaki; Tsuru, Takeshi; Uchida, Hiroyuki] Kyoto Univ, Dept Phys, Kyoto 6068502, Japan. [Krimm, Hans] Univ Space Res Assoc, 7178 Columbia Gateway Dr, Columbia, MD 21046 USA. [Kubota, Aya] Shibaura Inst Technol, Dept Elect Informat Syst, Saitama 3378570, Japan. [Long, Knox S.] Space Telescope Sci Inst, Baltimore, MD 21218 USA. [Lumb, David; Parmar, Arvind] ESTEC, ESA, NL-2200 AG Noordwijk, Netherlands. [Makishima, Kazuo; Shidatsu, Megumi] RIKEN, 2-1 Hirosawa, Wako, Saitama 3510198, Japan. [Matsumoto, Hironori] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi 4648602, Japan. [Matsushita, Kyoko; Sato, Kosuke] Tokyo Univ Sci, Dept Phys, Tokyo 1628601, Japan. [McCammon, Dan] Univ Wisconsin, Dept Phys, Madison, WI 53706 USA. [McNamara, Brian] Univ Waterloo, Waterloo, ON N2L 3G1, Canada. [Miller, Jon; Zoghbi, Abderahmen] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Murakami, Hiroshi] Tohoku Gakuin Univ, Fac Liberal Arts, Dept Informat Sci, Sendai, Miyagi 9813193, Japan. [Nakamori, Takeshi] Yamagata Univ, Dept Phys, Fac Sci, Yamagata 9908560, Japan. [Nobukawa, Masayoshi] Nara Univ Educ, Dept Teacher Training, Takabatake Cho, Nara 6308528, Japan. [Nobukawa, Masayoshi] Nara Univ Educ, Sch Educ, Takabatake Cho, Nara 6308528, Japan. [Nomachi, Masaharu] Osaka Univ, Res Ctr Nucl Phys Toyonaka, 1-1 Machikaneyama Machi, Toyonaka, Osaka 5600043, Japan. [O'Dell, Steve; Ramsey, Brian] NASA, George C Marshall Space Flight Ctr, Huntsville, AL 35812 USA. [Ota, Naomi; Yamauchi, Shigeo] Nara Womens Univ, Fac Sci, Dept Phys, Nara 6308506, Japan. [Paerels, Frits] Columbia Univ, Dept Astron, New York, NY 10027 USA. [Safi-Harb, Samar] Univ Manitoba, Dept Phys & Astron, Winnipeg, MB R3T 2N2, Canada. [Sawada, Makoto; Yoshida, Atsumasa] Aoyama Gakuin Univ, Dept Math & Phys, Sagamihara, Kanagawa 2525258, Japan. [Stawarz, Lukasz] Jagiellonian Univ, Astron Observ, PL-30244 Krakow, Poland. [Tajima, Hiroyasu] Nagoya Univ, Inst Space Earth Environm Res, Nagoya, Aichi 4648601, Japan. [Takeda, Shin'ichiro] Grad Univ OIST, Okinawa Inst Sci & Technol, Adv Med Instrumentat Unit, Okinawa 9040495, Japan. [Tashiro, Makoto; Terada, Yukikatsu] Saitama Univ, Dept Phys, Saitama 3388570, Japan. [Uchiyama, Hideki] Shizuoka Univ, Fac Educ, Sci Educ, Shizuoka 4228529, Japan. [Uno, Shin'ichiro] Nihon Fukushi Univ, Fac Hlth Sci, Mihama, Aichi 4750012, Japan. [Wik, Daniel] Johns Hopkins Univ, Dept Phys & Astron, Baltimore, MD 21218 USA. RP Fabian, AC (reprint author), Univ Cambridge, Inst Astron, Madingley Rd, Cambridge CB3 0HA, England. EM acf@ast.cam.ac.uk RI Yamasaki, Noriko/C-2252-2008; Porter, Frederick/D-3501-2012; Zoghbi, Abderahmen/A-8445-2017; Shidatsu, Megumi/C-5742-2017; OI Porter, Frederick/0000-0002-6374-1119; Zoghbi, Abderahmen/0000-0002-0572-9613; Kretschmar, Peter/0000-0001-9840-2048; , kouichi/0000-0003-4235-5304; De Coppi, Paolo/0000-0002-1659-0207 FU NASA Science Mission Directorate; DoE [DE-AC3-76SF00515]; NASA [NNX15AM19G]; US DoE by LLNL [DE-AC52-07NA27344]; NASA; European Space Agency; CNES; Centre National d'Etudes Spatiales; NWO, the Netherlands Organization for Scientific Research; Swiss Secretariat for Education, Research and Innovation SERI; ESA's PRODEX programme; Canadian Space Agency; JSPS/MEXT KAKENHI [15H02070, 15K05107, 23340071, 26109506, 24103002, 25400236, 25800119, 25400237, 25287042, 24540229, 25105516, 23540280, 25400235, 25247028, 26800095, 25400231, 26220703, 24105007, 23340055, 15H00773, 23000004, 15H02090, 15K17610, 15H05438, 15H00785, 24540232]; NWO via a Veni grant; JSPS; STFC [ST/L00075X/1]; JAXA; UK Science and Technology Funding Council (STFC) [ST/J003697/2]; ERC [340442]; JAXA/ISAS; JAXA/TKSC; NASA/GSFC; Noqsi Aerospace Ltd; Stanford U/KIPAC; ESA (Netherlands); SRON; CSA FX We acknowledge all the JAXA members who have contributed to the ASTRO-H (Hitomi) project. All US members gratefully acknowledge support through the NASA Science Mission Directorate. Stanford and SLAC members acknowledge support via DoE contract to SLAC National Accelerator Laboratory DE-AC3-76SF00515 and NASA grant NNX15AM19G. Part of this work was performed under the auspices of the US DoE by LLNL under contract DE-AC52-07NA27344 and also supported by NASA grants to LLNL. Support from the European Space Agency is gratefully acknowledged. French members acknowledge support from CNES, the Centre National d'Etudes Spatiales. SRON is supported by NWO, the Netherlands Organization for Scientific Research. The Swiss team acknowledges support of the Swiss Secretariat for Education, Research and Innovation SERI and ESA's PRODEX programme. The Canadian Space Agency is acknowledged for the support of Canadian members. We acknowledge support from JSPS/MEXT KAKENHI grant numbers 15H02070, 15K05107, 23340071, 26109506, 24103002, 25400236, 25800119, 25400237, 25287042, 24540229, 25105516, 23540280, 25400235, 25247028, 26800095, 25400231, 25247028, 26220703, 24105007, 23340055, 15H00773, 23000004, 15H02090, 15K17610, 15H05438, 15H00785 and 24540232. H. Akamatsu acknowledges support of NWO via a Veni grant. M. Axelsson acknowledges a JSPS International Research Fellowship. C. Done acknowledges STFC funding under grant ST/L00075X/1. P. Gandhi acknowledges a JAXA International Top Young Fellowship and UK Science and Technology Funding Council (STFC) grant ST/J003697/2. H. Russell, A. C. Fabian and C. Pinto acknowledge support from ERC Advanced Grant Feedback 340442. We thank contributions by many companies, including, in particular, NEC, Mitsubishi Heavy Industries, Sumitomo Heavy Industries and Japan Aviation Electronics Industry. Finally, we acknowledge strong support from the following engineers. JAXA/ISAS: C. Baluta, N. Bando, A. Harayama, K. Hirose, K. Ishimura, N. Iwata, T. Kawano, S. Kawasaki, K. Minesugi, C. Natsukari, H. Ogawa, M. Ogawa, M. Ohta, T. Okazaki, S.-i. Sakai, Y. Shibano, M. Shida, T. Shimada, A. Wada, T. Yamada; JAXA/TKSC: A. Okamoto, Y. Sato, K. Shinozaki, H. Sugita; Chubu U: Y. Namba; Ehime U: K. Ogi; Kochi U of Technology: T. Kosaka; Miyazaki U: Y. Nishioka; Nagoya U: H. Nagano; NASA/GSFC: T. Bialas, K. Boyce, E. Canavan, M. DiPirro, M. Kimball, C. Masters, D. Mcguinness, J. Miko, T. Muench, J. Pontius, P. Shirron, C. Simmons, G. Sneiderman, T. Watanabe; Noqsi Aerospace Ltd: J. Doty; Stanford U/KIPAC: M. Asai, K. Gilmore; ESA (Netherlands): C. Jewell; SRON: D. Haas, M. Frericks, P. Laubert, P. Lowes; U of Geneva: P. Azzarello; CSA: A. Koujelev, F. Moroso. NR 37 TC 7 Z9 7 U1 12 U2 20 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 0028-0836 EI 1476-4687 J9 NATURE JI Nature PD JUL 7 PY 2016 VL 535 IS 7610 BP 117 EP + DI 10.1038/nature18627 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DQ2EU UT WOS:000379015600035 ER PT J AU Cheng, QS Bilgin, CC Fonteney, G Chang, H Henderson, M Han, J Parvin, B AF Cheng, Qingsu Bilgin, Cemal Cagatay Fonteney, Gerald Chang, Hang Henderson, Matthew Han, Ju Parvin, Bahram TI Stiffness of the microenvironment upregulates ERBB2 expression in 3D cultures of MCF10A within the range of mammographic density SO SCIENTIFIC REPORTS LA English DT Article ID BREAST-CANCER RISK; GENE-EXPRESSION; 3-DIMENSIONAL CULTURE; EXTRACELLULAR-MATRIX; MALIGNANT PHENOTYPE; CROSS-LINKING; IN-VIVO; CELLS; COLLAGEN; GROWTH AB The effects of the stiffness of the microenvironment on the molecular response of 3D colony organization, at the maximum level of mammographic density (MD), are investigated. Phenotypic profiling reveals that 3D colony formation is heterogeneous and increased stiffness of the microenvironment, within the range of the MD, correlates with the increased frequency of aberrant 3D colony formation. Further integrative analysis of the genome-wide transcriptome and phenotypic profiling hypothesizes overexpression of ERBB2 in the premalignant MCF10A cell lines at a stiffness value that corresponds to the collagen component at high mammographic density. Subsequently, ERBB2 overexpression has been validated in the same cell line. Similar experiments with a more genetically stable cell line of 184A1 also revealed an increased frequency of aberrant colony formation with the increased stiffness; however, 184A1 did not demonstrate overexpression of ERBB2 at the same stiffness value of the high MD. These results suggest that stiffness exacerbates premalignant cell line of MCF10A. C1 [Cheng, Qingsu; Chang, Hang; Henderson, Matthew; Han, Ju; Parvin, Bahram] Univ Nevada, Dept Elect & Biomed Engn, 1664 N Virginia St, Reno, NV 89503 USA. [Cheng, Qingsu; Bilgin, Cemal Cagatay; Fonteney, Gerald; Chang, Hang; Parvin, Bahram] Lawrence Berkeley Natl Lab, Div Life Sci, 1 Cyclotron Rd,MS 977, Berkeley, CA 94720 USA. RP Parvin, B (reprint author), Univ Nevada, Dept Elect & Biomed Engn, 1664 N Virginia St, Reno, NV 89503 USA.; Parvin, B (reprint author), Lawrence Berkeley Natl Lab, Div Life Sci, 1 Cyclotron Rd,MS 977, Berkeley, CA 94720 USA. EM bparvin@unr.edu FU NIH [R01CA140663]; UNR FX This work was supported by NIH under the award number R01CA140663 and internal funds from UNR. NR 53 TC 1 Z9 1 U1 8 U2 8 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 7 PY 2016 VL 6 AR 28987 DI 10.1038/srep28987 PG 13 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DQ3VP UT WOS:000379132000001 PM 27383056 ER PT J AU Strelcov, E Ievlev, A Belianinov, A Tselev, A Kolmakov, A Kalinin, SV AF Strelcov, Evgheni Ievlev, Anton Belianinov, Alex Tselev, Alexander Kolmakov, Andrei Kalinin, Sergei V. TI Local coexistence of VO2 phases revealed by deep data analysis SO SCIENTIFIC REPORTS LA English DT Article ID METAL-INSULATOR-TRANSITION; MODELING MIXTURE ANALYSIS; VANADIUM DIOXIDE; RAMAN-SPECTROSCOPY; NANOPLATELETS; TEMPERATURE; NANOBEAM; DRIVEN; M2 AB We report a synergistic approach of micro-Raman spectroscopic mapping and deep data analysis to study the distribution of crystallographic phases and ferroelastic domains in a defected Al-doped VO2 microcrystal. Bayesian linear unmixing revealed an uneven distribution of the T phase, which is stabilized by the surface defects and uneven local doping that went undetectable by other classical analysis techniques such as PCA and SIMPLISMA. This work demonstrates the impact of information recovery via statistical analysis and full mapping in spectroscopic studies of vanadium dioxide systems, which is commonly substituted by averaging or single point-probing approaches, both of which suffer from information misinterpretation due to low resolving power. C1 [Strelcov, Evgheni; Ievlev, Anton; Belianinov, Alex; Tselev, Alexander; Kalinin, Sergei V.] Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA. [Strelcov, Evgheni; Ievlev, Anton; Belianinov, Alex; Tselev, Alexander; Kalinin, Sergei V.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Strelcov, Evgheni; Kolmakov, Andrei] NIST, Ctr Nanoscale Sci & Technol, Gaithersburg, MD 20899 USA. [Strelcov, Evgheni] Univ Maryland, Maryland Nanoctr, College Pk, MD 20742 USA. RP Strelcov, E (reprint author), Oak Ridge Natl Lab, Inst Funct Imaging Mat, Oak Ridge, TN 37831 USA.; Strelcov, E (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.; Strelcov, E (reprint author), NIST, Ctr Nanoscale Sci & Technol, Gaithersburg, MD 20899 USA.; Strelcov, E (reprint author), Univ Maryland, Maryland Nanoctr, College Pk, MD 20742 USA. EM Evgheni.strelcov@nist.gov RI Kolmakov, Andrei/B-1460-2017 OI Kolmakov, Andrei/0000-0001-5299-4121 FU Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; University of Maryland; National Institute of Standards and Technology Center for Nanoscale Science and Technology [70NANB10H193] FX This research was conducted at the Center for Nanophase Materials Sciences, which is sponsored at Oak Ridge National Laboratory by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. ES acknowledges support under the Cooperative Research Agreement between the University of Maryland and the National Institute of Standards and Technology Center for Nanoscale Science and Technology, Award 70NANB10H193, through the University of Maryland. NR 33 TC 0 Z9 0 U1 26 U2 40 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2045-2322 J9 SCI REP-UK JI Sci Rep PD JUL 7 PY 2016 VL 6 AR 29216 DI 10.1038/srep29216 PG 6 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DQ3ZQ UT WOS:000379143000001 PM 27384473 ER PT J AU Liu, ZY Duchon, T Wang, HR Grinter, DC Waluyo, I Zhou, J Liu, Q Jeong, B Crumlin, EJ Matolin, V Stacchiola, DJ Rodriguez, JA Senanayake, SD AF Liu, Zongyuan Duchon, Tomas Wang, Huanru Grinter, David C. Waluyo, Iradwikanari Zhou, Jing Liu, Qiang Jeong, Beomgyun Crumlin, Ethan J. Matolin, Vladimir Stacchiola, Dario J. Rodriguez, Jose A. Senanayake, Sanjaya D. TI Ambient pressure XPS and IRRAS investigation of ethanol steam reforming on Ni-CeO2(111) catalysts: an in situ study of C-C and O-H bond scission SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID RAY PHOTOELECTRON-SPECTROSCOPY; CEO2(111) THIN-FILMS; GAS SHIFT REACTION; HYDROGEN-PRODUCTION; CERIUM OXIDE; H-2 PRODUCTION; ROOM-TEMPERATURE; ACETIC-ACID; FUEL-CELL; ADSORPTION AB Ambient-Pressure X-ray Photoelectron Spectroscopy (AP-XPS) and Infrared Reflection Absorption Spectroscopy (AP-IRRAS) have been used to elucidate the active sites and mechanistic steps associated with the ethanol steam reforming reaction (ESR) over Ni-CeO2(111) model catalysts. Our results reveal that surface layers of the ceria substrate are both highly reduced and hydroxylated under reaction conditions while the small supported Ni nanoparticles are present as Ni-0/NixC. A multifunctional, synergistic role is highlighted in which Ni, CeOx and the interface provide an ensemble effect in the active chemistry that leads to H-2. Ni-0 is the active phase leading to both C-C and C-H bond cleavage in ethanol and it is also responsible for carbon accumulation. On the other hand, CeOx is important for the deprotonation of ethanol/water to ethoxy and OH intermediates. The active state of CeOx is a Ce3+(OH)(x) compound that results from extensive reduction by ethanol and the efficient dissociation of water. Additionally, we gain an important insight into the stability and selectivity of the catalyst by its effective water dissociation, where the accumulation of surface carbon can be mitigated by the increased presence of surface OH groups. The co-existence and cooperative interplay of Ni-0 and Ce3+(OH)(x) through a metal-support interaction facilitate oxygen transfer, activation of ethanol/water as well as the removal of coke. C1 [Liu, Zongyuan; Wang, Huanru; Grinter, David C.; Waluyo, Iradwikanari; Stacchiola, Dario J.; Rodriguez, Jose A.; Senanayake, Sanjaya D.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. [Liu, Zongyuan; Rodriguez, Jose A.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Duchon, Tomas; Matolin, Vladimir] Charles Univ Prague, Fac Math & Phys, V Holesovickach 2, Prague 8, Czech Republic. [Zhou, Jing] Univ Wyoming, Dept Chem, Laramie, WY 82071 USA. [Liu, Qiang; Jeong, Beomgyun; Crumlin, Ethan J.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Senanayake, SD (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM ssenanay@bnl.gov RI Stacchiola, Dario/B-1918-2009; Senanayake, Sanjaya/D-4769-2009; OI Stacchiola, Dario/0000-0001-5494-3205; Senanayake, Sanjaya/0000-0003-3991-4232; Grinter, David/0000-0001-6089-119X; Liu, Zongyuan/0000-0001-8526-5590 FU U.S. Department of Energy, Office of Science and Office of Basic Energy Sciences [DE-SC0012704]; Ministry of Education of the Czech Republic [LH15272]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX The research carried out at Brookhaven National Laboratory was supported by the U.S. Department of Energy, Office of Science and Office of Basic Energy Sciences under contract No. DE-SC0012704. The collaborative work with Charles University in Prague is part of the KONTAKT project that was supported by the Ministry of Education of the Czech Republic (LH15272). The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 60 TC 6 Z9 6 U1 47 U2 80 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD JUL 7 PY 2016 VL 18 IS 25 BP 16621 EP 16628 DI 10.1039/c6cp01212d PG 8 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DP7WY UT WOS:000378711100002 PM 27095305 ER PT J AU Dey, S Mardinly, J Wang, YQ Valdez, JA Holesinger, TG Uberuaga, BP Ditto, JJ Drazin, JW Castro, RHR AF Dey, Sanchita Mardinly, John Wang, Yongqiang Valdez, James A. Holesinger, Terry G. Uberuaga, Blas P. Ditto, Jeff J. Drazin, John W. Castro, Ricardo H. R. TI Irradiation-induced grain growth and defect evolution in nanocrystalline zirconia with doped grain boundaries SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID RADIATION TOLERANCE; SOLUTE SEGREGATION; AMORPHIZATION; RESISTANCE; CERAMICS; MOBILITY AB Grain boundaries are effective sinks for radiation-induced defects, ultimately impacting the radiation tolerance of nanocrystalline materials (dense materials with nanosized grains) against net defect accumulation. However, irradiation-induced grain growth leads to grain boundary area decrease, shortening potential benefits of nanostructures. A possible approach to mitigate this is the introduction of dopants to target a decrease in grain boundary mobility or a reduction in grain boundary energy to eliminate driving forces for grain growth (using similar strategies as to control thermal growth). Here we tested this concept in nanocrystalline zirconia doped with lanthanum. Although the dopant is observed to segregate to the grain boundaries, causing grain boundary energy decrease and promoting dragging forces for thermally activated boundary movement, irradiation induced grain growth could not be avoided under heavy ion irradiation, suggesting a different growth mechanism as compared to thermal growth. Furthermore, it is apparent that reducing the grain boundary energy reduced the effectiveness of the grain boundary as sinks, and the number of defects in the doped material is higher than in undoped (La-free) YSZ. C1 [Dey, Sanchita; Drazin, John W.; Castro, Ricardo H. R.] Univ Calif Davis, Dept Mat Sci & Engn, Davis, CA 95616 USA. [Dey, Sanchita; Drazin, John W.; Castro, Ricardo H. R.] Univ Calif Davis, NEAT ORU, Davis, CA 95616 USA. [Mardinly, John] Arizona State Univ, John Cowley Ctr HREM, LE CSSS, Tempe, AZ USA. [Wang, Yongqiang; Valdez, James A.; Uberuaga, Blas P.] Los Alamos Natl Lab, Mat Sci & Technol Div, POB 1663, Los Alamos, NM 87545 USA. [Holesinger, Terry G.] Los Alamos Natl Lab, Mat Phys & Applicat Div, POB 1663, Los Alamos, NM 87545 USA. [Ditto, Jeff J.] Univ Oregon, Dept Chem & Biochem, Eugene, OR 97403 USA. RP Castro, RHR (reprint author), Univ Calif Davis, Dept Mat Sci & Engn, Davis, CA 95616 USA.; Castro, RHR (reprint author), Univ Calif Davis, NEAT ORU, Davis, CA 95616 USA. EM rhrcastro@ucdavis.edu FU US Department of Energy [BES ER46795]; Ion Beam Materials Laboratory by The Center for Integrated Nanotechnologies (CINT), a DOE Nanoscience User Facility; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; National Nuclear Security Administration of the (U.S.) Department of Energy [DE-AC52-06NA25396] FX RHRC would like to thank US Department of Energy - BES ER46795 for support of this work. YQW acknowledges partial support of the Ion Beam Materials Laboratory by The Center for Integrated Nanotechnologies (CINT), a DOE Nanoscience User Facility jointly operated by Los Alamos and Sandia National Laboratories. BPU acknowledges support by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the (U.S.) Department of Energy under contract DE-AC52-06NA25396. NR 38 TC 1 Z9 1 U1 7 U2 7 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD JUL 7 PY 2016 VL 18 IS 25 BP 16921 EP 16929 DI 10.1039/c6cp01763k PG 9 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DP7WY UT WOS:000378711100035 PM 27282392 ER PT J AU Cama, CA Pelliccione, CJ Brady, AB Li, J Stach, EA Wang, JJ Wang, J Takeuchi, ES Takeuchi, KJ Marschilok, AC AF Cama, Christina A. Pelliccione, Christopher J. Brady, Alexander B. Li, Jing Stach, Eric A. Wang, Jiajun Wang, Jun Takeuchi, Esther S. Takeuchi, Kenneth J. Marschilok, Amy C. TI Redox chemistry of a binary transition metal oxide (AB(2)O(4)): a study of the Cu2+/Cu-0 and Fe3+/Fe-0 interconversions observed upon lithiation in a CuFe2O4 battery using X-ray absorption spectroscopy SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS LA English DT Article ID LITHIUM-ION BATTERIES; ANODE MATERIAL; FINE-STRUCTURE; NANOCRYSTALLINE MAGNETITE; NANOSTRUCTURED CUFE2O4; COMBUSTION SYNTHESIS; COPPER FERRITE; SIZE; ELECTROCHEMISTRY; MICROSCOPY AB Copper ferrite, CuFe2O4, is a promising candidate for application as a high energy electrode material in lithium based batteries. Mechanistic insight on the electrochemical reduction and oxidation processes was gained through the first X-ray absorption spectroscopic study of lithiation and delithiation of CuFe2O4. A phase pure tetragonal CuFe2O4 material was prepared and characterized using laboratory and synchrotron X-ray diffraction, Raman spectroscopy, and transmission electron microscopy. Ex situ X-ray absorption spectroscopy (XAS) measurements were used to study the battery redox processes at the Fe and Cu K-edges, using X-ray absorption near-edge structure (XANES), extended X-ray absorption fine structure (EXAFS), and transmission X-ray microscopy (TXM) spectroscopies. EXAFS analysis showed upon discharge, an initial conversion of 50% of the copper(II) to copper metal positioned outside of the spinel structure, followed by a migration of tetrahedral iron(III) cations to octahedral positions previously occupied by copper(II). Upon charging to 3.5 V, the copper metal remained in the metallic state, while iron metal oxidation to iron(III) was achieved. The results provide new mechanistic insight regarding the evolution of the local coordination environments at the iron and copper centers upon discharging and charging. C1 [Cama, Christina A.; Takeuchi, Esther S.; Takeuchi, Kenneth J.; Marschilok, Amy C.] SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA. [Pelliccione, Christopher J.; Stach, Eric A.; Wang, Jiajun; Wang, Jun; Takeuchi, Esther S.] Brookhaven Natl Lab, Energy Sci Directorate, Upton, NY 11973 USA. [Brady, Alexander B.; Li, Jing; Takeuchi, Esther S.; Takeuchi, Kenneth J.; Marschilok, Amy C.] SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. RP Takeuchi, ES; Takeuchi, KJ; Marschilok, AC (reprint author), SUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA.; Takeuchi, ES (reprint author), Brookhaven Natl Lab, Energy Sci Directorate, Upton, NY 11973 USA.; Takeuchi, ES; Takeuchi, KJ; Marschilok, AC (reprint author), SUNY Stony Brook, Dept Mat Sci & Engn, Stony Brook, NY 11794 USA. EM esther.takeuchi@stonybrook.edu; kenneth.takeuchi.1@stonybrook.edu; amy.marschilok@stonybrook.edu RI Stach, Eric/D-8545-2011 OI Stach, Eric/0000-0002-3366-2153 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0012673]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0012704]; DOE Office of Science [DE-SC0012704, DE-AC02-06CH11357]; National Synchrotron Light Source II, Brookhaven National Laboratory, under DOE [DE-SC0012704] FX The authors acknowledge the Center for Mesoscale Transport Properties, an Energy Frontier Research Center supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, under award #DE-SC0012673 for financial support. Use of the Center for Functional Nanomaterials at Brookhaven National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-SC0012704. This research used resources of the Advanced Photon Source, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. This research used the 28-ID beamline (XPD) of the National Synchrotron Light Source II, a U.S. Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Brookhaven National Laboratory under Contract No. DE-SC0012704. Use of APS Beamline 8BM is partially supported by the National Synchrotron Light Source II, Brookhaven National Laboratory, under DOE Contract No. DE-SC0012704. The authors express their appreciation to Sanjit Ghose, Milinda Abeykoon, Jianming Bai, and Eric Dooryhee for helpful assistance with the measurements at the BNL NSLS-II XPD 1 beamline. The authors acknowledge Yu-chen Karen Chen-Wiegart for preparing the custom Matlab program used to analyze the TXM data. NR 41 TC 2 Z9 2 U1 19 U2 42 PU ROYAL SOC CHEMISTRY PI CAMBRIDGE PA THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND SN 1463-9076 EI 1463-9084 J9 PHYS CHEM CHEM PHYS JI Phys. Chem. Chem. Phys. PD JUL 7 PY 2016 VL 18 IS 25 BP 16930 EP 16940 DI 10.1039/c6cp02974d PG 11 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DP7WY UT WOS:000378711100036 PM 27292604 ER PT J AU Pandini, A Morcos, F Khan, S AF Pandini, Alessandro Morcos, Faruck Khan, Shahid TI The Gearbox of the Bacterial Flagellar Motor Switch SO STRUCTURE LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; RESPONSE REGULATOR CHEY; ROTOR PROTEIN FLIG; ESCHERICHIA-COLI; SALMONELLA-TYPHIMURIUM; RESIDUE COEVOLUTION; TORQUE RING; COMPLEX; CONFORMATIONS; MOTIONS AB Switching of flagellar motor rotation sense dictates bacterial chemotaxis. Multi-subunit FliM-FliG rotor rings couple signal protein binding in FliM with reversal of a distant FliG C-terminal (FliG(C)) helix involved in stator contacts. Subunit dynamics were examined in conformer ensembles generated by molecular simulations from the X-ray structures. Principal component analysis extracted collective motions. Interfacial loop immobilization by complex formation coupled elastic fluctuations of the FliM middle (FliM(M)) and FliG middle (FliG(M)) domains. Coevolved mutations captured interfacial dynamics as well as contacts. FliG(M) rotation was amplified via two central hinges to the FliG(C) helix. Intrinsic flexibility, reported by the FliG(MC) ensembles, reconciled conformers with opposite FliG(C) helix orientations. FliG domain stacking deformed the inter-domain linker and reduced flexibility; but conformational changes were not triggered by engineered linker deletions that cause a rotation-locked phenotype. These facts suggest that binary rotation states arise from conformational selection by stacking interactions. C1 [Pandini, Alessandro] Brunel Univ London, Dept Comp Sci, Uxbridge UB8 3PH, Middx, England. [Pandini, Alessandro] Brunel Univ London, Synthet Biol Theme, Uxbridge UB8 3PH, Middx, England. [Pandini, Alessandro] Francis Crick Inst, Computat Cell & Mol Biol, London NW1 1AT, England. [Morcos, Faruck] Univ Texas Dallas, Dept Biol Sci, Richardson, TX 75080 USA. [Khan, Shahid] Lawrence Berkeley Natl Lab, Mol Biol Consortium, Berkeley, CA 94720 USA. RP Khan, S (reprint author), Lawrence Berkeley Natl Lab, Mol Biol Consortium, Berkeley, CA 94720 USA. EM khan@mbc-als.org RI Pandini, Alessandro/F-9854-2012 OI Pandini, Alessandro/0000-0002-4158-233X FU Royal Society Collaborative Exchange Grant [Ul175.70592]; Molecular Biology Consortium; Cancer Research UK; UK Medical Research Council; Wellcome Trust through the Taylor group [10179] FX This work was supported by the Royal Society Collaborative Exchange Grant Ul175.70592, the Molecular Biology Consortium (S.K) and the Francis Crick Institute which receives core funding from Cancer Research UK, the UK Medical Research Council, and Wellcome Trust through the Taylor (10179) group. NR 50 TC 0 Z9 0 U1 1 U2 1 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 0969-2126 EI 1878-4186 J9 STRUCTURE JI Structure PD JUL 6 PY 2016 VL 24 IS 7 BP 1209 EP 1220 DI 10.1016/j.str.2016.05.012 PG 12 WC Biochemistry & Molecular Biology; Biophysics; Cell Biology SC Biochemistry & Molecular Biology; Biophysics; Cell Biology GA DV9EU UT WOS:000383243800018 PM 27345932 ER PT J AU Aad, G Abbott, B Abdallah, J Abdinov, O Abeloos, B Aben, R Abolins, M AbouZeid, OS Abraham, NL Abramowicz, H Abreu, H Abreu, R Abulaiti, Y Acharya, BS Adamczyk, L Adams, DL Adelman, J Adomeit, S Adye, T Affolder, AA Agatonovic-Jovin, T Agricola, J Aguilar-Saavedraa, JA Ahlen, SP Ahmadov, F Aielli, G Akerstedt, H Akesson, TPA Akimov, AV Alberghi, GL Albert, J Albrand, S Verzini, MJA Aleksa, M Aleksandrov, IN Alexa, C Alexander, G Alexopoulos, T Alhroob, M Aliev, M Alimonti, G Alison, J Alkire, SP Allbrooke, BMM Allen, BW Allport, PP Aloisio, A Alonso, A Alonso, F Alpigiani, C Gonzalez, BA Piqueras, DA Alviggi, MG Amadio, BT Amako, K Coutinho, YA Amelung, C Amidei, D Dos Santos, SPA Amorim, A Amoroso, S Amram, N Amundsen, G Anastopoulos, C Ancu, LS Andari, N Andeen, T Anders, CF Anders, G Anders, JK Anderson, KJ Andreazza, A Andrei, V Angelidakis, S Angelozzi, I Anger, P Angerami, A Anghinolfi, F Anisenkov, AV Anjos, N Annovi, A Antonelli, M Antonov, A Antos, J Anulli, F Aoki, M Bella, LA Arabidze, G Arai, Y Araque, JP Arce, ATH Arduh, FA Arguin, JF Argyropoulos, S Arika, M Armbruster, AJ Armitage, LJ Arnaez, O Arnold, H Arratia, M Arslan, O Artamonov, A Artoni, G Artz, S Asai, S Asbah, N Ashkenazi, A Asman, B Asquith, L Assamagan, K Astalos, R Atkinson, M Atlay, NB Augsten, K Avolio, G Axen, B Ayoub, MK Azuelos, G Baak, MA Baas, AE Baca, MJ Bachacou, H Bachas, K Backes, M Backhaus, M Bagiacchi, P Bagnaia, P Bai, Y Baines, JT Baker, OK Baldin, EM Balek, P Balestri, T Balli, F Balunas, WK Banas, E Banerjee, S Bannoura, AAE Barak, L Barberio, EL Barberis, D Barbero, M Barillari, T Barisonzi, M Barklow, T Barlow, N Barnes, SL Barnett, BM Barnett, RM Barnovska, Z Baroncelli, A Barone, G Barr, AJ Navarro, LB Barreiro, F da Costa, JBG Bartoldus, R Barton, AE Bartos, P Basalaev, A Bassalat, A Basye, A Bates, RL Batista, SJ Batley, JR Battaglia, M Bauce, M Bauer, F Bawa, HS Beacham, JB Beattie, MD Beau, T Beauchemin, PH Bechtle, P Beck, HP Becker, K Becker, M Beckingham, M Becot, C Beddall, AJ Beddall, A Bednyakov, VA Bedognetti, M Bee, CP Beemster, LJ Beermann, TA Begel, M Behr, JK Belanger-Champagne, C Bell, AS Bell, WH Bella, G Bellagamba, L Bellerive, A Bellomo, M Belotskiy, K Beltramello, O Belyaev, NL Benary, O Benchekroun, D Bender, M Bendtz, K Benekos, N Benhammou, Y Noccioli, EB Benitez, J Garcia, JAB Benjamin, DP Bensinger, JR Bentvelsen, S Beresford, L Beretta, M Berge, D Kuutmann, EB Berger, N Berghaus, F Beringer, J Berlendis, S Bernard, NR Bernius, C Bernlochner, FU Berry, T Berta, P Bertella, C Bertoli, G Bertolucci, F Bertram, IA Bertsche, C Bertsche, D Besjes, GJ Bylund, OB Bessner, M Besson, N Betancourt, C Bethke, S Bevan, AJ Bhimji, W Bianchi, RM Bianchini, L Bianco, M Biebel, O Biedermann, D Bielski, R Biesuz, NV Biglietti, M De Mendizabal, JB Bilokon, H Bindi, M Binet, S Bingul, A Bini, C Biondi, S Bjergaard, DM Black, CW Black, JE Black, KM Blackburn, D Blair, RE Blanchard, JB Blanco, JE Blazek, T Bloch, I Blocker, C Blum, W Blumenschein, U Blunier, S Bobbink, GJ Bobrovnikov, VS Bocchetta, SS Bocci, A Bock, C Boehler, M Boerner, D Bogaerts, JA Bogavac, D Bogdanchikov, AG Bohm, C Boisvert, V Bold, T Boldea, V Boldyrev, AS Bomben, M Bona, M Boonekamp, M Borisov, A Borissov, G Bortfeldt, J Bortoletto, D Bortolotto, V Bos, K Boscherini, D Bosman, M Sola, JDB Boudreau, J Bouffard, J Bouhova-Thacker, EV Boumediene, D Bourdarios, C Boutle, SK Boveia, A Boyd, J Boyko, IR Bracinik, J Brandt, A Brandt, G Brandt, O Bratzler, U Brau, B Brau, JE Braun, HM Madden, WDB Brendlinger, K Brennan, AJ Brenner, L Brenner, R Bressler, S Bristow, TM Britton, D Britzger, D Brochu, FM Brock, I Brock, R Brooijmans, G Brooks, T Brooks, WK Brosamer, J Brost, E Broughton, JH de Renstrom, PAB Bruncko, D Bruneliere, R Bruni, A Bruni, G Brunt, BH Bruschi, M Bruscino, N Bryant, P Bryngemark, L Buanes, T Buat, Q Buchholz, P Buckley, AG Budagov, IA Buehrer, F Bugge, MK Bulekov, O Bullock, D Burckhart, H Burdin, S Burgard, CD Burghgrave, B Burka, K Burke, S Burmeister, I Busato, E Buscher, D Buscher, V Bussey, P Butler, JM Butt, AI Buttar, CM Butterworth, JM Butti, P Buttinger, W Buzatu, A Buzykaev, AR Urban, SC Caforio, D Cairo, VM Cakira, O Calace, N Calafiura, P Calandri, A Calderini, G Calfayan, P Caloba, LP Calvet, D Calvet, S Calvet, TP Toro, RC Camarda, S Camarri, P Cameron, D Armadans, RC Camincher, C Campana, S Campanelli, M Campoverde, A Canale, V Canepa, A Bret, MC Cantero, J Cantrilla, R Cao, T Garrido, MDMC Caprini, I Caprini, M Capua, M Caputo, R Carbone, RM Cardarelli, R Cardillo, F Carli, T Carlino, G Carminati, L Caron, S Carquin, E Carrillo-Montoya, GD Carter, JR Carvalho, J Casadei, D Casado, MP Casolino, M Casper, DW Castaneda-Miranda, E Castelli, A Gimenez, VC Castro, NF Catinaccio, A Catmore, JR Cattai, A Caudron, J Cavaliere, V Cavallaro, E Cavalli, D Cavalli-Sforza, M Cavasinni, V Ceradini, F Alberich, LC Cerio, BC Cerqueira, AS Cerri, A Cerrito, L Cerutti, F Cerv, M Cervelli, A Cetin, SA Chafaq, A Chakraborty, D Chalupkova, I Chan, SK Chan, YL Chang, P Chapman, JD Charlton, DG Chatterjee, A Chau, CC Barajas, CAC Che, S Cheatham, S Chegwidden, A Chekanov, S Chekulaev, SV Chelkov, GA Chelstowska, MA Chen, C Chen, H Chen, K Chen, S Chen, S Chen, X Chen, Y Cheng, HC Cheng, HJ Cheng, Y Cheplakov, A Cheremushkina, E El Moursli, RC Chernyatin, V Cheu, E Chevalier, L Chiarella, V Chiarelli, G Chiodini, G Chisholm, AS Chitan, A Chizhov, MV Choi, K Chomont, AR Chouridou, S Chow, BKB Christodoulou, V Chromek-Burckhart, D Chudoba, J Chuinard, AJ Chwastowski, JJ Chytka, L Ciapetti, G Ciftci, AK Cinca, D Cindro, V Cioara, IA Ciocio, A Cirotto, F Citron, ZH Ciubancan, M Clark, A Clark, BL Clark, MR Clark, PJ Clarke, RN Clement, C Coadou, Y Cobal, M Coccaro, A Cochran, J Coffey, L Colasurdo, L Cole, B Cole, S Colijn, AP Collot, J Colombo, T Compostella, G Muino, PC Coniavitis, E Connell, SH Connelly, IA Consorti, V Constantinescu, S Conta, C Conti, G Conventi, F Cooke, M Cooper, BD Cooper-Sarkar, AM Cornelissen, T Corradi, M Corriveau, F Corso-Radu, A Cortes-Gonzalez, A Cortiana, G Costa, G Costa, MJ Costanzo, D Cottin, G Cowan, G Cox, BE Cranmer, K Crawley, SJ Cree, G Crepe-Renaudin, S Crescioli, F Cribbs, WA Ortuzar, MC Cristinziani, M Croft, V Crosetti, G Donszelmann, TC Cummings, J Curatolo, M Cuth, J Cuthbert, C Czirr, H Czodrowski, P D'Auria, S D'Onofrio, M De Sousa, MJDS Da Via, C Dabrowski, W Dai, T Dale, O Dallaire, F Dallapiccola, C Dam, M Dandoy, JR Dang, NP Daniells, AC Dann, NS Danninger, M Hoffmann, MD Dao, V Darbo, G Darmora, S Dassoulas, J Dattagupta, A Davey, W David, C Davidek, T Davies, M Davison, P Davygora, Y Dawe, E Dawson, I Daya-Ishmukhametova, RK De, K de Asmundis, R De Benedetti, A De Castro, S De Cecco, S De Groot, N de Jong, P De la Torre, H De Lorenzi, F De Pedis, D De Salvo, A De Sanctis, U De Santo, A De Regie, JBD Dearnaley, WJ Debbe, R Debenedetti, C Dedovich, DV Deigaard, I Del Peso, J Del Prete, T Delgove, D Deliot, F Delitzsch, CM Deliyergiyev, M Dell'Acqua, A Dell'Asta, L Dell'Orso, M Della Pietra, M della Volpe, D Delmastro, M Delsart, PA Deluca, C DeMarco, DA Demers, S Demichev, M Demilly, A Denisov, SP Denysiuk, D Derendarz, D Derkaoui, JE Derue, F Dervan, P Desch, K Deterre, C Dette, K Deviveiros, PO Dewhurst, A Dhaliwal, S Di Ciaccio, A Di Ciaccio, L Di Clemente, WK Di Domenico, A Di Donato, C Di Girolamo, A Di Girolamo, B Di Mattia, A Di Micco, B Di Nardo, R Di Simone, A Di Sipio, R Di Valentino, D Diaconu, C Diamond, M Dias, FA Diaz, MA Diehl, EB Dietrich, J Diglio, S Dimitrievska, A 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Wienemann, P. Wiglesworth, C. Wiik-Fuchs, L. A. M. Wildauer, A. Wilk, F. Wilkens, H. G. Williams, H. H. Williams, S. Willis, C. Willocq, S. Wilson, J. A. Wingerter-Seez, I. Winklmeier, F. Winston, O. J. Winter, B. T. Wittgen, M. Wittkowski, J. Wollstadt, S. J. Wolter, M. W. Wolters, H. Wosiek, B. K. Wotschack, J. Woudstra, M. J. Wozniak, K. W. Wu, M. Wu, M. Wu, S. L. Wu, X. Wu, Y. Wyatt, T. R. Wynne, B. M. Xella, S. Xu, D. Xu, L. Yabsley, B. Yacoob, S. Yakabe, R. Yamaguchi, D. Yamaguchi, Y. Yamamoto, A. Yamamoto, S. Yamanaka, T. Yamauchi, K. Yamazaki, Y. Yan, Z. Yange, H. Yang, H. Yang, Y. Yang, Z. Yao, W-M. Yap, Y. C. Yasu, Y. Yatsenko, E. Wong, K. H. Yau Ye, J. Ye, S. Yeletskikh, I. Yen, A. L. Yildirim, E. Yorita, K. Yoshida, R. Yoshihara, K. Young, C. Young, C. J. S. Youssef, S. Yu, D. R. Yu, J. Yu, J. M. Yu, J. Yuan, L. Yuen, S. P. Y. Yusuff, I. Zabinski, B. Zaidan, R. Zaitsev, A. M. Zakharchuk, N. Zalieckas, J. Zaman, A. Zambito, S. Zanello, L. Zanzi, D. Zeitnitz, C. Zeman, M. Zemla, A. Zeng, J. C. Zeng, Q. Zengel, K. Zenin, O. Zenis, T. Zerwas, D. Zhang, D. Zhang, F. Zhang, G. Zhang, H. Zhang, J. Zhang, L. Zhang, R. Zhang, R. Zhang, X. Zhang, Z. Zhao, X. Zhao, Y. Zhao, Z. Zhemchugov, A. Zhong, J. Zhou, B. Zhou, C. Zhou, L. Zhou, L. Zhou, M. Zhou, N. Zhu, C. G. Zhu, H. Zhu, J. Zhu, Y. Zhuang, X. Zhukov, K. Zibell, A. Zieminska, D. Zimine, N. I. Zimmermann, C. Zimmermann, S. Zinonos, Z. Zinser, M. Ziolkowski, M. Zivkovic, L. Zobernig, G. Zoccoli, A. zur Nedden, M. Zurzolo, G. Zwalinski, L. CA ATLAS Collaboration TI Measurement of event-shape observables in Z -> l(+)l(-) events in pp collisions at root s=7 TeV with the ATLAS detector at the LHC SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article AB Event-shape observables measured using charged particles in inclusive Z-boson events are presented, using the electron and muon decay modes of the Z bosons. The measurements are based on an integrated luminosity of 1.1 fb(-1) of proton-proton collisions recorded by the ATLAS detector at the LHC at a centre-of-mass energy root s = 7 TeV. Charged-particle distributions, excluding the lepton-antilepton pair from the Z-boson decay, are measured in different ranges of transverse momentum of the Z boson. Distributions include multiplicity, scalar sum of transverse momenta, beam thrust, transverse thrust, spherocity, and F-parameter, which are in particular sensitive to properties of the underlying event at small values of the Z-boson transverse momentum. The measured observables are compared with predictions from PYTHIA 8, Sherpa, and HERWIG 7. Typically, all three Monte Carlo generators provide predictions that are in better agreement with the data at high Z-boson transverse momenta than at low Z-boson transverse momenta, and for the observables that are less sensitive to the number of charged particles in the event. C1 [Jackson, P.; Lee, L.; Petridis, A.; Robertson, S. H.; White, M. J.] Univ Adelaide, Dept Phys, Adelaide, SA, Australia. [Bouffard, J.; Edson, W.; Ernst, J.; Fischer, A.; Guindon, S.; Jain, V.] SUNY Albany, Dept Phys, Albany, NY 12222 USA. [Butt, A. I.; Czodrowski, P.; Dassoulas, J.; Gingrich, D. M.; Jabbar, S.; Karamaoun, A.; Moore, R. W.; Pinfold, J. L.] Univ Alberta, Dept Phys, Edmonton, AB, Canada. [Cakira, O.; Ciftci, A. K.; Yildiz, H. Duran] Ankara Univ, Dept Phys, Ankara, Turkey. [Kuday, S.] Istanbul Aydin Univ, Istanbul, Turkey. [Sultansoy, S.] TOBB Univ Econ & Technol, Div Phys, Ankara, Turkey. [Barnovska, Z.; Berger, N.; Delmastro, M.; Di Ciaccio, L.; Elles, S.; Grevtsov, K.; Guillemin, T.; Hryn'ova, T.; Jezequel, S.; Koletsou, I.; Lafaye, R.; Leveque, J.; Mastrandrea, P.; Sauvage, G.; Sauvan, E.; Simard, O.; Smart, B. H.; Todorov, T.; Wingerter-Seez, I.; Yatsenko, E.] CNRS IN2P3, LAPP, Annecy Le Vieux, France. 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B.; Malecki, Pa.; Olszewski, A.; Olszowska, J.; Stanecka, E.; Staszewski, R.; Trzebinski, M.; Trzupek, A.; Wolter, M. W.; Wosiek, B. K.; Wozniak, K. W.; Zabinski, B.] Polish Acad Sci, Inst Nucl Phys, Krakow, Poland. [Cao, T.; Firan, A.; Hetherly, J. W.; Kama, S.; Kehoe, R.; Sekula, S. J.; Stroynowski, R.; Turvey, A. J.; Varol, T.; Wang, H.; Ye, J.; Zhao, X.; Zhou, L.] So Methodist Univ, Dept Phys, Dallas, TX 75275 USA. [Izen, J. M.; Leyton, M.; Meirose, B.; Namasivayam, H.; Reeves, K.] Univ Texas Dallas, Dept Phys, Dallas, TX 75230 USA. [Aloisio, A.; Asbah, N.; Behr, J. K.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Hamburg, Germany. [Asbah, N.; Behr, J. K.; Bessner, M.; Bloch, I.; Britzger, D.; Deterre, C.; Dutta, B.; Eckardt, C.; Filipuzzi, M.; Flaschel, N.; Bravo, A. Gascon; Glazov, A.; Gregor, I. M.; Haleem, M.; Hamnett, P. G.; Hiller, K. H.; Howarth, J.; Huang, Y.; Katzy, J.; Keller, J. S.; Kondrashova, N.; Kuhl, T.; Lobodzinska, E.; Lohwasser, K.; Madsen, A.; Mamuzic, J.; Medinnis, M.; Moenig, K.; Garcia, R. F. Naranjo; Naumann, T.; O'Rourke, A. A.; Peschke, R.; Pirumov, H.; Poley, A.; Robinson, J. E. M.; Rubinskiy, I.; Schaefer, R.; Schmitt, S.; South, D.; Stanescu-Bellu, M.; Stanitzki, M. M.; Styles, N. A.; Tackmann, K.; Trofymov, A.; Wang, J.; Yildirim, E.; Zakharchuk, N.] DESY, Zeuthen, Germany. [Burmeister, I.; Dette, K.; Erdmann, J.; Esch, H.; Gossling, C.; Homann, M.; Jentzsch, J.; Klingenberg, R.; Kroeninger, K.; Schorlemmer, A. L. S.] Tech Univ Dortmund, Inst Expt Phys 4, Dortmund, Germany. [Anger, P.; Duschinger, D.; Friedrich, F.; Grohs, J. P.; Gutschow, C.; Hauswald, L.; Kobel, M.; Mader, W. F.; Novgorodova, O.; Siegert, F.; Socher, F.; Straessner, A.; Vest, A.; Wahrmund, S.] Tech Univ Dresden, Inst Kern & Teilchenphys, Dresden, Germany. [Arce, A. T. H.; Benjamin, D. P.; Bjergaard, D. M.; Bocci, A.; Cerio, B. C.; Goshaw, A. T.; Kajomovitz, E.; Kotwal, A.; Kruse, M. C.; Li, L.; Li, S.; Liu, M.; Oh, S. H.; Zhou, C.] Duke Univ, Dept Phys, Durham, NC 27706 USA. [Bristow, T. M.; Clark, P. J.; Dias, F. A.; Edwards, N. C.; Gao, Y.; Walls, F. M. Garay; Glaysher, P. C. F.; Harrington, R. D.; Leonidopoulos, C.; Martin, V. J.; Mills, C.; Pino, S. A. Olivares; Proissl, M.; Washbrook, A.; Wynne, B. M.] Univ Edinburgh, SUPA Sch Phys & Astron, Edinburgh, Midlothian, Scotland. [Aloisio, A.; Antonelli, M.; Beretta, M.; Bilokon, H.; Chiarella, V.; Curatolo, M.; Di Nardo, R.; Esposito, B.; Gatti, C.; Laurelli, P.; Maccarrone, G.; Mancini, G.; Sansoni, A.; Testa, M.; Vilucchi, E.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Frascati, Italy. [Aloisio, A.; Arnold, H.; Betancourt, C.; Boehler, M.; Bruneliere, R.; Buehrer, F.; Burgard, C. D.; Buescher, D.; Cardillo, F.; Coniavitis, E.; Consorti, V.; Dang, N. P.; Dao, V.; Di Simone, A.; Herten, G.; Jakobs, K.; Javurek, T.; Jenni, P.; Kiss, F.; Koeneke, K.; Kopp, A. K.; Kuehn, S.; Landgraf, U.; Luedtke, C.; Mohr, W.; Pagacova, M.; Parzefall, U.; Ronzani, M.; Rosbach, K.; Ruhr, F.; Rurikova, Z.; Sammel, D.; Schillo, C.; Schnoor, U.; Schumacher, M.; Sommer, P.; Sundermann, J. E.; Ta, D.; Temming, K. K.; Tsiskaridze, V.; Weiser, C.; Werner, M.; Zhang, L.; Zimmermann, S.] Univ Freiburg, Fak Math & Phys, Freiburg, Germany. [Aloisio, A.; Alonso, A.; Ancu, L. S.; Bell, W. H.; De Mendizabal, J. Bilbao; Calace, N.; Chatterjee, A.; Clark, A.; Coccaro, A.; Delitzsch, C. M.; della Volpe, D.; Ferrere, D.; Gadomski, S.; Golling, T.; Gonzalez-Sevilla, S.; Gramling, J.; Guescini, F.; Iacobucci, G.; Katre, A.; March, L.; Mermod, P.; Miucci, A.; Nackenhorst, O.; Paolozzi, L.; Ristic, B.; Schramm, S.; Sfyrla, A.; Vallecorsa, S.; Wu, X.] Univ Geneva, Sect Phys, Geneva, Switzerland. [Aloisio, A.; Alonso, A.; Barberis, D.; Darbo, G.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Gemme, C.; Guido, E.; Morettini, P.; Osculati, B.; Parodi, F.; Passaggio, S.; Rossi, L. P.; Sannino, M.; Schiavi, C.] Ist Nazl Fis Nucl, Sez Genova, Genoa, Italy. [Barberis, D.; Favareto, A.; Parodi, A. Ferretto; Gagliardi, G.; Gaudiello, A.; Osculati, B.; Parodi, F.; Sannino, M.; Schiavi, C.] Univ Genoa, Dipartimento Fis, Genoa, Italy. [Jejelava, J.; Tskhadadze, E. G.] Iv Javakhishvili Tbilisi State Univ, E Andronikashvili Inst Phys, Tbilisi, Rep of Georgia. [Djobava, T.; Durglishvili, A.; Khubua, J.; Mosidze, M.] Tbilisi State Univ, Inst High Energy Phys, Tbilisi, Rep of Georgia. [Duren, M.; Heinz, C.; Kreutzfeldt, K.; Stenzel, H.] Univ Giessen, Inst Phys 2, Giessen, Germany. [Bates, R. L.; Boutle, S. K.; Madden, W. D. Breaden; Britton, D.; Buckley, A. G.; Bussey, P.; Buttar, C. M.; Buzatu, A.; Cinca, D.; Crawley, S. J.; D'Auria, S.; Doyle, A. T.; Ferrando, J.; de Lima, D. E. Ferreira; Gul, U.; Knue, A.; Mullen, P.; O'Shea, V.; Owen, M.; Pollard, C. S.; Qin, G.; Quilty, D.; Ravenscroft, T.; Robson, A.; Denis, R. D. St.; Stewart, G. A.; Thompson, A. S.] Univ Glasgow, SUPA Sch Phys & Astron, Glasgow, Lanark, Scotland. [Agricola, J.; Aloisio, A.; Alonso, A.; Bindi, M.; Blumenschein, U.; Brandt, G.; Drechsler, E.; Graber, L.; Grosse-Knetter, J.; Guido, E.; Janus, M.; Kareem, M. J.; Kawamura, G.; Lai, S.; Lemmer, B.; Magradze, E.; Mantoani, M.; Mchedlidze, G.; Llacer, M. Moreno; Musheghyan, H.; Nadal, J.; Quadt, A.; Rieger, J.; Shabalina, E.; Stolte, P.; Veatch, J.; Weingarten, J.; Zinonos, Z.] Univ Gottingen, Inst Phys 2, Gottingen, Germany. [Albrand, S.; Aloisio, A.; Berlendis, S.; Camincher, C.; Collot, J.; Crepe-Renaudin, S.; Delsart, P. A.; Gabaldon, C.; Genest, M. H.; Hostachy, J-Y.; Ledroit-Guillon, F.; Lleres, A.; Lucotte, A.; Malek, F.; Petit, E.; Stark, J.; Trocme, B.; Wu, M.] Univ Grenoble Alpes, Lab Phys Subatom & Cosmol, CNRS IN2P3, Grenoble, France. [McFarlane, K. W.] Hampton Univ, Dept Phys, Hampton, VA 23668 USA. [Chan, S. K.; Clark, B. L.; Franklin, M.; Giromini, P.; Huth, J.; Ippolito, V.; Lazovich, T.; Mateos, D. Lopez; Mercurio, K. M.; Morii, M.; Rogan, C. S.; Skottowe, H. P.; Sun, S.; Tolley, E.; Tong, B.; Tuna, A. N.; Yen, A. L.; Zambito, S.] Harvard Univ, Lab Particle Phys & Cosmol, Cambridge, MA 02138 USA. [Andrei, V.; Baas, A. E.; Brandt, O.; Davygora, Y.; Djuvsland, J. I.; Dunford, M.; Geisler, M. P.; Hanke, P.; Jongmanns, J.; Kluge, E. -E.; Lang, V. S.; Meier, K.; Theenhausen, H. Meyer Zu; Villar, D. I. Narrias; Sahinsoy, M.; Scharf, V.; Schultz-Coulon, H. -C.; Stamen, R.; Starovoitov, P.; Suchek, S.; Wessels, M.] Heidelberg Univ, Kirchhoff Inst Phys, Heidelberg, Germany. [Anders, C. F.; Giulini, M.; Kolb, M.; Lisovyi, M.; Radescu, V.; Schaetzel, S.; Schoening, A.; Sosa, D.] Heidelberg Univ, Inst Phys, Heidelberg, Germany. [Kretzc, M.; Kugel, A.] Heidelberg Univ, ZITI Inst Tech Informat, Mannheim, Germany. [Nagasaka, Y.] Hiroshima Inst Technol, Fac Appl Informat Sci, Hiroshima, Japan. [Bortolotto, V.; Chan, Y. L.; Castillo, L. R. Flores; Lu, H.; Salvucci, A.; Tsui, K. M.] Chinese Univ Hong Kong, Dept Phys, Shatin, Hong Kong, Peoples R China. [Bortolotto, V.; Orlando, N.] Univ Hong Kong, Dept Phys, Hong Kong, Hong Kong, Peoples R China. [Bortolotto, V.; Prokofievc, K.] Hong Kong Univ Sci & Technol, Dept Phys, Clear Water Bay, Kowloon, Hong Kong, Peoples R China. [Choi, K.; Dattagupta, A.; Evans, H.; Gagnon, P.; Kopeliansky, R.; Lammers, S.; Martinez, N. Lorenzo; Luehring, F.; Ogren, H.; Penwell, J.; Weinert, B.; Zieminska, D.] Indiana Univ, Dept Phys, Bloomington, IN 47405 USA. [Jansky, R.; Kneringer, E.; Lukas, W.; Usanova, A.; Vigne, R.] Leopold Franzens Univ, Inst Astro & Teilchenphys, Innsbruck, Austria. [Argyropoulos, S.; Benitez, J.; Mallik, U.] Univ Iowa, Iowa City, IA USA. [Chen, C.; Cochran, J.; De Lorenzi, F.; Jiang, H.; Krumnack, N.; Pluth, D.; Prell, S.; Yu, J.] Iowa State Univ, Dept Phys & Astron, Ames, IA USA. [Ahmadov, F.; Aleksandrov, I. N.; Bednyakov, V. A.; Boyko, I. R.; Budagov, I. A.; Chelkov, G. A.; Cheplakov, A.; Chizhov, M. V.; Dedovich, D. V.; Demichev, M.; Gongadze, A.; Gostkin, M. I.; Huseynov, N.; Javadov, N.; Karpov, S. N.; Karpova, Z. M.; Khramov, E.; Kotov, V. M.; Kruchonak, U.; Kukhtin, V.; Ladygin, E.; Lyubushkin, V.; Minashvili, I. A.; Mineev, M.; Peshekhonov, V. D.; Plotnikova, E.; Potrap, I. N.; Pozdnyakov, V.; Rusakovich, N. A.; Sadykov, R.; Sapronov, A.; Shiyakova, M.; Soloshenko, A.; Vinogradov, V. B.; Yeletskikh, I.; Zhemchugov, A.; Zimine, N. I.] JINR Dubna, Joint Inst Nucl Res, Dubna, Russia. [Amako, K.; Aoki, M.; Arai, Y.; Hanagaki, K.; Ikegami, Y.; Ikeno, M.; Iwasaki, H.; Kanzaki, J.; Kohriki, T.; Kondo, T.; Kono, T.; Makida, Y.; Nagai, R.; Nagano, K.; Nakamura, K.; Nozaki, M.; Odaka, S.; Okuyama, T.; Sasaki, O.; Suzuki, S.; Takubo, Y.; Tanaka, S.; Terada, S.; Tokushuku, K.; Tsuno, S.; Unno, Y.; Yamamoto, A.; Yasu, Y.] KEK, High Energy Accelerator Res Org, Tsukuba, Ibaraki, Japan. [Chen, Y.; Hasegawa, M.; Kido, S.; Kishimoto, T.; Kurashige, H.; Maeda, J.; Ochi, A.; Shimizu, S.; Takeda, H.; Yakabe, R.; Yamazaki, Y.; Yuan, L.] Kobe Univ, Grad Sch Sci, Kobe, Hyogo, Japan. [Ishino, M.; Kunigo, T.; Monden, R.; Sumida, T.; Tashiro, T.] Kyoto Univ, Fac Sci, Kyoto, Japan. [Takashima, R.] Kyoto Univ, Kyoto, Japan. [Kawagoe, K.; Oda, S.; Otono, H.; Tojo, J.] Kyushu Univ, Dept Phys, Fukuoka, Japan. [Alconada Verzini, M. J.; Aloisio, A.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Univ Nacl La Plata, Inst Fis La Plata, La Plata, Buenos Aires, Argentina. [Alconada Verzini, M. J.; Alonso, F.; Arduh, F. A.; Dova, M. T.; Monticelli, F.; Wahlberg, H.] Consejo Nacl Invest Cient & Tecn, La Plata, Buenos Aires, Argentina. [Aloisio, A.; Alonso, A.; Barton, A. E.; Beattie, M. D.; Bertram, I. A.; Borissov, G.; Bouhova-Thacker, E. V.; Cheatham, S.; Dearnaley, W. J.; Fox, H.; Grimm, K.; Henderson, R. C. W.; Hughes, G.; Jones, R. W. L.; Kartvelishvili, V.; Long, R. E.; Love, P. A.; Muenstermann, D.; Parker, A. J.; Skinner, M. B.; Smizanska, M.; Walder, J.; Wharton, A. M.] Univ Lancaster, Dept Phys, Lancaster, England. [Aliev, M.; Bachas, K.; Chiodini, G.; Gorini, E.; Longo, L.; Primavera, M.; Spagnolo, S.; Ventura, A.] Ist Nazl Fis Nucl, Sez Lecce, Lecce, Italy. [Aliev, M.; Bachas, K.; Gorini, E.; Longo, L.; Spagnolo, S.; Ventura, A.] Univ Salento, Dipartimento Matemat & Fis, Lecce, Italy. [Affolder, A. A.; Anders, J. K.; Burdin, S.; D'Onofrio, M.; Dervan, P.; Gwilliam, C. B.; Hayward, H. S.; Jackson, M.; Jones, T. J.; King, B. T.; Klein, M.; Klein, U.; Kretzschmar, J.; Laycock, P.; Lehan, A.; Maxfield, S. J.; Mehta, A.; Readioff, N. P.; Schnellbach, Y. J.; Vossebeld, J. H.] Univ Liverpool, Oliver Lodge Lab, Liverpool, Merseyside, England. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Jozef Stefan Inst, Dept Phys, Ljubljana, Slovenia. [Cindro, V.; Deliyergiyev, M.; Filipcic, A.; Gorisek, A.; Kersevan, B. P.; Kramberger, G.; Macek, B.; Mandic, I.; Mikuz, M.; Muskinja, M.; Sfiligoj, T.; Sokhrannyi, G.] Univ Ljubljana, Ljubljana, Slovenia. [Armitage, L. J.; Bevan, A. J.; Bona, M.; Cerrito, L.; Fletcher, G.; Hays, J. M.; Hickling, R.; Landon, M. P. J.; Lloyd, S. L.; Morris, J. D.; Nooney, T.; Piccaro, E.; Rizvi, E.; Sandbach, R. L.; Snidero, G.] Queen Mary Univ London, Sch Phys & Astron, London, England. [Berry, T.; Blanco, J. E.; Boisvert, V.; Brooks, T.; Connelly, I. A.; Cowan, G.; Duguid, L.; Giannelli, M. Faucci; George, S.; Gibson, S. M.; Kempster, J. J.; Vazquez, J. G. Panduro; Pastore, Fr.; Savage, G.; Sowden, B. C.; Spano, F.; Teixeira-Dias, P.; Thomas-Wilsker, J.] Royal Holloway Univ London, Dept Phys, Surrey, England. [Bell, A. S.; Butterworth, J. M.; Campanelli, M.; Casadei, D.; Christodoulou, V.; Cooper, B. D.; Davison, P.; Falla, R. J.; Freeborn, D.; Gregersen, K.; Ortiz, N. G. Gutierrez; Hesketh, G. G.; Jansen, E.; Jiggins, S.; Konstantinidis, N.; Korn, A.; Kucuk, H.; Leney, K. J. C.; Martyniuk, A. C.; McClymont, L. I.; Mcfayden, J. A.; Nurse, E.; Richter, S.; Scanlon, T.; Sherwood, P.; Simmons, B.; Wardrope, D. R.; Waugh, B. M.] UCL, Dept Phys & Astron, London, England. [Greenwood, Z. D.; Grossi, G. C.; Jana, D. K.; Sawyer, L.; Subramaniam, R.] Louisiana Tech Univ, Ruston, LA 71270 USA. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] UPMC, Lab Phys Nucl & Hautes Energies, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] Univ Paris Diderot, Paris, France. [Beau, T.; Bomben, M.; Calderini, G.; Crescioli, F.; De Cecco, S.; Demilly, A.; Derue, F.; Francavilla, P.; Krasny, M. W.; Lacour, D.; Laforge, B.; Laplace, S.; Le Dortz, O.; Lefebvre, G.; Solis, A. Lopez; Malaescu, B.; Marchiori, G.; Nikolic-Audit, I.; Ocariz, J.; Pandini, C. E.; Pires, S.; Ridel, M.; Roos, L.; Trincaz-Duvoid, S.; Varouchas, D.; Yap, Y. C.] CNRS IN2P3, Paris, France. [Akesson, T. P. A.; Aloisio, A.; Bocchetta, S. S.; Bryngemark, L.; Doglioni, C.; Floderus, A.; Hawkins, A. D.; Hedberg, V.; Ivarsson, J.; Jarlskog, G.; Lytken, E.; Mjornmark, J. U.; Smirnova, O.; Viazlo, O.] Lund Univ, Fys Inst, Lund, Sweden. [Barreiro, F.; Cantero, J.; De la Torre, H.; Del Peso, J.; Glasman, C.; Merino, J. Llorente; Terron, J.] Univ Autonoma Madrid, Dept Fis Teor C 15, Madrid, Spain. [Artz, S.; Becker, M.; Bertella, C.; Blum, W.; Buescher, V.; Caputo, R.; Caudron, J.; Cuth, J.; Endner, O. C.; Ertel, E.; Fiedler, F.; Torregrosa, E. Fullana; Groh, S.; Heck, T.; Hohlfeld, M.; Hulsing, T. A.; Jakobi, K. B.; Kaluza, A.; Karnevskiy, M.; Kleinknecht, K.; Koepke, L.; Lin, T. H.; Masetti, L.; Mattmann, J.; Meyer, C.; Moritz, S.; Moyse, E. J. W.; Pleskot, V.; Rave, S.; Sander, H. G.; Schaeffer, J.; Schafer, U.; Schmitt, C.; Schmitz, S.; Schott, M.; Schuh, N.; Simioni, E.; Simon, M.; Tapprogge, S.; Urrejola, P.; Webb, S.; Wollstadt, S. J.; Zimmermann, C.; Zinser, M.] Johannes Gutenberg Univ Mainz, Inst Phys, Mainz, Germany. [Barnes, S. L.; Bielski, R.; Cox, B. E.; Da Via, C.; Dann, N. S.; Forcolin, G. T.; Forti, A.; Ponce, J. M. Iturbe; Keoshkerian, H.; Li, X.; Loebinger, F. K.; Marsden, S. P.; Masik, J.; Sanchez, F. J. Munoz; Neep, T. J.; Oh, A.; Ospanov, R.; Pater, J. R.; Peters, R. F. Y.; Pilkington, A. D.; Pin, A. W. J.; Price, D.; Qin, Y.; Queitsch-Maitland, M.; Raine, J. A.; Schwanenberger, C.; Schweiger, H.; Shaw, S. M.; Thompson, R. J.; Tomlinson, L.; Watts, S.; Wilk, F.; Woudstra, M. J.; Wyatt, T. R.] Univ Manchester, Sch Phys & Astron, Manchester, Lancs, England. [Aad, G.; Aloisio, A.; Barbero, M.; Calandri, A.; Calvet, T. P.; Coadou, Y.; Diaconu, C.; Diglio, S.; Djama, F.; Ellajosyula, V.; Feligioni, L.; Gao, J.; Hadef, A.; Hallewell, G. D.; Hubaut, F.; Kahn, S. J.; Knoops, E. B. F. G.; Le Guirriec, E.; Liu, J.; Liu, K.; Madaffari, D.; Mochizuki, K.; Monnier, E.; Muanza, S.; Nagy, E.; Pralavorio, P.; Rodina, Y.; Rozanov, A.; Talby, M.; Theveneaux-Pelzer, T.; Torres, R. E. Ticse; Tisserant, S.; Toth, J.; Touchard, F.; Vacavant, L.; Wang, C.] Aix Marseille Univ, CPPM, Marseille, France. [Bellomo, M.; Bernard, N. R.; Brau, B.; Dallapiccola, C.; Daya-Ishmukhametova, R. K.; Pais, P.; Picazio, A.; Willocq, S.] Univ Massachusetts, Dept Phys, Amherst, MA 01003 USA. [Belanger-Champagne, C.; Chuinard, A. J.; Corriveau, F.; Keyes, R. A.; Mantifel, R.; Prince, S.; Robertson, S. H.; Robichaud-Veronneau, A.; Stockton, M. C.; Stoebe, M.; Vachon, B.; Schroeder, T. Vazquez; Wang, K.; Warburton, A.] McGill Univ, Dept Phys, Montreal, PQ, Canada. [Barberio, E. L.; Brennan, A. J.; Dawe, E.; Jennens, D.; Kubota, T.; Milesi, M.; Nuti, F.; Rados, P.; Scutti, F.; Spiller, L. A.; Tan, K. G.; Taylor, G. N.; Taylor, P. T. E.; Ungaro, F. C.; Urquijo, P.; Volpi, M.; Zanzi, D.] Univ Melbourne, Sch Phys, Melbourne, Vic, Australia. [Amidei, D.; Chelstowska, M. A.; Cheng, H. C.; Dai, T.; Diehl, E. B.; Edgar, R. C.; Feng, H.; Ferretti, C.; Fleischmann, P.; Goldfarb, S.; Guan, L.; Levin, D.; Liu, H.; Lu, N.; Marley, D. E.; Mc Kee, S. P.; McCarn, A.; Neal, H. A.; Qian, J.; Schwarz, T. A.; Searcy, J.; Sekhon, K.; Wu, Y.; Yu, J. M.; Zhang, D.; Zhou, B.; Zhu, J.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Abolins, M.; Arabidze, G.; Brock, R.; Chegwidden, A.; Fisher, W. C.; Halladjian, G.; Hauser, R.; Hayden, D.; Huston, J.; Martin, B.; Mondragon, M. C.; Pope, B. G.; Schoenrock, B. D.; Schwienhorst, R.; Willis, C.] Michigan State Univ, Dept Phys & Astron, E Lansing, MI 48824 USA. [Alimonti, G.; Andreazza, A.; Carminati, L.; Cavalli, D.; Costa, G.; Fanti, M.; Giugni, D.; Lari, T.; Lazzaroni, M.; Mandelli, L.; Manzoni, S.; Mazza, S. M.; Meroni, C.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Resconi, S.; Shojaii, S.; Stabilea, A.; Tartarelli, G. F.; Troncon, C.; Turra, R.; Perez, M. Villaplana] Ist Nazl Fis Nucl, Sez Milano, Milan, Italy. [Andreazza, A.; Carminati, L.; Fanti, M.; Lazzaroni, M.; Manzoni, S.; Mazza, S. M.; Monzani, S.; Perini, L.; Ragusa, F.; Ratti, M. G.; Shojaii, S.; Turra, R.; Perez, M. Villaplana] Univ Milan, Dipartimento Fis, Milan, Italy. [Harkusha, S.; Kulchitsky, Y.; Kurochkin, Y. A.; Tsiareshka, P. V.] Natl Acad Sci Belarus, BI Stepanov Inst Phys, Minsk, Byelarus. [Hrynevich, A.] Natl Sci & Educ Ctr Particle & High Energy Phys, Minsk, Byelarus. [Arguin, J. -F.; Azuelos, G.; Dallaire, F.; Gagnon, L. G.; Gauthier, L.; Leroy, C.; Rezvani, R.; Saadi, D. Shoaleh] Univ Montreal, Grp Particle Phys, Montreal, PQ, Canada. [Akimov, A. V.; Gavrilenko, I. L.; Komar, A. A.; Mashinistov, R.; Mouraviev, S. V.; Nechaeva, P. Yu.; Shmeleva, A.; Snesarev, A. A.; Sulin, V. V.; Tikhomirov, V. O.; Zhukov, K.] Russian Acad Sci, PN Lebedev Phys Inst, Moscow, Russia. [Artamonov, A.; Gorbounov, P. A.; Khovanskiy, V.; Shatalov, P. B.; Tsukerman, I. I.] Inst Theoret & Expt Phys ITEP, Moscow, Russia. [Aloisio, A.; Antonov, A.; Belotskiy, K.; Belyaev, N. L.; Bulekov, O.; Dolgoshein, B. A.; Kantserov, V. A.; Krasnopevtsev, D.; Romaniouk, A.; Shulga, E.; Smirnov, S. Yu.; Smirnov, Y.; Soldatov, E. Yu.; Timoshenko, S.; Vorobev, K.] Natl Res Nucl Univ MEPhI, Moscow, Russia. [Gladilin, L. K.; Kramarenko, V. A.; Maevskiy, A.; Rud, V. I.; Sivoklokov, S. Yu.; Smirnova, L. N.; Turchikhin, S.] Moscow MV Lomonosov State Univ, DV Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Adomeit, S.; Bender, M.; Biebel, O.; Bock, C.; Bortfeldt, J.; Calfayan, P.; Chow, B. K. B.; Duckeck, G.; Heinrich, J. J.; Hertenberger, R.; Hoenig, F.; Legger, F.; Lorenz, J.; Loesel, P. J.; Maier, T.; Mann, A.; Mehlhase, S.; Meineck, C.; Mitrevski, J.; Mueller, R. S. P.; Rauscher, F.; Ruschke, A.; Sanders, M. P.; Schaile, D.; Unverdorben, C.; Valderanis, C.; Walker, R.; Wittkowski, J.] Univ Munich, Fak Phys, Munich, Germany. [Barillari, T.; Bethke, S.; Compostella, G.; Cortiana, G.; Ecker, K. M.; Flowerdew, M. J.; Giuliani, C.; Goblirsch-Kolb, M.; Ince, T.; Kiryunin, A. E.; Kluth, S.; Kortner, O.; Kortner, S.; Kroha, H.; Macchiolo, A.; Maier, A. A.; Menke, S.; Mueller, F.; Nagel, M.; Nisius, R.; Nowak, S.; Oberlack, H.; Richter, R.; Salihagic, D.; Sandstroem, R.; Schacht, P.; Schwegler, Ph.; Spettel, F.; Stonjek, S.; Terzo, S.; von der Schmitt, H.; Wildauer, A.] Max Planck Inst Phys & Astrophys, Werner Heisenberg Inst, Munich, Germany. [Fusayasu, T.; Shimojima, M.] Nagasaki Inst Appl Sci, Nagasaki, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Grad Sch Sci, Nagoya, Aichi, Japan. [Horii, Y.; Kawade, K.; Onogi, K.; Tomoto, M.; Wakabayashi, J.; Yamauchi, K.] Nagoya Univ, Kobayashi Maskawa Inst, Nagoya, Aichi, Japan. [Aloisio, A.; Alonso, A.; Alviggi, M. G.; Canale, V.; Carlino, G.; Cirotto, F.; Conventi, F.; de Asmundis, R.; Della Pietra, M.; Doria, A.; Izzo, V.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Sekhniaidze, G.; Zurzolo, G.] Ist Nazl Fis Nucl, Sez Napoli, Naples, Italy. [Aloisio, A.; Alviggi, M. G.; Canale, V.; Cirotto, F.; Merola, L.; Perrella, S.; Rossi, E.; Sanchez, A.; Zurzolo, G.] Univ Naples Federico II, Dipartimento Fis, Naples, Italy. [Gorelov, I.; Hoeferkamp, M. R.; Mc Fadden, N. C.; Seidel, S. C.; Taylor, A. C.; Toms, K.] Univ New Mexico, Dept Phys & Astron, Albuquerque, NM 87131 USA. [Caron, S.; Colasurdo, L.; Croft, V.; De Groot, N.; Filthaut, F.; Galea, C.; Konig, A. C.; Nektarijevic, S.; Strubig, A.] Radboud Univ Nijmegen, Nikhef, Inst Math Astrophys & Particle Phys, Nijmegen, Netherlands. [Aben, R.; Angelozzi, I.; Bedognetti, M.; Beemster, L. J.; Bentvelsen, S.; Berge, D.; Bobbink, G. J.; Bos, K.; Brenner, L.; Butti, P.; Castelli, A.; Colijn, A. P.; de Jong, P.; Deigaard, I.; Deluca, C.; Duda, D.; Ferrari, P.; Hartjes, F.; Hessey, N. P.; Hod, N.; Igonkina, O.; Kluit, P.; Koffeman, E.; Mahlstedt, J.; Meyer, J.; Oussoren, K. P.; Sabato, G.; Salek, D.; Slawinska, M.; Valencic, N.; Van Den Wollenberg, W.; Van Der Deijl, P. C.; Van der Geer, R.; Van der Graaf, H.; van Vulpen, I.; Vankov, P.; Verkerke, W.; Vermeulen, J. C.; Vreeswijk, M.; Weits, H.; Williams, S.] Nikhef Natl Inst Subat Phys, Amsterdam, Netherlands. [Adelman, J.; Andari, N.; Burghgrave, B.; Chakraborty, D.; Cole, S.; Saha, P.] Univ Illinois, Dept Phys, De Kalb, IL USA. [Aloisio, A.; Anisenkov, A. V.; Baldin, E. M.; Bobrovnikov, V. S.; Bogdanchikov, A. G.; Buzykaev, A. R.; Kazanin, V. F.; Kharlamov, A. G.; Korol, A. A.; Malyshev, V. M.; Maslennikov, A. L.; Maximov, D. A.; Peleganchuk, S. V.; Rezanova, O. L.; Soukharev, A. M.; Talyshev, A. A.; Tikhonov, Yu. A.] SB RAS, Budker Inst Nucl Phys, Novosibirsk, Russia. [Becot, C.; Bernius, C.; Cranmer, K.; Haas, A.; Heinrich, L.; Kaplan, B.; Karthik, K.; Konoplich, R.; Mincer, A. I.; Nemethy, P.; Neves, R. M.] NYU, Dept Phys, 4 Washington Pl, New York, NY 10003 USA. [Beacham, J. B.; Che, S.; Gan, K. K.; Ishmukhametov, R.; Kagan, H.; Kass, R. D.; Looper, K. A.; Shrestha, S.; Tannenwald, B. B.] Ohio State Univ, Columbus, OH 43210 USA. [Nakano, I.] Okayama Univ, Fac Sci, Okayama, Japan. [Abbott, B.; Alhroob, M.; Bertsche, C.; Bertsche, D.; De Benedetti, A.; Gutierrez, P.; Hasib, A.; Norberg, S.; Pearson, B.; Rifki, O.; Severini, H.; Skubic, P.; Strauss, M.] Univ Oklahoma, Homer L Dodge Dept Phys & Astron, Norman, OK 73019 USA. [Haley, J.; Jamin, D. O.; Khanov, A.; Rizatdinova, F.; Sidorov, D.] Oklahoma State Univ, Dept Phys, Stillwater, OK 74078 USA. [Chytka, L.; Hamal, P.; Hrabovsky, M.; Kvita, J.; Nozka, L.] Palacky Univ, RCPTM, Olomouc, Czech Republic. [Abreu, R.; Allen, B. W.; Brau, J. E.; Brost, E.; Hopkins, W. H.; Majewski, S.; Potter, C. T.; Radloff, P.; Sinev, N. B.; Strom, D. M.; Torrence, E.; Wanotayaroj, C.; Whalen, K.; Winklmeier, F.] Univ Oregon, Ctr High Energy Phys, Eugene, OR 97403 USA. [Abeloos, B.; Ayoub, M. K.; Bassalat, A.; Binet, S.; Bourdarios, C.; De Regie, J. B. De Vivie; Delgove, D.; Duflot, L.; Escalier, M.; Fayard, L.; Fournier, D.; Gkougkousis, E. L.; Goudet, C. R.; Grivaz, J. -F.; Hariri, F.; Henrot-Versille, S.; Hrivnac, J.; Iconomidou-Fayard, L.; Kado, M.; Lounis, A.; Maiani, C.; Makovec, N.; Morange, N.; Nellist, C.; Petroff, P.; Poggioli, L.; Puzo, P.; Rousseau, D.; Rybkin, G.; Schaffer, A. C.; Serin, L.; Simion, S.; Tanaka, R.; Zerwas, D.; Zhang, Z.; Zhao, Y.] Univ Paris Saclay, Univ Paris Sud, CNRS IN2P3, LAL, Orsay, France. [Endo, M.; Nomachi, M.; Sugaya, Y.; Teoh, J. J.; Yamaguchi, Y.] Osaka Univ, Grad Sch Sci, Osaka, Japan. [Bugge, M. K.; Cameron, D.; Catmore, J. R.; Feigl, S.; Franconi, L.; Garonne, V.; Gjelsten, B. K.; Gramstad, E.; Morisbak, V.; Nilsen, J. K.; Ould-Saada, F.; Pajchel, K.; Pedersen, M.; Raddum, S.; Read, A. L.; Rohne, O.; Sandaker, H.; Serfon, C.; Stapnes, S.; Strandlie, A.] Univ Oslo, Dept Phys, Oslo, Norway. [Artoni, G.; Barr, A. J.; Becker, K.; Beresford, L.; Bortoletto, D.; Cooper-Sarkar, A. M.; Ortuzar, M. Crispin; Fawcett, W. J.; Frost, J. A.; Gallas, E. J.; Giuli, F.; Gupta, S.; Gwenlan, C.; Hall, D.; Hays, C. P.; Henderson, J.; Howard, J.; Huffman, T. B.; Issever, C.; Kalderon, C. W.; Kogan, L. A.; Nagai, K.; Nickerson, R. B.; Norjoharuddeen, N.; Petrov, M.; Pickering, M. A.; Tseng, J. C-L.; Viehhauser, G. H. A.; Vigani, L.; Weidberg, A. R.; Zhong, J.] Univ Oxford, Dept Phys, Oxford, England. [Conta, C.; Dondero, P.; Ferrari, R.; Fraternali, M.; Gaudio, G.; Introzzi, G.; Lanza, A.; Livan, M.; Negri, A.; Polesello, G.; Rebuzzi, D. M.; Rimoldi, A.; Vercesi, V.] Ist Nazl Fis Nucl, Sez Pavia, Pavia, Italy. [Conta, C.; Dondero, P.; Fraternali, M.; Introzzi, G.; Livan, M.; Negri, A.; Rebuzzi, D. M.; Rimoldi, A.] Univ Pavia, Dipartimento Fis, Pavia, Italy. [Balunas, W. K.; Brendlinger, K.; Di Clemente, W. K.; Fletcher, R. R. M.; Haney, B.; Heim, S.; Hines, E.; Jackson, B.; Kroll, J.; Lipeles, E.; Machado Miguens, J.; Meyer, C.; Mistry, K. P.; Reichert, J.; Stahlman, J.; Thomson, E.; Vanguri, R.; Williams, H. H.; Yoshihara, K.] Univ Penn, Dept Phys, Philadelphia, PA 19104 USA. [Basalaev, A.; Ezhilov; Fedin, O. L.; Gratchev, V.; Levchenko, M.; Maleev, V. P.; Naryshkin, I.; Ryabov, Y. F.; Schegelsky, V. A.; Seliverstov, D. 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N.; Galhardo, B.; Gomes, A.; Goncalo, R.; Jorge, P. M.; Lopes, L.; Maio, A.; Maneira, J.; Oleiro Seabra, L. F.; Onofre, A.; Palma, A.; Pedro, R.; Pina, J.; Santos, H.; Saraiva, J. G.; Silva, J.; Delgado, A. Tavares; Veloso, F.; Wolters, H.] LIP, Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Amorim, A.; Conde Muino, P.; Da Cunha Sargedas De Sousa, M. J.; Gomes, A.; Jorge, P. M.; Machado Miguens, J.; Maio, A.; Maneira, J.; Palma, A.; Pedro, R.; Pina, J.; Delgado, A. Tavares] Univ Lisbon, Fac Ciencias, Lisbon, Portugal. [Carvalho, J.; Fiolhais, M. C. N.; Galhardo, B.; Veloso, F.; Wolters, H.] Univ Coimbra, Dept Phys, Coimbra, Portugal. [Gomes, A.; Maio, A.; Pina, J.; Saraiva, J. G.; Silva, J.] Univ Lisbon, Ctr Fis Nucl, Lisbon, Portugal. [Amor Dos Santos, S. P.; Onofre, A.] Univ Minho, Dept Fis, Braga, Portugal. [Aguilar-Saavedraa, J. A.] Univ Granada, Dept Fis Teor & Cosmos, Granada, Spain. [Aguilar-Saavedraa, J. A.] Univ Granada, CAFPE, Granada, Spain. Univ Nova Lisboa, Dep Fis, Caparica, Portugal. Univ Nova Lisboa, CEFITEC, Fac Ciencias & Tecnol, Caparica, Portugal. [Chudoba, J.; Havranek, M.; Hejbal, J.; Jakoubek, T.; Kepka, O.; Kupco, A.; Kus, V.; Lokajicek, M.; Lysak, R.; Marcisovsky, M.; Mikestikova, M.; Nemecek, S.; Penc, O.; Sicho, P.; Staroba, P.; Svatos, M.; Tasevsky, M.; Vrba, V.] Acad Sci Czech Republic, Inst Phys, Prague, Czech Republic. [Augsten, K.; Caforio, D.; Gallus, P.; Guenther, J.; Hubacek, Z.; Myska, M.; Pospisil, S.; Seifert, F.; Simak, V.; Slavicek, T.; Smolek, K.; Solar, M.; Sopczak, A.; Sopko, V.; Suk, M.; Turecek, D.; Vacek, V.; Vlasak, M.; Vokac, P.; Vykydal, Z.; Zeman, M.] Czech Tech Univ, Prague, Czech Republic. [Balek, P.; Berta, P.; Chalupkova, I.; Davidek, T.; Dolejsi, J.; Dolezal, Z.; Faltova, J.; Kodys, P.; Kosek, T.; Leitner, R.; Reznicek, P.; Scheirich, D.; Slovak, R.; Spousta, M.; Sykora, T.; Tas, P.; Todorova-Nova, S.; Valkar, S.; Vorobel, V.] Charles Univ Prague, Fac Math & Phys, Prague, Czech Republic. [Aloisio, A.; Borisov, A.; Cheremushkina, E.; Denisov, S. P.; Fakhrutdinov, R. M.; Fenyuk, A. B.; Golubkov, D.; Kamenshchikov, A.; Karyukhin, A. N.; Kozhin, A. S.; Minaenko, A. A.; Myagkov, A. G.; Nikolaenko, V.; Ryzhov, A.; Solodkov, A. A.; Solovyanov, O. V.; Starchenko, E. A.; Zaitsev, A. M.; Zenin, O.] NRC KI, State Res Ctr, Inst High Energy Phys Protvino, Protvino, Russia. [Adye, T.; Baines, J. T.; Barnett, B. M.; Burke, S.; Dewhurst, A.; Dopke, J.; Emeliyanov, D.; Gallop, B. J.; Gee, C. N. P.; Haywood, S. J.; Kirk, J.; Martin-Haugh, S.; McMahon, S. J.; Middleton, R. P.; Murray, W. J.; Phillips, P. W.; Sankey, D. P. C.; Sawyer, C.; Tyndel, M.; Wickens, F. 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[Aielli, G.; Camarri, P.; Cardarelli, R.; Di Ciaccio, A.; Iuppa, R.; Liberti, B.; Salamon, A.; Santonico, R.] Ist Nazl Fis Nucl, Sez Roma Tor Vergata, Rome, Italy. [Aielli, G.; Camarri, P.; Di Ciaccio, A.; Iuppa, R.; Salamon, A.; Santonico, R.] Univ Roma Tor Vergata, Dipartimento Fis, Rome, Italy. [Baroncelli, A.; Biglietti, M.; Ceradini, F.; Di Micco, B.; Farilla, A.; Graziania, E.; Iodice, M.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Stanescu, C.; Taccini, C.] Ist Nazl Fis Nucl, Sez Roma Tre, Rome, Italy. [Ceradini, F.; Di Micco, B.; Orestano, D.; Pastore, F.; Petrucci, F.; Puddu, D.; Salamanna, G.; Sessa, M.; Taccini, C.] Univ Rome Tre, Dipartimento Matemat & Fis, Rome, Italy. [Benchekroun, D.; Chafaq, A.; Hoummada, A.] Univ Hassan 2, Reseau Univ Phys Hautes Energies, Fac Sci Ain Chock, Casablanca, Morocco. [Ghazlane, H.] Ctr Natl Energie Sci Tech Nucl, Rabat, Morocco. Univ Cadi Ayyad, LPHEA Marrakech, Fac Sci Semlalia, Marrakech, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] Univ Mohamed Premier, Fac Sci, Oujda, Morocco. [Derkaoui, J. E.; Ouchrif, M.; Tayalati, Y.] LPTPM, Oujda, Morocco. [El Moursli, R. Cherkaoui; El Kacimi, M.; Fassie, F.; Goujdami, D.; Haddad, N.; Idrissi, Z.] Univ Mohammed 5, Fac Sci, Rabat, Morocco. [Bachacou, H.; Balli, F.; Bauer, F.; Blanchard, J. -B.; Boonekamp, M.; Chevalier, L.; Hoffmann, M. Dano; Deliot, F.; Denysiuk, D.; Etienvre, A. I.; Formica, A.; Da Costa, J. Goncalves Pinto Firmino; Guyot, C.; Jeanneau, F.; Lancon, E.; Laporte, J. F.; Le Quilleuc, E. P.; Lesage, A. A. J.; Mansoulie, B.; Meyer, J-P.; Ouraou, A.; Perego, M. M.; Peyaud, A.; Royon, C. R.; Saimpert, M.; Schoeffel, L.; Schwindling, J.] CEA Saclay Commissariat Energie Atom & Energies A, DSM IRFU Inst Rech Lois Fondamentales Univers, Gif Sur Yvette, France. [AbouZeid, O. S.; Battaglia, M.; Debenedetti, C.; Grillo, A. A.; Hance, M.; Kuhl, A.; Law, A. T.; Liang, Z.; Litke, A. M.; Lockman, W. S.; Nielsen, J.; Reece, R.; Rose, P.; Sadrozinski, H. F-W.; Schumm, B. A.; Seiden, A.] Univ Calif Santa Cruz, Santa Cruz Inst Particle Phys, Santa Cruz, CA 95064 USA. [Alpigiani, C.; Blackburn, D.; Goussiou, A. G.; Hsu, S. -C.; Johnson, W. J.; Lubatti, H. J.; Marx, M.; Meehan, S.; Rompotis, N.; Rosten, R.; Rothberg, J.; Russell, H. L.; De Bruin, P. H. Sales; Pastor, E. Torro; Watts, G.; Whallon, N. L.] Univ Washington, Dept Phys, Seattle, WA 98195 USA. [Anastopoulos, C.; Costanzo, D.; Donszelmann, T. Cuhadar; Dawson, I.; Fletcher, G. T.; Hamity, G. N.; Hodgkinson, M. C.; Hodgson, P.; Johansson, P.; Klinger, J. A.; Korolkova, E. V.; Kyriazopoulos, D.; Paredes, B. Lopez; Macdonald, C. M.; Miyagawa, P. S.; Parker, K. A.; Tovey, D. R.; Vickey, T.; Boeriu, O. E. Vickey] Univ Sheffield, Dept Phys & Astron, Sheffield, S Yorkshire, England. [Hasegawa, Y.; Takeshita, T.] Shinshu Univ, Dept Phys, Nagano, Japan. [Atlay, N. B.; Buchholz, P.; Czirr, H.; Fleck, I.; Gaur, B.; Ghasemi, S.; Ibragimov, I.; Li, Y.; Rosenthal, O.; Walkowiak, W.; Ziolkowski, M.] Univ Siegen, Fachbereich Phys, Siegen, Germany. [Buat, Q.; Horton, A. J.; Mori, D.; O'Neil, D. C.; Pachal, K.; Stelzer, B.; Temple, D.; Torres, H.; Van Nieuwkoop, J.; Vetterli, M. C.] Simon Fraser Univ, Dept Phys, Burnaby, BC, Canada. [Barklow, T.; Bartoldus, R.; Bawa, H. S.; Black, J. E.; Gao, Y. S.; Garelli, N.; Grenier, P.; Ilic, N.; Kagan, M.; Kocian, M.; Koi, T.; Malone, C.; Moss, J.; Mount, R.; Nachman, B. P.; Nef, P. D.; Piacquadio, G.; Rubbo, F.; Salnikov, A.; Schwartzman, A.; Su, D.; Tompkins, L.; Wittgen, M.; Young, C.; Zeng, Q.] SLAC Natl Accelerator Lab, Stanford, CA USA. [Astalos, R.; Bartos, P.; Blazek, T.; Plazak, L.; Sykora, I.; Tokar, S.; Zenis, T.] Comenius Univ, Fac Math Phys & Informat, Bratislava, Slovakia. [Antos, J.; Bruncko, D.; Kladiva, E.; Strizenec, P.; Urban, J.] Slovak Acad Sci, Inst Expt Phys, Dept Subnucl Phys, Kosice, Slovakia. [Castaneda-Miranda, E.; Hamilton, A.; Yacoob, S.] Univ Cape Town, Dept Phys, Cape Town, South Africa. [Connell, S. H.; Govender, N.] Univ Johannesburg, Dept Phys, Johannesburg, South Africa. [Hsu, C.; Kar, D.; Garcia, B. R. Mellado; Ruan, X.] Univ Witwatersrand, Sch Phys, Johannesburg, South Africa. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. Bessidskaia; Bohm, C.; Clement, C.; Cribbs, W. A.; Hellman, S.; Jon-And, K.; Khandanyan, H.; Klimek, P.; Lundberg, O.; Milstead, D. A.; Moa, T.; Molander, S.; Pani, P.; Plucinski, P.; Poettgen, R.; Rossetti, V.; Shaikh, N. W.; Shcherbakova, A.; Silverstein, S. B.; Sjolin, J.; Strandberg, S.; Ughetto, M.; Santurio, E. Valdes; Wallangen, V.] Stockholm Univ, Dept Phys, Stockholm, Sweden. [Abulaiti, Y.; Akerstedt, H.; Asman, B.; Bendtz, K.; Bertoli, G.; Bylund, O. 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[Asai, S.; Chen, S.; Dohmae, T.; Enari, Y.; Hanawa, K.; Kanaya, N.; Kataoka, Y.; Kato, C.; Kawamoto, T.; Kazama, S.; Kobayashi, A.; Kobayashi, T.; Komori, Y.; Mashimo, T.; Masubuchi, T.; Minami, Y.; Mori, T.; Morinaga, M.; Nakamura, T.; Ninomiya, Y.; Nobe, T.; Saito, T.; Sakamoto, H.; Sasaki, Y.; Tanaka, J.; Terashi, K.; Ueda, I.; Yamamoto, S.; Yamanaka, T.] Univ Tokyo, Dept Phys, Tokyo, Japan. [Bratzler, U.; Fukunaga, C.] Tokyo Metropolitan Univ, Grad Sch Sci & Technol, Tokyo, Japan. [Hirose, M.; Ishitsuka, M.; Jinnouchi, O.; Kobayashi, D.; Kuze, M.; Motohashi, K.; Pettersson, N. E.; Todome, K.; Yamaguchi, D.] Tokyo Inst Technol, Dept Phys, Tokyo, Japan. [Batista, S. J.; Chau, C. C.; DeMarco, D. A.; Di Sipio, R.; Diamond, M.; Krieger, P.; Liblong, A.; Mc Goldrick, G.; Orr, R. S.; Pascuzzi, V.; Polifka, R.; Rudolph, M. S.; Savard, P.; Sinervo, P.; Taenzer, J.; Teuscher, R. J.; Trischuk, W.; Veloce, L. M.; Venturi, N.] Univ Toronto, Dept Phys, Toronto, ON, Canada. [Canepa, A.; Chekulaev, S. V.; Jovicevic, J.; Koutsman, A.; Oram, C. J.; Codina, E. Perez; Schneider, B.; Seuster, R.; Stelzer-Chilton, O.; Tafirout, R.; Trigger, I. M.] TRIUMF, Vancouver, BC, Canada. [Garcia, J. A. Benitez; Ramos, J. Manjarres; Palacino, G.; Taylor, W.] York Univ, Dept Phys & Astron, Toronto, ON, Canada. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Fac Pure & Appl Sci, Tsukuba, Ibaraki, Japan. [Hara, K.; Ito, F.; Kasahara, K.; Kim, S. H.; Kiuchi, K.; Nagata, K.; Okawa, H.; Sato, K.; Ukegawa, F.] Univ Tsukuba, Ctr Integrated Res Fundamental Sci & Engn, Tsukuba, Ibaraki, Japan. [Beauchemin, P. H.; Meoni, E.; Sliwa, K.; Son, H.; Wetter, J.] Tufts Univ, Dept Phys & Astron, Medford, MA 02155 USA. [Casper, D. W.; Corso-Radu, A.; Frate, M.; Gerbaudo, D.; Guest, D.; Lankford, A. J.; Mete, A. S.; Nelson, A.; Scannicchio, D. A.; Schernau, M.; Shimmin, C. 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EM atlas.publications@cern.ch RI Villa, Mauro/C-9883-2009; Coccaro, Andrea/P-5261-2016; Brooks, William/C-8636-2013; Staroba, Pavel/G-8850-2014; Lazzaroni, Massimo/N-3675-2015; Kukla, Romain/P-9760-2016; Goncalo, Ricardo/M-3153-2016; Gavrilenko, Igor/M-8260-2015; Owen, Mark/Q-8268-2016; Di Domenico, Antonio/G-6301-2011; Doyle, Anthony/C-5889-2009; Shulga, Evgeny/R-1759-2016; Maleev, Victor/R-4140-2016; Carvalho, Joao/M-4060-2013; Boyko, Igor/J-3659-2013; Prokoshin, Fedor/E-2795-2012; Conde Muino, Patricia/F-7696-2011; Gladilin, Leonid/B-5226-2011; Grinstein, Sebastian/N-3988-2014; Zhukov, Konstantin/M-6027-2015; Livan, Michele/D-7531-2012; Tikhomirov, Vladimir/M-6194-2015; Ventura, Andrea/A-9544-2015; Warburton, Andreas/N-8028-2013; Mitsou, Vasiliki/D-1967-2009; Camarri, Paolo/M-7979-2015; Mindur, Bartosz/A-2253-2017; Mashinistov, Ruslan/M-8356-2015; Gutierrez, Phillip/C-1161-2011; Fabbri, Laura/H-3442-2012; Kantserov, Vadim/M-9761-2015; Chekulaev, Sergey/O-1145-2015; Snesarev, Andrey/H-5090-2013; Solodkov, Alexander/B-8623-2017; Zaitsev, Alexandre/B-8989-2017; Carli, Ina/C-2189-2017; Guo, Jun/O-5202-2015; Peleganchuk, Sergey/J-6722-2014; Yang, Haijun/O-1055-2015; Li, Liang/O-1107-2015; Monzani, Simone/D-6328-2017; Kuday, Sinan/C-8528-2014; Garcia, Jose /H-6339-2015 OI Villa, Mauro/0000-0002-9181-8048; Coccaro, Andrea/0000-0003-2368-4559; Brooks, William/0000-0001-6161-3570; Lazzaroni, Massimo/0000-0002-4094-1273; Kukla, Romain/0000-0002-1140-2465; Goncalo, Ricardo/0000-0002-3826-3442; Owen, Mark/0000-0001-6820-0488; Di Domenico, Antonio/0000-0001-8078-2759; Doyle, Anthony/0000-0001-6322-6195; Shulga, Evgeny/0000-0001-5099-7644; Carvalho, Joao/0000-0002-3015-7821; Boyko, Igor/0000-0002-3355-4662; Prokoshin, Fedor/0000-0001-6389-5399; Conde Muino, Patricia/0000-0002-9187-7478; Gladilin, Leonid/0000-0001-9422-8636; Grinstein, Sebastian/0000-0002-6460-8694; Livan, Michele/0000-0002-5877-0062; Tikhomirov, Vladimir/0000-0002-9634-0581; Ventura, Andrea/0000-0002-3368-3413; Warburton, Andreas/0000-0002-2298-7315; Mitsou, Vasiliki/0000-0002-1533-8886; Camarri, Paolo/0000-0002-5732-5645; Mindur, Bartosz/0000-0002-5511-2611; Mashinistov, Ruslan/0000-0001-7925-4676; Fabbri, Laura/0000-0002-4002-8353; Kantserov, Vadim/0000-0001-8255-416X; Solodkov, Alexander/0000-0002-2737-8674; Zaitsev, Alexandre/0000-0002-4961-8368; Carli, Ina/0000-0002-0411-1141; Guo, Jun/0000-0001-8125-9433; Peleganchuk, Sergey/0000-0003-0907-7592; Li, Liang/0000-0001-6411-6107; Monzani, Simone/0000-0002-0479-2207; Kuday, Sinan/0000-0002-0116-5494; FU ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW, Austria; FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq, Brazil; FAPESP, Brazil; NSERC, Canada; NRC, Canada; CFI, Canada; CERN; CONICYT, Chile; CAS, China; MOST, China; NSFC, China; COLCIENCIAS, Colombia; MSMT CR, Czech Republic; MPO CR, Czech Republic; VSC CR, Czech Republic; DNRF, Denmark; DNSRC, Denmark; IN2P3-CNRS, France; CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, Germany; HGF, Germany; MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, Israel; I-CORE, Israel; Benoziyo Center, Israel; INFN, Italy; MEXT, Japan; JSPS, Japan; CNRST, Morocco; FOM, Netherlands; NWO, Netherlands; RCN, Norway; MNiSW, Poland; NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia; NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS, Slovenia; MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC, Sweden; Wallenberg Foundation, Sweden; SERI, Switzerland; SNSF, Switzerland; Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE, United States of America; NSF, United States of America; BCKDF; Canada Council; CANARIE; CRC; Compute Canada; FQRNT; Ontario Innovation Trust, Canada; EPLANET; ERC; FP7; Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex; ANR; Region Auvergne; Fondation Partager le Savoir, France; DFG, Germany; AvH Foundation, Germany; EU-ESF; Greek NSRF; BSF; GIF; Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; Royal Society, United Kingdom; Leverhulme Trust, United Kingdom FX We thank CERN for the very successful operation of the LHC, as well as the support staff from our institutions without whom ATLAS could not be operated efficiently. We acknowledge the support of ANPCyT, Argentina; YerPhI, Armenia; ARC, Australia; BMWFW and FWF, Austria; ANAS, Azerbaijan; SSTC, Belarus; CNPq and FAPESP, Brazil; NSERC, NRC and CFI, Canada; CERN; CONICYT, Chile; CAS, MOST and NSFC, China; COLCIENCIAS, Colombia; MSMT CR, MPO CR and VSC CR, Czech Republic; DNRF and DNSRC, Denmark; IN2P3-CNRS, CEA-DSM/IRFU, France; GNSF, Georgia; BMBF, HGF, and MPG, Germany; GSRT, Greece; RGC, Hong Kong SAR, China; ISF, I-CORE and Benoziyo Center, Israel; INFN, Italy; MEXT and JSPS, Japan; CNRST, Morocco; FOM and NWO, Netherlands; RCN, Norway; MNiSW and NCN, Poland; FCT, Portugal; MNE/IFA, Romania; MES of Russia and NRC KI, Russian Federation; JINR; MESTD, Serbia; MSSR, Slovakia; ARRS and MIZS, Slovenia; DST/NRF, South Africa; MINECO, Spain; SRC and Wallenberg Foundation, Sweden; SERI, SNSF and Cantons of Bern and Geneva, Switzerland; MOST, Taiwan; TAEK, Turkey; STFC, United Kingdom; DOE and NSF, United States of America. In addition, individual groups and members have received support from BCKDF, the Canada Council, CANARIE, CRC, Compute Canada, FQRNT, and the Ontario Innovation Trust, Canada; EPLANET, ERC, FP7, Horizon 2020 and Marie Sklodowska-Curie Actions, European Union; Investissements d'Avenir Labex and Idex, ANR, Region Auvergne and Fondation Partager le Savoir, France; DFG and AvH Foundation, Germany; Herakleitos, Thales and Aristeia programmes co-financed by EU-ESF and the Greek NSRF; BSF, GIF and Minerva, Israel; BRF, Norway; Generalitat de Catalunya, Generalitat Valenciana, Spain; the Royal Society and Leverhulme Trust, United Kingdom. The crucial computing support from all WLCG partners is acknowledged gratefully, in particular from CERN and the ATLAS Tier-1 facilities at TRIUMF (Canada), NDGF (Denmark, Norway, Sweden), CC-IN2P3 (France), KIT/GridKA (Germany), INFN-CNAF (Italy), NL-T1 (Netherlands), PIC (Spain), ASGC (Taiwan), RAL (UK) and BNL (USA) and in the Tier-2 facilities worldwide. NR 55 TC 1 Z9 1 U1 21 U2 32 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 6 PY 2016 VL 76 IS 7 AR 375 DI 10.1140/epjc/s10052-016-4176-8 PG 40 WC Physics, Particles & Fields SC Physics GA DQ6XW UT WOS:000379351100001 ER PT J AU Tesfaye, AT Mashtalir, O Naguib, M Barsoum, MW Gogotsi, Y Djenizian, T AF Tesfaye, Alexander T. Mashtalir, Olha Naguib, Michael Barsoum, Michel W. Gogotsi, Yury Djenizian, Thierry TI Anodized Ti3SiC2 As an Anode Material for Li-ion Microbatteries SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE porous anodized Ti3SiC2; MAX phases; anodization; Li-ion microbatteries; anode ID LITHIUM STORAGE PROPERTIES; ORGANIZED TIO2 NANOTUBES; MICRO-BATTERY ANODES; ENERGY-STORAGE; MXENE NANOSHEETS; METAL-OXIDES; MAX PHASES; PERFORMANCE; CARBIDE; EXTRACTION AB We report on the synthesis of an anode material for Li-ion batteries by anodization of a common MAX phase, Ti3SiC2, in an aqueous electrolyte containing hydrofluoric acid (HF). The anodization led to the formation of a porous film containing anatase, a small quantity of free carbon, and silica. By varying the anodization parameters, various oxide morphologies were produced. The highest areal capacity was achieved by anodization at 60 V in an aqueous electrolyte containing 0.1 v/v HF for 3 h at room temperature. After 140 cycles performed at multiple applied current densities, an areal capacity of 380 mu Ah.cm(-2) (200 mu A.cm(-2)) has been obtained, making this new material, free of additives and binders, a promising candidate as a negative electrode for Li-ion microbatteries. C1 [Tesfaye, Alexander T.; Djenizian, Thierry] Aix Marseille Univ, CNRS, MADIREL Lab, UMR 7246, F-13397 Marseille, France. [Tesfaye, Alexander T.; Djenizian, Thierry] ALISTORE ERI European Res Inst, ER CNRS 3104, F-80039 Amiens, France. [Naguib, Michael; Barsoum, Michel W.; Gogotsi, Yury] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Mashtalir, Olha; Naguib, Michael; Barsoum, Michel W.; Gogotsi, Yury] Drexel Univ, AJ Drexel Nanomat Inst, Philadelphia, PA 19104 USA. [Djenizian, Thierry] Ecole Natl Super Mines, Flexible Elect Dept, CMP, F-13541 Gardanne, France. [Mashtalir, Olha] CUNY City Coll, Dept Chem, New York, NY 10031 USA. [Naguib, Michael] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37381 USA. RP Djenizian, T (reprint author), Aix Marseille Univ, CNRS, MADIREL Lab, UMR 7246, F-13397 Marseille, France.; Djenizian, T (reprint author), ALISTORE ERI European Res Inst, ER CNRS 3104, F-80039 Amiens, France.; Gogotsi, Y (reprint author), Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA.; Gogotsi, Y (reprint author), Drexel Univ, AJ Drexel Nanomat Inst, Philadelphia, PA 19104 USA.; Djenizian, T (reprint author), Ecole Natl Super Mines, Flexible Elect Dept, CMP, F-13541 Gardanne, France. EM gogotsi@drexel.edu; thierry.djenizian@univ-amu.fr OI Naguib, Michael/0000-0002-4952-9023 FU ALISTORE-ERI; Master for Energy Storage and Conversion (MESC) Erasmus Mundus Programme FX We thank ALISTORE-ERI for financial support. T.D. and Y.G. are grateful to the Master for Energy Storage and Conversion (MESC) Erasmus Mundus Programme for financial support. We thank Dr. Nareerat Plylahan, Dr. Taron Makaryan, Maissa Barr, and Carine Chassigneux for the XRD measurements and the Centralized Research Facility of Drexel University for providing access to XPS. NR 46 TC 1 Z9 1 U1 38 U2 86 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUL 6 PY 2016 VL 8 IS 26 BP 16670 EP 16676 DI 10.1021/acsami.6b03528 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DQ8JD UT WOS:000379456000017 PM 27282275 ER PT J AU Dogan, F Vaughey, JT Iddir, H Key, B AF Dogan, Fulya Vaughey, John T. Iddir, Hakim Key, Baris TI Direct Observation of Lattice Aluminum Environments in Li Ion Cathodes LiNi1-y-zCoyAlzO2 and Al-Doped LiNixMnyCozO2 via Al-27 MAS NMR Spectroscopy SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE NCA; NMC; lattice Al; Al segregation; transition-metal migration; Al-27 MAS NMR; DFT ID LOCAL ENVIRONMENTS; BATTERIES; CO; SUBSTITUTION; PERFORMANCE; STABILITY; OXIDE AB Direct observations of local lattice aluminum environments have been a major challenge for aluminum -bearing Li ion battery materials, such as LiNi1-y-zCoyAlzO2 Al(NCA) and aluminum-doped LiNixMnyCozO2 (NMC). Al-27 magic angle spinning (MAS) nuclear magnetic resonance (NMR) spectroscopy is the only structural probe currently available that can qualitatively and quantitatively characterize lattice and nonlattice (i.e., surface, coatings, segregation, secondary phase etc.) aluminum coordination and provide information that helps discern its effect in the lattice. In the present study, we use NMR to gain new insights into transition metal (TM)-O-Al coordination and evolution of lattice aluminum sites upon cycling. With the aid of first-principles DFT calculations, we show direct evidence of lattice Al sites, nonpreferential Ni/Co-O-Al ordering in NCA, and the lack of bulk lattice aluminum in aluminum -"doped" NMC. Aluminum coordination of the paramagnetic (lattice) and diamagnetic (nonlattice) nature is investigated for Al-doped NMC and NCA. For the latter, the evolution of the lattice site(s) upon cycling is also studied. A clear reordering of lattice aluminum environments due to nickel migration is observed in NCA upon extended cycling. C1 [Dogan, Fulya; Vaughey, John T.; Key, Baris] Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Iddir, Hakim] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Dogan, F (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. EM fdogan@anl.gov FU Vehicle Technologies Program; Hybrid and Electric Systems; U.S. Department of Energy Office of Science laboratory [DE-AC02-06CH11357] FX Support from the Vehicle Technologies Program, Hybrid and Electric Systems, in particular, David Howell, Tien Duong, and Peter Faguy, at the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, is gratefully acknowledged. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a U.S. Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. Dr. Daniel Abraham is acknowledged for valuable discussions and Dr. Eungje Lee is acknowledged for experimental support. Computer time allocations at the Fusion Computer Facility, Argonne National Laboratory, and at EMSL Pacific Northwest National Laboratory are gratefully acknowledged. NR 27 TC 4 Z9 4 U1 14 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUL 6 PY 2016 VL 8 IS 26 BP 16708 EP 16717 DI 10.1021/acsami.6b04516 PG 10 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DQ8JD UT WOS:000379456000022 PM 27299505 ER PT J AU Feng, XY Zou, HL Xiang, HF Guo, X Zhou, TP Wu, YC Xu, W Yan, PF Wang, CM Zhang, JG Yu, Y AF Feng, Xuyong Zou, Hailin Xiang, Hongfa Guo, Xin Zhou, Tianpei Wu, Yucheng Xu, Wu Yan, Pengfei Wang, Chongmin Zhang, Ji-Guang Yu, Yan TI Ultrathin Li4Ti5O12 Nanosheets as Anode Materials for Lithium and Sodium Storage SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE lithium titanate; nanosheets; polyether-assisted; hydrothermal process; lithium storage; sodium storage ID SOLID-STATE SYNTHESIS; LI-ION BATTERIES; ENERGY-STORAGE; ELECTROCHEMICAL PERFORMANCE; HOLLOW MICROSPHERES; ELECTRODE; COMPOSITES; MECHANISM; NANOFIBERS; GRAPHENE AB Ultrathin Li4Ti5O12 (LTO) nanosheets with ordered microstructures were prepared via a polyether-assisted hydrothermal process. Pluronic P123, a polyether, can impede the growth of Li2TiO3 in the precursor and also act as a structure directing agent to facilitate the (Li1.81H0.19)Ti2O5-2H(2)O precursor to form the LTO nanosheets with the ordered microstructure. Moreover, the addition of P123 can suppress the stacking of LTO nanosheets during calcining of the precursor, and the thickness of the nanosheets can be controlled to be about 4 nm. The microstructure of the as-prepared ultrathin and ordered nano sheets is helpful for Li+ or Na+ diffusion and charge transfer through the particles. Therefore, the ultrathin P123-assisted LTO (P-LTO) nanosheets show a rate capability much higher than that of the LTO sample without P123 in a Li battery with over 130 mAh g(-1) of capacity remaining at the 64C rate. For intercalation of larger size Na+ ions, the P-LTO still exhibits a capacity of 115 mAh g(-1) at a current rate of 10 C and a capacity retention of 96% after 400 cycles. C1 [Feng, Xuyong; Zou, Hailin; Xiang, Hongfa; Zhou, Tianpei; Wu, Yucheng] Hefei Univ Technol, Sch Mat Sci & Engn, Hefei 230009, Anhui, Peoples R China. [Xu, Wu; Zhang, Ji-Guang] Pacific NW Natl Lab, Energy & Environm Directorate, Richland, WA 99354 USA. [Wang, Chongmin] Pacific NW Natl Lab, Environm & Mol Sci Lab, Richland, WA 99354 USA. [Yu, Yan] Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, Hefei 230026, Anhui, Peoples R China. RP Xiang, HF; Wu, YC (reprint author), Hefei Univ Technol, Sch Mat Sci & Engn, Hefei 230009, Anhui, Peoples R China.; Yu, Y (reprint author), Univ Sci & Technol China, Dept Mat Sci & Engn, CAS Key Lab Mat Energy Convers, Hefei 230026, Anhui, Peoples R China. EM hfxiang@hfut.edu.cn; ycwu@hfut.edu.cn; yanyumse@ustc.edu.cn RI feng, xuyong/K-8843-2012; yan, pengfei/E-4784-2016; Xiang, Hongfa/I-5126-2012 OI yan, pengfei/0000-0001-6387-7502; Xiang, Hongfa/0000-0002-6182-1932 FU National Science Foundation of China [51372060, 51402289, 21373195]; Recruitment Program of Global Experts; program for New Century Excellent Talents in University [NCET-12-0515]; Fundamental Research Funds for the Central Universities [WK3430000004]; Collaborative Innovation Center of Suzhou Nano Science and Technology; China Postdoctoral Science Foundation [2015M580531]; Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies; Advanced Battery Materials Research (BMR) programs of the U.S. Department of Energy (DOE) [DE-AC02-05CH11231]; DOE's Office of Biological and Environmental Research at the Pacific Northwest National Laboratory (PNNL); DOE [DE-AC05-76RL01830] FX This study was supported by National Science Foundation of China (Grants 51372060, 51402289, and 21373195), the Recruitment Program of Global Experts, the program for New Century Excellent Talents in University (Grant NCET-12-0515), the Fundamental Research Funds for the Central Universities (Grant WK3430000004), and the Collaborative Innovation Center of Suzhou Nano Science and Technology. X.F. acknowledges the China Postdoctoral Science Foundation (Grant 2015M580531). The high-resolution TEM and SAED analyses were supported by the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, the Advanced Battery Materials Research (BMR) programs of the U.S. Department of Energy (DOE) under Contract DE-AC02-05CH11231 and were conducted in the William R. Wiley Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by the DOE's Office of Biological and Environmental Research located at the Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for the DOE under Contract DE-AC05-76RL01830. NR 44 TC 4 Z9 4 U1 31 U2 67 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUL 6 PY 2016 VL 8 IS 26 BP 16718 EP 16726 DI 10.1021/acsami.6b04752 PG 9 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DQ8JD UT WOS:000379456000023 PM 27294363 ER PT J AU Zhang, WR Li, MT Chen, AP Li, LG Zhu, YY Xia, ZH Lu, P Boullay, P Wu, LJ Zhu, YM MacManus-Driscoll, JL Jia, QX Zhou, HH Narayan, J Zhang, XH Wang, HY AF Zhang, Wenrui Li, Mingtao Chen, Aiping Li, Leigang Zhu, Yuanyuan Xia, Zhenhai Lu, Ping Boullay, Philippe Wu, Lijun Zhu, Yimei MacManus-Driscoll, Judith L. Jia, Quanxi Zhou, Honghui Narayan, Jagdish Zhang, Xinghang Wang, Haiyan TI Two-Dimensional Layered Oxide Structures Tailored by Self Assembled Layer Stacking via Interfacial Strain SO ACS APPLIED MATERIALS & INTERFACES LA English DT Article DE self-assembly; layered oxides; strain engineering multiferroic; interface ID NANOCOMPOSITE THIN-FILMS; SUPERCELL STRUCTURE; GRAPHENE; SUPERCONDUCTIVITY; HETEROSTRUCTURES; DEVICES AB Study of layered complex oxides emerge as one of leading topics in fundamental materials science because of the strong interplay among intrinsic charge, spin, orbital, and lattice. As a fundamental basis of heteroepitaxial thin film growth, interfacial strain can be used to design materials that exhibit new phenomena beyond their conventional forms. Here, we report a strain-driven self-assembly of bismuth-based supercell (SC) with a two-dimensional (2D) layered structure. With combined experimental analysis and first-principles calculations, we investigated the full SC structure and elucidated the fundamental growth mechanism achieved by the strain-enabled self-assembled atomic layer stacking. The unique SC structure exhibits room-temperature ferroelectricity, enhanced magnetic responses, and a distinct optical bandgap from the conventional double perovskite structure. This study reveals the important role of interfacial strain modulation and atomic rearrangement in self-assembling a layered singe-phase multiferroic thin film, which opens up a promising avenue in the search for and design of novel 2D layered complex oxides with enormous promise. C1 [Zhang, Wenrui; Li, Leigang; Zhu, Yuanyuan; Wang, Haiyan] Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA. [Li, Mingtao; Xia, Zhenhai] Univ North Texas, Dept Mat Sci & Engn, Denton, TX 76203 USA. [Li, Mingtao; Xia, Zhenhai] Univ North Texas, Dept Chem, Denton, TX 76203 USA. [Li, Mingtao] Xi An Jiao Tong Univ, State Key Lab Multiphase Flow Power Engn, Int Res Ctr Renewable Energy, Xian 710049, Shaanxi, Peoples R China. [Chen, Aiping; Wang, Haiyan] Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. [Chen, Aiping; Jia, Quanxi] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, MS K771, Los Alamos, NM 87545 USA. [Lu, Ping] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Boullay, Philippe] Normandie Univ, ENSICAEN, UNICAEN, CNRS,CRISMAT, 6 Blvd Marechal Juin, F-14050 Caen 4, France. [Wu, Lijun; Zhu, Yimei] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. [MacManus-Driscoll, Judith L.] Univ Cambridge, Dept Mat Sci, 27 Charles Babbage Rd, Cambridge, England. [Zhou, Honghui; Narayan, Jagdish] North Carolina State Univ, Dept Mat Sci & Engn, NSF Ctr Adv Mat & Smart Struct, Raleigh, NC 27695 USA. [Zhang, Xinghang] Texas A&M Univ, Dept Mech Engn, College Stn, TX 77843 USA. RP Wang, HY (reprint author), Texas A&M Univ, Dept Mat Sci & Engn, College Stn, TX 77843 USA.; Wang, HY (reprint author), Texas A&M Univ, Dept Elect & Comp Engn, College Stn, TX 77843 USA. EM hwang00@tamu.edu RI Zhang, Wenrui/D-1892-2015; Chen, Aiping/F-3212-2011 OI Zhang, Wenrui/0000-0002-0223-1924; Chen, Aiping/0000-0003-2639-2797 FU Office of Naval Research (ONR) [N00014-15-1-2362, N00014-16-1-2465]; U.S. National Science Foundation (NSF, Ceramic Program) [DMR-0846504]; NSF [DMR-1401266, DMR-1643911]; AFOSR MURI [FA9550-12-1-0037]; United States Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000]; United States Department of Energy, Office of Basic Energy Science, Division of Materials Science and Engineering [DE-SC0012704]; EPSRC [EP/N004272/1]; Office of Science, Office of Basic Energy Sciences of the United States Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Office of Naval Research (ONR, N00014-15-1-2362 at Texas A&M University and N00014-16-1-2465 at Purdue University, for thin film growth) and the U.S. National Science Foundation (NSF, Ceramic Program, Grant DMR-0846504, for high resolution STEM analysis). W.Z. and H.W. acknowledge support from the NSF (Grant DMR-1401266 at Texas A&M University and DMR-1643911 at Purdue University). M.L. and Z.X. acknowledge partial support from AFOSR MURI (Grant FA9550-12-1-0037). Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the United States Department of Energy's National Nuclear Security Administration under Contract DE-AC04-94AL85000. The high-resolution STEM work at Brookhaven National Laboratory was supported by the United States Department of Energy, Office of Basic Energy Science, Division of Materials Science and Engineering, under Contract No. DE-SC0012704. J.L.M.-D. acknowledges EPSRC grant EP/N004272/1. A portion of the electron microscopy experiments was performed at National Center for Electron Microscopy (NCEM), which is supported by the Office of Science, Office of Basic Energy Sciences of the United States Department of Energy under Contract DE-AC02-05CH11231. W.Z. is grateful to Drs. Peter Ercius, Jim Ciston, and Chengyu Song for additional help and fruitful discussions at NCEM. W.Z. thanks Qjyuan Wu for helpful discussion on the XPS analysis. NR 39 TC 1 Z9 1 U1 24 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1944-8244 J9 ACS APPL MATER INTER JI ACS Appl. Mater. Interfaces PD JUL 6 PY 2016 VL 8 IS 26 BP 16845 EP 16851 DI 10.1021/acsami.6b03773 PG 7 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Science & Technology - Other Topics; Materials Science GA DQ8JD UT WOS:000379456000038 PM 27295399 ER PT J AU Baek, DL Fox, RV Case, ME Sinclair, LK Schmidt, AB McIlwain, PR Mincher, BJ Wai, CM AF Baek, Donna L. Fox, Robert V. Case, Mary E. Sinclair, Laura K. Schmidt, Alex B. McIlwain, Patrick R. Mincher, Bruce J. Wai, Chien M. TI Extraction of Rare Earth Oxides Using Supercritical Carbon Dioxide Modified with Tri-n-Butyl Phosphate-Nitric Acid Adducts SO INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH LA English DT Article ID NITRATE COMPLEXATION; SOLVENT-EXTRACTION; FLUORESCENT LAMPS; TBP-HNO3 COMPLEX; LANTHANIDES; RECOVERY; NEODYMIUM; ELEMENTS; URANIUM; IONS AB A new tri-n-butylphosphate nitric acid (TBP-HNO3) adduct was prepared by combining TBP and fuming (90%) HNO3. The adduct was characterized, and its phase-equilibrium behavior in supercritical carbon dioxide is reported. Supercritical carbon dioxide (sc-CO2) was modified with this new adduct [TBP(HNO3)(5.2)(H2O)(1.7)], and the extraction efficacies of selected rare earth oxides (Y, Ce, Eu, Tb, and Dy) at 338 K and 34.5 MPa were compared with those obtained using an adduct formed from concentrated (70%) HNO3 and TBP [TBP(HNO3)(1.7)(H2O)(0.6)]. All rare earth oxides tested with both adduct species could be extracted with the exception of cerium oxide. The water and acid concentrations in the different adducts were found to play a significant role in rare earth oxide extraction efficiency. C1 [Baek, Donna L.; Fox, Robert V.; Case, Mary E.; Mincher, Bruce J.] Idaho Natl Lab, Idaho Falls, ID 83415 USA. [Case, Mary E.; Wai, Chien M.] Univ Idaho, Moscow, ID 83843 USA. [Sinclair, Laura K.] Cornell Univ, Ithaca, NY 14853 USA. [Schmidt, Alex B.] Boise State Univ, Boise, ID 83725 USA. [McIlwain, Patrick R.] Montana State Univ, Bozeman, MT 59717 USA. RP Baek, DL (reprint author), Idaho Natl Lab, Idaho Falls, ID 83415 USA. EM donna.baek@inl.gov RI Mincher, Bruce/C-7758-2017 FU Critical Materials Institute, an Energy Innovation Hub - U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office; Department of Energy Idaho Operations Office [DE-AC07-05ID14517] FX This research was supported by the Critical Materials Institute, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office. Work was completed at Idaho National Laboratory under Department of Energy Idaho Operations Office Contract DE-AC07-05ID14517. NR 28 TC 2 Z9 2 U1 10 U2 15 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0888-5885 J9 IND ENG CHEM RES JI Ind. Eng. Chem. Res. PD JUL 6 PY 2016 VL 55 IS 26 BP 7154 EP 7163 DI 10.1021/acs.iecr.6b00554 PG 10 WC Engineering, Chemical SC Engineering GA DQ8IY UT WOS:000379455400011 ER PT J AU Pattengale, B Yang, SZ Ludwig, J Huang, ZQ Zhang, XY Huang, J AF Pattengale, Brian Yang, Sizhuo Ludwig, John Huang, Zhuangqun Zhang, Xiaoyi Huang, Jier TI Exceptionally Long-Lived Charge Separated State in Zeolitic Imidazolate Framework: Implication for Photocatalytic Applications SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID METAL-ORGANIC FRAMEWORK; RAY-ABSORPTION SPECTROSCOPY; ADSORPTION; DYNAMICS; CATALYSTS; CRYSTALS; CAPTURE; CO2 AB Zeolitic imidazolate frameworks (ZIFs) have emerged as a novel class of porous metal organic frameworks (MOFs) for catalysis application because of their exceptional thermal and chemical stability. Inspired by the broad absorption of ZIF-67 in UV-vis-near IR region, we explored its excited state and charge separation dynamics, properties essential for photocatalytic applications, using optical (OTA) and X-ray transient absorption (XTA) spectroscopy. OTA results show that an exceptionally long-lived excited state is formed after photo excitation. This long-lived excited state was confirmed to be the charge-separated (CS) state with ligand-to-metal charge-transfer character using XTA. The surprisingly long-lived CS state, together with its intrinsic hybrid nature, all point to its potential application in heterogeneous photocatalysis and energy conversion. C1 [Pattengale, Brian; Yang, Sizhuo; Ludwig, John; Huang, Zhuangqun; Huang, Jier] Marquette Univ, Dept Chem, Milwaukee, WI 53201 USA. [Zhang, Xiaoyi] Argonne Natl Lab, Xray Sci Div, Argonne, IL 60349 USA. RP Huang, J (reprint author), Marquette Univ, Dept Chem, Milwaukee, WI 53201 USA. EM jier.huang@marquette.edu FU Marquette University; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX This work was supported by Marquette University New Faculty Startup Fund and Regular Research Grant. Use of the Advanced Photon Source and nanosecond and femtosecond-NIR transient absorption spectroscopy at the Center for Nanoscale Materials in Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under award no. DE-AC02-06CH11357. Z.H. acknowledges help with AFM measurements from the Molecular Materials Research Center of the Beckman Institute, California Institute of Technology. NR 41 TC 6 Z9 6 U1 61 U2 124 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 6 PY 2016 VL 138 IS 26 BP 8072 EP 8075 DI 10.1021/jacs.6b04615 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA DQ8JA UT WOS:000379455600008 PM 27322216 ER PT J AU Cao, Z Kim, D Hong, DC Yu, Y Xu, J Lin, S Wen, XD Nichols, EM Jeong, K Reimer, JA Yang, PD Chang, CJ AF Cao, Zhi Kim, Dohyung Hong, Dachao Yu, Yi Xu, Jun Lin, Song Wen, Xiaodong Nichols, Eva M. Jeong, Keunhong Reimer, Jeffrey A. Yang, Peidong Chang, Christopher J. TI A Molecular Surface Functionalization Approach to Tuning Nanoparticle Electrocatalysts for Carbon Dioxide Reduction SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID N-HETEROCYCLIC CARBENE; METAL-ORGANIC FRAMEWORKS; SINGLE-CRYSTAL FACES; ELECTROCHEMICAL REDUCTION; AU NANOPARTICLES; GOLD CATALYSIS; CO2 REDUCTION; UNDERPOTENTIAL DEPOSITION; CHEMICAL PRODUCTION; ELECTROREDUCTION AB Conversion of the greenhouse gas carbon dioxide (CO2) to value-added products is an important challenge for sustainable energy research, and nanomaterials offer a broad class of heterogeneous catalysts for such transformations. Here we report a molecular surface functionalization approach to tuning gold nanoparticle (Au NP) electrocatalysts for reduction of CO2 to CO. The N-heterocyclic (NHC) carbene-functionalized Au NP catalyst exhibits improved faradaic efficiency (FE = 83%) for reduction of CO2 to CO in water at neutral pH at an overpotential of 0.46 V with a 7.6-fold increase in current density compared to that of the parent Au NP (FE = 53%). Tafel plots of the NHC carbene-functionalized Au NP (72 mV/decade) vs parent Au NP (138 mV/decade) systems further show that the molecular ligand influences mechanistic pathways for CO2 reduction. The results establish molecular surface functionalization as a complementary approach to size, shape, composition, and defect control for nanoparticle catalyst design. C1 [Cao, Zhi; Hong, Dachao; Yu, Yi; Xu, Jun; Lin, Song; Nichols, Eva M.; Jeong, Keunhong; Reimer, Jeffrey A.; Yang, Peidong; Chang, Christopher J.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Kim, Dohyung; Yang, Peidong] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Chang, Christopher J.] Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA. [Chang, Christopher J.] Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA. [Lin, Song; Nichols, Eva M.; Chang, Christopher J.] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. [Yu, Yi; Yang, Peidong] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Wen, Xiaodong] Chinese Acad Sci, Inst Coal Chem, Taiyuan 030001, Shanxi, Peoples R China. [Wen, Xiaodong] Synfuels China, Beijing 100195, Peoples R China. [Yang, Peidong] Kavli Energy Nanosci Inst, Berkeley, CA 94720 USA. RP Yang, PD; Chang, CJ (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Yang, PD (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Chang, CJ (reprint author), Univ Calif Berkeley, Dept Mol & Cell Biol, 229 Stanley Hall, Berkeley, CA 94720 USA.; Chang, CJ (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Berkeley, CA 94720 USA.; Chang, CJ (reprint author), Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA.; Yang, PD (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Yang, PD (reprint author), Kavli Energy Nanosci Inst, Berkeley, CA 94720 USA. EM p_yang@berkeley.edu; chrischang@berkeley.edu RI Cao, Zhi/E-2174-2013; Lin, Song/F-5472-2014; OI Cao, Zhi/0000-0002-1050-2165; Lin, Song/0000-0002-8880-6476; Hong, Dachao/0000-0003-0581-1315; Xu, Jun/0000-0003-3507-0159 FU U.S. Department of Energy/Lawrence Berkeley National Laboratory [101528-002]; Office of Science, Office of Basic Energy Sciences, Materials Science and Engineering Division, U.S. Department of Energy [DE-AC02-05CH11231]; Samsung; National Science Foundation FX Financial support for synthesis, calculations, and some electrochemical measurements was provided by U.S. Department of Energy/Lawrence Berkeley National Laboratory Grant 101528-002 (C.J.C.). Financial support for nanocrystal catalysis in P.Y.'s laboratory work was supported by the Director, Office of Science, Office of Basic Energy Sciences, Materials Science and Engineering Division, U.S. Department of Energy under contract no. DE-AC02-05CH11231(Surface). C.J.C. and P.Y. are CIFAR Senior Fellows. C.J.C. is an Investigator with the Howard Hughes Medical Institute. D.K. acknowledges support from a Samsung Scholarship, and E.M.N. thanks the National Science Foundation for a Graduate Fellowship. We also thank Dr. Bo He and Dr. Xu Deng of LBNL for TEM image assistance. NR 55 TC 14 Z9 14 U1 104 U2 234 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 6 PY 2016 VL 138 IS 26 BP 8120 EP 8125 DI 10.1021/jacs.6b02878 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA DQ8JA UT WOS:000379455600017 PM 27322487 ER PT J AU Wei, H Luo, JW Li, SS Wang, LW AF Wei, Hai Luo, Jun-Wei Li, Shu-Shen Wang, Lin-Wang TI Revealing the Origin of Fast Electron Transfer in TiO2-Based Dye Sensitized Solar Cells SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID AMPHIPHILIC RUTHENIUM SENSITIZER; ENERGY-CONVERSION EFFICIENCY; NANOCRYSTALLINE TIO2 FILMS; ANATASE TIO2; PORPHYRIN SENSITIZERS; INJECTION DYNAMICS; CHARGE-TRANSFER; FORMIC-ACID; ZNO; ADSORPTION AB In dye-sensitized solar cells (DSCs), the electron transfer from photoexcited dye molecules to semiconductor substrates remains a major bottleneck. Replacing TiO2 with ZnO is expected to enhance the efficiency of DSCs, owing to the latter possesses a much larger electron mobility, but similar bandgap and band positions as TiO2 remain. However, the record efficiency of ZnO-based DSCs is only 7% compared with 13% of TiO2-based DSCs due to the even slower electron-transfer rate in ZnO-based DSCs, which becomes a long-standing puzzle. Here, we computationally investigate the electron transfer from the dye molecule into ZnO and TiO2, respectively, by performing the first-principles calculations within the frame of the Marcus theory. The predicted electron-transfer rate in the TiO2-based DSC is about 1.15 X 10(9) s(-1), a factor of 15 faster than that of the ZnO-based DSC, which is in good agreement with experimental data. We find that the much larger density of states of the TiO2 compared with ZnO near the conduction band edge is the dominant factor, which is responsible for the faster electron-transfer rate in TiO2-based DSCs. These denser states provide additional efficient channels for the electron transfer. We also provide design principles to boost the efficiency of DSCs through surface engineering of high mobility photoanode semiconductors. C1 [Wei, Hai; Luo, Jun-Wei; Li, Shu-Shen] Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, POB 912, Beijing 100083, Peoples R China. [Wei, Hai; Luo, Jun-Wei; Li, Shu-Shen] Univ Chinese Acad Sci, Beijing 100049, Peoples R China. [Wei, Hai; Luo, Jun-Wei; Li, Shu-Shen] Univ Sci & Technol China, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China. [Wang, Lin-Wang] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Luo, JW (reprint author), Chinese Acad Sci, Inst Semicond, State Key Lab Superlattices & Microstruct, POB 912, Beijing 100083, Peoples R China.; Luo, JW (reprint author), Univ Chinese Acad Sci, Beijing 100049, Peoples R China.; Luo, JW (reprint author), Univ Sci & Technol China, Synerget Innovat Ctr Quantum Informat & Quantum P, Hefei 230026, Anhui, Peoples R China.; Wang, LW (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM jwluo@semi.ac.cn; lwwang@lbl.gov FU National Young 1000 Talents Plan; National Science Foundation of China (NSFC) [61474116, 11374293]; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division through the Material Theory program in Lawrence Berkeley National Laboratory [DE-AC02-05CH11231, KC2301] FX This work was supported by the National Young 1000 Talents Plan and the National Science Foundation of China (NSFC grant nos. 61474116 and 11374293) (H.W. and J.W.L.) and the U.S. Department of Energy, Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract No. DE-AC02-05CH11231, through the Material Theory program [KC2301] in Lawrence Berkeley National Laboratory (L.W.W.). NR 61 TC 3 Z9 3 U1 19 U2 58 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 6 PY 2016 VL 138 IS 26 BP 8165 EP 8174 DI 10.1021/jacs.6b03524 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA DQ8JA UT WOS:000379455600022 PM 27282781 ER PT J AU Eren, B Weatherup, RS Liakakos, N Somorjai, GA Salmeron, M AF Eren, Baran Weatherup, Robert S. Liakakos, Nikos Somorjai, Gabor A. Salmeron, Miguel TI Dissociative Carbon Dioxide Adsorption and Morphological Changes on Cu(100) and Cu(111) at Ambient Pressures SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID RAY PHOTOELECTRON-SPECTROSCOPY; SCANNING-TUNNELING-MICROSCOPY; METHANOL SYNTHESIS; SURFACE-CHEMISTRY; COPPER SURFACES; LOW-TEMPERATURE; CO GAS; CATALYSTS; OXYGEN; CU AB Ambient-pressure X-ray photoelectron spectroscopy (APXPS) and high-pressure scanning tunneling microscopy (HPSTM) were used to study the structure and chemistry of model Cu(100) and Cu(111) catalyst surfaces in the adsorption and dissociation of CO2. It was found that the (100) face is more active in dissociating CO2 than the (111) face. Atomic oxygen formed after the dissociation of CO2 poisons the surface by blocking further adsorption of CO2. This "self-poisoning" mechanism explains the need to mix CO into the industrial feed for methanol production from CO2, as it scavenges the chemisorbed O. The HPSTM images show that the (100) surface breaks up into nanoclusters in the presence of CO2 at 20 Torr and above, producing active kink and step sites. If the surface is precovered with atomic oxygen, no such nanoclustering occurs. C1 [Eren, Baran; Weatherup, Robert S.; Somorjai, Gabor A.; Salmeron, Miguel] Lawrence Berkeley Natl Lab, Mat Sci Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Liakakos, Nikos] Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Somorjai, Gabor A.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Salmeron, Miguel] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. RP Salmeron, M (reprint author), Lawrence Berkeley Natl Lab, Mat Sci Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Salmeron, M (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM mbsalmeron@lbl.gov RI Eren, Baran/A-9644-2013; Weatherup, Robert/O-5725-2016 OI Weatherup, Robert/0000-0002-3993-9045 FU Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, U.S. Department of Energy (DOE) through the Chemical and Mechanical Properties of Surfaces, Interfaces and Nanostructures Program [DE-AC02-05CH11231, FWP: KC3101]; St. John's College, Cambridge; European Union [656870] FX This work was supported by the Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering, U.S. Department of Energy (DOE), under Contract DE-AC02-05CH11231 through the Chemical and Mechanical Properties of Surfaces, Interfaces and Nanostructures Program (FWP: KC3101). It used resources of the Advance Light Source, which is supported by the DOE Office of Science. R.S.W. acknowledges a Research Fellowship from St. John's College, Cambridge, and a Marie Sklodowska-Curie Individual Fellowship (Global) under Grant ARTIST (656870) from the European Union's Horizon 2020 Research and Innovation Programme. We thank Dr. Hendrik Bluhm and Dr. Ethan Crumlin for assistance with the experiments at the Advanced Light Source. NR 46 TC 0 Z9 0 U1 28 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 6 PY 2016 VL 138 IS 26 BP 8207 EP 8211 DI 10.1021/jacs.6b04039 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA DQ8JA UT WOS:000379455600026 PM 27280375 ER PT J AU Posada-Perez, S Ramirez, PJ Evans, J Vines, F Liu, P Illas, F Rodriguez, JA AF Posada-Perez, Sergio Ramirez, Pedro J. Evans, Jaime Vines, Francesc Liu, Ping Illas, Francesc Rodriguez, Jose A. TI Highly Active Au/delta-MoC and Cu/delta-MoC Catalysts for the Conversion of CO2: The Metal/C Ratio as a Key Factor Defining Activity, Selectivity, and Stability SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID GAS-SHIFT REACTION; AU-C INTERACTIONS; METHANOL SYNTHESIS; CARBON-DIOXIDE; CHARGE POLARIZATION; MOLYBDENUM CARBIDE; TUNGSTEN CARBIDE; HYDROGENATION; SURFACES; MECHANISM AB The ever growing increase of CO2 concentration in the atmosphere is one of the main causes of global warming. Thus, CO2 activation and conversion toward valuable added compounds is a major scientific challenge. A new set of Au/delta-MoC and Cu/delta-MoC catalysts exhibits high activity, selectivity, and stability for the reduction of CO2 to CO with some subsequent selective hydrogenation toward methanol. Sophisticated experiments under controlled conditions and calculations based on density functional theory have been used to study the unique behavior of these systems. A detailed comparison of the behavior of Au/beta-Mo2C and Au/delta-MoC catalysts provides evidence of the impact of the metal/carbon ratio in the carbide on the performance of the catalysts. The present results show that this ratio governs the chemical behavior of the carbide and the properties of the admetal, up to the point of being able to switch the rate and mechanism of the process for CO2 conversion. A control of the metal/carbon ratio paves the road for an efficient reutilization of this environmental harmful greenhouse gas. C1 [Posada-Perez, Sergio; Vines, Francesc; Illas, Francesc] Univ Barcelona, Dept Quim Fis, C Marti & Franques 1, E-08028 Barcelona, Spain. [Posada-Perez, Sergio; Vines, Francesc; Illas, Francesc] Univ Barcelona, Inst Quim Teor & Computac IQTCUB, C Marti & Franques 1, E-08028 Barcelona, Spain. [Ramirez, Pedro J.; Evans, Jaime] Cent Univ Venezuela, Fac Ciencias, Caracas 1020A, Venezuela. [Liu, Ping; Rodriguez, Jose A.] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Illas, F (reprint author), Univ Barcelona, Dept Quim Fis, C Marti & Franques 1, E-08028 Barcelona, Spain.; Illas, F (reprint author), Univ Barcelona, Inst Quim Teor & Computac IQTCUB, C Marti & Franques 1, E-08028 Barcelona, Spain.; Rodriguez, JA (reprint author), Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. EM francesc.illas@ub.edu; rodrigez@bnl.gov RI Illas, Francesc /C-8578-2011 OI Illas, Francesc /0000-0003-2104-6123 FU U.S. Department of Energy [DE-SC0012704]; Spanish MINECO/FEDER grant [CTQ2015-64618-R]; Generalitat de Catalunya [2014SGR97]; NOMAD Center of Excellence project; European Union [676580]; Spanish MEC [CTQ2012-30751]; MINECO [RYC-2012-10129]; ICREA Academia Award for Excellence in University Research; Red Espanola de Supercomputacion (RES) FX This manuscript has been authored by employees of Brookhaven Science Associates, LLC under Contract No. DE-SC0012704 with the U.S. Department of Energy. The research carried out at the Universitat de Barcelona was supported by the Spanish MINECO/FEDER grant CTQ2015-64618-R and, in part, by Generalitat de Catalunya (grants 2014SGR97 and XRQTC) and from the NOMAD Center of Excellence project; the latter project has received funding from the European Union's Horizon 2020 research and innovation programme under grant agreement no. 676580. S.P.P. acknowledges financial support from Spanish MEC predoctoral grant associated with CTQ2012-30751. F.V. thanks the MINECO for a postdoctoral Ramon y Cajal (RyC) research contract (RYC-2012-10129), and F.I. acknowledges additional support from the 2015 ICREA Academia Award for Excellence in University Research. Computational time at the MARENOSTRUM supercomputer has been provided by the Barcelona Super computing Centre (BSC) through a grant from Red Espanola de Supercomputacion (RES). NR 62 TC 6 Z9 6 U1 90 U2 159 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 6 PY 2016 VL 138 IS 26 BP 8269 EP 8278 DI 10.1021/jacs.6b04529 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA DQ8JA UT WOS:000379455600034 PM 27308923 ER PT J AU Wiedner, ES Bullock, RM AF Wiedner, Eric S. Bullock, R. Morris TI Electrochemical Detection of Transient Cobalt Hydride Intermediates of Electrocatalytic Hydrogen Production SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY LA English DT Article ID DIIMINE-DIOXIME COMPLEXES; TRANSITION-METAL HYDRIDES; 2ND COORDINATION SPHERE; AB-INITIO CALCULATIONS; PENDANT AMINES; ELECTRODE-POTENTIALS; MOLECULAR CATALYSIS; CHARGE SEPARATION; FUNCTIONAL MODELS; AQUEOUS-SOLUTION AB A large variety of molecular cobalt complexes are used as electrocatalysts for H-2 production, but the key cobalt hydride intermediates are frequently difficult to detect and characterize due to their high reactivity. We report that a combination of variable scan rate cyclic voltammetry and foot-of-the-wave analysis (FOWA) can be used to detect transient (CoH)-H-III and (CoH)-H-II intermediates of electrocatalytic H-2 production by [Co-II(PtBu2NPH2)(CH3CN)(3)](2+) and CoII(dmgBF(2))(2)(CH3CN)(2). In both cases, reduction of a transient catalytic intermediate occurs at a potential that coincides with the Co-II/I couple. Each reduction displays quasireversible electron-transfer kinetics, consistent with reduction of a CoIIIH intermediate to CoIIH, which is then protonated by acid to generate H-2. A bridge-protonated Co-I species was ruled out as a catalytic intermediate for Co-II(dmgBF(2))(2)(CH3CN)(2) from voltammograms recorded at 1000 psi of H-2. Density functional theory was used to calculate Co-III-H and Co-II-H bond strengths for both catalysts. Despite having very different ligands, the cobalt hydrides of both catalysts possess nearly identical heterolytic and homolytic Co-H bond strengths for the (CoH)-H-III and (CoH)-H-II intermediates. C1 [Wiedner, Eric S.; Bullock, R. Morris] Pacific Northwest Natl Lab, Ctr Mol Electrocatalysis, POB 999,K2-57, Richland, WA 99352 USA. RP Wiedner, ES (reprint author), Pacific Northwest Natl Lab, Ctr Mol Electrocatalysis, POB 999,K2-57, Richland, WA 99352 USA. EM eric.wiedner@pnnl.gov RI Bullock, R. Morris/L-6802-2016; OI Bullock, R. Morris/0000-0001-6306-4851; Wiedner, Eric/0000-0002-7202-9676 FU Center for Molecular Electrocatalysis, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences FX We thank Dr. Monte Helm and Dr. Aaron Appel for helpful discussions. This research was supported as part of the Center for Molecular Electrocatalysis, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. Computational resources were provided at the National Energy Research Scientific Computing Center (NERSC) at Lawrence Berkeley National Laboratory. Pacific Northwest National Laboratory is operated by Battelle for the U.S. Department of Energy. NR 87 TC 8 Z9 8 U1 28 U2 46 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0002-7863 J9 J AM CHEM SOC JI J. Am. Chem. Soc. PD JUL 6 PY 2016 VL 138 IS 26 BP 8309 EP 8318 DI 10.1021/jacs.6b04779 PG 10 WC Chemistry, Multidisciplinary SC Chemistry GA DQ8JA UT WOS:000379455600038 PM 27300721 ER PT J AU Li, GT Chern, M Jain, R Martin, JA Schackwitz, WS Jiang, LR Vega-Sanchez, ME Lipzen, AM Barry, KW Schmutz, J Ronald, PC AF Li, Guotian Chern, Mawsheng Jain, Rashmi Martin, Joel A. Schackwitz, Wendy S. Jiang, Liangrong Vega-Sanchez, Miguel E. Lipzen, Anna M. Barry, Kerrie W. Schmutz, Jeremy Ronald, Pamela C. TI Genome-Wide Sequencing of 41 Rice (Oryza sativa L.) Mutated Lines Reveals Diverse Mutations Induced by Fast-Neutron Irradiation SO MOLECULAR PLANT LA English DT Letter ID INSERTIONAL MUTAGENESIS; ARABIDOPSIS-THALIANA; GENES C1 [Li, Guotian; Chern, Mawsheng; Jain, Rashmi; Jiang, Liangrong; Ronald, Pamela C.] Univ Calif Davis, Dept Plant Pathol, Davis, CA 95616 USA. [Li, Guotian; Chern, Mawsheng; Jain, Rashmi; Jiang, Liangrong; Ronald, Pamela C.] Univ Calif Davis, Genome Ctr, Davis, CA 95616 USA. [Li, Guotian; Chern, Mawsheng; Jain, Rashmi; Vega-Sanchez, Miguel E.; Ronald, Pamela C.] Lawrence Berkeley Natl Lab, Feedstocks Div, Joint BioEnergy Inst, Berkeley, CA 94720 USA. [Martin, Joel A.; Schackwitz, Wendy S.; Lipzen, Anna M.; Barry, Kerrie W.; Schmutz, Jeremy] US DOE, Joint Genome Inst, Walnut Creek, CA 94598 USA. [Jiang, Liangrong] Xiamen Univ, Sch Life Sci, Xiamen 361102, Peoples R China. [Schmutz, Jeremy] HudsonAlpha Inst Biotechnol, Huntsville, AL 35806 USA. [Vega-Sanchez, Miguel E.] Monsanto Co, Chesterfield Village Campus, Chesterfield, MO 63017 USA. RP Ronald, PC (reprint author), Univ Calif Davis, Dept Plant Pathol, Davis, CA 95616 USA.; Ronald, PC (reprint author), Univ Calif Davis, Genome Ctr, Davis, CA 95616 USA.; Ronald, PC (reprint author), Lawrence Berkeley Natl Lab, Feedstocks Div, Joint BioEnergy Inst, Berkeley, CA 94720 USA. EM pcronald@ucdavis.edu RI Schmutz, Jeremy/N-3173-2013 OI Schmutz, Jeremy/0000-0001-8062-9172 NR 12 TC 3 Z9 3 U1 8 U2 10 PU CELL PRESS PI CAMBRIDGE PA 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA SN 1674-2052 EI 1752-9867 J9 MOL PLANT JI Mol. Plant. PD JUL 6 PY 2016 VL 9 IS 7 BP 1078 EP 1081 DI 10.1016/j.molp.2016.03.009 PG 4 WC Biochemistry & Molecular Biology; Plant Sciences SC Biochemistry & Molecular Biology; Plant Sciences GA DR1HE UT WOS:000379655800012 PM 27018389 ER PT J AU Clancy, JP Gretarsson, H Lee, EKH Tian, D Kim, J Upton, MH Casa, D Gog, T Islam, Z Jeon, BG Kim, KH Desgreniers, S Kim, YB Julian, SJ Kim, YJ AF Clancy, J. P. Gretarsson, H. Lee, E. K. H. Tian, Di Kim, J. Upton, M. H. Casa, D. Gog, T. Islam, Z. Jeon, Byung-Gu Kim, Kee Hoon Desgreniers, S. Kim, Yong Baek Julian, S. J. Kim, Young-June TI X-ray scattering study of pyrochlore iridates: Crystal structure, electronic, and magnetic excitations SO PHYSICAL REVIEW B LA English DT Article ID DIAMOND-ANVIL CELLS; SILICONE FLUID; R2IR2O7 R; IMAGE; EU AB We have investigated the structural, electronic, and magnetic properties of the pyrochlore iridates Eu2Ir2O7 and Pr2Ir2O7 using a combination of resonant elastic x-ray scattering, x-ray powder diffraction, and resonant inelastic x-ray scattering (RIXS). The structural parameters of Eu2Ir2O7 have been examined as a function of temperature and applied pressure, with a particular emphasis on regions of the phase diagram where electronic and magnetic phase transitions have been reported. We find no evidence of crystal symmetry change over the range of temperatures (similar to 6 to 300 K) and pressures (similar to 0.1 to 17 GPa) studied. We have also investigated the electronic and magnetic excitations in single-crystal samples of Eu2Ir2O7 and Pr2Ir2O7 using high-resolution Ir L-3-edge RIXS. In spite of very different ground state properties, we find that these materials exhibit qualitatively similar excitation spectra, with crystal field excitations at similar to 3-5 eV, spin-orbit excitations at similar to 0.5-1 eV, and broad low-lying excitations below similar to 0.15 eV. In single-crystal samples of "Eu-rich" Eu2Ir2O7 (found to possess an actual stoichiometry of Eu2.18Ir1.82O7.06) we observe highly damped magnetic excitations at similar to 45 meV, which display significant momentum dependence. We compare these results with recent dynamical structure factor calculations. C1 [Clancy, J. P.; Gretarsson, H.; Lee, E. K. H.; Tian, Di; Kim, Yong Baek; Julian, S. J.; Kim, Young-June] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. [Kim, J.; Upton, M. H.; Casa, D.; Gog, T.; Islam, Z.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Jeon, Byung-Gu; Kim, Kee Hoon] Seoul Natl Univ, Dept Phys & Astron, CeNSCMR, Seoul 151747, South Korea. [Desgreniers, S.] Univ Ottawa, Dept Phys, Lab Phys Solides Denses, Ottawa, ON K1N 6N5, Canada. RP Clancy, JP (reprint author), Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada. FU Natural Sciences and Engineering Research Council of Canada through a Discovery Grant and Research Tools and Instruments Grant; National Creative Research Initiative [2010-0018300]; US Department of Energy, Office of Science [DE-AC02-06CH11357]; Canada Foundation for Innovation; Natural Sciences and Engineering Research Council of Canada; University of Saskatchewan; Government of Saskatchewan; Western Economic Diversification Canada; National Research Council of Canada; Canadian Institutes of Health Research FX We would like to thank Arun Paramekanti and Jacob Ruff for valuable discussions. Work at the University of Toronto was supported by the Natural Sciences and Engineering Research Council of Canada through a Discovery Grant and Research Tools and Instruments Grant. Work at Seoul National University was supported by National Creative Research Initiative 2010-0018300. Use of the Advanced Photon Source at Argonne National Laboratory is supported by the US Department of Energy, Office of Science, under Contract No. DE-AC02-06CH11357. Use of the Canadian Light Source is supported by the Canada Foundation for Innovation, the Natural Sciences and Engineering Research Council of Canada, the University of Saskatchewan, the Government of Saskatchewan, Western Economic Diversification Canada, the National Research Council of Canada, and the Canadian Institutes of Health Research. NR 57 TC 1 Z9 1 U1 23 U2 38 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 6 PY 2016 VL 94 IS 2 AR 024408 DI 10.1103/PhysRevB.94.024408 PG 13 WC Physics, Condensed Matter SC Physics GA DR1YZ UT WOS:000379702100004 ER PT J AU Ewings, RA Perring, TG Sikora, O Abernathy, DL Tomioka, Y Tokura, Y AF Ewings, R. A. Perring, T. G. Sikora, O. Abernathy, D. L. Tomioka, Y. Tokura, Y. TI Spin excitations used to probe the nature of exchange coupling in the magnetically ordered ground state of Pr0.5Ca0.5MnO3 SO PHYSICAL REVIEW B LA English DT Article ID DOPED MANGANITES; CHARGE; PHYSICS; SCATTERING; OXIDES AB We have used time-of-flight inelastic neutron scattering to measure the spin wave spectrum of the canonical half-dopedmanganite Pr0.5Ca0.5MnO3 in its magnetic and orbitally ordered phase. The data, which cover multiple Brillouin zones and the entire energy range of the excitations, are compared with several different models that are all consistent with CE-type magnetic order, but arise through different exchange coupling schemes. The Goodenough model, i.e., an ordered state comprising strong nearest-neighbor ferromagnetic interactions along zigzag chains with antiferromagnetic interchain coupling, provides the best description of the data, provided that further neighbor interactions along the chains are included. We are able to rule out a coupling scheme involving formation of strongly bound ferromagnetic dimers, i.e., Zener polarons, on the basis of gross features of the observed spin wave spectrum. A model with weaker dimerization reproduces the observed dispersion but can be ruled out on the basis of discrepancies between the calculated and observed structure factors at certain positions in reciprocal space. Adding further neighbor interactions results in almost no dimerization, i.e., recovery of the Goodenough model. These results are consistent with theoretical analysis of the degenerate double exchange model for half-doping, and provide a recipe for how to interpret future measurements away from half-doping, where degenerate double exchange models predict more complex ground states. C1 [Ewings, R. A.; Perring, T. G.] STFC Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Perring, T. G.] London Ctr Nanotechnol, 17-19 Gordon St, London WC1H 0AH, England. [Sikora, O.] Univ Bristol, HH Wills Phys Lab, Bristol BS8 1TL, Avon, England. [Abernathy, D. L.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Tomioka, Y.] Natl Inst Adv Ind Sci & Technol, Elect & Photon Res Inst, Tsukuba Cent 4,1-1-1 Higashi, Tsukuba, Ibaraki 3058562, Japan. [Tokura, Y.] Univ Tokyo, Dept Appl Phys, Bunkyo Ku, Tokyo 1138656, Japan. [Tokura, Y.] RIKEN, Ctr Emergent Matter Sci, Wako, Saitama 3510198, Japan. [Sikora, O.] Jagiellonian Univ, Marian Smoluchowski Inst Phys, Prof Lojasiewicza 11, PL-30348 Krakow, Poland. RP Ewings, RA (reprint author), STFC Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. EM russell.ewings@stfc.ac.uk RI Tokura, Yoshinori/C-7352-2009; Abernathy, Douglas/A-3038-2012; BL18, ARCS/A-3000-2012 OI Abernathy, Douglas/0000-0002-3533-003X; FU Science and Technology Facilities Council of Great Britain; Polish National Science Center (NCN) [2012/04/A/ST3/00331]; EPSRC [EP/G0314060/1]; Scientific User Facilities Division, Office of Basic Energy Sciences, the US Department of Energy FX We are grateful to A. Daoud-Aladine, G. A. Sawatzky, J. P. Hill, and F. Kruger for helpful discussions, and to A. J. Wenban for work on the dimer spin wave model. This work was supported by the Science and Technology Facilities Council of Great Britain. O.S. acknowledges support by the Polish National Science Center (NCN) under Project. No. 2012/04/A/ST3/00331 and EPSRC Grant EP/G0314060/1. Research at ORNL's Spallation Neutron Source was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, the US Department of Energy. NR 58 TC 1 Z9 1 U1 5 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 6 PY 2016 VL 94 IS 1 AR 014405 DI 10.1103/PhysRevB.94.014405 PG 13 WC Physics, Condensed Matter SC Physics GA DR1YE UT WOS:000379700000003 ER PT J AU Portnichenko, PY Demishev, SV Semeno, AV Ohta, H Cameron, AS Surmach, MA Jang, H Friemel, G Dukhnenko, AV Shitsevalova, NY Filipov, VB Schneidewind, A Ollivier, J Podlesnyak, A Inosov, DS AF Portnichenko, P. Y. Demishev, S. V. Semeno, A. V. Ohta, H. Cameron, A. S. Surmach, M. A. Jang, H. Friemel, G. Dukhnenko, A. V. Shitsevalova, N. Yu. Filipov, V. B. Schneidewind, A. Ollivier, J. Podlesnyak, A. Inosov, D. S. TI Magnetic field dependence of the neutron spin resonance in CeB6 SO PHYSICAL REVIEW B LA English DT Article ID SCATTERING; SUPERCONDUCTORS; DYNAMICS; UPD2AL3; ORDER; MODE AB In zero magnetic field, the famous neutron spin resonance in the f-electron superconductor CeCoIn5 is similar to the recently discovered exciton peak in the nonsuperconducting CeB6. A magnetic field splits the resonance in CeCoIn5 into two components, indicating that it is a doublet. Here we employ inelastic neutron scattering (INS) to scrutinize the field dependence of spin fluctuations in CeB6. The exciton shows a markedly different behavior without any field splitting. Instead, we observe a second field-induced magnon whose energy increases with field. At the ferromagnetic zone center, however, we find only a single mode with a nonmonotonic field dependence. At low fields, it is initially suppressed to zero together with the antiferromagnetic order parameter, but then reappears at higher fields inside the hidden-order phase, following the energy of an electron spin resonance (ESR). This is a unique example of a ferromagnetic resonance in a heavy-fermion metal seen by both ESR and INS consistently over a broad range of magnetic fields. C1 [Portnichenko, P. Y.; Cameron, A. S.; Surmach, M. A.; Inosov, D. S.] Tech Univ Dresden, Inst Festkorperphys, D-01069 Dresden, Germany. [Demishev, S. V.; Semeno, A. V.] RAS, AM Prokhorov Gen Phys Inst, 38 Vavilov St, Moscow 119991, Russia. [Ohta, H.] Kobe Univ, Dept Phys, Nada Ku, Kobe, Hyogo 6578501, Japan. [Jang, H.; Friemel, G.] Max Planck Inst Festkorperforsch, Heisenbergstr 1, D-70569 Stuttgart, Germany. [Jang, H.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Dukhnenko, A. V.; Shitsevalova, N. Yu.; Filipov, V. B.] NAS, IM Frantsevich Inst Problems Mat Sci, 3 Krzhyzhanovsky St, UA-03680 Kiev, Ukraine. [Schneidewind, A.] Forschungszentrum Julich GmbH, JCNS, Outstn Heinz Maier Leibnitz Zentrum MLZ, Lichtenbergstr 1, D-85747 Garching, Germany. [Ollivier, J.] Inst Laue Langevin, 6 Rue Jules Horowitz,BP 156, F-38042 Grenoble, France. [Podlesnyak, A.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. RP Inosov, DS (reprint author), Tech Univ Dresden, Inst Festkorperphys, D-01069 Dresden, Germany. EM Dmytro.Inosov@tu-dresden.de RI Podlesnyak, Andrey/A-5593-2013; Inosov, Dmytro/B-6781-2008 OI Podlesnyak, Andrey/0000-0001-9366-6319; FU German Research Foundation (DFG) [IN 209/3-1]; German Research Foundation (DFG) via the Research Training Group GRK 1621 at the TU Dresden; RFBR [14-02-00800]; RAS Programme "Electron spin resonance, spin-dependent electronic effects and spin technologies"; RAS Programme "Electron correlations in strongly interacting systems"; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy FX We acknowledge stimulating discussions with V. Kataev and thank S. Elorfi (SNS) for technical support during the experiments. TOF data reduction was done using the HORACE software package [53]. This project was funded by the German Research Foundation (DFG) under Grant No. IN 209/3-1 and via the Research Training Group GRK 1621 at the TU Dresden. S.V.D. and A.V.S. acknowledge support from the RFBR Grant No. 14-02-00800 and from the RAS Programmes "Electron spin resonance, spin-dependent electronic effects and spin technologies" and "Electron correlations in strongly interacting systems." Research at the Spallation Neutron Source in Oak Ridge was supported by the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy. NR 53 TC 2 Z9 2 U1 9 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 6 PY 2016 VL 94 IS 3 AR 035114 DI 10.1103/PhysRevB.94.035114 PG 6 WC Physics, Condensed Matter SC Physics GA DR2EL UT WOS:000379717700004 ER PT J AU Stan, CV Dutta, R White, CE Prakapenka, V Duffy, TS AF Stan, Camelia V. Dutta, Rajkrishna White, Claire E. Prakapenka, Vitali Duffy, Thomas S. TI High-pressure polymorphism of PbF2 to 75 GPa SO PHYSICAL REVIEW B LA English DT Article ID X-RAY-DIFFRACTION; ORTHORHOMBIC LEAD FLUORIDE; CRYSTAL-STRUCTURE; PHASE-TRANSITION; NEUTRON-DIFFRACTION; ELASTIC-CONSTANTS; AX(2) COMPOUNDS; GROUND-STATE; ELECTRON-GAS; SYSTEM AB Lead fluoride, PbF2, was investigated experimentally in the laser-heated diamond anvil cell by x-ray diffraction to pressures of 75 GPa at room temperature and to 64.5 GPa and 2430 K, as well as through first-principles density functional theory calculations up to 70 GPa. During room temperature compression, no discontinuous changes in the x-ray diffraction pattern or volume were observed, but the lattice parameters displayed highly anomalous trends between 10-22 GPa with enhanced compressibility along the a direction and reduced or even negative compressibility along b and c. Theoretical calculations of valence electron densities at 22 GPa showed that alpha-PbF2 underwent a pressure-induced isosymmetric phase transition to a postcotunnite Co2Si structure and also revealed the detailed atomic rearrangements associated with the development of an extra Pb-F bond in the high-pressure phase. Our x-ray results and theoretical calculations are consistent with an isosymmetric phase transition smoothly occurring over 10-22 GPa rather than abruptly as previously suggested. The characteristic values for the cell constants a/c and (a + c)/b, which are used to distinguish among cotunnite-, Co2Si-, and Ni2In-type phases, require modification based on our results. An equation of state fit yields a bulk modulus, K-0, of 72(3) GPa for the cotunnite-type, and an ambient-pressure volume, V-0, of 182(2)angstrom(3), and K-0 = 81(4) GPa for the Co2Si-type phase when fixing the pressure derivative of the bulk modulus, K'(0) = 4. Upon heating above 1200 K at pressures at or above 25.9 GPa, PbF2 partially transformed to the hexagonal Ni2In-type phase but wholly or partially reverted back to Co2Si-type phase upon temperature quench. From 43-65 GPa, nearly complete transformation to the Ni2In-type PbF2 was observed at high temperature, but the material partially transformed back to the orthorhombic phase upon temperature quench. Our results show that high-pressure behavior of PbF2 is distinct from that of the alkaline earth fluorides with similar ionic radii. Our results also have relevance to understanding the behavior of lanthanide and actinide dioxides, which have been predicted theoretically to exhibit similar isosymmetric transitions at Mbar pressures. C1 [Stan, Camelia V.] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. [Dutta, Rajkrishna; Duffy, Thomas S.] Princeton Univ, Dept Geosci, Princeton, NJ 08544 USA. [White, Claire E.] Princeton Univ, Dept Civil & Environm Engn, Princeton, NJ 08544 USA. [White, Claire E.] Princeton Univ, Andlinger Ctr Energy & Environm, Princeton, NJ 08544 USA. [Prakapenka, Vitali] Univ Chicago, Argonne Natl Lab, GeoSoilEnviroCARS, Argonne, IL 60439 USA. RP Stan, CV (reprint author), Princeton Univ, Dept Chem, Princeton, NJ 08544 USA. RI White, Claire/A-1722-2011; Duffy, Thomas/C-9140-2017 OI White, Claire/0000-0002-4800-7960; Duffy, Thomas/0000-0002-5357-1259 FU National Science Foundation (NSF) [EAR-1415321]; US DOE [DE-AC02-06CH11357]; NSF Earth Sciences [EAR-1128799]; Department of Energy, Geosciences [DE-FG02-94ER14466] FX We thank Greg Finkelstein and Earl O'Bannon for experimental assistance and helpful discussion. This paper was supported by the National Science Foundation (NSF) (EAR-1415321). Use of the Advanced Photon Source, an Office of Science User Facility operated for the US Department of Energy (DOE) Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. We acknowledge the support of GeoSoilEnviroCARS (Sector 13), which is supported by the NSF Earth Sciences (Grant No. EAR-1128799), and the Department of Energy, Geosciences (Grant No. DE-FG02-94ER14466). NR 97 TC 0 Z9 0 U1 2 U2 13 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 6 PY 2016 VL 94 IS 2 AR 024104 DI 10.1103/PhysRevB.94.024104 PG 12 WC Physics, Condensed Matter SC Physics GA DR1YZ UT WOS:000379702100002 ER PT J AU Abazov, VM Abbott, B Acharya, BS Adams, M Adams, T Agnew, JP Alexeev, GD Alkhazov, G Alton, A Askew, A Atkins, S Augsten, K Aushev, V Aushev, Y Avila, C Badaud, F Bagby, L Baldin, B Bandurin, DV Banerjee, S Barberis, E Baringer, P Bartlett, JF Bassler, U Bazterra, V Bean, A Begalli, M Bellantoni, L Beri, SB Bernardi, G Bernhard, R Bertram, I Besancon, M Beuselinck, R Bhat, PC Bhatia, S Bhatnagar, V Blazey, G Blessing, S Bloom, K Boehnlein, A Boline, D Boos, EE Borissov, G Borysova, M Brandt, A Brandt, O Brochmann, M Brock, R Bross, A Brown, D Bu, XB Buehler, M Buescher, V Bunichev, V Burdin, S Buszello, CP Camacho-Perez, E Casey, BCK Castilla-Valdez, H Caughron, S Chakrabarti, S Chan, KM Chandra, A Chapon, E Chen, G Cho, SW Choi, S Choudhary, B Cihangir, S Claes, D Clutter, J Cooke, M Cooper, WE Corcoran, M Couderc, F Cousinou, MC Cuth, J Cutts, D Das, A Davies, G de Jong, SJ De La Cruz-Burelo, E Deliot, F Demina, R Denisov, D Denisov, SP Desai, S Deterre, C DeVaughan, K Diehl, HT Diesburg, M Ding, PF Dominguez, A Dubey, A Dudko, LV Duperrin, A Dutt, S Eads, M Edmunds, D Ellison, J Elvira, VD Enari, Y Evans, H Evdokimov, A Evdokimov, VN Faure, A Feng, L Ferbel, T Fiedler, F Filthaut, F Fisher, W Fisk, HE Fortner, M Fox, H Franc, J Fuess, S Garbincius, PH Garcia-Bellido, A Garcia-Gonzalez, JA Gavrilov, V Geng, W Gerber, CE Gershtein, Y Ginther, G Gogota, O Golovanov, G Grannis, PD Greder, S Greenlee, H Grenier, G Gris, P Grivaz, JF Grohsjean, A Grunendahl, S Grunewald, MW Guillemin, T Gutierrez, G Gutierrez, P Haley, J Han, L Harder, K Harel, A Hauptman, JM Hays, J Head, T Hebbeker, T Hedin, D Hegab, H Heinson, AP Heintz, U Hansel, C Heredia-De La Cruz, I Hernandez-Villanueva, M Herner, K Hesketh, G Hildreth, MD Hirosky, R Hoang, T Hobbs, JD Hoeneisen, B Hogan, J Hohlfeld, M Holzbauer, JL Howley, I Hubacek, Z Iashvili, I Ilchenko, Y Illingworth, R Ito, AS Jabeen, S Jaffre, M Jayasinghe, A Jeong, MS Jesik, R Jiang, P Johns, K Johnson, E Johnson, M Jonckheere, A Jonsson, P Joshi, J Jung, AW Juste, A Kajfasz, E Karmanov, D Katsanos, I Kaur, M Kehoe, R Kermiche, S Khalatyan, N Khanov, A Kharchilava, A Kharzheev, YN Kiselevich, I Kohli, JM Kozelov, AV Kraus, J Kumar, A Kupco, A Kurca, T Kuzmin, VA Lammers, S Lebrun, P Lee, HS Lee, SW Lee, WM Lei, X Lellouch, J Li, D Li, H Li, L Li, QZ Lim, JK Lincoln, D Linnemann, J Lipaev, VV Lipton, R Liu, H Liu, Y Lobodenko, A Lokajicek, M de Sa, RL Luna-Garcia, R Lyon, AL Maciel, AKA Madar, R Magana-Villalba, R Malik, S Malyshev, VL Mansour, J Martinez-Ortega, J McCarthy, R McGivern, CL Meijer, MM Melnitchouk, A Menezes, D Mercadante, PG Merkin, M Meyer, A Meyer, J Miconi, F Mondal, NK Mulhearn, M Nagy, E Narain, M Nayyar, R Neal, HA Negret, JP Neustroev, P Nguyen, HT Nunnemann, T Orduna, J Osman, N Pal, A Parashar, N Parihar, V Park, SK Partridge, R Parua, N Patwa, A Penning, B Perfilov, M Peters, Y Petridis, K Petrillo, G Petroff, P Pleier, MA Podstavkov, VM Popov, AV Prewitt, M Price, D Prokopenko, N Qian, J Quadt, A Quinn, B Ratoff, PN Razumov, I Ripp-Baudot, I Rizatdinova, F Rominsky, M Ross, A Royon, C Rubinov, P Ruchti, R Sajot, G Sanchez-Hernandez, A Sanders, MP Santos, AS Savage, G Savitskyi, M Sawyer, L Scanlon, T Schamberger, RD Scheglov, Y Schellman, H Schott, M Schwanenberger, C Schwienhorst, R Sekaric, J Severini, H Shabalina, E Shary, V Shaw, S Shchukin, AA Simak, V Skubic, P Slattery, P Snow, GR Snow, J Snyder, S Soldner-Rembold, S Sonnenschein, L Soustruznik, K Stark, J Stefaniuk, N Stoyanova, DA Strauss, M Suter, L Svoisky, P Titov, M Tokmenin, VV Tsai, YT Tsybychev, D Tuchming, B Tully, C Uvarov, L Uvarov, S Uzunyan, S Van Kooten, R van Leeuwen, WM Varelas, N Varnes, EW Vasilyev, IA Verkheev, AY Vertogradov, LS Verzocchi, M Vesterinen, M Vilanova, D Vokac, P Wahl, HD Wang, MHLS Warchol, J Watts, G Wayne, M Weichert, J Welty-Rieger, L Williams, MRJ Wilson, GW Wobisch, M Wood, DR Wyatt, TR Xie, Y Yamada, R Yang, S Yasuda, T Yatsunenko, YA Ye, W Ye, Z Yin, H Yip, K Youn, SW Yu, JM Zennamo, J Zhao, TG Zhou, B Zhu, J Zielinski, M Zieminska, D Zivkovic, L AF Abazov, V. M. Abbott, B. Acharya, B. S. Adams, M. Adams, T. Agnew, J. P. Alexeev, G. D. Alkhazov, G. Alton, A. Askew, A. Atkins, S. Augsten, K. Aushev, V. Aushev, Y. Avila, C. Badaud, F. Bagby, L. Baldin, B. Bandurin, D. V. Banerjee, S. Barberis, E. Baringer, P. Bartlett, J. F. Bassler, U. Bazterra, V. Bean, A. Begalli, M. Bellantoni, L. Beri, S. B. Bernardi, G. Bernhard, R. Bertram, I. Besancon, M. Beuselinck, R. Bhat, P. C. Bhatia, S. Bhatnagar, V. Blazey, G. Blessing, S. Bloom, K. Boehnlein, A. Boline, D. Boos, E. E. Borissov, G. Borysova, M. Brandt, A. Brandt, O. Brochmann, M. Brock, R. Bross, A. Brown, D. Bu, X. B. Buehler, M. Buescher, V. Bunichev, V. Burdin, S. Buszello, C. P. Camacho-Perez, E. Casey, B. C. K. Castilla-Valdez, H. Caughron, S. Chakrabarti, S. Chan, K. M. Chandra, A. Chapon, E. Chen, G. Cho, S. W. Choi, S. Choudhary, B. Cihangir, S. Claes, D. Clutter, J. Cooke, M. Cooper, W. E. Corcoran, M. Couderc, F. Cousinou, M. -C. Cuth, J. Cutts, D. Das, A. Davies, G. de Jong, S. J. De La Cruz-Burelo, E. Deliot, F. Demina, R. Denisov, D. Denisov, S. P. Desai, S. Deterre, C. DeVaughan, K. Diehl, H. T. Diesburg, M. Ding, P. F. Dominguez, A. Dubey, A. Dudko, L. V. Duperrin, A. Dutt, S. Eads, M. Edmunds, D. Ellison, J. Elvira, V. D. Enari, Y. Evans, H. Evdokimov, A. Evdokimov, V. N. Faure, A. Feng, L. Ferbel, T. Fiedler, F. Filthaut, F. Fisher, W. Fisk, H. E. Fortner, M. Fox, H. Franc, J. Fuess, S. Garbincius, P. H. Garcia-Bellido, A. Garcia-Gonzalez, J. A. Gavrilov, V. Geng, W. Gerber, C. E. Gershtein, Y. Ginther, G. Gogota, O. Golovanov, G. Grannis, P. D. Greder, S. Greenlee, H. Grenier, G. Gris, Ph. Grivaz, J. -F. Grohsjean, A. Gruenendahl, S. Gruenewald, M. W. Guillemin, T. Gutierrez, G. Gutierrez, P. Haley, J. Han, L. Harder, K. Harel, A. Hauptman, J. M. Hays, J. Head, T. Hebbeker, T. Hedin, D. Hegab, H. Heinson, A. P. Heintz, U. Hansel, C. Heredia-De La Cruz, I. Hernandez-Villanueva, M. Herner, K. Hesketh, G. Hildreth, M. D. Hirosky, R. Hoang, T. Hobbs, J. D. 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Meyer, J. Miconi, F. Mondal, N. K. Mulhearn, M. Nagy, E. Narain, M. Nayyar, R. Neal, H. A. Negret, J. P. Neustroev, P. Nguyen, H. T. Nunnemann, T. Orduna, J. Osman, N. Pal, A. Parashar, N. Parihar, V. Park, S. K. Partridge, R. Parua, N. Patwa, A. Penning, B. Perfilov, M. Peters, Y. Petridis, K. Petrillo, G. Petroff, P. Pleier, M. -A. Podstavkov, V. M. Popov, A. V. Prewitt, M. Price, D. Prokopenko, N. Qian, J. Quadt, A. Quinn, B. Ratoff, P. N. Razumov, I. Ripp-Baudot, I. Rizatdinova, F. Rominsky, M. Ross, A. Royon, C. Rubinov, P. Ruchti, R. Sajot, G. Sanchez-Hernandez, A. Sanders, M. P. Santos, A. S. Savage, G. Savitskyi, M. Sawyer, L. Scanlon, T. Schamberger, R. D. Scheglov, Y. Schellman, H. Schott, M. Schwanenberger, C. Schwienhorst, R. Sekaric, J. Severini, H. Shabalina, E. Shary, V. Shaw, S. Shchukin, A. A. Simak, V. Skubic, P. Slattery, P. Snow, G. R. Snow, J. Snyder, S. Soeldner-Rembold, S. Sonnenschein, L. Soustruznik, K. Stark, J. Stefaniuk, N. Stoyanova, D. A. Strauss, M. Suter, L. Svoisky, P. Titov, M. Tokmenin, V. V. Tsai, Y. -T. Tsybychev, D. Tuchming, B. Tully, C. Uvarov, L. Uvarov, S. Uzunyan, S. Van Kooten, R. van Leeuwen, W. M. Varelas, N. Varnes, E. W. Vasilyev, I. A. Verkheev, A. Y. Vertogradov, L. S. Verzocchi, M. Vesterinen, M. Vilanova, D. Vokac, P. Wahl, H. D. Wang, M. H. L. S. Warchol, J. Watts, G. Wayne, M. Weichert, J. Welty-Rieger, L. Williams, M. R. J. Wilson, G. W. Wobisch, M. Wood, D. R. Wyatt, T. R. Xie, Y. Yamada, R. Yang, S. Yasuda, T. Yatsunenko, Y. A. Ye, W. Ye, Z. Yin, H. Yip, K. Youn, S. W. Yu, J. M. Zennamo, J. Zhao, T. G. Zhou, B. Zhu, J. Zielinski, M. Zieminska, D. Zivkovic, L. CA D0 Collaboration TI B-s(0) lifetime measurement in the CP-odd decay channel B-s(0) -> J/Psi f(0)(980) SO PHYSICAL REVIEW D LA English DT Article AB The lifetime of the B-s(0) meson is measured in the decay channel B-s(0) -> J/Psi pi(+)pi(-) with 880 <= M pi+pi- <= 1080 MeV/c(2), which is mainly a CP-odd state and dominated by the f(0)(980) resonance. In 10.4 fb(-1) of data collected with the D0 detector in Run II of the Tevatron, the lifetime of the B-s(0) meson is measured to be tau(B-s(0)) = 1.70 +/- 0.14(stat) +/- 0.05(syst) ps. Neglecting CP violation in B-s(0)/(B) over bar (0)(s) mixing, the measurement can be translated into the width of the heavy mass eigenstate of the B-s(0), Gamma(H) = 0.59 +/- 0.05(stat) +/- 0.02(syst) ps(-1). C1 [Borysova, M.; Grohsjean, A.; Hansel, C.; Maciel, A. K. A.; Santos, A. S.] Ctr Brasileiro Pesquisas Fis, LAFEX, BR-22290 Rio De Janeiro, RJ, Brazil. [Begalli, M.; Dubey, A.] Univ Estado Rio de Janeiro, Rio De Janeiro, RJ, Brazil. [Mercadante, P. G.] Univ Fed ABC, BR-09210 Sao Paulo, Brazil. [Han, L.; Jiang, P.; Liu, Y.; Yang, S.] Univ Sci & Technol China, Hefei 230026, Peoples R China. [Avila, C.; Negret, J. P.] Univ Los Andes, Bogota 111711, Colombia. [Soustruznik, K.] Charles Univ Prague, Fac Math & Phys, Ctr Particle Phys, CR-11636 Prague 1, Czech Republic. [Alton, A.; Augsten, K.; Franc, J.; Hubacek, Z.; Simak, V.; Vokac, P.] Czech Tech Univ, Prague 11636 6, Czech Republic. [Kupco, A.; Lokajicek, M.; Royon, C.] Acad Sci Czech Republic, Inst Phys, Prague 18221, Czech Republic. [Hoeneisen, B.] Univ San Francisco Quito, Quito, Ecuador. [Badaud, F.; Gris, Ph.] Univ Clermont Ferrand, CNRS, IN2P3, LPC, F-63178 Aubiere, France. [Sajot, G.; Stark, J.] Univ Grenoble 1, CNRS, IN2P3, Inst Natl Polytech Grenoble,LPSC, F-38026 St Martin Dheres, France. [Cousinou, M. -C.; Duperrin, A.; Geng, W.; Kajfasz, E.; Kermiche, S.; Nagy, E.; Osman, N.] Aix Marseille Univ, CNRS, IN2P3, CPPM, F-13288 Marseille 09, France. 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[Partridge, R.] Purdue Univ, W Lafayette, IN 47907 USA. RP Abazov, VM (reprint author), Joint Nucl Res Inst, Dubna 141980, Russia. RI Dudko, Lev/D-7127-2012; Gutierrez, Phillip/C-1161-2011; Li, Liang/O-1107-2015 OI Dudko, Lev/0000-0002-4462-3192; Li, Liang/0000-0001-6411-6107 FU Department of Energy (U.S.); National Science Foundation (U.S.); Alternative Energies and Atomic Energy Commission (France); National Center for Scientific Research/National Institute of Nuclear and Particle Physics (France); Ministry of Education and Science of the Russian Federation (Russia); National Research Center "Kurchatov Institute" of the Russian Federation (Russia); Russian Foundation for Basic Research (Russia); National Council for the Development of Science and Technology (Brazil); Carlos Chagas Filho Foundation for the Support of Research in the State of Rio de Janeiro (Brazil); Department of Atomic Energy (India); Department of Science and Technology (India); Administrative Department of Science, Technology and Innovation (Colombia); National Council of Science and Technology (Mexico); National Research Foundation of Korea (Korea); Foundation for Fundamental Research on Matter (The Netherlands); Science and Technology Facilities Council (U.K.); The Royal Society (U.K.); Ministry of Education, Youth and Sports (Czech Republic); Bundesministerium fur Bildung und Forschung (Federal Ministry of Education and Research) (Germany); Deutsche Forschungsgemeinschaft (German Research Foundation) (Germany); Science Foundation Ireland (Ireland); Swedish Research Council (Sweden); China Academy of Sciences (China); National Natural Science Foundation of China (China); Ministry of Education and Science of Ukraine (Ukraine) FX We thank the staffs at Fermilab and collaborating institutions, and acknowledge support from the Department of Energy and National Science Foundation (U.S.); Alternative Energies and Atomic Energy Commission and National Center for Scientific Research/National Institute of Nuclear and Particle Physics (France); Ministry of Education and Science of the Russian Federation, National Research Center "Kurchatov Institute" of the Russian Federation, and Russian Foundation for Basic Research (Russia); National Council for the Development of Science and Technology and Carlos Chagas Filho Foundation for the Support of Research in the State of Rio de Janeiro (Brazil); Department of Atomic Energy and Department of Science and Technology (India); Administrative Department of Science, Technology and Innovation (Colombia); National Council of Science and Technology (Mexico); National Research Foundation of Korea (Korea); Foundation for Fundamental Research on Matter (The Netherlands); Science and Technology Facilities Council and The Royal Society (U.K.); Ministry of Education, Youth and Sports (Czech Republic); Bundesministerium fur Bildung und Forschung (Federal Ministry of Education and Research) and Deutsche Forschungsgemeinschaft (German Research Foundation) (Germany); Science Foundation Ireland (Ireland); Swedish Research Council (Sweden); China Academy of Sciences and National Natural Science Foundation of China (China); and Ministry of Education and Science of Ukraine (Ukraine). NR 18 TC 0 Z9 0 U1 3 U2 9 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 6 PY 2016 VL 94 IS 1 AR 012001 DI 10.1103/PhysRevD.94.012001 PG 7 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DR1QT UT WOS:000379680700001 ER PT J AU Abbott, T Abdalla, FB Allam, S Amara, A Annis, J Armstrong, R Bacon, D Banerji, M Bauer, AH Baxter, E Becker, MR Benoit-Levy, A Bernstein, RA Bernstein, GM Bertin, E Blazek, J Bonnett, C Bridle, SL Brooks, D Bruderer, C Buckley-Geer, E Burke, DL Busha, MT Capozzi, D Rosell, AC Kind, MC Carretero, J Castander, FJ Chang, C Clampitt, J Crocce, M Cunha, CE D'Andrea, CB da Costa, LN Das, R DePoy, DL Desai, S Diehl, HT Dietrich, JP Dodelson, S Doel, P Drlica-Wagner, A Efstathiou, G Eifler, TF Erickson, B Estrada, J Evrard, AE Neto, AF Fernandez, E Finley, DA Flaugher, B Fosalba, P Friedrich, O Frieman, J Gangkofner, C Garcia-Bellido, J Gaztanaga, E Gerdes, DW Gruen, D Gruendl, RA Gutierrez, G Hartley, W Hirsch, M Honscheid, K Huff, EM Jain, B James, DJ Jarvis, M Kacprzak, T Kent, S Kirk, D Krause, E Kravtsov, A Kuehn, K Kuropatkin, N Kwan, J Lahav, O Leistedt, B Li, TS Lima, M Lin, H MacCrann, N March, M Marshall, JL Martini, P McMahon, RG Melchior, P Miller, CJ Miquel, R Mohr, JJ Neilsen, E Nichol, RC Nicola, A Nord, B Ogando, R Palmese, A Peiris, HV Plazas, AA Refregier, A Roe, N Romer, AK Roodman, A Rowe, B Rykoff, ES Sabiu, C Sadeh, I Sako, M Samuroff, S Sanchez, E Sanchez, C Seo, H Sevilla-Noarbe, I Sheldon, E Smith, RC Soares-Santos, M Sobreira, F Suchyta, E Swanson, MEC Tarle, G Thaler, J Thomas, D Troxel, MA Vikram, V Walker, AR Wechsler, RH Weller, J Zhang, Y Zuntz, J AF Abbott, T. Abdalla, F. B. Allam, S. Amara, A. Annis, J. Armstrong, R. Bacon, D. Banerji, M. Bauer, A. H. Baxter, E. Becker, M. R. Benoit-Levy, A. Bernstein, R. A. Bernstein, G. M. Bertin, E. Blazek, J. Bonnett, C. Bridle, S. L. Brooks, D. Bruderer, C. Buckley-Geer, E. Burke, D. L. Busha, M. T. Capozzi, D. Rosell, A. Carnero Kind, M. Carrasco Carretero, J. Castander, F. J. Chang, C. Clampitt, J. Crocce, M. Cunha, C. E. D'Andrea, C. B. da Costa, L. N. Das, R. DePoy, D. L. Desai, S. Diehl, H. T. Dietrich, J. P. Dodelson, S. Doel, P. Drlica-Wagner, A. Efstathiou, G. Eifler, T. F. Erickson, B. Estrada, J. Evrard, A. E. Fausti Neto, A. Fernandez, E. Finley, D. A. Flaugher, B. Fosalba, P. Friedrich, O. Frieman, J. Gangkofner, C. Garcia-Bellido, J. Gaztanaga, E. Gerdes, D. W. Gruen, D. Gruendl, R. A. Gutierrez, G. Hartley, W. Hirsch, M. Honscheid, K. Huff, E. M. Jain, B. James, D. J. Jarvis, M. Kacprzak, T. Kent, S. Kirk, D. Krause, E. Kravtsov, A. Kuehn, K. Kuropatkin, N. Kwan, J. Lahav, O. Leistedt, B. Li, T. S. Lima, M. Lin, H. MacCrann, N. March, M. Marshall, J. L. Martini, P. McMahon, R. G. Melchior, P. Miller, C. J. Miquel, R. Mohr, J. J. Neilsen, E. Nichol, R. C. Nicola, A. Nord, B. Ogando, R. Palmese, A. Peiris, H. V. Plazas, A. A. Refregier, A. Roe, N. Romer, A. K. Roodman, A. Rowe, B. Rykoff, E. S. Sabiu, C. Sadeh, I. Sako, M. Samuroff, S. Sanchez, E. Sanchez, C. Seo, H. Sevilla-Noarbe, I. Sheldon, E. Smith, R. C. Soares-Santos, M. Sobreira, F. Suchyta, E. Swanson, M. E. C. Tarle, G. Thaler, J. Thomas, D. Troxel, M. A. Vikram, V. Walker, A. R. Wechsler, R. H. Weller, J. Zhang, Y. Zuntz, J. CA Dark Energy Survey Collaboration TI Cosmology from cosmic shear with Dark Energy Survey Science Verification data SO PHYSICAL REVIEW D LA English DT Article ID MATTER POWER SPECTRUM; WEAK-LENSING TOMOGRAPHY; LARGE-SCALE STRUCTURE; BARYON ACOUSTIC-OSCILLATIONS; INTRINSIC ALIGNMENTS; PARAMETER CONSTRAINTS; GALAXY ELLIPTICITIES; PRECISION COSMOLOGY; COVARIANCE-MATRIX; HUBBLE CONSTANT AB We present the first constraints on cosmology from the Dark Energy Survey (DES), using weak lensing measurements from the preliminary Science Verification (SV) data. We use 139 square degrees of SV data, which is less than 3% of the full DES survey area. Using cosmic shear 2-point measurements over three redshift bins we find sigma(8)(Omega(m)/0.3)(0.5) = 0.81 +/- 0.06 (68% confidence), after marginalizing over 7 systematics parameters and 3 other cosmological parameters. We examine the robustness of our results to the choice of data vector and systematics assumed, and find them to be stable. About 20% of our error bar comes from marginalizing over shear and photometric redshift calibration uncertainties. The current state-of-the-art cosmic shear measurements from CFHTLenS are mildly discrepant with the cosmological constraints from Planck CMB data; our results are consistent with both data sets. Our uncertainties are similar to 30% larger than those from CFHTLenS when we carry out a comparable analysis of the two data sets, which we attribute largely to the lower number density of our shear catalogue. We investigate constraints on dark energy and find that, with this small fraction of the full survey, the DES SV constraints make negligible impact on the Planck constraints. The moderate disagreement between the CFHTLenS and Planck values of sigma(8)(Omega(m)/0.3)(0.5) is present regardless of the value of w. C1 [Abbott, T.; James, D. J.; Smith, R. C.; Walker, A. R.] Natl Opt Astron Observ, Cerro Tololo Interamer Observ, Casilla 603, La Serena, Chile. [Abdalla, F. B.; Benoit-Levy, A.; Brooks, D.; Doel, P.; Hirsch, M.; Kirk, D.; Lahav, O.; Leistedt, B.; Palmese, A.; Peiris, H. V.; Rowe, B.; Sadeh, I.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Allam, S.; Annis, J.; Buckley-Geer, E.; Diehl, H. T.; Dodelson, S.; Drlica-Wagner, A.; Estrada, J.; Finley, D. A.; Flaugher, B.; Frieman, J.; Gutierrez, G.; Kent, S.; Kuropatkin, N.; Lin, H.; Neilsen, E.; Nord, B.; Soares-Santos, M.; Sobreira, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Amara, A.; Bruderer, C.; Chang, C.; Hartley, W.; Kacprzak, T.; Nicola, A.; Refregier, A.] ETH, Dept Phys, Wolfgang Pauli Str 16, CH-8093 Zurich, Switzerland. [Armstrong, R.] Princeton Univ, Dept Astrophys Sci, Peyton Hall, Princeton, NJ 08544 USA. [Bacon, D.; Capozzi, D.; D'Andrea, C. B.; Nichol, R. C.; Thomas, D.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [Banerji, M.; Efstathiou, G.; McMahon, R. G.] Univ Cambridge, Inst Astron, Madingley Rd, Cambridge CB3 0HA, England. [Banerji, M.; Efstathiou, G.; McMahon, R. G.] Univ Cambridge, Kavli Inst Cosmol, Madingley Rd, Cambridge CB3 0HA, England. [Bauer, A. H.; Carretero, J.; Castander, F. J.; Crocce, M.; Fosalba, P.; Gaztanaga, E.] IEEC CSIC, Inst Ciencies Espai, Campus UAB,Carrer Can Magrans S-N, Barcelona 08193, Spain. [Baxter, E.; Bernstein, G. M.; Clampitt, J.; Eifler, T. F.; Jain, B.; March, M.; Sako, M.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Becker, M. R.; Burke, D. L.; Busha, M. T.; Cunha, C. E.; Krause, E.; Roodman, A.; Rykoff, E. S.; Wechsler, R. H.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, POB 2450, Stanford, CA 94305 USA. [Becker, M. R.; Busha, M. T.; Wechsler, R. H.] Stanford Univ, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94305 USA. [Bernstein, R. A.] Carnegie Observ, 813 Santa Barbara St, Pasadena, CA 91101 USA. [Bertin, E.] Univ Paris 06, Sorbonne Univ, Inst Astrophys Paris, UMR 7095, F-75014 Paris, France. [Bertin, E.] CNRS, UMR 7095, Inst Astrophys Paris, F-75014 Paris, France. [Blazek, J.; Honscheid, K.; Huff, E. M.; Martini, P.; Melchior, P.; Seo, H.; Suchyta, E.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Bonnett, C.; Carretero, J.; Fernandez, E.; Miquel, R.; Sanchez, C.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Bridle, S. L.; MacCrann, N.; Samuroff, S.; Troxel, M. A.; Zuntz, J.] Univ Manchester, Sch Phys & Astron, Jodrell Bank, Ctr Astrophys, Oxford Rd, Manchester M13 9PL, Lancs, England. [Burke, D. L.; Roodman, A.; Rykoff, E. S.; Wechsler, R. H.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Rosell, A. Carnero; da Costa, L. N.; Jarvis, M.; Ogando, R.] Observ Nacl, Rua Gal Jose Cristino 77, BR-20921400 Rio De Janeiro, RJ, Brazil. [Rosell, A. Carnero; da Costa, L. N.; Fausti Neto, A.; Lima, M.; Ogando, R.; Sobreira, F.] Lab Interinst E Astron LIneA, Rua Gal Jose Cristino 77, BR-20921400 Rio De Janeiro, RJ, Brazil. [Kind, M. Carrasco; Gruendl, R. A.; Swanson, M. E. C.] Natl Ctr Supercomp Applicat, 1205 West Clark St, Urbana, IL 61801 USA. [Kind, M. Carrasco; Gruendl, R. A.; Sevilla-Noarbe, I.] Univ Illinois, Dept Astron, 1002 W Green St, Urbana, IL 61801 USA. [Das, R.; Erickson, B.; Evrard, A. E.; Gerdes, D. W.; Miller, C. J.; Tarle, G.; Zhang, Y.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [DePoy, D. L.; Li, T. S.; Marshall, J. L.] Texas A&M Univ, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [DePoy, D. L.; Li, T. S.; Marshall, J. L.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Desai, S.; Dietrich, J. P.; Gangkofner, C.; Mohr, J. J.] Univ Munich, Fac Phys, Scheinerstr 1, D-81679 Munich, Germany. [Desai, S.; Dietrich, J. P.; Gangkofner, C.; Mohr, J. J.; Weller, J.] Excellence Cluster Universe, Boltzmannstr 2, D-85748 Garching, Germany. [Dodelson, S.; Frieman, J.; Kravtsov, A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Eifler, T. F.; Plazas, A. A.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Evrard, A. E.; Miller, C. J.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Friedrich, O.; Gruen, D.; Mohr, J. J.; Weller, J.] Max Planck Inst Extraterr Phys, Giessenbachstr, D-85748 Garching, Germany. [Friedrich, O.; Gruen, D.; Weller, J.] Univ Munich, Fak Phys, Univ Sternwarte, Scheinerstr 1, D-81679 Munich, Germany. [Garcia-Bellido, J.] Univ Autonoma Madrid, Inst Fis Teor IFT UAM CSIC, E-28049 Madrid, Spain. [Honscheid, K.; Huff, E. M.; Melchior, P.; Suchyta, E.] Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. [Kuehn, K.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Kwan, J.; Vikram, V.] Argonne Natl Lab, 9700 South Cass Ave, Lemont, IL 60439 USA. [Lima, M.] Univ Sao Paulo, Inst Fis, Dept Fis Matemat, CP 66318, BR-05314970 Sao Paulo, Brazil. [Martini, P.] Ohio State Univ, Dept Astron, 174 W 18Th Ave, Columbus, OH 43210 USA. [Miquel, R.] Inst Catalana Recerca & Estudis Avancats, E-08010 Barcelona, Spain. [Roe, N.] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Romer, A. K.] Univ Sussex, Dept Phys & Astron, Pevensey Bldg, Brighton BN1 9QH, E Sussex, England. [Sabiu, C.] Korea Astron & Space Sci Inst, Daejeon 305348, South Korea. [Sanchez, E.; Sevilla-Noarbe, I.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. [Seo, H.] Ohio Univ, Dept Phys & Astron, 251B Clippinger Labs, Athens, OH 45701 USA. [Sheldon, E.] Brookhaven Natl Lab, Bldg 510, Upton, NY 11973 USA. [Thaler, J.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. RP MacCrann, N (reprint author), Univ Manchester, Sch Phys & Astron, Jodrell Bank, Ctr Astrophys, Oxford Rd, Manchester M13 9PL, Lancs, England. EM niall.maccrann@postgrad.manchester.ac.uk; joseph.zuntz@manchester.ac.uk RI Lima, Marcos/E-8378-2010; Ogando, Ricardo/A-1747-2010; Sobreira, Flavia/F-4168-2015; Fernandez, Enrique/L-5387-2014; Gaztanaga, Enrique/L-4894-2014; OI Ogando, Ricardo/0000-0003-2120-1154; Sobreira, Flavia/0000-0002-7822-0658; Garcia-Bellido, Juan/0000-0002-9370-8360; Fernandez, Enrique/0000-0002-6405-9488; Gaztanaga, Enrique/0000-0001-9632-0815; McMahon, Richard/0000-0001-8447-8869; Stern, Corvin/0000-0003-4406-6127; Rowe, Barnaby/0000-0002-7042-9174; Abdalla, Filipe/0000-0003-2063-4345 FU DoE [DE-AC02-98CH10886, DE-SC0007901, DE-FG02-91ER40690]; SFB-Transregio 33 'The Dark Universe' by the Deutsche Forschungsgemeinschaft (DFG); DFG cluster of excellence 'Origin and Structure of the Universe'; NSF [AST-0812790, AST-1138729]; JPL; U.S. Department of Energy; U.S. National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Center for Cosmology and Astro-Particle Physics at the Ohio State University; Mitchell Institute for Fundamental Physics and Astronomy at Texas AM University; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia, Tecnologia e Inovacao; Deutsche Forschungsgemeinschaft; Collaborating Institutions in the Dark Energy Survey; National Science Foundation [AST-1138766]; MINECO [AYA2012-39559, ESP2013-48274, FPA2013-47986]; Centro de Excelencia Severo Ochoa [SEV-2012-0234, SEV-2012-0249]; European Research Council under European Union Seventh Framework Programme; ERC grant [240672, 291329, 306478] FX We are grateful for the extraordinary contributions of our CTIO colleagues and the DECam Construction, Commissioning and Science Verification teams in achieving the excellent instrument and telescope conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the DES Data Management group. We are very grateful to Iain Murray for advice on importance sampling. We thank Catherine Heymans, Martin Kilbinger, Antony Lewis and Adam Moss for helpful discussion. This paper is DES paper DES-2015-0076 and FermiLab preprint number FERMILAB-PUB-15-285-AE. Sheldon is supported by DoE Grant No. DE-AC02-98CH10886. Gruen was supported by SFB-Transregio 33 'The Dark Universe' by the Deutsche Forschungsgemeinschaft (DFG) and the DFG cluster of excellence 'Origin and Structure of the Universe'. Gangkofner acknowledges the support by the DFG Cluster of Excellence 'Origin and Structure of the Universe'. Jarvis has been supported on this project by NSF Grants No. AST-0812790 and AST-1138729. Jarvis, Bernstein, and Jain are partially supported by DoE Grant No. DE-SC0007901. Melchior was supported by DoE Grant No. DE-FG02-91ER40690. Plazas was supported by DoE Grant No. DE-AC02-98CH10886 and by JPL, run by Caltech under a contract for NASA. Funding for the DES Projects has been provided by the U.S. Department of Energy, the U.S. National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, the Center for Cosmology and Astro-Particle Physics at the Ohio State University, the Mitchell Institute for Fundamental Physics and Astronomy at Texas A&M University, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia, Tecnologia e Inovacao, the Deutsche Forschungsgemeinschaft and the Collaborating Institutions in the Dark Energy Survey. The DES data management system is supported by the National Science Foundation under Grant No. AST-1138766. The Collaborating Institutions are Argonne National Laboratory, the University of California at Santa Cruz, the University of Cambridge, Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid, the University of Chicago, University College London, the DES-Brazil Consortium, the University of Edinburgh, the Eidgenossische Technische Hochschule (ETH) Zurich, Fermi National Accelerator Laboratory, the University of Illinois at Urbana-Champaign, the Institut de Ciencies de l'Espai (IEEC/CSIC), the Institut de Fisica d'Altes Energies, Lawrence Berkeley National Laboratory, the Ludwig-Maximilians Universitat Munchen and the associated Excellence Cluster Universe, the University of Michigan, the National Optical Astronomy Observatory, the University of Nottingham, The Ohio State University, the University of Pennsylvania, the University of Portsmouth, SLAC National Accelerator Laboratory, Stanford University, the University of Sussex, and Texas A&M University. The DES participants from Spanish institutions are partially supported by MINECO under Grants No. AYA2012-39559, ESP2013-48274, FPA2013-47986, and Centro de Excelencia Severo Ochoa SEV-2012-0234 and SEV-2012-0249.; r Research leading to these results has received funding from the European Research Council under the European Union Seventh Framework Programme (FP7/2007-2013) including ERC grant agreements 240672, 291329, and 306478. This paper has gone through internal review by the DES collaboration. NR 118 TC 8 Z9 8 U1 1 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 6 PY 2016 VL 94 IS 2 AR 022001 DI 10.1103/PhysRevD.94.022001 PG 22 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DR1RJ UT WOS:000379682300001 ER PT J AU Becker, MR Troxel, MA MacCrann, N Krause, E Eifler, TF Friedrich, O Nicola, A Refregier, A Amara, A Bacon, D Bernstein, GM Bonnett, C Bridle, SL Busha, MT Chang, C Dodelson, S Erickson, B Evrard, AE Frieman, J Gaztanaga, E Gruen, D Hartley, W Jain, B Jarvis, M Kacprzak, T Kirk, D Kravtsov, A Leistedt, B Peiris, HV Rykoff, ES Sabiu, C Sanchez, C Seo, H Sheldon, E Wechsler, RH Zuntz, J Abbott, T Abdalla, FB Allam, S Armstrong, R Banerji, M Bauer, AH Benoit-Levy, A Bertin, E Brooks, D Buckley-Geer, E Burke, DL Capozzi, D Rosell, AC Kind, MC Carretero, J Castander, FJ Crocce, M Cunha, CE D'Andrea, CB da Costa, LN DePoy, DL Desai, S Diehl, HT Dietrich, JP Doel, P Neto, AF Fernandez, E Finley, DA Flaugher, B Fosalba, P Gerdes, DW Gruendl, RA Gutierrez, G Honscheid, K James, DJ Kuehn, K Kuropatkin, N Lahav, O Li, TS Lima, M Maia, MAG March, M Martini, P Melchior, P Miller, CJ Miquel, R Mohr, JJ Nichol, RC Nord, B Ogando, R Plazas, AA Reil, K Romer, AK Roodman, A Sako, M Sanchez, E Scarpine, V Schubnell, M Sevilla-Noarbe, I Smith, RC Soares-Santos, M Sobreira, F Suchyta, E Swanson, MEC Tarle, G Thaler, J Thomas, D Vikram, V Walker, AR AF Becker, M. R. Troxel, M. A. MacCrann, N. Krause, E. Eifler, T. F. Friedrich, O. Nicola, A. Refregier, A. Amara, A. Bacon, D. Bernstein, G. M. Bonnett, C. Bridle, S. L. Busha, M. T. Chang, C. Dodelson, S. Erickson, B. Evrard, A. E. Frieman, J. Gaztanaga, E. Gruen, D. Hartley, W. Jain, B. Jarvis, M. Kacprzak, T. Kirk, D. Kravtsov, A. Leistedt, B. Peiris, H. V. Rykoff, E. S. Sabiu, C. Sanchez, C. Seo, H. Sheldon, E. Wechsler, R. H. Zuntz, J. Abbott, T. Abdalla, F. B. Allam, S. Armstrong, R. Banerji, M. Bauer, A. H. Benoit-Levy, A. Bertin, E. Brooks, D. Buckley-Geer, E. Burke, D. L. Capozzi, D. Carnero Rosell, A. Kind, M. Carrasco Carretero, J. Castander, F. J. Crocce, M. Cunha, C. E. D'Andrea, C. B. da Costa, L. N. DePoy, D. L. Desai, S. Diehl, H. T. Dietrich, J. P. Doel, P. Fausti Neto, A. Fernandez, E. Finley, D. A. Flaugher, B. Fosalba, P. Gerdes, D. W. Gruendl, R. A. Gutierrez, G. Honscheid, K. James, D. J. Kuehn, K. Kuropatkin, N. Lahav, O. Li, T. S. Lima, M. Maia, M. A. G. March, M. Martini, P. Melchior, P. Miller, C. J. Miquel, R. Mohr, J. J. Nichol, R. C. Nord, B. Ogando, R. Plazas, A. A. Reil, K. Romer, A. K. Roodman, A. Sako, M. Sanchez, E. Scarpine, V. Schubnell, M. Sevilla-Noarbe, I. Smith, R. C. Soares-Santos, M. Sobreira, F. Suchyta, E. Swanson, M. E. C. Tarle, G. Thaler, J. Thomas, D. Vikram, V. Walker, A. R. CA Dark Energy Survey Collaboration TI Cosmic shear measurements with Dark Energy Survey Science Verification data SO PHYSICAL REVIEW D LA English DT Article ID WEAK LENSING SURVEYS; POLARIZATION POWER SPECTRA; GALAXY SHAPE MEASUREMENT; LARGE-SCALE STRUCTURE; COVARIANCE-MATRIX; DISTANT GALAXIES; NOISE BIAS; STATISTICS; IMPACT; SIMULATIONS AB We present measurements of weak gravitational lensing cosmic shear two-point statistics using Dark Energy Survey Science Verification data. We demonstrate that our results are robust to the choice of shear measurement pipeline, either NGMIX or IM3SHAPE, and robust to the choice of two-point statistic, including both real and Fourier-space statistics. Our results pass a suite of null tests including tests for B-mode contamination and direct tests for any dependence of the two-point functions on a set of 16 observing conditions and galaxy properties, such as seeing, airmass, galaxy color, galaxy magnitude, etc. We furthermore use a large suite of simulations to compute the covariance matrix of the cosmic shear measurements and assign statistical significance to our null tests. We find that our covariance matrix is consistent with the halo model prediction, indicating that it has the appropriate level of halo sample variance. We compare the same jackknife procedure applied to the data and the simulations in order to search for additional sources of noise not captured by the simulations. We find no statistically significant extra sources of noise in the data. The overall detection significance with tomography for our highest source density catalog is 9.7 sigma. Cosmological constraints from the measurements in this work are presented in a companion paper. C1 [Becker, M. R.; Busha, M. T.; Wechsler, R. H.] Stanford Univ, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94305 USA. [Becker, M. R.; Krause, E.; Busha, M. T.; Rykoff, E. S.; Wechsler, R. H.; Burke, D. L.; Cunha, C. E.; Reil, K.; Roodman, A.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, POB 2450, Stanford, CA 94305 USA. [Troxel, M. A.; MacCrann, N.; Bridle, S. L.; Zuntz, J.] Univ Manchester, Sch Phys & Astron, Ctr Astrophys, Jodrell Bank, Oxford Rd, Manchester M13 9PL, Lancs, England. [Eifler, T. F.; Bernstein, G. M.; Jain, B.; Jarvis, M.; March, M.; Sako, M.] Univ Penn, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Eifler, T. F.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Friedrich, O.; Gruen, D.; Mohr, J. J.] Max Planck Inst Extraterr Phys, Giessenbachstr, D-85748 Garching, Germany. [Friedrich, O.; Gruen, D.; Dietrich, J. P.] Univ Munich, Fak Phys, Univ Sternwarte, Scheinerstr 1, D-81679 Munich, Germany. [Nicola, A.; Refregier, A.; Amara, A.; Chang, C.; Hartley, W.; Kacprzak, T.] ETH, Dept Phys, Wolfgang Pauli Str 16, CH-8093 Zurich, Switzerland. [Bacon, D.; Capozzi, D.; D'Andrea, C. B.; Nichol, R. C.; Thomas, D.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [Bonnett, C.; Sanchez, C.; Carretero, J.; Fernandez, E.; Miquel, R.] Univ Autonoma Barcelona, Inst Fis Altes Energies, E-08193 Barcelona, Spain. [Dodelson, S.; Frieman, J.; Allam, S.; Buckley-Geer, E.; Diehl, H. T.; Finley, D. A.; Flaugher, B.; Gutierrez, G.; Kuropatkin, N.; Nord, B.; Scarpine, V.; Soares-Santos, M.; Sobreira, F.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Dodelson, S.; Frieman, J.; Kravtsov, A.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Erickson, B.; Evrard, A. E.; Gerdes, D. W.; Miller, C. J.; Schubnell, M.; Tarle, G.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Evrard, A. E.; Miller, C. J.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Gaztanaga, E.; Bauer, A. H.; Carretero, J.; Castander, F. J.; Crocce, M.; Fosalba, P.] IEEC CSIC, Inst Ciencies Espai, Campus UAB,Carrer Can Magrans S-N, Barcelona 08193, Spain. [Kirk, D.; Leistedt, B.; Peiris, H. V.; Abdalla, F. B.; Benoit-Levy, A.; Brooks, D.; Doel, P.; Lahav, O.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Rykoff, E. S.; Wechsler, R. H.; Burke, D. L.; Reil, K.; Roodman, A.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Sabiu, C.] Korea Astron & Space Sci Inst, Daejeon 305348, South Korea. [Seo, H.; Honscheid, K.; Melchior, P.; Suchyta, E.] Ohio State Univ, Dept Phys, 174 W 18th Ave, Columbus, OH 43210 USA. [Sheldon, E.] Brookhaven Natl Lab, Bldg 510, Upton, NY 11973 USA. [Abbott, T.; James, D. J.; Smith, R. C.; Walker, A. R.] Natl Opt Astron Observ, Cerro Tololo Interamer Observ, Casilla 603, La Serena, Chile. [Abdalla, F. B.] Rhodes Univ, Dept Phys & Elect, POB 94, ZA-6140 Grahamstown, South Africa. [Armstrong, R.] Princeton Univ, Dept Astrophys Sci, Peyton Hall, Princeton, NJ 08544 USA. [Banerji, M.] Univ Cambridge, Inst Astron, Madingley Rd, Cambridge CB3 0HA, England. [Banerji, M.] Univ Cambridge, Kavli Inst Cosmol, Madingley Rd, Cambridge CB3 0HA, England. [Bertin, E.] CNRS, UMR 7095, Inst Astrophys Paris, F-75014 Paris, France. [Bertin, E.] Univ Paris 06, Sorbonne Univ, Inst Astrophys Paris, UMR 7095, F-75014 Paris, France. [Carnero Rosell, A.; da Costa, L. N.; Fausti Neto, A.; Lima, M.; Maia, M. A. G.; Ogando, R.; Sobreira, F.] Lab Interinst E Astron LIneA, Rua Gal Jose Cristino 77, BR-20921400 Rio De Janeiro, RJ, Brazil. [Carnero Rosell, A.; da Costa, L. N.; Maia, M. A. G.; Ogando, R.] Observ Nacl, Rua Gal Jose Cristino 77, BR-20921400 Rio De Janeiro, RJ, Brazil. [Kind, M. Carrasco; Gruendl, R. A.; Sevilla-Noarbe, I.] Univ Illinois, Dept Astron, 1002 W Green St, Urbana, IL 61801 USA. [Kind, M. Carrasco; Gruendl, R. A.; Swanson, M. E. C.] Natl Ctr Supercomp Applicat, 1205 West Clark St, Urbana, IL 61801 USA. [DePoy, D. L.; Li, T. S.] Texas A&M Univ, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [DePoy, D. L.; Li, T. S.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Desai, S.; Mohr, J. J.] Univ Munich, Fac Phys, Scheinerstr 1, D-81679 Munich, Germany. [Desai, S.; Dietrich, J. P.; Mohr, J. J.] Excellence Cluster Universe, Boltzmannstr 2, D-85748 Garching, Germany. [Honscheid, K.; Martini, P.; Melchior, P.; Suchyta, E.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Kuehn, K.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Lima, M.] Univ Sao Paulo, Inst Fis, Dept Fis Matemat, CP 66318, BR-05314970 Sao Paulo, SP, Brazil. [Martini, P.] Ohio State Univ, Dept Astron, Columbus, OH 43210 USA. [Miquel, R.] Inst Catalana Recerca & Estudis Avancats, E-08010 Barcelona, Spain. [Plazas, A. A.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Romer, A. K.] Univ Sussex, Dept Phys & Astron, Pevensey Bldg, Brighton BN1 9QH, E Sussex, England. [Sanchez, E.; Sevilla-Noarbe, I.] Ctr Invest Energet Medioambientales & Tecnol CIEM, Madrid, Spain. [Thaler, J.] Univ Illinois, Dept Phys, 1110 W Green St, Urbana, IL 61801 USA. [Thomas, D.] Www Sepnet Ac Uk, South East Phys Network, SEPnet, Southampton, Hants, England. [Vikram, V.] Argonne Natl Lab, 9700 South Cass Ave, Lemont, IL 60439 USA. RP Becker, MR (reprint author), Stanford Univ, Dept Phys, 382 Via Pueblo Mall, Stanford, CA 94305 USA.; Becker, MR (reprint author), Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, POB 2450, Stanford, CA 94305 USA. EM beckermr@stanford.edu RI Lima, Marcos/E-8378-2010; Ogando, Ricardo/A-1747-2010; Sobreira, Flavia/F-4168-2015; Fernandez, Enrique/L-5387-2014; Gaztanaga, Enrique/L-4894-2014; OI Ogando, Ricardo/0000-0003-2120-1154; Sobreira, Flavia/0000-0002-7822-0658; Fernandez, Enrique/0000-0002-6405-9488; Gaztanaga, Enrique/0000-0001-9632-0815; Abdalla, Filipe/0000-0003-2063-4345 FU University of Chicago Research Computing Center; National Science Foundation [ACI-1053575, AST-1138766]; European Research Council [240672]; DOE SciDAC grant; SFB-Transregio 33 "The Dark Universe" by the Deutsche Forschungsgemeinaft (DFG); DFG cluster of excellence "Origin and Structure of the Universe"; Swiss National Foundation [20021_14944, 20021_1439606]; NSF [AST-0812790, AST-1138729]; DoE [DE-SC0007901]; FAPESP; CNPq; NASA Astrophysics Data System; U.S. Department of Energy; U.S. National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Center for Cosmology and Astro-Particle Physics at the Ohio State University; Mitchell Institute for Fundamental Physics and Astronomy at Texas AM University; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia e Tecnologia; Deutsche Forschungsgemeinschaft; Collaborating Institutions in the Dark Energy Survey; MINECO [AYA2012-39559, ESP2013-48274, FPA2013-47986]; Centro de Excelencia Severo Ochoa [SEV-2012-0234]; ERDF funds from European Union; [NSF-AST-1211838] FX We are grateful for the extraordinary contributions of our CTIO colleagues and the DECam Construction, Commissioning and Science Verification teams in achieving the excellent instrument and telescope conditions that have made this work possible. The success of this project also relies critically on the expertise and dedication of the DES Data Management group. M. R. B. is grateful for the support of the University of Chicago Research Computing Center, and especially Doug Rudd, for the time used to carry out the N-body simulations carried out in this work. M. R. B. would also like to thank Stewart Marshall for his ongoing assistance in using SLAC computing resources. This work used the Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation grant number ACI-1053575. J. A. Z., M. A. T., S. L. B. acknowledge support from the European Research Council in the form of a Starting Grant with number 240672. M. R. B. and R. H. W. received partial support from NSF-AST-1211838 and from a DOE SciDAC grant. O. F. and D. G. were supported by SFB-Transregio 33 "The Dark Universe" by the Deutsche Forschungsgemeinaft (DFG) and the DFG cluster of excellence "Origin and Structure of the Universe." A.A., A.R., A.N. are supported in part by Grants No. 20021_14944 and No. 20021_1439606 from the Swiss National Foundation. Jarvis has been supported on this project by NSF Grants No. AST-0812790 and No. AST-1138729. Jarvis, Bernstein, and Jain are partially supported by DoE grant DE-SC0007901. M. L. is partially supported by FAPESP and CNPq. This work made extensive use of the NASA Astrophysics Data System and arXiv.org preprint server. Funding for the DES Projects has been provided by the U.S. Department of Energy, the U.S. National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, the Center for Cosmology and Astro-Particle Physics at the Ohio State University, the Mitchell Institute for Fundamental Physics and Astronomy at Texas A&M University, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia e Tecnologia, the Deutsche Forschungsgemeinschaft and the Collaborating Institutions in the Dark Energy Survey. The DES data management system is supported by the National Science Foundation under Grant Number AST-1138766. The DES participants from Spanish institutions are partially supported by MINECO under grants AYA2012-39559, ESP2013-48274, FPA2013-47986, and Centro de Excelencia Severo Ochoa SEV-2012-0234, some of which include ERDF funds from the European Union.; r The Collaborating Institutions are Argonne National Laboratory, the University of California at Santa Cruz, the University of Cambridge, Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas-Madrid, the University of Chicago, University College London, the DES-Brazil Consortium, the Eidgenossische Technische Hochschule (ETH) Zurich, Fermi National Accelerator Laboratory, the University of Edinburgh, the University of Illinois at Urbana-Champaign, the Institut de Ciencies de l'Espai (IEEC/CSIC), the Institut de Fisica d'Altes Energies, Lawrence Berkeley National Laboratory, the Ludwig-Maximilians Universitat and the associated Excellence Cluster Universe, the University of Michigan, the National Optical Astronomy Observatory, the University of Nottingham, The Ohio State University, the University of Pennsylvania, the University of Portsmouth, SLAC National Accelerator Laboratory, Stanford University, the University of Sussex, and Texas A&M University. This paper is Fermilab publication FERMILAB-PUB-15-303-AE and DES publication DES-2015-0061. This paper has gone through internal review by the DES collaboration. NR 78 TC 16 Z9 16 U1 1 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 6 PY 2016 VL 94 IS 2 AR 022002 DI 10.1103/PhysRevD.94.022002 PG 24 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DR1RJ UT WOS:000379682300002 ER PT J AU Bousso, R AF Bousso, Raphael TI Asymptotic entropy bounds SO PHYSICAL REVIEW D LA English DT Article ID BLACK-HOLES; 2ND LAW AB We show that known entropy bounds constrain the information carried off by radiation to null infinity. We consider distant, planar null hypersurfaces in asymptotically flat spacetime. Their focusing and area loss can be computed perturbatively on a Minkowski background, yielding entropy bounds in terms of the energy flux of the outgoing radiation. In the asymptotic limit, we obtain boundary versions of the quantum null energy condition, of the generalized Second Law, and of the quantum Bousso bound. C1 [Bousso, Raphael] Univ Calif Berkeley, Ctr Theoret Phys, Berkeley, CA 94720 USA. [Bousso, Raphael] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Bousso, Raphael] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Bousso, R (reprint author), Univ Calif Berkeley, Ctr Theoret Phys, Berkeley, CA 94720 USA.; Bousso, R (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA.; Bousso, R (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM bousso@lbl.gov FU Berkeley Center for Theoretical Physics; National Science Foundation [1214644, 1521446, 1316783]; FQXi; U.S. Department of Energy [DE-AC02-05CH11231] FX It is a pleasure to thank Andy Strominger for discussions and initial collaboration; see Ref. [23] for related work by Kapec, Raclariu, and Strominger. I also thank H. Casini, Z. Fisher, E. Flanagan, I. Halpern, G. Horowitz, D. Kapec, J. Koeller, J. Maldacena, and R. Wald for discussions and correspondence. I am grateful to Z. Fisher for producing Fig. 2 and to N. Engelhardt, E. Flanagan, A. Wall, and R. Wald for helpful comments on a draft. This work was supported in part by the Berkeley Center for Theoretical Physics, by the National Science Foundation (Grants No. 1214644, No. 1521446, and No. 1316783), by FQXi, and by the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 33 TC 1 Z9 1 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 6 PY 2016 VL 94 IS 2 AR 024018 DI 10.1103/PhysRevD.94.024018 PG 11 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DR1RJ UT WOS:000379682300014 ER PT J AU Davoudiasl, H Giardino, PP Zhang, C AF Davoudiasl, Hooman Giardino, Pier Paolo Zhang, Cen TI Higgs-like boson at 750 GeV and genesis of baryons SO PHYSICAL REVIEW D LA English DT Article ID DIPHOTON EXCESS; VIOLATION AB We propose that the diphoton excess at 750 GeV reported by ATLAS and CMS is due to the decay of an exo-Higgs scalar eta associated with the breaking of a new SU(2)(e) symmetry, dubbed exo-spin. New fermions, exo-quarks and exo-leptons, get TeV-scale masses through Yukawa couplings with eta and generate its couplings to gluons and photons at one loop. The matter content of our model yields a B - L anomaly under SU(2)(e), whose breaking we assume entails a first-order phase transition. A nontrivial B - L asymmetry may therefore be generated in the early Universe, potentially providing a baryogenesis mechanism through the Standard Model (SM) sphaleron processes. The spontaneous breaking of SU(2)(e) can, in principle, directly lead to electroweak symmetry breaking, thereby accounting for the proximity of the mass scales of the SM Higgs and the exo-Higgs. Our model can be distinguished from those comprising a singlet scalar and vector fermions by the discovery of TeV scale exo-vector bosons, corresponding to the broken SU(2)(e) generators, at the LHC. C1 [Davoudiasl, Hooman; Giardino, Pier Paolo; Zhang, Cen] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. RP Davoudiasl, H (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. EM hooman@bnl.gov; pgiardino@bnl.gov; cenzhang@bnl.gov FU United States Department of Energy [DE-SC0012704] FX We would like to thank Frank Paige for valuable discussions on collider signals. This work is supported in part by the United States Department of Energy under Grant No. DE-SC0012704. NR 34 TC 1 Z9 1 U1 3 U2 4 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 6 PY 2016 VL 94 IS 1 AR 015006 DI 10.1103/PhysRevD.94.015006 PG 8 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DR1QT UT WOS:000379680700007 ER PT J AU Bechtold, A Li, F Muller, K Simmet, T Ardelt, PL Finley, JJ Sinitsyn, NA AF Bechtold, A. Li, F. Mueller, K. Simmet, T. Ardelt, P-L. Finley, J. J. Sinitsyn, N. A. TI Quantum Effects in Higher-Order Correlators of a Quantum-Dot Spin Qubit SO PHYSICAL REVIEW LETTERS LA English DT Article ID LEGGETT-GARG INEQUALITY; ELECTRON-SPIN; VIOLATION; MECHANICS AB We measure time correlators of a spin qubit in an optically active quantum dot beyond the second order. Such higher-order correlators are shown to be directly sensitive to pure quantum effects that cannot be explained within the classical framework. They allow direct determination of ensemble and quantum dephasing times, T-2* and T-2, using only repeated projective measurements and without the need for coherent spin control. Our method enables studies of purely quantum behavior in solid state systems, including tests of the Leggett-Garg type of inequalities that rule out local hidden variable interpretation of the quantum-dot spin dynamics. C1 [Bechtold, A.; Mueller, K.; Simmet, T.; Ardelt, P-L.; Finley, J. J.] Tech Univ Munich, Walter Schottky Inst, D-85748 Garching, Germany. [Bechtold, A.; Mueller, K.; Simmet, T.; Ardelt, P-L.; Finley, J. J.] Tech Univ Munich, Phys Dept, D-85748 Garching, Germany. [Li, F.] Los Alamos Natl Lab, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. [Li, F.; Sinitsyn, N. A.] Los Alamos Natl Lab, Theoret Div, Los Alamos, NM 87545 USA. [Mueller, K.] Stanford Univ, EL Ginzton Lab, Stanford, CA 94305 USA. RP Finley, JJ (reprint author), Tech Univ Munich, Walter Schottky Inst, D-85748 Garching, Germany.; Finley, JJ (reprint author), Tech Univ Munich, Phys Dept, D-85748 Garching, Germany. EM jonathan.finley@wsi.tum.de; nsinitsyn@lanl.gov RI Li, Fuxiang/O-9132-2015 FU DFG [SFB-631]; EU; Alexander von Humboldt Foundation; ARO [W911NF-13-1-0309]; U.S. Department of Energy [DE-AC52-06NA25396]; LDRD program at LANL FX We gratefully acknowledge financial support from the DFG via SFB-631, Nanosystems Initiative Munich, the EU via S3 Nano and BaCaTeC. K. M. acknowledges financial support from the Alexander von Humboldt Foundation and the ARO (Grant No. W911NF-13-1-0309). Work at LANL was supported by the U.S. Department of Energy, Contract No. DE-AC52-06NA25396, and the LDRD program at LANL. NR 33 TC 1 Z9 1 U1 5 U2 6 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 6 PY 2016 VL 117 IS 2 AR 027402 DI 10.1103/PhysRevLett.117.027402 PG 5 WC Physics, Multidisciplinary SC Physics GA DR2IO UT WOS:000379728400012 PM 27447523 ER PT J AU Drozdetski, AV Tolokh, IS Pollack, L Baker, N Onufriev, AV AF Drozdetski, Aleksander V. Tolokh, Igor S. Pollack, Lois Baker, Nathan Onufriev, Alexey V. TI Opposing Effects of Multivalent Ions on the Flexibility of DNA and RNA SO PHYSICAL REVIEW LETTERS LA English DT Article ID MOLECULAR-DYNAMICS SIMULATIONS; DOUBLE-STRANDED-RNA; ELECTROSTATIC PERSISTENCE LENGTH; NUCLEIC-ACIDS; FORCE-FIELD; B-DNA; CONDENSATION; HELIX; SALT; POLYELECTROLYTES AB Increasing the concentration of counterions (salt) is known to reduce the bending persistence length of DNA. Here we use atomistic molecular dynamics simulations to predict that multivalent counterions have the opposite effect on double-stranded RNA, increasing its bending rigidity by at least 30%. This counterintuitive effect is observed for various tri- and tetravalent ions alike, and is robust to methodological details and the RNA sequence. In contrast to DNA, multivalent counterions bind inside the RNA major groove, causing significant contraction of the molecule along its helical axis-as a result, its further deformation due to bending becomes energetically more expensive compared to bending without bound multivalent ions. Thus, the relationship between mechanical properties of a charged polymer and its ionic atmosphere may be richer than previously thought. C1 [Drozdetski, Aleksander V.; Onufriev, Alexey V.] Virginia Tech, Dept Phys, Blacksburg, VA 24061 USA. [Tolokh, Igor S.; Onufriev, Alexey V.] Virginia Tech, Dept Comp Sci, Blacksburg, VA 24061 USA. [Pollack, Lois] Cornell Univ, Sch Appl & Engn Phys, Ithaca, NY 14853 USA. [Baker, Nathan] Pacific Northwest Natl Lab, Adv Comp Math & Data Div, Richland, WA 99352 USA. [Baker, Nathan] Brown Univ, Div Appl Math, Providence, RI 02912 USA. [Onufriev, Alexey V.] Virginia Tech, Ctr Soft Matter & Biol Phys, Blacksburg, VA 24061 USA. RP Drozdetski, AV (reprint author), Virginia Tech, Dept Phys, Blacksburg, VA 24061 USA. FU National Institutes of Health (NIH) [R01 GM099450] FX We thank Dr. Suzette Pabit for helpful discussions. This work was supported by the National Institutes of Health (NIH) R01 GM099450. The authors acknowledge Advanced Research Computing at Virginia Tech for providing computational resources. NR 47 TC 3 Z9 4 U1 7 U2 15 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 0031-9007 EI 1079-7114 J9 PHYS REV LETT JI Phys. Rev. Lett. PD JUL 6 PY 2016 VL 117 IS 2 AR 028101 DI 10.1103/PhysRevLett.117.028101 PG 5 WC Physics, Multidisciplinary SC Physics GA DR2IO UT WOS:000379728400014 PM 27447528 ER PT J AU He, YM Sobhani, A Lei, SD Zhang, ZH Gong, YJ Jin, ZH Zhou, W Yang, YC Zhang, Y Wang, XF Yakobson, B Vajtai, R Halas, NJ Li, B Xie, EQ Ajayan, P AF He, Yongmin Sobhani, Ali Lei, Sidong Zhang, Zhuhua Gong, Yongji Jin, Zehua Zhou, Wu Yang, Yingchao Zhang, Yuan Wang, Xifan Yakobson, Boris Vajtai, Robert Halas, Naomi J. Li, Bo Xie, Erqing Ajayan, Pulickel TI Layer Engineering of 2D Semiconductor Junctions SO ADVANCED MATERIALS LA English DT Article ID TRANSITION-METAL DICHALCOGENIDES; P-N-JUNCTIONS; 2-DIMENSIONAL MATERIALS; MOS2 TRANSISTORS; MONOLAYER; HETEROSTRUCTURES; PHOTOLUMINESCENCE; ELECTRONICS; GRAPHENE; DEVICES AB A new concept for junction fabrication by connecting multiple regions with varying layer thicknesses, based on the thickness dependence, is demonstrated. This type of junction is only possible in super-thin-layered 2D materials, and exhibits similar characteristics as p-n junctions. Rectification and photovoltaic effects are observed in chemically homogeneous MoSe2 junctions between domains of different thicknesses. C1 [He, Yongmin; Lei, Sidong; Zhang, Zhuhua; Jin, Zehua; Yang, Yingchao; Zhang, Yuan; Wang, Xifan; Yakobson, Boris; Vajtai, Robert; Li, Bo; Ajayan, Pulickel] Rice Univ, Dept Mat Sci & NanoEngn, Houston, TX 77005 USA. [He, Yongmin; Xie, Erqing] Lanzhou Univ, Sch Phys Sci & Technol, Lanzhou 730000, Gansu, Peoples R China. [Sobhani, Ali; Halas, Naomi J.] Rice Univ, Dept Elect & Comp Engn, Houston, TX 77005 USA. [Zhang, Zhuhua] Nanjing Univ Aeronaut & Astronaut, State Key Lab Mech & Control Mech Struct, Key Lab Intelligent Nano Mat & Devices, Minist Educ, Nanjing 210016, Jiangsu, Peoples R China. [Gong, Yongji] Rice Univ, Dept Chem, POB 1892, Houston, TX 77005 USA. [Zhou, Wu] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. RP Li, B; Ajayan, P (reprint author), Rice Univ, Dept Mat Sci & NanoEngn, Houston, TX 77005 USA.; Xie, EQ (reprint author), Lanzhou Univ, Sch Phys Sci & Technol, Lanzhou 730000, Gansu, Peoples R China. EM Bo.Li@rice.edu; xieeq@lzu.edu.cn; ajayan@rice.edu RI Gong, Yongji/L-7628-2016; Zhou, Wu/D-8526-2011; Zhang, Zhuhua/E-8162-2012; Lei, Sidong/A-8600-2016; OI Zhou, Wu/0000-0002-6803-1095; Lei, Sidong/0000-0001-9129-2202; Xie, Erqing/0000-0001-5647-6938 FU FAME, STARnet; Semiconductor Research Corporation program - MARCO; DARPA; China Scholarship Council; Fundamental Research Funds for the Central Universities in China [lzujbky-2015-303]; U.S. Department of Energy, Office of Science, Basic Energy Science, Materials Sciences and Engineering Division; ORNL's Center for Nanophase Materials Sciences (CNMS), DOE Office of Science User Facility FX This work was supported by FAME, one of the six centers of STARnet, a Semiconductor Research Corporation program sponsored by MARCO and DARPA. Y.H. acknowledges the financial support from China Scholarship Council. This work was also supported by the Fundamental Research Funds for the Central Universities in China (lzujbky-2015-303). Electron microscopy study was supported by the U.S. Department of Energy, Office of Science, Basic Energy Science, Materials Sciences and Engineering Division (W.Z.), and through a user project at ORNL's Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. NR 34 TC 2 Z9 2 U1 31 U2 94 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0935-9648 EI 1521-4095 J9 ADV MATER JI Adv. Mater. PD JUL 6 PY 2016 VL 28 IS 25 BP 5126 EP 5132 DI 10.1002/adma.201600278 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DQ1DA UT WOS:000378940100023 PM 27136275 ER PT J AU Damodaran, AR Agar, JC Pandya, S Chen, ZH Dedon, L Xu, RJ Apgar, B Saremi, S Martin, LW AF Damodaran, Anoop R. Agar, Joshua C. Pandya, Shishir Chen, Zuhuang Dedon, Liv Xu, Ruijuan Apgar, Brent Saremi, Sahar Martin, Lane W. TI New modalities of strain-control of ferroelectric thin films SO JOURNAL OF PHYSICS-CONDENSED MATTER LA English DT Review DE ferroelectrics; thin films; epitaxy; strain ID ATOMIC LAYER DEPOSITION; DOMAIN-WALL MOTION; ARTIFICIAL BATIO3/SRTIO3 SUPERLATTICES; ENHANCED ELECTROMECHANICAL RESPONSE; DEGENERATE ELECTRONIC STATES; NEUTRON POWDER DIFFRACTION; FERROIC PHASE-TRANSITIONS; BARIUM STRONTIUM-TITANATE; EPITAXIAL BATIO3 FILMS; LEAD MAGNESIUM NIOBATE AB Ferroelectrics, with their spontaneous switchable electric polarization and strong coupling between their electrical, mechanical, thermal, and optical responses, provide functionalities crucial for a diverse range of applications. Over the past decade, there has been significant progress in epitaxial strain engineering of oxide ferroelectric thin films to control and enhance the nature of ferroelectric order, alter ferroelectric susceptibilities, and to create new modes of response which can be harnessed for various applications. This review aims to cover some of the most important discoveries in strain engineering over the past decade and highlight some of the new and emerging approaches for strain control of ferroelectrics. We discuss how these new approaches to strain engineering provide promising routes to control and decouple ferroelectric susceptibilities and create new modes of response not possible in the confines of conventional strain engineering. To conclude, we will provide an overview and prospectus of these new and interesting modalities of strain engineering helping to accelerate their widespread development and implementation in future functional devices. C1 [Damodaran, Anoop R.; Agar, Joshua C.; Pandya, Shishir; Chen, Zuhuang; Dedon, Liv; Xu, Ruijuan; Apgar, Brent; Saremi, Sahar; Martin, Lane W.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Chen, Zuhuang; Martin, Lane W.] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Martin, LW (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. EM lwmartin@berkeley.edu RI Martin, Lane/H-2409-2011; Chen, Zuhuang/E-7131-2011 OI Martin, Lane/0000-0003-1889-2513; Chen, Zuhuang/0000-0003-1912-6490 FU Army Research Office [W911NF-14-1-0104]; Department of Energy [DE-SC0012375]; National Science Foundation [DMR-1124696, DMR-1451219, CMMI-1434147, OISE-1545907]; Office of Naval Research [N00014-10-1-0525]; Air Force Office of Scientific Research [FA9550-12-1-0471] FX The authors acknowledges support from the Army Research Office under grant W911NF-14-1-0104, the Department of Energy under grant DE-SC0012375, the National Science Foundation under grants DMR-1124696, DMR-1451219, CMMI-1434147, and OISE-1545907, the Office of Naval Research under grant N00014-10-1-0525, and the Air Force Office of Scientific Research under grant FA9550-12-1-0471. The authors have benefited from numerous collaborations within the programs at the University of California, Berkeley and the University of Illinois, Urbana-Champaign as well as numerous other valued collaborators around the world. NR 664 TC 4 Z9 4 U1 45 U2 86 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0953-8984 EI 1361-648X J9 J PHYS-CONDENS MAT JI J. Phys.-Condes. Matter PD JUL 6 PY 2016 VL 28 IS 26 AR 263001 DI 10.1088/0953-8984/28/26/263001 PG 36 WC Physics, Condensed Matter SC Physics GA DQ0ZH UT WOS:000378929800001 PM 27187744 ER PT J AU Arciniegas, MP Di Stasio, F Li, HB Altamura, D De Trizio, L Prato, M Scarpellini, A Moreels, I Krahne, R Manna, L AF Arciniegas, Milena P. Di Stasio, Francesco Li, Hongbo Altamura, Davide De Trizio, Luca Prato, Mirko Scarpellini, Alice Moreels, Iwan Krahne, Roman Manna, Liberato TI Self-Assembled Dense Colloidal Cu2Te Nanodisk Networks in P3HT Thin Films with Enhanced Photocurrent SO ADVANCED FUNCTIONAL MATERIALS LA English DT Article DE hexagonal nanodisks; nanocomposites; photocurrent; polymers; self-assembly ID HETEROJUNCTION SOLAR-CELLS; POLYMER; NANOCRYSTALS; NANOCOMPOSITES; PHOTODETECTORS; NANOPARTICLES; PERFORMANCE; POLY(3-HEXYLTHIOPHENE); PHOTOMULTIPLICATION; NANOSTRUCTURES AB The integration of colloidal nanocrystals with polymers adds optoelectronic functionalities to flexible and mechanically robust organic films. In particular, self-assembled structures of nanocrystals in polymers can act as functional components enhancing, for instance, transport or optical properties of the hybrid material. This study presents Cu2Te hexagonal nanodisks that assemble into ribbons with a face-to-face configuration in poly(3-hexylthiophene-2,5-diyl) through a controlled solvent evaporation process. The ribbons form weaving patterns that create 3D networks fully embedded in the thin polymer film at high nanodisk concentration. The photoresponse of these composite films measured in a layered vertical geometry demonstrates increased photocurrent with increasing nanocrystal loading. This study attributes this behavior to the presence of networks of Cu2Te nanodisks that form a bulk heterojunction with the semiconducting polymer, which improves exciton dissociation and the overall photoelectric response. C1 [Arciniegas, Milena P.; Di Stasio, Francesco; Li, Hongbo; De Trizio, Luca; Prato, Mirko; Scarpellini, Alice; Moreels, Iwan; Krahne, Roman; Manna, Liberato] Ist Italiano Tecnol, Via Morego 30, IT-16163 Genoa, Italy. [Altamura, Davide] CNR, Ist Cristallog, Via Amendola 122-O, I-70126 Bari, Italy. [Li, Hongbo] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Arciniegas, MP; Di Stasio, F (reprint author), Ist Italiano Tecnol, Via Morego 30, IT-16163 Genoa, Italy. EM milena.arciniegas@iit.it; francesco.distasio@iit.it RI Di Stasio, Francesco/F-4536-2011; Moreels, Iwan/E-5230-2011; Manna, Liberato/G-2339-2010; Prato, Mirko/D-8531-2012 OI Di Stasio, Francesco/0000-0002-2079-3322; Moreels, Iwan/0000-0003-3998-7618; Manna, Liberato/0000-0003-4386-7985; Prato, Mirko/0000-0002-2188-8059 FU European Union through the ERC [240111] FX MPA and FDS contributed equally to this work. MPA, HL, LDT, MP, AS, and LM acknowledge financial support from European Union through the FP7 starting ERC grant NANO-ARCH (Contract Number 240111). FDS thanks Marco Leoncini for the technical support on the Au film evaporation. MPA and AS thank Rosaria Brescia for the helpful discussion on HAADF-STEM analysis. MPA thanks Sara Accornero for the technical support on the XRD measurments. MPA and DA thank the staff of the XRD2 beamline of the Brazilian LNLS/CNPEM, Dr. Teresa Sibillano and Roberto Lassandro, for their technical support in X-ray scattering experiments. NR 58 TC 3 Z9 3 U1 18 U2 40 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1616-301X EI 1616-3028 J9 ADV FUNCT MATER JI Adv. Funct. Mater. PD JUL 5 PY 2016 VL 26 IS 25 BP 4535 EP 4542 DI 10.1002/adfm.201600751 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter SC Chemistry; Science & Technology - Other Topics; Materials Science; Physics GA DR4XD UT WOS:000379905800012 ER PT J AU Barauskas, D Pelenis, D Virzonis, D Baltrus, JP Baltrusaitis, J AF Barauskas, Dovydas Pelenis, Donatas Virzonis, Darius Baltrus, John P. Baltrusaitis, Jonas TI Greenhouse Gas Molecule CO2 Detection Using a Capacitive Micromachined Ultrasound Transducer SO ANALYTICAL CHEMISTRY LA English DT Article ID SILICON-NITRIDE FILMS; CHEMICAL SENSOR; EMISSIONS; CAPTURE AB We manufactured and tested a capacitive micromachined ultrasound transducer (CMUT)-based sensor for CO2 detection at environmentally relevant concentrations using polyethylenimine as a CO2 binding material. The assembly of a sensing chip was 10 x 20 mm, and up to 5 gases can potentially be detected simultaneously using a masking technique and different sensing materials. The limit of detection was calculated to be 0.033 CO2 vol % while the limit of quantification was calculated to be 0.102%. The sensor exhibited a linear response between 0.06% and 0.30% CO2 while concentrations dose to those in flue gas can also be measured using dilution with inert gas. C1 [Barauskas, Dovydas; Pelenis, Donatas; Virzonis, Darius] Kaunas Univ Technol, Panevezys Inst, Dept Elect Engn, Daukanto 12, LT-35212 Paneveys, Lithuania. [Barauskas, Dovydas; Pelenis, Donatas; Virzonis, Darius] Panevezys Mechatron Ctr, Lab Micro & Nano Technol, Pilenu 30, LT-36239 Paneveys, Lithuania. [Baltrus, John P.] US DOE, Natl Energy Technol Lab, 626 Cochrans Mill Rd, Pittsburgh, PA 15236 USA. [Baltrusaitis, Jonas] Lehigh Univ, Dept Chem & Biomol Engn, B336 Iacocca Hall,111 Res Dr, Bethlehem, PA 18015 USA. RP Baltrusaitis, J (reprint author), Lehigh Univ, Dept Chem & Biomol Engn, B336 Iacocca Hall,111 Res Dr, Bethlehem, PA 18015 USA. EM job314@lehigh.edu FU Lehigh University FX J.B. acknowledges startup funds by Lehigh University. NR 17 TC 0 Z9 0 U1 15 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JUL 5 PY 2016 VL 88 IS 13 BP 6662 EP 6665 DI 10.1021/acs.analchem.6b02085 PG 4 WC Chemistry, Analytical SC Chemistry GA DQ7CF UT WOS:000379363800007 PM 27321769 ER PT J AU Sgarlata, C Raymond, KN AF Sgarlata, Carmelo Raymond, Kenneth N. TI Untangling the Diverse Interior and Multiple Exterior Guest Interactions of a Supramolecular Host by the Simultaneous Analysis of Complementary Observables SO ANALYTICAL CHEMISTRY LA English DT Article ID TRANSITION-METAL CATALYSIS; EQUILIBRIUM-CONSTANTS; LIGAND CLUSTER; ANIONIC HOST; NMR DATA; WATER; RECOGNITION; THERMODYNAMICS; BINDING; ENCAPSULATION AB The entropic and enthalpic driving forces for encapsulation versus sequential exterior guest binding to the [Ga4L6](12-) supramolecular host in solution are very different, which significantly complicates the determination of these thermodynamic parameters. The simultaneous use of complementary techniques, such as NMR, UV-vis, and isothermal titration calorimetry, enables the disentanglement of such multiple host guest interactions. Indeed, data collected by each technique measure different components of the 'host guest equilibria and together provide a complete picture of the solution thermodynamics. Unfortunately, commercially available programs do not allow for global analysis of different physical observables. We thus resorted to a novel procedure for the simultaneous refinement of multiple parameters (Delta G degrees, Delta H degrees, and Delta S degrees) by treating different observables through a weighted nonlinear least-squares analysis of a constrained model. The refinement procedure is discussed for the multiple binding of the Et4N+ guest, but it is broadly applicable to the deconvolution of other intricate host guest equilibria. C1 [Raymond, Kenneth N.] Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. RP Raymond, KN (reprint author), Lawrence Berkeley Natl Lab, Div Chem Sci, Berkeley, CA 94720 USA. EM raymond@socrates.berkeley.edu FU Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL [DE-AC02-05CH11231] FX This research was supported by the Director, Office of Science, Office of Basic Energy Sciences, and the Division of Chemical Sciences, Geosciences, and Biosciences of the U.S. Department of Energy at LBNL (DE-AC02-05CH11231). We thank Dr. Jeff Mugridge, David Kaphan, and Professor Giuseppe Arena for helpful discussions. NR 54 TC 0 Z9 0 U1 10 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0003-2700 EI 1520-6882 J9 ANAL CHEM JI Anal. Chem. PD JUL 5 PY 2016 VL 88 IS 13 BP 6923 EP 6929 DI 10.1021/acs.analchem.6b01684 PG 7 WC Chemistry, Analytical SC Chemistry GA DQ7CF UT WOS:000379363800041 PM 27244346 ER PT J AU Rosa, PFS Oostra, A Thompson, JD Pagliuso, PG Fisk, Z AF Rosa, P. F. S. Oostra, A. Thompson, J. D. Pagliuso, P. G. Fisk, Z. TI Unusual Kondo-hole effect and crystal-field frustration in Nd-doped CeRhIn5 SO PHYSICAL REVIEW B LA English DT Article ID RESISTANCE; LATTICE AB We investigate single crystals of Ce1-xNdxRhIn5 by means of x-ray-diffraction, microprobe, magnetic susceptibility, heat capacity, and electrical resistivity measurements. Our data reveal that the antiferromagnetic transition of CeRhIn5, at T-N(Ce) = 3.8 K, is linearly suppressed with x(Nd). We associate this effect with the presence of a "Kondo hole" created by Nd substitution. The extrapolation of T-N(Ce) to zero temperature, however, occurs at x(c) similar to 0.3, which is below the two-dimensional percolation limit found in Ce1-xLaxRhIn5. This result strongly suggests the presence of a crystal-field induced magnetic frustration. Near x(Nd) similar to 0.2, the Ising antiferromagnetic order from Nd3+ ions is stabilized and T-N(Nd) increases up to 11 K in NdRhIn5. Our results shed light on the effects of magnetic doping in heavy-fermion antiferromagnets and stimulate the study of such systems under applied pressure. C1 [Rosa, P. F. S.; Oostra, A.; Fisk, Z.] Univ Calif Irvine, Irvine, CA 92697 USA. [Rosa, P. F. S.; Thompson, J. D.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Pagliuso, P. G.] Univ Estadual Campinas, Inst Fis Gleb Wataghin, BR-13083859 Campinas, SP, Brazil. RP Rosa, PFS (reprint author), Univ Calif Irvine, Irvine, CA 92697 USA.; Rosa, PFS (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. OI Ferrari Silveira Rosa, Priscila/0000-0002-3437-548X FU U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering; LANL LDRD program; FAPESP [2013/20181-0, 2012/04870-7]; CNPq [442230/2014-1, 304649/2013-9] FX Work at Los Alamos National Laboratory (LANL) was performed under the auspices of the U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Science and Engineering. P.F.S.R. acknowledges a Director's Postdoctoral Fellowship through the LANL LDRD program and FAPESP Grant No. 2013/20181-0. P.G.P. acknowledges FAPESP Grant No. 2012/04870-7 and CNPq Grants No. 442230/2014-1 and No. 304649/2013-9. NR 20 TC 0 Z9 0 U1 5 U2 11 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 5 PY 2016 VL 94 IS 4 AR 045101 DI 10.1103/PhysRevB.94.045101 PG 6 WC Physics, Condensed Matter SC Physics GA DR2EV UT WOS:000379718700004 ER PT J AU Tripathi, V Galda, A Barman, H Vinokur, VM AF Tripathi, Vikram Galda, Alexey Barman, Himadri Vinokur, Valerii M. TI Parity-time symmetry-breaking mechanism of dynamic Mott transitions in dissipative systems SO PHYSICAL REVIEW B LA English DT Article ID HERMITIAN QUANTUM-MECHANICS; METAL-INSULATOR-TRANSITION; DIELECTRIC-BREAKDOWN; DIRECTED PERCOLATION; ENERGY CURRENT; HUBBARD-MODEL; FIELD; LOCALIZATION; SPECTRA; ARRAYS AB We describe the critical behavior of the electric field-driven (dynamic) Mott insulator-to-metal transitions in dissipative Fermi and Bose systems in terms of non-Hermitian Hamiltonians invariant under simultaneous parity (P) and time-reversal (T) operations. The dynamic Mott transition is identified as a PT symmetry-breaking phase transition, with the Mott insulating state corresponding to the regime of unbroken PT symmetry with a real energy spectrum. We establish that the imaginary part of the Hamiltonian arises from the combined effects of the driving field and inherent dissipation. We derive the renormalization and collapse of the Mott gap at the dielectric breakdown and describe the resulting critical behavior of transport characteristics. The obtained critical exponent is in an excellent agreement with experimental findings. C1 [Tripathi, Vikram; Galda, Alexey; Vinokur, Valerii M.] Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA. [Tripathi, Vikram; Barman, Himadri] Tata Inst Fundamental Res, Dept Theoret Phys, Homi Bhabha Rd, Mumbai 400005, Maharashtra, India. RP Tripathi, V (reprint author), Argonne Natl Lab, Div Mat Sci, 9700 S Cass Ave, Argonne, IL 60439 USA.; Tripathi, V (reprint author), Tata Inst Fundamental Res, Dept Theoret Phys, Homi Bhabha Rd, Mumbai 400005, Maharashtra, India. FU U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division (Materials Theory Institute at ANL); University of Chicago Center in Delhi; DST (India) Swarnajayanti grant [DST/SJF/PSA-0212012-13]; DAE (India) FX We thank T. I. Baturina for critical reading of the manuscript and many valuable suggestions, and D. Dhar and T. V. Ramakrishnan for illuminating discussions. The work is supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division (V.T. is partially supported by Materials Theory Institute at ANL), by the University of Chicago Center in Delhi, and DST (India) Swarnajayanti grant (No. DST/SJF/PSA-0212012-13). H.B. is grateful for support from DAE (India) and computational resources from the Department of Theoretical Physics, Tata Institute of Fundamental Research. NR 44 TC 2 Z9 2 U1 3 U2 5 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 5 PY 2016 VL 94 IS 4 AR 041104 DI 10.1103/PhysRevB.94.041104 PG 5 WC Physics, Condensed Matter SC Physics GA DR2EV UT WOS:000379718700002 ER PT J AU Longo, AF Feng, Y Lai, B Landing, WM Shelley, RU Nenes, A Mihalopoulos, N Violaki, K Ingall, ED AF Longo, Amelia F. Feng, Yan Lai, Barry Landing, William M. Shelley, Rachel U. Nenes, Athanasios Mihalopoulos, Nikolaos Violaki, Kalliopi Ingall, Ellery D. TI Influence of Atmospheric Processes on the Solubility and Composition of Iron in Saharan Dust SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID NORTH-AFRICAN DUST; THERMODYNAMIC-EQUILIBRIUM MODEL; MINERAL DUST; MARINE AEROSOLS; SOUTHERN-OCEAN; CHEMICAL-COMPOSITION; PHYTOPLANKTON BLOOM; NUTRIENT-LIMITATION; PARTICULATE MATTER; SULFUR-DIOXIDE AB Aerosol iron was examined in Saharan dust plumes using a combination of iron near-edge X-ray absorption spectroscopy and wet-chemical techniques. Aerosol samples were collected at three sites located in the Mediterranean, the Atlantic, and Bermuda to characterize iron at different atmospheric transport lengths and time scales. Iron(III) oxides were a component of aerosols at all sampling sites and dominated the aerosol iron in Mediterranean samples. In Atlantic samples, iron(II and III) sulfate, iron(III) phosphate, and iron(II) silicates were also contributors to aerosol composition. With increased atmospheric transport time, iron(II) sulfates are found to become more abundant, aerosol iron oxidation state became more reduced, and aerosol acidity increased. Atmospheric processing including acidic reactions and photoreduction likely influence the form of iron minerals and oxidation state in Saharan dust aerosols and contribute to increases in aerosol-iron solubility. C1 [Longo, Amelia F.; Nenes, Athanasios; Ingall, Ellery D.] Georgia Inst Technol, Sch Earth & Atmospher Sci, 311 Ferst Dr, Atlanta, GA 30332 USA. [Nenes, Athanasios] Georgia Inst Technol, Sch Chem & Biomol Engn, 311 Ferst Dr, Atlanta, GA 30332 USA. [Feng, Yan] Argonne Natl Lab, Div Environm Sci, 9700 South Cass Ave, Argonne, IL 60439 USA. [Lai, Barry] Argonne Natl Lab, Adv Photon Source, 9700 South Cass Ave, Argonne, IL 60439 USA. [Landing, William M.; Shelley, Rachel U.] Florida State Univ, Dept Earth Ocean & Atmospher Sci, Tallahassee, FL 32306 USA. [Nenes, Athanasios] Fdn Res & Technol, Patras 70013, Greece. [Nenes, Athanasios; Mihalopoulos, Nikolaos] Natl Observ Athens, GR-15236 Penteli, Greece. [Mihalopoulos, Nikolaos; Violaki, Kalliopi] Univ Crete, Dept Chem, Iraklion 71003, Greece. Inst Univ Europeen Mer, Lab Sci Environm Marin, F-29280 Plouzane, France. RP Ingall, ED (reprint author), Georgia Inst Technol, Sch Earth & Atmospher Sci, 311 Ferst Dr, Atlanta, GA 30332 USA. EM ellery.ingall@eas.gatech.edu FU National Science Foundation [OCE-1357375, OCE-0929919, OCE-1034764]; Argonne National Laboratory under the U.S. Department of Energy [DE-AC02-06CH11357]; European Union; Greek national funds through the Operational Program "Education and Lifelong Learning" of the National Strategic Reference Framework Research Funding Program, ARISTEIA FX This material is based upon work supported by the National Science Foundation under grants OCE-1357375 (EDI), OCE-0929919 (WML), and OCE-1034764 (WML). The data used to produce these results are available upon request to the corresponding author. Any opinions, findings, and conclusions or recommendations expressed in this material are those of the authors and do not necessarily reflect the views of the National Science Foundation. Use of the Advanced Photon Source and support to Y.F. and B.L. are provided by Argonne National Laboratory under the U.S. Department of Energy contract no. DE-AC02-06CH11357. N.M. and KV. acknowledge support from European Union (European Social Fund) and Greek national funds through the Operational Program "Education and Lifelong Learning" of the National Strategic Reference Framework Research Funding Program, ARISTEIA. NR 86 TC 5 Z9 5 U1 15 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 5 PY 2016 VL 50 IS 13 SI SI BP 6912 EP 6920 DI 10.1021/acs.est.6b02605 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DQ7DE UT WOS:000379366300039 PM 27286140 ER PT J AU Zhao, PH Begg, JD Zavarin, M Tumey, SJ Williams, R Dai, ZRR Kips, R Kersting, AB AF Zhao, Pihong Begg, James D. Zavarin, Mavrik Tumey, Scott J. Williams, Ross Dai, Zurong R. Kips, Ruth Kersting, Annie B. TI Plutonium(IV) and (V) Sorption to Goethite at Sub-Femtomolar to Micromolar Concentrations: Redox Transformations and Surface Precipitation SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID NEVADA TEST-SITE; MINERAL SURFACES; OXIDATION-STATE; ILLITE SURFACE; NATURAL-WATERS; FAR-FIELD; GROUNDWATER; REDUCTION; PU(V); ADSORPTION AB Pu(IV) and Pu(V) sorption to goethite was investigated over a concentration range of 10(-15)-10(-5) M at pH 8. Experiments with initial Pu concentrations of 10(-15) - 10(-8) M produced linear Pu sorption isotherms, demonstrating that Pu sorption to goethite is not concentration-dependent across this concentration range. Equivalent Pu(IV) and Pu(V) sorption K-d values obtained at 1 and 2-week sampling time points indicated that Pu(V) is rapidly reduced to Pu(IV) on the goethite surface. Further, it suggested that Pu surface redox transformations are sufficiently rapid to achieve an equilibrium state within 1 week, regardless of the initial Pu oxidation state. At initial concentrations >10(-8) M, both Pu oxidation states exhibited deviations from linear sorption behavior and less Pu was adsorbed than at lower concentrations. NanoSIMS and HRTEM analysis of samples with initial Pu concentrations of 10(-8) - 10(-6) M indicated that Pu surface and/or bulk precipitation was likely responsible for this deviation. In 10(-6) M Pu(IV) and Pu(V) samples, HRTEM analysis showed the formation of a body centered cubic (bcc) Pu4O7 structure on the goethite surface, confirming that reduction of Pu(V) had occurred on the mineral surface and that epitaxial distortion previously observed for Pu(IV) sorption occurs with Pu(V) as well. C1 [Zhao, Pihong; Begg, James D.; Zavarin, Mavrik; Williams, Ross; Dai, Zurong R.; Kips, Ruth; Kersting, Annie B.] Lawrence Livermore Natl Lab, Glenn T Seaborg Inst, Phys & Life Sci, 7000 East Ave, Livermore, CA 94550 USA. [Tumey, Scott J.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Phys & Life Sci, 7000 East Ave, Livermore, CA 94550 USA. RP Begg, JD (reprint author), Lawrence Livermore Natl Lab, Glenn T Seaborg Inst, Phys & Life Sci, 7000 East Ave, Livermore, CA 94550 USA. EM begg2@llnl.gov FU Subsurface Biogeochemical Research Program of the U.S. Department of Energy's Office of Biological and Environmental Research; LLNL [DE-AC52-07NA27344, LLNL-JRNL-680462-DRAFT] FX We thank four anonymous reviewers who greatly improved the clarity of the manuscript. This work was supported by the Subsurface Biogeochemical Research Program of the U.S. Department of Energy's Office of Biological and Environmental Research. Prepared by LLNL under Contract DE-AC52-07NA27344. LLNL-JRNL-680462-DRAFT. NR 52 TC 1 Z9 1 U1 26 U2 41 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 5 PY 2016 VL 50 IS 13 SI SI BP 6948 EP 6956 DI 10.1021/acs.est.6b00605 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DQ7DE UT WOS:000379366300043 PM 27268262 ER PT J AU Cheng, YW Hubbard, CG Li, L Bouskill, N Molins, S Zheng, LG Sonnenthal, E Conrad, ME Engelbrektson, A Coates, JD Ajo-Franklin, JB AF Cheng, Yiwei Hubbard, Christopher G. Li, Li Bouskill, Nicholas Molins, Sergi Zheng, Liange Sonnenthal, Eric Conrad, Mark E. Engelbrektson, Anna Coates, John D. Ajo-Franklin, Jonathan B. TI Reactive Transport Model of Sulfur Cycling as Impacted by Perchlorate and Nitrate Treatments SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID GEOCHEMICAL TRANSPORT; ISOTOPE FRACTIONATION; SOURING CONTROL; OIL-RESERVOIR; SULFIDE PRODUCTION; REDUCING BACTERIA; SULFATE REDUCTION; TEMPERATURE-RANGE; HYDROGEN-SULFIDE; YUCCA MOUNTAIN AB Microbial souring in oil reservoirs produces toxic, corrosive hydrogen sulfide through microbial sulfate reduction, often accompanying (sea)water flooding during secondary oil recovery. With data from column experiments as constraints, we developed the first reactive-transport model of a new candidate inhibitor, perchlorate, and compared it with the commonly used inhibitor, nitrate. Our model provided a good fit to the data, which suggest that perchlorate is more effective than nitrate on a per mole of inhibitor basis. Critically, we used our model to gain insight into the underlying competing mechanisms controlling the action of each inhibitor. This analysis suggested that competition by heterotrophic perchlorate reducers and direct inhibition by nitrite produced from heterotrophic nitrate reduction were the most important mechanisms for the perchlorate and nitrate treatments, respectively, in the modeled column experiments. This work demonstrates modeling to be a powerful tool for increasing and testing our understanding of reservoir-souring generation, prevention, and remediation processes, allowing us to incorporate insights derived from laboratory experiments into a framework that can potentially be used to assess risk and design optimal treatment schemes. C1 [Cheng, Yiwei; Hubbard, Christopher G.; Bouskill, Nicholas; Molins, Sergi; Zheng, Liange; Sonnenthal, Eric; Conrad, Mark E.; Ajo-Franklin, Jonathan B.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Li, Li] Penn State Univ, University Pk, PA 16802 USA. [Engelbrektson, Anna; Coates, John D.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. RP Cheng, YW (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM yiweicheng@lbl.gov RI Molins, Sergi/A-9097-2012; Sonnenthal, Eric/A-4336-2009; Hubbard, Christopher/J-6150-2014; Ajo-Franklin, Jonathan/G-7169-2015; zheng, liange/B-9748-2011; Bouskill, Nick/G-2390-2015; Cheng, Yiwei/H-6670-2016; Li, Li/A-6077-2008 OI Molins, Sergi/0000-0001-7675-3218; Hubbard, Christopher/0000-0002-8217-8122; zheng, liange/0000-0002-9376-2535; Cheng, Yiwei/0000-0003-1014-0325; Li, Li/0000-0002-1641-3710 FU Energy Biosciences Institute FX This work was funded by the Energy Biosciences Institute. We acknowledge the associate editor, Dr. T. David Waite, for handling this manuscript and the four anonymous reviewers for their constructive reviews that have improved the manuscript. NR 58 TC 1 Z9 1 U1 15 U2 27 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 5 PY 2016 VL 50 IS 13 SI SI BP 7010 EP 7018 DI 10.1021/acs.est.6b00081 PG 9 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DQ7DE UT WOS:000379366300050 PM 27267666 ER PT J AU Formo, EV Potterf, CB Yang, MX Unocic, RR Leonard, DN Pawel, M AF Formo, Eric V. Potterf, Caroline B. Yang, Miaoxin Unocic, Raymond R. Leonard, Donovan N. Pawel, Michelle TI How a Nanostructure's Shape Affects its Lifetime in the Environment: Comparing a Silver Nanocube to a Nanoparticle When Dispersed in Aqueous Media SO ENVIRONMENTAL SCIENCE & TECHNOLOGY LA English DT Article ID NOBLE-METAL NANOCRYSTALS; POLYOL SYNTHESIS; DISSOLUTION; RELEASE; WATER; AGGREGATION; PERSISTENCE; TOXICITY; KINETICS; SIZE AB Herein, we detail how the morphology of a nanomaterial affects its environmental lifetime in aquatic ecosystems. In particular, we focus on the cube and particle nanostructures of Ag and age them in various aquatic mediums including synthetic hard water, pond water, and seawater. Our results show that in the synthetic hard water and pond water cases, there was little difference in the rate of morphological changes as determined by UV-vis spectroscopy. However, when these samples were analyzed with transmission electron microscopy, radically different mechanisms in the loss of their original nanostructures were observed. Specifically, for the nanocube we observed that the corners of the cubes had become more rounded, whereas the aged nanoparticles formed large aggregates. Most interestingly, when the seawater samples were analyzed, the nanocubes showed a substantially higher stability in maintaining the nano length scale in comparison to nanoparticles overtime. Moreover, high-resolution transmission electron microscopy analysis allowed us to determine that Ag+ ions diffused away from both the edge and from the faces of the cube, whereas the nanoparticle rapidly aggregated under the harsh seawater conditions. C1 [Formo, Eric V.; Potterf, Caroline B.] Univ Georgia, Georgia Electron Microscopy, Athens, GA 30622 USA. [Yang, Miaoxin] Georgia Inst Technol, Dept Biomed Engn, Atlanta, GA 30332 USA. [Unocic, Raymond R.; Leonard, Donovan N.; Pawel, Michelle] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. RP Formo, EV (reprint author), Univ Georgia, Georgia Electron Microscopy, Athens, GA 30622 USA. EM eformo@uga.edu FU NSF Division of Chemistry in the Harrop Laboratory at the University of Georgia [CHE-0953102] FX Fabrication of the nanostructures as well as high resolution (S)TEM imaging and EDS work was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. UV vis spectroscopy used in this experiment was obtained from use of an instrument purchased with funds from NSF Division of Chemistry (CHE-0953102) in the Harrop Laboratory at the University of Georgia. NR 36 TC 2 Z9 2 U1 17 U2 29 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0013-936X EI 1520-5851 J9 ENVIRON SCI TECHNOL JI Environ. Sci. Technol. PD JUL 5 PY 2016 VL 50 IS 13 SI SI BP 7082 EP 7089 DI 10.1021/acs.est.6b01172 PG 8 WC Engineering, Environmental; Environmental Sciences SC Engineering; Environmental Sciences & Ecology GA DQ7DE UT WOS:000379366300058 PM 27253183 ER PT J AU Wistisen, TN Uggerhoj, UI Wienands, U Markiewicz, TW Noble, RJ Benson, BC Smith, T Bagli, E Bandiera, L Germogli, G Guidi, V Mazzolari, A Holtzapple, R Tucker, S AF Wistisen, T. N. Uggerhoj, U. I. Wienands, U. Markiewicz, T. W. Noble, R. J. Benson, B. C. Smith, T. Bagli, E. Bandiera, L. Germogli, G. Guidi, V. Mazzolari, A. Holtzapple, R. Tucker, S. TI Channeling, volume reflection, and volume capture study of electrons in a bent silicon crystal SO PHYSICAL REVIEW ACCELERATORS AND BEAMS LA English DT Article ID CHARGED-PARTICLES; UNDULATOR; RADIATION AB We present the experimental data and analysis of experiments conducted at SLAC National Accelerator Laboratory investigating the processes of channeling, volume-reflection and volume-capture along the (111) plane in a strongly bent quasimosaic silicon crystal. These phenomena were investigated at 5 energies: 3.35, 4.2, 6.3, 10.5, and 14.0 GeV with a crystal with bending radius of 0.15 m, corresponding to curvatures of 0.053, 0.066, 0.099, 0.16, and 0.22 times the critical curvature, respectively. Based on the parameters of fitting functions we have extracted important parameters describing the channeling process such as the dechanneling length, the angle of volume reflection, the surface transmission, and the widths of the distribution of channeled particles parallel and orthogonal to the plane. C1 [Wistisen, T. N.; Uggerhoj, U. I.] Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus, Denmark. [Wienands, U.; Markiewicz, T. W.; Noble, R. J.; Benson, B. C.; Smith, T.] SLAC Natl Accelerator Lab, 2575 Sand Hill Rd, Menlo Pk, CA 94025 USA. [Bagli, E.; Bandiera, L.; Germogli, G.; Guidi, V.; Mazzolari, A.] Univ Ferrara, Dept Phys & Earth Sci, Via Saragat 1-C, I-44122 Ferrara, Italy. [Bagli, E.; Bandiera, L.; Germogli, G.; Guidi, V.; Mazzolari, A.] INFN, Sect Ferrara, Via Saragat 1-C, I-44122 Ferrara, Italy. [Holtzapple, R.; Tucker, S.] Calif Polytech State Univ San Luis Obispo, San Luis Obispo, CA 93407 USA. [Wienands, U.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Wistisen, TN (reprint author), Aarhus Univ, Dept Phys & Astron, DK-8000 Aarhus, Denmark. RI Bagli, Enrico/E-5906-2012; Uggerhoj, Ulrik/A-1802-2012 OI Bagli, Enrico/0000-0003-3913-7701; Uggerhoj, Ulrik/0000-0002-8229-1512 FU U.S. DOE [DE- AC02-76SF00515]; U.S. National Science Foundation [PHY-1068662]; Danish Council for Independent Research-Natural Sciences FNU; Italian Istituto Nazionale di Fisica Nucleare (INFN) FX This work was partially supported by the U.S. DOE under Contract No. DE- AC02-76SF00515, by the U.S. National Science Foundation (Grant No. PHY-1068662), by the Danish Council for Independent Research-Natural Sciences FNU, and the Italian Istituto Nazionale di Fisica Nucleare (INFN) through the CHANEL experiment. We wish to acknowledge also Mr. Persiani Andrea and Mr. Manfredi Claudio of Perman (Loiano, Italy) for their support with crystal holders manufacturing. Gilles Frequet from Fogale Nanotech for precise measurement of crystal thickness by means of a T-MAP IR interferometer. NR 33 TC 2 Z9 2 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9888 J9 PHYS REV ACCEL BEAMS JI Phys. Rev. Accel. Beams PD JUL 5 PY 2016 VL 19 IS 7 AR 071001 DI 10.1103/PhysRevAccelBeams.19.071001 PG 11 WC Physics, Nuclear; Physics, Particles & Fields SC Physics GA DQ6YO UT WOS:000379353200002 ER PT J AU Bull, CL Playford, HY Knight, KS Stenning, GBG Tucker, MG AF Bull, C. L. Playford, H. Y. Knight, K. S. Stenning, G. B. G. Tucker, M. G. TI Magnetic and structural phase diagram of the solid solution LaCoxMn1-xO3 SO PHYSICAL REVIEW B LA English DT Article ID NEUTRON-DIFFRACTION; SPIN-GLASSES; PEROVSKITES; TRANSITION; LACOO3; CO; LA2COMNO6; MN; DYNAMICS; SYMMETRY AB We present a structural and magnetic phase diagram of the solid solution LaCoxMn1-xO3. We show by neutron diffraction that the monoclinic structure previously observed for the elpasolite form La2CoMnO6 (LaCo0.5Mn0.5O3) is also observed for another member of the solid solution x = 0.35. We also present the transition temperatures for the orthorhombic/monoclinic structures of the series to the rhombohedral structure and determine the expected transition temperatures from rhombohedral to cubic symmetry. We present the magnetic structures as determined by neutron diffraction for materials with lower cobalt content and provide evidence, including ac and dc susceptibility measurements, for the possible glassy nature of the magnetism in the cobalt-rich materials in the series. Based on high-resolution neutron diffraction, we also suggest that there is a limit to the LaCoxMn1-xO3 solid solution at x = 0.85. Finally we present a possible, previously unreported, low-temperature monoclinic structure for the sample LaCo(0.75)Mn(0.2)5O(3). C1 [Bull, C. L.; Playford, H. Y.; Knight, K. S.; Stenning, G. B. G.; Tucker, M. G.] Rutherford Appleton Lab, STFC ISIS Facil, Didcot OX11 0QX, Oxon, England. [Knight, K. S.] Nat Hist Museum, Dept Earth Sci, Cromwell Rd, London SW7 5BD, England. [Knight, K. S.] UCL, Dept Earth Sci, Gower St, London WC1E 6BT, England. [Tucker, M. G.] Diamond Light Source Ltd, Didcot OX11 0DE, Oxon, England. [Tucker, M. G.] Spallat Neutron Source, One Bethel Valley Rd,MS-6475, Oak Ridge, TN 37830 USA. RP Bull, CL (reprint author), Rutherford Appleton Lab, STFC ISIS Facil, Didcot OX11 0QX, Oxon, England. EM craig.bull@stfc.ac.uk NR 49 TC 1 Z9 1 U1 11 U2 18 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 5 PY 2016 VL 94 IS 1 AR 014102 DI 10.1103/PhysRevB.94.014102 PG 11 WC Physics, Condensed Matter SC Physics GA DR1YA UT WOS:000379699600001 ER PT J AU Heidler, J Fechner, M Chopdekar, RV Piamonteze, C Dreiser, J Jenkins, CA Arenholz, E Rusponi, S Brune, H Spaldin, NA Nolting, F AF Heidler, J. Fechner, M. Chopdekar, R. V. Piamonteze, C. Dreiser, J. Jenkins, C. A. Arenholz, E. Rusponi, S. Brune, H. Spaldin, N. A. Nolting, F. TI Magnetoelectroelastic control of magnetism in an artificial multiferroic SO PHYSICAL REVIEW B LA English DT Article ID RAY CIRCULAR-DICHROISM; TUNNEL-JUNCTIONS; SPIN POLARIZATION; ULTRATHIN FILMS; EXCHANGE BIAS; ANISOTROPY; COBALT; FIELD; CO; HETEROSTRUCTURES AB We study the coexistence of strain-and charge-mediated magnetoelectric coupling in a cobalt (0-7 nm) wedge on ferroelectric (011)-oriented [Pb(Mg-1/3/Nb-2/3)O-3](0.68)-[PbTiO3](0.32) using surface-sensitive x-ray magnetic circular dichroism spectroscopy at the Co L-3,L-2 edges. Three distinct electric field driven remanent magnetization states can be set in the Co film at room temperature. Ab initio density functional theory calculations unravel the relative contributions of both strain and charge to the observed magnetic anisotropy changes illustrating magnetoelectroelastic coupling at artificial multiferroic interfaces. C1 [Heidler, J.; Chopdekar, R. V.; Piamonteze, C.; Dreiser, J.; Nolting, F.] Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland. [Heidler, J.] Paul Scherrer Inst, SwissFEL, CH-5232 Villigen, Switzerland. [Fechner, M.; Spaldin, N. A.] ETH, Mat Theory, CH-8093 Zurich, Switzerland. [Chopdekar, R. V.] Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland. [Chopdekar, R. V.] Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. [Jenkins, C. A.; Arenholz, E.] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Rusponi, S.; Brune, H.] Ecole Polytech Fed Lausanne, Inst Phys, CH-1015 Lausanne, Switzerland. RP Chopdekar, RV; Piamonteze, C (reprint author), Paul Scherrer Inst, Swiss Light Source, CH-5232 Villigen, Switzerland.; Chopdekar, RV (reprint author), Paul Scherrer Inst, Lab Micro & Nanotechnol, CH-5232 Villigen, Switzerland.; Chopdekar, RV (reprint author), Univ Calif Davis, Dept Chem Engn & Mat Sci, Davis, CA 95616 USA. EM rchopdekar@ucdavis.edu; cinthia.piamonteze@psi.ch RI Brune, Harald/E-7284-2017; Piamonteze, Cinthia/E-9740-2016; OI Brune, Harald/0000-0003-4459-3111; Chopdekar, Rajesh/0000-0001-6727-6501; Rusponi, Stefano/0000-0002-8494-5532 FU Swiss Nanoscience Institute; EU [NMP3-LA-2010 246102]; ETH Zurich; ERC [291151]; Max Rossler Prize of the ETH Zurich; Swiss National Supercomputing Centre (CSCS) [s624]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was financially supported by the Swiss Nanoscience Institute, EU's Seventh Framework Programme IFOX (NMP3-LA-2010 246102), by the ETH Zurich (NAS), by the ERC Advanced Grant program, No. 291151 (MF and NAS), by the Max Rossler Prize of the ETH Zurich (NAS) and by a grant from the Swiss National Supercomputing Centre (CSCS) under project ID s624. The x-ray absorption measurements were performed on the EPFL/PSI X-Treme beamline at the Swiss Light Source, Paul Scherrer Institut, Switzerland and at beamline 6.3.1 at the Advanced Light Source, Lawrence Berkeley National Laboratory, California, USA. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We thank Christof Schneider for his assistance in structural characterization and Marcus Schmidt for technical support. NR 48 TC 0 Z9 0 U1 23 U2 47 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 5 PY 2016 VL 94 IS 1 AR 014401 DI 10.1103/PhysRevB.94.014401 PG 7 WC Physics, Condensed Matter SC Physics GA DR1YA UT WOS:000379699600005 ER PT J AU Lin, SZ AF Lin, Shi-Zeng TI Edge instability in a chiral stripe domain under an electric current and skyrmion generation SO PHYSICAL REVIEW B LA English DT Article ID MAGNETIC SKYRMIONS; SPIN-TORQUE; DYNAMICS; MOTION; WALLS; LATTICE AB Motivated by the recent experimental observations on the skyrmion creation by cutting chiral stripe domains under a current drive [Jiang et al., Science 349, 283 (2015)], we study the mechanism of skyrmion generation by simulating the dynamics of stripe domains. Our theory for skyrmion generation is based on the fact that there are two half skyrmions attached to the ends of a stripe domain. These half skyrmions move due to the coupling between the skyrmion topological charge and current. As a consequence, the stripe domain is bent or stretched depending on the direction of motion of the half skyrmions. For a large current, skyrmions are created by chopping the stripe domains via strong bending or stretching. Our theory provides an explanation to the experiments and is supported by the new experiments. Furthermore, we predict that skyrmions can also be generated using a Bloch stripe domain under a spin transfer torque which can be realized in B20 compounds. C1 [Lin, Shi-Zeng] Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. RP Lin, SZ (reprint author), Los Alamos Natl Lab, Div Theoret, Los Alamos, NM 87545 USA. EM szl@lanl.gov RI Lin, Shi-Zeng/B-2906-2008 OI Lin, Shi-Zeng/0000-0002-4368-5244 FU Institutional Computing Program at LANL; LANL Directed Research and Development program FX The authors are indebted to Axel Hoffmann and Wanjun Jiang for sharing the experimental data prior to publication and for the helpful discussions. Computer resources for numerical calculations were supported by the Institutional Computing Program at LANL. This work was funded by the LANL Directed Research and Development program. NR 37 TC 2 Z9 2 U1 17 U2 28 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 5 PY 2016 VL 94 IS 2 AR 020402 DI 10.1103/PhysRevB.94.020402 PG 6 WC Physics, Condensed Matter SC Physics GA DR1YV UT WOS:000379701700001 ER PT J AU Yang, J Duan, C Huang, Q Brown, C Neuefeind, J Louca, D AF Yang, J. Duan, C. Huang, Q. Brown, C. Neuefeind, J. Louca, Despina TI Strong correlations between vacancy and magnetic ordering in superconducting K0.8Fe2-ySe2 SO PHYSICAL REVIEW B LA English DT Article ID PHASE-SEPARATION; KXFE2-YSE2 AB The coexistence of magnetic and nonmagnetic phases in the superconducting potassium iron selenide, KxFe2-ySe2, has been intensely debated. With superconductivity proposed to appear in a stoichiometric, nonmagnetic phase with I4/mmm crystal symmetry, the proposed nonsuperconducting phase is magnetic and has a lower symmetry, I4/m. The latter consists of Fe vacancies that go through a disordered-to-ordered transition in which the partially filled Fe sites create a supercell upon ordering. We show, using neutron scattering on the optimally doped composition, K0.8Fe2-ySe2, that the absence of magnetism does not signal the presence of superconductivity. Moreover, the degree of vacancy order is coupled to the strength of the magnetic order. Superconductivity coincides with the presence of the magnetic order parameter, albeit the latter is significantly weaker than previously reported, contradicting the current understanding of this similar to 30K superconductor. C1 [Yang, J.; Duan, C.; Louca, Despina] Univ Virginia, Charlottesville, VA 22904 USA. [Huang, Q.; Brown, C.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Neuefeind, J.] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Louca, D (reprint author), Univ Virginia, Charlottesville, VA 22904 USA. EM louca@virginia.edu RI Brown, Craig/B-5430-2009 OI Brown, Craig/0000-0002-9637-9355 FU U.S. Department of Energy, Office of Basic Energy Sciences [DE-FG02-01ER45927]; Office of Basic Energy Sciences, Division of Scientific User Facilities; US Department of Commerce FX The authors would like to acknowledge valuable discussions with W. Bao, T. Egami, A. Bianconi, and W. Ku. The work at the University of Virginia was supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-FG02-01ER45927, and that at Oak Ridge National Laboratory, by the Office of Basic Energy Sciences, Division of Scientific User Facilities. The work at NIST was supported by the US Department of Commerce. NR 42 TC 0 Z9 0 U1 9 U2 12 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9950 EI 2469-9969 J9 PHYS REV B JI Phys. Rev. B PD JUL 5 PY 2016 VL 94 IS 2 AR 024503 DI 10.1103/PhysRevB.94.024503 PG 6 WC Physics, Condensed Matter SC Physics GA DR1YV UT WOS:000379701700013 ER PT J AU Jansen, GR Schuster, MD Signoracci, A Hagen, G Navratil, P AF Jansen, G. R. Schuster, M. D. Signoracci, A. Hagen, G. Navratil, P. TI Open sd-shell nuclei from first principles SO PHYSICAL REVIEW C LA English DT Article ID COUPLED-CLUSTER METHODS; MODEL; STATE; MATTER; RADII AB We extend the ab initio coupled-cluster effective interaction (CCEI) method to open-shell nuclei with protons and neutrons in the valence space and compute binding energies and excited states of isotopes of neon and magnesium. We employ a nucleon-nucleon and three-nucleon interaction from chiral effective field theory evolved to a lower cutoff via a similarity renormalization group transformation. We find good agreement with experiment for binding energies and spectra, while charge radii of neon isotopes are underestimated. For the deformed nuclei Ne-20 and Mg-24, we reproduce rotational bands and electric quadrupole transitions within uncertainties estimated from an effective field theory for deformed nuclei, thereby demonstrating that collective phenomena in sd-shell nuclei emerge from complex ab initio calculations. C1 [Jansen, G. R.; Schuster, M. D.] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. [Jansen, G. R.; Signoracci, A.; Hagen, G.] Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. [Signoracci, A.; Hagen, G.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Navratil, P.] TRIUMF, 4004 Wesbrook Mall, Vancouver, BC V6T 2A3, Canada. RP Jansen, GR (reprint author), Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA.; Jansen, GR (reprint author), Oak Ridge Natl Lab, Div Phys, Oak Ridge, TN 37831 USA. FU Office of Nuclear Physics, US Department of Energy (Oak Ridge National Laboratory) [DE-SC0008499]; NSERC Grant [491045-2011]; Field Work Proposal at Oak Ridge National Laboratory [ERKBP57]; National Research Council Canada; Office of Science of the Department of Energy [DE-AC05-00OR22725] FX We would in particular like to thank Ragnar Stroberg for computing the rms deviations from experiment for our CCEI results and for providing us with shell-model results for the sd-shell nuclei considered in this work by using the USD-B interaction. We also thank Heiko Hergert, Jason Holt, Jonathan Engel, and Thomas Papenbrock for useful discussions. We are particularly grateful to Thomas Papenbrock for generating Figure 4 and contributing to the discussion related to the effective field theory for deformed nuclei. This work was supported by the Office of Nuclear Physics, US Department of Energy (Oak Ridge National Laboratory), DE-SC0008499 (NUCLEI SciDAC collaboration), NSERC Grant No. 491045-2011, and the Field Work Proposal ERKBP57 at Oak Ridge National Laboratory. Computer time was provided by the Innovative and Novel Computational Impact on Theory and Experiment (INCITE) program. TRIUMF receives funding via a contribution through the National Research Council Canada. This research used resources of the Oak Ridge Leadership Computing Facility located in the Oak Ridge National Laboratory, which is supported by the Office of Science of the Department of Energy under Contract No. DE-AC05-00OR22725, and used computational resources of the National Center for Computational Sciences and the National Institute for Computational Sciences.; This manuscript has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan. (http://energy.gov/downloads/doepublic-access-plan). NR 69 TC 6 Z9 6 U1 3 U2 7 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2469-9985 EI 2469-9993 J9 PHYS REV C JI Phys. Rev. C PD JUL 5 PY 2016 VL 94 IS 1 AR 011301 DI 10.1103/PhysRevC.94.011301 PG 6 WC Physics, Nuclear SC Physics GA DR2FI UT WOS:000379720000001 ER PT J AU Hu, W Chiang, CT Li, Y LoVerde, M AF Hu, Wayne Chiang, Chi-Ting Li, Yin LoVerde, Marilena TI Separating the Universe into real and fake energy densities SO PHYSICAL REVIEW D LA English DT Article ID SIMULATIONS; MATTER AB The separate universe technique provides a means of establishing consistency relations between short-wavelength observables and the long-wavelength matter density fluctuations within which they evolve by absorbing the latter into the cosmological background. We extend it to cases where nongravitational forces introduce a Jeans scale in other species like dynamical dark energy or massive neutrinos. The technique matches the synchronous gauge matter density fluctuations to the local expansion using the acceleration equation and accounts for the temporal nonlocality and scale dependence of the long-wavelength response of small scale matter observables, e.g., the nonlinear power spectrum, halo abundance and the implied halo bias, and N-point correlation functions. Above the Jeans scale, the local Friedmann equation relates the expansion to real energy densities and a curvature that is constant in comoving coordinates. Below the Jeans scale, the curvature evolves and acts like a fake density component. In all cases, the matter evolution on small scales is correctly modeled as we illustrate using scalar field dark energy with adiabatic or isocurvature initial conditions across the Jeans scale set by its finite sound speed. C1 [Hu, Wayne] Univ Chicago, Enrico Fermi Inst, Dept Astron & Astrophys, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Chiang, Chi-Ting; LoVerde, Marilena] SUNY Stony Brook, CN Yang Inst Theoret Phys, Dept Phys & Astron, Stony Brook, NY 11794 USA. [Li, Yin] Univ Calif Berkeley, Dept Phys, Berkeley Ctr Cosmol Phys, Berkeley, CA 94720 USA. [Li, Yin] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Li, Yin] Univ Tokyo, UTIAS, Kavli Inst Phys & Math Universe WPI, Chiba 2778583, Japan. RP Hu, W (reprint author), Univ Chicago, Enrico Fermi Inst, Dept Astron & Astrophys, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. FU U.S. Department of Energy [DE-FG02-13ER41958]; NASA [ATP NNX15AK22G]; Kavli Institute for Cosmological Physics at the University of Chicago [NSF PHY-0114422, NSF PHY-0551142]; [NSF PHY-1316617] FX We thank Uros Seljak and Masahiro Takada for useful discussions. W. H. was supported by U.S. Department of Energy Contract No. DE-FG02-13ER41958, NASA Grant No. ATP NNX15AK22G, and the Kavli Institute for Cosmological Physics at the University of Chicago through Grants No. NSF PHY-0114422 and No. NSF PHY-0551142 and an endowment from the Kavli Foundation and its founder Fred Kavli. C. C. and M. L. are supported by Grant No. NSF PHY-1316617. NR 35 TC 1 Z9 1 U1 0 U2 1 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 5 PY 2016 VL 94 IS 2 AR 023002 DI 10.1103/PhysRevD.94.023002 PG 15 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DR2GK UT WOS:000379722800003 ER PT J AU Martin, A Roy, TS AF Martin, Adam Roy, Tuhin S. TI Cautionary tale of mismeasured tails from q/g bias SO PHYSICAL REVIEW D LA English DT Article ID HADRON-COLLISIONS; JET; MULTIPLICITY; ALGORITHMS; GLUON; QUARK AB Jet substructure techniques such as subjet pT-asymmetry, mass-drop, and grooming have become powerful and widely used tools in experimental searches at the LHC. While these tools provide much-desired handles to separate signal from background, they can introduce unexpected mass scales into the analysis. These scales may be misinterpreted as excesses if these are not correctly incorporated into background modeling. As an example, we study the ATLAS hadronic di-W/Z resonance search. There, we find that the substructure analysis-in particular the combination of a subjet asymmetry cut with the requirement on the number of tracks within a jet-induces a mass scale where the dominant partonic subprocess in the background changes from pp -> g + q/(q) over bar to pp -> q (q) over bar. In light of this scale, modeling the QCD background using a simple smooth function with monotonically decreasing slope appears insufficient. C1 [Martin, Adam] Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. [Roy, Tuhin S.] Tata Inst Fundamental Res, Dept Theoret Phys, Bombay 400005, Maharashtra, India. [Roy, Tuhin S.] Los Alamos Natl Lab, Theory Div T2, Los Alamos, NM 87545 USA. RP Martin, A (reprint author), Univ Notre Dame, Dept Phys, Notre Dame, IN 46556 USA. FU U.S. National Science Foundation [PHY-1417118] FX The authors would like to thank Stephen D. Ellis for his helpful comments during the course of this work, and while preparing the draft. This work was supported in part by the U.S. National Science Foundation under Grant No. PHY-1417118. A. M. thanks Boston University for computing resources. A significant part of the computations were performed on the Mapache cluster in the High Performance Computing facility at Los Alamos National Laboratory. NR 61 TC 3 Z9 3 U1 3 U2 3 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0010 EI 2470-0029 J9 PHYS REV D JI Phys. Rev. D PD JUL 5 PY 2016 VL 94 IS 1 AR 014003 DI 10.1103/PhysRevD.94.014003 PG 13 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DR2GB UT WOS:000379721900007 ER PT J AU Seshadhri, C Smith, AM Vorobeychik, Y Mayo, JR Armstrong, RC AF Seshadhri, C. Smith, Andrew M. Vorobeychik, Yevgeniy Mayo, Jackson R. Armstrong, Robert C. TI Characterizing short-term stability for Boolean networks over any distribution of transfer functions SO PHYSICAL REVIEW E LA English DT Article ID GENETIC NETWORKS; MODELS; YEAST; BEHAVIOR AB We present a characterization of short-term stability of Kauffman's N K (random) Boolean networks under arbitrary distributions of transfer functions. Given such a Boolean network where each transfer function is drawn from the same distribution, we present a formula that determines whether short-term chaos (damage spreading) will happen. Our main technical tool which enables the formal proof of this formula is the Fourier analysis of Boolean functions, which describes such functions as multilinear polynomials over the inputs. Numerical simulations on mixtures of threshold functions and nested canalyzing functions demonstrate the formula's correctness. C1 [Seshadhri, C.] Univ Calif Santa Cruz, Santa Cruz, CA 95064 USA. [Smith, Andrew M.; Mayo, Jackson R.; Armstrong, Robert C.] Sandia Natl Labs, POB 969, Livermore, CA 94551 USA. [Vorobeychik, Yevgeniy] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. RP Seshadhri, C (reprint author), Univ Calif Santa Cruz, Santa Cruz, CA 95064 USA. FU U.S. Department of Energy [DE-AC04-94AL85000] FX Sandia is a multiprogram laboratory operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy under Contract No. DE-AC04-94AL85000. NR 29 TC 1 Z9 1 U1 0 U2 0 PU AMER PHYSICAL SOC PI COLLEGE PK PA ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA SN 2470-0045 EI 2470-0053 J9 PHYS REV E JI Phys. Rev. E PD JUL 5 PY 2016 VL 94 IS 1 AR 012301 DI 10.1103/PhysRevE.94.012301 PG 7 WC Physics, Fluids & Plasmas; Physics, Mathematical SC Physics GA DR2HC UT WOS:000379724600008 PM 27575142 ER PT J AU Perez-Blanco, H Vineyard, E AF Perez-Blanco, H. Vineyard, Edward TI Feasibility and operating costs of an air cycle for CCHP in a fast food restaurant SO APPLIED THERMAL ENGINEERING LA English DT Article DE Brayton air-cycle; Trigeneration; Energy costs; Fast food restaurant AB This work considers the possibilities of an air-based Brayton cycle to provide the power, heating and cooling needs of fast-food restaurants. A model of the cycle based on conventional turbomachinery loss coefficients is formulated. The heating, cooling and power capabilities of the cycle are extracted from simulation results. Power and thermal loads for restaurants in Knoxville, TN and in International Falls, MN, are considered. It is found that the cycle can meet the loads by setting speed and mass flow-rate apportionment between the power and cooling functional sections. The associated energy costs appear elevated when compared to the cost of operating individual components or a more conventional, absorption-based CHP system. A first-order estimate of capital investments is provided. Suggestions for future work whereby the operational costs could be reduced are given in the conclusions. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Perez-Blanco, H.] Penn State Univ, Mech & Nucl Engn, University Pk, PA 16802 USA. [Vineyard, Edward] Oak Ridge Natl Lab, Computat Sci & Engn Div, Oak Ridge, TN USA. RP Perez-Blanco, H (reprint author), Penn State Univ, Mech & Nucl Engn, University Pk, PA 16802 USA. EM hpb1@gmail.com; vineyardea@ornl.gov OI Vineyard, Edward/0000-0003-4695-7441 FU CHP DOE program; ORNL; Penn State FX The authors wish to acknowledge the support of the CHP DOE program, and of ORNL, for enabling the resources to complete this work. The sabbatical from Penn State awarded to H. Perez-Blanco was also instrumental in allowing the unconstrained time to characterize air cycles. The comments and suggestions of Dr. K. Gluesenkamp are warmly acknowledged. NR 21 TC 0 Z9 0 U1 1 U2 2 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 1359-4311 J9 APPL THERM ENG JI Appl. Therm. Eng. PD JUL 5 PY 2016 VL 104 BP 818 EP 828 DI 10.1016/j.applthermaleng.2016.05.030 PG 11 WC Thermodynamics; Energy & Fuels; Engineering, Mechanical; Mechanics SC Thermodynamics; Energy & Fuels; Engineering; Mechanics GA DQ5UK UT WOS:000379270400080 ER PT J AU Holmes, ST Alkan, F Iuliucci, RJ Mueller, KT Dybowski, C AF Holmes, Sean T. Alkan, Fahri Iuliucci, Robbie J. Mueller, Karl T. Dybowski, Cecil TI Analysis of the Bond-Valence Method for Calculating Si-29 and P-31 Magnetic Shielding in Covalent Network Solids SO JOURNAL OF COMPUTATIONAL CHEMISTRY LA English DT Article DE NMR; silicon; phosphorus; DFT; VMTA/BV; GIPAW ID NMR CHEMICAL-SHIFTS; DENSITY-FUNCTIONAL METHODS; CRYSTAL-STRUCTURE; 1ST-PRINCIPLES CALCULATIONS; CALCIUM PHOSPHATES; TIN(II) COMPOUNDS; LOCAL-STRUCTURE; ELECTRON-GAS; HEAVY-NUCLEI; STATE AB Si-29 and P-31 magnetic-shielding tensors in covalent network solids have been evaluated using periodic and cluster-based calculations. The cluster-based computational methodology employs pseudoatoms to reduce the net charge (resulting from missing co-ordination on the terminal atoms) through valence modification of terminal atoms using bond-valence theory (VMTA/BV). The magnetic-shielding tensors computed with the VMTA/BV method are compared to magnetic-shielding tensors determined with the periodic GIPAW approach. The cluster-based all-electron calculations agree with experiment better than the GIPAW calculations, particularly for predicting absolute magnetic shielding and for predicting chemical shifts. The performance of the DFT functionals CA-PZ, PW91, PBE, rPBE, PBEsol, WC, and PBE0 are assessed for the prediction of Si-29 and P-31 magnetic-shielding constants. Calculations using the hybrid functional PBE0, in combination with the VMTA/BV approach, result in excellent agreement with experiment. (C) 2016 Wiley Periodicals, Inc. C1 [Holmes, Sean T.; Alkan, Fahri; Dybowski, Cecil] Univ Delaware, Dept Chem & Biochem, Newark, DE 19716 USA. [Iuliucci, Robbie J.] Washington & Jefferson Coll, Dept Chem, Washington, PA 15301 USA. [Mueller, Karl T.] Penn State Univ, Dept Chem, University Pk, PA 16802 USA. [Mueller, Karl T.] Pacific NW Natl Lab, Phys & Computat Sci Directorate, Richland, WA 99352 USA. RP Dybowski, C (reprint author), Univ Delaware, Dept Chem & Biochem, Newark, DE 19716 USA. EM dybowski@udel.edu FU National Science Foundation [CHE-0956006, CHE-1213451] FX Contract grant sponsor: National Science Foundation; Contract grant numbers: CHE-0956006 and CHE-1213451 NR 71 TC 2 Z9 2 U1 8 U2 18 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0192-8651 EI 1096-987X J9 J COMPUT CHEM JI J. Comput. Chem. PD JUL 5 PY 2016 VL 37 IS 18 BP 1704 EP 1710 DI 10.1002/jcc.24389 PG 7 WC Chemistry, Multidisciplinary SC Chemistry GA DQ4HA UT WOS:000379163500006 PM 27117609 ER PT J AU He, YY Ford, ME Zhu, MH Liu, QC Wu, ZL Wachs, IE AF He, Yuanyuan Ford, Michael E. Zhu, Minghui Liu, Qingcai Wu, Zili Wachs, Israel E. TI Selective catalytic reduction of NO by NH3 with WO3-TiO2 catalysts: Influence of catalyst synthesis method SO APPLIED CATALYSIS B-ENVIRONMENTAL LA English DT Article DE Catalysts; Co-precipitated; TiO2; WO3; Spectroscopy; Raman; IR; Temperature programmed surface reaction (TPSR); Reaction; NO; NH3; Selective catalytic reduction (SCR) ID TUNGSTEN-OXIDE CATALYSTS; VANADIA-TITANIA CATALYSTS; SITU RAMAN-SPECTROSCOPY; HIGH-TEMPERATURE SCR; NITRIC-OXIDE; V2O5-WO3/TIO2 CATALYSTS; METAL-OXIDES; PHYSICOCHEMICAL PROPERTIES; STRUCTURAL DETERMINATION; PHOTOCATALYTIC ACTIVITY AB A series of supported WO3/TiO2 catalysts was prepared by a new synthesis procedure involving co precipitation of an aqueous TiO(OH)(2) and (NH4)(10)W12O41*5H(2)O slurry under controlled pH conditions. The morphological properties, surface WO. molecular structures, surface acidity and surface chemistry of the co-precipitated WO3/TiO2 catalysts were determined with BET, in situ Raman, in situ IR, steady-state NO/NH3/O-2 SCR and NO/NH3-temperature-programmed surface reaction (TPSR) spectroscopy, respectively. Time-resolved isotopic O-18-O-16 exchange with IR spectroscopy demonstrated that tungsten oxide was present as surface WO, sites on the TiO2 support with mono-oxo O = WO4 coordination. In contrast to previous studies employing impregnation synthesis that found only surface one mono-oxo O = WO4 site (similar to 1010-1016 cm(-1)) on TiO2, the co-precipitation procedure resulted in the formation of two distinct surface WO. sites: mono-oxo O = WO4 (1012-1014 cm(-1))and a second mono-oxo O = WO4 (similar to 983-985 cm(-1)). The new surface mono-oxo O = WO4 (similar to 983-985 cm(-1)) site is thought to be associated with surface defects on the co-precipitated titania support. The co-precipitated catalysts exhibited slightly enhanced SCR reactivity that is thought to be related to the presence of the new surface O = WO4 sites. Additional factors, however, may also be contributing. This is the first study that attempts to relate the molecular level structural properties of co-precipitated WO3-TiO2 catalysts with their surface reactivity for SCR. (C) 2016 Elsevier B.V. All rights reserved. C1 [He, Yuanyuan; Ford, Michael E.; Zhu, Minghui; Wachs, Israel E.] Lehigh Univ, Dept Chem & Biomol Engn, Operando Mol Spect & Catalysis Lab, 7 Asa Dr, Bethlehem, PA 18015 USA. [He, Yuanyuan; Liu, Qingcai] Chongqing Univ, Coll Mat Sci & Engn, Chongqing 400030, Peoples R China. [Wu, Zili] Oak Ridge Natl Lab, Div Chem Sci, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. [Wu, Zili] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. RP Wachs, IE (reprint author), Lehigh Univ, Dept Chem & Biomol Engn, Iaccoca Hall,111 Res Dr, Bethlehem, PA 18015 USA. EM iew0@lehigh.edu OI Zhu, Minghui/0000-0003-1593-9320 FU China Scholarship Council (CSC) [51274263, 51204220]; Center for Understanding & Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME); Energy Frontier Research Center - DOE, Office of Science, Office of Basic Energy Sciences [DE-SC0012577] FX Ms. Yuanyuan He is grateful for financial support from the China Scholarship Council (CSC) for the State Scholarship and National Natural Science Funds of China (Nos. 51274263 and 51204220). Prof. I.E. Wachs (Lehigh University), M. Zhu (Lehigh) and Dr. Zili Wu (Oak Ridge National Laboratory) were supported by the Center for Understanding & Control of Acid Gas-Induced Evolution of Materials for Energy (UNCAGE-ME), an Energy Frontier Research Center funded by DOE, Office of Science, Office of Basic Energy Sciences under grant DE-SC0012577. A portion of this research including the isotopic exchange was conducted at the Center for Nanophase Materials Sciences, which is a DOE office of the Science User Facility. The authors thank D. G. Gregory and Ms. Q. Guo of Lehigh University for experimental assistance in obtaining BET and BJH data. DGG is also thanked for assistance in obtaining the XRD spectra. Dr. Henry Luftman of Lehigh University is thanked for collecting the HS-LEIS data. NR 66 TC 4 Z9 4 U1 13 U2 185 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0926-3373 EI 1873-3883 J9 APPL CATAL B-ENVIRON JI Appl. Catal. B-Environ. PD JUL 5 PY 2016 VL 188 BP 123 EP 133 DI 10.1016/j.apcatb.2016.01.072 PG 11 WC Chemistry, Physical; Engineering, Environmental; Engineering, Chemical SC Chemistry; Engineering GA DH3HG UT WOS:000372677500014 ER PT J AU Leblebici, SY Leppert, L Li, Y Reyes-Lillo, SE Wickenburg, S Wong, E Lee, J Melli, M Ziegler, D Angell, DK Ogletree, DF Ashby, PD Toma, FM Neaton, JB Sharp, ID Weber-Bargioni, A AF Leblebici, Sibel Y. Leppert, Linn Li, Yanbo Reyes-Lillo, Sebastian E. Wickenburg, Sebastian Wong, Ed Lee, Jiye Melli, Mauro Ziegler, Dominik Angell, Daniel K. Ogletree, D. Frank Ashby, Paul D. Toma, Francesca M. Neaton, Jeffrey B. Sharp, Ian D. Weber-Bargioni, Alexander TI Facet-dependent photovoltaic efficiency variations in single grains of hybrid halide perovskite SO NATURE ENERGY LA English DT Article ID SOLAR-CELLS; THIN-FILMS; RECOMBINATION; PERFORMANCE; CH3NH3PBI3; MICROSCOPY; TRANSPORT; DYNAMICS; BEHAVIOR; LENGTHS AB Photovoltaic devices based on hybrid perovskite materials have exceeded 22% efficiency due to high charge-carrier mobilities and lifetimes. Properties such as photocurrent generation and open-circuit voltage are influenced by the microscopic structure and orientation of the perovskite crystals, but are difficult to quantify on the intra-grain length scale and are often treated as homogeneous within the active layer. Here, we map the local short-circuit photocurrent, open-circuit photovoltage, and dark drift current in state-of-the-art methylammonium lead iodide solar cells using photoconductive atomic force microscopy. We find, within individual grains, spatially correlated heterogeneity in short-circuit current and open-circuit voltage up to 0.6V. These variations are related to different crystal facets and have a direct impact on the macroscopic power conversion efficiency. We attribute this heterogeneity to a facet-dependent density of trap states. These results imply that controlling crystal grain and facet orientation will enable a systematic optimization of polycrystalline and single-crystal devices for photovoltaic and lighting applications. C1 [Leblebici, Sibel Y.; Leppert, Linn; Reyes-Lillo, Sebastian E.; Wickenburg, Sebastian; Wong, Ed; Lee, Jiye; Melli, Mauro; Ziegler, Dominik; Angell, Daniel K.; Ogletree, D. Frank; Ashby, Paul D.; Neaton, Jeffrey B.; Weber-Bargioni, Alexander] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Leblebici, Sibel Y.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Leppert, Linn; Reyes-Lillo, Sebastian E.; Neaton, Jeffrey B.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Li, Yanbo; Toma, Francesca M.; Sharp, Ian D.] Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Li, Yanbo; Toma, Francesca M.; Sharp, Ian D.] Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Ziegler, Dominik] Scuba Probe Technol LLC, 255 Lina Ave, Alameda, CA 94501 USA. [Neaton, Jeffrey B.] Kavli Energy NanoSci Inst Berkeley, Berkeley, CA 94720 USA. RP Weber-Bargioni, A (reprint author), Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA.; Sharp, ID (reprint author), Lawrence Berkeley Natl Lab, Joint Ctr Artificial Photosynth, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Sharp, ID (reprint author), Lawrence Berkeley Natl Lab, Div Chem Sci, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM idsharp@lbl.gov; afweber-bargioni@lbl.gov OI Li, Yanbo/0000-0002-3017-762X FU National Science Foundation Graduate Research Fellowship [NSF DGE 1106400]; Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub; Office of Science of the US Department of Energy [DE-SC0004993]; AvH foundation; US Department of Energy, Office of Science, SBIR/STTR Program Office [DE-SC0013212]; DOE Early Career Grant; US Department of Energy (DOE), Office of Basic Energy Sciences, Scientific User Facilities Division [DE-AC02-05CH11231]; Laboratory Directed Research and Development Program at the Lawrence Berkeley National Laboratory [DE-AC02-05CH11231] FX This material is based on work supported by the National Science Foundation Graduate Research Fellowship under Grant No. (NSF DGE 1106400) and by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the US Department of Energy under Award Number DE-SC0004993. L.L. thanks the AvH foundation for financial support through the Feodor-Lynen program. D.Z. acknowledges support by the US Department of Energy, Office of Science, SBIR/STTR Program Office, under Award Number DE-SC0013212. A.W.-B., M.M., J.L. and S.Y.L. were supported by a DOE Early Career Grant. Work at the Molecular Foundry was supported by the US Department of Energy (DOE), Office of Basic Energy Sciences, Scientific User Facilities Division, under contract no. DE-AC02-05CH11231 and user proposal 4233. J.B.N., S.E.R.-L. and F.M.T. acknowledge support from the Laboratory Directed Research and Development Program at the Lawrence Berkeley National Laboratory under Contract No. DE-AC02-05CH11231. NR 45 TC 18 Z9 18 U1 7 U2 7 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2058-7546 J9 NAT ENERGY JI Nat. Energy PD JUL 4 PY 2016 VL 1 AR 16093 DI 10.1038/NENERGY.2016.93 PG 7 WC Energy & Fuels; Materials Science, Multidisciplinary SC Energy & Fuels; Materials Science GA EK8MN UT WOS:000394178100001 ER PT J AU Kattel, S Yu, WT Yang, XF Yan, BH Huang, YQ Wan, WM Liu, P Chen, JGG AF Kattel, Shyam Yu, Weiting Yang, Xiaofang Yan, Binhang Huang, Yanqiang Wan, Weiming Liu, Ping Chen, Jingguang G. TI CO2 Hydrogenation over Oxide-Supported PtCo Catalysts: The Role of the Oxide Support in Determining the Product Selectivity SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE bimetallic catalysts; carbon dioxide; heterogeneous catalysis; hydrogenation; supported catalysts ID FISCHER-TROPSCH SYNTHESIS; TOTAL-ENERGY CALCULATIONS; WAVE BASIS-SET; HETEROGENEOUS CATALYSTS; SURFACE-CHEMISTRY; METHANOL; REDUCTION; AU; CONVERSION; INTERFACE AB By simply changing the oxide support, the selectivity of a metal-oxide catalysts can be tuned. For the CO2 hydrogenation over PtCo bimetallic catalysts supported on different reducible oxides (CeO2, ZrO2, and TiO2), replacing a TiO2 support by CeO2 or ZrO2 selectively strengthens the binding of C, O-bound and O-bound species at the PtCo-oxide interface, leading to a different product selectivity. These results reveal mechanistic insights into how the catalytic performance of metal-oxide catalysts can be fine-tuned. C1 [Kattel, Shyam; Yang, Xiaofang; Yan, Binhang; Liu, Ping; Chen, Jingguang G.] Brookhaven Natl Lab, Dept Chem, 2 Ctr St, Upton, NY 11973 USA. [Yu, Weiting; Wan, Weiming; Chen, Jingguang G.] Columbia Univ, Dept Chem Engn, 1500 W 120th St, New York, NY 10027 USA. [Huang, Yanqiang] Chinese Acad Sci, Dalian Inst Chem Phys, Dalian 116023, Peoples R China. RP Liu, P; Chen, JGG (reprint author), Brookhaven Natl Lab, Dept Chem, 2 Ctr St, Upton, NY 11973 USA.; Chen, JGG (reprint author), Columbia Univ, Dept Chem Engn, 1500 W 120th St, New York, NY 10027 USA. EM pingliu3@bnl.gov; jgchen@columbia.edu FU U.S. Department of Energy, Office of Science [DE-SC0012704]; US Department of Energy; National Energy Research Scientific Computing Center (NERSC); Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science (Contract No. DE-SC0012704). The DFT calculations were performed using computational resources at the Center for Functional Nanomaterials, a user facility at BNL, supported by the US Department of Energy and the National Energy Research Scientific Computing Center (NERSC), which is supported by the Office of Science of the U.S. Department of Energy (DE-AC02-05CH11231). NR 44 TC 3 Z9 3 U1 64 U2 67 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JUL 4 PY 2016 VL 55 IS 28 BP 7968 EP 7973 DI 10.1002/anie.201601661 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA DV9IC UT WOS:000383253100012 PM 27159088 ER PT J AU Xie, Y Shaffer, DW Lewandowska-Andralojc, A Szalda, DJ Concepcion, JJ AF Xie, Yan Shaffer, David W. Lewandowska-Andralojc, Anna Szalda, David J. Concepcion, Javier J. TI Water Oxidation by Ruthenium Complexes Incorporating Multifunctional Bipyridyl Diphosphonate Ligands SO ANGEWANDTE CHEMIE-INTERNATIONAL EDITION LA English DT Article DE catalysis; electrochemistry; phosphonates; ruthenium; water splitting ID SINGLE-SITE; PHOTOSYSTEM-II; OXIDE SURFACES; DIMER COMPLEX; BLUE DIMER; CATALYSTS; PHOTOSYNTHESIS; MECHANISM; BRIDGE AB We describe herein the synthesis and characterization of ruthenium complexes with multifunctional bipyridyl diphosphonate ligands as well as initial water oxidation studies. In these complexes, the phosphonate groups provide redox-potential leveling through charge compensation and sigma donation to allow facile access to high oxidation states. These complexes display unique pH-dependent electrochemistry associated with deprotonation of the phosphonic acid groups. The position of these groups allows them to shuttle protons in and out of the catalytic site and reduce activation barriers. A mechanism for water oxidation by these catalysts is proposed on the basis of experimental results and DFT calculations. The unprecedented attack of water at a neutral six-coordinate [Ru-IV] center to yield an anionic seven-coordinate [Ru-IV-OH](-) intermediate is one of the key steps of a single-site mechanism in which all species are anionic or neutral. These complexes are among the fastest single-site catalysts reported to date. C1 [Xie, Yan; Shaffer, David W.; Lewandowska-Andralojc, Anna; Concepcion, Javier J.] Brookhaven Natl Lab, Div Chem, Upton, NY 11973 USA. [Szalda, David J.] CUNY, Baruch Coll, Dept Nat Sci, New York, NY 10010 USA. [Lewandowska-Andralojc, Anna] Adam Mickiewicz Univ, Fac Chem, Umultowska 89b, PL-61614 Poznan, Poland. RP Concepcion, JJ (reprint author), Brookhaven Natl Lab, Div Chem, Upton, NY 11973 USA. EM jconcepc@bnl.gov RI Lewandowska-Andralojc, Anna/A-8149-2012; OI Shaffer, David/0000-0002-8807-1617 FU U.S. Department of Energy, Office of Science, Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences [DE-SC00112704] FX This research was carried out at Brookhaven National Laboratory and supported by the U.S. Department of Energy, Office of Science, Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences under contract DE-SC00112704. NR 23 TC 2 Z9 2 U1 21 U2 21 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1433-7851 EI 1521-3773 J9 ANGEW CHEM INT EDIT JI Angew. Chem.-Int. Edit. PD JUL 4 PY 2016 VL 55 IS 28 BP 8067 EP 8071 DI 10.1002/anie.201601943 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA DV9IC UT WOS:000383253100033 PM 27166584 ER PT J AU Khachatryan, V Sirunyan, AM Tumasyan, A Adam, W Asilar, E Bergauer, T Brandstetter, J Brondolin, E Dragicevic, M Ero, J Flechl, M Friedl, M Fruhwirth, R Ghete, VM Hartl, C Hormann, N Hrubec, J Jeitler, M Knunz, V Konig, A Krammer, M Kratschmer, I Liko, D Matsushita, T Mikulec, I Rabady, D Rad, N Rahbaran, B Rohringer, H Schieck, J Schofbeck, R Strauss, J Treberer-Treberspurg, W Waltenberger, W Wulz, CE Mossolov, V Shumeiko, N Gonzalez, JS Alderweireldt, S Cornelis, T De Wolf, EA Janssen, X Knutsson, A Lauwers, J Luyckx, S Van De Klundert, M Van Haevermaet, H Van Mechelen, P Van Remortel, N Van Spilbeeck, A Abu Zeid, S Blekman, F D'Hondt, J Daci, N De Bruyn, I Deroover, K Heracleous, N Keaveney, J Lowette, S Moreels, L Olbrechts, A Python, Q Strom, D Tavernier, S Van Doninck, W Van Mulders, P Van Onsem, GP Van 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CA CMS Collaboration TI Measurement of inclusive jet production and nuclear modifications in pPb collisions at root s(NN)=5.02 TeV SO EUROPEAN PHYSICAL JOURNAL C LA English DT Article ID QUARK-GLUON PLASMAS; P-PB COLLISIONS; ROOT(NN)-N-S=5.02 TEV; ATLAS DETECTOR; CENTRALITY; BIAS; LHC AB Inclusive jet production in pPb collisions at a nucleon-nucleon (NN) center-of-mass energy of root s(NN) = 5.02 TeV is studied with the CMS detector at the LHC. A data sample corresponding to an integrated luminosity of 30.1 nb(-1) is analyzed. The jet transverse momentum spectra are studied in seven pseudorapidity intervals covering the range -2.0 < eta(CM) < 1.5 in the NN center-of-mass frame. The jet production yields at forward and backward pseudorapidity are compared and no significant asymmetry about eta(CM) = 0 is observed in the measured kinematic range. The measurements in the pPb system are compared to reference jet spectra obtained by extrapolation from previous measurements in pp collisions at root s = 7 TeV. In all pseudorapidity ranges, nuclear modifications in inclusive jet production are found to be small, as predicted by next-to-leading order perturbative QCD calculations that incorporate nuclear effects in the parton distribution functions. C1 [Khachatryan, V.; Sirunyan, A. M.; Tumasyan, A.] Yerevan Phys Inst, Yerevan, Armenia. [Adam, W.; Asilar, E.; Bergauer, T.; Brandstetter, J.; Brondolin, E.; Dragicevic, M.; Eroe, J.; Flechl, M.; Friedl, M.; Fruehwirth, R.; Ghete, V. M.; Hartl, C.; Hoermann, N.; Hrubec, J.; Jeitler, M.; Knuenz, V.; Koenig, A.; Krammer, M.; Kraetschmer, I.; Liko, D.; Matsushita, T.; Mikulec, I.; Rabady, D.; Rad, N.; Rahbaran, B.; Rohringer, H.; Schieck, J.; Schoefbeck, R.; Strauss, J.; Treberer-Treberspurg, W.; Waltenberger, W.; Wulz, C. -E.] Inst Hochenergiephys OeAW, Vienna, Austria. 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J.; Ulrich, R.; Wagner-Kuhr, J.; Wayand, S.; Weber, M.; Weiler, T.; Williamson, S.; Woehrmann, C.; Wolf, R.] Inst Expt Kernphys, Karlsruhe, Germany. [Anagnostou, G.; Daskalakis, G.; Geralis, T.; Giakoumopoulou, V. A.; Kyriakis, A.; Loukas, D.; Psallidas, A.; Topsis-Giotis, I.] NCSR Demokritos, INPP, Aghia Paraskevi, Greece. [Agapitos, A.; Kesisoglou, S.; Panagiotou, A.; Saoulidou, N.; Tziaferi, E.] Univ Athens, Athens, Greece. [Evangelou, I.; Flouris, G.; Foudas, C.; Kokkas, P.; Loukas, N.; Manthos, N.; Papadopoulos, I.; Paradas, E.; Strologas, J.] Univ Ioannina, Ioannina, Greece. [Bencze, G.; Hajdu, C.; Hazi, A.; Hidas, P.; Horvath, D.; Sikler, F.; Veszpremi, V.; Vesztergombi, G.; Zsigmond, A. J.] Wigner Res Ctr Phys, Budapest, Hungary. [Beni, N.; Czellar, S.; Karancsi, J.; Molnar, J.; Szillasi, Z.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Bartok, M.; Makovec, A.; Raics, P.; Trocsanyi, Z. L.; Ujvari, B.] Univ Debrecen, Debrecen, Hungary. [Choudhury, S.; Mal, P.; Mandal, K.; Sahoo, D. K.; Sahoo, N.; Swain, S. K.] Natl Inst Sci Educ & Res, Bhubaneswar, Orissa, India. [Bansal, S.; Beri, S. B.; Bhatnagar, V.; Chawla, R.; Gupta, R.; Bhawandeep, U.; Kalsi, A. K.; Kaur, A.; Kaur, M.; Kumar, R.; Mehta, A.; Mittal, M.; Singh, J. B.; Walia, G.] Panjab Univ, Chandigarh, India. [Kumar, Ashok; Bhardwaj, A.; Choudhary, B. C.; Garg, R. B.; Malhotra, S.; Naimuddin, M.; Nishu, N.; Ranjan, K.; Sharma, R.; Sharma, V.] Univ Delhi, Delhi, India. [Bhattacharya, S.; Chatterjee, K.; Dey, S.; Dutta, S.; Majumdar, N.; Modak, A.; Mondal, K.; Mukhopadhyay, S.; Roy, A.; Roy, D.; Chowdhury, S. Roy; Sarkar, S.; Sharan, M.] Saha Inst Nucl Phys, Kolkata, India. [Chudasama, R.; Dutta, D.; Jha, V.; Kumar, V.; Mohanty, A. K.; Pant, L. M.; Shukla, P.; Topkar, A.] Bhabha Atom Res Ctr, Mumbai, Maharashtra, India. [Aziz, T.; Banerjee, S.; Bhowmik, S.; Chatterjee, R. M.; Dewanjee, R. K.; Dugad, S.; Ganguly, S.; Ghosh, S.; Guchait, M.; Gurtu, A.; Jain, Sa.; Kole, G.; Kumar, S.; Mahakud, B.; Maity, M.; Majumder, G.; Mazumdar, K.; Mitra, S.; Mohanty, G. B.; Parida, B.; Sarkar, T.; Sur, N.; Sutar, B.; Wickramage, N.] Tata Inst Fundamental Res, Mumbai, Maharashtra, India. [Chauhan, S.; Dube, S.; Kapoor, A.; Kothekar, K.; Sharma, S.] Indian Inst Sci Educ & Res IISER, Pune, Maharashtra, India. [Bakhshiansohi, H.; Behnamian, H.; Etesami, S. M.; Fahim, A.; Khakzad, M.; Najafabadi, M. Mohammadi; Naseri, M.; Mehdiabadi, S. Paktinat; Hosseinabadi, F. Rezaei; Safarzadeh, B.; Zeinali, M.] Inst Res Fundamental Sci IPM, Tehran, Iran. [Felcini, M.; Grunewald, M.] Univ Coll Dublin, Dublin, Ireland. [Abbrescia, M.; Calabria, C.; Caputo, C.; Colaleo, A.; Creanza, D.; Cristella, L.; De Filippis, N.; De Palma, M.; Fiore, L.; Iaselli, G.; Maggi, G.; Maggi, M.; Miniello, G.; My, S.; Nuzzo, S.; Pompili, A.; Pugliese, G.; Radogna, R.; Ranieri, A.; Selvaggi, G.; Silvestris, L.; Venditti, R.] INFN Sez Baria, Bari, Italy. [Abbrescia, M.; Calabria, C.; Caputo, C.; Cristella, L.; De Palma, M.; Miniello, G.; Nuzzo, S.; Pompili, A.; Radogna, R.; Selvaggi, G.; Venditti, R.] Univ Bari, Bari, Italy. [Creanza, D.; De Filippis, N.; Iaselli, G.; Maggi, G.; My, S.; Pugliese, G.] Politecn Bari, Bari, Italy. [Abbiendi, G.; Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Cavallo, F. R.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Dallavalle, G. M.; Fabbri, F.; Fanfani, A.; Fasanella, D.; Giacomelli, P.; Grandi, C.; Guiducci, L.; Marcellini, S.; Masetti, G.; Montanari, A.; Navarria, F. L.; Perrotta, A.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.] INFN Sez Bologna, Bologna, Italy. [Bonacorsi, D.; Braibant-Giacomelli, S.; Brigliadori, L.; Campanini, R.; Capiluppi, P.; Castro, A.; Chhibra, S. S.; Codispoti, G.; Cuffiani, M.; Fanfani, A.; Fasanella, D.; Guiducci, L.; Navarria, F. L.; Rossi, A. M.; Rovelli, T.; Siroli, G. P.; Tosi, N.] Univ Bologna, Bologna, Italy. [Chiorboli, M.; Costa, S.; Di Mattia, A.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] INFN Sez Catania, Catania, Italy. [Cappello, G.; Chiorboli, M.; Costa, S.; Giordano, F.; Potenza, R.; Tricomi, A.; Tuve, C.] Univ Catania, Catania, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Viliani, L.] INFN Sez Firenze, Florence, Italy. [Barbagli, G.; Ciulli, V.; Civinini, C.; D'Alessandro, R.; Focardi, E.; Gori, V.; Lenzi, P.; Meschini, M.; Paoletti, S.; Sguazzoni, G.; Viliani, L.] Univ Florence, Florence, Italy. [Fabbri, F.; Benussi, L.; Bianco, S.; Piccolo, D.; Primavera, F.] INFN Lab Nazl Frascati, Frascati, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] INFN Sez Genovaa, Genoa, Italy. [Calvelli, V.; Ferro, F.; Lo Vetere, M.; Monge, M. R.; Robutti, E.; Tosi, S.] Univ Genoa, Genoa, Italy. [Brianza, L.; Dinardo, M. E.; Fiorendi, S.; Gennai, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Malvezzi, S.; Manzoni, R. A.; Marzocchi, B.; Menasce, D.; Moroni, L.; Paganoni, M.; Pedrini, D.; Ragazzi, S.; Redaelli, N.; de Fatis, T. Tabarelli] INFN Sez Milano Bicocca, Milan, Italy. [Dinardo, M. E.; Fiorendi, S.; Gerosa, R.; Ghezzi, A.; Govoni, P.; Manzoni, R. A.; Marzocchi, B.; Paganoni, M.; Ragazzi, S.; de Fatis, T. Tabarelli] Univ Milano Bicocca, Milan, Italy. [Buontempo, S.; Cavallo, N.; Di Guida, S.; Esposito, M.; Fabozzi, F.; Iorio, A. O. M.; Lanza, G.; Lista, L.; Meola, S.; Merola, M.; Paolucci, P.; Sciacca, C.] INFN Sez Napoli, Naples, Italy. [Di Guida, S.; Esposito, M.; Iorio, A. O. M.; Sciacca, C.] Univ Naples Federico II, Naples, Italy. [Cavallo, F. R.; Fabozzi, F.] Univ Basilicata, Potenza, Italy. [Di Guida, S.; Meola, S.] Univ G Marconi, Rome, Italy. [Azzi, P.; Bacchetta, N.; Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Checchia, P.; Dall'Osso, M.; Dorigo, T.; Dosselli, U.; Fanzago, F.; Gasparini, F.; Gasparini, U.; Gozzelino, A.; Kanishchev, K.; Lacaprara, S.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Torassa, E.; Tosi, M.; Zanetti, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] INFN Sez Padova, Padua, Italy. [Benato, L.; Bisello, D.; Boletti, A.; Branca, A.; Carlin, R.; Dall'Osso, M.; Gasparini, F.; Gasparini, U.; Margoni, M.; Meneguzzo, A. T.; Pazzini, J.; Pozzobon, N.; Ronchese, P.; Simonetto, F.; Tosi, M.; Zotto, P.; Zucchetta, A.; Zumerle, G.] Univ Padua, Padua, Italy. [Kanishchev, K.] Univ Trento, Trento, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] INFN Sez Paviaa, Pavia, Italy. [Braghieri, A.; Magnani, A.; Montagna, P.; Ratti, S. P.; Re, V.; Riccardi, C.; Salvini, P.; Vai, I.; Vitulo, P.] Univ Pavia, Pavia, Italy. [Solestizi, L. Alunni; Bilei, G. M.; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Menichelli, M.; Saha, A.; Santocchia, A.] INFN Sez Perugia, Perugia, Italy. [Solestizi, L. Alunni; Ciangottini, D.; Fano, L.; Lariccia, P.; Mantovani, G.; Santocchia, A.] Univ Perugia, Perugia, Italy. [Androsov, K.; Azzurri, P.; Bagliesi, G.; Bernardini, J.; Boccali, T.; Castaldi, R.; Ciocci, M. A.; Dell'Orso, R.; Donato, S.; Foa, L.; Giassi, A.; Grippo, M. T.; Ligabue, F.; Lomtadze, T.; Martini, L.; Messineo, A.; Palla, F.; Rizzi, A.; Savoy-Navarro, A.; Serban, A. T.; Spagnolo, P.; Tenchini, R.; Tonelli, G.; Venturi, A.; Verdini, P. G.] INFN Sez Pisa, Pisa, Italy. [Martini, L.; Messineo, A.; Rizzi, A.; Tonelli, G.] Univ Pisa, Pisa, Italy. [Donato, S.; Foa, L.; Ligabue, F.] Scuola Normale Super Pisa, Pisa, Italy. [Barone, L.; Cavallari, F.; D'imperio, G.; Del Re, D.; Diemoz, M.; Gelli, S.; Jorda, C.; Longo, E.; Margaroli, F.; Meridiani, P.; Organtini, G.; Paramatti, R.; Preiato, F.; Rahatlou, S.; Rovelli, C.; Santanastasio, F.; Traczyk, P.] INFN Sez Romaa, Rome, Italy. [Barone, L.; D'imperio, G.; Del Re, D.; Gelli, S.; Longo, E.; Margaroli, F.; Organtini, G.; Preiato, F.; Rahatlou, S.; Santanastasio, F.; Traczyk, P.] Univ Rome, Rome, Italy. [Amapane, N.; Arcidiacono, R.; Argiro, S.; Arneodo, M.; Bellan, R.; Biino, C.; Cartiglia, N.; Costa, M.; Covarelli, R.; Degano, A.; Demaria, N.; Finco, L.; Kiani, B.; Mariotti, C.; Maselli, S.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Pastrone, N.; Pelliccioni, M.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Ruspa, M.; Sacchi, R.; Solano, A.; Staiano, A.] INFN Sez Torino, Turin, Italy. [Amapane, N.; Argiro, S.; Bellan, R.; Costa, M.; Covarelli, R.; Degano, A.; Finco, L.; Kiani, B.; Migliore, E.; Monaco, V.; Monteil, E.; Obertino, M. M.; Pacher, L.; Angioni, G. L. Pinna; Ravera, F.; Romero, A.; Sacchi, R.; Solano, A.] Univ Turin, Turin, Italy. [Arcidiacono, R.; Arneodo, M.; Ruspa, M.] Univ Piemonte Orientale, Novara, Italy. [Belforte, S.; Candelise, V.; Casarsa, M.; Cossutti, F.; Della Ricca, G.; Gobbo, B.; La Licata, C.; Marone, M.; Schizzi, A.; Zanetti, A.] INFN Sez Trieste, Trieste, Italy. [Belforte, S.; Candelise, V.; Della Ricca, G.; La Licata, C.; Marone, M.; Schizzi, A.] Univ Trieste, Trieste, Italy. [Kropivnitskaya, A.; Nam, S. K.] Kangwon Natl Univ, Chunchon, South Korea. [Kim, D. H.; Kim, G. N.; Kim, M. S.; Kong, D. J.; Lee, S.; Oh, Y. D.; Sakharov, A.; Son, D. C.] Kyungpook Natl Univ, Daegu, South Korea. [Cifuentes, J. A. Brochero; Kim, H.; Kim, T. J.] Chonbuk Natl Univ, Jeonju, South Korea. [Song, S.] Chonnam Natl Univ, Inst Universe & Elementary Particles, Kwangju, South Korea. [Lee, S.; Kim, H.; Cho, S.; Choi, S.; Go, Y.; Gyun, D.; Hong, B.; Kim, Y.; Lee, B.; Lee, K.; Lee, K. S.; Lim, J.; Park, S. K.; Roh, Y.] Korea Univ, Seoul, South Korea. [Yoo, H. D.] Seoul Natl Univ, Seoul, South Korea. [Choi, M.; Kim, J. H.; Lee, J. S. H.; Park, I. C.; Ryu, G.; Ryu, M. S.] Univ Seoul, Seoul, South Korea. [Choi, Y.; Goh, J.; Kim, D.; Kwon, E.; Lee, J.; Yu, I.] Sungkyunkwan Univ, Suwon, South Korea. [Dudenas, V.; Juodagalvis, A.; Vaitkus, J.] Vilnius Univ, Vilnius, Lithuania. [Ahmed, I.; Ibrahim, Z. A.; Komaragiri, J. R.; Ali, M. A. B. Md; Idris, F. Mohamad; Abdullah, W. A. T. Wan; Yusli, M. N.; Zolkapli, Z.] Univ Malaya, Natl Ctr Particle Phys, Kuala Lumpur, Malaysia. [Casimiro Linares, E.; Castilla-Valdez, H.; De La Cruz-Burelo, E.; Heredia-De La Cruz, I.; Hernandez-Almada, A.; Lopez-Fernandez, R.; Mejia Guisao, J.; Sanchez-Hernandez, A.] Ctr Invest & Estudios Avanzados IPN, Mexico City, DF, Mexico. [Carrillo Moreno, S.; Vazquez Valencia, F.] Univ Iberoamer, Mexico City, DF, Mexico. [Pedraza, I.; Salazar Ibarguen, A.] Benemerita Univ Autonoma Puebla, Puebla, Mexico. [Morelos Pineda, A.] Univ Autonoma San Luis Potosi, San Luis Potosi, Mexico. [Krofcheck, D.] Univ Auckland, Auckland, New Zealand. [Butler, P. H.] Univ Canterbury, Christchurch, New Zealand. [Ahmad, M.; Ahmad, A.; Hassan, Q.; Hoorani, H. R.; Khan, W. A.; Khurshid, T.; Shoaib, M.; Waqas, M.] Quaid I Azam Univ, Natl Ctr Phys, Islamabad, Pakistan. [Bialkowska, H.; Bluj, M.; Boimska, B.; Frueboes, T.; Gorski, M.; Kazana, M.; Nawrocki, K.; Romanowska-Rybinska, K.; Szleper, M.; Zalewski, P.] Natl Ctr Nucl Res, Otwock, Poland. [Brona, G.; Bunkowski, K.; Byszuk, A.; Doroba, K.; Kalinowski, A.; Konecki, M.; Krolikowski, J.; Misiura, M.; Olszewski, M.; Walczak, M.] Univ Warsaw, Inst Expt Phys, Fac Phys, Warsaw, Poland. [Bargassa, P.; Da Cruz E Silva, C. Beirao; Di Francesco, A.; Ferreira Parracho, P. G.; Gallinaro, M.; Hollar, J.; Leonardo, N.; Lloret Iglesias, L.; Nguyen, F.; Rodrigues Antunes, J.; Seixas, J.; Toldaiev, O.; Vadruccio, D.; Varela, J.; Vischia, P.] Lab Instrumentacao & Fis Expt Particulas, Lisbon, Portugal. [Afanasiev, S.; Bunin, P.; Gavrilenko, M.; Golutvin, I.; Gorbunov, I.; Kamenev, A.; Karjavin, V.; Lanev, A.; Malakhov, A.; Matveev, V.; Moisenz, P.; Palichik, V.; Perelygin, V.; Shmatov, S.; Shulha, S.; Skatchkov, N.; Smirnov, V.; Zarubin, A.] Joint Inst Nucl Res, Dubna, Russia. [Golovtsov, V.; Ivanov, Y.; Kim, V.; Kuznetsova, E.; Levchenko, P.; Murzin, V.; Oreshkin, V.; Smirnov, I.; Sulimov, V.; Uvarov, L.; Vavilov, S.; Vorobyev, A.] Petersburg Nucl Phys Inst, St Petersburg, Russia. [Andreev, Yu.; Dermenev, A.; Gninenko, S.; Golubev, N.; Karneyeu, A.; Kirsanov, M.; Krasnikov, N.; Pashenkov, A.; Tlisov, D.; Toropin, A.] Inst Nucl Res, Moscow, Russia. [Epshteyn, V.; Gavrilov, V.; Lychkovskaya, N.; Popov, V.; Pozdnyakov, I.; Safronov, G.; Spiridonov, A.; Vlasov, E.; Zhokin, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Chadeeva, M.; Chistov, R.; Danilov, M.; Rusinov, V.; Tarkovskii, E.] Natl Res Nucl Univ, Moscow Engn Phys Inst MEPhI, Moscow, Russia. [Andreev, V.; Azarkin, M.; Dremin, I.; Kirakosyan, M.; Leonidov, A.; Mesyats, G.; Rusakov, S. V.] PN Lebedev Phys Inst, Moscow, Russia. [Baskakov, A.; Belyaev, A.; Boos, E.; Ershov, A.; Gribushin, A.; Kaminskiy, A.; Kodolova, O.; Korotkikh, V.; Lokhtin, I.; Miagkov, I.; Obraztsov, S.; Petrushanko, S.; Savrin, V.; Snigirev, A.; Vardanyan, I.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Azhgirey, I.; Bayshev, I.; Bitioukov, S.; Kachanov, V.; Kalinin, A.; Konstantinov, D.; Krychkine, V.; Petrov, V.; Ryutin, R.; Sobol, A.; Tourtchanovitch, L.; Troshin, S.; Tyurin, N.; Uzunian, A.; Volkov, A.] State Res Ctr Russian Federat, Inst High Energy Phys, Protvino, Russia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Adzic, P.; Cirkovic, P.; Devetak, D.; Milosevic, J.; Rekovic, V.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Alcaraz Maestre, J.; Calvo, E.; Cerrada, M.; Chamizo Llatas, M.; Colino, N.; De La Cruz, B.; Delgado Peris, A.; Escalante Del Valle, A.; Fernandez Bedoya, C.; Fernandez Ramos, J. P.; Flix, J.; Fouz, M. C.; Garcia-Abia, P.; Gonzalez Lopez, O.; Goy Lopez, S.; Hernandez, J. M.; Josa, M. I.; Navarro De Martino, E.; Perez-Calero Yzquierdo, A.; Puerta Pelayo, J.; Quintario Olmeda, A.; Redondo, I.; Romero, L.; Soares, M. S.] CIEMAT, Madrid, Spain. [Albajar, C.; de Troconiz, J. F.; Missiroli, M.; Moran, D.] Univ Autonoma Madrid, Madrid, Spain. [Cuevas, J.; Fernandez Menendez, J.; Folgueras, S.; Gonzalez Caballero, I.; Palencia Cortezon, E.; Vizan Garcia, J. M.] Univ Oviedo, Oviedo, Spain. [Cabrillo, I. J.; Calderon, A.; Castineiras De Saa, J. R.; Curras, E.; De Castro Manzano, P.; Fernandez, M.; Garcia-Ferrero, J.; Gomez, G.; Lopez Virto, A.; Marco, J.; Marco, R.; Martinez Rivero, C.; Matorras, F.; Piedra Gomez, J.; Rodrigo, T.; Rodriguez-Marrero, A. Y.; Ruiz-Jimeno, A.; Scodellaro, L.; Trevisani, N.; Vila, I.; Vilar Cortabitarte, R.] Univ Cantabria, CSIC, Inst Fis Cantabria IFCA, Santander, Spain. [Abbaneo, D.; Auffray, E.; Auzinger, G.; Bachtis, M.; Baillon, P.; Ball, A. H.; Barney, D.; Benaglia, A.; Bendavid, J.; Benhabib, L.; Berruti, G. M.; Bloch, P.; Bocci, A.; Bonato, A.; Botta, C.; Breuker, H.; Camporesi, T.; Castello, R.; Cepeda, M.; Cerminara, G.; D'Alfonso, M.; d'Enterria, D.; Dabrowski, A.; Daponte, V.; David, A.; De Gruttola, M.; De Guio, F.; De Roeck, A.; De Visscher, S.; Di Marco, E.; Dobson, M.; Dordevic, M.; Dorney, B.; Du Pree, T.; Duggan, D.; Dunser, M.; Dupont, N.; Elliott-Peisert, A.; Franzoni, G.; Fulcher, J.; Funk, W.; Gigi, D.; Gill, K.; Giordano, D.; Girone, M.; Glege, F.; Guida, R.; Gundacker, S.; Guthoff, M.; Hammer, J.; Harris, P.; Hegeman, J.; Innocente, V.; Janot, P.; Kirschenmann, H.; Kortelainen, M. J.; Kousouris, K.; Krajczar, K.; Lecoq, P.; Lourenco, C.; Lucchini, M. T.; Magini, N.; Malgeri, L.; Mannelli, M.; Martelli, A.; Masetti, L.; Meijers, F.; Mersi, S.; Meschi, E.; Moortgat, F.; Morovic, S.; Mulders, M.; Nemallapudi, M. V.; Neugebauer, H.; Orfanelli, S.; Orsini, L.; Pape, L.; Perez, E.; Peruzzi, M.; Petrilli, A.; Petrucciani, G.; Pfeiffer, A.; Pierini, M.; Piparo, D.; Racz, A.; Reis, T.; Rolandi, G.; Rovere, M.; Ruan, M.; Sakulin, H.; Schafer, C.; Schwick, C.; Seidel, M.; Sharma, A.; Silva, P.; Simon, M.; Sphicas, P.; Steggemann, J.; Stieger, B.; Stoye, M.; Takahashi, Y.; Treille, D.; Triossi, A.; Tsirou, A.; Veres, G. I.; Wardle, N.; Wohri, H. K.; Zagozdzinska, A.; Zeuner, W. D.] CERN, European Org Nucl Res, Geneva, Switzerland. [Bertl, W.; Deiters, K.; Erdmann, W.; Horisberger, R.; Ingram, Q.; Kaestli, H. C.; Kotlinski, D.; Langenegger, U.; Rohe, T.] Paul Scherrer Inst, Villigen, Switzerland. [Bachmair, F.; Bani, L.; Bianchini, L.; Casal, B.; Dissertori, G.; Dittmar, M.; Donega, M.; Eller, P.; Grab, C.; Heidegger, C.; Hits, D.; Hoss, J.; Kasieczka, G.; Lecomte, P.; Lustermann, W.; Mangano, B.; Marionneau, M.; del Arbol, P. Martinez Ruiz; Masciovecchio, M.; Meinhard, M. T.; Meister, D.; Micheli, F.; Musella, P.; Nessi-Tedaldi, F.; Pandolfi, F.; Pata, J.; Pauss, F.; Perrin, G.; Perrozzi, L.; Quittnat, M.; Rossini, M.; Schonenberger, M.; Starodumov, A.; Takahashi, M.; Tavolaro, V. R.; Theofilatos, K.; Wallny, R.] Swiss Fed Inst Technol, Inst Particle Phys, Zurich, Switzerland. [Aarrestad, T. K.; Amsler, C.; Caminada, L.; Canelli, M. F.; Chiochia, V.; De Cosa, A.; Galloni, C.; Hinzmann, A.; Hreus, T.; Kilminster, B.; Lange, C.; Ngadiuba, J.; Pinna, D.; Rauco, G.; Robmann, P.; Salerno, D.; Yang, Y.] Univ Zurich, Zurich, Switzerland. [Chen, K. H.; Doan, T. H.; Jain, Sh.; Khurana, R.; Konyushikhin, M.; Kuo, C. M.; Lin, W.; Lu, Y. J.; Pozdnyakov, A.; Yu, S. S.] Natl Cent Univ, Chungli, Taiwan. [Kumar, Arun; Chang, P.; Chang, Y. H.; Chang, Y. W.; Chao, Y.; Chen, K. F.; Chen, P. H.; Dietz, C.; Fiori, F.; Grundler, U.; Hou, W. -S.; Hsiung, Y.; Liu, Y. F.; Lu, R. -S.; Moya, M. Minano; Petrakou, E.; Tsai, J. F.; Tzeng, Y. M.] Natl Taiwan Univ NTU, Taipei, Taiwan. [Asavapibhop, B.; Kovitanggoon, K.; Singh, G.; Srimanobhas, N.; Suwonjandee, N.] Chulalongkorn Univ, Dept Phys, Fac Sci, Bangkok, Thailand. [Adiguzel, A.; Damarseckin, S.; Demiroglu, Z. S.; Dozen, C.; Dumanoglu, I.; Girgis, S.; Gokbulut, G.; Guler, Y.; Gurpinar, E.; Hos, I.; Kangal, E. E.; Topaksu, A. Kayis; Onengut, G.; Ozdemir, K.; Ozturk, S.; Cerci, D. Sunar; Tali, B.; Topakli, H.; Zorbilmez, C.] Cukurova Univ, Adana, Turkey. [Bilin, B.; Bilmis, S.; Isildak, B.; Karapinar, G.; Yalvac, M.; Zeyrek, M.] Middle E Tech Univ, Dept Phys, Ankara, Turkey. [Gulmez, E.; Kaya, M.; Kaya, O.; Yetkin, E. A.; Yetkin, T.] Bogazici Univ, Istanbul, Turkey. [Cakir, A.; Cankocak, K.; Sen, S.; Vardarli, F. I.] Istanbul Tech Univ, Istanbul, Turkey. [Grynyov, B.] Natl Acad Sci Ukraine, Inst Scintillat Mat, Kharkov, Ukraine. [Levchuk, L.; Sorokin, P.] Kharkov Inst Phys & Technol, Natl Sci Ctr, Kharkov, Ukraine. [Aggleton, R.; Ball, F.; Beck, L.; Brooke, J. J.; Burns, D.; Clement, E.; Cussans, D.; Flacher, H.; Goldstein, J.; Grimes, M.; Heath, G. P.; Heath, H. F.; Jacob, J.; Kreczko, L.; Lucas, C.; Meng, Z.; Newbold, D. M.; Paramesvaran, S.; Poll, A.; Sakuma, T.; El Nasr-storey, S. Seif; Senkin, S.; Smith, D.; Smith, V. J.] Univ Bristol, Bristol, Avon, England. [Belyaev, A.; Brew, C.; Brown, R. M.; Calligaris, L.; Cieri, D.; Cockerill, D. J. A.; Coughlan, J. A.; Harder, K.; Harper, S.; Olaiya, E.; Petyt, D.; Shepherd-Themistocleous, C. H.; Thea, A.; Tomalin, I. R.; Williams, T.; Worm, S. D.] Rutherford Appleton Lab, Didcot, Oxon, England. [Baber, M.; Bainbridge, R.; Buchmuller, O.; Bundock, A.; Burton, D.; Casasso, S.; Citron, M.; Colling, D.; Corpe, L.; Dauncey, P.; Davies, G.; De Wit, A.; Della Negra, M.; Dunne, P.; Elwood, A.; Futyan, D.; Hall, G.; Iles, G.; Lane, R.; Lucas, R.; Lyons, L.; Magnan, A. -M.; Malik, S.; Nash, J.; Nikitenko, A.; Pela, J.; Pesaresi, M.; Raymond, D. M.; Richards, A.; Rose, A.; Seez, C.; Tapper, A.; Uchida, K.; Acosta, M. Vazquez; Virdee, T.; Zenz, S. C.] Imperial Coll, London, England. [Cole, J. E.; Hobson, P. R.; Khan, A.; Kyberd, P.; Leslie, D.; Reid, I. D.; Symonds, P.; Teodorescu, L.; Turner, M.] Brunel Univ, Uxbridge, Middx, England. [Borzou, A.; Call, K.; Dittmann, J.; Hatakeyama, K.; Liu, H.; Pastika, N.] Baylor Univ, Waco, TX 76798 USA. [Charaf, O.; Cooper, S. I.; Henderson, C.; Rumerio, P.] Univ Alabama, Tuscaloosa, AL USA. [Arcaro, D.; Avetisyan, A.; Bose, T.; Gastler, D.; Rankin, D.; Richardson, C.; Rohlf, J.; Sulak, L.; Zou, D.] Boston Univ, Boston, MA 02215 USA. [Alimena, J.; Benelli, G.; Berry, E.; Cutts, D.; Ferapontov, A.; Garabedian, A.; Hakala, J.; Heintz, U.; Jesus, O.; Laird, E.; Landsberg, G.; Mao, Z.; Narain, M.; Piperov, S.; Sagir, S.; Syarif, R.] Brown Univ, Providence, RI 02912 USA. [Chauhan, S.; Breedon, R.; Breto, G.; Sanchez, M. Calderon De la Barca; Chertok, M.; Conway, J.; Conway, R.; Cox, P. T.; Erbacher, R.; Funk, G.; Gardner, M.; Ko, W.; Lander, R.; Mclean, C.; Mulhearn, M.; Pellett, D.; Pilot, J.; Ricci-Tam, F.; Shalhout, S.; Smith, J.; Squires, M.; Stolp, D.; Tripathi, M.; Wilbur, S.; Yohay, R.] Univ Calif Davis, Davis, CA 95616 USA. [Weber, M.; Cousins, R.; Everaerts, P.; Florent, A.; Hauser, J.; Ignatenko, M.; Saltzberg, D.; Takasugi, E.; Valuev, V.] Univ Calif Los Angeles, Los Angeles, CA USA. [Burt, K.; Clare, R.; Ellison, J.; Gary, J. W.; Hanson, G.; Heilman, J.; Paneva, M. Ivova; Jandir, P.; Kennedy, E.; Lacroix, F.; Long, O. R.; Malberti, M.; Negrete, M. Olmedo; Shrinivas, A.; Wei, H.; Wimpenny, S.; Yates, B. R.] Univ Calif Riverside, Riverside, CA 92521 USA. [Sharma, V.; Branson, J. G.; Cerati, G. B.; Cittolin, S.; D'Agnolo, R. T.; Derdzinski, M.; Holzner, A.; Kelley, R.; Klein, D.; Letts, J.; Macneill, I.; Olivito, D.; Padhi, S.; Pieri, M.; Sani, M.; Simon, S.; Tadel, M.; Vartak, A.; Wasserbaech, S.; Welke, C.; Wurthwein, F.; Yagil, A.; Della Porta, G. Zevi] Univ Calif San Diego, La Jolla, CA 92093 USA. [Bradmiller-Feld, J.; Campagnari, C.; Dishaw, A.; Dutta, V.; Flowers, K.; Sevilla, M. Franco; Geffert, P.; George, C.; Golf, F.; Gouskos, L.; Gran, J.; Incandela, J.; Mccoll, N.; Mullin, S. D.; Richman, J.; Stuart, D.; Suarez, I.; West, C.; Yoo, J.] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. [Anderson, D.; Apresyan, A.; Bornheim, A.; Bunn, J.; Chen, Y.; Duarte, J.; Mott, A.; Newman, H. B.; Pena, C.; Spiropulu, M.; Vlimant, J. R.; Xie, S.; Zhu, R. Y.] CALTECH, Pasadena, CA 91125 USA. [Andrews, M. B.; Azzolini, V.; Calamba, A.; Carlson, B.; Ferguson, T.; Paulini, M.; Russ, J.; Sun, M.; Vogel, H.; Vorobiev, I.] Carnegie Mellon Univ, Pittsburgh, PA 15213 USA. [Cumalat, J. P.; Ford, W. T.; Gaz, A.; Jensen, F.; Johnson, A.; Krohn, M.; Mulholland, T.; Nauenberg, U.; Stenson, K.; Wagner, S. R.] Univ Colorado, Boulder, CO 80309 USA. [Alexander, J.; Chatterjee, A.; Chaves, J.; Chu, J.; Dittmer, S.; Eggert, N.; Mirman, N.; Kaufman, G. Nicolas; Patterson, J. R.; Rinkevicius, A.; Ryd, A.; Skinnari, L.; Soffi, L.; Sun, W.; Tan, S. M.; Teo, W. D.; Thom, J.; Thompson, J.; Tucker, J.; Weng, Y.; Wittich, P.] Cornell Univ, Ithaca, NY USA. [Banerjee, S.; Abdullin, S.; Albrow, M.; Apollinari, G.; Bauerdick, L. A. T.; Beretvas, A.; Berryhill, J.; Bhat, P. C.; Bolla, G.; Burkett, K.; Butler, J. N.; Cheung, H. W. K.; Chlebana, F.; Cihangir, S.; Elvira, V. D.; Fisk, I.; Freeman, J.; Gottschalk, E.; Gray, L.; Green, D.; Grunendahl, S.; Gutsche, O.; Hanlon, J.; Hare, D.; Harris, R. M.; Hasegawa, S.; Hirschauer, J.; Hu, Z.; Jayatilaka, B.; Jindariani, S.; Johnson, M.; Joshi, U.; Klima, B.; Kreis, B.; Lammel, S.; Lewis, J.; Linacre, J.; Lincoln, D.; Lipton, R.; Liu, T.; De Sa, R. Lopes; Lykken, J.; Maeshima, K.; Marraffino, J. M.; Maruyama, S.; Mason, D.; McBride, P.; Merkel, P.; Mrenna, S.; Nahn, S.; Newman-Holmes, C.; O'Dell, V.; Pedro, K.; Prokofyev, O.; Rakness, G.; Sexton-Kennedy, E.; Soha, A.; Spalding, W. J.; Spiegel, L.; Stoynev, S.; Strobbe, N.; Taylor, L.; Tkaczyk, S.; Tran, N. V.; Uplegger, L.; Vaandering, E. W.; Vernieri, C.; Verzocchi, M.; Vidal, R.; Wang, M.; Weber, H. A.; Whitbeck, A.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Acosta, D.; Avery, P.; Bortignon, P.; Bourilkov, D.; Brinkerhoff, A.; Carnes, A.; Carver, M.; Curry, D.; Das, S.; Field, R. D.; Furic, I. K.; Konigsberg, J.; Korytov, A.; Kotov, K.; Ma, P.; Matchev, K.; Mei, H.; Milenovic, P.; Mitselmakher, G.; Rank, D.; Rossin, R.; Shchutska, L.; Snowball, M.; Sperka, D.; Terentyev, N.; Thomas, L.; Wang, J.; Wang, S.; Yelton, J.] Univ Florida, Gainesville, FL USA. [Hewamanage, S.; Linn, S.; Markowitz, P.; Martinez, G.; Rodriguez, J. L.] Florida Int Univ, Miami, FL 33199 USA. [Ackert, A.; Adams, J. R.; Adams, T.; Askew, A.; Bein, S.; Bochenek, J.; Diamond, B.; Haas, J.; Hagopian, S.; Hagopian, V.; Johnson, K. F.; Khatiwada, A.; Prosper, H.; Weinberg, M.] Florida State Univ, Tallahassee, FL 32306 USA. [Baarmand, M. M.; Bhopatkar, V.; Colafranceschi, S.; Hohlmann, M.; Kalakhety, H.; Noonan, D.; Roy, T.; Yumiceva, F.] Florida Inst Technol, Melbourne, FL 32901 USA. [Adams, M. R.; Apanasevich, L.; Berry, D.; Betts, R. R.; Bucinskaite, I.; Cavanaugh, R.; Evdokimov, O.; Gauthier, L.; Gerber, C. E.; Hofman, D. J.; Kurt, P.; O'Brien, C.; Gonzalez, I. D. Sandoval; Turner, P.; Varelas, N.; Wu, Z.; Zakaria, M.; Zhang, J.] Univ Illinois, Chicago, IL USA. [Bilki, B.; Clarida, W.; Dilsiz, K.; Durgut, S.; Gandrajula, R. P.; Haytmyradov, M.; Khristenko, V.; Merlo, J. -P.; Mermerkaya, H.; Mestvirishvili, A.; Moeller, A.; Nachtman, J.; Ogul, H.; Onel, Y.; Ozok, F.; Penzo, A.; Snyder, C.; Tiras, E.; Wetzel, J.; Yi, K.] Univ Iowa, Iowa City, IA USA. [Anderson, I.; Barnett, B. A.; Blumenfeld, B.; Cocoros, A.; Eminizer, N.; Fehling, D.; Feng, L.; Gritsan, A. V.; Maksimovic, P.; Osherson, M.; Roskes, J.; Sarica, U.; Swartz, M.; Xiao, M.; Xin, Y.; You, C.] Johns Hopkins Univ, Baltimore, MD USA. [Baringer, P.; Bean, A.; Bruner, C.; Kenny, R. P., III; Majumder, D.; Malek, M.; Mcbrayer, W.; Murray, M.; Sanders, S.; Stringer, R.; Wang, Q.] Univ Kansas, Lawrence, KS 66045 USA. [Ivanov, A.; Kaadze, K.; Khalil, S.; Makouski, M.; Maravin, Y.; Mohammadi, A.; Saini, L. K.; Skhirtladze, N.; Toda, S.] Kansas State Univ, Manhattan, KS 66506 USA. [Lange, D.; Rebassoo, F.; Wright, D.] Lawrence Livermore Natl Lab, Livermore, CA USA. [Anelli, C.; Baden, A.; Baron, O.; Belloni, A.; Calvert, B.; Eno, S. C.; Ferraioli, C.; Gomez, J. A.; Hadley, N. J.; Jabeen, S.; Kellogg, R. G.; Kolberg, T.; Kunkle, J.; Lu, Y.; Mignerey, A. C.; Shin, Y. H.; Skuja, A.; Tonjes, M. B.; Tonwar, S. C.] Univ Maryland, College Pk, MD 20742 USA. [Wang, J.; Apyan, A.; Barbieri, R.; Baty, A.; Bi, R.; Bierwagen, K.; Brandt, S.; Busza, W.; Cali, I. A.; Demiragli, Z.; Di Matteo, L.; Ceballos, G. Gomez; Goncharov, M.; Gulhan, D.; Iiyama, Y.; Innocenti, G. M.; Klute, M.; Kovalskyi, D.; Lai, Y. S.; Lee, Y. -J.; Levin, A.; Luckey, P. D.; Marini, A. C.; Mcginn, C.; Mironov, C.; Narayanan, S.; Niu, X.; Paus, C.; Roland, C.; Roland, G.; Salfeld-Nebgen, J.; Stephans, G. S. F.; Sumorok, K.; Tatar, K.; Varma, M.; Velicanu, D.; Veverka, J.; Wang, T. W.; Wyslouch, B.; Yang, M.; Zhukova, V.] MIT, Cambridge, MA 02139 USA. [Benvenuti, A. C.; Dahmes, B.; Evans, A.; Finkel, A.; Gude, A.; Hansen, P.; Kalafut, S.; Kao, S. C.; Klapoetke, K.; Kubota, Y.; Lesko, Z.; Mans, J.; Nourbakhsh, S.; Ruckstuhl, N.; Rusack, R.; Tambe, N.; Turkewitz, J.] Univ Minnesota, Minneapolis, MN USA. [Acosta, J. G.; Oliveros, S.] Univ Mississippi, Oxford, MS USA. [Avdeeva, E.; Bartek, R.; Bloom, K.; Bose, S.; Claes, D. R.; Dominguez, A.; Fangmeier, C.; Suarez, R. Gonzalez; Kamalieddin, R.; Knowlton, D.; Kravchenko, I.; Meier, F.; Monroy, J.; Ratnikov, F.; Siado, J. E.; Snow, G. R.] Univ Nebraska, Lincoln, NE USA. [Alyari, M.; Dolen, J.; George, J.; Godshalk, A.; Harrington, C.; Iashvili, I.; Kaisen, J.; Kharchilava, A.; Kumar, A.; Rappoccio, S.; Roozbahani, B.] SUNY Buffalo, Buffalo, NY USA. [Zhang, J.; Alverson, G.; Barberis, E.; Baumgartel, D.; Chasco, M.; Hortiangtham, A.; Massironi, A.; Morse, D. M.; Nash, D.; Orimoto, T.; De Lima, R. Teixeira; Trocino, D.; Wang, R. -J.; Wood, D.] Northeastern Univ, Boston, MA 02115 USA. [Bhattacharya, S.; Hahn, K. A.; Kubik, A.; Low, J. F.; Mucia, N.; Odell, N.; Pollack, B.; Schmitt, M.; Sung, K.; Trovato, M.; Velasco, M.] Northwestern Univ, Evanston, IL USA. [Dev, N.; Hildreth, M.; Jessop, C.; Karmgard, D. J.; Kellams, N.; Lannon, K.; Marinelli, N.; Meng, F.; Mueller, C.; Musienko, Y.; Planer, M.; Reinsvold, A.; Ruchti, R.; Smith, G.; Taroni, S.; Valls, N.; Wayne, M.; Wolf, M.; Woodard, A.] Univ Notre Dame, Notre Dame, IN 46556 USA. [Antonelli, L.; Brinson, J.; Bylsma, B.; Durkin, L. S.; Flowers, S.; Hart, A.; Hill, C.; Hughes, R.; Ji, W.; Ling, T. Y.; Liu, B.; Luo, W.; Puigh, D.; Rodenburg, M.; Winer, B. L.; Wulsin, H. W.] Ohio State Univ, Columbus, OH 43210 USA. [Driga, O.; Elmer, P.; Hardenbrook, J.; Hebda, P.; Koay, S. A.; Lujan, P.; Marlow, D.; Medvedeva, T.; Mooney, M.; Olsen, J.; Palmer, C.; Piroue, P.; Stickland, D.; Tully, C.; Zuranski, A.] Princeton Univ, Princeton, NJ 08544 USA. [Malik, S.] Univ Puerto Rico, Mayaguez, PR USA. [Kumar, A.; Barker, A.; Barnes, V. E.; Benedetti, D.; Bortoletto, D.; Gutay, L.; Jha, M. K.; Jones, M.; Jung, A. W.; Jung, K.; Miller, D. H.; Neumeister, N.; Radburn-Smith, B. C.; Shi, X.; Shipsey, I.; Silvers, D.; Sun, J.; Svyatkovskiy, A.; Wang, F.; Xie, W.; Xu, L.] Purdue Univ, W Lafayette, IN 47907 USA. [Parashar, N.; Stupak, J.] Purdue Univ Calumet, Hammond, LA USA. [Adair, A.; Akgun, B.; Chen, Z.; Ecklund, K. M.; Geurts, F. J. M.; Guilbaud, M.; Li, W.; Michlin, B.; Northup, M.; Padley, B. P.; Redjimi, R.; Roberts, J.; Rorie, J.; Tu, Z.; Zabel, J.] Rice Univ, Houston, TX USA. [Betchart, B.; Bodek, A.; de Barbaro, P.; Demina, R.; Eshaq, Y.; Ferbel, T.; Galanti, M.; Garcia-Bellido, A.; Han, J.; Hindrichs, O.; Khukhunaishvili, A.; Lo, K. H.; Tan, P.; Verzetti, M.] Univ Rochester, Rochester, NY 14627 USA. [Chou, J. P.; Contreras-Campana, E.; Ferencek, D.; Gershtein, Y.; Halkiadakis, E.; Heindl, M.; Hidas, D.; Hughes, E.; Kaplan, S.; Elayavalli, R. Kunnawalkam; Lath, A.; Nash, K.; Saka, H.; Salur, S.; Schnetzer, S.; Sheffield, D.; Somalwar, S.; Stone, R.; Thomas, S.; Thomassen, P.; Walker, M.] Rutgers State Univ, Piscataway, NJ USA. [Foerster, M.; Riley, G.; Rose, K.; Spanier, S.; York, A.; Thapa, K.] Univ Tennessee, Knoxville, TN USA. [Rose, A.; Bouhali, O.; Hernandez, A. Castaneda; Celik, A.; Dalchenko, M.; De Mattia, M.; Delgado, A.; Dildick, S.; Eusebi, R.; Gilmore, J.; Huang, T.; Kamon, T.; Krutelyov, V.; Mueller, R.; Osipenkov, I.; Pakhotin, Y.; Patel, R.; Perloff, A.; Safonov, A.; Tatarinov, A.; Ulmer, K. A.] Texas A&M Univ, College Stn, TX USA. [Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P. R.; Faulkner, J.; Kunori, S.; Lamichhane, K.; Lee, S. W.; Libeiro, T.; Undleeb, S.; Volobouev, I.] Texas Tech Univ, Lubbock, TX 79409 USA. [Mao, Y.; Appelt, E.; Delannoy, A. G.; Greene, S.; Gurrola, A.; Janjam, R.; Johns, W.; Maguire, C.; Melo, A.; Ni, H.; Sheldon, P.; Tuo, S.; Velkovska, J.; Xu, Q.] Vanderbilt Univ, 221 Kirkland Hall, Nashville, TN 37235 USA. [Arenton, M. W.; Cox, B.; Francis, B.; Goodell, J.; Hirosky, R.; Ledovskoy, A.; Li, H.; Lin, C.; Neu, C.; Sinthuprasith, T.; Sun, X.; Wang, Y.; Wolfe, E.; Wood, J.; Xia, F.] Univ Virginia, Charlottesville, VA USA. [Clarke, C.; Harr, R.; Karchin, P. E.; Don, C. Kottachchi Kankanamge; Lamichhane, P.; Sturdy, J.] Wayne State Univ, Detroit, MI USA. [Sharma, A.; Belknap, D. A.; Carlsmith, D.; Dasu, S.; Dodd, L.; Duric, S.; Gomber, B.; Grothe, M.; Herndon, M.; Herve, A.; Klabbers, P.; Lanaro, A.; Levine, A.; Long, K.; Loveless, R.; Mohapatra, A.; Ojalvo, I.; Perry, T.; Pierro, G. A.; Polese, G.; Ruggles, T.; Sarangi, T.; Savin, A.; Smith, N.; Smith, W. H.; Taylor, D.; Verwilligen, P.; Woods, N.] Univ Wisconsin, Madison, WI USA. [Fruehwirth, R.; Jeitler, M.; Schieck, J.; Wulz, C. -E.] Vienna Univ Technol, Vienna, Austria. [Rabady, D.; Merlin, J. A.; Pantaleo, F.; Hartmann, F.; Kornmayer, A.; Szillasi, Z.; Mohanty, A. K.; Silvestris, L.; Battilana, C.; Tosi, N.; Viliani, L.; Primavera, F.; Manzoni, R. A.; Meola, S.; Paolucci, P.; Azzi, P.; Dall'Osso, M.; Pazzini, J.; Zucchetta, A.; Ciangottini, D.; Azzurri, P.; Donato, S.; D'imperio, G.; Del Re, D.; Traczyk, P.; Arcidiacono, R.; Finco, L.; Ulmer, K. A.] CERN, European Org Nucl Res, Geneva, Switzerland. [Zhang, F.] Peking Univ, State Key Lab Nucl Phys & Technol, Beijing, Peoples R China. [Beluffi, C.] Univ Strasbourg, Univ Haute Alsace Mulhouse, CNRS IN2P3, Inst Pluridisciplinaire Hubert Curien, Strasbourg, France. [Popov, A.; Zhukov, V.; Katkov, I.] Lomonosov Moscow State Univ, Skobeltsyn Inst Nucl Phys, Moscow, Russia. [Chinellato, J.; Tonelli Manganote, E. J.] Univ Estadual Campinas, Campinas, SP, Brazil. [Moon, C. S.] CNRS IN2P3, Paris, France. IN2P3 CNRS, Lab Leprince Ringuet, Ecole Polytech, Palaiseau, France. [Finger, M.; Finger, M., Jr.; Tsamalaidze, Z.] Joint Inst Nucl Res, Dubna, Russia. [Abdelalim, A. A.; Mahrous, A.] Helwan Univ, Cairo, Egypt. [Abdelalim, A. A.] Zewail City Sci & Technol, Zewail, Egypt. [Radi, A.] British Univ Egypt, Cairo, Egypt. [Radi, A.] Ain Shams Univ, Cairo, Egypt. [Agram, J. -L.; Conte, E.; Fontaine, J. -C.] Univ Haute Alsace, Mulhouse, France. [Toriashvili, T.] Tbilisi State Univ, Tbilisi, Rep of Georgia. [Borras, K.] Rhein Westfal TH Aachen, Phys Inst A 3, Aachen, Germany. [Gallo, E.] Univ Hamburg, Hamburg, Germany. [Hempel, M.; Karacheban, O.; Lohmann, W.] Brandenburg Tech Univ Cottbus, Cottbus, Germany. [Horvath, D.] Inst Nucl Res ATOMKI, Debrecen, Hungary. [Vesztergombi, G.; Veres, G. I.] Eotvos Lorand Univ, Budapest, Hungary. [Karancsi, J.] Univ Debrecen, Debrecen, Hungary. [Bartok, M.] Wigner Res Ctr Phys, Budapest, Hungary. [Choudhury, S.] Indian Inst Sci Educ & Res, Bhopal, India. [Bhowmik, S.; Maity, M.; Sarkar, T.] Visva Bharati Univ, Santini Ketan, W Bengal, India. [Gurtu, A.] King Abdulaziz Univ, Jeddah, Saudi Arabia. [Wickramage, N.] Univ Ruhuna, Matara, Sri Lanka. [Etesami, S. M.] Isfahan Univ Technol, Esfahan, Iran. [Fahim, A.] Univ Tehran, Dept Engn Sci, Tehran, Iran. [Safarzadeh, B.] Islamic Azad Univ, Sci & Res Branch, Plasma Phys Res Ctr, Tehran, Iran. [Ciocci, M. A.; Grippo, M. T.] Univ Siena, Siena, Italy. [Savoy-Navarro, A.] Purdue Univ, W Lafayette, IN 47907 USA. [Ali, M. A. B. Md] Int Islamic Univ Malaysia, Kuala Lumpur, Malaysia. [Idris, F. Mohamad] Agensi Nuklear Malaysia, MOSTI, Kajang, Malaysia. [Heredia-De La Cruz, I.] Consejo Nacl Ciencia & Technol, Mexico City, DF, Mexico. [Byszuk, A.; Zagozdzinska, A.] Warsaw Univ Technol, Inst Elect Syst, Warsaw, Poland. [Matveev, V.; Musienko, Y.] Inst Nucl Res, Moscow, Russia. [Matveev, V.; Azarkin, M.; Dremin, I.; Leonidov, A.] Natl Res Nucl Univ, MEPhI, Moscow, Russia. [Kim, V.] St Petersburg State Polytech Univ, St Petersburg, Russia. [Kaminskiy, A.] INFN Sez Padova, Padua, Italy. [Kaminskiy, A.] Univ Padua, Padua, Italy. [Kaminskiy, A.] Univ Trento, Trento, Italy. [Adzic, P.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Di Marco, E.] INFN Sez Roma, Rome, Italy. [Di Marco, E.] Univ Roma, Rome, Italy. [Orfanelli, S.] Natl Tech Univ Athens, Athens, Greece. [Rolandi, G.] Scuola Normale Sez INFN, Pisa, Italy. [Sphicas, P.] Univ Athens, Athens, Greece. [Starodumov, A.; Nikitenko, A.] Inst Theoret & Expt Phys, Moscow, Russia. [Amsler, C.] Albert Einstein Ctr Fundamental Phys, Bern, Switzerland. [Kangal, E. E.] Mersin Univ, Mersin, Turkey. [Onengut, G.] Cag Univ, Mersin, Turkey. [Ozdemir, K.] Piri Reis Univ, Istanbul, Turkey. [Ozturk, S.; Topakli, H.] Gaziosmanpasa Univ, Tokat, Turkey. [Cerci, D. Sunar; Tali, B.] Adiyaman Univ, Adiyaman, Turkey. [Isildak, B.] Ozyegin Univ, Istanbul, Turkey. [Karapinar, G.] Izmir Inst Technol, Izmir, Turkey. [Kaya, M.] Marmara Univ, Istanbul, Turkey. [Kaya, O.] Kafkas Univ, Kars, Turkey. [Yetkin, E. A.] Istanbul Bilgi Univ, Istanbul, Turkey. [Yetkin, T.] Yildiz Tech Univ, Istanbul, Turkey. [Sen, S.] Hacettepe Univ, Ankara, Turkey. [Newbold, D. M.; Belyaev, A.; Lucas, R.] Rutherford Appleton Lab, Didcot, Oxon, England. [Belyaev, A.; Acosta, M. Vazquez] Univ Southampton, Sch Phys & Astron, Southampton, Hants, England. [Acosta, M. Vazquez; Wasserbaech, S.] Inst Astrofis Canarias, San Cristobal la Laguna, Spain. [Wasserbaech, S.; Milenovic, P.] Utah Valley Univ, Orem, UT USA. [Milenovic, P.; Colafranceschi, S.] Univ Belgrade, Fac Phys, Belgrade, Serbia. [Milenovic, P.; Colafranceschi, S.] Univ Belgrade, Vinca Inst Nucl Sci, Belgrade, Serbia. [Colafranceschi, S.; Bilki, B.] Univ Rome, Fac Ingn, Rome, Italy. [Bilki, B.; Mermerkaya, H.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Mermerkaya, H.; Ozok, F.] Erzincan Univ, Erzincan, Turkey. [Ozok, F.; Bouhali, O.; Hernandez, A. Castaneda] Mimar Sinan Univ, Istanbul, Turkey. [Bouhali, O.; Hernandez, A. Castaneda; Kamon, T.] Texas A&M Univ Qatar, Doha, Qatar. [Kamon, T.] Kyungpook Natl Univ, Daegu, South Korea. RP Khachatryan, V (reprint author), Yerevan Phys Inst, Yerevan, Armenia. RI Goh, Junghwan/Q-3720-2016; Flix, Josep/G-5414-2012; Chistov, Ruslan/B-4893-2014; Ruiz, Alberto/E-4473-2011; Chadeeva, Marina/C-8789-2016; Nguyen, Federico/Q-8994-2016; Petrushanko, Sergey/D-6880-2012; Govoni, Pietro/K-9619-2016; Yazgan, Efe/C-4521-2014; Leonidov, Andrey/M-4440-2013; Paulini, Manfred/N-7794-2014; Smirnov, Vitaly/B-5001-2017; Moraes, Arthur/F-6478-2010; Calderon, Alicia/K-3658-2014; Della Ricca, Giuseppe/B-6826-2013; Manganote, Edmilson/K-8251-2013; Lokhtin, Igor/D-7004-2012; Raidal, Martti/F-4436-2012; Konecki, Marcin/G-4164-2015; Vogel, Helmut/N-8882-2014; Benussi, Luigi/O-9684-2014; Andreev, Vladimir/M-8665-2015; TUVE', Cristina/P-3933-2015; Xie, Si/O-6830-2016; Leonardo, Nuno/M-6940-2016; Ogul, Hasan/S-7951-2016; Dremin, Igor/K-8053-2015; Azarkin, Maxim/N-2578-2015; Danilov, Mikhail/C-5380-2014; Kirakosyan, Martin/N-2701-2015; Puljak, Ivica/D-8917-2017 OI Goh, Junghwan/0000-0002-1129-2083; Flix, Josep/0000-0003-2688-8047; Chistov, Ruslan/0000-0003-1439-8390; Ruiz, Alberto/0000-0002-3639-0368; Chadeeva, Marina/0000-0003-1814-1218; Nguyen, Federico/0000-0002-6713-1596; Govoni, Pietro/0000-0002-0227-1301; Yazgan, Efe/0000-0001-5732-7950; Paulini, Manfred/0000-0002-6714-5787; Moraes, Arthur/0000-0002-5157-5686; Della Ricca, Giuseppe/0000-0003-2831-6982; Konecki, Marcin/0000-0001-9482-4841; Vogel, Helmut/0000-0002-6109-3023; Benussi, Luigi/0000-0002-2363-8889; TUVE', Cristina/0000-0003-0739-3153; Xie, Si/0000-0003-2509-5731; Leonardo, Nuno/0000-0002-9746-4594; Ogul, Hasan/0000-0002-5121-2893; Danilov, Mikhail/0000-0001-9227-5164; FU Austrian Federal Ministry of Science, Research and Economy; Austrian Science Fund; Belgian Fonds de la Recherche Scientifique; Fonds voor Wetenschappelijk Onderzoek; CNPq; CAPES; FAPERJ; FAPESP; Bulgarian Ministry of Education and Science; CERN; Chinese Academy of Sciences; Ministry of Science and Technology; National Natural Science Foundation of China; Colombian Funding Agency (COLCIENCIAS); Croatian Ministry of Science, Education and Sport; Croatian Science Foundation; Research Promotion Foundation, Cyprus; Ministry of Education and Research; Estonian Research Council [IUT23-4, IUT23-6]; European Regional Development Fund, Estonia; Academy of Finland; Finnish Ministry of Education and Culture; Helsinki Institute of Physics; Institut National de Physique Nucleaire et de Physique des Particules/CNRS; Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; Bundesministerium fur Bildung und Forschung; Deutsche Forschungsgemeinschaft; Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; General Secretariat for Research and Technology, Greece; National Scientific Research Foundation, and National Innovation Office, Hungary; Department of Atomic Energy, India; Department of Science and Technology, India; Institute for Studies in Theoretical Physics and Mathematics, Iran; Science Foundation, Ireland; Istituto Nazionale di Fisica Nucleare, Italy; Ministry of Science, ICT and Future Planning, Republic of Korea; National Research Foundation (NRF), Republic of Korea; Lithuanian Academy of Sciences; Ministry of Education; University of Malaya (Malaysia); CINVESTAV; CONACYT; SEP; UASLP-FAI; Ministry of Business, Innovation and Employment, New Zealand; Pakistan Atomic Energy Commission; Ministry of Science and Higher Education, Poland; National Science Centre, Poland; Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; Ministry of Education and Science of the Russian Federation; Federal Agency of Atomic Energy of the Russian Federation; Russian Academy of Sciences; Russian Foundation for Basic Research; Ministry of Education, Science and Technological Development of Serbia; Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio, Spain; ETH Board; ETH Zurich; PSI; SNF; UniZH; Canton Zurich; SER; Ministry of Science and Technology, Taipei; Thailand Center of Excellence in Physics; Institute for the Promotion of Teaching Science and Technology of Thailand; Special Task Force for Activating Research; National Science and Technology Development Agency of Thailand; Scientific and Technical Research Council of Turkey; Turkish Atomic Energy Authority; National Academy of Sciences of Ukraine; State Fund for Fundamental Researches, Ukraine; Science and Technology Facilities Council, UK; US Department of Energy; US National Science Foundation; Marie-Curie program; European Research Council; EPLANET(European Union); Leventis Foundation; A. P. Sloan Foundation; Alexander von Humboldt Foundation; Belgian Federal Science Policy Office; Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; Council of Science and Industrial Research, India; HOMING PLUS program of the Foundation for Polish Science - European Union; OPUS program of the National Science Center (Poland); Compagnia di San Paolo (Torino); MIUR (Italy) [20108T4XTM]; EU-ESF; Greek NSRF; National Priorities Research Program by Qatar National Research Fund; Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); Welch Foundation [C-1845] FX We congratulate our colleagues in the CERN accelerator departments for the excellent performance of the LHC and thank the technical and administrative staffs at CERN and at other CMS institutes for their contributions to the success of the CMS effort. In addition, we gratefully acknowledge the computing centers and personnel of the Worldwide LHC Computing Grid for delivering so effectively the computing infrastructure essential to our analyses.; Finally, we acknowledge the enduring support for the construction and operation of the LHC and the CMS detector provided by the following funding agencies: the Austrian Federal Ministry of Science, Research and Economy and the Austrian Science Fund; the Belgian Fonds de la Recherche Scientifique, and Fonds voor Wetenschappelijk Onderzoek; the Brazilian Funding Agencies (CNPq, CAPES, FAPERJ, and FAPESP); the Bulgarian Ministry of Education and Science; CERN; the Chinese Academy of Sciences, Ministry of Science and Technology, and National Natural Science Foundation of China; the Colombian Funding Agency (COLCIENCIAS); the Croatian Ministry of Science, Education and Sport, and the Croatian Science Foundation; the Research Promotion Foundation, Cyprus; the Ministry of Education and Research, Estonian Research Council via IUT23-4 and IUT23-6 and European Regional Development Fund, Estonia; the Academy of Finland, Finnish Ministry of Education and Culture, and Helsinki Institute of Physics; the Institut National de Physique Nucleaire et de Physique des Particules/CNRS, and Commissariat a l'Energie Atomique et aux Energies Alternatives/CEA, France; the Bundesministerium fur Bildung und Forschung, Deutsche Forschungsgemeinschaft, and Helmholtz-Gemeinschaft Deutscher Forschungszentren, Germany; the General Secretariat for Research and Technology, Greece; the National Scientific Research Foundation, and National Innovation Office, Hungary; the Department of Atomic Energy and the Department of Science and Technology, India; the Institute for Studies in Theoretical Physics and Mathematics, Iran; the Science Foundation, Ireland; the Istituto Nazionale di Fisica Nucleare, Italy; the Ministry of Science, ICT and Future Planning, and National Research Foundation (NRF), Republic of Korea; the Lithuanian Academy of Sciences; the Ministry of Education, and University of Malaya (Malaysia); the Mexican Funding Agencies (CINVESTAV, CONACYT, SEP, and UASLP-FAI); the Ministry of Business, Innovation and Employment, New Zealand; the Pakistan Atomic Energy Commission; the Ministry of Science and Higher Education and the National Science Centre, Poland; the Fundacao para a Ciencia e a Tecnologia, Portugal; JINR, Dubna; the Ministry of Education and Science of the Russian Federation, the Federal Agency of Atomic Energy of the Russian Federation, Russian Academy of Sciences, and the Russian Foundation for Basic Research; the Ministry of Education, Science and Technological Development of Serbia; the Secretaria de Estado de Investigacion, Desarrollo e Innovacion and Programa Consolider-Ingenio 2010, Spain; the Swiss Funding Agencies (ETH Board, ETH Zurich, PSI, SNF, UniZH, Canton Zurich, and SER); the Ministry of Science and Technology, Taipei; the Thailand Center of Excellence in Physics, the Institute for the Promotion of Teaching Science and Technology of Thailand, Special Task Force for Activating Research and the National Science and Technology Development Agency of Thailand; the Scientific and Technical Research Council of Turkey, and Turkish Atomic Energy Authority; the National Academy of Sciences of Ukraine, and State Fund for Fundamental Researches, Ukraine; the Science and Technology Facilities Council, UK; the US Department of Energy, and the US National Science Foundation. Individuals have received support from the Marie-Curie program and the European Research Council and EPLANET(European Union); the Leventis Foundation; the A. P.; Sloan Foundation; the Alexander von Humboldt Foundation; the Belgian Federal Science Policy Office; the Fonds pour la Formation a la Recherche dans l'Industrie et dans l'Agriculture (FRIA-Belgium); the Agentschap voor Innovatie door Wetenschap en Technologie (IWT-Belgium); the Ministry of Education, Youth and Sports (MEYS) of the Czech Republic; the Council of Science and Industrial Research, India; the HOMING PLUS program of the Foundation for Polish Science, cofinanced from European Union, Regional Development Fund; the OPUS program of the National Science Center (Poland); the Compagnia di San Paolo (Torino); MIUR project 20108T4XTM (Italy); the Thalis and Aristeia programs cofinanced by EU-ESF and the Greek NSRF; the National Priorities Research Program by Qatar National Research Fund; the Rachadapisek Sompot Fund for Postdoctoral Fellowship, Chulalongkorn University (Thailand); the Chulalongkorn Academic into Its 2nd Century Project Advancement Project (Thailand); and the Welch Foundation, contract C-1845. NR 57 TC 0 Z9 0 U1 20 U2 31 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 1434-6044 EI 1434-6052 J9 EUR PHYS J C JI Eur. Phys. J. C PD JUL 4 PY 2016 VL 76 IS 7 AR 372 DI 10.1140/epjc/s10052-016-4205-7 PG 25 WC Physics, Particles & Fields SC Physics GA DR1EK UT WOS:000379648600001 PM 28280445 ER PT J AU Zhang, SG Li, HX Appel, AM Hall, MB Bullock, RM AF Zhang, Shaoguang Li, Haixia Appel, Aaron M. Hall, Michael B. Bullock, R. Morris TI Facile P-C/C-H Bond-Cleavage Reactivity of Nickel Bis(diphosphine) Complexes SO CHEMISTRY-A EUROPEAN JOURNAL LA English DT Article DE C-H bond cleavage; density functional calculations; nickel; P-C bond cleavage; phosphines ID C-H; PINCER COMPLEXES; PENDANT AMINES; ELECTROCATALYTIC OXIDATION; COORDINATION CHEMISTRY; CATALYST DEACTIVATION; MOLECULAR-STRUCTURE; DIPHOSPHINE LIGAND; ACTIVATION; HYDRIDE AB Unusual cleavage of P-C and C-H bonds of the P2N2 ligand, in heteroleptic [Ni(P2N2)(diphosphine)](2+) complexes under mild conditions, results in the formation of an iminium formyl nickelate featuring a C,P,P-tridentate coordination mode. The structures of both the heteroleptic [Ni(P2N2)(diphosphine)](2+) complexes and the resulting iminium formyl nickelate have been characterized by NMR spectroscopy and single-crystal X-ray diffraction analysis. Density functional theory (DFT) calculations were employed to investigate the mechanism of the P-C/C-H bond cleavage, which involves C-H bond cleavage, hydride rotation, Ni-C/P-H bond formation, and P-C bond cleavage. C1 [Zhang, Shaoguang; Appel, Aaron M.; Bullock, R. Morris] Pacific Northwest Natl Lab, POB 999,K2-12, Richland, WA 99352 USA. [Li, Haixia; Hall, Michael B.] Texas A&M Univ, Dept Chem, College Stn, TX 77845 USA. RP Bullock, RM (reprint author), Pacific Northwest Natl Lab, POB 999,K2-12, Richland, WA 99352 USA.; Hall, MB (reprint author), Texas A&M Univ, Dept Chem, College Stn, TX 77845 USA. EM mbhall@tamu.edu; morris.bullock@pnnl.gov OI Appel, Aaron/0000-0002-5604-1253 FU U.S. Department of Energy, Office of Science (Office of Basic Energy Sciences); U.S. Department of Energy, Office of Science (Division of Chemical Sciences, Geosciences Biosciences); National Science Foundation [CHE-1300787]; Welch Foundation [A-0648] FX The research at Pacific Northwest National Laboratory (PNNL) was supported by the U.S. Department of Energy, Office of Science (Office of Basic Energy Sciences; Division of Chemical Sciences, Geosciences & Biosciences). The PNNL is operated by Battelle for the US Department of Energy. H.L. and M.B.H. thank the National Science Foundation (CHE-1300787) and the Welch Foundation (A-0648) for financial support and the Texas A&M Supercomputing Facility for providing computing resources. NR 43 TC 0 Z9 0 U1 11 U2 18 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 0947-6539 EI 1521-3765 J9 CHEM-EUR J JI Chem.-Eur. J. PD JUL 4 PY 2016 VL 22 IS 28 BP 9493 EP 9497 DI 10.1002/chem.201601469 PG 5 WC Chemistry, Multidisciplinary SC Chemistry GA DS0FS UT WOS:000380271400006 PM 27189413 ER PT J AU Liu, FC Shadike, Z Wang, XF Shi, SQ Zhou, YN Chen, GY Yang, XQ Weng, LH Zhao, JT Fu, ZW AF Liu, Fang-Chao Shadike, Zulipiya Wang, Xiao-Fang Shi, Si-Qi Zhou, Yong-Ning Chen, Guo-Ying Yang, Xiao-Qing Weng, Lin-Hong Zhao, Jing-Tai Fu, Zheng-Wen TI A Novel Small-Molecule Compound of Lithium Iodine and 3-Hydroxypropionitride as a Solid-State Electrolyte for Lithium-Air Batteries SO INORGANIC CHEMISTRY LA English DT Article ID PERFORMANCE; MEMBRANES AB A novel small-molecule compound of lithium iodine and 3-hydroxypropionitrile (HPN) has been successfully synthesized. Our combined experimental and theoretical studies indicated that LiIHPN is a Li-ion conductor, which is utterly different from the I--anion conductor of LiI(HPN)(2) reported previously. Solid-state lithium-air batteries based on LiIHPN as the electrolyte exhibit a reversible discharge capacity of more than 2100 mAh g(-1) with a cyclic performance over 10 cycles. Our findings provide a new way to design solid-state electrolytes toward high-performance lithium-air batteries. C1 [Liu, Fang-Chao; Shadike, Zulipiya; Chen, Guo-Ying; Weng, Lin-Hong; Fu, Zheng-Wen] Fudan Univ, Dept Chem, Shanghai Key Lab Mol Catalysts & Innovat Mat, Shanghai 200433, Peoples R China. [Liu, Fang-Chao; Shadike, Zulipiya; Chen, Guo-Ying; Weng, Lin-Hong; Fu, Zheng-Wen] Fudan Univ, Laser Chem Inst, Shanghai 200433, Peoples R China. [Zhou, Yong-Ning] Fudan Univ, Dept Mat Sci, Shanghai 200433, Peoples R China. [Wang, Xiao-Fang; Shi, Si-Qi; Zhao, Jing-Tai] Shanghai Univ, Sch Mat Sci & Engn, Shanghai 200444, Peoples R China. [Yang, Xiao-Qing] Brookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA. RP Fu, ZW (reprint author), Fudan Univ, Dept Chem, Shanghai Key Lab Mol Catalysts & Innovat Mat, Shanghai 200433, Peoples R China.; Fu, ZW (reprint author), Fudan Univ, Laser Chem Inst, Shanghai 200433, Peoples R China.; Shi, SQ; Zhao, JT (reprint author), Shanghai Univ, Sch Mat Sci & Engn, Shanghai 200444, Peoples R China. EM sqshi@shu.edu.cn; jtzhao@mail.sic.ac.cn; zwfu@fudan.edu.cn RI Shi, Siqi/E-1245-2011; LIU, FANGCHAO/D-8137-2017 FU NSAF [U1430104, 51372228]; Science & Technology Commission of Shanghai Municipality [08DZ2270500]; Shanghai Pujiang Program [14PJ1403900]; U.S. Department of Energy, the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies [DE-SC0012704] FX This work was financially supported by the NSAF (Grants U1430104 and 51372228), Science & Technology Commission of Shanghai Municipality (Grant 08DZ2270500), and Shanghai Pujiang Program (Grant 14PJ1403900). All of the computations were performed on the high-performance computing platform of Shanghai University. The work at Brookhaven National Laboratory was supported by the U.S. Department of Energy, the Assistant Secretary for Energy Efficiency and Renewable Energy, Office of Vehicle Technologies, under Contract DE-SC0012704. NR 28 TC 0 Z9 0 U1 23 U2 47 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0020-1669 EI 1520-510X J9 INORG CHEM JI Inorg. Chem. PD JUL 4 PY 2016 VL 55 IS 13 BP 6504 EP 6510 DI 10.1021/acs.inorgchem.6b00564 PG 7 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DQ8JC UT WOS:000379455900021 PM 27308962 ER PT J AU Capece, AM Patino, MI Raitses, Y Koel, BE AF Capece, A. M. Patino, M. I. Raitses, Y. Koel, B. E. TI Secondary electron emission from lithium and lithium compounds SO APPLIED PHYSICS LETTERS LA English DT Article ID MAGNETIC-FIELD; PLASMA; SURFACES; TARGETS AB In this work, measurements of electron-induced secondary electron emission ( SEE) yields of lithium as a function of composition are presented. The results are particularly relevant for magnetic fusion devices such as tokamaks, field-reversed configurations, and stellarators that consider Li as a plasma-facing material for improved plasma confinement. SEE can reduce the sheath potential at the wall and cool electrons at the plasma edge, resulting in large power losses. These effects become significant as the SEE coefficient, gamma(e), approaches one, making it imperative to maintain a low yield surface. This work demonstrates that the yield from Li strongly depends on chemical composition and substantially increases after exposure to oxygen and water vapor. The total yield was measured using a retarding field analyzer in ultrahigh vacuum for primary electron energies of 20-600 eV. The effect of Li composition was determined by introducing controlled amounts of O-2 and H2O vapor while monitoring film composition with Auger electron spectroscopy and temperature programmed desorption. The results show that the energy at which gamma(e) = 1 decreases with oxygen content and is 145 eV for a Li film that is 17% oxidized and drops to less than 25 eV for a fully oxidized film. This work has important implications for laboratory plasmas operating under realistic vacuum conditions in which oxidation significantly alters the electron emission properties of Li walls. Published by AIP Publishing. C1 [Capece, A. M.; Patino, M. I.; Raitses, Y.] Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. [Capece, A. M.] Coll New Jersey, Dept Phys, Ewing, NJ 08628 USA. [Koel, B. E.] Princeton Univ, Dept Chem & Biol Engn, Princeton, NJ 08540 USA. [Patino, M. I.] Univ Calif Los Angeles, Dept Mech & Aerosp Engn, Los Angeles, CA 90095 USA. RP Capece, AM (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA.; Capece, AM (reprint author), Coll New Jersey, Dept Phys, Ewing, NJ 08628 USA. EM capecea@tcnj.edu OI Koel, Bruce/0000-0002-0032-4991 FU DOE [DE-AC02-09CH11466]; AFOSR [FA9550-11-1-0282, AF9550-09-1-0695]; DOE Office of Science Graduate Student Research Program; U.S. Department of Energy, Office of Science/Fusion Energy Sciences [DE-SC0012890] FX The authors would like to thank Alex Merzhevskiy for technical assistance. This work was supported by DOE Contract No. DE-AC02-09CH11466, AFOSR Grant Nos. FA9550-11-1-0282 and AF9550-09-1-0695, and DOE Office of Science Graduate Student Research Program. B. E. Koel acknowledges support of this work by the U.S. Department of Energy, Office of Science/Fusion Energy Sciences, under Award No. DE-SC0012890. NR 33 TC 0 Z9 0 U1 7 U2 16 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0003-6951 EI 1077-3118 J9 APPL PHYS LETT JI Appl. Phys. Lett. PD JUL 4 PY 2016 VL 109 IS 1 AR 011605 DI 10.1063/1.4955461 PG 5 WC Physics, Applied SC Physics GA DR0GW UT WOS:000379587000009 ER PT J AU Diehl, AD Meehan, TF Bradford, YM Brush, MH Dahdul, WM Dougall, DS He, YQ Osumi-Sutherland, D Ruttenberg, A Sarntivijai, S Van Slyke, CE Vasilevsky, NA Haendel, MA Blake, JA Mungall, CJ AF Diehl, Alexander D. Meehan, Terrence F. Bradford, Yvonne M. Brush, Matthew H. Dahdul, Wasila M. Dougall, David S. He, Yongqun Osumi-Sutherland, David Ruttenberg, Alan Sarntivijai, Sirarat Van Slyke, Ceri E. Vasilevsky, Nicole A. Haendel, Melissa A. Blake, Judith A. Mungall, Christopher J. TI The Cell Ontology 2016: enhanced content, modularization, and ontology interoperability SO JOURNAL OF BIOMEDICAL SEMANTICS LA English DT Article ID MAMMALIAN EXPRESSION ATLAS; MODEL ORGANISM DATABASE; FLOW-CYTOMETRY DATA; GENE ONTOLOGY; ANATOMY ONTOLOGY; INTEGRATION; SUPPORT; UNIFICATION; IMMUNOLOGY; ENTITIES AB Background: The Cell Ontology (CL) is an OBO Foundry candidate ontology covering the domain of canonical, natural biological cell types. Since its inception in 2005, the CL has undergone multiple rounds of revision and expansion, most notably in its representation of hematopoietic cells. For in vivo cells, the CL focuses on vertebrates but provides general classes that can be used for other metazoans, which can be subtyped in species-specific ontologies. Construction and content: Recent work on the CL has focused on extending the representation of various cell types, and developing new modules in the CL itself, and in related ontologies in coordination with the CL. For example, the Kidney and Urinary Pathway Ontology was used as a template to populate the CL with additional cell types. In addition, subtypes of the class 'cell in vitro' have received improved definitions and labels to provide for modularity with the representation of cells in the Cell Line Ontology and Reagent Ontology. Recent changes in the ontology development methodology for CL include a switch from OBO to OWL for the primary encoding of the ontology, and an increasing reliance on logical definitions for improved reasoning. Utility and discussion: The CL is now mandated as a metadata standard for large functional genomics and transcriptomics projects, and is used extensively for annotation, querying, and analyses of cell type specific data in sequencing consortia such as FANTOM5 and ENCODE, as well as for the NIAID ImmPort database and the Cell Image Library. The CL is also a vital component used in the modular construction of other biomedical ontologies-for example, the Gene Ontology and the cross-species anatomy ontology, Uberon, use CL to support the consistent representation of cell types across different levels of anatomical granularity, such as tissues and organs. Conclusions: The ongoing improvements to the CL make it a valuable resource to both the OBO Foundry community and the wider scientific community, and we continue to experience increased interest in the CL both among developers and within the user community. C1 [Diehl, Alexander D.] Univ Buffalo, Sch Med & Biomed Sci, Dept Neurol, Buffalo, NY USA. [Meehan, Terrence F.; Osumi-Sutherland, David; Sarntivijai, Sirarat] European Mol Biol Lab, European Bioinformat Inst, Cambridge CB10 1SD, England. [Bradford, Yvonne M.; Van Slyke, Ceri E.] 5291 Univ Oregon, ZFIN, Zebrafish Model Organism Database, Eugene, OR 97403 USA. [Brush, Matthew H.; Vasilevsky, Nicole A.; Haendel, Melissa A.] Oregon Hlth & Sci Univ, Ontol Dev Grp, Lib, Portland, OR 97239 USA. [Dahdul, Wasila M.] Univ S Dakota, Dept Biol, Vermillion, SD 57069 USA. [Dahdul, Wasila M.] Natl Evolutionary Synth Ctr, Durham, NC 27705 USA. [Dougall, David S.] Univ Texas, Southwestern Med Ctr, Dallas, TX 75235 USA. [He, Yongqun] Univ Michigan, Sch Med, Unit Lab Anim Med, Ann Arbor, MI 48109 USA. [Ruttenberg, Alan] Univ Buffalo, Sch Dent Med, Oral Diagnost Sci, Buffalo, NY USA. [Blake, Judith A.] Jackson Lab, Bar Harbor, ME 04609 USA. [Mungall, Christopher J.] Lawrence Berkeley Natl Lab, Genom Div, Berkeley, CA 94720 USA. RP Diehl, AD (reprint author), Univ Buffalo, Sch Med & Biomed Sci, Dept Neurol, Buffalo, NY USA. EM addiehl@buffalo.edu OI Dahdul, Wasila/0000-0003-3162-7490; Sarntivijai, Sirarat/0000-0002-2548-641X; Meehan, Terrence/0000-0003-1980-3228; Vasilevsky, Nicole/0000-0001-5208-3432 FU NHGRI [HG002273-09Z, HG002273]; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; NIGMS [2R01GM080646-06]; NIAID [HHSN272201200028C]; NIH [HG002659, 1R01AI081062]; NIH Office of the Director [1R24OD011883]; NSF [DBI-0641025, DBI-1062404, DBI-1062542]; National Evolutionary Synthesis Center [NSF EF-0423641, NSF EF-0905606]; International Neuroinformatics Coordinating Facility FX We would kindly thank Barry Smith, Lindsay Cowell, Anna Maria Masci, Richard Scheuermann, Jose Mejino, David Hill, Terry Hayamizu, Morgan Hightshoe, Wade Valleau, Jane Lomax, Paola Roncaglia, Tanya Berardini, Heiko Dietze, Maryann Martone, Stephan Larson, Gordon Shepherd, Jyl Boline, Mihail Bota, Giorgio Ascoli, Paul Katz, Robert Burgess, Patrick Ray, Jonathan Bona, Paula Mabee, Laurel Cooper, Ramona Walls, Pankaj Jaiswal, Darren Natale, Cathy Wu, Cecilia Arighi, Alistair Forrest, Hideya Kawaji, Helen Parkison, Simon Jupp, Robert Stevens, Ryan Brinkmann, Melanie Courtot, Raphael Gottardo, Cliburn Chan, Jie Zheng, Shai Shen-Orr, and Yannick Pouliot, for discussions about and contributions to the Cell Ontology project. ADD, TFM, CJM, and JAB were supported by NHGRI grants HG002273-09Z and HG002273 for portions of this work. CJM's work was supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. ADD and AR are supported by NIGMS grant 2R01GM080646-06 and NIAID contract HHSN272201200028C for portions of this work. YMB and CVS are supported by NIH HG002659 for portions of this work. MAH, MHB, and NAV are supported for portion of this work by 1R24OD011883 from the NIH Office of the Director. WD is supported by NSF grants DBI-0641025, DBI-1062404, and DBI-1062542, and by the National Evolutionary Synthesis Center under NSF EF-0423641 and NSF EF-0905606 for portions of this work. YH was supported by NIH 1R01AI081062. Any opinions, findings, and conclusions or recommendations expressed in this material are those of the author(s) and do not necessarily reflect the views of the National Science Foundation or the National Institutes of Health. We gratefully acknowledge the support of the International Neuroinformatics Coordinating Facility for portions of this work. NR 66 TC 3 Z9 3 U1 5 U2 7 PU BIOMED CENTRAL LTD PI LONDON PA 236 GRAYS INN RD, FLOOR 6, LONDON WC1X 8HL, ENGLAND SN 2041-1480 J9 J BIOMED SEMANT JI J. Biomed. Semant. PD JUL 4 PY 2016 VL 7 AR 44 DI 10.1186/s13326-016-0088-7 PG 10 WC Mathematical & Computational Biology SC Mathematical & Computational Biology GA DQ3OX UT WOS:000379112700001 PM 27377652 ER PT J AU Waldspurger, C Berger, E Bhattacharjee, A Pedretti, K Peter, S Rossbach, C AF Waldspurger, Carl Berger, Emery Bhattacharjee, Abhishek Pedretti, Kevin Peter, Simon Rossbach, Chris TI Sweet Spots and Limits for Virtualization SO ACM SIGPLAN NOTICES LA English DT Article AB This year at VEE, we added a panel to discuss the state of virtualization: what problems are solved? what problems are important? and what problems may not be worth solving? The panelist are experts in areas ranging from hardware virtualization up to language-level virtualization. C1 [Berger, Emery] Univ Massachusetts Amherst, Amherst, MA 01003 USA. [Bhattacharjee, Abhishek] Rutgers State Univ, New Brunswick, NJ USA. [Pedretti, Kevin] Sandia Natl Labs, Livermore, CA 94550 USA. [Peter, Simon; Rossbach, Chris] Univ Texas Austin, Austin, TX 78712 USA. [Rossbach, Chris] VMWare Res Grp, Austin, TX USA. RP Berger, E (reprint author), Univ Massachusetts Amherst, Amherst, MA 01003 USA. NR 0 TC 0 Z9 0 U1 0 U2 0 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0362-1340 EI 1558-1160 J9 ACM SIGPLAN NOTICES JI ACM Sigplan Not. PD JUL PY 2016 VL 51 IS 7 BP 177 EP 177 DI 10.1145/2892242.2892249 PG 1 WC Computer Science, Software Engineering SC Computer Science GA EN3DR UT WOS:000395889700016 ER PT J AU Bera, MK Antonio, MR AF Bera, Mrinal K. Antonio, Mark R. TI Aggregation of Heteropolyanions Implicates the Presence of Zundel Ions Near Air-Water Interfaces SO CHEMISTRYSELECT LA English DT Article DE Heteropolyacids; Heteropolyanions; Air-water interface; Protons; X-ray scattering ID X-RAY REFLECTIVITY; AQUEOUS-SOLUTIONS; LIQUID WATER; ACID HEXAHYDRATE; SURFACE-TENSION; PROTON-TRANSFER; EXCESS PROTON; ANIONS; ELECTROLYTES; SPECTROSCOPY AB Protons play crucial roles in the interactions between hetero-polyanions (HPAs) in aqueous solutions and solid acid salts. We report the aggregation behaviours of Keggin HPAs near the surfaces of heteropolyacid solutions. The structure of the aggregated HPA layer near the solution-vapour phase boundary closely resembles the solid-state crystal structure of the hetero-polyacids in which the HPAs are connected by Zundel ions. The resemblance not only implicates the presence of protons in the form of planar Zundel ions near the air-water interface but, also, suggests that these align parallel to the interface. This study demonstrates an indirect means of assessing the impact of protons on HPA interactions near air-water interfaces and, in general, provides new insights about interfacial proton chemistry of heteropolyacids. C1 [Bera, Mrinal K.; Antonio, Mark R.] Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA. [Bera, Mrinal K.] ESRF, DUBBLE CRG, CS40220, F-38043 Grenoble 9, France. RP Bera, MK; Antonio, MR (reprint author), Argonne Natl Lab, Chem Sci & Engn Div, Argonne, IL 60439 USA.; Bera, MK (reprint author), ESRF, DUBBLE CRG, CS40220, F-38043 Grenoble 9, France. EM mrinal.bera@esrf.fr; mantonio@anl.gov FU National Science Foundation [NSF/CHE-1346572]; U.S. DOE [DE-AC02-06CH11357] FX We gratefully acknowledge the assistance of Dr. Binhua Lin in performing the experiments at the ChemMatCARS beamline at Sector 15, Advanced Photon Source, Argonne National Laboratory. ChemMatCARS Sector 15 is supported by the National Science Foundation under grant number NSF/CHE-1346572. This work and the use of the Advanced Photon Source, an Office of Science User Facility operated for the U.S. Department of Energy (DOE) Office of Science by Argonne National Laboratory, is supported by the U.S. DOE under Contract No. DE-AC02-06CH11357. NR 39 TC 0 Z9 0 U1 1 U2 1 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 2365-6549 J9 CHEMISTRYSELECT JI ChemistrySelect PD JUL 1 PY 2016 VL 1 IS 10 BP 2107 EP 2112 DI 10.1002/slct.201600441 PG 6 WC Chemistry, Multidisciplinary SC Chemistry GA EM6JD UT WOS:000395417800004 ER PT J AU Deng, LL Ibrahim, YM Baker, ES Aly, NA Hamid, AM Zhang, X Zheng, XY Garimella, SVB Webb, IK Prost, SA Sandoval, JA Norheim, RV Anderson, GA Tolmachev, AV Smith, RD AF Deng, Liulin Ibrahim, Yehia M. Baker, Erin S. Aly, Noor A. Hamid, Ahmed M. Zhang, Xing Zheng, Xueyun Garimella, Sandilya V. B. Webb, Ian K. Prost, Spencer A. Sandoval, Jeremy A. Norheim, Randolph V. Anderson, Gordon A. Tolmachev, Aleksey V. Smith, Richard D. TI Ion Mobility Separations of Isomers based upon Long Path Length Structures for Lossless Ion Manipulations Combined with Mass Spectrometry SO CHEMISTRYSELECT LA English DT Article DE Structures for Lossless Ion Manipulations (SLIM); Ion Mobility Spectrometry; Mass Spectrometry; Isomers ID RESOLUTION; IDENTIFICATION; CHROMATOGRAPHY; CONFORMATIONS AB Mass spectrometry (MS)-based multi-omic measurements, including proteomics, metabolomics, lipidomics, and glycomics, are increasingly transforming our ability to characterize and understand biological systems. Multi-omic analyses and the desire for comprehensive measurement coverage presently have limitations due to the chemical diversity and range of abundances of biomolecules in complex samples. Advances addressing these challenges increasingly are based upon the ability to quickly separate, react and otherwise manipulate sample components for analysis by MS. Here we report on a new approach using Structures for Lossless Ion Manipulations (SLIM) to enable long serpentine path ion mobility spectrometry (IMS) separations followed by MS analyses. This approach provides previously unachieved resolution for biomolecular species, in conjunction with more effective ion utilization, and a basis for greatly improved characterization of very small sample sizes. C1 [Deng, Liulin; Ibrahim, Yehia M.; Baker, Erin S.; Aly, Noor A.; Hamid, Ahmed M.; Zhang, Xing; Zheng, Xueyun; Garimella, Sandilya V. B.; Webb, Ian K.; Prost, Spencer A.; Sandoval, Jeremy A.; Norheim, Randolph V.; Anderson, Gordon A.; Tolmachev, Aleksey V.; Smith, Richard D.] Pacific Northwest Natl Lab, Div Biol Sci, 902 Battelle Blvd, Richland, WA 99352 USA. [Deng, Liulin; Ibrahim, Yehia M.; Baker, Erin S.; Aly, Noor A.; Hamid, Ahmed M.; Zhang, Xing; Zheng, Xueyun; Garimella, Sandilya V. B.; Webb, Ian K.; Prost, Spencer A.; Sandoval, Jeremy A.; Norheim, Randolph V.; Anderson, Gordon A.; Tolmachev, Aleksey V.; Smith, Richard D.] Pacific Northwest Natl Lab, Environm Mol Sci Lab, 902 Battelle Blvd, Richland, WA 99352 USA. RP Smith, RD (reprint author), Pacific Northwest Natl Lab, Div Biol Sci, 902 Battelle Blvd, Richland, WA 99352 USA.; Smith, RD (reprint author), Pacific Northwest Natl Lab, Environm Mol Sci Lab, 902 Battelle Blvd, Richland, WA 99352 USA. EM rds@pnnl.gov OI Zheng, Xueyun/0000-0001-9782-4521 FU National Institute of General Medical Sciences [P41 GM103493]; U.S. Department of Energy Office of Biological and Environmental Research Genome Sciences Pan-omics Program at Pacific Northwest National Laboratory (PNNL); Laboratory Directed Research and Development Program at PNNL; DOE [DE-AC05-76RL0 1830] FX Portions of this research were supported by grants from the National Institute of General Medical Sciences (P41 GM103493), the U.S. Department of Energy Office of Biological and Environmental Research Genome Sciences Pan-omics Program at Pacific Northwest National Laboratory (PNNL), the Laboratory Directed Research and Development Program at PNNL. This research was performed at the W. R. Wiley Environmental Molecular Sciences Laboratory (EMSL), a DOE national scientific user facility at the Pacific Northwest National Laboratory (PNNL). PNNL is operated by Battelle for the DOE under contract DE-AC05-76RL0 1830. NR 29 TC 9 Z9 9 U1 4 U2 4 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 2365-6549 J9 CHEMISTRYSELECT JI ChemistrySelect PD JUL 1 PY 2016 VL 1 IS 10 BP 2396 EP 2399 DI 10.1002/slct.201600460 PG 4 WC Chemistry, Multidisciplinary SC Chemistry GA EM6JD UT WOS:000395417800045 ER PT J AU Dhall, S Alamat, R Castro, A Sarker, AH Mao, JH Chan, A Hang, B Martins-Green, M AF Dhall, Sandeep Alamat, Raquelle Castro, Anthony Sarker, Altaf H. Mao, Jian-Hua Chan, Alex Hang, Bo Martins-Green, Manuela TI Tobacco toxins deposited on surfaces (third hand smoke) impair wound healing SO CLINICAL SCIENCE LA English DT Article DE angiogenesis; cytokine; DNA damage; inflammation; reactive oxygen species and antioxidants; toxicants ID MATRIX-METALLOPROTEINASE; CIGARETTE-SMOKING; THIRDHAND-SMOKE; BLOOD-FLOW; COLLAGEN PRODUCTION; TISSUE INHIBITOR; DNA-DAMAGE; HUMAN SKIN; G-CSF; EXPRESSION AB Third hand smoke (THS) is the accumulation of second hand smoke (SHS) toxins on surfaces in homes, cars, clothing and hair of smokers. It is known that 88M US nonsmokers >= 3 years old living in homes of smokers are exposed to THS toxicants and show blood cotinine levels of >= 0.05 ng/ml, indicating that the toxins are circulating in their circulatory systems. The goal of the present study is to investigate the mechanisms by which THS causes impaired wound healing. We show that mice living under conditions that mimic THS exposure in humans display delayed wound closure, impaired collagen deposition, altered inflammatory response, decreased angiogenesis, microvessels with fibrin cuffs and a highly proteolytic wound environment. Moreover, THS-exposed mouse wounds have high levels of oxidative stress and significantly lower levels of antioxidant activity leading to molecular damage, including protein nitration, lipid peroxidation and DNA damage that contribute to tissue dysfunction. Furthermore, we show that elastase is elevated, suggesting that elastin is degraded and the plasticity of the wound tissue is decreased. Taken together, our results lead us to conclude that THS toxicants delay and impair wound healing by disrupting the sequential processes that lead to normal healing. In addition, the lack of elastin results in loss of wound plasticity, which may be responsible for reopening of wounds. C1 [Dhall, Sandeep; Alamat, Raquelle; Castro, Anthony; Chan, Alex; Martins-Green, Manuela] Univ Calif Riverside, Dept Cell Biol & Neurosci, Riverside, CA 92521 USA. [Sarker, Altaf H.; Mao, Jian-Hua; Hang, Bo] Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94720 USA. RP Martins-Green, M (reprint author), Univ Calif Riverside, Dept Cell Biol & Neurosci, Riverside, CA 92521 USA. EM manuela.martins@ucr.edu FU Tobacco Research Disease Related Program (TRDRP) [22RT-0121, 23DT-0103] FX This work was supported by the Tobacco Research Disease Related Program (TRDRP) [grant numbers 22RT-0121 and 23DT-0103 (to M.M.-G.)]. NR 65 TC 1 Z9 1 U1 1 U2 2 PU PORTLAND PRESS LTD PI LONDON PA CHARLES DARWIN HOUSE, 12 ROGER STREET, LONDON WC1N 2JU, ENGLAND SN 0143-5221 EI 1470-8736 J9 CLIN SCI JI Clin. Sci. PD JUL 1 PY 2016 VL 130 IS 14 BP 1269 EP 1284 DI 10.1042/CS20160236 PG 16 WC Medicine, Research & Experimental SC Research & Experimental Medicine GA EK2MI UT WOS:000393761000012 PM 27129193 ER PT J AU Liu, SQ Zhuang, QL Chen, M Gu, LH AF Liu, Shaoqing Zhuang, Qianlai Chen, Min Gu, Lianhong TI Quantifying spatially and temporally explicit CO2 fertilization effects on global terrestrial ecosystem carbon dynamics SO ECOSPHERE LA English DT Article DE atmospheric CO2; carbon dynamics; gross primary production; net ecosystem production; process-based ecosystem model ID ATMOSPHERIC CO2; STOMATAL CONDUCTANCE; SEASONAL AMPLITUDE; BOUNDARY-LAYER; USE EFFICIENCY; AMERIFLUX DATA; TALL TOWER; MODEL; PHOTOSYNTHESIS; DIOXIDE AB Current terrestrial ecosystem models are usually driven with global average annual atmospheric carbon dioxide (CO2) concentration data at the global scale. However, high-precision CO2 measurement from eddy flux towers showed that seasonal, spatial surface atmospheric CO2 concentration differences were as large as 35 ppmv and the site-level tests indicated that the CO2 variation exhibited different effects on plant photosynthesis. Here we used a process-based ecosystem model driven with two spatially and temporally explicit CO2 data sets to analyze the atmospheric CO2 fertilization effects on the global carbon dynamics of terrestrial ecosystems from 2003 to 2010. Our results demonstrated that CO2 seasonal variation had a negative effect on plant carbon assimilation, while CO2 spatial variation exhibited a positive impact. When both CO2 seasonal and spatial effects were considered, global gross primary production and net ecosystem production were 1.7 Pg C.yr(-1) and 0.08 Pg C.yr(-1) higher than the simulation using uniformly distributed CO2 data set and the difference was significant in tropical and temperate evergreen broadleaf forest regions. This study suggests that the CO2 observation network should be expanded so that the realistic CO2 variation can be incorporated into the land surface models to adequately account for CO2 fertilization effects on global terrestrial ecosystem carbon dynamics. C1 [Liu, Shaoqing; Zhuang, Qianlai] Purdue Univ, Dept Earth Atmospher & Planetary Sci, W Lafayette, IN 47907 USA. [Zhuang, Qianlai] Purdue Univ, Dept Agron, W Lafayette, IN 47907 USA. [Chen, Min] Carnegie Inst Sci, Dept Global Ecol, Stanford, CA 94305 USA. [Gu, Lianhong] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Zhuang, QL (reprint author), Purdue Univ, Dept Earth Atmospher & Planetary Sci, W Lafayette, IN 47907 USA.; Zhuang, QL (reprint author), Purdue Univ, Dept Agron, W Lafayette, IN 47907 USA. EM qzhuang@purdue.edu OI Gu, Lianhong/0000-0001-5756-8738 FU NASA Land Use and Land Cover Change program [NASA-NNX09A126G]; Department of Energy [DE-FG02-08ER64599]; National Science Foundation [NSF-102891, NSF-0919331]; NSF Carbon and Water in the Earth Program [NSF-0630319]; NSF CDI Type II project [IIS-1028291] FX The model forcing data are provided by the Land Surface Hydrology Research Group at Princeton University. This research is funded through projects to Q.Z. by NASA Land Use and Land Cover Change program (NASA-NNX09A126G), Department of Energy (DE-FG02-08ER64599), National Science Foundation (NSF-102891 and NSF-0919331), NSF Carbon and Water in the Earth Program (NSF-0630319), and NSF CDI Type II project (IIS-1028291). NR 48 TC 0 Z9 0 U1 1 U2 1 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2150-8925 J9 ECOSPHERE JI Ecosphere PD JUL PY 2016 VL 7 IS 7 AR e01391 DI 10.1002/ecs2.1391 PG 13 WC Ecology SC Environmental Sciences & Ecology GA EK3FK UT WOS:000393811600001 ER PT J AU Guo, SC Liu, YQ Xu, XY Wang, ZR AF Guo, S. C. Liu, Y. Q. Xu, X. Y. Wang, Z. R. TI Cancellation of drift kinetic effects between thermal and energetic particles on the resistive wall mode stabilization SO NUCLEAR FUSION LA English DT Article DE instability; macroturbulence; plasma physics; energetic particles; magnetohydrodynamics; kinetic instability ID ACTIVE FEEDBACK STABILIZATION; EXTERNAL-MODES; STABILITY; TOKAMAKS AB Drift kinetic stabilization of the resistive wall mode (RWM) is computationally investigated using MHD-kinetic hybrid code MARS-K following the non-perturbative approach (Liu et al 2008 Phys. Plasmas 15 112503), for both reversed field pinch (RFP) and tokamak plasmas. Toroidal precessional drift resonance effects from trapped energetic ions (EIs) and various kinetic resonances between the mode and the guiding center drift motions of thermal particles are included into the self-consistent toroidal computations. The results show cancellation effects of the drift kinetic damping on the RWM between the thermal particles and EIs contributions, in both RFP and tokamak plasmas, even though each species alone can provide damping and stabilize RWM instability by respective kinetic resonances. The degree of cancellation generally depends on the EIs equilibrium distribution, the particle birth energy, as well as the toroidal flow speed of the plasma. C1 [Guo, S. C.; Xu, X. Y.] Consorzio RFX, Corso Stati Unit 4, I-35127 Padua, Italy. [Liu, Y. Q.] CCFE Culham Sci Ctr, Abingdon OX14 3DB, Oxon, England. [Liu, Y. Q.] Southwestern Inst Phys, POB 432, Chengdu 610041, Peoples R China. [Liu, Y. Q.] Chalmers, Dept Earth & Space Sci, SE-41296 Gothenburg, Sweden. [Wang, Z. R.] Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. RP Liu, YQ (reprint author), CCFE Culham Sci Ctr, Abingdon OX14 3DB, Oxon, England.; Liu, YQ (reprint author), Southwestern Inst Phys, POB 432, Chengdu 610041, Peoples R China.; Liu, YQ (reprint author), Chalmers, Dept Earth & Space Sci, SE-41296 Gothenburg, Sweden. EM yueqiang.liu@ccfe.ac.uk FU Euratom research and training programme [633053]; RCUK Energy Programme [EP/I501045]; National Natural Science Foundation of China (NSFC) [11428512]; National Magnetic Confinement Fusion Science Program [2015GB104004] FX This work has been carried out within the framework of the EUROfusion Consortium and has received funding from the Euratom research and training programme 2014-2018 under grant agreement No 633053 and from the RCUK Energy Programme (grant number EP/I501045). Work is also part funded by National Natural Science Foundation of China (NSFC) (grant numbers 11428512) and by National Magnetic Confinement Fusion Science Program under grant No. 2015GB104004. The views and opinions expressed herein do not necessarily reflect those of the European Commission. NR 31 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0029-5515 EI 1741-4326 J9 NUCL FUSION JI Nucl. Fusion PD JUL PY 2016 VL 56 IS 7 AR 076006 DI 10.1088/0029-5515/56/7/076006 PG 12 WC Physics, Fluids & Plasmas SC Physics GA DQ0YV UT WOS:000378928600008 ER PT J AU Inman, D Warner, E Stright, D Macknick, J Peck, C AF Inman, D. Warner, E. Stright, D. Macknick, J. Peck, C. TI Estimating biofuel feedstock water footprints using system dynamics SO JOURNAL OF SOIL AND WATER CONSERVATION LA English DT Article DE biofuel; corn; database; soybean; water consumption; water footprint ID ENVIRONMENTAL IMPACTS; FRESH-WATER; BIOENERGY; CONSUMPTION; PATHWAYS; ETHANOL; BIOMASS; ENERGY AB Increased biofuel production has prompted concerns about the environmental tradeoffs of biofuels compared to petroleum-based fuels. Biofuel production in general, and feedstock production in particular, is under increased scrutiny. Water footprinting (measuring direct and indirect water use) has been proposed as one measure to evaluate water use in the context of concerns about depleting rural water supplies through activities such as irrigation for large-scale agriculture. Water footprinting literature has often been limited in one or more key aspects: complete assessment across multiple water stocks (e.g., vadose zone, surface, and ground water stocks), geographical resolution of data, consistent representation of many feedstocks, and flexibility to perform scenario analysis. We developed a model called BioSpatial H2O using a system dynamics modeling and database framework. BioSpatial H2O could be used to consistently evaluate the complete water footprints of multiple biomass feedstocks at high geospatial resolutions. BioSpatial H2O has the flexibility to perform simultaneous scenario analysis of current and potential future crops under alternative yield and climate conditions. In this proof-of-concept paper, we modeled corn grain (Zea mays L.) and soybeans (Glycine max) under current conditions as illustrative results. BioSpatial H2O links to a unique database that houses annual spatially explicit climate, soil, and plant physiological data. Parameters from the database are used as inputs to our system dynamics model for estimating annual crop water requirements using daily time steps. Based on our review of the literature, estimated green water footprints are comparable to other modeled results, suggesting that BioSpatial H2O is computationally sound for future scenario analysis. Our modeling framework builds on previous water use analyses to provide a platform for scenario-based assessment. BioSpatial H2O's system dynamics is a flexible and user-friendly interface for on-demand, spatially explicit, water use scenario analysis for many US agricultural crops. Built-in controls permit users to quickly make modifications to the model assumptions, such as those affecting yield, and to see the implications of those results in real time. BioSpatial H2O's dynamic capabilities and adjustable climate data allow for analyses of water use and management scenarios to inform current and potential future bioenergy policies. The model could also be adapted for scenario analysis of alternative climatic conditions and comparison of multiple crops. The results of such an analysis would help identify risks associated with water use competition among feedstocks in certain regions. Results could also inform research and development efforts that seek to reduce water-related risks of biofuel pathways. C1 [Inman, D.; Warner, E.; Stright, D.; Macknick, J.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Peck, C.] Lexidyne LCC, Colorado Springs, CO USA. RP Inman, D (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. FU Office of Electricity Delivery and Energy Reliability FX This work was supported by the Office of Electricity Delivery and Energy Reliability. To our knowledge, the authors do not have any other potential conflicts of interest. NR 64 TC 0 Z9 0 U1 6 U2 6 PU SOIL WATER CONSERVATION SOC PI ANKENY PA 945 SW ANKENY RD, ANKENY, IA 50023-9723 USA SN 0022-4561 EI 1941-3300 J9 J SOIL WATER CONSERV JI J. Soil Water Conserv. PD JUL-AUG PY 2016 VL 71 IS 4 BP 343 EP 355 DI 10.2489/jswc.71.4.343 PG 13 WC Ecology; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA EH7KF UT WOS:000391951000010 ER PT J AU Leng, HX Loy, J Amin, V Weiss, EA Pelton, M AF Leng, Haixu Loy, James Amin, Victor Weiss, Emily A. Pelton, Matthew TI Electron Transfer from Single Semiconductor Nanocrystals to Individual Acceptor Molecules SO ACS ENERGY LETTERS LA English DT Article ID CDSE QUANTUM DOTS; ULTRAFAST CHARGE SEPARATION; TIO2 NANOPARTICLES; TRANSFER DYNAMICS; EXCITON DISSOCIATION; METHYL VIOLOGEN; HOLE TRANSFER; BLINKING; MECHANISMS; ADSORPTION AB This Letter reports the measurement of photoinduced electron-transfer rates from individual CdSe/CdS nanocrystals, or quantum dots (QDs), to methyl viologen acceptor molecules adsorbed on the QD surfaces, using time-resolved photoluminescence at the single-nano crystal level. For each QD measured, the electron-transfer rate is constant over time, and the photoluminescence blinking dynamics are independent of the measured transfer rate. The total electron-transfer rate is distributed in discrete, constant increments, corresponding to discrete numbers of adsorbed molecules on each QD. The results thus validate previous assumptions that viologen molecules adsorb independently on QD surfaces and that the total electron transfer rate from a single QD to multiple molecules on its surface is simply the sum of the transfer rates to the individual molecules. The measurement provides an optical method to count the number of active acceptor molecules bound to a single nanocrystal and opens up new possibilities for mechanistic studies of charge transfer at the nanoscale. C1 [Leng, Haixu; Loy, James; Pelton, Matthew] Univ Maryland Baltimore Cty, Dept Phys, 1000 Hilltop Circle, Baltimore, MD 21250 USA. [Amin, Victor; Weiss, Emily A.] Northwestern Univ, Dept Chem, 145 Sheridan Rd, Evanston, IL 60208 USA. [Pelton, Matthew] Argonne Natl Lab, Ctr Nanoscale Mat, 9700 South Cass Ave, Argonne, IL 60639 USA. [Amin, Victor] SendGrid, 1451 Larimer St 200, Denver, CO 80202 USA. RP Pelton, M (reprint author), Univ Maryland Baltimore Cty, Dept Phys, 1000 Hilltop Circle, Baltimore, MD 21250 USA.; Pelton, M (reprint author), Argonne Natl Lab, Ctr Nanoscale Mat, 9700 South Cass Ave, Argonne, IL 60639 USA. EM mpelton@umbc.edu FU Institute for Sustainability and Energy at Northwestern; National Institute of Standards and Technology [14D295]; National Science Foundation [DGE-1324585]; International Institute for Nanotechnology, MRSEC [NSF DMR-1121262]; Keck Foundation; State of Illinois; Northwestern University; Center for Nanoscale Materials, a U.S. Department of Energy Office of Science User Facility [DE-AC02-06CH11357] FX This project was supported by the Institute for Sustainability and Energy at Northwestern and by the National Institute of Standards and Technology under award number 14D295. This material is based upon work supported by the National Science Foundation through a Graduate Research Fellowship to V.A. (Grant DGE-1324585). Electron microscopy was performed in the NUANCE Center at Northwestern University. NUANCE is supported by the International Institute for Nanotechnology, MRSEC (NSF DMR-1121262), the Keck Foundation, the State of Illinois, and Northwestern University. This work was performed, in part, at the Center for Nanoscale Materials, a U.S. Department of Energy Office of Science User Facility under Contract DE-AC02-06CH11357. The authors thank Dmitriy Dolzhnikov for his help in acquiring electron microscopy images of the particles. NR 47 TC 3 Z9 3 U1 7 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2380-8195 J9 ACS ENERGY LETT JI ACS Energy Lett. PD JUL PY 2016 VL 1 IS 1 BP 9 EP 15 DI 10.1021/acsenergylett.6b00047 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Science & Technology - Other Topics; Materials Science GA EE5AS UT WOS:000389617700003 ER PT J AU Lian, C Liu, K Van Aken, KL Gogotsi, Y Wesolowski, DJ Liu, HL Jiang, DE Wu, JZ AF Lian, C. Liu, K. Van Aken, K. L. Gogotsi, Y. Wesolowski, D. J. Liu, H. L. Jiang, D. E. Wu, J. Z. TI Enhancing the Capacitive Performance of Electric Double-Layer Capacitors with Ionic Liquid Mixtures SO ACS ENERGY LETTERS LA English DT Article ID CARBON ELECTRODES; ELECTROCHEMICAL CAPACITORS; ENERGY-STORAGE; SUPERCAPACITORS; ELECTROLYTES; INTERFACES AB Formulating room-temperature ionic liquid (RTIL) mixed electrolytes was recently proposed as an effective and convenient strategy to increase the capacitive performance of electrochemical capacitors. Here we investigate the electrical double-layer (EDL) structure and the capacitance of two RTILs, 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide (EMI-TFSI) and 1-ethyl-3-methylimidazolium tetrafluoroborate (EMI-BF4), and their mixtures with onion-like carbon electrodes using experiment and classical density functional theory. The principal difference between these ionic liquids is the smaller diameter of the BF4- anion relative to the TFSI- anion and the EMI+ cation. A volcano-shaped trend is identified for the capacitance versus the composition of the RTIL mixture. The mixture effect, which makes more counterions pack on and more co-ions leave from the electrode surface, leads to an increase of the counterion density within the EDL and thus a larger capacitance. These theoretical predictions are in good agreement with our experimental observations and offer guidance for designing RTIL mixtures for EDL supercapacitors. C1 [Lian, C.; Liu, K.; Wu, J. Z.] Univ Calif Riverside, Dept Chem & Environm Engn, Riverside, CA 92521 USA. [Lian, C.; Liu, H. L.] East China Univ Sci & Technol, State Key Lab Chem Engn, Shanghai 200237, Peoples R China. [Van Aken, K. L.; Gogotsi, Y.] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Van Aken, K. L.; Gogotsi, Y.] Drexel Univ, AJ Drexel Nanomat Inst, Philadelphia, PA 19104 USA. [Wesolowski, D. J.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Jiang, D. E.] Univ Calif Riverside, Dept Chem, Riverside, CA 92521 USA. RP Wu, JZ (reprint author), Univ Calif Riverside, Dept Chem & Environm Engn, Riverside, CA 92521 USA. EM jwu@engr.ucr.edu OI Lian, Cheng/0000-0002-9016-832X FU Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences; National Natural Science Foundation of China [91334203, 21376074]; 111 Project of China [B08021]; Chinese Scholarship Council FX This research was sponsored by the Fluid Interface Reactions, Structures and Transport (FIRST) Center, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences. C.L. and H.L.L. acknowledge the financial support by the National Natural Science Foundation of China (91334203, 21376074) and the 111 Project of China (B08021). C.L. is also grateful to the Chinese Scholarship Council for the visiting fellowship. The numerical calculations were performed at the National Energy Research Scientific Computing Center (NERSC). NR 47 TC 4 Z9 4 U1 16 U2 16 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2380-8195 J9 ACS ENERGY LETT JI ACS Energy Lett. PD JUL PY 2016 VL 1 IS 1 BP 21 EP 26 DI 10.1021/acsenergylett.6b00010 PG 6 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Science & Technology - Other Topics; Materials Science GA EE5AS UT WOS:000389617700005 ER PT J AU Sanehira, EM de Villers, BJT Schulz, P Reese, MO Ferrere, S Zhu, K Lin, LY Berry, JJ Luther, JM AF Sanehira, Erin M. de Villers, Bertrand J. Tremolet Schulz, Philip Reese, Matthew O. Ferrere, Suzanne Zhu, Kai Lin, Lih Y. Berry, Joseph J. Luther, Joseph M. TI Influence of Electrode Interfaces on the Stability of Perovskite Solar Cells: Reduced Degradation Using MoOx/Al for Hole Collection SO ACS ENERGY LETTERS LA English DT Article ID TRANSITION-METAL OXIDES; HALIDE PEROVSKITES; CH3NH3PBI3 PEROVSKITE; HIGH-EFFICIENCY; GAP STATES; LAYER; PERFORMANCE; PASSIVATION; HUMIDITY; DEPOSITION AB We investigated and characterized the stability of the power output from methylammonium lead iodide perovskite photovoltaic devices produced with various hole-collecting anode configurations consisting of Au, Ag, MoOx/Au, MoOx/Ag, and MoOx/Al. The unencapsulated devices were operated under constant illumination and constant load conditions in laboratory ambient with periodic current-voltage testing. Although the initial efficiencies of devices were comparable across these configurations, the stability of these devices varied significantly due to subtle differences in the electrode structure. Specifically, we found that devices with MoOx/Al electrodes are more stable than devices with more conventional, and more costly, Au and Ag electrodes. We demonstrate that a thin MoOx layer inhibits decomposition of the perovskite films under illumination in ambient laboratory conditions and greater improvements in device stability are achieved specifically with MoOx/Al electrodes. We investigated the role of the MoOx interlayer in the MoOx/Al electrodes by exploring the effect of relative humidity and the MoOx interlayer thickness on the perovskite solar cell stability. C1 [Sanehira, Erin M.; de Villers, Bertrand J. Tremolet; Schulz, Philip; Reese, Matthew O.; Ferrere, Suzanne; Zhu, Kai; Berry, Joseph J.; Luther, Joseph M.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Sanehira, Erin M.; Lin, Lih Y.] Univ Washington, Dept Elect Engn, Seattle, WA 98195 USA. RP Luther, JM (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM joey.luther@nrel.gov FU hybrid perovskite solar cell program of the National Center for Photovoltaics - U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Office of Solar Energy Technology [DE-AC36-08GO28308DOE]; National Renewable Energy Laboratory (NREL); NASA Space Technology Research Fellowship FX Support on this work for B.J.T.d.V., P.S., M.O.R, S.F., K.Z., J.J.B., and J.M.L. was provided by the hybrid perovskite solar cell program of the National Center for Photovoltaics funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Office of Solar Energy Technology under Award Number DE-AC36-08GO28308DOE with the National Renewable Energy Laboratory (NREL). Support for E.M.S. and L.Y.L was provided by the NASA Space Technology Research Fellowship. We thank Bobby To for SEM images, Alfred Hicks for the schematic image, Nathan Neale for TiO2 nanoparticles, and Arrelaine Dameron for insightful discussions. NR 57 TC 18 Z9 18 U1 18 U2 18 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2380-8195 J9 ACS ENERGY LETT JI ACS Energy Lett. PD JUL PY 2016 VL 1 IS 1 BP 38 EP 45 DI 10.1021/acsenergylett.6b00013 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Science & Technology - Other Topics; Materials Science GA EE5AS UT WOS:000389617700008 ER PT J AU Zhou, YY Zhu, K AF Zhou, Yuanyuan Zhu, Kai TI Perovskite Solar Cells Shine in the "Valley of the Sun" SO ACS ENERGY LETTERS LA English DT Editorial Material C1 [Zhou, Yuanyuan] Brown Univ, Sch Engn, Providence, RI 02906 USA. [Zhu, Kai] Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. RP Zhu, K (reprint author), Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. EM Kai.Zhu@nrel.gov RI Zhou, Yuanyuan/G-2173-2011 OI Zhou, Yuanyuan/0000-0002-8364-4295 NR 5 TC 15 Z9 15 U1 2 U2 2 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2380-8195 J9 ACS ENERGY LETT JI ACS Energy Lett. PD JUL PY 2016 VL 1 IS 1 BP 64 EP 67 DI 10.1021/acsenergylett.6b00069 PG 4 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Science & Technology - Other Topics; Materials Science GA EE5AS UT WOS:000389617700012 ER PT J AU Yang, Y Wu, KF Shabaev, A Efros, AL Lian, TQ Beard, MC AF Yang, Ye Wu, Kaifeng Shabaev, Andrew Efros, Alexander L. Lian, Tianquan Beard, Matthew C. TI Direct Observation of Photoexcited Hole Localization in CdSe Nanorods SO ACS ENERGY LETTERS LA English DT Article ID MULTIPLE EXCITON DISSOCIATION; ULTRAFAST CHARGE SEPARATION; SEMICONDUCTOR QUANTUM DOTS; ELECTRON-TRANSFER; HYDROGEN-PRODUCTION; METHYLENE-BLUE; NANOCRYSTALS; DYNAMICS; HETEROSTRUCTURES; COMPLEXES AB Quantum-confined 1D semiconductor nanostructures are being investigated for hydrogen generation photocatalysts. In the photoreaction, after fast electron transfer, holes that remain in the nanostructure play an important role in the total quantum yield of hydrogen production. Unfortunately, knowledge of hole dynamics is limited due to lack of convenient spectroscopic signatures. Here, we directly probe hole localization dynamics within CdSe nanorods (NRs) by combining transient absorption (TA) and time-resolved terahertz (TRTS) spectroscopy. We show that when methylene blue is used as an electron acceptor, the resulting electron transfer occurs with a time constant of 3.5 +/- 0.1 ps and leaves behind a delocalized hole. However, the hole quickly localizes in the Coulomb potential well generated by the reduced electron acceptor near the NR surface with time constant of 11.7 +/- 0.2 ps. Our theoretical investigation suggests that the hole becomes confined to a similar to +/- 0.8 nm region near the reduced electron acceptor and the activation energy to detrap the hole from the potential well can be as large as 235 meV. C1 [Yang, Ye; Beard, Matthew C.] Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. [Wu, Kaifeng; Lian, Tianquan] Emory Univ, Dept Chem, 1515 Pierce Dr, Atlanta, GA 30322 USA. [Shabaev, Andrew; Efros, Alexander L.] Naval Res Lab, Ctr Computat Mat Sci, Washington, DC 20375 USA. RP Beard, MC (reprint author), Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. FU Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences, Office of Science, of the U.S. Department of Energy [DE-AC36-08GO28308, DE-FG02-12ER16347]; Center for Advanced Solar Photophysics, an Energy Frontiers Research Center - Office of Basic Energy Science, Office of Science within the U.S. Department of Energy; Office of Naval Research (ONR) through the Naval Research Laboratory Basic Research Program FX Work at NREL (Contract Number DE-AC36-08GO28308) and Emory (Grant No. DE-FG02-12ER16347) was supported by the Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences, Office of Science, of the U.S. Department of Energy. Theoretical calculations were supported as part of the Center for Advanced Solar Photophysics, an Energy Frontiers Research Center funded by the Office of Basic Energy Science, Office of Science within the U.S. Department of Energy. A.L.E. acknowledges the financial support of the Office of Naval Research (ONR) through the Naval Research Laboratory Basic Research Program. NR 48 TC 1 Z9 1 U1 12 U2 12 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2380-8195 J9 ACS ENERGY LETT JI ACS Energy Lett. PD JUL PY 2016 VL 1 IS 1 BP 76 EP 81 DI 10.1021/acsenergylett.6b00036 PG 6 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Science & Technology - Other Topics; Materials Science GA EE5AS UT WOS:000389617700014 ER PT J AU Orr, FM AF Orr, Franklin M., Jr. TI Addressing Climate Change with Clean Energy Technology SO ACS ENERGY LETTERS LA English DT Editorial Material C1 [Orr, Franklin M., Jr.] US DOE, Sci Energy, Washington, DC 20585 USA. RP Orr, FM (reprint author), US DOE, Sci Energy, Washington, DC 20585 USA. NR 0 TC 2 Z9 2 U1 0 U2 0 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2380-8195 J9 ACS ENERGY LETT JI ACS Energy Lett. PD JUL PY 2016 VL 1 IS 1 BP 113 EP 114 DI 10.1021/acsenergylett.6b00136 PG 2 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Science & Technology - Other Topics; Materials Science GA EE5AS UT WOS:000389617700020 ER PT J AU Hoque, MNF Yang, MJ Li, Z Islam, N Pan, X Zhu, K Fan, ZY AF Hoque, Md Nadim Ferdous Yang, Mengjin Li, Zhen Islam, Nazifah Pan, Xuan Zhu, Kai Fan, Zhaoyang TI Polarization and Dielectric Study of Methylammonium Lead Iodide Thin Film to Reveal its Nonferroelectric Nature under Solar Cell Operating Conditions SO ACS ENERGY LETTERS LA English DT Article ID ANOMALOUS HYSTERESIS; PEROVSKITE; CH3NH3PBI3; 1ST-PRINCIPLES; TRANSPORT; ORIGIN AB Researchers have debated whether methylammonium lead iodide (MAPbI(3)), with a perovskite crystal structure, is ferroelectric and therefore contributes to the current voltage hysteresis commonly observed in hybrid perovskite solar cells (PSCs). We thoroughly investigated temperature-dependent polarization, dielectric, and impedance spectroscopies, and we found no evidence of ferroelectric effect in a MAPbI(3) thin film at normal operating conditions. Therefore, the effect does not contribute to the hysteresis in PSCs, whereas the large component of ionic migration observed may play a critical role. Our temperature-based polarization and dielectric studies find that MAPbI3 exhibits different electrical behaviors below and above ca. 45 degrees C, suggesting a phase transition around this temperature. In particular, we report the activation energies of ionic migration for the two phases and temperature-dependent permittivity of MAPbI(3). This study contributes to the understanding performance of hybrid perovskites. C1 [Hoque, Md Nadim Ferdous; Islam, Nazifah; Fan, Zhaoyang] Texas Tech Univ, Dept Elect & Comp Engn, Lubbock, TX 79409 USA. [Hoque, Md Nadim Ferdous; Islam, Nazifah; Fan, Zhaoyang] Texas Tech Univ, Nano Tech Ctr, Lubbock, TX 79409 USA. [Yang, Mengjin; Li, Zhen; Zhu, Kai] Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. [Pan, Xuan] Beijing Inst Hydrogeol & Engn Geol, Beijing 100195, Peoples R China. RP Fan, ZY (reprint author), Texas Tech Univ, Dept Elect & Comp Engn, Lubbock, TX 79409 USA.; Fan, ZY (reprint author), Texas Tech Univ, Nano Tech Ctr, Lubbock, TX 79409 USA.; Zhu, K (reprint author), Natl Renewable Energy Lab, Chem & Nanosci Ctr, Golden, CO 80401 USA. EM kai.zhu@nrel.gov; zhaoyang.fan@ttu.edu OI Hoque, Md Nadim Ferdous/0000-0002-0662-6915 FU National Science Foundation [CBET-1438681]; U.S. Department of Energy [DE-AC36-08-GO28308]; U.S. Department of Energy SunShot Initiative under the Next Generation Photovoltaics 3 program [DE-FOA-0000990] FX Funding for the work at Texas Tech University from the National Science Foundation (CBET-1438681) is acknowledged. The work at the National Renewable Energy Laboratory was supported by the U.S. Department of Energy under Contract No. DE-AC36-08-GO28308. K.Z. acknowledges the support by the U.S. Department of Energy SunShot Initiative under the Next Generation Photovoltaics 3 program (DE-FOA-0000990). NR 45 TC 5 Z9 5 U1 7 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2380-8195 J9 ACS ENERGY LETT JI ACS Energy Lett. PD JUL PY 2016 VL 1 IS 1 BP 142 EP 149 DI 10.1021/acsenergylett.6b00093 PG 8 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Science & Technology - Other Topics; Materials Science GA EE5AS UT WOS:000389617700024 ER PT J AU Aguiar, JA Wozny, S Alkurd, NR Yang, MJ Kovarik, L Holesinger, TG Al-Jassim, M Zhu, K Zhou, WL Berry, JJ AF Aguiar, Jeffery A. Wozny, Sarah Alkurd, Nooraldeen R. Yang, Mengjin Kovarik, Libor Holesinger, Terry G. Al-Jassim, Mowafak Zhu, Kai Zhou, Weilie Berry, Joseph J. TI Effect of Water Vapor, Temperature, and Rapid Annealing on Formamidinium Lead Triiodide Perovskite Crystallization SO ACS ENERGY LETTERS LA English DT Article ID SOLAR-CELLS; SEQUENTIAL DEPOSITION; CH3NH3PBI3 PEROVSKITE; STATE; PERFORMANCE; FILMS; EFFICIENCY; TRIHALIDE; CH(3)NH(3)PBL(3); TRANSFORMATION AB Perovskite-based solar cells are one of the emerging candidates for radically lower cost photovoltaics. Herein, we report on the synthesis and crystallization of organic-inorganic formamidinium lead triiodide perovskite films under controlled atmospheric and environmental conditions. Using in situ (scanning) transmission electron microscopy, we make observations of the crystallization process of these materials in nitrogen and oxygen gas with and without the presence of water vapor. Complementary planar samples were also fabricated in the presence of water vapor and characterized by in situ X-ray diffraction. Direct observations of the material structure and final morphology indicate that the exposure to water vapor results in a porous film that is metastable, regardless of the presence of argon, nitrogen, or oxygen. However, the optimal crystallization temperature of 175 degrees C is unperturbed across conditions. Rapid modulation about the annealing temperature of 175 degrees C in +/- 25 degrees C steps (150-200 degrees C) promotes crystallization and significantly improves the film morphology by overcoming the presence of impregnated water trapped in the material. Following this processing protocol, we demonstrate substantial growth to micron-size grains via observation inside of an environmentally controlled transmission electron microscope. Adapting this insight from our in situ microscopy, we are able to provide an informed materials protocol to control the structure and morphology of these organic-inorganic semiconductors, which is readily applicable to benchtop device growth strategies. C1 [Aguiar, Jeffery A.; Yang, Mengjin; Al-Jassim, Mowafak; Zhu, Kai; Berry, Joseph J.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Wozny, Sarah; Alkurd, Nooraldeen R.; Zhou, Weilie] Univ New Orleans, Adv Mat Res Inst, New Orleans, LA 70148 USA. [Kovarik, Libor] Pacific Northwest Natl Lab, Environm Mol Sci Lab, POB 999, Richland, WA 99352 USA. [Holesinger, Terry G.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM USA. RP Aguiar, JA; Berry, JJ (reprint author), Natl Renewable Energy Lab, Golden, CO 80401 USA. EM Jeffery.Aguiar@nrel.gov; Joe.Berry@nrel.gov FU National Renewable Energy Laboratory, Non-Proprietary Partnering Program within the U.S. Department of Energy [DE-AC36-08-GO28308]; U.S. Department of Energy [DE-AC05-76RL01830]; Office of Biological and Environmental Research; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division [2013LANL8400] FX This work was supported by the National Renewable Energy Laboratory as a part of the Non-Proprietary Partnering Program under Contract No. DE-AC36-08-GO28308 within the U.S. Department of Energy. A portion of the research is part of the Chemical Imaging Initiative at Pacific Northwest National Laboratory (PNNL). It was conducted under the Laboratory Directed Research and Development Program at PNNL, a multiprogram national laboratory operated by Battelle for the U.S. Department of Energy under Contract DE-AC05-76RL01830. The work was performed at EMSL, a DOE Office of Science User Facility sponsored by the Office of Biological and Environmental Research and located at PNNL. The in situ X-ray diffraction experiments were performed at the National Renewable Energy Laboratory. TGH and in situ (S)TEM work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division under Grant Number 2013LANL8400. NR 41 TC 0 Z9 0 U1 8 U2 8 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2380-8195 J9 ACS ENERGY LETT JI ACS Energy Lett. PD JUL PY 2016 VL 1 IS 1 BP 155 EP 161 DI 10.1021/acsenergylett.6b00042 PG 7 WC Chemistry, Physical; Electrochemistry; Energy & Fuels; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Electrochemistry; Energy & Fuels; Science & Technology - Other Topics; Materials Science GA EE5AS UT WOS:000389617700026 ER PT J AU Mo, K Lv, W Tung, HM Yun, D Miao, YB Lan, KC Stubbins, JF AF Mo, Kun Lv, Wei Tung, Hsiao-Ming Yun, Di Miao, Yinbin Lan, Kuan-Che Stubbins, James F. TI Biaxial Thermal Creep of Alloy 617 and Alloy 230 for VHTR Applications SO JOURNAL OF ENGINEERING MATERIALS AND TECHNOLOGY-TRANSACTIONS OF THE ASME LA English DT Article DE VHTR; alloy 617; alloy 230; creep ID 850 DEGREES-C; HIGH-TEMPERATURE; IRRADIATION CREEP; FATIGUE LIFE; CRACK-GROWTH; NICKEL-ALLOY; BEHAVIOR; HELIUM; DEFORMATION; MECHANISMS AB In this study, we employed pressurized creep tubes to investigate the biaxial thermal creep behavior of Inconel 617 (alloy 617) and Haynes 230 (alloy 230). Both alloys are considered to he the primary candidate structural materials for very high-temperature reactors (VITITRs) due to their exceptional high-temperature mechanical properties. The current creep experiments were conducted at 900 degrees C for the effective stress range of 15-35 MPa. For both alloys, complete creep strain development with primary, secondary, and tertiary regimes was observed in all the studied conditions. Tertiary creep was found to he dominant over the entire creep lives of both alloys. With increasing applied creep stress, the fraction of the secondary creep regime decreases. The nucleation, diffusion, and coarsening of creep voids and carbides on grain boundaries were found to be the main reasons for the limited secondary regime and were also found to be the major causes of creep fracture. The creep curves computed using the adjusted creep equation of the form epsilon= cosh 1(1 rt) + P-sigma ntm agree well with the experimental results for both alloys at die temperatures of 850-950 degrees C. C1 [Mo, Kun; Yun, Di; Miao, Yinbin] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. [Lv, Wei; Miao, Yinbin; Lan, Kuan-Che; Stubbins, James F.] Univ Illinois, Dept Nucl Plasma & Radiol Engn, 104 South Wright St, Urbana, IL 61801 USA. [Tung, Hsiao-Ming] Atom Energy Council, Inst Nucl Energy Res, Taoyuan 325, Taiwan. [Yun, Di] Xi An Jiao Tong Univ, Dept Nucl Sci & Technol, Xian 710049, Peoples R China. RP Mo, K (reprint author), Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. EM kunmo@anl.gov OI Miao, Yinbin/0000-0002-3128-4275 FU U.S. Department of Energy [DE-FC07-07ID14819, DOE NEUP 09-516, DE-AC02-06CH11357, DE-FG02-07ER46453, DE-FG02-07ER46471] FX This work was supported by the U.S. Department of Energy under Grant Nos. DE-FC07-07ID14819 and DOE NEUP 09-516. Argonne National Laboratory's work was supported under U.S. Department of Energy Contract No. DE-AC02-06CH11357. The authors would like to thank Haynes International, Inc., for providing testing materials. The microstructural analysis was carried out in part in the Frederick Seitz Materials Research Laboratory Central Facilities, University of Illinois, which was partially supported by the U.S. Department of Energy under Grant Nos. DE-FG02-07ER46453 and DE-FG02-07ER46471. NR 48 TC 0 Z9 0 U1 2 U2 2 PU ASME PI NEW YORK PA TWO PARK AVE, NEW YORK, NY 10016-5990 USA SN 0094-4289 EI 1528-8889 J9 J ENG MATER-T ASME JI J. Eng. Mater. Technol.-Trans. ASME PD JUL PY 2016 VL 138 IS 3 AR 031015 DI 10.1115/1.4033322 PG 8 WC Engineering, Mechanical; Materials Science, Multidisciplinary SC Engineering; Materials Science GA EE6ZB UT WOS:000389762100015 ER PT J AU Fisk, WJ Paulson, JA Kolbe, LJ Barnett, CL AF Fisk, William J. Paulson, Jerome A. Kolbe, Lloyd J. Barnett, Claire L. TI Significance of the School Physical Environment - A Commentary SO JOURNAL OF SCHOOL HEALTH LA English DT Editorial Material ID INDOOR AIR; RESPIRATORY SYMPTOMS; ASTHMATIC SYMPTOMS; FUNGAL DNA; HEALTH; SCHOOLCHILDREN; PERFORMANCE; ASSOCIATION; CLASSROOMS; CHILDREN C1 [Fisk, William J.] Lawrence Berkeley Natl Lab, Indoor Environm Grp, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Paulson, Jerome A.] George Washington Univ, Pediat & Environm & Occupat Hlth, Sch Med & Hlth Sci, 1113 N Howard St, Alexandria, VA USA. [Paulson, Jerome A.] George Washington Univ, Milken Inst, Sch Publ Hlth, 1113 N Howard St, Alexandria, VA USA. [Kolbe, Lloyd J.] Indiana Univ, Appl Hlth Sci, Sch Publ Hlth, 1205 St,Georges Lane, Vero Beach, FL 32967 USA. [Barnett, Claire L.] Hlth Sch Network, 773 Madison Ave, Albany, NY 12208 USA. RP Fisk, WJ (reprint author), Lawrence Berkeley Natl Lab, Indoor Environm Grp, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM wjfisk@lbl.gov; jerry@envirohealthdoctor.com; lkolbe@indiana.edu; cbarnett@healthyschools.org FU Healthy Schools Network; Indoor Environments Division, Office of Radiation and Indoor Air of the US Environmental Protection Agency (EPA) [DW-89-92337001]; US Department of Energy [DE-AC02-05CH11231] FX Preparation of this commentary was supported by the Healthy Schools Network. The original review of papers and tabulation of study results was funded through interagency agreement DW-89-92337001 between the Indoor Environments Division, Office of Radiation and Indoor Air of the US Environmental Protection Agency (EPA) and the US Department of Energy under contract DE-AC02-05CH11231. NR 50 TC 0 Z9 0 U1 2 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0022-4391 EI 1746-1561 J9 J SCHOOL HEALTH JI J. Sch. Health PD JUL PY 2016 VL 86 IS 7 BP 483 EP 487 DI 10.1111/josh.12400 PG 5 WC Education & Educational Research; Education, Scientific Disciplines; Health Care Sciences & Services; Public, Environmental & Occupational Health SC Education & Educational Research; Health Care Sciences & Services; Public, Environmental & Occupational Health GA DW5MW UT WOS:000383690600001 PM 27246672 ER PT J AU Benning, C Sweetlove, L AF Benning, Christoph Sweetlove, Lee TI Synthetic biology for basic and applied plant research SO PLANT JOURNAL LA English DT Editorial Material C1 [Benning, Christoph] Michigan State Univ, US Dept Energy, Plant Res Lab, E Lansing, MI 48824 USA. [Sweetlove, Lee] Univ Oxford, Dept Plant Sci, South Parks Rd, Oxford OX1 3RB, England. RP Benning, C (reprint author), Michigan State Univ, US Dept Energy, Plant Res Lab, E Lansing, MI 48824 USA. EM Benning@cns.msu.edu; lee.sweetlove@plants.ox.ac.uk NR 10 TC 0 Z9 0 U1 3 U2 3 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0960-7412 EI 1365-313X J9 PLANT J JI Plant J. PD JUL PY 2016 VL 87 IS 1 SI SI BP 3 EP 4 DI 10.1111/tpj.13245 PG 2 WC Plant Sciences SC Plant Sciences GA DW3UZ UT WOS:000383569900001 PM 27483204 ER PT J AU Gonzalez-Esquer, CR Newnham, SE Kerfeld, CA AF Gonzalez-Esquer, C. Raul Newnham, Sarah E. Kerfeld, Cheryl A. TI Bacterial microcompartments as metabolic modules for plant synthetic biology SO PLANT JOURNAL LA English DT Article DE bacterial microcompartment; carboxysome; synthetic biology; scaffold; nanoreactor ID CYANOBACTERIUM SYNECHOCYSTIS PCC6803; INORGANIC CARBON TRANSPORTERS; CARBOXYSOME SHELL; THIOBACILLUS-NEAPOLITANUS; CO2 FIXATION; PDU MICROCOMPARTMENT; STRUCTURAL INSIGHTS; ALPHA-CARBOXYSOMES; CRYSTAL-STRUCTURE; RUBISCO ACTIVASE AB Bacterial microcompartments (BMCs) are megadalton-sized protein assemblies that enclose segments of metabolic pathways within cells. They increase the catalytic efficiency of the encapsulated enzymes while sequestering volatile or toxic intermediates from the bulk cytosol. The first BMCs discovered were the carboxysomes of cyanobacteria. Carboxysomes compartmentalize the enzyme ribulose-1,5-bisphosphate carboxylase/oxygenase (RuBisCO) with carbonic anhydrase. They enhance the carboxylase activity of RuBisCO by increasing the local concentration of CO2 in the vicinity of the enzyme's active site. As a metabolic module for carbon fixation, carboxysomes could be transferred to eukaryotic organisms (e.g. plants) to increase photosynthetic efficiency. Within the scope of synthetic biology, carboxysomes and other BMCs hold even greater potential when considered a source of building blocks for the development of nanoreactors or three-dimensional scaffolds to increase the efficiency of either native or heterologously expressed enzymes. The carboxysome serves as an ideal model system for testing approaches to engineering BMCs because their expression in cyanobacteria provides a sensitive screen for form (appearance of polyhedral bodies) and function (ability to grow on air). We recount recent progress in the re-engineering of the carboxysome shell and core to offer a conceptual framework for the development of BMC-based architectures for applications in plant synthetic biology. C1 [Gonzalez-Esquer, C. Raul; Newnham, Sarah E.; Kerfeld, Cheryl A.] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. [Kerfeld, Cheryl A.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Kerfeld, Cheryl A.] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. [Kerfeld, Cheryl A.] Univ Calif Berkeley, Berkeley Synthet Biol Inst, Berkeley, CA 94720 USA. [Kerfeld, Cheryl A.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. RP Kerfeld, CA (reprint author), Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA.; Kerfeld, CA (reprint author), Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.; Kerfeld, CA (reprint author), Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA.; Kerfeld, CA (reprint author), Univ Calif Berkeley, Berkeley Synthet Biol Inst, Berkeley, CA 94720 USA.; Kerfeld, CA (reprint author), Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. EM ckerfeld@lbl.gov FU Office of Science of the U.S. Department of Energy [DE-FG02-91ER20021]; MSU AgBIO Research; Strategic Partnership Grants Program at Michigan State University [14-SPG-Full-2962] FX CRG-E, SEN and CAK are supported by the Office of Science of the U.S. Department of Energy DE-FG02-91ER20021 and MSU AgBIO Research. CRG-E and CAK acknowledge the sponsorship from the Strategic Partnership Grants Program at Michigan State University (Grant 14-SPG-Full-2962). We thank Aiko Turmo, Dr Fei Cai and Dr Clement Aussignargues for their critical reading of the manuscript and gratefully acknowledge members of the Kerfeld lab for helpful discussions. NR 104 TC 2 Z9 2 U1 7 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0960-7412 EI 1365-313X J9 PLANT J JI Plant J. PD JUL PY 2016 VL 87 IS 1 SI SI BP 66 EP 75 DI 10.1111/tpj.13166 PG 10 WC Plant Sciences SC Plant Sciences GA DW3UZ UT WOS:000383569900006 PM 26991644 ER PT J AU Shih, PM Liang, Y Loque, D AF Shih, Patrick M. Liang, Yan Loque, Dominique TI Biotechnology and synthetic biology approaches for metabolic engineering of bioenergy crops SO PLANT JOURNAL LA English DT Article DE synthetic biology; metabolic engineering; bioenergy; energy crops; genome editing; transgene expression control ID ZINC-FINGER NUCLEASES; REGULATED GENE-EXPRESSION; PLANT-CELL WALLS; CRISPR/CAS9 SYSTEM; TRANSGENIC PLANTS; TRANSCRIPTIONAL REGULATION; HOMOLOGOUS RECOMBINATION; PHOTORESPIRATORY BYPASS; TARGETED MUTAGENESIS; BIOFUEL PRODUCTION AB The Green Revolution has fuelled an exponential growth in human population since the mid-20th century. Due to population growth, food and energy demands will soon surpass supply capabilities. To overcome these impending problems, significant improvements in genetic engineering will be needed to complement breeding efforts in order to accelerate the improvement of agronomical traits. The new field of plant synthetic biology has emerged in recent years and is expected to support rapid, precise, and robust engineering of plants. In this review, we present recent advances made in the field of plant synthetic biology, specifically in genome editing, transgene expression regulation, and bioenergy crop engineering, with a focus on traits related to lignocellulose, oil, and soluble sugars. Ultimately, progress and innovation in these fields may facilitate the development of beneficial traits in crop plants to meet society's bioenergy needs. C1 [Shih, Patrick M.; Liang, Yan; Loque, Dominique] Joint BioEnergy Inst, Emery Stn East, 5885 Hollis St,4th Floor, Emeryville, CA 94608 USA. [Shih, Patrick M.; Liang, Yan; Loque, Dominique] Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Loque, Dominique] Univ Lyon 1, INSA Lyon, CNRS, Microbiol Adaptat & Pathogenie UMR5240, 10 Rue Raphael Dubois, F-69622 Villeurbanne, France. RP Loque, D (reprint author), Joint BioEnergy Inst, Emery Stn East, 5885 Hollis St,4th Floor, Emeryville, CA 94608 USA.; Loque, D (reprint author), Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, 1 Cyclotron Rd, Berkeley, CA 94720 USA.; Loque, D (reprint author), Univ Lyon 1, INSA Lyon, CNRS, Microbiol Adaptat & Pathogenie UMR5240, 10 Rue Raphael Dubois, F-69622 Villeurbanne, France. EM dloque@lbl.gov FU United States Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; Gordon and Betty Moore Foundation [GBMF 2550.04] FX This work was part of the DOE Early Career Award and the DOE Joint BioEnergy Institute (http://www.jbei.org) supported by the United States Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the US Department of Energy. The US Government retains, and the publisher by accepting the article for publication acknowledges, that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide licence to publish or reproduce the published form of this manuscript, or allow others to do so, for US Government purposes. P.M.S. was supported by the Gordon and Betty Moore Foundation through Grant GBMF 2550.04 to the Life Sciences Research Foundation. NR 137 TC 1 Z9 1 U1 11 U2 12 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0960-7412 EI 1365-313X J9 PLANT J JI Plant J. PD JUL PY 2016 VL 87 IS 1 SI SI BP 103 EP 117 DI 10.1111/tpj.13176 PG 15 WC Plant Sciences SC Plant Sciences GA DW3UZ UT WOS:000383569900009 PM 27030440 ER PT J AU O'Malley, D Karra, S Currier, RP Makedonska, N Hyman, JD Viswanathan, HS AF O'Malley, D. Karra, S. Currier, R. P. Makedonska, N. Hyman, J. D. Viswanathan, H. S. TI Where Does Water Go During Hydraulic Fracturing? SO GROUNDWATER LA English DT Article ID BARNETT SHALE; POROUS-MEDIA; GAS; FRACKING; FLOW AB During hydraulic fracturing millions of gallons of water are typically injected at high pressure into deep shale formations. This water can be housed in fractures, within the shale matrix, and can potentially migrate beyond the shale formation via fractures and/ or faults raising environmental concerns. We describe a generic framework for producing estimates of the volume available in fractures and undamaged shale matrix where water injected into a representative shale site could reside during hydraulic fracturing, and apply it to a representative site that incorporates available field data. The amount of water that can be stored in the fractures is estimated by calculating the volume of all the fractures associated with a discrete fracture network (DFN) based on real data and using probability theory to estimate the volume of smaller fractures that are below the lower cutoff for the fracture radius in the DFN. The amount of water stored in the matrix is estimated utilizing two distinct methods-one using a two-phase model at the pore-scale and the other using a single-phase model at the continuum scale. Based on these calculations, it appears that most of the water resides in the matrix with a lesser amount in the fractures. C1 [O'Malley, D.; Karra, S.; Makedonska, N.; Hyman, J. D.; Viswanathan, H. S.] Los Alamos Natl Lab, Earth & Environm Sci Div, Computat Earth Sci, Los Alamos, NM 87545 USA. [Currier, R. P.] Los Alamos Natl Lab, Div Chem, Phys Chem & Appl Spect, Los Alamos, NM 87545 USA. [Hyman, J. D.] Los Alamos Natl Lab, Div Theoret, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP O'Malley, D (reprint author), Los Alamos Natl Lab, Earth & Environm Sci Div, Computat Earth Sci, Los Alamos, NM 87545 USA. EM omalled@lanl.gov OI Hyman, Jeffrey /0000-0002-4224-2847; Karra, Satish/0000-0001-7847-6293 FU Los Alamos National Laboratory's Laboratory Directed Research and Development Program [20140002DR]; LANL FX The authors thank the Los Alamos National Laboratory's Laboratory Directed Research and Development Program for their support through 20140002DR. The authors thank Bill Carey of Los Alamos National Laboratory for performing the shear fracture experiment on the Utica shale sample and providing us with the image data of the fractured sample. The authors also thank Robert Kleinberg and three anonymous reviewers for their comments which substantially improved the manuscript. DO was partially supported by a LANL Director's Postdoctoral Fellowship during the preparation of this manuscript. NR 35 TC 1 Z9 1 U1 6 U2 6 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0017-467X EI 1745-6584 J9 GROUNDWATER JI Groundwater PD JUL-AUG PY 2016 VL 54 IS 4 BP 488 EP 497 DI 10.1111/gwat.12380 PG 10 WC Geosciences, Multidisciplinary; Water Resources SC Geology; Water Resources GA ED2ZK UT WOS:000388718600005 PM 26469857 ER PT J AU Kormos, PR Luce, CH Wenger, SJ Berghuijs, WR AF Kormos, Patrick R. Luce, Charles H. Wenger, Seth J. Berghuijs, Wouter R. TI Trends and sensitivities of low streamflow extremes to discharge timing and magnitude in Pacific Northwest mountain streams SO WATER RESOURCES RESEARCH LA English DT Article ID WESTERN UNITED-STATES; FRESH-WATER ECOSYSTEMS; CLIMATE-CHANGE IMPACTS; MEAN ANNUAL RUNOFF; PATH-ANALYSIS; LOW FLOWS; POTENTIAL EVAPOTRANSPIRATION; IRRIGATED AGRICULTURE; HYDROLOGICAL DROUGHT; SPATIAL VARIABILITY AB Path analyses of historical streamflow data from the Pacific Northwest indicate that the precipitation amount has been the dominant control on the magnitude of low streamflow extremes compared to the air temperature-affected timing of snowmelt runoff. The relative sensitivities of low streamflow to precipitation and temperature changes have important implications for adaptation planning because global circulation models produce relatively robust estimates of air temperature changes but have large uncertainties in projected precipitation amounts in the Pacific Northwest U.S. Quantile regression analyses indicate that low streamflow extremes from the majority of catchments in this study have declined from 1948 to 2013, which may significantly affect terrestrial and aquatic ecosystems, and water resource management. Trends in the 25th percentile of mean annual streamflow have declined and the center of timing has occurred earlier. We quantify the relative influences of total precipitation and air temperature on the annual low streamflow extremes from 42 stream gauges using mean annual streamflow as a proxy for precipitation amount effects and streamflow center of timing as a proxy for temperature effects on low flow metrics, including 7q10 summer (the minimum 7 day flow during summer with a 10 year return period), mean August, mean September, mean summer, 7q10 winter, and mean winter flow metrics. These methods have the benefit of using only readily available streamflow data, which makes our results robust against systematic errors in high elevation distributed precipitation data. Winter low flow metrics are weakly tied to both mean annual streamflow and center of timing. C1 [Kormos, Patrick R.; Luce, Charles H.] US Forest Serv, Rocky Mt Res Stn, Boise, ID 83709 USA. [Kormos, Patrick R.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37830 USA. [Kormos, Patrick R.] US Agr Res Serv, Northwest Watershed Res Ctr, Boise, ID 83712 USA. [Wenger, Seth J.] Univ Georgia, Odum Sch Ecol, River Basin Ctr, Athens, GA 30602 USA. [Berghuijs, Wouter R.] Univ Bristol, Dept Civil Engn, Bristol, Avon, England. RP Kormos, PR (reprint author), US Forest Serv, Rocky Mt Res Stn, Boise, ID 83709 USA.; Kormos, PR (reprint author), Oak Ridge Inst Sci & Educ, Oak Ridge, TN 37830 USA.; Kormos, PR (reprint author), US Agr Res Serv, Northwest Watershed Res Ctr, Boise, ID 83712 USA. EM patrick.kormos@ars.usda.gov RI Luce, Charles/A-9267-2008; Berghuijs, Wouter/F-4937-2017 OI Luce, Charles/0000-0002-6938-9662; Berghuijs, Wouter/0000-0002-7447-0051 FU DOE [DE-AC05-06OR23100]; NASA [NNX14AC91G] FX We thank USDA-ARS Northwest Watershed Research Center and Boise State University for general support. Data used in this study are available from the resources cited in the article text. This research was supported in part by an appointment to the U.S. Forest Service Research Participation Program administered by the Oak Ridge Institute for Science and Education through an interagency agreement between the U.S. Department of Energy and the U.S. Department of Agriculture Forest Service. ORISE is managed by the Oak Ridge Associated Universities (ORAU) under DOE contract number DE-AC05-06OR23100. This work is also partially funded by NASA grand number NNX14AC91G. All opinions expressed in this paper are the author's and do not necessarily reflect the policies and views of USDA, DOE, or ORAU/ORISE. USDA is an equal opportunity provider and employer. NR 144 TC 1 Z9 1 U1 18 U2 18 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD JUL PY 2016 VL 52 IS 7 BP 4990 EP 5007 DI 10.1002/2015WR018125 PG 18 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA DW5KO UT WOS:000383683800002 ER PT J AU Lee, JH Yoon, HK Kitanidis, PK Werth, CJ Valocchi, AJ AF Lee, Jonghyun Yoon, Hongkyu Kitanidis, Peter K. Werth, Charles J. Valocchi, Albert J. TI Scalable subsurface inverse modeling of huge data sets with an application to tracer concentration breakthrough data from magnetic resonance imaging SO WATER RESOURCES RESEARCH LA English DT Article ID COMPONENT GEOSTATISTICAL APPROACH; GENERALIZED COVARIANCE FUNCTIONS; HETEROGENEOUS POROUS-MEDIA; PARAMETER-ESTIMATION; UNCERTAINTY QUANTIFICATION; HYDRAULIC CONDUCTIVITY; TEMPORAL MOMENTS; EQUATIONS; TRANSPORT; SYSTEMS AB Characterizing subsurface properties is crucial for reliable and cost-effective groundwater supply management and contaminant remediation. With recent advances in sensor technology, large volumes of hydrogeophysical and geochemical data can be obtained to achieve high-resolution images of subsurface properties. However, characterization with such a large amount of information requires prohibitive computational costs associated with "big data'' processing and numerous large-scale numerical simulations. To tackle such difficulties, the principal component geostatistical approach (PCGA) has been proposed as a "Jacobian-free'' inversion method that requires much smaller forward simulation runs for each iteration than the number of unknown parameters and measurements needed in the traditional inversion methods. PCGA can be conveniently linked to any multiphysics simulation software with independent parallel executions. In this paper, we extend PCGA to handle a large number of measurements (e.g., 106 or more) by constructing a fast preconditioner whose computational cost scales linearly with the data size. For illustration, we characterize the heterogeneous hydraulic conductivity (K) distribution in a laboratory-scale 3-D sand box using about 6 million transient tracer concentration measurements obtained using magnetic resonance imaging. Since each individual observation has little information on the K distribution, the data were compressed by the zeroth temporal moment of breakthrough curves, which is equivalent to the mean travel time under the experimental setting. Only about 2000 forward simulations in total were required to obtain the best estimate with corresponding estimation uncertainty, and the estimated K field captured key patterns of the original packing design, showing the efficiency and effectiveness of the proposed method. C1 [Lee, Jonghyun; Kitanidis, Peter K.] Stanford Univ, Dept Civil & Environm Engn, Stanford, CA 94305 USA. [Yoon, Hongkyu] Sandia Natl Labs, Geosci Res & Applicat Grp, POB 5800, Albuquerque, NM 87185 USA. [Werth, Charles J.] Univ Texas Austin, Dept Civil & Environm Engn, Austin, TX 78712 USA. [Valocchi, Albert J.] Univ Illinois, Dept Civil & Environm Engn, Urbana, IL 61801 USA. RP Lee, JH (reprint author), Stanford Univ, Dept Civil & Environm Engn, Stanford, CA 94305 USA. EM jonghyun@stanford.edu FU National Science Foundation through its ReNUWIt Engineering Research Center [NSF EEC-1028968]; Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001114]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The research was funded by the National Science Foundation through its ReNUWIt Engineering Research Center (www.renuwit.org; NSF EEC-1028968). H.Y. was supported as part of the Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under award DE-SC0001114. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. We thank Arvind Saibaba for his helpful comments on preconditioner construction and Amalia Kokkinaki for constructive suggestions. The measurement data used in this study can be made available by Hongkyu Yoon (hyoon@sandia.gov) upon request. NR 51 TC 0 Z9 0 U1 2 U2 2 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD JUL PY 2016 VL 52 IS 7 BP 5213 EP 5231 DI 10.1002/2015WR018483 PG 19 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA DW5KO UT WOS:000383683800015 ER PT J AU Fang, K Shen, C Fisher, JB Niu, J AF Fang, Kuai Shen, Chaopeng Fisher, Joshua B. Niu, Jie TI Improving Budyko curve-based estimates of long-term water partitioning using hydrologic signatures from GRACE SO WATER RESOURCES RESEARCH LA English DT Article ID SURFACE PROCESSES MODEL; GROUNDWATER DEPLETION; CLIMATE-CHANGE; ANNUAL RUNOFF; EVAPOTRANSPIRATION; FRAMEWORK; BALANCES; CONSTRAINTS; VARIABILITY; SATELLITES AB The Budyko hypothesis provides a first-order estimate of water partitioning into runoff (Q) and evapotranspiration (E). Observations, however, often show significant departures from the Budyko curve; moreover, past improvements to Budyko curve tend to lose predictive power when migrated between regions or to small scales. Here to estimate departures from the Budyko curve, we use hydrologic signatures extracted from Gravity Recovery And Climate Experiment (GRACE) terrestrial water storage anomalies. The signatures include GRACE amplitude as a fraction of precipitation (A/P), interannual variability, and 1-month lag autocorrelation. We created a group of linear models embodying two alternate hypotheses that departures can be predicted by (a) Taylor series expansion based on the deviation of physical characteristics (seasonality, snow fraction, and vegetation index) from reference conditions and (b) surrogate indicators covarying with E, e.g., A/P. These models are fitted using a mesoscale USA data set (HUC4) and then evaluated using world data sets and USA basins <1 x 10(5) km(2). The model with A/P could reduce error by 50% compared to Budyko itself. We found that seasonality and fraction of precipitation as snow account for a major portion of the predictive power of A/P, while the remainder is attributed to unexplained basin characteristics. When migrated to a global data set, type b models performed better than type a. This contrast in transferability is argued to be due to data set limitations and catchment coevolution. The GRACE-based correction performs well for USA basins >1000 km(2) and, according to comparison with other global data sets, is suitable for data fusion purposes, with GRACE error as estimates of uncertainty. C1 [Fang, Kuai; Shen, Chaopeng] Penn State Univ, Dept Civil & Environm Engn, State Coll, PA 16801 USA. [Fisher, Joshua B.] CALTECH, Jet Prop Lab, Pasadena, CA USA. [Niu, Jie] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Niu, Jie] Univ Calif Santa Barbara, Santa Barbara, CA 93106 USA. RP Shen, C (reprint author), Penn State Univ, Dept Civil & Environm Engn, State Coll, PA 16801 USA. EM cshen@engr.psu.edu OI Fisher, Joshua/0000-0003-4734-9085; Shen, Chaopeng/0000-0002-0685-1901 FU Office of Biological and Environmental Research of the US Department of Energy [DE-SC0010620] FX This work was supported by Office of Biological and Environmental Research of the US Department of Energy under contract DE-SC0010620. We thank David Wolock from USGS for providing shapefiles for the USGS basins. Data generated from this study are presented in figure format in the paper, and the data sets can be requested from the corresponding author. We thank Murugesu Sivapalan for some useful discussion about incomplete coevolution. J.B.F. contributed to this work from the Jet Propulsion Laboratory, California Institute of Technology, under a contract with the National Aeronautics and Space Administration. Constructive comments from anonymous reviewers and the Associate Editor have helped to improve the manuscript. NR 77 TC 1 Z9 1 U1 10 U2 10 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD JUL PY 2016 VL 52 IS 7 BP 5537 EP 5554 DI 10.1002/2016WR018748 PG 18 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA DW5KO UT WOS:000383683800035 ER PT J AU Ransom, KM Grote, MN Deinhart, A Eppich, G Kendall, C Sanborn, ME Souders, AK Wimpenny, J Yin, QZ Young, M Harter, T AF Ransom, Katherine M. Grote, Mark N. Deinhart, Amanda Eppich, Gary Kendall, Carol Sanborn, Matthew E. Souders, A. Kate Wimpenny, Joshua Yin, Qing-zhu Young, Megan Harter, Thomas TI Bayesian nitrate source apportionment to individual groundwater wells in the Central Valley by use of elemental and isotopic tracers SO WATER RESOURCES RESEARCH LA English DT Article ID SAN-JOAQUIN VALLEY; SOURCE IDENTIFICATION; STABLE-ISOTOPES; BORON ISOTOPES; CONTAMINATION SOURCES; NITROGEN-ISOTOPE; FRESH-WATER; ANTHROPOGENIC CONTAMINATION; MASS-SPECTROMETRY; TRACING SOURCES AB Groundwater quality is a concern in alluvial aquifers that underlie agricultural areas, such as in the San Joaquin Valley of California. Shallow domestic wells (less than 150 m deep) in agricultural areas are often contaminated by nitrate. Agricultural and rural nitrate sources include dairy manure, synthetic fertilizers, and septic waste. Knowledge of the relative proportion that each of these sources contributes to nitrate concentration in individual wells can aid future regulatory and land management decisions. We show that nitrogen and oxygen isotopes of nitrate, boron isotopes, and iodine concentrations are a useful, novel combination of groundwater tracers to differentiate between manure, fertilizers, septic waste, and natural sources of nitrate. Furthermore, in this work, we develop a new Bayesian mixing model in which these isotopic and elemental tracers were used to estimate the probability distribution of the fractional contributions of manure, fertilizers, septic waste, and natural sources to the nitrate concentration found in an individual well. The approach was applied to 56 nitrate-impacted private domestic wells located in the San Joaquin Valley. Model analysis found that some domestic wells were clearly dominated by the manure source and suggests evidence for majority contributions from either the septic or fertilizer source for other wells. But, predictions of fractional contributions for septic and fertilizer sources were often of similar magnitude, perhaps because modeled uncertainty about the fraction of each was large. For validation of the Bayesian model, fractional estimates were compared to surrounding land use and estimated source contributions were broadly consistent with nearby land use types. C1 [Ransom, Katherine M.; Harter, Thomas] Univ Calif Davis, Dept Land Air & Water Resources, Davis, CA 95616 USA. [Grote, Mark N.] Univ Calif Davis, Dept Anthropol, Davis, CA 95616 USA. [Deinhart, Amanda; Eppich, Gary] Lawrence Livermore Natl Lab, Livermore, CA USA. [Kendall, Carol; Young, Megan] US Geol Survey, Menlo Pk, CA USA. [Sanborn, Matthew E.; Souders, A. Kate; Wimpenny, Joshua; Yin, Qing-zhu] Univ Calif Davis, Dept Earth & Planetary Sci, Davis, CA 95616 USA. RP Harter, T (reprint author), Univ Calif Davis, Dept Land Air & Water Resources, Davis, CA 95616 USA. EM thharter@ucdavis.edu OI Sanborn, Matthew/0000-0003-3218-1195 FU California State Water Resources Control Board [04-184-555-0, 11-168-150]; White Family Graduate Student Award FX Funding for our research was provided by the California State Water Resources Control Board contracts 04-184-555-0 and 11-168-150 as well as from the White Family Graduate Student Award (2014). We would like to thank Arash Massoudieh for his help with model development. In addition, we acknowledge the eight dairy land owners who have collaborated with us and allowed groundwater monitoring at their facilities and the many domestic well owners who allowed us to sample wells on their property. We are grateful for the suggestions of Randy L. Bassett and two anonymous reviewers. We would also like to express our appreciation to Bassett for motivating us almost a decade ago to consider keeping extra water samples from well sampling campaigns for later boron isotope analysis should the need arise. NR 79 TC 0 Z9 0 U1 5 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0043-1397 EI 1944-7973 J9 WATER RESOUR RES JI Water Resour. Res. PD JUL PY 2016 VL 52 IS 7 BP 5577 EP 5597 DI 10.1002/2015WR018523 PG 21 WC Environmental Sciences; Limnology; Water Resources SC Environmental Sciences & Ecology; Marine & Freshwater Biology; Water Resources GA DW5KO UT WOS:000383683800037 ER PT J AU Aguilar-Arevalo, A Bertou, X Bonifazi, C Butner, M Cancelo, G Vazquez, AC Vergara, BC Chavez, CR Da Motta, H D'Olivo, JC Dos Anjos, J Estrada, J Moroni, GF Ford, R Foguel, A Torres, KPH Izraelevitch, F Kavner, A Kilminster, B Kuk, K Lima, HP Makler, M Molina, J Moreno-Granados, G Moro, JM Paolini, EE Haro, MS Tiffenberg, J Trillaud, F Wagner, S AF Aguilar-Arevalo, A. Bertou, X. Bonifazi, C. Butner, M. Cancelo, G. Castaneda Vazquez, A. Cervantes Vergara, B. Chavez, C. R. Da Motta, H. D'Olivo, J. C. Dos Anjos, J. Estrada, J. Fernandez Moroni, G. Ford, R. Foguel, A. Hernandez Torres, K. P. Izraelevitch, F. Kavner, A. Kilminster, B. Kuk, K. Lima, H. P., Jr. Makler, M. Molina, J. Moreno-Granados, G. Moro, J. M. Paolini, E. E. Sofo Haro, M. Tiffenberg, J. Trillaud, F. Wagner, S. TI Results of the engineering run of the Coherent Neutrino Nucleus Interaction Experiment (CONNIE) SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Detector design and construction technologies and materials; Neutrino detectors; Solid state detectors ID STELLAR COLLAPSE; NOBEL LECTURE; SCATTERING; ELECTRON; SEARCH; MUON; CCDS AB The CONNIE detector prototype is operating at a distance of 30 m from the core of a 3.8 GWth nuclear reactor with the goal of establishing Charge-Coupled Devices (CCD) as a new technology for the detection of coherent elastic neutrino-nucleus scattering. We report on the results of the engineering run with an active mass of 4 g of silicon. The CCD array is described, and the performance observed during the first year is discussed. A compact passive shield was deployed around the detector, producing an order of magnitude reduction in the background rate. The remaining background observed during the run was stable, and dominated by internal contamination in the detector packaging materials. The in-situ calibration of the detector using X-ray lines from fluorescence demonstrates good stability of the readout system. The event rates with the reactor ON and OFF are compared, and no excess is observed coming from nuclear fission at the power plant. The upper limit for the neutrino event rate is set two orders of magnitude above the expectations for the standard model. The results demonstrate the cryogenic CCD-based detector can be remotely operated at the reactor site with stable noise below 2e(-) RMS and stable background rates. The success of the engineering test provides a clear path for the upgraded 100 g detector to be deployed during 2016. C1 [Aguilar-Arevalo, A.; Castaneda Vazquez, A.; Cervantes Vergara, B.; D'Olivo, J. C.; Hernandez Torres, K. P.; Moreno-Granados, G.; Trillaud, F.] Univ Nacl Autonoma Mexico, Mexico City, DF, Mexico. [Bertou, X.; Sofo Haro, M.] Consejo Nacl Invest Cient & Tecn, Inst Balseiro, Ctr Atom Bariloche, CNEA, Buenos Aires, DF, Argentina. [Bonifazi, C.; Foguel, A.] Univ Fed Rio de Janeiro, Inst Fis, Rio De Janeiro, Brazil. [Butner, M.; Cancelo, G.; Ford, R.; Izraelevitch, F.; Tiffenberg, J.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Chavez, C. R.; Molina, J.] Univ Nacl Asuncion, Fac Ingn, San Lorenzo, Paraguay. [Da Motta, H.; Dos Anjos, J.; Foguel, A.; Lima, H. P., Jr.; Makler, M.] Ctr Brasileiro Pesquisas Fis, Rio De Janeiro, Brazil. [Fernandez Moroni, G.; Paolini, E. E.] Univ Nacl Sur, Dept Ingn Elect & Comp, Bahia Blanca, Buenos Aires, Argentina. [Fernandez Moroni, G.] Univ Nacl Sur, CONICET, Inst Invest Ingn Elect Alfredo Desages, Bahia Blanca, Buenos Aires, Argentina. [Kavner, A.] Univ Michigan, Ann Arbor, MI 48109 USA. [Kilminster, B.] Univ Zurich, Phys Inst, Zurich, Switzerland. [Moro, J. M.] Univ Nacl Sur, Dept Ingn, Bahia Blanca, Buenos Aires, Argentina. [Paolini, E. E.] Comis Invest Cient, La Plata, Buenos Aires, Argentina. [Wagner, S.] Pontificia Univ Catolica Rio de Janeiro, Rio de Janeiro, Brazil. RP Moroni, GF (reprint author), Univ Nacl Sur, Dept Ingn Elect & Comp, Bahia Blanca, Buenos Aires, Argentina.; Moroni, GF (reprint author), Univ Nacl Sur, CONICET, Inst Invest Ingn Elect Alfredo Desages, Bahia Blanca, Buenos Aires, Argentina. EM fmoroni.guillermo@gmail.com FU Ministerio da Ciencia, Tecnologia e Inovacao (MCTI); FAPERJ [E-26/110.145/2013]; CNPq; FINEP; PAPIIT-UNAM [IB100413, IN112213]; CONACYT [240666]; Agencia Nacional de Promocion Cientifica y Tecnologica in Argentina [PICT-2014-1225, PICT 2013-2128] FX We thank Central Nuclear Almirante Alvaro Alberto Eletronuclear, for access to the Angra II reactor site and for the support of their personnel, in particular Ilson Soares, to the CONNIE activities. We thank the Silicon Detector Facility team at Fermi National Accelerator Laboratory for being the host lab for the assembly and testing of the detectors components used in the CONNIE experiment. We acknowledge the support from Ministerio da Ciencia, Tecnologia e Inovacao (MCTI) and the Brazilian funding agencies FAPERJ (grant E-26/110.145/2013), CNPq, and FINEP; and the Mexican agencies PAPIIT-UNAM (grants IB100413, and IN112213), and CONACYT (grant No. 240666); and Agencia Nacional de Promocion Cientifica y Tecnologica in Argentina (PICT-2014-1225, PICT 2013-2128). We thank Ricardo Galvao and Ronald Shellard for their support to the experiment. NR 49 TC 2 Z9 2 U1 2 U2 2 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD JUL PY 2016 VL 11 AR P07024 DI 10.1088/1748-0221/11/07/P07024 PG 20 WC Instruments & Instrumentation SC Instruments & Instrumentation GA EC0BQ UT WOS:000387763000015 ER PT J AU Benoit, M de Mendizabal, JB Casse, G Chen, H Chen, K Di Bello, FA Ferrere, D Golling, T Gonzalez-Sevilla, S Iacobucci, G Lanni, F Liu, H Meloni, F Meng, L Miucci, A Muenstermann, D Nessi, M Peric, I Rimoldi, M Ristic, B Pinto, MVB Vossebeld, J Weber, M Wu, W Xu, L AF Benoit, M. de Mendizabal, J. Bilbao Casse, G. Chen, H. Chen, K. Di Bello, F. A. Ferrere, D. Golling, T. Gonzalez-Sevilla, S. Iacobucci, G. Lanni, F. Liu, H. Meloni, F. Meng, L. Miucci, A. Muenstermann, D. Nessi, M. Peric, I. Rimoldi, M. Ristic, B. Pinto, M. Vicente Barrero Vossebeld, J. Weber, M. Wu, W. Xu, L. TI Results of the 2015 testbeam of a 180nm AMS High-Voltage CMOS sensor prototype SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Electronic detector readout concepts (solid-state); Particle tracking detectors (Solid-state detectors); Si microstrip and pad detectors; Solid state detectors AB Active pixel sensors based on the High-Voltage CMOS technology are being investigated as a viable option for the future pixel tracker of the ATLAS experiment at the High-Luminosity LHC. This paper reports on the testbeam measurements performed at the H8 beamline of the CERN Super Proton Synchrotron on a High-Voltage CMOS sensor prototype produced in 180 nm AMS technology. Results in terms of tracking efficiency and timing performance, for different threshold and bias conditions, are shown. C1 [Benoit, M.; de Mendizabal, J. Bilbao; Di Bello, F. A.; Ferrere, D.; Golling, T.; Gonzalez-Sevilla, S.; Iacobucci, G.; Meng, L.; Miucci, A.; Muenstermann, D.; Nessi, M.; Ristic, B.; Pinto, M. Vicente Barrero] Univ Geneva, DPNC, 24 Quai Ernest Ansermet, CH-1211 Geneva 4, Switzerland. [Casse, G.; Meng, L.; Vossebeld, J.] Univ Liverpool, Dept Phys, Oliver Lodge Lab, Liverpool L69 7ZE, Merseyside, England. [Chen, H.; Chen, K.; Lanni, F.; Liu, H.; Wu, W.; Xu, L.] Brookhaven Natl Lab, POB 5000, Upton, NY 11973 USA. [Liu, H.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Meloni, F.; Miucci, A.; Rimoldi, M.; Weber, M.] Univ Bern, Albert Einstein Ctr Fundamental Phys, Sidlerstr 5, CH-3012 Bern, Switzerland. [Meloni, F.; Miucci, A.; Rimoldi, M.; Weber, M.] Univ Bern, High Energy Phys Lab, Sidlerstr 5, CH-3012 Bern, Switzerland. [Nessi, M.; Ristic, B.] CERN, European Org Nucl Res, 385 Route Meyrin, CH-1217 Meyrin, Switzerland. [Peric, I.] Karlsruhe Inst Technol, Kaiserstr 12, D-76131 Karlsruhe, Germany. [Muenstermann, D.] Univ Lancaster, Dept Phys, Lancaster LA1 4YB, England. RP Gonzalez-Sevilla, S (reprint author), Univ Geneva, DPNC, 24 Quai Ernest Ansermet, CH-1211 Geneva 4, Switzerland. EM Sergio.Gonzalez@unige.ch OI Benoit, Mathieu/0000-0002-8623-1699; Muenstermann, Daniel/0000-0001-6223-2497 FU SNSF [200020_156083, 20FL20_160474, 200020_163402] FX We gratefully acknowledge the support by the CERN PS and SPS instrumentation team. We thank Allan Clark for a careful reading of the manuscript. The research presented in this paper was supported by the SNSF grants 200020_156083, 20FL20_160474 and 200020_163402. NR 11 TC 1 Z9 1 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD JUL PY 2016 VL 11 AR P07019 DI 10.1088/1748-0221/11/07/P07019 PG 15 WC Instruments & Instrumentation SC Instruments & Instrumentation GA EC0BQ UT WOS:000387763000010 ER PT J AU Kalicy, G Allison, L Cao, T Dzhygadlo, R Horn, T Hyde, C Ilieva, Y Nadel-Turonski, P Park, K Peters, K Schwarz, C Schwiening, J Stevens, J Xi, W Zorn, C AF Kalicy, G. Allison, L. Cao, T. Dzhygadlo, R. Horn, T. Hyde, C. Ilieva, Y. Nadel-Turonski, P. Park, K. Peters, K. Schwarz, C. Schwiening, J. Stevens, J. Xi, W. Zorn, C. CA PID Consortium Integrated Program TI High-performance DIRC detector for the future Electron Ion Collider experiment SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT International Workshop on Fast Cherenkov Detectors - Photon Detection, DIRC Design and DAQ CY NOV 11-13, 2015 CL Giessen, GERMANY DE Cherenkov and transition radiation; Cherenkov detectors; Photon detectors for UV; visible and IR photons (vacuum) AB A radially-compact subsystem providing particle identification (e/pi, pi/K, K/p) over a wide momentum range is an essential requirement for the central detector of an Electron-Ion Collider (EIC). With a radial size of only a few cm, a detector based on Detection of Internally Reflected Cherenkov light (DIRC) principle is a very attractive solution. The R&D undertaken by the EIC PID consortium achieved the goal of showing feasibility of a high-performance DIRC that would extend the momentum coverage well beyond state-of-the-art allowing 3 sigma separation of pi/K up to 6 GeV/c, e/K up to 1.8 GeV/c and p/K up to 10 GeV/c. A key component to reach such a performance is a special 3-layer spherical compound lens. This article describes the status of the design and R&D for the DIRC at EIC detector, with a focus on the detailed Monte Carlo simulation results for the high-performance DIRC. C1 [Kalicy, G.; Allison, L.; Hyde, C.; Park, K.] Old Dominion Univ, Norfolk, VA 23529 USA. [Cao, T.; Ilieva, Y.] Univ South Carolina, Columbia, SC USA. [Dzhygadlo, R.; Peters, K.; Schwarz, C.; Schwiening, J.] GSI Helmholtzzentrum Schwerionenforsch GmbH, Darmstadt, Germany. [Horn, T.] Catholic Univ Amer, Washington, DC 20064 USA. [Nadel-Turonski, P.; Stevens, J.; Xi, W.; Zorn, C.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA USA. RP Kalicy, G (reprint author), Old Dominion Univ, Norfolk, VA 23529 USA. NR 9 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD JUL PY 2016 VL 11 AR C07015 DI 10.1088/1748-0221/11/07/C07015 PG 12 WC Instruments & Instrumentation SC Instruments & Instrumentation GA EC0BE UT WOS:000387761700015 ER PT J AU Stevens, J Barbosa, F Bessuille, J Chudakov, E Dzhygadlo, R Fanelli, C Frye, J Hardin, J Kelsey, J Patsyuk, M Schwartz, C Schwiening, J Shepherd, M Whitlatch, T Williams, M AF Stevens, J. Barbosa, F. Bessuille, J. Chudakov, E. Dzhygadlo, R. Fanelli, C. Frye, J. Hardin, J. Kelsey, J. Patsyuk, M. Schwartz, C. Schwiening, J. Shepherd, M. Whitlatch, T. Williams, M. TI The GLUEX DIRC project SO JOURNAL OF INSTRUMENTATION LA English DT Article; Proceedings Paper CT International Workshop on Fast Cherenkov Detectors - Photon Detection, DIRC Design and DAQ CY NOV 11-13, 2015 CL Giessen, GERMANY DE Cherenkov detectors; Particle identification methods AB The GLUEX experiment was designed to search for and study the pattern of gluonic excitations in the meson spectrum produced through photoproduction reactions at a new tagged photon beam facility in Hall D at Jefferson Laboratory. The particle identification capabilities of the GLUEX experiment will be enhanced by constructing a DIRC (Detection of Internally Reflected Cherenkov light) detector, utilizing components of the decommissioned BaBar DIRC. The DIRC will allow systematic studies of kaon final states that are essential for inferring the quark flavor content of both hybrid and conventional mesons. The design for the GLUEX DIRC is presented, including the new expansion volumes that are currently under development. C1 [Stevens, J.; Barbosa, F.; Chudakov, E.; Whitlatch, T.] Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. [Dzhygadlo, R.; Schwartz, C.; Schwiening, J.] GSI Helmholtzzentrum Schwerionenforsch GmbH, Darmstadt, Germany. [Bessuille, J.; Fanelli, C.; Hardin, J.; Kelsey, J.; Patsyuk, M.; Williams, M.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Frye, J.; Shepherd, M.] Indiana Univ, Bloomington, IN USA. RP Stevens, J (reprint author), Thomas Jefferson Natl Accelerator Facil, Newport News, VA 23606 USA. EM jrsteven@jlab.org NR 11 TC 1 Z9 1 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD JUL PY 2016 VL 11 AR C07010 DI 10.1088/1748-0221/11/07/C07010 PG 8 WC Instruments & Instrumentation SC Instruments & Instrumentation GA EC0BE UT WOS:000387761700010 ER PT J AU Sutherland, JC AF Sutherland, J. C. TI Calibration of photoelastic modulator based dichrometers: maintaining constant phase across the spectrum SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Spectrometers; Instrumentation for synchrotron radiation accelerators; Optical detector readout concepts ID CIRCULAR-DICHROISM; CALCIUM-FLUORIDE; REFRACTIVE-INDEX; FUSED-SILICA; BIREFRINGENCE; COEFFICIENT; WAVELENGTH; ANISOTROPY; RANGE; NM AB Photoelastic modulators can alter the polarization state of a beam of ultraviolet, visible or infrared photons by means of periodic stress-induced differences in the refractive index of a transparent material that forms the optical element of the device and is isotropic in the absence of stress. They have found widespread application in instruments that characterize or alter the polarization state of a beam in fields as diverse as astronomy, structural biology, materials science and ultraviolet lithography for the manufacture of nano-scale integrated circuits. Measurement of circular dichroism, the differential absorption of left-and right circularly polarized light, and of strain-induced birefringence of optical components are major applications. Instruments using synchrotron radiation and photoelastic modulators with CaF2 optical elements have extended circular dichroism measurements down to wavelengths of about 130 nm in the vacuum ultraviolet. Maintaining a constant phase shift between two orthogonal polarization states across a spectrum requires that the amplitude of the modulated stress be changed as a function of wavelength. For commercially available photoelastic modulators, the voltage that controls the amplitude of modulation required to produce a specified phase shift, which is a surrogate for the stress modulation amplitude, has been shown to be an approximately linear function of wavelength in the spectral region where the optical element is transparent. But, extrapolations of such straight lines cross zero voltage at a non-zero wavelength, not at zero-wavelength. For modulators with calcium fluoride and fused silica optical elements, the zero-crossing wavelength is always in the spectral region where the optical element of the modulator strongly absorbs the incident radiation, and at a wavelength less than the longestwavelength apparent resonance deduced from experimental values of the refractive index fit to the Sellmeier equation. Using a model that relates the refractive indices of a stressed optical element to the refractive index of its unstressed state, an expression for the modulator control voltage was derived that closely fits the experimental data. This result provides a theoretical rational for the apparently linear constant-phase programming voltage, and thus provides theoretical backing for the calibration procedure frequently used for these modulators. Other factors that can influence the calibration of a photoelastic modulator, including temperature and atmospheric pressure, are discussed briefly. C1 [Sutherland, J. C.] Augusta Univ, Dept Phys, Augusta, GA 20912 USA. [Sutherland, J. C.] Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA. [Sutherland, J. C.] East Carolina Univ, Dept Phys, Greenville, NC 27858 USA. RP Sutherland, JC (reprint author), Augusta Univ, Dept Phys, Augusta, GA 20912 USA.; Sutherland, JC (reprint author), Brookhaven Natl Lab, Dept Biol, Upton, NY 11973 USA.; Sutherland, JC (reprint author), East Carolina Univ, Dept Phys, Greenville, NC 27858 USA. EM jsutherland@augusta.edu FU State of North Carolina; State of North Georgia FX Brookhaven National Laboratory is operated under contract to the United States Department of Energy. East Carolina University and Augusta University are supported in part by the States of North Carolina and Georgia, respectively. I thank Hinds Instruments for providing reprints of several papers relating to the operation and performance of photoelastic modulators and for helpful discussions regarding the deployment of PEMs below normal room temperatures. NR 32 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD JUL PY 2016 VL 11 AR P07016 DI 10.1088/1748-0221/11/07/P07016 PG 22 WC Instruments & Instrumentation SC Instruments & Instrumentation GA EC0BQ UT WOS:000387763000007 ER PT J AU Benk, MP Wojdyla, A Chao, WL Salmassi, F Oh, S Wang, YG Miyakawa, RH Naulleau, PP Goldberg, KA AF Benk, Markus P. Wojdyla, Antoine Chao, Weilun Salmassi, Farhad Oh, Sharon Wang, Yow-Gwo Miyakawa, Ryan H. Naulleau, Patrick P. Goldberg, Kenneth A. TI Emulation of anamorphic imaging on the SHARP extreme ultraviolet mask microscope SO JOURNAL OF MICRO-NANOLITHOGRAPHY MEMS AND MOEMS LA English DT Article DE extreme ultraviolet; anamorphic; mask; microscope; zone plate; high-numerical aperture AB The SHARP high-numerical aperture actinic reticle review project is a synchrotron-based, extreme ultraviolet (EUV) microscope dedicated to photomask research. SHARP emulates the illumination and imaging conditions of current EUV lithography scanners and those several generations into the future. An anamorphic imaging optic with increased mask-side numerical aperture (NA) in the horizontal and increased demagnification in the vertical direction has been proposed to overcome limitations of current multilayer coatings and extend EUV lithography beyond 0.33 NA. Zoneplate lenses with an anamorphic 4 x / 8x NA of 0.55 are fabricated and installed in the SHARP microscope to emulate anamorphic imaging. SHARP's Fourier synthesis illuminator with a range of angles exceeding the collected solid angle of the newly designed elliptical zoneplates can produce arbitrary angular source spectra matched to anamorphic imaging. A target with anamorphic dense features down to 50-nm critical dimension is fabricated using 40 nm of nickel as the absorber. In a demonstration experiment, anamorphic imaging at 0.55 4 x / 8x NA and 6 deg central ray angle (CRA) is compared with conventional imaging at 0.5 4x NA and 8 deg CRA. A significant contrast loss in horizontal features is observed in the conventional images. The anamorphic images show the same image quality in the horizontal and vertical directions. (C) 2016 Society of Photo-Optical Instrumentation Engineers (SPIE) C1 [Benk, Markus P.; Wojdyla, Antoine; Chao, Weilun; Salmassi, Farhad; Oh, Sharon; Wang, Yow-Gwo; Miyakawa, Ryan H.; Naulleau, Patrick P.; Goldberg, Kenneth A.] Lawrence Berkeley Natl Lab, Ctr Xray Opt, 1 Cyclotron Rd, Berkeley, CA 94720 USA. RP Benk, MP (reprint author), Lawrence Berkeley Natl Lab, Ctr Xray Opt, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM mpbenk@lbl.gov NR 16 TC 1 Z9 1 U1 1 U2 1 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 1932-5150 EI 1932-5134 J9 J MICRO-NANOLITH MEM JI J. Micro-Nanolithogr. MEMS MOEMS PD JUL PY 2016 VL 15 IS 3 AR 033501 DI 10.1117/1.JMM.15.3.033501 PG 8 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Optics SC Engineering; Science & Technology - Other Topics; Materials Science; Optics GA EC6AX UT WOS:000388219500012 ER PT J AU Burckel, DB AF Burckel, D. Bruce TI Device-level and module-level three-dimensional integrated circuits created using oblique processing SO JOURNAL OF MICRO-NANOLITHOGRAPHY MEMS AND MOEMS LA English DT Article DE three-dimensional integrated circuits; interconnects; oblique processing ID FABRICATION AB This paper demonstrates that another class of three-dimensional integrated circuits (3-D-ICs) exists, distinct from through-silicon-via-centric and monolithic 3-D-ICs. Furthermore, it is possible to create devices that are 3-D "at the device level" (i.e., with active channels oriented in each of the three coordinate axes), by performing standard CMOS fabrication operations at an angle with respect to the wafer surface into high aspect ratio silicon substrates using membrane projection lithography (MPL). MPL requires only minimal fixturing changes to standard CMOS equipment, and no change to current state-of-the-art lithography. Eliminating the constraint of two-dimensional planar device architecture enables a wide range of interconnect topologies which could help reduce interconnect resistance/capacitance, and potentially improve performance. (C) The Authors. Published by SPIE under a Creative Commons Attribution 3.0 Unported License. C1 [Burckel, D. Bruce] Sandia Natl Labs, POB 5800, Albuquerque, NM 87106 USA. RP Burckel, DB (reprint author), Sandia Natl Labs, POB 5800, Albuquerque, NM 87106 USA. EM dbburck@sandia.gov FU Laboratory Directed Research and Development program at Sandia National Laboratories; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX Supported by the Laboratory Directed Research and Development program at Sandia National Laboratories, a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 17 TC 0 Z9 0 U1 0 U2 0 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 1932-5150 EI 1932-5134 J9 J MICRO-NANOLITH MEM JI J. Micro-Nanolithogr. MEMS MOEMS PD JUL PY 2016 VL 15 IS 3 AR 034504 DI 10.1117/1.JMM.15.3.034504 PG 6 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Optics SC Engineering; Science & Technology - Other Topics; Materials Science; Optics GA EC6AX UT WOS:000388219500028 ER PT J AU Shaw, S Miller, KJ Colaux, JL Cademartiri, L AF Shaw, Santosh Miller, Kyle J. Colaux, Julien L. Cademartiri, Ludovico TI Optics-free, plasma-based lithography in inorganic resists made up of nanoparticles SO JOURNAL OF MICRO-NANOLITHOGRAPHY MEMS AND MOEMS LA English DT Article DE optics-free lithography; inorganic photoresists; colloids nanoparticles; plasma; low-cost and rapid; self-assembly ID COLLOIDAL NANOCRYSTALS; FILMS AB We describe a lithographic approach-nanocrystal plasma polymerization-based lithography-in which colloidal nanocrystal assemblies (CNAs) are used as the inorganic resist and, potentially, the active material. The patterning process is based on a change in the dispersibility of the CNAs in solvents as a result of the exposure to plasmas. Plasmas can etch the capping ligands from the exposed area. During the development step, the unexposed area of CNAs is redispersed, leaving behind the patterned area, similar to what is expected from negative photoresist. (C) 2016 Society of Photo-Optical Instrumentation Engineers (SPIE) C1 [Shaw, Santosh; Miller, Kyle J.; Cademartiri, Ludovico] Iowa State Univ, L Cademartiri Lab, Mat Sci & Engn, 2240 Hoover Hall, Ames, IA 50011 USA. [Colaux, Julien L.] Univ Surrey, Surrey Ion Beam Ctr, Nodus Lab, Guildford GU2 7XH, Surrey, England. [Cademartiri, Ludovico] Iowa State Univ, Chem & Biol Engn, 2114 Sweeney Hall, Ames, IA 50011 USA. [Cademartiri, Ludovico] US DOE, Ames Lab, Ames, IA 50011 USA. RP Cademartiri, L (reprint author), Iowa State Univ, L Cademartiri Lab, Mat Sci & Engn, 2240 Hoover Hall, Ames, IA 50011 USA.; Cademartiri, L (reprint author), Iowa State Univ, Chem & Biol Engn, 2114 Sweeney Hall, Ames, IA 50011 USA.; Cademartiri, L (reprint author), US DOE, Ames Lab, Ames, IA 50011 USA. EM lcademar@iastate.edu RI Cademartiri, Ludovico/A-4142-2008 OI Cademartiri, Ludovico/0000-0001-8805-9434 FU MSR-Intel program of Semiconductor Research Corporation [2015-IN-2582]; Iowa State University of Science and Technology FX This research has been supported by MSR-Intel program of Semiconductor Research Corporation under Award Number 2015-IN-2582. Initial effort on particle synthesis was supported by Iowa State University of Science and Technology through a startup grant to LC. We thank S. Schlorholtz and C. Pan for assistance with XRD measurements and patterning experiments, respectively. NR 20 TC 1 Z9 1 U1 3 U2 3 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 1932-5150 EI 1932-5134 J9 J MICRO-NANOLITH MEM JI J. Micro-Nanolithogr. MEMS MOEMS PD JUL PY 2016 VL 15 IS 3 AR 031607 DI 10.1117/1.JMM.15.3.031607 PG 6 WC Engineering, Electrical & Electronic; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Optics SC Engineering; Science & Technology - Other Topics; Materials Science; Optics GA EC6AX UT WOS:000388219500007 ER PT J AU Jacobs, CB Ievlev, AV Collins, LF Muckley, ES Joshi, PC Ivanov, IN AF Jacobs, Christopher B. Ievlev, Anton V. Collins, Liam F. Muckley, Eric S. Joshi, Pooran C. Ivanov, Ilia N. TI Imaging of electrical response of NiOx under controlled environment with sub-25-nm resolution SO JOURNAL OF PHOTONICS FOR ENERGY LA English DT Article DE nickel oxide; humidity; local conductivity; Kelvin probe force microscopy; conductive atomic force microscopy ID PROBE FORCE MICROSCOPY; THIN-FILMS; ELECTRONIC-STRUCTURE; OXIDE SURFACES; SOLAR-CELLS; ADSORPTION; NIO(100); NICKEL; NIO(111); NI(111) AB The spatially resolved electrical response of polycrystalline NiOx films, composed of 40 nm crystallites, was investigated under different relative humidity (RH) levels. The topological and electrical properties (surface potential and resistance) were characterized with sub-25-nm resolution using Kelvin probe force microscopy and conductive scanning probe microscopy under argon atmosphere with 0%, 50%, and 80% RH. The dimensionality of surface features obtained through autocorrelation analysis of topological maps increased linearly with increased RH, as water was adsorbed onto the film surface. Surface potential decreased from 280 to 100 mV and resistance decreased from 5 G Omega to 3 G Omega, in a nonlinear fashion when RH was increased from 0% to 80%. Spatially resolved surface potential and resistance of the NiOx films was found to be heterogeneous throughout the film, with distinct surface features that grew in size from 60 to 175 nm at 0% and 80% RH levels, respectively. The heterogeneous character of the topological, surface potential, and resistance properties of the polycrystalline NiOx film observed under dry conditions decreased with increased RH, yielding nearly homogeneous surface properties at 80% RH, suggesting that the nanoscale potential and resistance properties converge with the mesoscale properties as water is adsorbed onto the NiOx film. (C) 2016 Society of Photo-Optical Instrumentation Engineers (SPIE) C1 [Jacobs, Christopher B.; Ievlev, Anton V.; Collins, Liam F.; Muckley, Eric S.; Ivanov, Ilia N.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, POB 2008, Oak Ridge, TN 37831 USA. [Joshi, Pooran C.] Oak Ridge Natl Lab, Mat Sci & Technol Div, POB 2008, Oak Ridge, TN 37831 USA. RP Ivanov, IN (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, POB 2008, Oak Ridge, TN 37831 USA. EM ivanovin@ornl.gov RI Ievlev, Anton/H-3678-2012; OI Ievlev, Anton/0000-0003-3645-0508; Jacobs, Christopher/0000-0001-7906-6368; Muckley, Eric/0000-0001-7114-5424; ivanov, ilia/0000-0002-6726-2502 FU U.S. Department of Energy (DOE), Advanced Manufacturing Office, Low Temperature Material Synthesis Program [CPS 24762, CPS 24764]; Laboratory Directed Research and Development Program (LDRD) of Oak Ridge National Laboratory; U.S. Department of Energy [DE-AC05-00OR22725] FX This research was conducted at the Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. NiOx sample preparation was supported by the U.S. Department of Energy (DOE), Advanced Manufacturing Office, Low Temperature Material Synthesis Program (CPS 24762 and CPS 24764). C.J. acknowledges support by the Laboratory Directed Research and Development Program (LDRD) of Oak Ridge National Laboratory. This paper has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this paper, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 25 TC 1 Z9 1 U1 4 U2 4 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 1947-7988 J9 J PHOTON ENERGY JI J. Photonics Energy PD JUL-SEP PY 2016 VL 6 IS 3 AR 038001 DI 10.1117/1.JPE.6.038001 PG 8 WC Materials Science, Multidisciplinary; Optics; Physics, Applied SC Materials Science; Optics; Physics GA EC6FQ UT WOS:000388232300009 ER PT J AU Mieno, H Kabe, R Notsuka, N Allendorf, MD Adachi, C AF Mieno, Hiroyuki Kabe, Ryota Notsuka, Naoto Allendorf, Mark D. Adachi, Chihaya TI Long-Lived Room-Temperature Phosphorescence of Coronene in Zeolitic Imidazolate Framework ZIF-8 SO ADVANCED OPTICAL MATERIALS LA English DT Article ID METAL-ORGANIC FRAMEWORKS; BENZOPHENONE PHOSPHORESCENCE; IMPARTING FUNCTIONALITY; COORDINATION POLYMERS; NANOPOROUS MATERIALS; MOF NANOPARTICLES; EXCITED-STATES; ENCAPSULATION; FLUORESCENCE; PHOTOCHEMISTRY C1 [Mieno, Hiroyuki; Kabe, Ryota; Notsuka, Naoto; Adachi, Chihaya] Kyushu Univ, Ctr Organ Photon & Elect Res OPERA, Nishi Ku, 744 Motooka, Fukuoka 8190395, Japan. [Kabe, Ryota; Adachi, Chihaya] Kyushu Univ, JST ERATO Adachi Mol Exciton Engn Project, Nishi Ku, 744 Motooka, Fukuoka 8190395, Japan. [Allendorf, Mark D.] Sandia Natl Labs, Livermore, CA 94551 USA. [Adachi, Chihaya] Kyushu Univ, Int Inst Carbon Neutral Energy Res WPI I2CNER, Nishi Ku, 744 Motooka, Fukuoka 8190395, Japan. RP Kabe, R; Adachi, C (reprint author), Kyushu Univ, Ctr Organ Photon & Elect Res OPERA, Nishi Ku, 744 Motooka, Fukuoka 8190395, Japan.; Kabe, R; Adachi, C (reprint author), Kyushu Univ, JST ERATO Adachi Mol Exciton Engn Project, Nishi Ku, 744 Motooka, Fukuoka 8190395, Japan.; Adachi, C (reprint author), Kyushu Univ, Int Inst Carbon Neutral Energy Res WPI I2CNER, Nishi Ku, 744 Motooka, Fukuoka 8190395, Japan. EM kabe@opera.kyushu-u.ac.jp; adachi@opera.kyushu-u.ac.jp OI Kabe, Ryota/0000-0002-3647-4262 FU Japan Science and Technology Agency (JST); ERATO; Adachi Molecular Exciton Engineering Project; International Institute for Carbon Neutral Energy Research (WPI-I2CNER) - Ministry of Education, Culture, Sports, Science and Technology (MEXT); U.S. Department of Energy Office of Energy Efficiency and Renewable Energy SunShot Program [DE-EE0000990-1634]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Japan Science and Technology Agency (JST), ERATO, Adachi Molecular Exciton Engineering Project, the International Institute for Carbon Neutral Energy Research (WPI-I2CNER) sponsored by the Ministry of Education, Culture, Sports, Science and Technology (MEXT), and by the U.S. Department of Energy Office of Energy Efficiency and Renewable Energy SunShot Program under award number DE-EE0000990-1634. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 50 TC 5 Z9 5 U1 30 U2 31 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 2195-1071 J9 ADV OPT MATER JI Adv. Opt. Mater. PD JUL PY 2016 VL 4 IS 7 BP 1015 EP 1021 DI 10.1002/adom.201600103 PG 7 WC Materials Science, Multidisciplinary; Optics SC Materials Science; Optics GA DW4FV UT WOS:000383599000005 ER PT J AU Rosseel, TM Maruyama, I Le Pape, Y Kontani, O Giorla, AB Remec, I Wall, JJ Sircar, M Andrade, C Ordonez, M AF Rosseel, Thomas M. Maruyama, Ippei Le Pape, Yann. Kontani, Osamu Giorla, Alain B. Remec, Igor Wall, James J. Sircar, Madhumita Andrade, Carmen Ordonez, Manuel TI Review of the Current State of Knowledge on the Effects of Radiation on Concrete SO JOURNAL OF ADVANCED CONCRETE TECHNOLOGY LA English DT Review ID ALKALI-SILICA REACTION; BEAM-INDUCED AMORPHIZATION; 90 DEGREES-C; GAMMA-IRRADIATION; NUCLEAR RADIATION; PROPERTY CHANGES; CEMENT PASTE; ALPHA-QUARTZ; EARLY AGE; S-H AB A review of the current state of knowledge on the effects of radiation on concrete in nuclear power production applications is presented. Emphasis is placed on the effects of radiation damage, as reflected by changes in engineering properties of concrete, in the evaluation of the long-term operation and for plant life or aging management of nuclear power plants (NPPs) in Japan, Spain, and the United States. National issues and concerns are described for Japan and the United States followed by a discussion of the fundamental understanding of the effects of radiation on concrete. Specifically, the effects of temperature, moisture content, and irradiation on ordinary Portland cement paste and the role of temperature and neutron energy spectra on radiation-induced volumetric expansion (RIVE) of aggregate-forming minerals are described. This is followed by a discussion of the bounding conditions for extended operation; the significance of accelerated irradiation conditions; the role of temperature and creep; and how these issues are being incorporated into numerical and meso-scale models. From these insights on radiation damage, analyses of these effects on concrete structures are reviewed, and the current status of work in Japan and the United States is described. Also discussed is the recent formation of a new international scientific and technical organization, the International Committee on Irradiated Concrete, to provide a forum for timely information exchanges among organizations pursuing the identification, quantification, and modeling of the effects of radiation on concrete in commercial nuclear applications. The paper concludes with a discussion of research gaps, including (1) interpreting test-reactor data, (2) evaluating service-irradiated concrete for aging management and to inform radiation damage models with the Zorita NPP (Spain) serving as the first comprehensive test case, (3) irradiated-assisted alkali-silica reactions, and (4) RIVE under constrained conditions. C1 [Rosseel, Thomas M.; Le Pape, Yann.; Giorla, Alain B.; Remec, Igor] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. [Maruyama, Ippei] Nagoya Univ, Nagoya, Aichi, Japan. [Kontani, Osamu] Kajima Corp, Tokyo, Japan. [Wall, James J.] Elect Power Res Inst, Charlotte, NC USA. [Sircar, Madhumita] US Nucl Regulatory Commiss, Washington, DC 20555 USA. [Andrade, Carmen] Inst Eduardo Torroja Ciencias Construcc, Madrid, Spain. [Ordonez, Manuel] ENRESA, Madrid, Spain. RP Rosseel, TM; Le Pape, Y (reprint author), Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA.; Maruyama, I (reprint author), Nagoya Univ, Nagoya, Aichi, Japan. EM rosseeltm@ornl.gov; ippei@dali.nuac.nagoya-u.ac.jp; lepapeym@ornl.gov OI Rosseel, Thomas/0000-0001-9917-7073 FU US DOE, Office of Nuclear Energy, Light Water Reactor Sustainability Program; Nuclear Regulation Authority, Japan; EPRI Long Term Operations Program; US NRC; Consejo de Seguridad Nuclear; IETcc-CSIC; ENRESA FX The authors gratefully thank the following sponsors: US DOE, Office of Nuclear Energy, Light Water Reactor Sustainability Program (TMR, YLP, ABG, and IR); the Nuclear Regulation Authority, Japan (IM and OK); the EPRI Long Term Operations Program (JJW); the US NRC (MS); Consejo de Seguridad Nuclear (CA and MO); IETcc-CSIC (CA); and ENRESA (MO) for support of work on the effects of radiation on concrete. The authors also express their appreciation to Drs. Kevin Field and Elena Tajuelo Rodriguez for their review of the document and their helpful comments and suggestions. NR 98 TC 1 Z9 1 U1 5 U2 5 PU JAPAN CONCRETE INST PI CHIYODA-KU PA SOGO HANZOMON BLDG 12F, NO 7, KOJIMACHI 1-CHOME, CHIYODA-KU, TOKYO 102-0083, JAPAN SN 1346-8014 EI 1347-3913 J9 J ADV CONCR TECHNOL JI J. Adv. Concr. Technol. PD JUL PY 2016 VL 14 IS 7 BP 368 EP 383 DI 10.3151/jact.14.368 PG 16 WC Construction & Building Technology; Engineering, Civil; Materials Science, Multidisciplinary SC Construction & Building Technology; Engineering; Materials Science GA EA5RK UT WOS:000386679800005 ER PT J AU Adams, C Bambaugh, A Bilki, B Butler, J Corriveau, F Cundiff, T Drake, G Francis, K Furst, B Guarino, V Haberichter, B Hazen, E Hoff, J Holm, S Kreps, A DeLurgio, P Matijas, Z Dal Monte, L Mucia, N Norbeck, E Northacker, D Onel, Y Pollack, B Repond, J Schlereth, J Skrzecz, F Smith, JR Trojand, D Underwood, D Velasco, M Walendziak, J Wood, K Wu, S Xia, L Zhang, Q Zhao, A AF Adams, C. Bambaugh, A. Bilki, B. Butler, J. Corriveau, F. Cundiff, T. Drake, G. Francis, K. Furst, B. Guarino, V. Haberichter, B. Hazen, E. Hoff, J. Holm, S. Kreps, A. DeLurgio, P. Matijas, Z. Dal Monte, L. Mucia, N. Norbeck, E. Northacker, D. Onel, Y. Pollack, B. Repond, J. Schlereth, J. Skrzecz, F. Smith, J. R. Trojand, D. Underwood, D. Velasco, M. Walendziak, J. Wood, K. Wu, S. Xia, L. Zhang, Q. Zhao, A. TI Design, construction and commissioning of the Digital Hadron Calorimeter - DHCAL SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Calorimeter methods; Resistive-plate chambers AB A novel hadron calorimeter is being developed for future lepton colliding beam detectors. The calorimeter is optimized for the application of Particle Flow Algorithms (PFAs) to the measurement of hadronic jets and features a very finely segmented readout with 1 x 1 cm(2) cells. The active media of the calorimeter are Resistive Plate Chambers (RPCs) with a digital, i.e. one-bit, readout. To first order the energy of incident particles in this calorimeter is reconstructed as being proportional to the number of pads with a signal over a given threshold. A large-scale prototype calorimeter with approximately 500,000 readout channels has been built and underwent extensive testing in the Fermilab and CERN test beams. This paper reports on the design, construction, and commissioning of this prototype calorimeter. C1 [Adams, C.; Bilki, B.; Cundiff, T.; Drake, G.; Francis, K.; Furst, B.; Guarino, V.; Haberichter, B.; Kreps, A.; DeLurgio, P.; Matijas, Z.; Repond, J.; Schlereth, J.; Skrzecz, F.; Smith, J. R.; Underwood, D.; Walendziak, J.; Wood, K.; Xia, L.; Zhang, Q.; Zhao, A.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Zhang, Q.] Chinese Acad Sci, Inst High Energy Phys, POB 918, Beijing 100049, Peoples R China. [Butler, J.; Hazen, E.; Wu, S.] Boston Univ, 590 Commonwealth Ave, Boston, MA 02215 USA. [Bambaugh, A.; Hoff, J.; Holm, S.; Dal Monte, L.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Bilki, B.; Norbeck, E.; Northacker, D.; Onel, Y.] Univ Iowa, Dept Phys & Astron, 203 Van Allen Hall, Iowa City, IA 52242 USA. [Corriveau, F.; Trojand, D.] McGill Univ, 3600 Univ St, Montreal, PQ H3A 2T8, Canada. [Mucia, N.; Pollack, B.; Velasco, M.] Northwestern Univ, 2145 Sheridan Rd, Evanston, IL 60208 USA. [Smith, J. R.] Univ Texas Arlington, POB 19059, Arlington, TX 76019 USA. [Francis, K.] Northern Illinois Univ, De Kalb, IL 60115 USA. [Trojand, D.] Univ Windsor, Windsor, ON N9B 3P4, Canada. [Zhang, Q.] Xi An Jiao Tong Univ, Shanghai, Peoples R China. RP Repond, J (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM repond@anl.gov NR 12 TC 1 Z9 1 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD JUL PY 2016 VL 11 AR P07007 DI 10.1088/1748-0221/11/07/P07007 PG 22 WC Instruments & Instrumentation SC Instruments & Instrumentation GA EC0BO UT WOS:000387762700007 ER PT J AU Saha, K Benmaimon, R Prabhakaran, A Rappaport, ML Heber, O Schwalm, D Zajfman, D AF Saha, K. Benmaimon, R. Prabhakaran, A. Rappaport, M. L. Heber, O. Schwalm, D. Zajfman, D. TI Position information by signal analysis in real time from resistive anode microchannel plate detector SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Data acquisition concepts; Data processing methods; Data reduction methods; Digital signal processing (DSP) ID RESOLUTION; PHOTON; SYSTEMS; ENCODER; STORAGE; WEDGE AB Resistive anode multichannel plate detectors are extensively used for imaging photons, electrons and ions. We present a method to acquire position information from such detector systems by considering simple parameters of the signals produced from the resistive anode encoder. Our technique is easy to implement and computes position in real time during experiments. Position information can be obtained using our method without the need for dedicated position analyser units. C1 [Saha, K.; Benmaimon, R.; Prabhakaran, A.; Rappaport, M. L.; Heber, O.; Schwalm, D.; Zajfman, D.] Weizmann Inst Sci, Dept Particle Phys & Astrophys, 234 Herzl St, IL-7610001 Rehovot, Israel. [Schwalm, D.] Max Planck Inst Kernphys, Saupfercheckweg 1, D-69117 Heidelberg, Germany. [Prabhakaran, A.] Pacific Northwest Natl Lab, Richland, WA USA. RP Saha, K (reprint author), Weizmann Inst Sci, Dept Particle Phys & Astrophys, 234 Herzl St, IL-7610001 Rehovot, Israel. EM koushik.saha@weizmann.ac.il FU Nella Benoziyo Fund; COST XLIC Action [CM 1204]; Joseph Meyerhoff program FX This work was supported by Nella Benoziyo Fund and by COST CM 1204 XLIC Action. D.S. acknowledges support by Joseph Meyerhoff program. NR 23 TC 1 Z9 1 U1 3 U2 3 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD JUL PY 2016 VL 11 AR T07006 DI 10.1088/1748-0221/11/07/T07006 PG 9 WC Instruments & Instrumentation SC Instruments & Instrumentation GA EC0BV UT WOS:000387763500006 ER PT J AU Sherman, KE Ke, R Rouster, SD Abdel-Hameed, EA Park, C Palascak, J Perelson, AS AF Sherman, K. E. Ke, R. Rouster, S. D. Abdel-Hameed, E. A. Park, C. Palascak, J. Perelson, A. S. TI Viral dynamic modelling of Hepatitis C and resistance-associated variants in haemophiliacs SO HAEMOPHILIA LA English DT Article DE direct-acting antivirals; HCV; haemophilia; resistance-associated variants; treatment response; viral dynamic models ID STAGE LIVER-DISEASE; INTERFERON-ALPHA; TELAPREVIR; MUTATIONS; THERAPY AB Aim: Chronic hepatitis C virus (HCV) infection is an important source of morbidity and mortality among haemophiliacs. Limited data are available regarding treatment intervention using direct-acting antivirals (DAAs) and theoretical concerns regarding accumulation of drug-associated resistance variants (RAVs) remain. We conducted a pilot study of treatment with telaprevir/pegylated interferon-alfa/ribavirin to evaluate treatment response and the role of lead-in DAA therapy on mutational selection of resistance variants. Methods: Ultra-deep sequence analysis was performed at baseline, 48 hours and 168 hours after treatment initiation. Results: No dominant RAVs were identified at baseline, but low-level RAVs were noted at baseline in all subjects. Viral dynamic models were used to assess treatment responses. The efficacy parameter (epsilon) for lead-in ranged from 0 to 0.9745 (mean = 0.514). Subsequent addition of telaprevir resulted in a mean efficacy of more than 0.999. This was comparable to subjects who started all three medications simultaneously. A total of 80% achieved SVR. While rapid shifts in the RAV population following DAA initiation were observed, treatment failure associated with A156V was observed in only one patient. Adverse event profiles were similar to that observed in non-haemophilia cohorts. There was no evidence of factor inhibitor formation. There was no evidence that lead-in provided benefit in terms of response efficacy. Conclusion: These data support DAA-based therapy in those with inherited bleeding disorders. C1 [Sherman, K. E.; Rouster, S. D.; Abdel-Hameed, E. A.; Park, C.] Univ Cincinnati, Coll Med, Div Digest Dis, Cincinnati, OH USA. [Ke, R.; Perelson, A. S.] Los Alamos Natl Lab, Theoret Biol & Biophys Grp, Los Alamos, NM USA. [Palascak, J.] Univ Cincinnati, Coll Med, Div Hematol & Oncol, Cincinnati, OH USA. RP Sherman, KE (reprint author), Univ Cincinnati, Coll Med, Div Digest Dis, Med, 231 Albert Sabin Way, Cincinnati, OH 45267 USA. EM Kenneth.sherman@uc.edu FU NCATS NIH HHS [UL1 TR000077, UL1 TR001425]; NHLBI NIH HHS [R34 HL109334]; NIAID NIH HHS [R01 AI028433]; NIDDK NIH HHS [K24 DK070528]; NIEHS NIH HHS [P30 ES006096]; NIH HHS [R01 OD011095] NR 14 TC 0 Z9 0 U1 1 U2 1 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1351-8216 EI 1365-2516 J9 HAEMOPHILIA JI Haemophilia PD JUL PY 2016 VL 22 IS 4 BP 543 EP 548 DI 10.1111/hae.12918 PG 6 WC Hematology SC Hematology GA EB5BC UT WOS:000387387000033 PM 26936587 ER PT J AU Coplen, TB Holden, NE AF Coplen, Tyler B. Holden, Norman E. TI Review of footnotes and annotations to the 1949-2013 tables of standard atomic weights and tables of isotopic compositions of the elements (IUPAC Technical Report) SO PURE AND APPLIED CHEMISTRY LA English DT Review DE artificial isotopic separation; atomic weight intervals; atomic weight variations; mononuclidic element; normal material; Oklo natural reactor; stable isotope; undisclosed isotopic fractionation ID OKLO AB The Commission on Isotopic Abundances and Atomic Weights uses annotations given in footnotes that are an integral part of the Tables of Standard Atomic Weights to alert users to the possibilities of quite extraordinary occurrences, as well as sources with abnormal atomic-weight values outside an otherwise acceptable range. The basic need for footnotes to the Standard Atomic Weights Table and equivalent annotations to the Table of Isotopic Compositions of the Elements arises from the necessity to provide users with information that is relevant to one or more elements, but that cannot be provided using numerical data in columns. Any desire to increase additional information conveyed by annotations to these Tables is tempered by the need to preserve a compact format and a style that can alert users, who would not be inclined to consult either the last full element-by-element review or the full text of a current Standard Atomic Weights of the Elements report. Since 1989, the footnotes of the Tables of Standard Atomic Weights and the annotations in column 5 of the Table of Isotopic Compositions of the Elements have been harmonized by use of three lowercase footnotes, "g", "m", and "r", that signify geologically exceptionally specimens ("g"), modified isotopic compositions in material subjected to undisclosed or inadvertent isotopic fractionation ("m"), and the range in isotopic composition of normal terrestrial material prevents more precise atomic-weight value being given ("r"). As some elements are assigned intervals for their standard atomic-weight values (applies to 12 elements since 2009), footnotes "g" and "r" are no longer needed for these elements. C1 [Coplen, Tyler B.] US Geol Survey, 959 Natl Ctr, Reston, VA 22092 USA. [Holden, Norman E.] Brookhaven Natl Lab, Upton, NY 11973 USA. RP Coplen, TB (reprint author), US Geol Survey, 959 Natl Ctr, Reston, VA 22092 USA. EM tbcoplen@usgs.gov FU U.S. Geological Survey National Research Program FX Comments by H. A. J. Meijer (University of Groningen, Groningen, The Netherlands), J. Meija (National Research Council Canada, Ottawa, Canada), and J.K. Bohlke (U.S. Geological Survey, Reston, Virginia, USA) improved this work and are appreciated. The support of the U.S. Geological Survey National Research Program made this report possible. The following IUPAC project contributed to this Technical Report: 2015-030-2-200. NR 37 TC 1 Z9 1 U1 3 U2 3 PU WALTER DE GRUYTER GMBH PI BERLIN PA GENTHINER STRASSE 13, D-10785 BERLIN, GERMANY SN 0033-4545 EI 1365-3075 J9 PURE APPL CHEM JI Pure Appl. Chem. PD JUL PY 2016 VL 88 IS 7 BP 689 EP 699 DI 10.1515/pac-2016-0203 PG 11 WC Chemistry, Multidisciplinary SC Chemistry GA EB2KJ UT WOS:000387188700003 ER PT J AU Tang, WB Cai, P Huo, WW Li, HX Tang, JW Zhu, DM Xie, H Chen, PF Hang, B Wang, SY Xia, YK AF Tang, Weibing Cai, Peng Huo, Weiwei Li, Hongxing Tang, Junwei Zhu, Dongmei Xie, Hua Chen, Pingfa Hang, Bo Wang, Shouyu Xia, Yankai TI Suppressive action of miRNAs to ARP2/3 complex reduces cell migration and proliferation via RAC isoforms in Hirschsprung disease SO JOURNAL OF CELLULAR AND MOLECULAR MEDICINE LA English DT Article DE microRNA; ARP2/3 complex; RAC isoforms; gene regulation; Hirschsprung disease ID ENTERIC NERVOUS-SYSTEM; NEURAL CREST CELLS; MESSENGER-RNA; MICRORNAS; CANCER; DIFFERENTIATION; PROTEIN; COLON; GENE; INHIBITION AB Hirschsprung disease (HSCR) is a congenital disorder caused by the defective function of the embryonic enteric neural crest. The impaired migration of embryonic enteric neural crest plays an important role in the pathogenesis of this disease. Recent studies showed that the ARP2/3 complex and RAC isoforms had effects on actin cytoskeleton remodelling, which contributes to migration. Moreover, some regulatory relationships were identified between ARP2/3 complex and RAC isoforms. Although microRNAs (miRNAs) have been known to modulate target gene expression on the post-transcriptional level, little is known about the regulation among miRNAs, ARP2/3 complex and RAC isoforms. Here, we report that down-regulation of ARP2 and ARP3, two main subunits of ARP2/3 complex, suppressed migration and proliferation in 293T and SH-SY5Y cell lines via the inhibition of RAC1 and RAC2. Meanwhile, as the target genes, ARP2 and ARP3 are reduced by increased miR-24-1* and let-7a*, respectively, in 70 HSCR samples as compared with 74 normal controls. Co-immunoprecipitation showed that aberrant reduction in ARP2 and ARP3 could weaken the function of ARP2/3 complex. Our study demonstrates that the miR-24-1*/let-7a*-ARP2/3 complex-RAC isoforms pathway may represent a novel pathogenic mechanism for HSCR. C1 [Tang, Weibing; Li, Hongxing; Tang, Junwei; Zhu, Dongmei; Xie, Hua; Chen, Pingfa] Nanjing Med Univ, Nanjing Childrens Hosp, Dept Pediat Surg, Nanjing, Jiangsu, Peoples R China. [Tang, Weibing; Huo, Weiwei; Li, Hongxing; Tang, Junwei; Zhu, Dongmei; Xie, Hua; Chen, Pingfa; Wang, Shouyu; Xia, Yankai] Nanjing Med Univ, Inst Toxicol, Sch Publ Hlth, State Key Lab Reprod Med, Nanjing, Jiangsu, Peoples R China. [Cai, Peng] Soochow Univ, Childrens Hosp, Suzhou, Peoples R China. [Huo, Weiwei; Wang, Shouyu; Xia, Yankai] Nanjing Med Univ, Minist Educ, Key Lab Modern Toxicol, Nanjing, Jiangsu, Peoples R China. [Hang, Bo] Lawrence Berkeley Natl Lab, Dept Cell & Mol Biol, Div Life Sci, Berkeley, CA USA. [Wang, Shouyu] Nanjing Med Univ, Dept Mol Cell Biol & Toxicol, Jiangsu Key Lab Canc Biomarkers Prevent & Treatme, Canc Ctr,Sch Publ, Nanjing, Jiangsu, Peoples R China. RP Xia, YK (reprint author), Nanjing Med Univ, Inst Toxicol, Sch Publ Hlth, State Key Lab Reprod Med, Nanjing, Jiangsu, Peoples R China.; Xia, YK (reprint author), Nanjing Med Univ, Minist Educ, Key Lab Modern Toxicol, Nanjing, Jiangsu, Peoples R China. EM yankaixia@njmu.edu.cn FU Natural Science Foundation of China [NSFC 81370473]; Natural Science Foundation of Jiangsu Province of China [BK20131388]; Scientific Research Project of Jiangsu Provincial Department of Health [H201342]; Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD) FX The authors thank Drs. Jie Zhang, Huan Chen, Xiaofeng Lv, Changgui Lu, Wei-wei Jiang and Wei Li (Nanjing Children's Hospital Affiliated to Nanjing Medical University) for sample collection. This work was supported by the Natural Science Foundation of China (grant no. NSFC 81370473), Natural Science Foundation of Jiangsu Province of China (grant no. BK20131388) and the Scientific Research Project of Jiangsu Provincial Department of Health (grant no. H201342) and the Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD). NR 50 TC 1 Z9 1 U1 2 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1582-4934 J9 J CELL MOL MED JI J. Cell. Mol. Med. PD JUL PY 2016 VL 20 IS 7 BP 1266 EP 1275 DI 10.1111/jcmm.12799 PG 10 WC Cell Biology; Medicine, Research & Experimental SC Cell Biology; Research & Experimental Medicine GA DW4BU UT WOS:000383587800007 PM 26991540 ER PT J AU Hung, MS Chen, IC You, L Jablons, DM Li, YC Mao, JH Xu, ZD Lung, JH Yang, CT Liu, ST AF Hung, Ming-Szu Chen, I-Chuan You, Liang Jablons, David M. Li, Ya-Chin Mao, Jian-Hua Xu, Zhidong Lung, Jr-Hau Yang, Cheng-Ta Liu, Shih-Tung TI Knockdown of cullin 4A inhibits growth and increases chemosensitivity in lung cancer cells SO JOURNAL OF CELLULAR AND MOLECULAR MEDICINE LA English DT Article DE Cul4A; lung cancer; chemotherapy; p21 ID EPITHELIAL-MESENCHYMAL TRANSITION; MALIGNANT PLEURAL MESOTHELIOMA; TUMORIGENIC PHENOTYPE; DOWN-REGULATION; BREAST-CANCER; CUL4A; GENE; OVEREXPRESSION; TARGETS; P21 AB Cullin 4A (Cul4A) has been observed to be overexpressed in various cancers. In this study, the role of Cul4A in the growth and chemosensitivity in lung cancer cells were studied. We showed that Cul4A is overexpressed in lung cancer cells and tissues. Knockdown of the Cul4A expression by shRNA in lung cancer cells resulted in decreased cellular proliferation and growth in lung cancer cells. Increased sensitivity to gemcitabine, a chemotherapy drug, was also noted in those Cul4A knockdown lung cancer cells. Moreover, increased expression of p21, transforming growth factor (TGF)-beta inducible early gene-1 (TIEG1) and TGF beta-induced (TGFBI) was observed in lung cancer cells after Cul4A knockdown, which may be partially related to increased chemosensitivity to gemcitabine. G0/G1 cell cycle arrest was also noted after Cul4A knockdown. Notably, decreased tumour growth and increased chemosensitivity to gemcitabine were also noted after Cul4A knockdown in lung cancer xenograft nude mice models. In summary, our study showed that targeting Cul4A with RNAi or other techniques may provide a possible insight to the development of lung cancer therapy in the future. C1 [Hung, Ming-Szu; Li, Ya-Chin] Chang Gung Mem Hosp, Dept Pulm & Crit Care Med, Div Thorac Oncol, Chiayi, Taiwan. [Hung, Ming-Szu] Chang Gung Univ, Dept Med, Coll Med, Taoyuan, Taiwan. [Hung, Ming-Szu] Chang Gung Univ Sci & Technol, Dept Resp Care, Chiayi, Taiwan. [Chen, I-Chuan] Chang Gung Mem Hosp, Dept Emergency Med, Chiayi, Taiwan. [Chen, I-Chuan] Chang Gung Univ Sci & Technol, Dept Nursing, Chiayi, Taiwan. [You, Liang; Jablons, David M.; Xu, Zhidong] Univ Calif San Francisco, Dept Surg, Ctr Comprehens Canc, Thorac Oncol Lab, San Francisco, CA USA. [Mao, Jian-Hua] Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA USA. [Lung, Jr-Hau] Chang Gung Mem Hosp, Dept Med Res & Dev, Chiayi, Taiwan. [Yang, Cheng-Ta] Chang Gung Univ, Dept Resp Care, Coll Med, Taoyuan, Taiwan. [Yang, Cheng-Ta] Chang Gung Mem Hosp, Dept Pulm & Crit Care Med, Taoyuan, Taiwan. [Liu, Shih-Tung] Chang Gung Univ, Dept Microbiol & Immunol, Coll Med, Taoyuan, Taiwan. RP Hung, MS (reprint author), Chang Gung Mem Hosp, Dept Pulm & Crit Care Med, Div Thorac Oncol, Chiayi, Taiwan.; Hung, MS (reprint author), Chang Gung Univ, Dept Med, Coll Med, Taoyuan, Taiwan.; Hung, MS (reprint author), Chang Gung Univ Sci & Technol, Dept Resp Care, Chiayi, Taiwan. EM m12049@adm.cgmh.org.tw FU Chang Gung Memorial Hospital [CMRP 680461, CMRPG6E0081, NMRP 696031]; National Science Council, Taiwan [99-2314-B-182-056-MY2] FX This study was supported by grants from Chang Gung Memorial Hospital (CMRP 680461, CMRPG6E0081 and NMRP 696031) and National Science Council, Taiwan (99-2314-B-182-056-MY2). We would like to acknowledge the BD FACS Canto II flow cytometer service provided by the Expensive Advanced Instrument Core Laboratory, Department of Medical Research and Development, Chang Gung Memorial Hospital at Chiayi. NR 39 TC 1 Z9 1 U1 0 U2 0 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1582-4934 J9 J CELL MOL MED JI J. Cell. Mol. Med. PD JUL PY 2016 VL 20 IS 7 BP 1295 EP 1306 DI 10.1111/jcmm.12811 PG 12 WC Cell Biology; Medicine, Research & Experimental SC Cell Biology; Research & Experimental Medicine GA DW4BU UT WOS:000383587800010 PM 26969027 ER PT J AU Alduino, C Alfonso, K Artusa, DR Avignone, FT Azzolini, O Balata, M Banks, TI Bari, G Beeman, JW Bellini, F Bersani, A Biare, D Biassoni, M Bragazzi, F Brofferio, C Buccheri, A Bucci, C Bulfon, C Caminata, A Canonica, L Cao, XG Capelli, S Capodiferro, M Cappelli, L Carbone, L Cardani, L Cariello, M Carniti, P Casali, N Cassina, L Cereseto, R Ceruti, G Chiarini, A Chiesa, D Chott, N Clemenza, M Conventi, D Copello, S Cosmelli, C Cremonesi, O Creswick, RJ Cushman, JS D'Addabbo, A Dafinei, I Davis, CJ Dell'Oro, S Deninno, MM Di Domizio, S Di Vacri, ML DiPaolo, L Drobizhev, A Erme, G Fang, DQ Faverzani, M Fernandes, G Ferri, E Ferroni, F Fiorini, E Freedman, SJ Fujikawa, BK Gaigher, R Giachero, A Gironi, L Giuliani, A Gladstone, L Gorla, P Gotti, C Guetti, M Gutierrez, TD Haller, EE Han, K Hansen, E Heeger, KM Hennings-Yeomans, R Hickerson, KP Huang, HZ Iannone, M Ioannucci, L Kadel, R Keppel, G Kolomensky, YG Leder, A Lim, KE Liu, X Ma, YG Maino, M Marini, L Martinez, M Maruyama, RH Mazza, R Mei, Y Meijer, S Michinelli, R Miller, D Moggi, N Morganti, S Mosteiro, PJ Nastasi, M Nisi, S Nones, C Norman, EB Nucciotti, A O'Donnell, T Orio, F Orlandi, D Ouellet, JL Pagliarone, CE Pallavicini, M Palmieri, V Pancaldi, G Pattavina, L Pavan, M Pedrotta, R Pelosi, A Perego, M Pessina, G Pettinacci, V Piperno, G Pirro, S Pozzi, S Previtali, E Rosenfeld, C Rusconi, C Sala, E Sangiorgio, S Santone, D Scielzo, ND Singh, V Sisti, M Smith, AR Stivanello, F Taffarello, L Tatananni, L Tenconi, M Terranova, F Tessaro, M Tomei, C Trentalange, S Ventura, G Vignati, M Wagaarachchi, SL Wallig, J Wang, BS Wang, HW Wilson, J Winslow, LA Wise, T Zanotti, L Zarra, C Zhang, GQ Zhu, BX Zimmermann, S Zucchelli, S AF Alduino, C. Alfonso, K. Artusa, D. R. Avignone, F. T., III Azzolini, O. Balata, M. Banks, T. I. Bari, G. Beeman, J. W. Bellini, F. Bersani, A. Biare, D. Biassoni, M. Bragazzi, F. Brofferio, C. Buccheri, A. Bucci, C. Bulfon, C. Caminata, A. Canonica, L. Cao, X. G. Capelli, S. Capodiferro, M. Cappelli, L. Carbone, L. Cardani, L. Cariello, M. Carniti, P. Casali, N. Cassina, L. Cereseto, R. Ceruti, G. Chiarini, A. Chiesa, D. Chott, N. Clemenza, M. Conventi, D. Copello, S. Cosmelli, C. Cremonesi, O. Creswick, R. J. Cushman, J. S. D'Addabbo, A. Dafinei, I. Davis, C. J. Dell'Oro, S. Deninno, M. M. Di Domizio, S. Di Vacri, M. L. DiPaolo, L. Drobizhev, A. Erme, G. Fang, D. Q. Faverzani, M. Fernandes, G. Ferri, E. Ferroni, F. Fiorini, E. Freedman, S. J. Fujikawa, B. K. Gaigher, R. Giachero, A. Gironi, L. Giuliani, A. Gladstone, L. Gorla, P. Gotti, C. Guetti, M. Gutierrez, T. D. Haller, E. E. Han, K. Hansen, E. Heeger, K. M. Hennings-Yeomans, R. Hickerson, K. P. Huang, H. Z. Iannone, M. Ioannucci, L. Kadel, R. Keppel, G. Kolomensky, Yu. G. Leder, A. Lim, K. E. Liu, X. Ma, Y. G. Maino, M. Marini, L. Martinez, M. Maruyama, R. H. Mazza, R. Mei, Y. Meijer, S. Michinelli, R. Miller, D. Moggi, N. Morganti, S. Mosteiro, P. J. Nastasi, M. Nisi, S. Nones, C. Norman, E. B. Nucciotti, A. O'Donnell, T. Orio, F. Orlandi, D. Ouellet, J. L. Pagliarone, C. E. Pallavicini, M. Palmieri, V. Pancaldi, G. Pattavina, L. Pavan, M. Pedrotta, R. Pelosi, A. Perego, M. Pessina, G. Pettinacci, V. Piperno, G. Pirro, S. Pozzi, S. Previtali, E. Rosenfeld, C. Rusconi, C. Sala, E. Sangiorgio, S. Santone, D. Scielzo, N. D. Singh, V. Sisti, M. Smith, A. R. Stivanello, F. Taffarello, L. Tatananni, L. Tenconi, M. Terranova, F. Tessaro, M. Tomei, C. Trentalange, S. Ventura, G. Vignati, M. Wagaarachchi, S. L. Wallig, J. Wang, B. S. Wang, H. W. Wilson, J. Winslow, L. A. Wise, T. Zanotti, L. Zarra, C. Zhang, G. Q. Zhu, B. X. Zimmermann, S. Zucchelli, S. CA CUORE Collaboration TI CUORE-0 detector: design, construction and operation SO JOURNAL OF INSTRUMENTATION LA English DT Article DE Calorimeters; Cryogenics; Double-beta decay detectors ID DOUBLE-BETA DECAY; LARGE-MASS BOLOMETERS; FRONT-END; RADIOACTIVE CONTAMINATION; RESPONSE STABILIZATION; RARE EVENTS; CUORICINO; TE-130; NOISE; ARRAY AB The CUORE experiment will search for neutrinoless double-beta decay of Te-130 with an array of 988 TeO2 bolometers arranged in 19 towers. CUORE-0, the first tower assembled according to the CUORE procedures, was built and commissioned at Laboratori Nazionali del Gran Sasso, and took data from March 2013 to March 2015. In this paper we describe the design, construction and operation of the CUORE-0 experiment, with an emphasis on the improvements made over a predecessor experiment, Cuoricino. In particular, we demonstrate with CUORE-0 data that the design goals of CUORE are within reach. C1 [Cardani, L.] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA. [Piperno, G.] Ist Nazl Fis Nucl, Lab Nazl Frascati, Via E Fermi 40, I-00044 Rome, Italy. [Alduino, C.; Artusa, D. R.; Avignone, F. T., III; Chott, N.; Creswick, R. J.; Rosenfeld, C.; Wilson, J.] Univ South Carolina, Dept Phys & Astron, Columbia, SC 29208 USA. [Alfonso, K.; Hansen, E.; Hickerson, K. P.; Huang, H. Z.; Liu, X.; Trentalange, S.; Zhu, B. X.] Univ Calif Los Angeles, Dept Phys & Astron, Los Angeles, CA 90095 USA. [Artusa, D. R.; Balata, M.; Bucci, C.; Canonica, L.; Cappelli, L.; D'Addabbo, A.; Dell'Oro, S.; Di Vacri, M. L.; Erme, G.; Gorla, P.; Guetti, M.; Ioannucci, L.; Nisi, S.; Orlandi, D.; Pagliarone, C. E.; Pattavina, L.; Pirro, S.; Santone, D.; Tatananni, L.; Zarra, C.] Ist Nazl Fis Nucl, Lab Nazl Gran Sasso, I-67010 Laquila, Italy. [Azzolini, O.; Conventi, D.; Keppel, G.; Palmieri, V.; Stivanello, F.] Ist Nazl Fis Nucl, Lab Nazl Legnaro, I-35020 Padua, Italy. [Banks, T. I.; Drobizhev, A.; Freedman, S. J.; Hennings-Yeomans, R.; Kolomensky, Yu. G.; O'Donnell, T.; Ouellet, J. L.; Singh, V.; Wagaarachchi, S. L.] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. [Banks, T. I.; Biare, D.; DiPaolo, L.; Drobizhev, A.; Freedman, S. J.; Fujikawa, B. K.; Hennings-Yeomans, R.; Kolomensky, Yu. G.; Mei, Y.; Meijer, S.; Miller, D.; O'Donnell, T.; Ouellet, J. L.; Smith, A. R.; Wagaarachchi, S. L.] Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Bari, G.; Chiarini, A.; Deninno, M. M.; Michinelli, R.; Moggi, N.; Pancaldi, G.; Zucchelli, S.] Ist Nazl Fis Nucl, Sez Bologna, I-40127 Bologna, Italy. [Beeman, J. W.; Haller, E. E.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Bellini, F.; Cardani, L.; Casali, N.; Cosmelli, C.; Ferroni, F.; Martinez, M.; Piperno, G.] Sapienza Univ Roma, Dipartimento Fis, I-00185 Rome, Italy. [Bellini, F.; Buccheri, A.; Bulfon, C.; Capodiferro, M.; Cardani, L.; Casali, N.; Cosmelli, C.; Dafinei, I.; Ferroni, F.; Iannone, M.; Martinez, M.; Morganti, S.; Mosteiro, P. J.; Orio, F.; Pelosi, A.; Pettinacci, V.; Piperno, G.; Tomei, C.; Vignati, M.] Ist Nazl Fis Nucl, Sez Roma, I-00185 Rome, Italy. [Bersani, A.; Bragazzi, F.; Caminata, A.; Cappelli, L.; Cariello, M.; Cereseto, R.; Copello, S.; Di Domizio, S.; Fernandes, G.; Marini, L.; Pallavicini, M.] Ist Nazl Fis Nucl, Sez Genova, I-16146 Genoa, Italy. [Biassoni, M.; Brofferio, C.; Capelli, S.; Carniti, P.; Cassina, L.; Chiesa, D.; Clemenza, M.; Faverzani, M.; Ferri, E.; Fiorini, E.; Gironi, L.; Gotti, C.; Maino, M.; Nastasi, M.; Nucciotti, A.; Pavan, M.; Pozzi, S.; Sala, E.; Sisti, M.; Terranova, F.; Zanotti, L.] Univ Milano Bicocca, Dipartimento Fis, I-20126 Milan, Italy. [Biassoni, M.; Brofferio, C.; Capelli, S.; Carbone, L.; Carniti, P.; Cassina, L.; Ceruti, G.; Chiesa, D.; Clemenza, M.; Cremonesi, O.; Faverzani, M.; Ferri, E.; Fiorini, E.; Gaigher, R.; Giachero, A.; Gironi, L.; Gotti, C.; Maino, M.; Mazza, R.; Nastasi, M.; Nucciotti, A.; Pavan, M.; Perego, M.; Pessina, G.; Pozzi, S.; Previtali, E.; Rusconi, C.; Sala, E.; Sisti, M.; Terranova, F.; Zanotti, L.] Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20126 Milan, Italy. [Cao, X. G.; Fang, D. Q.; Ma, Y. G.; Wang, H. W.; Zhang, G. Q.] Shanghai Inst Appl Phys, Chinese Acad Sci, Shanghai 201800, Peoples R China. [Cappelli, L.; Erme, G.; Pagliarone, C. E.] Univ Cassino & Lazio Merid, Dipartimento Ingn Civile & Meccan, I-03043 Cassino, Italy. [Copello, S.; Di Domizio, S.; Fernandes, G.; Marini, L.; Pallavicini, M.] Univ Genoa, Dipartimento Fis, I-16146 Genoa, Italy. [Cushman, J. S.; Davis, C. J.; Han, K.; Heeger, K. M.; Lim, K. E.; Maruyama, R. H.; Wise, T.] Yale Univ, Dept Phys, New Haven, CT 06520 USA. [Dell'Oro, S.] Ist Nazl Fis Nucl, Gran Sasso Sci Inst, I-67100 Laquila, Italy. [Di Vacri, M. L.; Santone, D.] Univ Aquila, Dipartimento Sci Fis & Chim, I-67100 Laquila, Italy. [Giuliani, A.; Tenconi, M.] Univ Paris Saclay, Univ Paris Sud, CNRS, CSNSM,IN2P3, F-91405 Orsay, France. [Canonica, L.; Gladstone, L.; Hansen, E.; Leder, A.; Ouellet, J. L.; Winslow, L. A.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Gutierrez, T. D.; Meijer, S.; Miller, D.] Calif Polytech State Univ San Luis Obispo, Dept Phys, San Luis Obispo, CA 93407 USA. [Haller, E. E.] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Han, K.] Shanghai Jiao Tong Univ, Dept Phys & Astron, Shanghai 200240, Peoples R China. [Kadel, R.; Kolomensky, Yu. G.] Lawrence Berkeley Natl Lab, Div Phys, Berkeley, CA 94720 USA. [Martinez, M.] Univ Zaragoza, Lab Fis Nucl & Astroparticulas, E-50009 Zaragoza, Spain. [Moggi, N.] Univ Bologna, Alma Mater Studiorum, Dipartimento Sci Qual Vita, I-47921 Bologna, Italy. [Nones, C.] CEA Saclay, Serv Phys Particules, F-91191 Gif Sur Yvette, France. [Norman, E. B.; Sangiorgio, S.; Scielzo, N. D.; Wang, B. S.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Norman, E. B.; Wang, B. S.] Univ Calif Berkeley, Dept Nucl Engn, Berkeley, CA 94720 USA. [Pedrotta, R.; Taffarello, L.; Tessaro, M.] Ist Nazl Fis Nucl, Sez Padova, I-35131 Padua, Italy. [Ventura, G.] Univ Florence, Dipartimento Fis, I-50125 Florence, Italy. [Ventura, G.] Ist Nazl Fis Nucl, Sez Firenze, I-50125 Florence, Italy. [Wallig, J.; Zimmermann, S.] Lawrence Berkeley Natl Lab, Div Engn, Berkeley, CA 94720 USA. [Wise, T.] Univ Wisconsin, Dept Phys, 1150 Univ Ave, Madison, WI 53706 USA. [Zucchelli, S.] Univ Bologna, Alma Mater Studiorum, Dipartimento Fis & Astron, I-40127 Bologna, Italy. RP Cremonesi, O (reprint author), Ist Nazl Fis Nucl, Sez Milano Bicocca, I-20126 Milan, Italy. EM cuore-spokesperson@lngs.infn.it RI Gironi, Luca/P-2860-2016; capelli, silvia/G-5168-2012; Maruyama, Reina/A-1064-2013; Bellini, Fabio/D-1055-2009; Martinez, Maria/K-4827-2012; Casali, Nicola/C-9475-2017; Han, Ke/D-3697-2017; Giachero, Andrea/I-1081-2013; Chiesa, Davide/H-7240-2014; Sisti, Monica/B-7550-2013; Di Domizio, Sergio/L-6378-2014; OI Gironi, Luca/0000-0003-2019-0967; capelli, silvia/0000-0002-0300-2752; Maruyama, Reina/0000-0003-2794-512X; Bellini, Fabio/0000-0002-2936-660X; Martinez, Maria/0000-0002-9043-4691; Casali, Nicola/0000-0003-3669-8247; Han, Ke/0000-0002-1609-7367; Giachero, Andrea/0000-0003-0493-695X; Chiesa, Davide/0000-0003-1978-1727; Sisti, Monica/0000-0003-2517-1909; Di Domizio, Sergio/0000-0003-2863-5895; D'Addabbo, Antonio/0000-0003-2668-962X FU Istituto Nazionale di Fisica Nucleare (INFN); National Science Foundation [NSF-PHY-0605119, NSF-PHY-0500337, NSF-PHY-0855314, NSF-PHY-0902171, NSF-PHY-0969852, NSF-PHY-1307204, NSF-PHY-1314881, NSF-PHY-1401832, NSF-PHY-1404205]; Alfred P. Sloan Foundation; University of Wisconsin Foundation; Yale University; US Department of Energy (DOE) Office of Science [DE-AC02-05CH11231, DE-AC52-07NA27344, DE-SC0012654]; DOE Office of Science, Office of Nuclear Physics [DE-FG02-08ER41551, DE-FG03-00ER41138] FX The CUORE Collaboration thanks the directors and staff of the Laboratori Nazionali del Gran Sasso and the technical staff of our laboratories. This work was supported by the Istituto Nazionale di Fisica Nucleare (INFN); the National Science Foundation under Grant Nos. NSF-PHY-0605119, NSF-PHY-0500337, NSF-PHY-0855314, NSF-PHY-0902171, NSF-PHY-0969852, NSF-PHY-1307204, NSF-PHY-1314881, NSF-PHY-1401832, and NSF-PHY-1404205; the Alfred P. Sloan Foundation; the University of Wisconsin Foundation; and Yale University. This material is also based upon work supported by the US Department of Energy (DOE) Office of Science under Contract Nos. DE-AC02-05CH11231, DE-AC52-07NA27344, and DE-SC0012654; and by the DOE Office of Science, Office of Nuclear Physics under Contract Nos. DE-FG02-08ER41551 and DE-FG03-00ER41138. This research used resources of the National Energy Research Scientific Computing Center (NERSC). NR 64 TC 5 Z9 5 U1 14 U2 15 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-0221 J9 J INSTRUM JI J. Instrum. PD JUL PY 2016 VL 11 AR P07009 DI 10.1088/1748-0221/11/07/P07009 PG 38 WC Instruments & Instrumentation SC Instruments & Instrumentation GA EA8JI UT WOS:000386880700001 ER PT J AU Levinson, RS Manley, DK West, TH AF Levinson, Rebecca S. Manley, Dawn K. West, Todd H. TI History v. Simulation: An Analysis of the Drivers of Alternative Energy Vehicle Sales SO SAE INTERNATIONAL JOURNAL OF ALTERNATIVE POWERTRAINS LA English DT Article AB Simulations of the US light duty vehicle stock help policy makers, investors, and auto manufacturers make informed decisions to influence the future of the stock and its associated green house gas emissions. Such simulations require an underlying framework that captures the key elements of consumer purchasing decisions, which can be uncertain. This uncertainty in a simulation's logic is usually convolved with uncertainty in the underlying assumptions about the futures of energy prices and technology innovation and availability. By comparing simulated alternative energy vehicle (AEV) sales to historical sales data, one can assess the simulation's ability to capture the dynamics of consumer choice, independent of many of those underlying uncertainties, thereby determining the factors that most strongly impact sales. The market for diesel vehicles, hybrid electric vehicles, and to a lesser extent plug-in hybrid electric vehicles and all-electric vehicles, has now matured sufficiently to make such a study possible. In this work, we measure the results of the Sandia ParaChoice model under a variety of input assumptions against historical sales data. We observe that (1) the underlying simulation logic is sound, capturing key drivers of consumer choice, (2) AEV model availability has a significant impact on sales, and (3) AEV consumers are very likely aware of purchasing incentives and factoring those incentives into their purchasing decisions. C1 [Levinson, Rebecca S.; Manley, Dawn K.; West, Todd H.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Levinson, RS (reprint author), Sandia Natl Labs, Livermore, CA 94550 USA. EM rslevin@sandia.gov NR 62 TC 0 Z9 0 U1 1 U2 1 PU SAE INT PI WARRENDALE PA 400 COMMONWEALTH DR, WARRENDALE, PA 15096 USA SN 2167-4191 EI 2167-4205 J9 SAE INT J ALTERN POW JI SAE Int. J. Altern. Powertrains PD JUL PY 2016 VL 5 IS 2 BP 357 EP 373 DI 10.4271/2016-01-9142 PG 17 WC Transportation Science & Technology SC Transportation GA EA3MU UT WOS:000386507800015 ER PT J AU Elmer, JW Wu, AS AF Elmer, John W. Wu, Amanda S. TI In-Situ Synchrotron and Neutron Radiation Advanced Welding Research SO WELDING JOURNAL LA English DT Editorial Material C1 [Elmer, John W.] Lawrence Livermore Natl Lab, Mat Proc, Livermore, CA 94550 USA. [Wu, Amanda S.] Lawrence Livermore Natl Lab, Mat Engn Div, Livermore, CA USA. RP Elmer, JW (reprint author), Lawrence Livermore Natl Lab, Mat Proc, Livermore, CA 94550 USA. EM elmer1@llnl.gov NR 3 TC 0 Z9 0 U1 2 U2 2 PU AMER WELDING SOC PI MIAMI PA 550 N W LEJEUNE RD, MIAMI, FL 33126 USA SN 0043-2296 J9 WELD J JI Weld. J. PD JUL PY 2016 VL 95 IS 7 BP 53 EP 54 PG 2 WC Metallurgy & Metallurgical Engineering SC Metallurgy & Metallurgical Engineering GA DZ6TS UT WOS:000385995400012 ER PT J AU Gao, JB Nguyen, SC Bronstein, ND Alivisatos, AP AF Gao, Jianbo Nguyen, Son C. Bronstein, Noah D. Alivisatos, A. Paul TI Solution-Processed, High-Speed, and High-Quantum-Efficiency Quantum Dot Infrared Photodetectors SO ACS PHOTONICS LA English DT Article DE quantum dots; photodetector; high speed; quantum efficiency; transport; trap states; multiple trapping and release ID EXPONENTIAL BAND TAILS; TRANSIENT PHOTOCONDUCTIVITY; CHARGE-TRANSPORT; GRAPHENE; SILICON; PBSE; SEMICONDUCTORS; PHOTOCURRENT; SPECTROSCOPY; DYNAMICS AB For over a decade, much effort has been focused on passivation of the high density of localized electronic trap states in colloidal semiconductor quantum dots (QDs), which lead to reduced performance in solar cell, light-emitting diode, laser, and photoconductor applications. However, here we take advantage of the naturally occurring high density of trap states to demonstrate solution-processed high-speed PbSe quantum dot near-infrared photodetectors. Carrier transport dynamics studies reveal multiple trapping and release transport dynamics in band tail states. A sandwich microstrip transmission line photodetector utilizing these QD films was fabricated to achieve high performance by allowing carriers to be swept to the electrodes before they fall into the band tail states. This device demonstrates external quantum efficiency, responsivity, and response time (full width at half-maximum) of 54%, 0.36 A/W, and 74 ps, respectively. C1 [Gao, Jianbo; Nguyen, Son C.; Bronstein, Noah D.; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Gao, Jianbo; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA. [Alivisatos, A. Paul] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Alivisatos, A. Paul] Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USA. [Alivisatos, A. Paul] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. RP Alivisatos, AP (reprint author), Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA.; Alivisatos, AP (reprint author), Univ Calif Berkeley, Dept Mat Sci & Engn, Berkeley, CA 94720 USA.; Alivisatos, AP (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Alivisatos, AP (reprint author), Univ Calif Berkeley, Kavli Energy Nanosci Inst, Berkeley, CA 94720 USA.; Alivisatos, AP (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM paul.alivisatos@berkeley.edu RI Alivisatos , Paul /N-8863-2015 OI Alivisatos , Paul /0000-0001-6895-9048 FU Physical Chemistry of Inorganic Nanostructures Program, Office of Basic Energy Sciences of the United States Department of Energy [KC3103, DE-AC02-05CH11231] FX This work is supported by the Physical Chemistry of Inorganic Nanostructures Program, KC3103, Office of Basic Energy Sciences of the United States Department of Energy, under Contract No. DE-AC02-05CH11231. We would also like to thank Danny Hellebusch for useful discussion. NR 39 TC 4 Z9 4 U1 25 U2 25 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2330-4022 J9 ACS PHOTONICS JI ACS Photonics PD JUL PY 2016 VL 3 IS 7 BP 1217 EP 1222 DI 10.1021/acsphotonics.6b00211 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Optics; Physics, Applied; Physics, Condensed Matter SC Science & Technology - Other Topics; Materials Science; Optics; Physics GA DS0OS UT WOS:000380297200012 ER PT J AU Gao, W Nyein, HYY Shahpar, Z Fahad, HM Chen, K Emaminejad, S Gao, YJ Tai, LC Ota, H Wu, E Bullock, J Zeng, YP Lien, DH Javey, A AF Gao, Wei Nyein, Hnin Y. Y. Shahpar, Ziba Fahad, Hossain M. Chen, Kevin Emaminejad, Sam Gao, Yuji Tai, Li-Chia Ota, Hiroki Wu, Eric Bullock, James Zeng, Yuping Lien, Der-Hsien Javey, Ali TI Wearable Microsensor Array for Multiplexed Heavy Metal Monitoring of Body Fluids SO ACS SENSORS LA English DT Article DE flexible electronics; wearable biosensors; heavy metals monitoring; sweat; multiplexed sensing; temperature compensation ID ANODIC-STRIPPING VOLTAMMETRY; HUMAN SWEAT; ELECTRONIC SKIN; ELECTROCHEMICAL SENSOR; TRACE-METALS; COPPER; MICROELECTRODE; SPECTROMETRY; PERSPIRATION; EXCRETION AB A flexible and wearable microsensor array is described for simultaneous multiplexed monitoring of heavy metals in human body fluids. Zn, Cd, Pb, Cu, and Hg ions are chosen as target analytes for detection via electrochemical square wave anodic stripping voltammetry (SWASV) on Au and Bi microelectrodes. The oxidation peaks of these metals are calibrated and compensated by incorporating a skin temperature sensor. High selectivity, repeatability, and flexibility of the sensor arrays are presented. Human sweat and urine samples are collected for heavy metal analysis, and measured results from the microsensors are validated through inductively coupled plasma mass spectrometry (ICP-MS). Real-time on-body evaluation of heavy metal (e.g., zinc and copper) levels in sweat of human subjects by cycling is performed to examine the change in concentrations with time. This platform is anticipated to provide insightful information about an individual's health state such as heavy metal exposure and aid the related clinical investigations. C1 [Gao, Wei; Nyein, Hnin Y. Y.; Shahpar, Ziba; Fahad, Hossain M.; Chen, Kevin; Emaminejad, Sam; Gao, Yuji; Tai, Li-Chia; Ota, Hiroki; Wu, Eric; Bullock, James; Zeng, Yuping; Lien, Der-Hsien; Javey, Ali] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Gao, Wei; Nyein, Hnin Y. Y.; Shahpar, Ziba; Fahad, Hossain M.; Chen, Kevin; Emaminejad, Sam; Gao, Yuji; Tai, Li-Chia; Ota, Hiroki; Wu, Eric; Bullock, James; Lien, Der-Hsien; Javey, Ali] Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94720 USA. [Gao, Wei; Nyein, Hnin Y. Y.; Chen, Kevin; Emaminejad, Sam; Gao, Yuji; Tai, Li-Chia; Ota, Hiroki; Bullock, James; Lien, Der-Hsien; Javey, Ali] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Javey, A (reprint author), Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA.; Javey, A (reprint author), Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94720 USA.; Javey, A (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM ajavey@berkeley.edu RI Gao, Wei/A-1347-2011 OI Gao, Wei/0000-0002-8503-4562 FU NSF Nanomanufacturing Systems; Office of Science, Office of Basic Energy Sciences, Material Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231]; Robert N. Noyce Fellowship in Microelectronics; Japan Society for the Promotion of Science (JSPS) Fellowship FX This work was supported by NSF Nanomanufacturing Systems for Mobile Computing and Energy Technologies (NASCENT) Center. The sensor fabrication was performed in the Electronic Materials (E-MAT) laboratory funded by the Director, Office of Science, Office of Basic Energy Sciences, Material Sciences and Engineering Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. K.C. acknowledges support from the Robert N. Noyce Fellowship in Microelectronics. H.O. acknowledges support from the Japan Society for the Promotion of Science (JSPS) Fellowship. NR 43 TC 5 Z9 5 U1 36 U2 36 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2379-3694 J9 ACS SENSORS JI ACS Sens. PD JUL PY 2016 VL 1 IS 7 BP 866 EP 874 DI 10.1021/acssensors.6b00287 PG 9 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology SC Chemistry; Science & Technology - Other Topics GA DY9OY UT WOS:000385464900008 ER PT J AU Luo, XY Wu, TP Lu, J Amine, K AF Luo, Xiangyi Wu, Tianpin Lu, Jun Amine, Khalil TI Protocol of Electrochemical Test and Characterization of Aprotic Li-O-2 Battery SO JOVE-JOURNAL OF VISUALIZED EXPERIMENTS LA English DT Article DE Engineering; Issue 113; aprotic Li-O-2 battery; porous cathode; aprotic electrolyte; lithium anode; chemical engineering; electrochemistry; characterization ID LITHIUM-OXYGEN BATTERIES; NONAQUEOUS ELECTROLYTE; AIR BATTERIES; MORPHOLOGY; ANODE; REACTIVITY; DEPOSITION; INSIGHTS; SOLVENT; METAL AB We demonstrate a method for electrochemical testing of an aprotic Li-O-2 battery. An aprotic Li-O-2 battery is made of a Li-metal anode, an aprotic electrolyte, and an O-2-breathing cathode. The aprotic electrolyte is a solution of lithium salt with aprotic solvent; and porous carbon is commonly used as the cathode substrate. To improve the performance, an electrocatalyst is deposited onto the porous carbon substrate by certain deposition methods, such as atomic layer deposition (ALD) and wet-chemistry reaction. The as-prepared cathode materials are characterized by scanning electron microscopy (SEM), transmission electron microscopy (TEM), and X-ray absorption near edge structure (XANES). A Swagelok-type cell, sealed in a glass chamber filled with pure O-2, is used for the electrochemical test on a battery test system. The cells are tested under either capacity-controlled mode or voltage controlled mode. The reaction products are investigated by electron microscopy, X-ray diffraction (XRD), X-ray photoelectron spectroscopy (XPS), attenuated total reflection Fourier transform infrared (ATR-FTIR) spectroscopy, and Raman spectroscopy to study the possible pathway of oxygen reduction reaction (ORR) and oxygen evolution reaction (OER). This protocol demonstrates a systematic and efficient arrangement of routine tests of the aprotic Li-O-2 battery, including the electrochemical test and characterization of battery materials. C1 [Luo, Xiangyi; Lu, Jun; Amine, Khalil] Argonne Natl Lab, Dept Chem Sci & Engn, Argonne, IL 60439 USA. [Wu, Tianpin] Argonne Natl Lab, Adv Photon Sources, Xray Sci Div, Argonne, IL 60439 USA. RP Lu, J; Amine, K (reprint author), Argonne Natl Lab, Dept Chem Sci & Engn, Argonne, IL 60439 USA. EM junlu@anl.gov; amine@anl.gov FU U.S. Department of Energy, FreedomCAR and Vehicle Technologies Office; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-06CH11357] FX Research at Argonne National Laboratory was funded by U.S. Department of Energy, FreedomCAR and Vehicle Technologies Office. Use of the Advanced Photon Source and research carried out in the Electron Microscopy Center at Argonne National Laboratory was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-06CH11357. NR 51 TC 1 Z9 1 U1 5 U2 5 PU JOURNAL OF VISUALIZED EXPERIMENTS PI CAMBRIDGE PA 1 ALEWIFE CENTER, STE 200, CAMBRIDGE, MA 02140 USA SN 1940-087X J9 JOVE-J VIS EXP JI J. Vis. Exp. PD JUL PY 2016 IS 113 AR e53740 DI 10.3791/53740 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DZ1TG UT WOS:000385622600019 ER PT J AU Lozhkin, AV Brown, TA Anderson, PM Glushkova, OY Melekestsev, IV AF Lozhkin, A. V. Brown, T. A. Anderson, P. M. Glushkova, O. Yu. Melekestsev, I. V. TI The Importance of Radiocarbon Dates and Tephra for Developing Chronologies of Holocene Environmental Changes from Lake Sediments, North Far East SO RUSSIAN JOURNAL OF PACIFIC GEOLOGY LA English DT Article DE tephra; chronology; lake sediments; radiocarbon dates; Holocene; Far East of Russia ID CALDERA-FORMING ERUPTION; NORTHEASTERN SIBERIA; RUSSIA; KAMCHATKA; BERINGIA; REGION; ORIGIN; RECORD; ASHES AB Developing continuous chronologies of paleoenvironmental change in northern areas of the Far East using C-14 can be problematic because of the low organic content in lake sediments. However, Holocene age-models can be supplemented by widespread tephra deposits reported in the Magadan region. The best documented of these tephras has been correlated to the KO tephra from southern Kamchatka dated to 7600 BP. Although a key chronostratigraphic marker, no detailed compendium of the distribution of this tephra and its associated 14C dates has been available from sites in the northern Far East. We provide such a summary. Known locally as the Elikchan tephra, lake cores indicate an ash fall that extended similar to 1800 km north of the Kamchatkan caldera with a similar to 500 km wide trajectory in the Magadan region. Other Holocene tephras preserved in lake sediments have poorer age control and possibly date to similar to 2500 BP, similar to 2700 BP and similar to 6000 BP. These ashes seem to be restricted to coastal or near-coastal sites. A single record of a similar to 25,000 BP tephra has also been documented similar to 100 km to the northeast of Magadan. C1 [Lozhkin, A. V.; Glushkova, O. Yu.] Russian Acad Sci, Far East Branch, Northeast Interdisciplinary Sci Res Inst, Magadan 685000, Russia. [Brown, T. A.] Lawrence Livermore Natl Lab, Ctr Accelerator Mass Spectrometry, Livermore, CA 94551 USA. [Anderson, P. M.] Univ Washington, Earth & Space Sci & Quaternary Res Ctr, Seattle, WA 98195 USA. [Melekestsev, I. V.] Russian Acad Sci, Far East Branch, Inst Volcanol & Seismol, Petropavlovsk Kamchatski 683006, Russia. RP Lozhkin, AV (reprint author), Russian Acad Sci, Far East Branch, Northeast Interdisciplinary Sci Res Inst, Magadan 685000, Russia. EM lozhkin@neisri.ru FU US National Science Foundation [ATM-8915415, ATM-9317569, ATM-00-117406]; Far East Branch Russian Academy of Sciences [15-I-2-067]; Russian Foundation for Fundamental Research [15-05-06420]; U.S. Department of Energy by the University of California, Lawrence Livermore National Laboratory [W-7405-Eng-48] FX Field work and core analyses were funded by grants to the US National Science Foundation (ATM-8915415, ATM-9317569, ATM-00-117406), the Far East Branch Russian Academy of Sciences (15-I-2-067) and the Russian Foundation for Fundamental Research (15-05-06420). Part of this work was performed under the auspices of the U.S. Department of Energy by the University of California, Lawrence Livermore National Laboratory under contract no. W-7405-Eng-48. We thank Julya Korzun for help in preparing the figures. NR 38 TC 0 Z9 0 U1 1 U2 1 PU MAIK NAUKA/INTERPERIODICA/SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013-1578 USA SN 1819-7140 EI 1819-7159 J9 RUSS J PAC GEOL JI Russ. J. Pac. Geol. PD JUL PY 2016 VL 10 IS 4 BP 249 EP 262 DI 10.1134/S1819714016040047 PG 14 WC Geosciences, Multidisciplinary SC Geology GA DY7HB UT WOS:000385299200002 ER PT J AU Abbott, BP Abbott, R Abbott, TD Abernathy, MR Acernese, F Ackley, K Adams, C Adams, T Addesso, P Adhikari, RX Adya, VB Affeldt, C Agathos, M Agatsuma, K Aggarwal, N Aguiar, OD Aiello, L Ain, A Ajith, P Allen, B Allocca, A Altin, PA Anderson, SB Anderson, WG Arai, K Araya, MC Arceneaux, CC Areeda, JS Arnaud, N Arun, KG Ascenzi, S Ashton, G Ast, M Aston, SM Astone, P Aufmuth, P Aulbert, C Babak, S Bacon, P Bader, MKM Baker, PT Baldaccini, F Ballardin, G Ballmer, SW Barayoga, JC Barclay, SE Barish, BC Barker, D Barone, F Barr, B Barsotti, L Barsuglia, M Barta, D Barthelmy, S Bartlett, J Bartos, I Bassiri, R Basti, A Batch, JC Baune, C Bavigadda, V Bazzan, M Behnke, B Bejger, M Bell, AS Bell, CJ Berger, BK Bergman, J Bergmann, G Berry, CPL Bersanetti, D Bertolini, A Betzwieser, J Bhagwat, S Bhandare, R Bilenko, IA Billingsley, G Birch, J Birney, R Biscans, S Bisht, A Bitossi, M Biwer, C Bizouard, MA Blackburn, JK Blair, CD Blair, DG Blair, RM Bloemen, S Bock, O Bodiya, TP Boer, M Bogaert, G Bogan, C Bohe, A Bojtos, P Bond, C Bondu, F Bonnand, R Boom, BA Bork, R Boschi, V Bose, S Bouffanais, Y Bozzi, A Bradaschia, C Brady, PR Braginsky, VB Branchesi, M Brau, JE Briant, T Brillet, A Brinkmann, M Brisson, V Brockill, P Brooks, AF Brown, DA Brown, DD Brown, NM Buchanan, CC Buikema, A Bulik, T Bulten, HJ Buonanno, A Buskulic, D Buy, C Byer, RL Cadonati, L Cagnoli, G Cahillane, C Bustillo, JC Callister, T Calloni, E Camp, JB Cannon, KC Cao, J Capano, CD Capocasa, E Carbognani, F Caride, S Diaz, JC Casentini, C Caudill, S Cavaglia, M Cavalier, F Cavalieri, R Cella, G Cepeda, CB Baiardi, LC Cerretani, G Cesarini, E Chakraborty, R Chalermsongsak, T Chamberlin, SJ Chan, M Chao, S Charlton, P Chassande-Mottin, E Chen, HY Chen, Y Cheng, C Chincarini, A Chiummo, A Cho, HS Cho, M Chow, JH Christensen, N Chu, Q Chua, S Chung, S Ciani, G Clara, F Clark, JA Cleva, F Coccia, E Cohadon, PF Colla, A Collette, CG Cominsky, L Constancio, M Conte, A Conti, L Cook, D Corbitt, TR Cornish, N Corsi, A Cortese, S Costa, CA Coughlin, MW Coughlin, SB Coulon, JP Countryman, ST Couvares, P Cowan, EE Coward, DM Cowart, MJ Coyne, DC Coyne, R Craig, K Creighton, JDE Cripe, J Crowder, SG Cumming, A Cunningham, L Cuoco, E Dal Canton, T Danilishin, SL D'Antonio, S Danzmann, K Darman, NS Dattilo, V Dave, I Daveloza, HP Davier, M Davies, GS Daw, EJ Day, R DeBra, D Debreczeni, G Degallaix, J De Laurentis, M Deleglise, S Del Pozzo, W Denker, T Dent, T Dereli, H Dergachev, V DeRosa, RT De Rosa, R DeSalvo, R Dhurandhar, S Diaz, MC Di Fiore, L Di Giovanni, M Di Lieto, A Di Pace, S Di Palma, I Di Virgilio, A Dojcinoski, G Dolique, V Donovan, F Dooley, KL Doravari, S Douglas, R Downes, TP Drago, M Drever, RWP Driggers, JC Du, Z Ducrot, M Dwyer, SE Edo, TB Edwards, MC Effler, A Eggenstein, HB Ehrens, P Eichholz, J Eikenberry, SS Engels, W Essick, RC Etzel, T Evans, M Evans, TM Everett, R Factourovich, M Fafone, V Fair, H Fairhurst, S Fan, X Fang, Q Farinon, S Farr, B Farr, WM Favata, M Fays, M Fehrmann, H Fejer, MM Ferrante, I Ferreira, EC Ferrini, F Fidecaro, F Fiori, I Fiorucci, D Fisher, RP Flaminio, R Fletcher, M Fournier, JD Franco, S Frasca, S Frasconi, F Frei, Z Freise, A Frey, R Frey, V Fricke, TT Fritschel, P Frolov, VV Fulda, P Fyffe, M Gabbard, HAG Gair, JR Gammaitoni, L Gaonkar, SG Garufi, F Gatto, A Gaur, G Gehrels, N Gemme, G Gendre, B Genin, E Gennai, A George, J Gergely, L Germain, V Ghosh, A Ghosh, S Giaime, JA Giardina, KD Giazotto, A Gill, K Glaefke, A Goetz, E Goetz, R Gondan, L Gonzalez, G Castro, JMG Gopakumar, A Gordon, NA Gorodetsky, ML Gossan, SE Gosselin, M Gouaty, R Graef, C Graff, PB Granata, M Grant, A Gras, S Gray, C Greco, G Green, AC Groot, P Grote, H Grunewald, S Guidi, GM Guo, X Gupta, A Gupta, MK Gushwa, KE Gustafson, EK Gustafson, R Hacker, JJ Hall, BR Hall, ED Hammond, G Haney, M Hanke, MM Hanks, J Hanna, C Hannam, MD Hanson, J Hardwick, T Haris, K Harms, J Harry, GM Harry, IW Hart, MJ Hartman, MT Haster, CJ Haughian, K Heidmann, A Heintze, MC Heitmann, H Hello, P Hemming, G Hendry, M Heng, IS Hennig, J Heptonstall, AW Heurs, M Hild, S Hoak, D Hodge, KA Hofman, D Hollitt, SE Holt, K Holz, DE Hopkins, P Hosken, DJ Hough, J Houston, EA Howell, EJ Hu, YM Huang, S Huerta, EA Huet, D Hughey, B Husa, S Huttner, SH Huynh-Dinh, T Idrisy, A Indik, N Ingram, DR Inta, R Isa, HN Isac, JM Isi, M Islas, G Isogai, T Iyer, BR Izumi, K Jacqmin, T Jang, H Jani, K Jaranowski, P Jawahar, S Jimenez-Forteza, F Johnson, WW Jones, DI Jones, R Jonker, RJG Ju, L Kalaghatgi, CV Kalogera, V Kandhasamy, S Kang, G Kanner, JB Karki, S Kasprzack, M Katsavounidis, E Katzman, W Kaufer, S Kaur, T Kawabe, K Kawazoe, F Kefelian, F Kehl, MS Keitel, D Kelley, DB Kells, W Kennedy, R Key, JS Khalaidovski, A Khalili, FY Khan, I Khan, S Khan, Z Khazanov, EA Kijbunchoo, N Kim, C Kim, J Kim, K Kim, N Kim, N Kim, YM King, EJ King, PJ Kinzel, DL Kissel, JS Kleybolte, L Klimenko, S Koehlenbeck, SM Kokeyama, K Koley, S Kondrashov, V Kontos, A Korobko, M Korth, WZ Kowalska, I Kozak, DB Kringel, V Krolak, A Krueger, C Kuehn, G Kumar, P Kuo, L Kutynia, A Lackey, BD Landry, M Lange, J Lantz, B Lasky, PD Lazzarini, A Lazzaro, C Leaci, P Leavey, S Lebigot, EO Lee, CH Lee, HK Lee, HM Lee, K Lenon, A Leonardi, M Leong, JR Leroy, N Letendre, N Levin, Y Levine, BM Li, TGF Libson, A Littenberg, TB Lockerbie, NA Logue, J Lombardi, AL Lord, JE Lorenzini, M Loriette, V Lormand, M Losurdo, G Lough, JD Luck, H Lundgren, P Luo, J Lynch, R Ma, Y MacDonald, T Machenschalk, B MacInnis, M Macleod, DM Magana-Sandoval, F Magee, RM Mageswaran, M Majorana, E Maksimovic, I Malvezzi, V Man, N Mandel, I Mandic, V Mangano, V Mansell, GL Manske, M Mantovani, M Marchesoni, F Marion, F Marka, S Marka, Z Markosyan, AS Maros, E Martelli, F Martellini, L Martin, IW Martin, RM Martynov, DV Marx, JN Mason, K Masserot, A Massinger, TJ Masso-Reid, M Matichard, F Matone, L Mavalvala, N Mazumder, N Mazzolo, G McCarthy, R McClelland, DE McCormick, S McGuire, SC McIntyre, G McIver, J McManus, DJ McWilliams, ST Meacher, D Meadors, GD Meidam, J Melatos, A Mendell, G Mendoza-Gandara, D Mercer, RA Merilh, E Merzougui, M Meshkov, S Messenger, C Messick, C Meyers, PM Mezzani, F Miao, H Michel, C Middleton, H Mikhailov, EE Milano, L Miller, J Millhouse, M Minenkov, Y Ming, J Mirshekari, S Mishra, C Mitra, S Mitrofanov, VP Mitselmakher, G Mittleman, R Moggi, A Mohan, M Mohapatra, SRP Montani, M Moore, BC Moore, CJ Moraru, D Moreno, G Morriss, SR Mossavi, K Mours, B Mow-Lowry, CM Mueller, CL Mueller, G Muir, AW Mukherjee, A Mukherjee, D Mukherjee, S Mukund, N Mullavey, A Munch, J Murphy, DJ Murray, PG Mytidis, A Nardecchia, I Naticchioni, L Nayak, RK Necula, V Nedkova, K Nelemans, G Neri, M Neunzert, A Newton, G Nguyen, TT Nielsen, AB Nissanke, S Nitz, A Nocera, F Nolting, D Normandin, MEN Nuttall, LK Oberling, J Ochsner, E O'Dell, J Oelker, E Ogin, GH Oh, JJ Oh, SH Ohme, F Oliver, M Oppermann, P Oram, RJ O'Reilly, B O'Shaughnessy, R Ottaway, DJ Ottens, RS Overmier, H Owen, BJ Pai, A Pai, SA Palamos, JR Palashov, O Palliyaguru, N Palomba, C Pal-Singh, A Pan, H Pankow, C Pannarale, F Pant, BC Paoletti, F Paoli, A Papa, MA Paris, HR Parker, W Pascucci, D Pasqualetti, A Passaquieti, R Passuello, D Patricelli, B Patrick, Z Pearlstone, BL Pedraza, M Pedurand, R Pekowsky, L Pele, A Penn, S Perreca, A Phelps, M Piccinni, O Pichot, M Piergiovanni, F Pierro, V Pillant, G Pinard, L Pinto, IM Pitkin, M Poggiani, R Popolizio, P Post, A Powell, J Prasad, J Predoi, V Premachandra, SS Prestegard, T Price, LR Prijatelj, M Principe, M Privitera, S Prodi, GA Prokhorov, L Puncken, O Punturo, M Puppo, P Purrer, M Qi, H Qin, J Quetschke, V Quintero, EA Quitzow-James, R Raab, FJ Rabeling, DS Radkins, H Raffai, P Raja, S Rakhmanov, M Rapagnani, P Raymond, V Razzano, M Re, V Read, J Reed, CM Regimbau, T 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J Steinlechner, S Steinmeyer, D Stephens, BC Stone, R Strain, KA Straniero, N Stratta, G Strauss, NA Strigin, S Sturani, R Stuver, AL Summerscales, TZ Sun, L Sutton, PJ Swinkels, BL SzczepaNczyk, MJ Tacca, M Talukder, D Tanner, DB Tpai, M Tarabrin, SP Taracchini, A Taylor, R Theeg, T Thirugnanasambandam, P Thomas, EG Thomas, M Thomas, P Thorne, KA Thorne, KS Thrane, E Tiwari, S Tiwari, V Tokmakov, KV Tomlinson, C Tonelli, M Torres, CV Torrie, CI Tyr, D Travasso, F Traylor, G Trifiro, D Tringali, MC Trozzo, L Tse, M Turconi, M Tuyenbayev, D Ugolini, D Unnikrishnan, CS Urban, AL Usman, SA Vahlbruch, H Vajente, G Valdes, G van Bakel, N van Beuzekom, M van den Brand, JFJ Van den Broeck, C Vander-Hyde, DC van der Schaaf, L van Heijningen, JV van Veggel, AA Vardaro, M Vass, S Vasuth, M Vaulin, R Vecchio, A Vedovato, G Veitch, J Veitch, PJ Venkateswara, K Verkindt, D Vetrano, F Vicere, A Vinciguerra, S Vine, DJ Vinet, JY Vitale, S Vo, T Vocca, H Vorvick, C Voss, D Vousden, WD Vyatchanin, SP 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CA LIGO Sci Collaboration Virgo Colla ASKAP Collaboration BOOTES Collaboration Dark Energy Survey Collaboration Dark Energy Camera GW-EM Collabor Fermi GBM Collaboration FERMI LAT Collaboration GRAvitational Wave Inaf TeAm GRAWI INTEGRAL Collaboration IPTF Collaboration InterPlanetary Network J-GEM Collaboration LA Silla-QUEST Survey Liverpool Telescope Collaboration Low Frequency Array LOFAR Collabo MASTER Collaboration MAXI Collaboration MWA Collaboration Pan-STARRS Collaboration PESSTO Collaboration Pi Sky Collaboration SkyMapper Collaboration Swift Collaboration Tarot Zadko Algerian Natl Observ C TOROS Collaboration VISTA Collaboration TI SUPPLEMENT: "LOCALIZATION AND BROADBAND FOLLOW-UP OF THE GRAVITATIONAL-WAVE TRANSIENT GW150914" (2016, ApJL, 826, L13) SO ASTROPHYSICAL JOURNAL SUPPLEMENT SERIES LA English DT Article DE gravitational waves; methods: observational ID ADVANCED LIGO; ELECTROMAGNETIC COUNTERPARTS; DARK ENERGY; TELESCOPE; MISSION; VIRGO; EVENTS; SEARCH; CAMERA AB This Supplement provides supporting material for Abbott et al. (2016a). We briefly summarize past electromagnetic (EM) follow-up efforts as well as the organization and policy of the current EM follow-up program. We compare the four probability sky maps produced for the gravitational-wave transient GW150914, and provide additional details of the EM follow-up observations that were performed in the different bands. C1 [Abbott, B. P.; Abbott, R.; Abernathy, M. R.; Adhikari, R. X.; Anderson, S. B.; Arai, K.; Araya, M. C.; Barayoga, J. C.; Barish, B. C.; Berger, B. K.; Billingsley, G.; Blackburn, J. K.; Bork, R.; Brooks, A. F.; Cahillane, C.; Callister, T.; Cepeda, C. B.; Chakraborty, R.; Chalermsongsak, T.; Couvares, P.; Coyne, D. C.; Dergachev, V.; Drever, R. W. P.; Ehrens, P.; Etzel, T.; Gossan, S. E.; Gushwa, K. E.; Gustafson, E. K.; Hall, E. D.; Heptonstall, A. W.; Hodge, K. A.; Isi, M.; Kanner, J. B.; Kells, W.; Kondrashov, V.; Korth, W. Z.; Kozak, D. B.; Lazzarini, A.; Li, T. G. F.; Mageswaran, M.; Maros, E.; Martynov, D. V.; Marx, J. 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[Allocca, A.; Basti, A.; Boschi, V.; Cerretani, G.; Di Lieto, A.; Ferrante, I.; Fidecaro, F.; Castro, J. M. G.; Passaquieti, R.; Patricelli, B.; Poggiani, R.; Razzano, M.; Tonelli, M.] Univ Pisa, I-56127 Pisa, Italy. [Allocca, A.; Basti, A.; Boschi, V.; Bradaschia, C.; Cella, G.; Cerretani, G.; Di Lieto, A.; Di Virgilio, A.; Ferrante, I.; Fidecaro, F.; Frasconi, F.; Gennai, A.; Giazotto, A.; Castro, J. M. G.; Moggi, A.; Paoletti, F.; Passaquieti, R.; Passuello, D.; Patricelli, B.; Poggiani, R.; Razzano, M.; Tonelli, M.; Trozzo, L.] Ist Nazl Fis Nucl, Sez Pisa, I-56127 Pisa, Italy. [Altin, P. A.; Chow, J. H.; Mansell, G. L.; McClelland, D. E.; McManus, D. J.; Nguyen, T. T.; Rabeling, D. S.; Scott, S. M.; Shaddock, D. A.; Slagmolen, B. J. J.; Wade, A. R.; Ward, R. L.; Yap, M. J.; Onken, C. A.; Scalzo, R. A.; Schmidt, B. P.; Wolf, C.; Yuan, F.] Australian Natl Univ, GPO Box 4, Canberra, ACT 0200, Australia. [Arceneaux, C. C.; Cavaglia, M.; Dooley, K. L.; Gabbard, H. A. 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[Astone, P.; Colla, A.; Conte, A.; Di Giovanni, M.; Di Pace, S.; Frasca, S.; Leaci, P.; Majorana, E.; Mezzani, F.; Naticchioni, L.; Palomba, C.; Piccinni, O.; Puppo, P.; Rapagnani, P.; Ricci, F.] INFN, Sez Roma, I-00185 Rome, Italy. [Babak, S.; Behnke, B.; Bohe, A.; Buonanno, A.; Di Palma, I.; Grunewald, S.; Harry, I. W.; Leaci, P.; Meadors, G. D.; Ming, J.; Papa, M. A.; Privitera, S.; Puerrer, M.; Raymond, V.; Schutz, B. F.; Singh, A.; Taracchini, A.; Walsh, S.] Max Planck Inst Gravitat Phys, Albert Einstein Inst, D-14476 Potsdam, Germany. [Bacon, P.; Barsuglia, M.; Bouffanais, Y.; Buy, C.; Capocasa, E.; Chassande-Mottin, E.; Fiorucci, D.; Gatto, A.; Lebigot, E. O.; Tacca, M.] Univ Paris Diderot, Sorbonne Paris Cite, Observ Paris, APC,CNRS,IN2P3,CEA,Irfu, F-75205 Paris 13, France. [Baker, P. T.; Cornish, N.; Millhouse, M.] Montana State Univ, Bozeman, MT 59717 USA. [Baldaccini, F.; Gammaitoni, L.; Travasso, F.; Vocca, H.] Univ Perugia, I-06123 Perugia, Italy. 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M.; McCarthy, R.; Mendell, G.; Merilh, E.; Moraru, D.; Moreno, G.; Oberling, J.; Raab, F. J.; Radkins, H.; Reed, C. M.; Ryan, K.; Sadecki, T.; Sandberg, V.; Savage, R. L.; Sevigny, A.; Sigg, D.; Thomas, P.; Vorvick, C.; Warner, J.; Weaver, B.; Worden, J.] LIGO Hanford Observ, Richland, WA 99352 USA. [Barta, D.; Debreczeni, G.; Vasuth, M.] Wigner RCP, RMKI, Konkoly Thege Miklos Ut 29-33, H-1121 Budapest, Hungary. [Barthelmy, S.; Camp, J. B.; Gehrels, N.; Singer, L. P.; Cline, T.; Cenko, S. B.; Marshall, F. E.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Bartos, I.; Countryman, S. T.; Factourovich, M.; Marka, S.; Marka, Z.; Matone, L.; Murphy, D. J.; Staley, A.] Columbia Univ, New York, NY 10027 USA. [Bassiri, R.; Byer, R. L.; DeBra, D.; Fejer, M. M.; Kim, N.; Lantz, B.; MacDonald, T.; Markosyan, A. S.; Paris, H. R.; Patrick, Z.; Shapiro, B.; Wechsler, R. H.] Stanford Univ, Stanford, CA 94305 USA. [Bazzan, M.; Vardaro, M.] Univ Padua, Dipartimento Fis & Astron, I-35131 Padua, Italy. [Bazzan, M.; Conti, L.; Lazzaro, C.; Vardaro, M.; Vedovato, G.; Zangrando, L.; Zendri, J. -P.] INFN, Sez Padova, I-35131 Padua, Italy. [Bejger, M.; Rosinska, D.] CAMK PAN, PL-00716 Warsaw, Poland. [Berry, C. P. L.; Bond, C.; Brown, D. D.; Del Pozzo, W.; Farr, W. M.; Freise, A.; Green, A. C.; Haster, C. -J.; Mandel, I.; Miao, H.; Middleton, H.; Mow-Lowry, C. M.; Thomas, E. G.; Tyr, D.; Vecchio, A.; Veitch, J.; Vinciguerra, S.; Vousden, W. D.; Wang, H.; Wang, M.] Univ Birmingham, Birmingham B15 2TT, W Midlands, England. [Bersanetti, D.; Neri, M.] Univ Genoa, I-16146 Genoa, Italy. [Bersanetti, D.; Chincarini, A.; Farinon, S.; Gemme, G.; Neri, M.; Rei, L.; Sorrentino, F.] INFN, Sez Genova, I-16146 Genoa, Italy. [Bhandare, R.; Dave, I.; George, J.; Pai, S. A.; Pant, B. C.; Raja, S.] RRCAT, Indore 452013, MP, India. [Bilenko, I. A.; Braginsky, V. B.; Gorodetsky, M. L.; Khalili, F. Y.; Mitrofanov, V. P.; Prokhorov, L.; Strigin, S.; Vyatchanin, S. P.] Lomonosov Moscow State Univ, Fac Phys, Moscow 119991, Russia. [Birney, R.; Reid, S.; Vine, D. J.] Univ West Scotland, SUPA, Paisley PA1 2BE, Renfrew, Scotland. [Blair, C. D.; Blair, D. G.; Chu, Q.; Chung, S.; Coward, D. M.; Fang, Q.; Howell, E. J.; Ju, L.; Kaur, T.; Ma, Y.; Qin, J.; Wang, Y.; Wen, L.; Zhao, C.; Zhu, X. J.] Univ Western Australia, Crawley, WA 6009, Australia. [Bloemen, S.; Ghosh, S.; Groot, P.; Nelemans, G.; Nissanke, S.; Setyawati, Y.; Shah, S.; Jonker, P. G.] Radboud Univ Nijmegen, IMAPP, Dept Astrophys, POB 9010, NL-6500 GL Nijmegen, Netherlands. [Boer, M.; Bogaert, G.; Brillet, A.; Cleva, F.; Coulon, J. -P.; Dereli, H.; Fournier, J. -D.; Gendre, B.; Heitmann, H.; Kefelian, F.; Man, N.; Martellini, L.; Merzougui, M.; Pichot, M.; Regimbau, T.; Siellez, K.; Turconi, M.; Vinet, J. -Y.; Wei, L. -W.; Laugier, R.] Univ Cote dAzur, CNRS, Observ Cote dAzur, Artemis, CS 34229, Nice 4, France. [Bojtos, P.; Frei, Z.; Gondan, L.; Raffai, P.] MTA Eotvos Univ, Lendulet Astrophys Res Grp, H-1117 Budapest, Hungary. [Bondu, F.] Univ Rennes 1, CNRS, Inst Phys Rennes, F-35042 Rennes, France. [Bose, S.; Hall, B. R.; Magee, R. M.; Mazumder, N.] Washington State Univ, Pullman, WA 99164 USA. [Branchesi, M.; Baiardi, L. C.; Greco, G.; Guidi, G. M.; Harms, J.; Martelli, F.; Montani, M.; Piergiovanni, F.; Stratta, G.; Vetrano, F.; Vicere, A.] Univ Urbino Carlo Bo, I-61029 Urbino, Italy. [Branchesi, M.; Baiardi, L. C.; Greco, G.; Guidi, G. M.; Harms, J.; Losurdo, G.; Martelli, F.; Montani, M.; Piergiovanni, F.; Stratta, G.; Vetrano, F.; Vicere, A.] INFN, Sez Firenze, I-50019 Florence, Italy. [Brau, J. E.; Frey, R.; Karki, S.; Palamos, J. R.; Quitzow-James, R.; Roma, V. J.; Schale, P.; Schofield, R. M. S.; Talukder, D.] Univ Oregon, Eugene, OR 97403 USA. 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EM lsc-spokesperson@ligo.org RI Prokhorov, Leonid/I-2953-2012; Gammaitoni, Luca/B-5375-2009; Ciani, Giacomo/G-1036-2011; Sigg, Daniel/I-4308-2015; Di Virgilio, Angela Dora Vittoria/E-9078-2015; Garufi, Fabio/K-3263-2015; Sergeev, Alexander/F-3027-2017; Vitek, Stanislav/B-3332-2015; Harms, Jan/J-4359-2012; Jelinek, Martin/E-5290-2016; Marchesoni, Fabio/A-1920-2008; Cesarini, Elisabetta/C-4507-2017; Costa, Cesar/G-7588-2012; Hild, Stefan/A-3864-2010; Roberts, Oliver/N-6284-2016; Mihara, Tatehiro/C-5536-2017; Di Venere, Leonardo/C-7619-2017; Chow, Jong/A-3183-2008; Hudec, Rene/G-9018-2014; Frey, Raymond/E-2830-2016; Serino, Motoko/D-3890-2017; Caballero-Garcia, Maria/D-5659-2017; Bartos, Imre/A-2592-2017; Punturo, Michele/I-3995-2012; Gaztanaga, Enrique/L-4894-2014; zhou, hua/A-6862-2017; Cella, Giancarlo/A-9946-2012; prodi, giovanni/B-4398-2010; Ogando, Ricardo/A-1747-2010; Leonardi, Matteo/G-9694-2015; Galbany, Lluis/A-8963-2017; Elias-Rosa, Nancy/D-3759-2014; Reimer, Olaf/A-3117-2013; 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Gaztanaga, Enrique/0000-0001-9632-0815; Cella, Giancarlo/0000-0002-0752-0338; prodi, giovanni/0000-0001-5256-915X; Ogando, Ricardo/0000-0003-2120-1154; Galbany, Lluis/0000-0002-1296-6887; Elias-Rosa, Nancy/0000-0002-1381-9125; Reimer, Olaf/0000-0001-6953-1385; Ferrante, Isidoro/0000-0002-0083-7228; Pata, Petr/0000-0002-6561-9088; Gemme, Gianluca/0000-0002-1127-7406; Vecchio, Alberto/0000-0002-6254-1617; Losurdo, Giovanni/0000-0003-0452-746X; Iyer, Bala R./0000-0002-4141-5179; Sorrentino, Fiodor/0000-0002-9605-9829; Wayth, Randall/0000-0002-6995-4131; Travasso, Flavio/0000-0002-4653-6156; Tiwari, Shubhanshu/0000-0003-1611-6625; Funk, Stefan/0000-0002-2012-0080 FU United States National Science Foundation (NSF); Science and Technology Facilities Council (STFC) of the United Kingdom; Max-Planck Society; State of Niedersachsen/Germany; Australian Research Council; Netherlands Organisation for Scientific Research; EGO consortium; Council of Scientific and Industrial Research of India; Department of Science and Technology, India; Science & Engineering Research Board (SERB), India; Ministry of Human Resource Development, India; Spanish Ministerio de Economia y Competitividad; Conselleria d'Economia i Competitivitat and Conselleria d'Educacio Cultura i Universitats of the Govern de les Illes Balears; National Science Centre of Poland; European Commission; Royal Society; Scottish Funding Council; Scottish Universities Physics Alliance; Hungarian Scientific Research Fund (OTKA); Lyon Institute of Origins (LIO); National Research Foundation of Korea; Industry Canada; Province of Ontario through Ministry of Economic Development and Innovation; National Science and Engineering Research Council Canada; Canadian Institute for Advanced Research; Brazilian Ministry of Science, Technology, and Innovation; Russian Foundation for Basic Research; Leverhulme Trust; Research Corporation; Ministry of Science and Technology (MOST), Taiwan; Kavli Foundation; Australian Government; National Collaborative Research Infrastructure Strategy; Government of Western Australia; United States Department of Energy; United States National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Center for Cosmology and Astro-Particle Physics at the Ohio State University; Mitchell Institute for Fundamental Physics and Astronomy at Texas AM University; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia, Tecnologia e Inovacao; Deutsche Forschungsgemeinschaft; Collaborating Institutions in the Dark Energy Survey; National Science Foundation [AST-1138766, AST-1238877]; MINECO [AYA2012-39559, ESP2013-48274, FPA2013-47986]; Centro de Excelencia Severo Ochoa [SEV-2012-0234]; European Research Council under European Union's Seventh Framework Programme; ERC [240672, 291329, 306478]; NASA (United States); DOE (United States); IN2P3/CNRS (France); CEA/Irfu (France); ASI (Italy); INFN (Italy); MEXT (Japan); KEK (Japan); JAXA (Japan); Wallenberg Foundation; Swedish Research Council; National Space Board (Sweden); NASA in the United States; DRL in Germany; INAF for the project "Gravitational Wave Astronomy with the first detections of adLIGO and adVIRGO experiments"; ESA (Denmark); ESA (France); ESA (Germany); ESA (Italy); ESA (Switzerland); ESA (Spain); German INTEGRAL through DLR grant [50 OG 1101]; US under NASA Grant [NNX15AU74G]; National Science Foundation PIRE program grant [1545949]; Hubble Fellowship [HST-HF-51325.01]; KAKENHI of MEXT Japan [24103003, 15H00774, 15H00788]; JSPS [15H02069, 15H02075]; "Optical and Near-Infrared Astronomy Inter-University Cooperation Program" - MEXT; UK Science and Technology Facilities Council; ERC Advanced Investigator Grant [267697]; Lomonosov Moscow State University Development programm; Moscow Union OPTICA; Russian Science Foundation [16-12-00085, RFBR15-02-07875]; National Research Foundation of South Africa; Australian Government Department of Industry and Science and Department of Education (National Collaborative Research Infrastructure Strategy: NCRIS); NVIDIA at Harvard University; University of Hawaii; National Aeronautics and Space Administration's Planetary Defense Office [NNX14AM74G]; Queen's University Belfast; National Aeronautics and Space Administration through Planetary Science Division of the NASA Science Mission Directorate [NNX08AR22G]; European Research Council under European Union's Seventh Framework Programme/ERC [291222]; STFC grants [ST/I001123/1, ST/L000709/1]; European Union FP7 programme through ERC [320360]; STFC through an Ernest Rutherford Fellowship; FONDECYT [3140326]; Australian Research Council Centre of Excellence for All-sky Astrophysics (CAASTRO) [CE110001020]; NASA in the US; UK Space Agency in the UK; Agenzia Spaziale Italiana (ASI) in Italy; Ministerio de Ciencia y Tecnologia (MinCyT); Consejo Nacional de Investigaciones Cientificas y Tecnologicas (CONICET) from Argentina; USA NSF PHYS [1156600]; NSF [1242090] FX The authors gratefully acknowledge the support of the United States National Science Foundation (NSF) for the construction and operation of the LIGO Laboratory and Advanced LIGO as well as the Science and Technology Facilities Council (STFC) of the United Kingdom, the Max-Planck Society (MPS), and the State of Niedersachsen/Germany for support of the construction of Advanced LIGO and construction and operation of the GEO 600 detector. Additional support for Advanced LIGO was provided by the Australian Research Council. The authors gratefully acknowledge the Italian Istituto Nazionale di Fisica Nucleare (INFN), the French Centre National de la Recherche Scientifique (CNRS), and the Foundation for Fundamental Research on Matter supported by the Netherlands Organisation for Scientific Research, for the construction and operation of the Virgo detector, and the creation and support of the EGO consortium. The authors also gratefully acknowledge research support from these agencies as well as by the Council of Scientific and Industrial Research of India, Department of Science and Technology, India, Science & Engineering Research Board (SERB), India, Ministry of Human Resource Development, India, the Spanish Ministerio de Economia y Competitividad, the Conselleria d'Economia i Competitivitat and Conselleria d'Educacio Cultura i Universitats of the Govern de les Illes Balears, the National Science Centre of Poland, the European Commission, the Royal Society, the Scottish Funding Council, the Scottish Universities Physics Alliance, the Hungarian Scientific Research Fund (OTKA), the Lyon Institute of Origins (LIO), the National Research Foundation of Korea, Industry Canada and the Province of Ontario through the Ministry of Economic Development and Innovation, the National Science and Engineering Research Council Canada, Canadian Institute for Advanced Research, the Brazilian Ministry of Science, Technology, and Innovation, Russian Foundation for Basic Research, the Leverhulme Trust, the Research Corporation, Ministry of Science and Technology (MOST), Taiwan, and the Kavli Foundation. The authors gratefully acknowledge the support of the NSF, STFC, MPS, INFN, CNRS, and the State of Niedersachsen/Germany for provision of computational resources.; The Australian SKA Pathfinder is part of the Australia Telescope National Facility which is managed by CSIRO. The operation of ASKAP is funded by the Australian Government with support from the National Collaborative Research Infrastructure Strategy. Establishment of the Murchison Radio-astronomy Observatory was funded by the Australian Government and the Government of Western Australia. ASKAP uses advanced supercomputing resources at the Pawsey Supercomputing Centre. We acknowledge the Wajarri Yamatji people as the traditional owners of the Observatory site.; A.J.C.T. acknowledges support from the Junta de Andalucia (Project P07-TIC-03094) and Univ. of Auckland and NIWA for installing of the Spanish BOOTES-3 station in New Zealand, and support from the Spanish Ministry Projects AYA2012-39727-C03-01 and 2015-71718R.; Funding for the DES Projects has been provided by the United States Department of Energy, the United States National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana-Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, the Center for Cosmology and Astro-Particle Physics at the Ohio State University, the Mitchell Institute for Fundamental Physics and Astronomy at Texas A&M University, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia, Tecnologia e Inovacao, the Deutsche Forschungsgemeinschaft, and the Collaborating Institutions in the Dark Energy Survey.; The DES data management system is supported by the National Science Foundation under Grant Number AST-1138766. The DES participants from Spanish institutions are partially supported by MINECO under grants AYA2012-39559, ESP2013-48274, FPA2013-47986, and Centro de Excelencia Severo Ochoa SEV-2012-0234. Research leading to these results has received funding from the European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013) including ERC grant agreements 240672, 291329, and 306478.; The Fermi LAT Collaboration acknowledges support for LAT development, operation, and data analysis from NASA and DOE (United States), CEA/Irfu and IN2P3/CNRS (France), ASI and INFN (Italy), MEXT, KEK, and JAXA (Japan), and the K.A. Wallenberg Foundation, the Swedish Research Council and the National Space Board (Sweden). Science analysis support in the operations phase from INAF (Italy) and CNES (France) is also gratefully acknowledged. The Fermi GBM Collaboration acknowledges the support of NASA in the United States and DRL in Germany.; GRAWITA acknowledges the support of INAF for the project "Gravitational Wave Astronomy with the first detections of adLIGO and adVIRGO experiments."; This work exploited data by INTEGRAL, an ESA project with instruments and science data center funded by ESA member states (especially the PI countries: Denmark, France, Germany, Italy, Switzerland, Spain), and with the participation of Russia and the USA. The SPI ACS detector system has been provided by MPE Garching/Germany. We acknowledge the German INTEGRAL support through DLR grant 50 OG 1101.; IPN work is supported in the US under NASA Grant ;NNX15AU74G.; This work is partly based on observations obtained with the Samuel Oschin 48 in Telescope and the 60 in Telescope at the Palomar Observatory as part of the Intermediate Palomar Transient Factory (iPTF) project, a scientific collaboration among the California Institute of Technology, Los Alamos National Laboratory, the University of Wisconsin, Milwaukee, the Oskar Klein Center, the Weizmann Institute of Science, the TANGO Program of the University System of Taiwan, and the Kavli Institute for the Physics and Mathematics of the universe. M.M.K. and Y.C. acknowledge funding from the National Science Foundation PIRE program grant 1545949. A.A.M. acknowledges support from the Hubble Fellowship HST-HF-51325.01. Part of the research was carried out at the Jet Propulsion Laboratory, California Institute of Technology, under a contract with NASA.; J-GEM is financially supported by KAKENHI Grant No. 24103003, 15H00774, and 15H00788 of MEXT Japan, 15H02069 and 15H02075 of JSPS, and the "Optical and Near-Infrared Astronomy Inter-University Cooperation Program" supported by MEXT.; The Liverpool Telescope is operated on the island of La Palma by Liverpool John Moores University in the Spanish Observatorio del Roque de los Muchachos of the Instituto de Astrofisica de Canarias with financial support from the UK Science and Technology Facilities Council.; LOFAR, the Low Frequency Array designed and constructed by ASTRON, has facilities in several countries, which are owned by various parties (each with their own funding sources), and that are collectively operated by the International LOFAR Telescope (ILT) foundation under a joint scientific policy. R. Fender acknowledges support from ERC Advanced Investigator Grant 267697.; MASTER Global Robotic Net is supported in parts by Lomonosov Moscow State University Development programm, Moscow Union OPTICA, Russian Science Foundation 16-12-00085, RFBR15-02-07875, National Research Foundation of South Africa.; We thank JAXA and RIKEN for providing MAXI data. The MAXI team is partially supported by KAKENHI grant Nos. 24103002, 24540239, 24740186, and 23000004 of MEXT, Japan.; This work uses the Murchison Radio-astronomy Observatory, operated by CSIRO. We acknowledge the Wajarri Yamatji people as the traditional owners of the observatory site. Support for the operation of the MWA is provided by the Australian Government Department of Industry and Science and Department of Education (National Collaborative Research Infrastructure Strategy: NCRIS), under a contract to Curtin University administered by Astronomy Australia Limited. The MWA acknowledges the iVEC Petabyte Data Store and the Initiative in Innovative Computing and the CUDA Center for Excellence sponsored by NVIDIA at Harvard University.; Pan-STARRS is supported by the University of Hawaii and the National Aeronautics and Space Administration's Planetary Defense Office under grant No. NNX14AM74G. The PanSTARRS-LIGO effort is in collaboration with the LIGO Consortium and supported by Queen's University Belfast. The Pan-STARRS1 Sky Surveys have been made possible through contributions by the Institute for Astronomy, the University of Hawaii, the Pan-STARRS Project Office, the Max Planck Society and its participating institutes, the Max Planck Institute for Astronomy, Heidelberg, and the Max Planck Institute for Extraterrestrial Physics, Garching, The Johns Hopkins University, Durham University, the University of Edinburgh, the Queen's University Belfast, the Harvard-Smithsonian Center for Astrophysics, the Las Cumbres Observatory Global Telescope Network Incorporated, the National Central University of Taiwan, the Space Telescope Science Institute, and the National Aeronautics and Space Administration under grant No. NNX08AR22G issued through the Planetary Science Division of the NASA Science Mission Directorate, the National Science Foundation grant No. AST-1238877, the University of Maryland, Eotvos Lorand University (ELTE), and the Los Alamos National Laboratory. This work is based (in part) on observations collected at the European Organisation for Astronomical Research in the Southern Hemisphere, Chile as part of PESSTO, (the Public ESO Spectroscopic Survey for Transient Objects Survey) ESO programs 188.D-3003, 191.D-0935.; S.J.S. acknowledges funding from the European Research Council under the European Union's Seventh Framework Programme (FP7/2007-2013)/ERC Grant agreement No. [291222] and STFC grants ST/I001123/1 and ST/L000709/1. M.F. is supported by the European Union FP7 programme through ERC grant No. 320360. K.M. acknowledges support from the STFC through an Ernest Rutherford Fellowship.; F.O.E. acknowledges support from FONDECYT through postdoctoral grant 3140326.; Parts of this research were conducted by the Australian Research Council Centre of Excellence for All-sky Astrophysics (CAASTRO), through project No. CE110001020.; Funding for Swift is provided by NASA in the US, by the UK Space Agency in the UK, and by the Agenzia Spaziale Italiana (ASI) in Italy. This work made use of data supplied by the UK Swift Science Data Centre at the University of Leicester. We acknowledge the use of public data from the Swift data archive.; The TOROS Collaboration acknowledges support from Ministerio de Ciencia y Tecnologia (MinCyT) and Consejo Nacional de Investigaciones Cientificas y Tecnologicas (CONICET) from Argentina and grants from the USA NSF PHYS 1156600 and NSF HRD 1242090. NR 51 TC 8 Z9 8 U1 68 U2 68 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0067-0049 EI 1538-4365 J9 ASTROPHYS J SUPPL S JI Astrophys. J. Suppl. Ser. PD JUL PY 2016 VL 225 IS 1 AR 8 DI 10.3847/0067-0049/225/1/8 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DU6FG UT WOS:000382309000008 ER PT J AU Cui, S He, LP Hong, XC Zhu, XD Petrovic, C Li, SY AF Cui, Shan He, Lan-Po Hong, Xiao-Chen Zhu, Xiang-De Petrovic, Cedomir Li, Shi-Yan TI Multiband nodeless superconductivity near the charge-density-wave quantum critical point in ZrTe3-xSex SO CHINESE PHYSICS B LA English DT Article DE superconductivity; charge-density-wave order; thermal transport measurement; gap structure ID SUPERLATTICES AB It was found that selenium doping can suppress the charge-density-wave (CDW) order and induce bulk superconductivity in ZrTe3. The observed superconducting dome suggests the existence of a CDW quantum critical point (QCP) in ZrTe3-xSex near x approximate to 0.04. To elucidate the superconducting state near the CDW QCP, we measure the thermal conductivity of two ZrTe3-xSex single crystals (x = 0.044 and 0.051) down to 80 mK. For both samples, the residual linear term kappa(0)/T at zero field is negligible, which is a clear evidence for nodeless superconducting gap. Furthermore, the field dependence of kappa(0)/T manifests a multigap behavior. These results demonstrate multiple nodeless superconducting gaps in ZrTe3-xSex, which indicates conventional superconductivity despite of the existence of a CDW QCP. C1 [Cui, Shan; He, Lan-Po; Hong, Xiao-Chen; Li, Shi-Yan] Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Cui, Shan; He, Lan-Po; Hong, Xiao-Chen; Li, Shi-Yan] Fudan Univ, Adv Mat Lab, Shanghai 200433, Peoples R China. [Zhu, Xiang-De] Chinese Acad Sci, High Field Magnet Lab, Hefei 230031, Peoples R China. [Zhu, Xiang-De] Univ Sci & Technol China, Hefei 230031, Peoples R China. [Li, Shi-Yan] Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China. [Zhu, Xiang-De; Petrovic, Cedomir] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA. RP Li, SY (reprint author), Fudan Univ, Dept Phys, State Key Lab Surface Phys, Shanghai 200433, Peoples R China.; Li, SY (reprint author), Fudan Univ, Adv Mat Lab, Shanghai 200433, Peoples R China.; Li, SY (reprint author), Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China. EM shiyan_li@fudan.edu.cn FU National Basic Research Program of China [2012CB821402, 2015CB921401]; National Natural Science Foundation of China [91421101, 11422429, 11204312]; Program for Professor of Special Appointment (Eastern Scholar) at Shanghai Institutions of Higher Learning, China; STCSM of China [15XD1500200]; US DOE [DESC00112704] FX Project supported by the National Basic Research Program of China (Grant Nos. 2012CB821402 and 2015CB921401), the National Natural Science Foundation of China (Grant Nos. 91421101, 11422429, and 11204312), the Program for Professor of Special Appointment (Eastern Scholar) at Shanghai Institutions of Higher Learning, China, and STCSM of China (Grant No. 15XD1500200). Work at Brookhaven National Laboratory was supported by the US DOE under Contract No. DESC00112704. NR 23 TC 0 Z9 0 U1 12 U2 12 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1674-1056 EI 1741-4199 J9 CHINESE PHYS B JI Chin. Phys. B PD JUL PY 2016 VL 25 IS 7 AR 077403 DI 10.1088/1674-1056/25/7/077403 PG 4 WC Physics, Multidisciplinary SC Physics GA DX2UD UT WOS:000384225800058 ER PT J AU Sheffield, J Spong, DA AF Sheffield, John Spong, Donald A. TI Catalyzed D-D Stellarator Reactor SO FUSION SCIENCE AND TECHNOLOGY LA English DT Article DE Stellarator reactor; catalyzed D-D ID POWER-PLANTS; FUSION; SYSTEMS; PLASMAS AB The advantages of using the catalyzed deuterium-deuterium (D-D) approach for a fusion reactor-lower and less energetic neutron flux and no need for a tritium breeding blanket-have been evaluated in previous papers, giving examples of both tokamak and stellarator reactors. This paper presents an update for the stellarator example, taking account of more recent empirical transport scaling results and design studies of lower-aspect-ratio stellarators. We use a modified version of the Generic Magnetic Fusion Reactor model to cost a stellarator-type reactor. Recently, this model has been updated to reflect the improved science and technology base and costs in the magnetic fusion program. It is shown that an interesting catalyzed D-D, stellarator power plant might be possible if the following parameters could be achieved: R/< a > approximate to 4, required improvement factor to ISS04 scaling, F-R = 0.9 to 1.15, approximate to 8.0% to 11.5%, Z(eff) approximate to 1.45 plus a relativistic temperature correction, fraction of fast ions lost approximate to 0.07, B-m approximate to 14 to 16 T, and R approximate to 18 to 24 m. C1 [Sheffield, John] 1070 Rome Dr, Roswell, GA 30075 USA. [Spong, Donald A.] Oak Ridge Natl Lab, Fus Mat & Nucl Sci Div, One Bethel Valley Rd, Oak Ridge, TN 37831 USA. RP Sheffield, J (reprint author), 1070 Rome Dr, Roswell, GA 30075 USA. EM john.sheffield@aol.com FU U.S. Department of Energy, Office of Science [DE-AC05-00OR22725]; UT-Battelle, LLC; UT-Battelle [4000126754]; University of Tennessee [4000126754] FX We appreciate the valuable input of A. Dinklage and N. Uckan and that of the two reviewers who gave crucial advice on improving the accuracy and logic of the paper. The work of D. A. S. has been supported by the U.S. Department of Energy, Office of Science, under contract DE-AC05-00OR22725 with UT-Battelle, LLC. The work of J. S. was covered in part under contract 4000126754 between UT-Battelle and the University of Tennessee. NR 21 TC 0 Z9 0 U1 1 U2 1 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 1536-1055 EI 1943-7641 J9 FUSION SCI TECHNOL JI Fusion Sci. Technol. PD JUL PY 2016 VL 70 IS 1 BP 36 EP 53 DI 10.13182/FST15-161 PG 18 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DY2OT UT WOS:000384932600003 ER PT J AU G-Michael, T Marchand, B Tucker, JD Marston, TM Sternlicht, DD Azimi-Sadjadi, MR AF G-Michael, Tesfaye Marchand, Bradley Tucker, J. Derek Marston, Timothy M. Sternlicht, Daniel D. Azimi-Sadjadi, Mahmood R. TI Image-Based Automated Change Detection for Synthetic Aperture Sonar by Multistage Coregistration and Canonical Correlation Analysis SO IEEE JOURNAL OF OCEANIC ENGINEERING LA English DT Article DE Automated change detection; canonical correlation analysis (CCA); coherent change detection; coregistration; synthetic aperture sonar (SAS) ID SEA-FLOOR ROUGHNESS; SAR DATA; PHASE AB In this paper, an automated change detection technique is presented that compares new and historical seafloor images created with sidescan synthetic aperture sonar ( SAS) for changes occurring over time. The method consists of a four-stage process: a coarse navigational alignment that relates and approximates pixel locations of reference and repeat-pass data sets; fine-scale coregistration using the scale-invariant feature transform ( SIFT) algorithm to match features between overlapping data sets; local coregistration that improves phase coherence; and finally, change detection utilizing a canonical correlation analysis (CCA) algorithm to detect changes. The method was tested using data collected with a high-frequency SAS in a sandy shallow-water environment. Successful results of this multistage change detection method are presented here, and the robustness of the techniques that exploit phase and amplitude levels of the backscattered signals is discussed. It is shown that the coherent nature of the SAS data can be exploited and utilized in this environment over time scales ranging from hours through several days. Robustness of the coregistration methods and analysis of scene coherence over time is characterized by analysis of repeat pass as well as synthetically modified data sets. C1 [G-Michael, Tesfaye; Marchand, Bradley; Sternlicht, Daniel D.] Naval Surface Warfare Ctr, Panama City Div, Panama City, FL 32407 USA. [Tucker, J. Derek] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Marston, Timothy M.] Univ Washington, Appl Phys Lab, Seattle, WA 98105 USA. [Azimi-Sadjadi, Mahmood R.] Colorado State Univ, Elect & Comp Engn Dept, Ft Collins, CO 80523 USA. RP G-Michael, T (reprint author), Naval Surface Warfare Ctr, Panama City Div, Panama City, FL 32407 USA. EM tesfaye.g-michael@navy.mil; bradley.marchand@navy.mil; jdtuck@sandia.gov; marston@apl.washington.edu; daniel.sternlicht@navy.mil; azimi@engr.colostate.edu FU U.S. Office of Naval Research (ONR) FX This work was supported by the U.S. Office of Naval Research (ONR). NR 44 TC 1 Z9 1 U1 5 U2 5 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0364-9059 EI 1558-1691 J9 IEEE J OCEANIC ENG JI IEEE J. Ocean. Eng. PD JUL PY 2016 VL 41 IS 3 BP 592 EP 612 DI 10.1109/JOE.2015.2465631 PG 21 WC Engineering, Civil; Engineering, Ocean; Engineering, Electrical & Electronic; Oceanography SC Engineering; Oceanography GA DY1GB UT WOS:000384841800010 ER PT J AU Bryner, D Huffer, F Srivastava, A Tucker, JD AF Bryner, Darshan Huffer, Fred Srivastava, Anuj Tucker, J. Derek TI Underwater Minefield Detection in Clutter Data Using Spatial Point-Process Models SO IEEE JOURNAL OF OCEANIC ENGINEERING LA English DT Article DE Maximum-likelihood estimation; simulated annealing; spatial point process; synthetic aperture sonar; Thomas process ID 2-STEP ESTIMATION; STATISTICS; INFERENCE AB In this paper, we study the problem of detection of underwater minefields amidst dense clutter as that of statistical inference under a spatial point-process model. Specifically, we model the locations ( mine and clutter) as samples of a Thomas point process with parent locations representing mines and children representing clutter. Accordingly, the parents are distributed according to a homogeneous Poisson process and, given the parent locations, the children are distributed as independent Poisson processes with intensity functions that are Gaussian densities centered at the parents. This provides a likelihood function for parent locations given the observed clutter ( children). Under this model, we develop a framework for penalized maximum-likelihood (ML) estimation of model parameters and parent locations. The optimization is performed using a combination of analytical and Monte Carlo methods; the Monte Carlo part relies on a birth-death-move procedure for adding/removing points in the parent set. This framework is illustrated using both simulated and real data sets, the latter obtained courtesy of Naval Surface Warfare Center Panama City Division (NSWC-PCD), Panama City, FL, USA. The results, evaluated both qualitatively and quantitatively, underscore success in estimating parent locations and other parameters, at a reasonable computation cost. C1 [Bryner, Darshan] NSWC, PCD, Panama City, FL 32407 USA. [Huffer, Fred; Srivastava, Anuj] Florida State Univ, Dept Stat, Tallahassee, FL 32306 USA. [Tucker, J. Derek] Sandia Natl Labs, Albuquerque, NM 87015 USA. RP Bryner, D (reprint author), NSWC, PCD, Panama City, FL 32407 USA. EM dar-shan.bryner@navy.mil; huffer@stat.fsu.edu; anuj@stat.fsu.edu; jdtuck@sandia.gov FU U.S. Office of Naval Research (ONR) FX This work was supported by the U.S. Office of Naval Research (ONR). This work is approved for public release; distribution is unlimited. NR 29 TC 0 Z9 0 U1 1 U2 1 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0364-9059 EI 1558-1691 J9 IEEE J OCEANIC ENG JI IEEE J. Ocean. Eng. PD JUL PY 2016 VL 41 IS 3 BP 670 EP 681 DI 10.1109/JOE.2015.2493598 PG 12 WC Engineering, Civil; Engineering, Ocean; Engineering, Electrical & Electronic; Oceanography SC Engineering; Oceanography GA DY1GB UT WOS:000384841800015 ER PT J AU Grant, RE Gavrilovska, A AF Grant, Ryan E. Gavrilovska, Ada TI HOT INTERCONNECTS 23 Introduction SO IEEE MICRO LA English DT Editorial Material C1 [Grant, Ryan E.] Sandia Natl Labs, Ctr Computat Res, Livermore, CA 94550 USA. [Gavrilovska, Ada] Georgia Tech, Coll Comp, Atlanta, GA USA. RP Grant, RE (reprint author), Sandia Natl Labs, Ctr Computat Res, Livermore, CA 94550 USA. EM regrant@sandia.gov; ada@cc.gatech.edu NR 4 TC 0 Z9 0 U1 0 U2 0 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 0272-1732 EI 1937-4143 J9 IEEE MICRO JI IEEE Micro PD JUL-AUG PY 2016 VL 36 IS 4 BP 4 EP 5 PG 2 WC Computer Science, Hardware & Architecture; Computer Science, Software Engineering SC Computer Science GA DY2FS UT WOS:000384909100002 ER PT J AU Kim, B Hong, S Ahn, G No, K AF Kim, Bongsoo Hong, Seungbum Ahn, Gun No, Kwangsoo TI Synthesis of Ferroelectric Lead Titanate Nanohoneycomb Arrays via Lead Supplement Process SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY LA English DT Article DE nanohoneycomb; lead supplement process; ferroelectricity/ferroelectric materials; lead titanate; nanomaterials; piezoelectric materials/properties ID FABRICATION; PBTIO3; COMPOSITES; MICROSCOPY; NANOTUBES; GROWTH; FILMS AB Here, we demonstrate a novel process to convert TiO2 nanotubes into ferroelectric nanohoneycombs, comprised of vertically aligned PbTiO3 nanotubes. Tube bottom opening process enabled effective infiltration of lead acetate precursor into the nanotubes. Nanohoneycombs, which were converted via additional lead supplement process, showed uniform conversion and well-defined ferroelectric properties with the effective piezoelectric coefficient of approximately 20 pm/V, which was measured by piezoresponse force microscopy. C1 [Kim, Bongsoo; Hong, Seungbum; Ahn, Gun; No, Kwangsoo] Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea. [Hong, Seungbum] Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. RP Hong, S; No, K (reprint author), Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Taejon 305701, South Korea.; Hong, S (reprint author), Argonne Natl Lab, Div Mat Sci, Lemont, IL 60439 USA. EM hong@anl.gov; ksno@kaist.ac.kr RI Hong, Seungbum/B-7708-2009; No, Kwangsoo/C-1983-2011 OI Hong, Seungbum/0000-0002-2667-1983; FU Mid-career Researcher Program through the National Research Foundation of Korea - Ministry of Education, Science and Technology [2010-0015063]; U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division FX This research was supported by the Mid-career Researcher Program (2010-0015063) through the National Research Foundation of Korea funded by Ministry of Education, Science and Technology. Work at Argonne National Laboratory (S. H., data analysis and writing of manuscript) was supported by the U.S. Department of Energy, Office of Science, Materials Sciences and Engineering Division. NR 26 TC 0 Z9 0 U1 5 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0002-7820 EI 1551-2916 J9 J AM CERAM SOC JI J. Am. Ceram. Soc. PD JUL PY 2016 VL 99 IS 7 BP 2221 EP 2225 DI 10.1111/jace.14307 PG 5 WC Materials Science, Ceramics SC Materials Science GA DY3MB UT WOS:000384995800002 ER PT J AU Bentzel, GW Naguib, M Lane, NJ Vogel, SC Presser, V Dubois, S Lu, J Hultman, L Barsoum, MW Caspi, EN AF Bentzel, Grady W. Naguib, Michael Lane, Nina J. Vogel, Sven C. Presser, Volker Dubois, Sylvain Lu, Jun Hultman, Lars Barsoum, Michel W. Caspi, El'ad N. TI High-Temperature Neutron Diffraction, Raman Spectroscopy, and First-Principles Calculations of Ti3SnC2 and Ti2SnC SO JOURNAL OF THE AMERICAN CERAMIC SOCIETY LA English DT Article DE first principles; MAX phases; processing; Raman spectroscopy; thermal expansion ID INITIO MOLECULAR-DYNAMICS; MAX PHASES; M2SNC M; MECHANICAL-PROPERTIES; POWDER DIFFRACTION; ELASTIC PROPERTIES; SCATTERING; HF; NB; ZR AB Herein, we report-for the first time-on the additive-free bulk synthesis of Ti3SnC2. A detailed experimental study of the structure of the latter together with a secondary phase, Ti2SnC, is presented through the use of X-ray diffraction (XRD), and high-resolution transmission microscopy (HRTEM). A previous sample of Ti3SnC2, made using Fe as an additive and Ti2SnC as a secondary phase, was studied by high-temperature neutron diffraction (HTND) and XRD. The room-temperature crystallographic parameters of the two MAX phases in the two samples are quite similar. Based on Rietveld analysis of the HTND data, the average linear thermal expansion coefficients of Ti3SnC2 in the a and c directions were found to be 8.5 (2).10(-6) K-1 and 8.9 (1) . 10(-6) K-1, respectively. The respective values for the Ti2SnC phase are 10.1 (3) . 10(-6) K-1 and 10.8 (6) . 10(-6) K-1. Unlike other MAX phases, the atomic displacement parameters of the Sn atoms in Ti3SnC2 are comparable to those of the Ti and C atoms. When the predictions of the atomic displacement parameters obtained from density functional theory are compared to the experimental results, good quantitative agreement is found for the Sn atoms. In the case of the Ti and C atoms, the agreement is more qualitative. We also used first principles to calculate the elastic properties of both Ti2SnC and Ti3SnC2 and their Raman active modes. The latter are compared to experiment and the agreement was found to be good. C1 [Bentzel, Grady W.; Naguib, Michael; Lane, Nina J.; Presser, Volker; Barsoum, Michel W.; Caspi, El'ad N.] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA. [Vogel, Sven C.] Los Alamos Natl Lab, Mat Sci Radiat & Dynam Extremes MST 8, Los Alamos, NM 87545 USA. [Dubois, Sylvain] Univ Poitiers, CNRS, ENSMA, Dept Phys & Mecan Mat,Inst P,SP2MI,UPR 3346, Teleport 2,Blvd Marie & Pierre Curie,BP30179, F-86962 Futuroscope, France. [Lu, Jun; Hultman, Lars] Linkoping Univ, Thin Film Phys Div, Dept Phys Chem & Biol IFM, SE-58183 Linkoping, Sweden. [Caspi, El'ad N.] Nucl Res Ctr Negev, Dept Phys, POB 9001, IL-84190 Beer Sheva, Israel. RP Caspi, EN (reprint author), Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA.; Caspi, EN (reprint author), Nucl Res Ctr Negev, Dept Phys, POB 9001, IL-84190 Beer Sheva, Israel. EM ecaspi@coe.drexel.edu RI Presser, Volker/F-1975-2010; Sylvain, DUBOIS/A-4724-2013 OI Presser, Volker/0000-0003-2181-0590; Sylvain, DUBOIS/0000-0003-1881-7185 FU Army Research Office [W911NF-1-1-10525]; Alexander von Humboldt Foundation; German Academic Exchange Service (DAAD) Short Term Grant Scholarship; Office of Basic Energy Sciences (DOE); Knut and Alice Wallenberg Foundation; DOE [DEAC5206NA25396] FX This work was funded by Army Research Office (W911NF-1-1-10525). V.P. acknowledges the financial support of the Alexander von Humboldt Foundation. MN is grateful to the the German Academic Exchange Service (DAAD) Short Term Grant Scholarship that partially supported him. This work has benefited from the use of the Lujan Neutron Scattering Center at LANSCE, which is funded by the Office of Basic Energy Sciences (DOE). L.H., J.L., and M.B. also acknowledge the Swedish Research Council and the Swedish Government Strategic Research Area Grant in Materials Science (MAT-LiU) as well as the Ultra-Electron Microscopy Laboratory at Linkoping supported by the Knut and Alice Wallenberg Foundation. Los Alamos National Laboratory is operated by Los Alamos National Security LLC under DOE Contract DEAC5206NA25396. NR 47 TC 1 Z9 1 U1 15 U2 15 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0002-7820 EI 1551-2916 J9 J AM CERAM SOC JI J. Am. Ceram. Soc. PD JUL PY 2016 VL 99 IS 7 BP 2233 EP 2242 DI 10.1111/jace.14210 PG 10 WC Materials Science, Ceramics SC Materials Science GA DY3MB UT WOS:000384995800005 ER PT J AU Armbruster, U Leonelli, L Galvis, VC Strand, D Quinn, EH Jonikas, MC Niyogi, KK AF Armbruster, Ute Leonelli, Lauriebeth Galvis, Viviana Correa Strand, Deserah Quinn, Erica H. Jonikas, Martin C. Niyogi, Krishna K. TI Regulation and Levels of the Thylakoid K+/H+ Antiporter KEA3 Shape the Dynamic Response of Photosynthesis in Fluctuating Light SO PLANT AND CELL PHYSIOLOGY LA English DT Article DE Arabidopsis; KEA3; Non-photochemical quenching; PSII quantum efficiency; Thylakoid membrane ID PHOTOSYSTEM-I; ARABIDOPSIS; DISSIPATION; METABOLISM; COMPLEX; TRANSPORTERS; IRRADIANCE; EFFICIENCY; DECREASE; ENERGY AB Crop canopies create environments of highly fluctuating light intensities. In such environments, photoprotective mechanisms and their relaxation kinetics have been hypothesized to limit photosynthetic efficiency and therefore crop yield potential. Here, we show that overexpression of the Arabidopsis thylakoid K+/H+ antiporter KEA3 accelerates the relaxation of photoprotective energy-dependent quenching after transitions from high to low light in Arabidopsis and tobacco. This, in turn, enhances PSII quantum efficiency in both organisms, supporting that in wild-type plants, residual light energy quenching following a high to low light transition represents a limitation to photosynthetic efficiency in fluctuating light. This finding underscores the potential of accelerating quenching relaxation as a building block for improving photosynthetic efficiency in the field. Additionally, by overexpressing natural KEA3 variants with modification to the C-terminus, we show that KEA3 activity is regulated by a mechanism involving its lumen-localized C-terminus, which lowers KEA3 activity in high light. This regulatory mechanism fine-tunes the balance between photoprotective energy dissipation in high light and maximum quantum yield in low light, likely to be critical for efficient photosynthesis in fluctuating light conditions. C1 [Armbruster, Ute; Leonelli, Lauriebeth; Quinn, Erica H.; Niyogi, Krishna K.] Univ Calif Berkeley, Howard Hughes Med Inst, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Armbruster, Ute; Jonikas, Martin C.] Carnegie Inst Sci, Dept Plant Biol, 290 Panama St, Stanford, CA 94305 USA. [Armbruster, Ute; Galvis, Viviana Correa; Strand, Deserah] Max Planck Inst Mol Plant Physiol, Muhlenberg 1, D-14476 Potsdam, Germany. [Niyogi, Krishna K.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. RP Armbruster, U (reprint author), Univ Calif Berkeley, Howard Hughes Med Inst, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA.; Armbruster, U (reprint author), Carnegie Inst Sci, Dept Plant Biol, 290 Panama St, Stanford, CA 94305 USA.; Armbruster, U (reprint author), Max Planck Inst Mol Plant Physiol, Muhlenberg 1, D-14476 Potsdam, Germany. EM ute.armbruster78@gmail.com FU Carnegie Institution for Science; Max Planck Society; Bill & Melinda Gates Foundation RIPE project at the University of Illinois; Howard Hughes Medical Institute; Gordon and Betty Moore Foundation [GBMF3070]; Deutsche Forschungsgemeinschaft [AR 808/1-1, AR 808/1-2] FX This work was supported by the Carnegie Institution for Science; the Max Planck Society; the Bill & Melinda Gates Foundation RIPE project at the University of Illinois [a subaward]; the Howard Hughes Medical Institute; the Gordon and Betty Moore Foundation [grant GBMF3070 to K.K.N.]; the Deutsche Forschungsgemeinschaft [AR 808/1-1, 1-2 to U.A.]. NR 33 TC 2 Z9 2 U1 5 U2 5 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0032-0781 EI 1471-9053 J9 PLANT CELL PHYSIOL JI Plant Cell Physiol. PD JUL PY 2016 VL 57 IS 7 BP 1557 EP 1567 DI 10.1093/pcp/pcw085 PG 11 WC Plant Sciences; Cell Biology SC Plant Sciences; Cell Biology GA DX9LG UT WOS:000384716300020 PM 27335350 ER PT J AU Smallwood, CL Kaindl, RA Lanzara, A AF Smallwood, Christopher L. Kaindl, Robert A. Lanzara, Alessandra TI Ultrafast angle-resolved photoemission spectroscopy of quantum materials SO EPL LA English DT Article ID CHARGE-DENSITY-WAVE; CUPRATE SUPERCONDUCTOR; TOPOLOGICAL INSULATOR; FLOQUET-BLOCH; COOPER PAIRS; DYNAMICS; GRAPHENE; METALS; SPECTROMETER; HARMONICS AB Techniques in time- and angle-resolved photoemission spectroscopy have facilitated a number of recent advances in the study of quantum materials. We review developments in this field related to the study of incoherent nonequilibrium electron dynamics, the analysis of interactions between electrons and collective excitations, the exploration of dressed-state physics, and the illumination of unoccupied band structure. Future prospects are also discussed. Copyright (C) EPLA, 2016 C1 [Smallwood, Christopher L.] Univ Colorado, JILA, Boulder, CO 80309 USA. [Smallwood, Christopher L.] NIST, Boulder, CO 80309 USA. [Kaindl, Robert A.; Lanzara, Alessandra] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Lanzara, Alessandra] Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. RP Lanzara, A (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Lanzara, A (reprint author), Univ Calif Berkeley, Dept Phys, Berkeley, CA 94720 USA. EM alanzara@lbl.gov FU Ultrafast Materials Program at Lawrence Berkeley National Laboratory - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-05CH11231]; NRC Research Associateship award at NIST FX This work was supported as part of the Ultrafast Materials Program at Lawrence Berkeley National Laboratory, funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract No. DE-AC02-05CH11231. CLS acknowledges support from an NRC Research Associateship award at NIST. NR 81 TC 0 Z9 0 U1 17 U2 17 PU EPL ASSOCIATION, EUROPEAN PHYSICAL SOCIETY PI MULHOUSE PA 6 RUE DES FRERES LUMIERE, MULHOUSE, 68200, FRANCE SN 0295-5075 EI 1286-4854 J9 EPL-EUROPHYS LETT JI EPL PD JUL PY 2016 VL 115 IS 2 AR 27001 DI 10.1209/0295-5075/115/27001 PG 7 WC Physics, Multidisciplinary SC Physics GA DX5YF UT WOS:000384457900021 ER PT J AU McGuire, AD Koven, C Lawrence, DM Clein, JS Xia, JY Beer, C Burke, E Chen, GS Chen, XD Delire, C Jafarov, E MacDougall, AH Marchenko, S Nicolsky, D Peng, SS Rinke, A Saito, K Zhang, WX Alkama, R Bohn, TJ Ciais, P Decharme, B Ekici, A Gouttevin, I Hajima, T Hayes, DJ Ji, DY Krinner, G Lettenmaier, DP Luo, YQ Miller, PA Moore, JC Romanovsky, V Schadel, C Schaefer, K Schuur, EAG Smith, B Sueyoshi, T Zhuang, QL AF McGuire, A. David Koven, Charles Lawrence, David M. Clein, Joy S. Xia, Jiangyang Beer, Christian Burke, Eleanor Chen, Guangsheng Chen, Xiaodong Delire, Christine Jafarov, Elchin MacDougall, Andrew H. Marchenko, Sergey Nicolsky, Dmitry Peng, Shushi Rinke, Annette Saito, Kazuyuki Zhang, Wenxin Alkama, Ramdane Bohn, Theodore J. Ciais, Philippe Decharme, Bertrand Ekici, Altug Gouttevin, Isabelle Hajima, Tomohiro Hayes, Daniel J. Ji, Duoying Krinner, Gerhard Lettenmaier, Dennis P. Luo, Yiqi Miller, Paul A. Moore, John C. Romanovsky, Vladimir Schaedel, Christina Schaefer, Kevin Schuur, Edward A. G. Smith, Benjamin Sueyoshi, Tetsuo Zhuang, Qianlai TI Variability in the sensitivity among model simulations of permafrost and carbon dynamics in the permafrost region between 1960 and 2009 SO GLOBAL BIOGEOCHEMICAL CYCLES LA English DT Article DE carbon cycle; climate change; permafrost; permafrost carbon feedback; sensitivity; soil carbon ID EARTH SYSTEM MODELS; GLOBAL VEGETATION MODELS; NET PRIMARY PRODUCTION; CLIMATE-CHANGE; SOIL CARBON; ARCTIC TUNDRA; TERRESTRIAL BIOSPHERE; METHANE EMISSIONS; ACTIVE LAYER; C DYNAMICS AB A significant portion of the large amount of carbon (C) currently stored in soils of the permafrost region in the Northern Hemisphere has the potential to be emitted as the greenhouse gases CO2 and CH4 under a warmer climate. In this study we evaluated the variability in the sensitivity of permafrost and C in recent decades among land surface model simulations over the permafrost region between 1960 and 2009. The 15 model simulations all predict a loss of near-surface permafrost (within 3m) area over the region, but there are large differences in the magnitude of the simulated rates of loss among the models (0.2 to 58.8x10(3)km(2)yr(-1)). Sensitivity simulations indicated that changes in air temperature largely explained changes in permafrost area, although interactions among changes in other environmental variables also played a role. All of the models indicate that both vegetation and soil C storage together have increased by 156 to 954TgCyr(-1) between 1960 and 2009 over the permafrost region even though model analyses indicate that warming alone would decrease soil C storage. Increases in gross primary production (GPP) largely explain the simulated increases in vegetation and soil C. The sensitivity of GPP to increases in atmospheric CO2 was the dominant cause of increases in GPP across the models, but comparison of simulated GPP trends across the 1982-2009 period with that of a global GPP data set indicates that all of the models overestimate the trend in GPP. Disturbance also appears to be an important factor affecting C storage, as models that consider disturbance had lower increases in C storage than models that did not consider disturbance. To improve the modeling of C in the permafrost region, there is the need for the modeling community to standardize structural representation of permafrost and carbon dynamics among models that are used to evaluate the permafrost C feedback and for the modeling and observational communities to jointly develop data sets and methodologies to more effectively benchmark models. C1 [McGuire, A. David] Univ Alaska Fairbanks, Alaska Cooperat Fish & Wildlife Res Unit, US Geol Survey, Fairbanks, AK USA. [Koven, Charles] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Lawrence, David M.] Natl Ctr Atmospher Res, POB 3000, Boulder, CO 80307 USA. [Clein, Joy S.] Univ Alaska Fairbanks, Inst Arctic Biol, Fairbanks, AK USA. [Xia, Jiangyang] China Normal Univ, Sch Ecol & Environm Sci, Tiantong Natl Stn Forest Ecosyst, Shanghai, Peoples R China. [Beer, Christian; Ekici, Altug] Stockholm Univ, Dept Environm Sci & Analyt Chem ACES & Bolin Ctr, Stockholm, Sweden. [Burke, Eleanor] Met Off Hadley Ctr, Exeter, Devon, England. [Chen, Guangsheng; Hayes, Daniel J.] Oak Ridge Natl Lab, Div Environm Sci, POB 2008, Oak Ridge, TN 37831 USA. [Chen, Xiaodong] Univ Washington, Dept Civil & Environm Engn, Seattle, WA 98195 USA. [Delire, Christine; Alkama, Ramdane; Decharme, Bertrand] Meteo France, GAME, CNRS, UMR 3589, Toulouse, France. [Jafarov, Elchin] Univ Colorado Boulder, Inst Arctic Alpine Res, Boulder, CO USA. [MacDougall, Andrew H.] Univ Victoria, Sch Earth & Ocean Sci, Victoria, BC, Canada. [Marchenko, Sergey; Nicolsky, Dmitry; Romanovsky, Vladimir] Univ Alaska Fairbanks, Inst Geophys, Fairbanks, AK 99775 USA. [Peng, Shushi; Ciais, Philippe] CEA CNRS UVSQ, Lab Sci Climat & Environm, UMR 8212, Gif Sur Yvette, France. [Peng, Shushi; Gouttevin, Isabelle; Krinner, Gerhard] Univ Grenoble Alpes, LGGE, UMR 5183, CNRS, BP53, Grenoble, France. [Rinke, Annette] Helmholtz Ctr Polar & Marine Res, Alfred Wegener Inst, Potsdam, Germany. [Rinke, Annette; Ji, Duoying; Moore, John C.] Beijing Normal Univ, Coll Global Change & Earth Syst Sci, State Key Lab Earth Surface Proc & Resource Ecol, Beijing, Peoples R China. [Saito, Kazuyuki; Hajima, Tomohiro; Sueyoshi, Tetsuo] Japan Agcy Marine Earth Sci & Technol, Dept Integrated Climate Change Project Res, Yokohama, Kanagawa, Japan. [Zhang, Wenxin; Miller, Paul A.; Smith, Benjamin] Lund Univ, Dept Phys Geog & Ecosyst Sci, Lund, Sweden. [Bohn, Theodore J.] Arizona State Univ, Sch Earth & Space Explorat, Tempe, AZ USA. [Gouttevin, Isabelle] UR HHLY, Irstea, 5 Rue Doua,CS 70077, Villeurbanne, France. [Lettenmaier, Dennis P.] Univ Calif Los Angeles, Dept Geog, Los Angeles, CA 90024 USA. [Luo, Yiqi] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Schaedel, Christina; Schuur, Edward A. G.] No Arizona Univ, Ctr Ecosyst Sci & Soc, Flagstaff, AZ USA. [Schaedel, Christina; Schuur, Edward A. G.] No Arizona Univ, Dept Biol Sci, Flagstaff, AZ USA. [Schaefer, Kevin] Univ Colorado Boulder, Natl Snow & Ice Data Ctr, Boulder, CO USA. [Zhuang, Qianlai] Purdue Univ, W Lafayette, IN 47907 USA. RP McGuire, AD (reprint author), Univ Alaska Fairbanks, Alaska Cooperat Fish & Wildlife Res Unit, US Geol Survey, Fairbanks, AK USA. EM admcguire@alaska.edu RI Krinner, Gerhard/A-6450-2011; Smith, Benjamin/I-1212-2016; Moore, John/B-2868-2013; Koven, Charles/N-8888-2014; OI Krinner, Gerhard/0000-0002-2959-5920; Smith, Benjamin/0000-0002-6987-5337; Moore, John/0000-0001-8271-5787; Koven, Charles/0000-0002-3367-0065; JAFAROV, ELCHIN/0000-0002-8310-3261; Rinke, Annette/0000-0002-6685-9219 FU National Science Foundation through Research Coordination Network program; National Science Foundation through Study of Environmental Arctic Change program; U.S. Geological Survey; U.S. Department of Energy Office of Science (Biological and Environmental Research); University of Victoria; NSERC CGS; NSERC CREATE; Joint DECC/Defra Met Office Hadley Centre Climate Programme [GA01101]; European Union FP7-ENVIRONMENT project [PAGE21]; program CLASSIQUE of the French "Agence Nationale pour la Recherche"; Program for Risk Information on Climate Change, MEXT, Japan; Modeling the Regional and Global Earth System activity; Lund University Centre for the study of Climate and Carbon Cycle FX Support for this study was provided by the National Science Foundation through the Research Coordination Network program and through the Study of Environmental Arctic Change program, the U.S. Geological Survey, the U.S. Department of Energy Office of Science (Biological and Environmental Research), the University of Victoria, NSERC CGS, NSERC CREATE, Joint DECC/Defra Met Office Hadley Centre Climate Programme (GA01101), the European Union FP7-ENVIRONMENT project PAGE21, the program CLASSIQUE of the French "Agence Nationale pour la Recherche," the Program for Risk Information on Climate Change, MEXT, Japan, the Modeling the Regional and Global Earth System activity, and the Lund University Centre for the study of Climate and Carbon Cycle. Any use of trade, firm, or product names is for descriptive purposes only and does not imply endorsement by the U.S. Government. The simulation data analyzed in this manuscript is available through the National Snow and Ice Data Center through e-mail request to Kevin Schaefer (kevin.schaefer@nsidc.org). NR 121 TC 4 Z9 4 U1 29 U2 29 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 0886-6236 EI 1944-9224 J9 GLOBAL BIOGEOCHEM CY JI Glob. Biogeochem. Cycle PD JUL PY 2016 VL 30 IS 7 BP 1015 EP 1037 DI 10.1002/2016GB005405 PG 23 WC Environmental Sciences; Geosciences, Multidisciplinary; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Geology; Meteorology & Atmospheric Sciences GA DV0BK UT WOS:000382582400004 ER PT J AU Barone, M Arunajatesan, S AF Barone, Matthew Arunajatesan, Srinivasan TI Pressure Loadings in a Rectangular Cavity with and Without a Captive Store SO JOURNAL OF AIRCRAFT LA English DT Article; Proceedings Paper CT 52nd AIAA Aerospace Sciences Meeting CY JAN 12-18, 2014 CL National Harbor, MD SP AIAA AB Simulations of the flow past a rectangular cavity containing a model captive store are performed using a hybrid Reynolds-averaged Navier-Stokes/large-eddy simulation model. Calculated pressure fluctuation spectra are validated using measurements made on the same configuration in a trisonic wind tunnel at Mach numbers of 0.60, 0.80, and 1.47. The simulation results are used to calculate unsteady integrated forces and moments acting on the store. Spectra of the forces and moments, along with correlations calculated for force/moment pairs, reveal that a complex relationship exists between the unsteady integrated forces and the measured resonant cavity modes, as indicated in the cavity wall pressure measurements. The structure of identified cavity resonant tones is examined by visualization of filtered surface pressure fields. C1 [Barone, Matthew] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Arunajatesan, Srinivasan] Sandia Natl Labs, Aerosci Dept, Albuquerque, NM 87185 USA. [Barone, Matthew] Aerosci Dept, 1515 Eubank Blvd SE, Albuquerque, NM 87123 USA. RP Barone, M (reprint author), Aerosci Dept, 1515 Eubank Blvd SE, Albuquerque, NM 87123 USA. EM mbarone@sandia.gov NR 10 TC 0 Z9 0 U1 0 U2 0 PU AMER INST AERONAUTICS ASTRONAUTICS PI RESTON PA 1801 ALEXANDER BELL DRIVE, STE 500, RESTON, VA 22091-4344 USA SN 0021-8669 EI 1533-3868 J9 J AIRCRAFT JI J. Aircr. PD JUL-AUG PY 2016 VL 53 IS 4 BP 982 EP 991 DI 10.2514/1.C033600 PG 10 WC Engineering, Aerospace SC Engineering GA DX3TN UT WOS:000384297100010 ER PT J AU Boriskina, SV Green, MA Catchpole, K Yablonovitch, E Beard, MC Okada, Y Lany, S Gershon, T Zakutayev, A Tahersima, MH Sorger, VJ Naughton, MJ Kempa, K Dagenais, M Yao, Y Xu, L Sheng, X Bronstein, ND Rogers, JA Alivisatos, AP Nuzzo, RG Gordon, JM Wu, DM Wisser, MD Salleo, A Dionne, J Bermel, P Greffet, JJ Celanovic, I Soljacic, M Manor, A Rotschild, C Raman, A Zhu, LX Fan, SH Chen, G AF Boriskina, Svetlana V. Green, Martin A. Catchpole, Kylie Yablonovitch, Eli Beard, Matthew C. Okada, Yoshitaka Lany, Stephan Gershon, Talia Zakutayev, Andriy Tahersima, Mohammad H. Sorger, Volker J. Naughton, Michael J. Kempa, Krzysztof Dagenais, Mario Yao, Yuan Xu, Lu Sheng, Xing Bronstein, Noah D. Rogers, John A. Alivisatos, A. Paul Nuzzo, Ralph G. Gordon, Jeffrey M. Wu, Di M. Wisser, Michael D. Salleo, Alberto Dionne, Jennifer Bermel, Peter Greffet, Jean-Jacques Celanovic, Ivan Soljacic, Marin Manor, Assaf Rotschild, Carmel Raman, Aaswath Zhu, Linxiao Fan, Shanhui Chen, Gang TI Roadmap on optical energy conversion SO JOURNAL OF OPTICS LA English DT Article DE optical energy conversion; light harvesting; solar technology; photovoltaics; solar cell ID RADIATIVE HEAT-TRANSFER; SILICON SOLAR-CELL; SHOCKLEY-QUEISSER LIMIT; CLOSELY-SPACED BODIES; HIGH-EFFICIENCY; UP-CONVERSION; NEAR-FIELD; THERMOPHOTOVOLTAIC SYSTEMS; PHOTONIC CRYSTALS; POWER CONVERSION AB For decades, progress in the field of optical (including solar) energy conversion was dominated by advances in the conventional concentrating optics and materials design. In recent years, however, conceptual and technological breakthroughs in the fields of nanophotonics and plasmonics combined with a better understanding of the thermodynamics of the photon energy-conversion processes reshaped the landscape of energy-conversion schemes and devices. Nanostructured devices and materials that make use of size quantization effects to manipulate photon density of states offer a way to overcome the conventional light absorption limits. Novel optical spectrum splitting and photon-recycling schemes reduce the entropy production in the optical energy-conversion platforms and boost their efficiencies. Optical design concepts are rapidly expanding into the infrared energy band, offering new approaches to harvest waste heat, to reduce the thermal emission losses, and to achieve noncontact radiative cooling of solar cells as well as of optical and electronic circuitries. Light-matter interaction enabled by nanophotonics and plasmonics underlie the performance of the third-and fourth-generation energy-conversion devices, including up-and down-conversion of photon energy, near-field radiative energy transfer, and hot electron generation and harvesting. Finally, the increased market penetration of alternative solar energy-conversion technologies amplifies the role of cost-driven and environmental considerations. This roadmap on optical energy conversion provides a snapshot of the state of the art in optical energy conversion, remaining challenges, and most promising approaches to address these challenges. Leading experts authored 19 focused short sections of the roadmap where they share their vision on a specific aspect of this burgeoning research field. The roadmap opens up with a tutorial section, which introduces major concepts and terminology. It is our hope that the roadmap will serve as an important resource for the scientific community, new generations of researchers, funding agencies, industry experts, and investors. C1 [Boriskina, Svetlana V.; Chen, Gang] MIT, Dept Mech Engn, Cambridge, MA 02139 USA. [Green, Martin A.] Univ New South Wales, Sch Photovolta & Renewable Energy Engn, ACAP, Sydney, NSW, Australia. [Catchpole, Kylie] Australian Natl Univ, Res Sch Engn, Ctr Sustainable Energy Syst, Canberra, ACT 2601, Australia. [Yablonovitch, Eli; Alivisatos, A. Paul] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Yablonovitch, Eli] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Beard, Matthew C.; Lany, Stephan; Zakutayev, Andriy] Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. [Okada, Yoshitaka] Univ Tokyo, Res Ctr Adv Sci & Technol, Meguro Ku, 4-6-1 Komaba, Tokyo, Japan. [Gershon, Talia] IBM TJ Watson Res Ctr, 1101 Kitchawan Rd, Yorktown Hts, NY 10598 USA. [Tahersima, Mohammad H.; Sorger, Volker J.] George Washington Univ, Dept Elect & Comp Engn, 801 22nd St NW, Washington, DC 20052 USA. [Naughton, Michael J.; Kempa, Krzysztof] Boston Coll, Dept Phys, Chestnut Hill, MA 02467 USA. [Dagenais, Mario] Univ Maryland, Dept Elect Engn, College Pk, MD 20742 USA. [Yao, Yuan; Xu, Lu; Rogers, John A.; Nuzzo, Ralph G.] Univ Illinois, Dept Chem, Frederick Seitz Mat Res Lab, Urbana, IL 61801 USA. [Sheng, Xing; Rogers, John A.; Nuzzo, Ralph G.] Univ Illinois, Dept Mat Sci & Engn, Urbana, IL 61801 USA. [Bronstein, Noah D.; Alivisatos, A. Paul] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Gordon, Jeffrey M.] Ben Gurion Univ Negev, Dept Solar Energy & Environm Phys, Blaustein Inst Desert Res, Sede Boqer Campus, IL-84990 Sede Boqer, Israel. [Wu, Di M.] Stanford Univ, Dept Chem, 333 Campus Dr, Stanford, CA 94305 USA. [Wisser, Michael D.; Salleo, Alberto; Dionne, Jennifer] Stanford Univ, Dept Mat Sci & Engn, 496 Lomita Mall, Stanford, CA 94305 USA. [Bermel, Peter] Purdue Univ, Elect & Comp Engn, Birck Nanotechnol Ctr, 1205 West State St, W Lafayette, IN 47907 USA. [Greffet, Jean-Jacques] Univ Paris Saclay, CNRS, Inst Opt, Lab Charles Fabry, 2 Ave Fresnel, F-91127 Palaiseau, France. [Celanovic, Ivan; Soljacic, Marin] MIT, Dept Phys, Cambridge, MA 02139 USA. [Manor, Assaf] Technion Israel Inst Technol, Russel Berrie Nanotechnol Inst, IL-32000 Haifa, Israel. [Rotschild, Carmel] Technion Israel Inst Technol, Dept Mech Engn, IL-32000 Haifa, Israel. [Raman, Aaswath; Zhu, Linxiao; Fan, Shanhui] Stanford Univ, Dept Elect Engn, Stanford, CA 94305 USA. [Alivisatos, A. Paul] Univ Calif Berkeley, Dept Mat Sci & Engn, Kavli Energy NanoScience Inst, Berkeley, CA 94720 USA. [Green, Martin A.] Univ New South Wales, Sydney, NSW, Australia. [Catchpole, Kylie] Australian Natl Univ, Canberra, ACT, Australia. [Yablonovitch, Eli; Beard, Matthew C.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Okada, Yoshitaka; Lany, Stephan; Zakutayev, Andriy] Univ Tokyo, Tokyo, Japan. [Tahersima, Mohammad H.; Sorger, Volker J.] George Washington Univ, Washington, DC USA. [Naughton, Michael J.; Kempa, Krzysztof] Boston Coll, Chestnut Hill, MA 02167 USA. [Dagenais, Mario] Univ Illinois, Urbana, IL 61801 USA. [Yao, Yuan; Xu, Lu] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Gordon, Jeffrey M.] Ben Gurion Univ Negev, IL-84105 Beer Sheva, Israel. [Boriskina, Svetlana V.] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. [Wu, Di M.; Wisser, Michael D.; Salleo, Alberto; Dionne, Jennifer] Stanford Univ, Stanford, CA 94305 USA. [Bermel, Peter] Purdue Univ, W Lafayette, IN 47907 USA. [Greffet, Jean-Jacques] Univ Paris Saclay, CNRS, Inst Opt, Palaiseau, France. [Manor, Assaf; Rotschild, Carmel] Technion Israel Inst Technol, Haifa, Israel. RP Boriskina, SV (reprint author), MIT, Dept Mech Engn, Cambridge, MA 02139 USA. EM sborisk@mit.edu RI Chen, Gang/J-1325-2014; Greffet, Jean-Jacques/Q-2427-2015; Sheng, Xing/B-7661-2011; Alivisatos , Paul /N-8863-2015; Manor, Assaf/L-4058-2016; OI Chen, Gang/0000-0002-3968-8530; Greffet, Jean-Jacques/0000-0002-4048-2150; Sheng, Xing/0000-0002-8744-1700; Alivisatos , Paul /0000-0001-6895-9048; Manor, Assaf/0000-0002-9502-2442; Catchpole, Kylie/0000-0003-4858-1820; BEARD, MATTHEW/0000-0002-2711-1355; Okada, Yoshitaka/0000-0002-1547-5477 FU 'Solid State Solar-Thermal Energy Conversion Center (S3TEC), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001299/DE-FG02-09ER46577]; DOE-BES Award [DE-FG02-02ER45977] FX The author thanks S. Boriskina, V. Chiloyan, B. L. Liao, W. C. Hsu, J. Tong, and J. W. Zhou for helpful discussions. This work was supported, in part, by the 'Solid State Solar-Thermal Energy Conversion Center (S3TEC), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award No. DE-SC0001299/DE-FG02-09ER46577 (for TPV applications) and by DOE-BES Award No. DE-FG02-02ER45977 (for extracting photons from the near field to the far field). NR 198 TC 8 Z9 8 U1 52 U2 52 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 2040-8978 EI 2040-8986 J9 J OPTICS-UK JI J. Opt. PD JUL PY 2016 VL 18 IS 7 AR 073004 DI 10.1088/2040-8978/18/7/073004 PG 48 WC Optics SC Optics GA DW8LZ UT WOS:000383908800007 ER PT J AU Chen, HT Taylor, AJ Yu, NF AF Chen, Hou-Tong Taylor, Antoinette J. Yu, Nanfang TI A review of metasurfaces: physics and applications SO REPORTS ON PROGRESS IN PHYSICS LA English DT Review DE metamaterials and metasurfaces; wavefront shaping and beam forming; polarization; active metasurfaces; nonlinearity; dielectric metamaterials; surface and guided waves ID DIELECTRIC RESONATOR ANTENNAS; QUARTER-WAVE PLATE; ELECTROMAGNETICALLY INDUCED TRANSPARENCY; TUNABLE TERAHERTZ METAMATERIALS; LINEAR-POLARIZATION CONVERSION; ORBITAL ANGULAR-MOMENTUM; PANCHARATNAM-BERRY PHASE; GRADIENT META-SURFACES; SPLIT-RING RESONATORS; BROAD-BAND AB Metamaterials are composed of periodic subwavelength metal/dielectric structures that resonantly couple to the electric and/or magnetic components of the incident electromagnetic fields, exhibiting properties that are not found in nature. This class of micro-and nano-structured artificial media have attracted great interest during the past 15 years and yielded ground-breaking electromagnetic and photonic phenomena. However, the high losses and strong dispersion associated with the resonant responses and the use of metallic structures, as well as the difficulty in fabricating the micro-and nanoscale 3D structures, have hindered practical applications of metamaterials. Planar metamaterials with subwavelength thickness, or metasurfaces, consisting of single-layer or few-layer stacks of planar structures, can be readily fabricated using lithography and nanoprinting methods, and the ultrathin thickness in the wave propagation direction can greatly suppress the undesirable losses. Metasurfaces enable a spatially varying optical response (e.g. scattering amplitude, phase, and polarization), mold optical wavefronts into shapes that can be designed at will, and facilitate the integration of functional materials to accomplish active control and greatly enhanced nonlinear response. This paper reviews recent progress in the physics of metasurfaces operating at wavelengths ranging from microwave to visible. We provide an overview of key metasurface concepts such as anomalous reflection and refraction, and introduce metasurfaces based on the Pancharatnam-Berry phase and Huygens' metasurfaces, as well as their use in wavefront shaping and beam forming applications, followed by a discussion of polarization conversion in few-layer metasurfaces and their related properties. An overview of dielectric metasurfaces reveals their ability to realize unique functionalities coupled with Mie resonances and their low ohmic losses. We also describe metasurfaces for wave guidance and radiation control, as well as active and nonlinear metasurfaces. Finally, we conclude by providing our opinions of opportunities and challenges in this rapidly developing research field. C1 [Chen, Hou-Tong] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. [Taylor, Antoinette J.] Los Alamos Natl Lab, Associate Directorate Chem Life & Earth Sci, Los Alamos, NM 87545 USA. [Yu, Nanfang] Columbia Univ, Dept Appl Phys & Appl Math, New York, NY 10027 USA. RP Chen, HT (reprint author), Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA. EM chenht@lanl.gov; ttaylor@lanl.gov; ny2214@columbia.edu RI Chen, Hou-Tong/C-6860-2009 OI Chen, Hou-Tong/0000-0003-2014-7571 FU Los Alamos National Laboratory LDRD Program; NSF [ECCS-1307948]; AFOSR Multidisciplinary University Research Initiative program [FA9550-14-1-0389]; DARPA Young Faculty Award [D15AP00111]; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX HTC acknowledges support in part from the Los Alamos National Laboratory LDRD Program. NY acknowledges support from NSF (grant ECCS-1307948), the AFOSR Multidisciplinary University Research Initiative program (grant FA9550-14-1-0389), and DARPA Young Faculty Award (grant D15AP00111). This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences Nanoscale Science Research Center operated jointly by Los Alamos and Sandia National Laboratories. Los Alamos National Laboratory, an affirmative action/equal opportunity employer, is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. DE-AC52-06NA25396. NR 255 TC 5 Z9 5 U1 131 U2 137 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0034-4885 EI 1361-6633 J9 REP PROG PHYS JI Rep. Prog. Phys. PD JUL PY 2016 VL 79 IS 7 AR 076401 DI 10.1088/0034-4885/79/7/076401 PG 40 WC Physics, Multidisciplinary SC Physics GA DW9DL UT WOS:000383955800011 ER PT J AU Dracoulis, GD Walker, PM Kondev, FG AF Dracoulis, G. D. Walker, P. M. Kondev, F. G. TI Review of metastable states in heavy nuclei SO REPORTS ON PROGRESS IN PHYSICS LA English DT Review DE nuclear structure; isomers; decay properties ID HIGH-SPIN ISOMERS; MULTI-QUASI-PARTICLE; GAMMA-RAY SPECTROSCOPY; CORE-EXCITED-STATES; HIGH-K ISOMERS; GENERATOR-COORDINATE METHOD; ELECTRIC QUADRUPOLE-MOMENT; DEEP-INELASTIC COLLISIONS; HALF-LIFE MEASUREMENTS; FRS-ESR FACILITY AB The structure of nuclear isomeric states is reviewed in the context of their role in contemporary nuclear physics research. Emphasis is given to high-spin isomers in heavy nuclei, with A greater than or similar to 150. The possibility to exploit isomers to study some of the most exotic nuclei is a recurring theme. In spherical nuclei, the role of octupole collectivity is discussed in detail, while in deformed nuclei the limitations of the K quantum number are addressed. Isomer targets and isomer beams are considered, along with applications related to energy storage, astrophysics, medicine, and experimental advances. C1 [Dracoulis, G. D.] RSPE Australian Natl Univ, Dept Nucl Phys, Canberra, ACT 0200, Australia. [Walker, P. M.] Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. [Kondev, F. G.] Argonne Natl Lab, Nucl Engn Div, Argonne, IL 60439 USA. RP Walker, PM (reprint author), Univ Surrey, Dept Phys, Guildford GU2 7XH, Surrey, England. EM P.Walker@Surrey.ac.uk; kondev@anl.gov FU Australian Research Council Discovery programme; UK Science and Technology Facilities Council [ST/L005743/1]; U.S. Department of Energy, Office of Science, Office of Nuclear Physics [DE-AC02-06CH11357] FX Special thanks for their physics input go to B Fornal, G Lane, M Reed, and F Xu. G Dracoulis received support from the Australian Research Council Discovery programme. Phil Walker is supported by the UK Science and Technology Facilities Council under grant No. ST/L005743/1. F Kondev is supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics under contract No. DE-AC02-06CH11357. NR 478 TC 3 Z9 3 U1 7 U2 7 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0034-4885 EI 1361-6633 J9 REP PROG PHYS JI Rep. Prog. Phys. PD JUL PY 2016 VL 79 IS 7 AR 076301 DI 10.1088/0034-4885/79/7/076301 PG 46 WC Physics, Multidisciplinary SC Physics GA DW9DL UT WOS:000383955800009 PM 27243336 ER PT J AU Hong, S Nakhmanson, SM Fong, DD AF Hong, Seungbum Nakhmanson, Serge M. Fong, Dillon D. TI Screening mechanisms at polar oxide heterointerfaces SO REPORTS ON PROGRESS IN PHYSICS LA English DT Review DE oxide heterostructures; polar interfaces; ferroelectricity ID 2-DIMENSIONAL ELECTRON-GAS; FIELD-EFFECT TRANSISTOR; FERROELECTRIC THIN-FILMS; CHARGE GRADIENT MICROSCOPY; TRANSITION-METAL OXIDES; OXYGEN-SURFACE EXCHANGE; BOUNDARY-CONDITIONS; DEFECT CHEMISTRY; BAND OFFSETS; AB-INITIO AB The interfaces of polar oxide heterostructures can display electronic properties unique from the oxides they border, as they require screening from either internal or external sources of charge. The screening mechanism depends on a variety of factors, including the band structure at the interface, the presence of point defects or adsorbates, whether or not the oxide is ferroelectric, and whether or not an external field is applied. In this review, we discuss both theoretical and experimental aspects of different screening mechanisms, giving special emphasis to ways in which the mechanism can be altered to provide novel or tunable functionalities. We begin with a theoretical introduction to the problem and highlight recent progress in understanding the impact of point defects on polar interfaces. Different case studies are then discussed, for both the high thickness regime, where interfaces must be screened and each interface can be considered separately, and the low thickness regime, where the degree and nature of screening can be manipulated and the interfaces are close enough to interact. We end with a brief outlook toward new developments in this rapidly progressing field. C1 [Hong, Seungbum; Fong, Dillon D.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. [Hong, Seungbum] Korea Adv Inst Sci & Technol, Dept Mat Sci Engn, Daejeon 305701, South Korea. [Nakhmanson, Serge M.] Univ Connecticut, Dept Mat Sci & Engn, Storrs, CT 06269 USA. [Nakhmanson, Serge M.] Univ Connecticut, Inst Mat Sci, Storrs, CT 06269 USA. [Nakhmanson, Serge M.] Univ Connecticut, Dept Phys, Storrs, CT 06269 USA. RP Hong, S (reprint author), Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA.; Hong, S (reprint author), Korea Adv Inst Sci & Technol, Dept Mat Sci Engn, Daejeon 305701, South Korea. EM hong@anl.gov; serge.nakhmanson@uconn.edu; fong@anl.gov RI Hong, Seungbum/B-7708-2009 OI Hong, Seungbum/0000-0002-2667-1983 FU National Science Foundation [DMR 1309114]; U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering FX SMN is grateful to M Stengel, J Junquera and C Noguera for many insightful discussions, and acknowledges support from the National Science Foundation (DMR 1309114). SH and DDF were supported by the U.S. Department of Energy (DOE), Office of Science, Office of Basic Energy Sciences (BES), Division of Materials Sciences and Engineering. NR 351 TC 1 Z9 1 U1 36 U2 36 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0034-4885 EI 1361-6633 J9 REP PROG PHYS JI Rep. Prog. Phys. PD JUL PY 2016 VL 79 IS 7 AR 076501 DI 10.1088/0034-4885/79/7/076501 PG 40 WC Physics, Multidisciplinary SC Physics GA DW9DL UT WOS:000383955800012 ER PT J AU Norman, MR AF Norman, M. R. TI Materials design for new superconductors SO REPORTS ON PROGRESS IN PHYSICS LA English DT Review DE materials design; superconductors; materials genome ID HIGH-TEMPERATURE SUPERCONDUCTIVITY; HIGH-TC SUPERCONDUCTIVITY; HEAVY-FERMION COMPOUNDS; ELECTRONIC-STRUCTURE; INTERFACE SUPERCONDUCTIVITY; LAYERED SUPERCONDUCTOR; COPPER OXIDES; ANTIFERROMAGNET; PEROVSKITE; INSULATOR AB Since the announcement in 2011 of the Materials Genome Initiative by the Obama administration, much attention has been given to the subject of materials design to accelerate the discovery of new materials that could have technological implications. Although having its biggest impact for more applied materials like batteries, there is increasing interest in applying these ideas to predict new superconductors. This is obviously a challenge, given that superconductivity is a many body phenomenon, with whole classes of known superconductors lacking a quantitative theory. Given this caveat, various efforts to formulate materials design principles for superconductors are reviewed here, with a focus on surveying the periodic table in an attempt to identify cuprate analogues. C1 [Norman, M. R.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Norman, MR (reprint author), Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. EM norman@anl.gov RI Norman, Michael/C-3644-2013 FU Center for Emergent Superconductivity, an Energy Frontier Research Center - US DOE, Office of Science [DE-AC0298CH1088] FX This work was supported by the Center for Emergent Superconductivity, an Energy Frontier Research Center funded by the US DOE, Office of Science, under Award No. DE-AC0298CH1088. The author thanks many of his colleagues for discussions that have helped form the opinions expressed here. NR 112 TC 3 Z9 3 U1 49 U2 53 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0034-4885 EI 1361-6633 J9 REP PROG PHYS JI Rep. Prog. Phys. PD JUL PY 2016 VL 79 IS 7 AR 074502 DI 10.1088/0034-4885/79/7/074502 PG 9 WC Physics, Multidisciplinary SC Physics GA DW9DL UT WOS:000383955800003 PM 27214291 ER PT J AU Boll, R Erk, B Coffee, R Trippel, S Kierspel, T Bomme, C Bozek, JD Burkett, M Carron, S Ferguson, KR Foucar, L Kupper, J Marchenko, T Miron, C Patanen, M Osipov, T Schorb, S Simon, M Swiggers, M Techert, S Ueda, K Bostedt, C Rolles, D Rudenko, A AF Boll, Rebecca Erk, Benjamin Coffee, Ryan Trippel, Sebastian Kierspel, Thomas Bomme, Cedric Bozek, John D. Burkett, Mitchell Carron, Sebastian Ferguson, Ken R. Foucar, Lutz Kuepper, Jochen Marchenko, Tatiana Miron, Catalin Patanen, Minna Osipov, Timur Schorb, Sebastian Simon, Marc Swiggers, Michelle Techert, Simone Ueda, Kiyoshi Bostedt, Christoph Rolles, Daniel Rudenko, Artem TI Charge transfer in dissociating iodomethane and fluoromethane molecules ionized by intense femtosecond X-ray pulses SO STRUCTURAL DYNAMICS LA English DT Article ID ELECTRON LASER-PULSES; IONIZATION; EXCITATION; COLLISIONS; DYNAMICS; ATOMS; IONS; CH3F AB Ultrafast electron transfer in dissociating iodomethane and fluoromethane molecules was studied at the Linac Coherent Light Source free-electron laser using an ultraviolet-pump, X-ray-probe scheme. The results for both molecules are discussed with respect to the nature of their UV excitation and different chemical properties. Signatures of long-distance intramolecular charge transfer are observed for both species, and a quantitative analysis of its distance dependence in iodomethane is carried out for charge states up to I21+. The reconstructed critical distances for electron transfer are in good agreement with a classical over-the-barrier model and with an earlier experiment employing a near-infrared pump pulse. (C) 2016 Author(s). C1 [Boll, Rebecca; Erk, Benjamin; Bomme, Cedric; Techert, Simone; Rolles, Daniel] Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany. [Boll, Rebecca] Max Planck Inst Nucl Phys, D-69117 Heidelberg, Germany. [Coffee, Ryan; Bozek, John D.; Carron, Sebastian; Ferguson, Ken R.; Osipov, Timur; Schorb, Sebastian; Swiggers, Michelle; Bostedt, Christoph] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Trippel, Sebastian; Kierspel, Thomas; Kuepper, Jochen] DESY, Ctr Free Electron Laser Sci, D-22607 Hamburg, Germany. [Kierspel, Thomas; Kuepper, Jochen] Univ Hamburg, Ctr Ultrafast Imaging, D-22761 Hamburg, Germany. [Burkett, Mitchell; Rolles, Daniel; Rudenko, Artem] Kansas State Univ, JR Macdonald Lab, Manhattan, KS 66506 USA. [Foucar, Lutz] Max Planck Inst Med Res, D-69120 Heidelberg, Germany. [Kuepper, Jochen] Univ Hamburg, Dept Phys, D-22761 Hamburg, Germany. [Marchenko, Tatiana; Simon, Marc] UPMC Univ Paris 06, Sorbonne Univ, CNRS, Lab Chim Phys Mat & Rayonnement,UMR 7614, F-75005 Paris, France. [Miron, Catalin; Patanen, Minna] Synchrotron SOLEIL, BP 48, F-91192 Gif Sur Yvette, France. [Miron, Catalin] Horia Hulubei Natl Inst Phys & Nucl Engn, Extreme Light Infrastruct Nucl Phys, RO-077125 Magurele, Jud Ilfov, Romania. [Patanen, Minna] Univ Oulu, Mol Mat Res Community, POB 3000, FIN-90014 Oulu, Finland. [Techert, Simone] Max Planck Inst Biophys Chem, D-37077 Gottingen, Germany. [Techert, Simone] Univ Gottingen, Inst Xray Phys, D-37077 Gottingen, Germany. [Ueda, Kiyoshi] Tohoku Univ, IMRAM, Sendai, Miyagi 9808577, Japan. [Bostedt, Christoph] Argonne Natl Lab, Lemont, IL 60439 USA. [Bostedt, Christoph] Northwestern Univ, Dept Phys & Astron, Evanston, IL 60208 USA. RP Boll, R (reprint author), Deutsch Elektronen Synchrotron DESY, D-22607 Hamburg, Germany.; Boll, R (reprint author), Max Planck Inst Nucl Phys, D-69117 Heidelberg, Germany. EM rebecca.boll@desy.de; rudenko@phys.ksu.edu RI Kupper, Jochen/A-5564-2008; Bozek, John/E-9260-2010; MIRON, Catalin/D-3446-2009; Rudenko, Artem/C-7412-2009; Trippel, Sebastian/J-7825-2015; OI Kupper, Jochen/0000-0003-4395-9345; Bozek, John/0000-0001-7486-7238; MIRON, Catalin/0000-0002-8302-7158; Rudenko, Artem/0000-0002-9154-8463; Trippel, Sebastian/0000-0002-1895-3868; Boll, Rebecca/0000-0001-6286-4064 NR 49 TC 2 Z9 2 U1 16 U2 23 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2329-7778 J9 STRUCT DYNAM-US JI Struct. Dyn.-US PD JUL PY 2016 VL 3 IS 4 AR 043207 DI 10.1063/1.4944344 PG 15 WC Chemistry, Physical; Physics, Atomic, Molecular & Chemical SC Chemistry; Physics GA DW8CK UT WOS:000383880700009 PM 27051675 ER PT J AU De Wilde, J Richards, G Benyahia, S AF De Wilde, Juray Richards, George Benyahia, Sofiane TI Qualitative numerical study of simultaneous high-G-intensified gas-solids contact, separation and segregation in a bi-disperse rotating fluidized bed in a vortex chamber SO ADVANCED POWDER TECHNOLOGY LA English DT Article DE Fluidization; Process intensification; Segregation; High-G; Vortex chamber ID CHEMICAL-LOOPING COMBUSTION; STATIC GEOMETRY; PARTICLES; REACTOR; FLOW AB Coupled discrete particle method - computational fluid dynamics simulations are carried out to demonstrate the potential of combined high-G-intensified gas-solids contact, gas-solids separation and segregation in a rotating fluidized bed in a static vortex chamber. A case study with two distinct types of particles is focused on. When feeding solids using a standard solids inlet design, a dense and uniform rotating fluidized bed is formed, guaranteeing intense gas-solids contact. The presence of both types of particles near the chimney region reduces, however, the strength of the central vortex and is detrimental for separation and segregation. Optimization of the solids inlet design is required, as illustrated by stopping the solids feeding. High-G separation and segregation of the batch of particles is demonstrated, as the strength of the central vortex is restored. The flexibility with respect to the gas flow rate of the bed density and uniformity and of the gas-solids separation and segregation is demonstrated, a unique feature of vortex chamber generated rotating fluidized beds. With the particles considered in this case study, turbulent dispersion by large eddies in the gas phase is shown to have only a minor impact on the height of the inner bed of small/light particles. (C) 2016 The Society of Powder Technology Japan. Published by Elsevier B.V. and The Society of Powder Technology Japan. All rights reserved. C1 [De Wilde, Juray; Richards, George; Benyahia, Sofiane] US DOE, Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. [De Wilde, Juray] Catholic Univ Louvain, Mat & Proc Engn IMAP, Pl St Barbe 2, B-1348 Louvain, Belgium. RP De Wilde, J (reprint author), Catholic Univ Louvain, Mat & Proc Engn IMAP, Pl St Barbe 2, B-1348 Louvain, Belgium. EM juray.dewilde@uclouvain.be; Sofiane.Benyahia@netl.doe.gov FU U.S. Department of Energy FX This research was supported in part by an appointment to the National Energy Technology Laboratory Research Participation Program, sponsored by the U.S. Department of Energy and administered by the Oak Ridge Institute for Science and Education. S.B. acknowledges the help of Jean-Francois Dietiker (WVU/NETL) in answering questions related to geometry design and integration with the CFD code MFIX. J.D.W. would like to thank Dr. Bhima Sastri (U.S. Department of Energy, HQ) for his help in organizing this research collaboration and follow-up of the project. NR 42 TC 0 Z9 0 U1 6 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 0921-8831 EI 1568-5527 J9 ADV POWDER TECHNOL JI Adv. Powder Technol. PD JUL PY 2016 VL 27 IS 4 BP 1453 EP 1463 DI 10.1016/j.apt.2016.05.005 PG 11 WC Engineering, Chemical SC Engineering GA DW0UB UT WOS:000383357200049 ER PT J AU Liu, TY Zhu, C Kou, TY Worsley, MA Qian, F Condes, C Duoss, EB Spadaccini, CM Li, Y AF Liu, Tianyu Zhu, Cheng Kou, Tianyi Worsley, Marcus A. Qian, Fang Condes, Cecilia Duoss, Eric B. Spadaccini, Christopher M. Li, Yat TI Ion Intercalation Induced Capacitance Improvement for Graphene-Based Supercapacitor Electrodes SO CHEMNANOMAT LA English DT Article DE capacitance; graphene-based electrodes; ion intercalation; supercapacitors ID ENERGY-STORAGE; ELECTROCHEMICAL CAPACITORS; ACTIVATED CARBON; GRAPHITE FOIL; EXFOLIATION; PERFORMANCE; SHEETS; OXIDE; COMPOSITES; FUNCTIONALIZATION AB Here we demonstrate a facile electrochemical method that can substantially improve the capacitance of graphene-based electrodes while still retaining their excellent rate capability. This method involves two ion-intercalation steps (lithium-ion intercalation and perchlorate-ion intercalation), followed by hydrolysis of perchlorate ion intercalation compounds. Lithium ion intercalation mainly leads to surface exfoliation, whilst the hydrolysis of perchlorate ion intercalation compounds functionalizes the graphene surface with oxygen moieties. Electrochemically treated graphitic paper electrode shows 1000 times enhancement in areal capacitance. Without the need of post-treatment annealing, the treated graphitic paper maintains an outstanding rate capability of 84% (0.5 mAcm(-2) to 5 mAcm(-2)). The same strategy can also be extended to boost the gravimetric capacitance of lightweight 3D printed graphene aerogels. The treated graphene aerogel achieved an outstanding gravimetric capacitance of 101.7 Fg(-1) (10 Ag-1) with an excellent rate capability of 81.6% (0.5 Ag-1 to 10 Ag-1). C1 [Liu, Tianyu; Kou, Tianyi; Condes, Cecilia; Li, Yat] Univ Calif Santa Cruz, Dept Chem & Biochem, 1156 High St, Santa Cruz, CA 95064 USA. [Zhu, Cheng; Duoss, Eric B.; Spadaccini, Christopher M.] Lawrence Livermore Natl Lab, Engn Directorate, 7000 East Ave, Livermore, CA 94550 USA. [Worsley, Marcus A.; Qian, Fang] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, 7000 East Ave, Livermore, CA 94550 USA. RP Li, Y (reprint author), Univ Calif Santa Cruz, Dept Chem & Biochem, 1156 High St, Santa Cruz, CA 95064 USA. EM yatli@ucsc.edu OI Li, Yat/0000-0002-8058-2084 FU Lawrence Livermore National Laboratory under U.S. Department of Energy [DE-AC52-07NA27344]; LDRD award [14-SI-004 (LLNL-JRNL-691106)] FX This work was supported by Lawrence Livermore National Laboratory under the auspices of the U.S. Department of Energy under Contract DE-AC52-07NA27344, through LDRD award 14-SI-004 (LLNL-JRNL-691106). We acknowledge Dr. Tom Yuzvinsky from University of California, Santa Cruz for SEM images acquisition and acknowledge the W. M. Keck Center for Nanoscale Opto-fluidics for use of the FEI Quanta 3D Dual-beam scanning electron microscope. The authors also thank Prof. Jin Z. Zhang, Mr. Jesse Hausser and Mr. Jorge Jimenez from University of California, Santa Cruz, for offering access to Renishaw Raman spectrometer, help in XRD characterization and assistance for FT-IR spectra acquisition, respectively. NR 42 TC 2 Z9 2 U1 33 U2 34 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY EI 2199-692X J9 CHEMNANOMAT JI ChemNanoMat PD JUL PY 2016 VL 2 IS 7 SI SI BP 635 EP 641 DI 10.1002/cnma.201600107 PG 7 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DW6PQ UT WOS:000383773800007 ER PT J AU Li, YC Fu, GY Watson, M Harrison, S Paranthaman, MP AF Li, Yunchao Fu, Guoyi Watson, Mark Harrison, Stephen Paranthaman, M. Parans TI Monodispersed Li4Ti5O12 with Controlled Morphology as High Power Lithium Ion Battery Anodes SO CHEMNANOMAT LA English DT Article DE high-rate anode; lithium-ion batteries (LIBs); safe batteries; solid electrolyte interface (SEI); spinel Li4Ti5O12 (LTO) ID TIO2 NANOTUBE ARRAYS; ELECTROCHEMICAL PROPERTIES; RECHARGEABLE LITHIUM; ENHANCED PERFORMANCE; SPINEL; CHALLENGES; MICROSPHERES; STORAGE AB Monodispersed Li4Ti5O12 (LTO) nanoparticles with controlled microstructure were successfully synthesized by a combination of hydrolysis and hydrothermal method followed by a post-annealing process. The scanning electron microscopy images showed that particles with a size of 30-50 nm were precisely controlled throughout the synthesis process. The electrochemical tests of the as-prepared LTO electrodes in a half-cell proved its high rate performance and outstanding cyclability which benefits from the preserved well-controlled nanoparticle size and morphology. LTO electrodes were also tested in a full cell configuration in pairing with LiFePO4 cathodes, which demonstrated a capacity of 147.3 mAhg(-1). In addition, we have also demonstrated that LTO materials prepared using lithium salts separated from geothermal brine solutions had good cyclability. These demonstrations provide a promising way for making low-cost, large-scale LTO electrode materials for energy storage applications. C1 [Li, Yunchao; Paranthaman, M. Parans] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Fu, Guoyi; Watson, Mark] Cristal USA Inc, Glen Burnie, MD 21060 USA. [Harrison, Stephen] Simbol Mat, Pleasanton, CA 94588 USA. [Li, Yunchao; Paranthaman, M. Parans] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN 37996 USA. [Harrison, Stephen] Rakehill Technol, Benicia, CA USA. RP Paranthaman, MP (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.; Paranthaman, MP (reprint author), Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN 37996 USA. EM paranthamanm@ornl.gov OI Paranthaman, Mariappan/0000-0003-3009-8531; Li, Yunchao/0000-0001-5460-5855 FU Materials Sciences and Engineering Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy; Critical Material Institute, an Energy Innovation Hub - U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office; U.S. Department of Energy [DE-AC05-00OR22725] FX Research was sponsored by the Materials Sciences and Engineering Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy. Battery evaluation using geothermal derived lithium salts was supported in part by the Critical Material Institute, an Energy Innovation Hub funded by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office. Notice: This Communication has been authored by UT-Battelle, LLC under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this Communication, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doepublic-access-plan). NR 32 TC 1 Z9 1 U1 17 U2 17 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY EI 2199-692X J9 CHEMNANOMAT JI ChemNanoMat PD JUL PY 2016 VL 2 IS 7 SI SI BP 642 EP 646 DI 10.1002/cnma.201600106 PG 5 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DW6PQ UT WOS:000383773800008 ER PT J AU Yoo, HD Li, YF Liang, YL Lan, YC Wang, F Yao, Y AF Yoo, Hyun Deog Li, Yifei Liang, Yanliang Lan, Yucheng Wang, Feng Yao, Yan TI Intercalation Pseudocapacitance of Exfoliated Molybdenum Disulfide for Ultrafast Energy Storage SO CHEMNANOMAT LA English DT Article DE energy storage; exfoliated structure; intercalation pseudocapacitance; molybdenum disulfide; supercapacitor ID MOS2 NANOSHEETS; SUPERCAPACITORS; NANOCOMPOSITES; BATTERIES; ELECTRODE; DENSITY; 1T AB We report intercalation pseudocapacitance of 250 Fg(-1) for exfoliated molybdenum disulfide (MoS2) in non-aqueous electrolytes that contain lithium ions. The exfoliated MoS2 shows surface-limited reaction kinetics with high rate capability up to 3 min of charge or discharge. The intercalation pseudocapacitance originates from the extremely fast kinetics due to the enhanced ionic and electronic transport enabled by the slightly expanded layer structure as well as the metallic 1T-phase. The exfoliated MoS2 could be also used in a Li-Mg-ion hybrid capacitor, which shows full cell specific capacitance of 240 Fg(-1). C1 [Yoo, Hyun Deog; Li, Yifei; Liang, Yanliang; Yao, Yan] Univ Houston, Dept Elect & Comp Engn, Houston, TX 77204 USA. [Yoo, Hyun Deog; Li, Yifei; Liang, Yanliang; Yao, Yan] Univ Houston, Mat Sci & Engn Program, Houston, TX 77204 USA. [Lan, Yucheng] Morgan State Univ, Dept Phys & Engn Phys, Baltimore, MD 21251 USA. [Wang, Feng] Brookhaven Natl Lab, Sustainable Energy Technol Dept, Upton, NY 11973 USA. [Yao, Yan] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. RP Yao, Y (reprint author), Univ Houston, Dept Elect & Comp Engn, Houston, TX 77204 USA.; Yao, Y (reprint author), Univ Houston, Mat Sci & Engn Program, Houston, TX 77204 USA.; Yao, Y (reprint author), Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. EM yyao4@uh.edu FU U.S. Office of Naval Research [N00014-13-1-0543] FX Y.Y. acknowledges funding support from the U.S. Office of Naval Research (No. N00014-13-1-0543). NR 26 TC 1 Z9 1 U1 34 U2 34 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY EI 2199-692X J9 CHEMNANOMAT JI ChemNanoMat PD JUL PY 2016 VL 2 IS 7 SI SI BP 688 EP 691 DI 10.1002/cnma.201600117 PG 4 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DW6PQ UT WOS:000383773800017 ER PT J AU Xing, ZY Luo, XY Qi, YT Stickle, WF Amine, K Lu, J Ji, XL AF Xing, Zhenyu Luo, Xiangyi Qi, Yitong Stickle, William F. Amine, Khalil Lu, Jun Ji, Xiulei TI Nitrogen-Doped Nanoporous Graphenic Carbon: An Efficient Conducting Support for O-2 Cathode SO CHEMNANOMAT LA English DT Article DE composite carbon; graphenic; Li-O-2 battery; nanoporous carbon; N-doping ID LITHIUM-OXYGEN BATTERIES; RECHARGEABLE LI-O-2 BATTERIES; AIR BATTERIES; SULFUR BATTERIES; CATALYSTS; PERFORMANCE; NANOTUBES; REDUCTION; NANOSHEETS; ELECTRODE AB Herein, we synthesize a nanoporous N-doped graphenic carbon with high surface area and a higher graphenization/graphitic degree by further developing the metallothermic reduction of gaseous CO2 by adding N-2 into the gas flow. The N-doped nanoporous carbon is composed of both a highly porous graphenic and nongraphitic matrix and homogeneously dispersed ordered graphitic nanodomains, which constitute a very unique composite carbon structure. The resulting N-doped graphenic carbon exhibits much more favorable reactivity as a carbon conducting support in the O-2 cathode of Li-O-2 batteries, increasing the specific capacity of the GC electrode from 5300 to 9600 mAhg(-1). The N-doped carbon also exhibits lower overpotentials during initial cycling for the charging process as well as an enhanced cycling performance compared to the undoped carbon. These results demonstrate that N-doping has a strong correlation with the enhanced performance of O-2 cathode of Li-O-2 batteries. C1 [Xing, Zhenyu; Qi, Yitong; Ji, Xiulei] Oregon State Univ, Dept Chem, Corvallis, OR 97331 USA. [Luo, Xiangyi; Amine, Khalil; Lu, Jun] Argonne Natl Lab, Lemont, IL 60439 USA. [Stickle, William F.] Hewlett Packard Corp, 1000 NE Circle Blvd, Corvallis, OR 97330 USA. RP Ji, XL (reprint author), Oregon State Univ, Dept Chem, Corvallis, OR 97331 USA.; Lu, J (reprint author), Argonne Natl Lab, Lemont, IL 60439 USA. EM junlu@anl.gov; david.ji@oregonstate.edu FU Oregon State University (OSU); U.S. Department of Energy from the Vehicle Technologies Office, Department of Energy, Office of Energy Efficiency and Renewable Energy (EERE) [DE-AC0206CH11357]; Advanced Photon Source; Electron Microscopy Center at Argonne National Laboratory FX This research was financially supported by the Oregon State University (OSU) and U.S. Department of Energy under Contract DE-AC0206CH11357 from the Vehicle Technologies Office, Department of Energy, Office of Energy Efficiency and Renewable Energy (EERE). We are thankful to Professor Chih-Hung Chang and Mr. Changqing Pan for Raman analysis. Also, we acknowledge grants of experiment time from the Advanced Photon Source and the Electron Microscopy Center at Argonne National Laboratory. NR 62 TC 0 Z9 0 U1 19 U2 19 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 2199-692X J9 CHEMNANOMAT JI ChemNanoMat PD JUL PY 2016 VL 2 IS 7 SI SI BP 692 EP 697 DI 10.1002/cnma.201600112 PG 6 WC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DW6PQ UT WOS:000383773800018 ER PT J AU Ivanov, AS Bryantsev, VS AF Ivanov, Alexander S. Bryantsev, Vyacheslav S. TI A Computational Approach to Predicting Ligand Selectivity for the Size-Based Separation of Trivalent Lanthanides SO EUROPEAN JOURNAL OF INORGANIC CHEMISTRY LA English DT Article DE Selectivity; Lanthanides; Size-based separation; Density functional calculations; Solvation effects ID DENSITY-FUNCTIONAL THEORY; MIXED CLUSTER/CONTINUUM MODELS; BASIS-SETS; DONOR LIGANDS; COMPLEXATION; EXTRACTION; SOLVATION; ENERGY; PSEUDOPOTENTIALS; SIMULATIONS AB Reprocessing of high-level waste is a key step in advancing sustainable energy systems. The development of efficient chelating agents for trivalent f-block metal ions is essential for increasing the efficiency of nuclear-waste remediation and extractive hydrometallurgy of rare-earth elements. Although computer-aided screening could lead to a more rapid discovery of superior ligands, an accurate theoretical description of the solvation effects for trivalent metal ions is currently a stumbling block in qualitative predictions for selectivity trends along the lanthanide series. In this work, we propose a robust model to describe the differential effect of solvation in the competitive binding of a ligand with lanthanides by including weakly coordinated counterions in the complexes of more than a +1 charge. The success of this approach in quantitatively reproducing aqueous selectivities demonstrates its potential for the design and screening of new ligands for efficient size-based separation. C1 [Ivanov, Alexander S.; Bryantsev, Vyacheslav S.] Oak Ridge Natl Lab, Div Chem Sci, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. RP Bryantsev, VS (reprint author), Oak Ridge Natl Lab, Div Chem Sci, 1 Bethel Valley Rd, Oak Ridge, TN 37831 USA. EM bryantsevv@ornl.gov FU Fuel Cycle Research and Development Program, Office of Nuclear Energy, U.S. Department of Energy; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported by the Fuel Cycle Research and Development Program, Office of Nuclear Energy, U.S. Department of Energy and used resources of the National Energy Research Scientific Computing Center, a DOE Office of Science User Facility supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 38 TC 1 Z9 1 U1 9 U2 9 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1434-1948 EI 1099-0682 J9 EUR J INORG CHEM JI Eur. J. Inorg. Chem. PD JUL PY 2016 IS 21 BP 3474 EP 3479 DI 10.1002/ejic.201600319 PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DW4IS UT WOS:000383607000017 ER PT J AU Young, EE Bryant, CD Lee, SE Peng, X Cook, B Nair, HK Dreher, KJ Zhang, X Palmer, AA Chung, JM Mogil, JS Chesler, EJ Lariviere, WR AF Young, E. E. Bryant, C. D. Lee, S. E. Peng, X. Cook, B. Nair, H. K. Dreher, K. J. Zhang, X. Palmer, A. A. Chung, J. M. Mogil, J. S. Chesler, E. J. Lariviere, W. R. TI Systems genetic and pharmacological analysis identifies candidate genes underlying mechanosensation in the von Frey test SO GENES BRAIN AND BEHAVIOR LA English DT Article DE Casein kinase 1; linkage mapping; microarray; quantitative trait locus; transcript abundance; voltage-gated calcium channels; von Frey ID PERIPHERAL NEUROPATHIC PAIN; DEPENDENT CALCIUM-CHANNELS; COMPLEX TRAIT ANALYSIS; KINASE-I FAMILY; NERVE INJURY; SPINAL-CORD; METHAMPHETAMINE SENSITIVITY; SYNAPTIC-TRANSMISSION; UP-REGULATION; MOUSE AB Mechanical sensitivity is commonly affected in chronic pain and other neurological disorders. To discover mechanisms of individual differences in punctate mechanosensation, we performed quantitative trait locus (QTL) mapping of the response to von Frey monofilament stimulation in BXD recombinant inbred (BXD) mice. Significant loci were detected on mouse chromosome (Chr) 5 and 15, indicating the location of underlying polymorphisms that cause heritable variation in von Frey response. Convergent evidence from public gene expression data implicates candidate genes within the loci: von Frey thresholds were strongly correlated with baseline expression of Cacna2d1, Ift27 and Csnk1e in multiple brain regions of BXD strains. Systemic gabapentin and PF-670462, which target the protein products of Cacna2d1 and Csnk1e, respectively, significantly increased von Frey thresholds in a genotype-dependent manner in progenitors and BXD strains. Real-time polymerase chain reaction confirmed differential expression of Cacna2d1 and Csnk1e in multiple brain regions in progenitors and showed differential expression of Cacna2d1 and Csnk1e in the dorsal root ganglia of the progenitors and BXD strains grouped by QTL genotype. Thus, linkage mapping, transcript covariance and pharmacological testing suggest that genetic variation affecting Cacna2d1 and Csnk1e may contribute to individual differences in von Frey filament response. This study implicates Cacna2d1 and Ift27 in basal mechanosensation in line with their previously suspected role in mechanical hypersensitivity. Csnk1e is implicated for von Frey response for the first time. Further investigation is warranted to identify the specific polymorphisms involved and assess the relevance of these findings to clinical conditions of disturbed mechanosensation. C1 [Young, E. E.; Peng, X.; Cook, B.; Nair, H. K.; Dreher, K. J.; Zhang, X.; Lariviere, W. R.] Univ Pittsburgh, Sch Med, Dept Anesthesiol, Pittsburgh, PA 15261 USA. [Young, E. E.] Univ Connecticut, Sch Nursing, 231 Glenbrook Rd,Unit 4026, Storrs, CT 06269 USA. [Young, E. E.] Univ Connecticut, Inst Syst Genom, 231 Glenbrook Rd,Unit 4026, Storrs, CT 06269 USA. [Bryant, C. D.] Boston Univ, Sch Med, Dept Pharmacol & Expt Therapeut, Boston, MA 02118 USA. [Bryant, C. D.] Boston Univ, Sch Med, Dept Psychiat, Boston, MA 02118 USA. [Lee, S. E.; Mogil, J. S.] Univ Texas Med Branch, Dept Neurosci & Cell Biol, Galveston, TX 77555 USA. [Palmer, A. A.] Univ Chicago, Dept Psychiat & Behav Neurosci, Chicago, IL 60637 USA. [Palmer, A. A.] Univ Chicago, Dept Human Genet, Chicago, IL 60637 USA. [Palmer, A. A.] Univ Calif San Diego, Dept Psychiat, La Jolla, CA 92093 USA. [Mogil, J. S.] McGill Univ, Dept Psychol, Montreal, PQ, Canada. [Mogil, J. S.] McGill Univ, Alan Edwards Ctr Res Pain, Montreal, PQ, Canada. [Chesler, E. J.] Oak Ridge Natl Lab, Mammalian Genet & Genom, Oak Ridge, TN USA. [Chesler, E. J.] Jackson Lab, 600 Main St, Bar Harbor, ME 04609 USA. RP Young, EE (reprint author), Univ Connecticut, Sch Nursing, 231 Glenbrook Rd,Unit 4026, Storrs, CT 06269 USA.; Young, EE (reprint author), Univ Connecticut, Inst Syst Genom, 231 Glenbrook Rd,Unit 4026, Storrs, CT 06269 USA. EM erin.young@uconn.edu FU Department of Anesthesiology of the University of Pittsburgh School of Medicine; University of Pittsburgh School of Health Sciences Bridge Funding; NIH [1R01DA021198, T32DA007255, 1F32DA026697, R01DA021336, 5R01NS031680, 2P01NS011255, R01DA15191, DA020677, R01AA18776]; Office of Biological and Environmental Research, Office of Science, U.S. Department of Energy [DE-AC05-00OR22725]; UT-Battelle, LLC FX Funding for this study was obtained from: the Department of Anesthesiology of the University of Pittsburgh School of Medicine, the University of Pittsburgh School of Health Sciences Bridge Funding (W.R.L.); NIH grants 1R01DA021198 (W.R.L); T32DA007255 and 1F32DA026697 (C.D.B); R01DA021336 (A.A.P.); 5R01NS031680 and 2P01NS011255 (J.M.C.); R01DA15191 (J.S.M.); DA020677 (E.J.C.), R01AA18776 (E.J.C.); and the Office of Biological and Environmental Research, Office of Science, U.S. Department of Energy, under Contract DE-AC05-00OR22725 with UT-Battelle, LLC (E.J.C.). We thank Pfizer Global R&D (Groton, CT, USA) for the generous gift of a portion of the PF-670462 used. NR 71 TC 0 Z9 0 U1 1 U2 1 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1601-1848 EI 1601-183X J9 GENES BRAIN BEHAV JI Genes Brain Behav. PD JUL PY 2016 VL 15 IS 6 BP 604 EP 615 DI 10.1111/gbb.12302 PG 12 WC Behavioral Sciences; Neurosciences SC Behavioral Sciences; Neurosciences & Neurology GA DW6QF UT WOS:000383775300007 PM 27231153 ER PT J AU Wu, H Ren, SP Garzoglio, G Timm, S Bernabeu, G Chadwick, K Noh, SY AF Wu, Hao Ren, Shangping Garzoglio, Gabriele Timm, Steven Bernabeu, Gerard Chadwick, Keith Noh, Seo-Young TI A Reference Model for Virtual Machine Launching Overhead SO IEEE TRANSACTIONS ON CLOUD COMPUTING LA English DT Article DE VM launching overhead; reference model; cloud; FermiCloud; virtual machine; vm launching; vm startup time; launch; overhead; model; predict ID CLOUD; FERMICLOUD AB Cloud bursting is one of the key research topics in the cloud computing communities. A well designed cloud bursting module enables private clouds to automatically launch virtual machines (VMs) to public clouds when more resources are needed. One of the main challenges in developing a cloud bursting module is to decide when and where to launch a VM so that all resources are most effectively and efficiently utilized and the system performance is optimized. However, based on system operational data obtained from FermiCloud, a private cloud developed by the Fermi National Accelerator Laboratory for scientific workflows, the VM launching overhead is not a constant. It varies with physical resource utilization, such as CPU and I/O device utilizations, at the time when a VM is launched. Hence, to make judicious decisions as to when and where a VM should be launched, a VM launching overhead reference model is needed. In this paper, we first develop a VM launching overhead reference model based on operational data we have obtained on FermiCloud. Second, we apply the developed reference model on FermiCloud and compare calculated VM launching overhead values based on the model with measured overhead values on FermiCloud. Our empirical results on FermiCloud indicate that the developed reference model is accurate. We believe, with the guidance of the developed reference model, efficient resource allocation algorithms can be developed for cloud bursting process to minimize the operational cost and resource waste. C1 [Wu, Hao; Ren, Shangping] IIT, Dept Comp Sci, 10 W 31st St,013, Chicago, IL 60616 USA. [Garzoglio, Gabriele; Timm, Steven; Bernabeu, Gerard; Chadwick, Keith] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Noh, Seo-Young] Korea Inst Sci & Technol Informat, Natl Inst Supercomp & Networking, Daejeon, South Korea. RP Wu, H (reprint author), IIT, Dept Comp Sci, 10 W 31st St,013, Chicago, IL 60616 USA. EM hwu28@iit.edu; ren@iit.edu; garzogli@fnal.gov; timm@fnal.gov; gerard1@fnal.gov; chadwick@fnal.gov; rsyoung@kisti.re.kr NR 17 TC 0 Z9 0 U1 0 U2 0 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2168-7161 J9 IEEE TRANS CLOUD COM JI IEEE Trans. Cloud Comput. PD JUL-SEP PY 2016 VL 4 IS 3 BP 250 EP 264 DI 10.1109/TCC.2014.2369439 PG 15 WC Computer Science, Software Engineering SC Computer Science GA DW9PK UT WOS:000383993600001 ER PT J AU Ogasawara, K Livi, SA Allegrini, F Broiles, TW Dayeh, MA Desai, MI Ebert, RW Llera, K Vines, SK McComas, DJ AF Ogasawara, K. Livi, S. A. Allegrini, F. Broiles, T. W. Dayeh, M. A. Desai, M. I. Ebert, R. W. Llera, K. Vines, S. K. McComas, D. J. TI Next-generation solid-state detectors for charged particle spectroscopy SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Review DE space plasma; solid state detector ID CVD-DIAMOND DETECTORS; SINGLE-CRYSTAL DIAMOND; HAMAMATSU AVALANCHE PHOTODIODE; ION COMPOSITION SPECTROMETER; LOW-ENERGY ELECTRONS; LIFT-OFF PROCESS; X-RAY-DETECTOR; LARGE-AREA; RADIATION HARDNESS; SILICON DETECTORS AB The performance of silicon avalanche photodiodes (APDs) and single crystal chemical vapor deposit diamond detectors (DDs) is reviewed in comparison with conventional silicon-based solid-state detectors (SSDs) from the perspective of space plasma applications. Although the low-energy threshold and the energy resolution are equivalent to SSDs, DDs offer a high radiation tolerance and very low leakage currents due to a wider band gap than silicon. In addition, DDs can operate at higher temperatures, are insensitive to light (>226nm), and are capable of timing analysis due to the higher intrinsic carrier mobility. APDs also offer several advantageous features. Specifically, APDs have a lower energy threshold (<0.9keV) and a higher energy resolution (<0.7keV full width at half maximum at room temperature), along with a linear response due to a strong electric field causing signal amplifications within the detector. Therefore, APDs can be used to detect lower energy particles, covering a larger portion of the energy spectrum than conventional SSDs. Further, the strong internal electric field gives them a subnanosecond response time by the charge mobility saturation, allowing them to make precise timing measurements of ions. These novel detector techniques can be potentially applied to improve the measurements of suprathermal particles, whose energies lie between typical ranges of conventional sensors for low-energy plasmas and energetic particles. Although the origin and evolution of the suprathermal particles are the key to understanding the acceleration and heating processes in space plasma, they are not well understood due to the technical difficulties of making the measurement. C1 [Ogasawara, K.; Livi, S. A.; Allegrini, F.; Broiles, T. W.; Dayeh, M. A.; Desai, M. I.; Ebert, R. W.; Llera, K.; Vines, S. K.; McComas, D. J.] Southwest Res Inst, San Antonio, TX 78238 USA. [Livi, S. A.; Allegrini, F.; Desai, M. I.; Llera, K.; Vines, S. K.; McComas, D. J.] Univ Texas San Antonio, San Antonio, TX USA. [McComas, D. J.] Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. RP Ogasawara, K (reprint author), Southwest Res Inst, San Antonio, TX 78238 USA. EM kogasawara@swri.org FU Southwest Research Institute's Internal Research and Development (IRD) programs; NASA [NNX12AE76G, NNX13AG17G, NNG13PR06C] FX The fundamental development of APDs and DDs in this study was supported by Southwest Research Institute's Internal Research and Development (IR&D) programs. The APD flight verification was performed as a part of Ground-to-Rocket Electrodynamics-Electrons Correlative Experiment (GREECE) mission in NASA program NNX12AE76G. Capabilities of SSD applications for suprathermal ion instruments were investigated through NASA grant NNX13AG17G. The APD development for a CubeSat based Compact Radiation bElt Explorer (CeREs) was supported by NASA grant NNG13PR06C. The data analyzed here are available upon request from authors. NR 127 TC 1 Z9 1 U1 6 U2 6 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6075 EP 6091 DI 10.1002/2016JA022559 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100006 ER PT J AU Sarno-Smith, LK Liemohn, MW Skoug, RM Larsen, BA Moldwin, MB Katus, RM Wygant, JR AF Sarno-Smith, Lois K. Liemohn, Michael W. Skoug, Ruth M. Larsen, Brian A. Moldwin, Mark B. Katus, Roxanne M. Wygant, John R. TI Local time variations of high-energy plasmaspheric ion pitch angle distributions SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE magnetosphere; plasmasphere; pitch angles; algorithm; spacecraft potential corrections ID VAN ALLEN PROBES; POLAR-CAP; PLASMAPAUSE; MAGNETOSPHERE; BOUNDARY; DAYSIDE; ORBIT; HISS AB Recent observations from the Van Allen Probes Helium Oxygen Proton Electron (HOPE) instrument revealed a persistent depletion in the 1-10eV ion population in the postmidnight sector during quiet times in the 2 < L < 3 region. This study explores the source of this ion depletion by developing an algorithm to classify 26 months of pitch angle distributions measured by the HOPE instrument. We correct the HOPE low energy fluxes for spacecraft potential using measurements from the Electric Field and Waves (EFW) instrument. A high percentage of low count pitch angle distributions is found in the postmidnight sector coupled with a low percentage of ion distributions peaked perpendicular to the field line. A peak in loss cone distributions in the dusk sector is also observed. These results characterize the nature of the dearth of the near 90 degrees pitch angle 1-10eV ion population in the near-Earth postmidnight sector. This study also shows, for the first time, low-energy HOPE differential number fluxes corrected for spacecraft potential and 1-10eV H+ fluxes at different levels of geomagnetic activity. C1 [Sarno-Smith, Lois K.; Liemohn, Michael W.; Moldwin, Mark B.] Univ Michigan, Dept Climate & Space Sci & Engn, Ann Arbor, MI 48109 USA. [Skoug, Ruth M.; Larsen, Brian A.] Los Alamos Natl Lab, Los Alamos, NM USA. [Katus, Roxanne M.] West Virginia Univ, Dept Phys, Morgantown, WV USA. [Wygant, John R.] Univ Minnesota, Dept Phys & Astron, Minneapolis, MN 55455 USA. RP Sarno-Smith, LK (reprint author), Univ Michigan, Dept Climate & Space Sci & Engn, Ann Arbor, MI 48109 USA. EM loisks@umich.edu OI Sarno-Smith, Lois/0000-0002-0964-7607 FU University of Michigan Rackham Graduate school; NASA; NSF [NWX11AO60G, NWX144AC02G, AGS-1265651, AGS-1102863]; U.S. Department of Energy; NASA Van Allen Probes mission; [LA-UR-15-29276] FX The Michigan co-authors would like to thank the University of Michigan Rackham Graduate school, NASA, and the NSF for sponsoring this work under grants NWX11AO60G, NWX144AC02G, AGS-1265651, and AGS-1102863. We would also like to thank Alex Shane and Kristie Llera for their contributions. Work at Los Alamos National Laboratory was performed under the auspices of the U.S. Department of Energy, with support from the NASA Van Allen Probes mission and LA-UR-15-29276. Data used to generate figures for this project came from the Van Allen Probes data center at . NR 29 TC 2 Z9 2 U1 0 U2 0 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6234 EP 6244 DI 10.1002/2015JA022301 PG 11 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100016 ER PT J AU Halford, AJ Fraser, BJ Morley, SK Elkington, SR Chan, AA AF Halford, A. J. Fraser, B. J. Morley, S. K. Elkington, S. R. Chan, A. A. TI Dependence of EMIC wave parameters during quiet, geomagnetic storm, and geomagnetic storm phase times SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE electromagnetic ion cyclotron waves; geomagnetic storms; wave parameters; CRRES satellite; ULF waves; geomagnetic index ID ION-CYCLOTRON WAVES; VAN ALLEN PROBES; MAGNETIC PULSATIONS; RELATIVISTIC ELECTRONS; GEOSYNCHRONOUS ORBIT; STATISTICAL-ANALYSIS; SYNCHRONOUS ORBIT; RADIATION-BELT; MAGNETOSPHERE; CRRES AB As electromagnetic ion cyclotron (EMIC) waves may play an important role in radiation belt dynamics, there has been a push to better include them into global simulations. How to best include EMIC wave effects is still an open question. Recently many studies have attempted to parameterize EMIC waves and their characteristics by geomagnetic indices. However, this does not fully take into account important physics related to the phase of a geomagnetic storm. In this paper we first consider how EMIC wave occurrence varies with the phase of a geomagnetic storm and the SYM-H, AE, and Kp indices. We show that the storm phase plays an important role in the occurrence probability of EMIC waves. The occurrence rates for a given value of a geomagnetic index change based on the geomagnetic condition. In this study we also describe the typical plasma and wave parameters observed in L and magnetic local time for quiet, storm, and storm phase. These results are given in a tabular format in the supporting information so that more accurate statistics of EMIC wave parameters can be incorporated into modeling efforts. C1 [Halford, A. J.] Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA. [Halford, A. J.] NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. [Fraser, B. J.] Univ Newcastle, Ctr Space Phys, Callaghan, NSW, Australia. [Morley, S. K.] Los Alamos Natl Lab, Space Sci & Applicat ISR 1, Los Alamos, NM USA. [Elkington, S. R.] Univ Colorado, LASP, Boulder, CO 80309 USA. [Chan, A. A.] Rice Univ, Dept Phys & Astron, Houston, TX USA. RP Halford, AJ (reprint author), Dartmouth Coll, Dept Phys & Astron, Hanover, NH 03755 USA.; Halford, AJ (reprint author), NASA, Goddard Space Flight Ctr, Greenbelt, MD 20771 USA. EM alexa.halford@gmail.com RI Morley, Steven/A-8321-2008 OI Morley, Steven/0000-0001-8520-0199 FU Australian Research Council [DP0772504, LX0882515]; University of Newcastle Postgraduate Research Scholarship; NASA [NNX15AF66G, NNX14ACO4G, NNX15AF59G, NNX15AI93G, NNX14AN55G]; U.S. Department of Energy Laboratory Directed Research and Development (LDRD) [20150127ER]; Japan Society for Promotion of Science (JSPS) [127008, 168069, 178061, 188071, 198053, 208041, 218046, 228040, 238033, 248032] FX This research was partly supported by Australian Research Council Project grant DP0772504 and Linkage International grant LX0882515. A.J. Halford was supported during her PhD by a University of Newcastle Postgraduate Research Scholarship and continued support by NASA under grant number NNX15AF66G. S.K.M. was supported by U.S. Department of Energy Laboratory Directed Research and Development (LDRD) award 20150127ER. S.E. was supported by NASA grant NNX14ACO4G and NNX15AF59G. A.A.C. was supported by NASA grant NNX15AI93G and NNX14AN55G. The SYM-H, Kp, and AE index were generated by the Kyoto data service whose construction of this database has been supported in part (as "Solar-Terrestrial Physics Database") by grants 127008, 168069, 178061, 188071, 198053, 208041, 218046, 228040, 238033, and 248032 under the Japan Society for Promotion of Science (JSPS) and can be found on the kyoto website http://wdc.kugi.kyoto-u.ac.jp/index.html. The event list used in this study is available on request from the corresponding author, A.J. Halford (alexa.j.halford@Dartmouth.edu). CRRES ephemeris and number density data are available on request from B.J. Fraser (brian.fraser@newcastle.edu.au). A.J.H. would like to thank Alex Glocer for useful discussions. NR 81 TC 3 Z9 3 U1 1 U2 1 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6277 EP 6291 DI 10.1002/2016JA022694 PG 15 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100019 ER PT J AU Colpitts, CA Cattell, CA Kozyra, JU Thomsen, MF Lavraud, B AF Colpitts, C. A. Cattell, C. A. Kozyra, J. U. Thomsen, M. F. Lavraud, B. TI Satellite observations of energy-banded ions during large geomagnetic storms: Event studies, statistics, and comparisons to source models SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE banded; ions; geomagnetic; storms; satellite ID SHEET BOUNDARY-LAYER; AURORAL RED ARCS; PLASMA SHEET; RING CURRENT; INNER MAGNETOSPHERE; MAGNETIC STORMS; DMSP SATELLITES; SOLAR FILAMENT; FEBRUARY 1986; MAIN PHASE AB Energy-banded ions from tens to ten thousands of eV are observed in the low-latitude auroral and subauroral zones during every large (minimum Dst<-150nT) geomagnetic storm encountered by the FAST satellite. The banded ions persist for many FAST orbits, lasting up to 12h, in both the northern and southern hemispheres. The energy-banded ions often have more than six distinct bands, and the O+, He+, and H+ bands are often observed at the same energies. The bands are extensive in latitude (similar to 50-75 degrees on the dayside, often extending to 45 degrees) and magnetic local time, covering all magnetic local time over the data set of storms. The distributions are peaked in the perpendicular direction at the altitudes of the FAST satellite (similar to 350-4175km), although in some cases the precipitating component dominates for the lowest energy bands. At the same time, for some of the events studied in detail, long-lasting intervals of field-aligned energy dispersed ions from similar to 100eV to 40keV are seen in Los Alamos National Laboratory geosynchronous observations, primarily on the dayside and after magnetosheath encounters (i.e., highly compressed magnetosphere). We present both case and statistical studies of the banded ions. These bands are a new phenomenon associated with all large storms, which are distinctly different from other banded populations, and are not readily interpreted using previous models for particle sources, transport, and loss. The energy-banded ions are an energetically important component of the inner magnetosphere during the most intense magnetic storms. C1 [Colpitts, C. A.; Cattell, C. A.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Kozyra, J. U.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Thomsen, M. F.] Los Alamos Natl Lab, Los Alamos, NM USA. [Lavraud, B.] Inst Rech Astrophys & Planetol, Toulouse, France. RP Colpitts, CA (reprint author), Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. EM chrisc@fields.space.umn.edu FU NASA [NNX07AG37G, NNX12AJ53G, NNX14AF32G]; Los Alamos National Laboratory FX The FAST data used for the figures in this paper are available at http://sprg.ssl.berkeley.edu/fast/scienceprod/welcome.html. The Kyoto Dst data are available at http://wdc.kugi.kyoto-u.ac.jp/dstdir/index.html. The ACE solar wind data are available at http://www.srl.caltech.edu/ACE/ASC/. LANL MPA color spectrograms are available at http://www.mpa.lanl.gov/cgi-bin/search.cgi. M.F.T. is grateful to Los Alamos National Laboratory for support as a guest scientist. This work was supported by NASA grants NNX07AG37G, NNX12AJ53G, and NNX14AF32G. NR 61 TC 0 Z9 0 U1 2 U2 2 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6353 EP 6377 DI 10.1002/2016JA022481 PG 25 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100024 ER PT J AU Su, ZP Gao, ZL Zhu, H Li, W Zheng, HN Wang, YM Wang, S Spence, HE Reeves, GD Baker, DN Blake, JB Funsten, HO Wygant, JR AF Su, Zhenpeng Gao, Zhonglei Zhu, Hui Li, Wen Zheng, Huinan Wang, Yuming Wang, Shui Spence, H. E. Reeves, G. D. Baker, D. N. Blake, J. B. Funsten, H. O. Wygant, J. R. TI Nonstorm time dropout of radiation belt electron fluxes on 24 September 2013 SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE radiation belt dropout; precipitation loss; numerical modeling; wave-particle interaction; plasmaspheric hiss; EMIC ID VAN ALLEN PROBES; RELATIVISTIC ELECTRONS; INNER MAGNETOSPHERE; GEOMAGNETIC STORMS; EMIC WAVES; MAGNETIC STORM; DIFFUSION-COEFFICIENTS; RESONANT SCATTERING; LOCAL TIME; ACCELERATION AB Radiation belt electron flux dropouts during the main phase of geomagnetic storms have received increasing attention in recent years. Here we focus on a rarely reported nonstorm time dropout event observed by Van Allen Probes on 24 September 2013. Within several hours, the radiation belt electron fluxes exhibited a significant (up to 2 orders of magnitude) depletion over a wide range of radial distances (L > 4.5), energies (approximate to 500keV to several MeV) and equatorial pitch angles (0 degrees(e)180 degrees). STEERB simulations show that the relativistic electron loss in the region L = 4.5-6.0 was primarily caused by the pitch angle scattering of observed plasmaspheric hiss and electromagnetic ion cyclotron waves. Our results emphasize the complexity of radiation belt dynamics and the importance of wave-driven precipitation loss even during nonstorm times. C1 [Su, Zhenpeng; Gao, Zhonglei; Zheng, Huinan; Wang, Yuming; Wang, Shui] Univ Sci & Technol China, Dept Geophys & Planetary Sci, CAS Key Lab Geospace Environm, Hefei, Peoples R China. [Su, Zhenpeng; Gao, Zhonglei; Zheng, Huinan] Univ Sci & Technol China, Collaborat Innovat Ctr Astronaut Sci & Technol, Hefei, Peoples R China. [Gao, Zhonglei] Univ Sci & Technol China, Sch Earth & Space Sci, Mengcheng Natl Geophys Observ, Hefei, Peoples R China. [Zhu, Hui] Univ Calif Los Angeles, Dept Earth Planetary & Space Sci, Los Angeles, CA USA. [Li, Wen] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA USA. [Spence, H. E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Reeves, G. D.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. [Reeves, G. D.] New Mexico Consortium, Space Sci Div, Los Alamos, NM USA. [Baker, D. N.] Univ Colorado, Atmospher & Space Phys Lab, Campus Box 392, Boulder, CO 80309 USA. [Blake, J. B.] Aerosp Corp, POB 92957, Los Angeles, CA 90009 USA. [Funsten, H. O.] Los Alamos Natl Lab, ISR Div, Los Alamos, NM USA. [Wygant, J. R.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. RP Su, ZP (reprint author), Univ Sci & Technol China, Dept Geophys & Planetary Sci, CAS Key Lab Geospace Environm, Hefei, Peoples R China.; Su, ZP (reprint author), Univ Sci & Technol China, Collaborat Innovat Ctr Astronaut Sci & Technol, Hefei, Peoples R China. EM szpe@mail.ustc.edu.cn RI Wang, Yuming/A-8968-2012; OI Wang, Yuming/0000-0002-8887-3919; Gao, Zhonglei/0000-0001-7397-930X; Su, Zhenpeng/0000-0001-5577-4538; Reeves, Geoffrey/0000-0002-7985-8098 FU National Natural Science Foundation of China [41422405, 41274169, 41274174, 41174125, 41131065, 41421063, 41231066, 41304134]; Chinese Academy of Sciences [KZCX2-EW-QN510, KZZD-EW-01-4]; National Key Basic Research Special Foundation of China [2011CB811403]; Fundamental Research Funds for the Central Universities [WK2080000077] FX We acknowledge the "Quantitative Assessment of Radiation Belt Modeling" focus group for motivating this study, acknowledge J. H. King, N. Papatashvilli, and CDAWeb for the use of interplanetary parameters and magnetospheric indices, and acknowledge the University of Iowa as the source for the EMFISIS data (this acknowledgment does not imply endorsement of the publication by the University of Iowa or its researchers), acknowledge V. Angelopoulos, J. W. Bonnell, F. S. Mozer, A. Roux, R. E. Ergun, U. Auster, K. H. Glassmeier, and W. Baumjohann for the use of THEMIS data. This work was supported by the National Natural Science Foundation of China grants 41422405, 41274169, 41274174, 41174125, 41131065, 41421063, 41231066, and 41304134, the Chinese Academy of Sciences grant KZCX2-EW-QN510 and KZZD-EW-01-4, the National Key Basic Research Special Foundation of China grant 2011CB811403, and the Fundamental Research Funds for the Central UniversitiesWK2080000077. Data are available at the following websites: http://cdaweb.gsfc.nasa.gov/cdaweb/istp_public/(geomagnetic activity indices, interplanetary parameters and THEMIS), http://emfisis.physics.uiowa.edu/Flight/(EMFISIS), http://www.rbsp-ect.lanl.gov/data_pub/(ECT), http://www.space.umn.edu/rbspefw-data/(EFW) and http://satdat.ngdc.noaa.gov/sem/poes/data/(POES). NR 95 TC 5 Z9 5 U1 8 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6400 EP 6416 DI 10.1002/2016JA022546 PG 17 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100026 ER PT J AU Xu, SS Liemohn, MW Dong, CF Mitchell, DL Bougher, SW Ma, YJ AF Xu, Shaosui Liemohn, Michael W. Dong, Chuanfei Mitchell, David L. Bougher, Stephen W. Ma, Yingjuan TI Pressure and ion composition boundaries at Mars SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE Mars; boundary; ion composition boundary; pressure boundary; magnetic pileup boundary; induced magnetosphere ID SOLAR-WIND INTERACTION; ELECTRON-IMPACT IONIZATION; MAGNETIC PILEUP BOUNDARY; 3-D HYBRID SIMULATION; UPPER-ATMOSPHERE; GLOBAL-SURVEYOR; UP BOUNDARY; PLASMA INTERACTION; FLUID SIMULATIONS; MAG/ER EXPERIMENT AB This study analyzes results from a multifluid MHD simulation to investigate the shape and structure of the pressure and composition boundaries at Mars, which can provide physical insight for the observational analysis. These boundaries are examined via the unity contours and gradients of the plasma , as well as , which includes the dynamic pressure in the numerator, and the ion mass and number density ratios. It is found that unity contours are well aligned with the gradient extrema, indicating that the unity contour is a topological boundary. In addition, these two transitions of pressure and composition are of a thickness of 0.05-0.1R(M) near the subsolar region to 1-1.5R(M) in the tail. The comparison of the pressure and composition boundaries indicates that the two are very similar and that not only the plasma sheet but also the full volume of the lobes are dominated by planetary ions. It suggests that the tail escape for ions not only concentrates in the central plasma sheet but also the magnetic lobes. It is also worthy pointing out that the ion number density ratio unity contour is found to be systematically smaller than other unity boundaries, which calls for attention when the ion number density is used to identify such boundaries. Finally, the comparison between the boundaries of this study and two analytical fittings is carried out. We found a good agreement with the Vignes fitting, with little flaring in the tail, in contrast to a larger flaring angle from the Trotignon fitting. C1 [Xu, Shaosui; Mitchell, David L.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Xu, Shaosui; Liemohn, Michael W.; Dong, Chuanfei; Bougher, Stephen W.] Univ Michigan, Dept Climate & Space Sci & Engn, Ann Arbor, MI 48109 USA. [Dong, Chuanfei] Princeton Univ, Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. [Ma, Yingjuan] Univ Calif Los Angeles, Inst Geophys & Planetary Phys, Los Angeles, CA 90024 USA. RP Xu, SS (reprint author), Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA.; Xu, SS (reprint author), Univ Michigan, Dept Climate & Space Sci & Engn, Ann Arbor, MI 48109 USA. EM shaosui.xu@ssl.berkeley.edu RI Dong, Chuanfei/E-6485-2010; Ma, Yingjuan/B-4895-2017 OI Dong, Chuanfei/0000-0002-8990-094X; Ma, Yingjuan/0000-0003-2584-7091 FU NASA [NNX13AG26G, NNS14AH19G]; NASA Mars Scout Program FX The authors would like to thank NASA for support of this project under grants NNX13AG26G and NNS14AH19G. The authors also thank support from the NASA Mars Scout Program. The authors thank Zhenguang Huang and Judit Szente for teaching S. Xu Tecplot, which makes this study possible. The BATS-R-US code is publicly available from http://csem.engin.umich.edu/tools/swmf. For distribution of the model results used in this study, please contact C. Dong (dcfy@pppl.gov). NR 54 TC 0 Z9 0 U1 4 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6417 EP 6429 DI 10.1002/2016JA022644 PG 13 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100027 ER PT J AU Yue, C Li, W Nishimura, Y Zong, QG Ma, QL Bortnik, J Thorne, RM Reeves, GD Spence, HE Kletzing, CA Wygant, JR Nicolls, MJ AF Yue, Chao Li, Wen Nishimura, Yukitoshi Zong, Qiugang Ma, Qianli Bortnik, Jacob Thorne, Richard M. Reeves, Geoffrey D. Spence, Harlan E. Kletzing, Craig A. Wygant, John R. Nicolls, Michael J. TI Rapid enhancement of low-energy (< 100eV) ion flux in response to interplanetary shocks based on two Van Allen Probes case studies: Implications for source regions and heating mechanisms SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE enhancement of low-energy ion flux; response to IP shocks; adiabatic accelerations; ionospheric ion outflows ID DAWN-DUSK ASYMMETRY; INNER MAGNETOSPHERE; GEOSYNCHRONOUS ORBIT; IMAGER OBSERVATIONS; CYCLOTRON WAVES; MAGNETIC-FIELD; SUBSTORMS; WIND; ENERGIZATION; LOCATION AB Interactions between interplanetary (IP) shocks and the Earth's magnetosphere manifest many important space physics phenomena including low-energy ion flux enhancements and particle acceleration. In order to investigate the mechanisms driving shock-induced enhancement of low-energy ion flux, we have examined two IP shock events that occurred when the Van Allen Probes were located near the equator while ionospheric and ground observations were available around the spacecraft footprints. We have found that, associated with the shock arrival, electromagnetic fields intensified, and low-energy ion fluxes, including H+, He+, and O+, were enhanced dramatically in both the parallel and perpendicular directions. During the 2 October 2013 shock event, both parallel and perpendicular flux enhancements lasted more than 20min with larger fluxes observed in the perpendicular direction. In contrast, for the 15 March 2013 shock event, the low-energy perpendicular ion fluxes increased only in the first 5min during an impulse of electric field, while the parallel flux enhancement lasted more than 30min. In addition, ionospheric outflows were observed after shock arrivals. From a simple particle motion calculation, we found that the rapid response of low-energy ions is due to drifts of plasmaspheric population by the enhanced electric field. However, the fast acceleration in the perpendicular direction cannot solely be explained by ExB drift but betatron acceleration also plays a role. Adiabatic acceleration may also explain the fast response of the enhanced parallel ion fluxes, while ion outflows may contribute to the enhanced parallel fluxes that last longer than the perpendicular fluxes. C1 [Yue, Chao; Li, Wen; Nishimura, Yukitoshi; Ma, Qianli; Bortnik, Jacob; Thorne, Richard M.] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90095 USA. [Yue, Chao] Univ Corp Atmospheric Res, Boulder, CO 80301 USA. [Zong, Qiugang] Peking Univ, Inst Space Phys & Appl Technol, Beijing, Peoples R China. [Reeves, Geoffrey D.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. [Reeves, Geoffrey D.] New Mexico Consortium, Space Sci Div, Los Alamos, NM USA. [Spence, Harlan E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Kletzing, Craig A.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Wygant, John R.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Nicolls, Michael J.] SRI Int, 333 Ravenswood Ave, Menlo Pk, CA 94025 USA. RP Yue, C (reprint author), Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90095 USA.; Yue, C (reprint author), Univ Corp Atmospheric Res, Boulder, CO 80301 USA. EM yuechao@atmos.ucla.edu RI Yue, Chao/C-2535-2015; OI Yue, Chao/0000-0001-9720-5210; Ma, Qianli/0000-0001-5452-4756; Reeves, Geoffrey/0000-0002-7985-8098 FU NASA Living With a Star Jack Eddy Postdoctoral Fellowship Program; NASA [NNX15AI62G, NNX13AI61G, NNX14AI18G, NAS5-01072]; NSF [PLR-1341359, AGS-1405054, 1564510]; AFOSR [FA9550-15-1-0179] FX This work was supported by the NASA Living With a Star Jack Eddy Postdoctoral Fellowship Program, administered by the UCAR Visiting Scientist Programs, NASA grants NNX15AI62G, NNX13AI61G, and NNX14AI18G, NSF grants PLR-1341359, AGS-1405054, and 1564510, and AFOSR grant FA9550-15-1-0179. We acknowledge use of Van Allen Probes data, made publicly available through NASA prime contract number NAS5-01072, including the Level 3 HOPE flux data obtained from the RBSP-ECT website (www.rbsp-ect.lanl.gov/data_pub/rbspb/hope/level3/PA/), the Level 3 magnetic field data obtained from the RBSP EMFISIS website (emfisis.physics.uiowa.edu/Flight/RBSP-B/L3), and the Level 3 electric field data were obtained from the RBSP EFW website (rbsp.space.umn.edu/data/rbsp/rbspb/l3/). We thank the Space Physics Data Facility at the NASA Goddard Space Flight Center for providing the OMNI data (ftp://spdf.gsfc.nasa.gov/pub/data/omni/omni_cdaweb/) and the Applied Physics Laboratory at the Johns Hopkins University and the William B. Hanson Center for Space Sciences at the University of Texas at Dallas for DMSP data. Contact the authors to access the PFISR and DMSP data. NR 46 TC 0 Z9 0 U1 5 U2 5 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6430 EP 6443 DI 10.1002/2016JA022808 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100028 ER PT J AU Allen, RC Zhang, JC Kistler, LM Spence, HE Lin, RL Klecker, B Dunlop, MW Andre, M Jordanova, VK AF Allen, R. C. Zhang, J. -C. Kistler, L. M. Spence, H. E. Lin, R. -L. Klecker, B. Dunlop, M. W. Andre, M. Jordanova, V. K. TI A statistical study of EMIC waves observed by Cluster: 2. Associated plasma conditions SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE EMIC waves; magnetosphere; Cluster; Shabansky orbits ID ION-CYCLOTRON WAVES; VAN ALLEN PROBES; 1-2 MAGNETIC PULSATIONS; DAWN-DUSK ASYMMETRY; STORM MAIN PHASE; RING CURRENT; GEOSYNCHRONOUS ORBIT; CLUSTER/WHISPER OBSERVATIONS; EQUATORIAL MAGNETOSPHERE; GLOBAL CHARACTERISTICS AB This is the second in a pair of papers discussing a statistical study of electromagnetic ion cyclotron (EMIC) waves detected during 10years (2001-2010) of Cluster observations. In the first paper, an analysis of EMIC wave properties (i.e., wave power, polarization, normal angle, and wave propagation angle) is presented in both the magnetic latitude (MLAT)-distance as well as magnetic local time (MLT)-L frames. This paper focuses on the distribution of EMIC wave-associated plasma conditions as well as two EMIC wave generation proxies (the electron plasma frequency to gyrofrequency ratio proxy and the linear theory proxy) in these same frames. Based on the distributions of hot H+ anisotropy, electron and hot H+ density measurements, hot H+ parallel plasma beta, and the calculated wave generation proxies, three source regions of EMIC waves appear to exist: (1) the well-known overlap between cold plasmaspheric or plume populations with hot anisotropic ring current populations in the postnoon to dusk MLT region; (2) regions all along the dayside magnetosphere at high L shells related to dayside magnetospheric compression and drift shell splitting; and (3) off-equator regions possibly associated with the Shabansky orbits in the dayside magnetosphere. C1 [Allen, R. C.; Zhang, J. -C.; Kistler, L. M.; Spence, H. E.] Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA. [Allen, R. C.; Zhang, J. -C.; Kistler, L. M.; Spence, H. E.] Univ New Hampshire, Dept Phys, Durham, NH 03824 USA. [Allen, R. C.] Southwest Res Inst, Space Sci & Engn Div, San Antonio, TX 78238 USA. [Allen, R. C.] Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. [Lin, R. -L.] Chinese Acad Sci, Natl Space Sci Ctr, Beijing, Peoples R China. [Klecker, B.] Max Planck Inst Extraterr Phys, Garching, Germany. [Dunlop, M. W.] Rutherford Appleton Lab, SSTD, Div Space Sci, Didcot, Oxon, England. [Andre, M.] Swedish Inst Space Phys IRF, Uppsala, Sweden. [Jordanova, V. K.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Allen, RC (reprint author), Univ New Hampshire, Ctr Space Sci, Durham, NH 03824 USA.; Allen, RC (reprint author), Univ New Hampshire, Dept Phys, Durham, NH 03824 USA.; Allen, RC (reprint author), Southwest Res Inst, Space Sci & Engn Div, San Antonio, TX 78238 USA.; Allen, RC (reprint author), Univ Texas San Antonio, Dept Phys & Astron, San Antonio, TX 78249 USA. EM robert.allen@swri.edu RI Allen, Robert/F-5187-2011; OI Allen, Robert/0000-0003-2079-5683; Jordanova, Vania/0000-0003-0475-8743 FU NASA at UNH [NNX11AO82G, NNX15AF66G, NNX11AB65G]; RBSP-ECT - JHU/APL under NASA's Prime [967399, NAS5-01072] FX NASA supported work at UNH under grants NNX11AO82G, NNX15AF66G, and NNX11AB65G. This work was also supported by RBSP-ECT funding provided by JHU/APL contract 967399 under NASA's Prime contract NAS5-01072. The authors thank the Cluster team for their data and software. C. Torrence and G. Compo at University of Colorado and the THEMIS Science Support Team supplied IDL routines. N. A. Tsyganenko of University of St. Petersburg in the Russian Federation and H. Korth of JHU/APL provided the Tsyganenko magnetic field model and the IDL/Geopack module. Solar wind plasma and IMF data, Dst, and Kp indices were obtained from the GSFC/SPDF OMNIWeb interface at URL: http://omniweb.gsfc.nasa.gov. The authors would also like to thank the Cluster instrument teams (FGM and CODIF) along with the Cluster Science Archive at URL http://www.cosmos.esa.int/web/csa. Finally, we would like to thank UCLA for the website on statistical analysis methods at URL http://statistics.ats.ucla.edu/stat/mult_pkg/whatstat/. The first author would also like to thank S.K. Vines for the valuable discussion and sanity checks. NR 89 TC 3 Z9 3 U1 0 U2 0 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6458 EP 6479 DI 10.1002/2016JA022541 PG 22 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100030 ER PT J AU Liang, J Lin, Y Johnson, JR Wang, XY Wang, ZX AF Liang, Ji Lin, Yu Johnson, Jay R. Wang, Xueyi Wang, Zheng-Xiong TI Kinetic Alfven waves in three-dimensional magnetic reconnection SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE magnetic reconnection; Alfven waves; kinetic Alfven waves; hybrid simulation; magnetotail; guide field ID 2-DIMENSIONAL HYBRID SIMULATION; FIELD-ALIGNED CURRENTS; SHEET BOUNDARY-LAYER; MAGNETOTAIL RECONNECTION; DAYSIDE MAGNETOPAUSE; PATCHY RECONNECTION; PLASMA; GENERATION; TAIL; MECHANISM AB Alfvenic waves are believed to be fundamentally important in magnetic reconnection. Kinetic dynamics of particles can break the Alfven speed limit in the evolution and propagation of perturbations during reconnection. In this paper, the generation and signatures of kinetic Alfven waves (KAWs) associated with magnetic reconnection in a current sheet is investigated using a three-dimensional (3-D) hybrid code under a zero or finite guide field. In order to understand the wave structures in the general cases of multiple X line reconnection, cases with a single X line of various lengths are examined. The KAWs are identified using the wave dispersion relation, electromagnetic polarization relations, as well as spectral analysis. In the cases in which the X line is so long to extend through the entire simulation domain in the current direction, quasi 2-D configurations of reconnection are developed behind a leading flux/plasma bulge. KAWs with perpendicular wave number k(i)approximate to 1 (with (i) being the ion Larmor radius) are found throughout the transient plasma bulge region and propagate outward along magnetic field lines with a slightly super-Alfvenic velocity. These KAWs are generated from the X line and coexist with the whistler structure of the ion diffusion region under a small guide field. In the cases in which the X line has a finite length 2 approximate to 10d(i), with being the half length of the X line and d(i) the ion inertial length, the KAWs originated from the X line are of 3-D nature. Under a finite guide field, KAWs propagate along the oblique magnetic field lines into the unperturbed regions in the current direction, carrying parallel electric field and Poynting fluxes. The critical X line length for the generation of 3-D-like structures is found to be 2(c)30d(i). The structure, propagation, energy, spectrum, and damping of the KAWs are examined. Dependence of the structure of KAWs on the guide field is also investigated. C1 [Liang, Ji; Wang, Zheng-Xiong] Dalian Univ Technol, Sch Phys & Optoelect Technol, Key Lab Mat Modificat Beams, Minist Educ, Dalian, Peoples R China. [Liang, Ji; Lin, Yu; Wang, Xueyi] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Johnson, Jay R.] Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. RP Wang, ZX (reprint author), Dalian Univ Technol, Sch Phys & Optoelect Technol, Key Lab Mat Modificat Beams, Minist Educ, Dalian, Peoples R China.; Lin, Y (reprint author), Auburn Univ, Dept Phys, Auburn, AL 36849 USA. EM ylin@physics.auburn.edu; zxwang@dlut.edu.cn FU Fundamental Research Funds for the Central Universities [DUT15YQ103, 3132014328]; DoE [DE-SC0010486]; NSF [AGS 1405225]; China Scholarship Council (CSC) FX This work was supported by the Fundamental Research Funds for the Central Universities (DUT15YQ103 and 3132014328) and the DoE grant DE-SC0010486 and NSF grant AGS 1405225 to Auburn University. The support provided by China Scholarship Council (CSC) during a visit of Ji Liang to Auburn University is acknowledged. Computer resources were provided by the Alabama Supercomputer Center and the cluster for plasma major of Peking University. The authors thank Xiang Lv for his help and discussions on the simulation code and model. The authors declare that there are no conflicts of interest regarding the publication of this paper. The data can be obtained by contacting the authors through email (jiliang@mail.dlut.edu.cn). NR 64 TC 1 Z9 1 U1 1 U2 1 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6526 EP 6548 DI 10.1002/2016JA022505 PG 23 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100034 ER PT J AU Skoug, RM Funsten, HO Mobius, E Harper, RW Kihara, KH Bower, JS AF Skoug, R. M. Funsten, H. O. Mobius, E. Harper, R. W. Kihara, K. H. Bower, J. S. TI A wide field of view plasma spectrometer SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE plasma spectrometer; pinhole camera; energy-angle filter ID MICROCHANNEL PLATE DETECTORS; ENERGETIC PARTICLE; SOLAR-WIND; ELECTROSTATIC ANALYZER; SPACE; RECONNECTION; PERFORMANCE; TURBULENCE; SATELLITE; EXPLORER AB We present a fundamentally new type of space plasma spectrometer, the wide field of view plasma spectrometer, whose field of view is >1.25 ster using fewer resources than traditional methods. The enabling component is analogous to a pinhole camera with an electrostatic energy-angle filter at the image plane. Particle energy-per-charge is selected with a tunable bias voltage applied to the filter plate relative to the pinhole aperture plate. For a given bias voltage, charged particles from different directions are focused by different angles to different locations. Particles with appropriate locations and angles can transit the filter plate and are measured using a microchannel plate detector with a position-sensitive anode. Full energy and angle coverage are obtained using a single high-voltage power supply, resulting in considerable resource savings and allowing measurements at fast timescales. We present laboratory prototype measurements and simulations demonstrating the instrument concept and discuss optimizations of the instrument design for application to space measurements. C1 [Skoug, R. M.; Funsten, H. O.; Harper, R. W.; Kihara, K. H.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Mobius, E.; Bower, J. S.] Univ New Hampshire, Durham, NH 03824 USA. RP Skoug, RM (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM rskoug@lanl.gov FU U.S. Department of Energy; LANL Laboratory Directed Research and Development program [20130564ER] FX Work at Los Alamos was performed under the auspices of the U.S. Department of Energy. Data including prototype measurements and simulation results are presented in the figures. This work was supported by the LANL Laboratory Directed Research and Development program, 20130564ER. NR 42 TC 1 Z9 1 U1 3 U2 3 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6590 EP 6601 DI 10.1002/2016JA022581 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100038 ER PT J AU Zhang, XJ Li, W Ma, Q Thorne, RM Angelopoulos, V Bortnik, J Chen, L Kletzing, CA Kurth, WS Hospodarsky, GB Baker, DN Reeves, GD Spence, HE Blake, JB Fennell, JF AF Zhang, X-J. Li, W. Ma, Q. Thorne, R. M. Angelopoulos, V. Bortnik, J. Chen, L. Kletzing, C. A. Kurth, W. S. Hospodarsky, G. B. Baker, D. N. Reeves, G. D. Spence, H. E. Blake, J. B. Fennell, J. F. TI Direct evidence for EMIC wave scattering of relativistic electrons in space SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE EMIC waves; relativistic electron loss; wave-particle interaction; Fokker-Planck equation; electron precipitation; equatorial pitch angle distribution ID RADIATION BELT ELECTRONS; GEOMAGNETIC STORMS; ELECTROMAGNETIC-WAVES; PRECIPITATION; LOSSES; MAGNETOSPHERE; ENERGIZATION; MAGNETOMETER; SIMULATION; TRANSPORT AB Electromagnetic ion cyclotron (EMIC) waves have been proposed to cause efficient losses of highly relativistic (>1MeV) electrons via gyroresonant interactions. Simultaneous observations of EMIC waves and equatorial electron pitch angle distributions, which can be used to directly quantify the EMIC wave scattering effect, are still very limited, however. In the present study, we evaluate the effect of EMIC waves on pitch angle scattering of ultrarelativistic (>1MeV) electrons during the main phase of a geomagnetic storm, when intense EMIC wave activity was observed in situ (in the plasma plume region with high plasma density) on both Van Allen Probes. EMIC waves captured by Time History of Events and Macroscale Interactions during Substorms (THEMIS) probes and on the ground across the Canadian Array for Real-time Investigations of Magnetic Activity (CARISMA) are also used to infer their magnetic local time (MLT) coverage. From the observed EMIC wave spectra and local plasma parameters, we compute wave diffusion rates and model the evolution of electron pitch angle distributions. By comparing model results with local observations of pitch angle distributions, we show direct, quantitative evidence of EMIC wave-driven relativistic electron losses in the Earth's outer radiation belt. C1 [Zhang, X-J.; Li, W.; Ma, Q.; Thorne, R. M.; Bortnik, J.] Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90095 USA. [Zhang, X-J.; Angelopoulos, V.] Univ Calif Los Angeles, Dept Earth Planetary & Space Sci, Los Angeles, CA 90095 USA. [Zhang, X-J.; Angelopoulos, V.] Univ Calif Los Angeles, Inst Geophys & Space Phys, Los Angeles, CA 90095 USA. [Chen, L.] Univ Texas Dallas, Dept Phys, Richardson, TX 75083 USA. [Kletzing, C. A.; Kurth, W. S.; Hospodarsky, G. B.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Baker, D. N.] Univ Colorado, Atmospher & Space Phys Lab, Campus Box 392, Boulder, CO 80309 USA. [Reeves, G. D.] Los Alamos Natl Lab, Space Sci & Applicat Grp, Los Alamos, NM USA. [Reeves, G. D.] New Mexico Consortium, Div Space Sci, Los Alamos, NM USA. [Spence, H. E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Blake, J. B.; Fennell, J. F.] Aerosp Corp, POB 92957, Los Angeles, CA 90009 USA. RP Zhang, XJ (reprint author), Univ Calif Los Angeles, Dept Atmospher & Ocean Sci, Los Angeles, CA 90095 USA.; Zhang, XJ (reprint author), Univ Calif Los Angeles, Dept Earth Planetary & Space Sci, Los Angeles, CA 90095 USA.; Zhang, XJ (reprint author), Univ Calif Los Angeles, Inst Geophys & Space Phys, Los Angeles, CA 90095 USA. EM xjzhang@ucla.edu OI Ma, Qianli/0000-0001-5452-4756 FU JHU/APL under NASA [967399, 921647, NAS5-01072]; AFOSR [FA9550-15-1-0158]; NASA [NNX15AI96G, NNX15AF61G, NNX11AR64G, NNX13AI61G, NNX14AI18G, NNX15AF55G]; NSF [AGS 1564510] FX This work was supported by RBSP-ECT and EMFISIS funding provided by JHU/APL contracts 967399 and 921647 under NASA's prime contract NAS5-01072. The analysis at UCLA was supported by AFOSR award FA9550-15-1-0158; NASA grants NNX15AI96G, NNX15AF61G, NNX11AR64G, NNX13AI61G, and NNX14AI18G; and the NSF grant AGS 1564510. L. Chen acknowledges the support of NASA grant NNX15AF55G. We are thankful to Van Allen Probes and THEMIS, POES, and CARISMA (Canadian Array for Realtime Investigations of Magnetic Activity) for the online data access and data analysis tools. Specifically, we acknowledge the Van Allen Probes EMFISIS data obtained from https://emfisis.physics.uiowa.edu/data/index, REPT and MagEIS data obtained from http://www.rbsp-ect.lanl.gov/data_pub/, THEMIS wave data obtained from http://themis.ssl.berkeley.edu/themisdata/, and the NOAA POES data obtained from http://satdat.ngdc.noaa.gov/sem/poes/data/. The authors thank I.R. Mann, D.K. Milling, and the rest of the CARISMA team for the CARISMA data obtained from http://data.carisma.ca. CARISMA is operated by the University of Alberta, funded by the Canadian Space Agency. We also thank the World Data Center for Geomagnetism, Kyoto, for providing the AU and AL indices and the Space Physics Data Facility at the NASA Goddard Space Flight Center for providing the OMNI data used in this study. NR 48 TC 2 Z9 2 U1 3 U2 3 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6620 EP 6631 DI 10.1002/2016JA022521 PG 12 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100040 ER PT J AU Baker, DN Jaynes, AN Kanekal, SG Foster, JC Erickson, PJ Fennell, JF Blake, JB Zhao, H Li, X Elkington, SR Henderson, MG Reeves, GD Spence, HE Kletzing, CA Wygant, JR AF Baker, D. N. Jaynes, A. N. Kanekal, S. G. Foster, J. C. Erickson, P. J. Fennell, J. F. Blake, J. B. Zhao, H. Li, X. Elkington, S. R. Henderson, M. G. Reeves, G. D. Spence, H. E. Kletzing, C. A. Wygant, J. R. TI Highly relativistic radiation belt electron acceleration, transport, and loss: Large solar storm events of March and June 2015 SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE radiation belts; magnetosphere; electron acceleration ID ALLEN PROBES OBSERVATIONS; ULTRARELATIVISTIC ELECTRONS; PROMPT ENERGIZATION; DIFFUSION; PROTONS; RING AB Two of the largest geomagnetic storms of the last decade were witnessed in 2015. On 17 March 2015, a coronal mass ejection-driven event occurred with a Dst (storm time ring current index) value reaching -223nT. On 22 June 2015 another strong storm (Dst reaching -204nT) was recorded. These two storms each produced almost total loss of radiation belt high-energy (E1MeV) electron fluxes. Following the dropouts of radiation belt fluxes there were complex and rather remarkable recoveries of the electrons extending up to nearly 10MeV in kinetic energy. The energized outer zone electrons showed a rich variety of pitch angle features including strong butterfly distributions with deep minima in flux at =90 degrees. However, despite strong driving of outer zone earthward radial diffusion in these storms, the previously reported impenetrable barrier at L approximate to 2.8 was pushed inward, but not significantly breached, and no E2.0MeV electrons were seen to pass through the radiation belt slot region to reach the inner Van Allen zone. Overall, these intense storms show a wealth of novel features of acceleration, transport, and loss that are demonstrated in the present detailed analysis. C1 [Baker, D. N.; Jaynes, A. N.; Zhao, H.; Li, X.; Elkington, S. R.] Univ Colorado Boulder, Lab Atmospher & Space Phys, Boulder, CO 80309 USA. [Kanekal, S. G.] NASA, Goddard Space Flight Ctr, Greenbelt, MD USA. [Foster, J. C.; Erickson, P. J.] MIT, Haystack Observ, Westford, MA 01886 USA. [Fennell, J. F.; Blake, J. B.] Aerosp Corp, POB 92957, Los Angeles, CA 90009 USA. [Henderson, M. G.; Reeves, G. D.] Los Alamos Natl Lab, Los Alamos, NM USA. [Spence, H. E.] Univ New Hampshire, Inst Study Earth Oceans & Space, Durham, NH 03824 USA. [Kletzing, C. A.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Wygant, J. R.] Univ Minnesota, Dept Phys & Astron, Minneapolis, MN 55455 USA. RP Baker, DN (reprint author), Univ Colorado Boulder, Lab Atmospher & Space Phys, Boulder, CO 80309 USA. EM Daniel.Baker@LASP.colorado.edu RI Henderson, Michael/A-3948-2011 OI Henderson, Michael/0000-0003-4975-9029 FU RBSP-ECT funding through JHU/APL [967399, NAS5-01072] FX The research presented here was supported by RBSP-ECT funding through JHU/APL contract 967399 (under prime NASA contract NAS5-01072). All data used in this paper are currently available via CDAweb (http://cdaweb.gsfc.nasa.gov/) or through the individual Van Allen Probes instrument suite web pages, with the exception of background-corrected REPT data which are available directly from the REPT team. NR 32 TC 5 Z9 5 U1 3 U2 3 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6647 EP 6660 DI 10.1002/2016JA022502 PG 14 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100043 PM 27867796 ER PT J AU Yuan, ZG Yu, XD Wang, DD Huang, SY Li, HM Yu, T Qiao, Z Wygant, JR Funsten, HO AF Yuan, Zhigang Yu, Xiongdong Wang, Dedong Huang, Shiyong Li, Haimeng Yu, Tao Qiao, Zheng Wygant, John R. Funsten, Herbert O. TI In situ evidence of the modification of the parallel propagation of EMIC waves by heated He+ ions SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE EMIC waves; He+ ion heating; stop band; Van Allen Probes; ring current ions ID CYCLOTRON WAVES; RADIATION BELT; RING CURRENT; ELECTROMAGNETIC-WAVES; PLASMASPHERIC PLUME; LOW-FREQUENCY; PLASMAPAUSE; MAGNETOSPHERE; GENERATION; DISPERSION AB With observations of the Van Allen Probe B, we report in situ evidence of the modification of the parallel propagating electromagnetic ion cyclotron (EMIC) waves by heated He+ ions. In the outer boundary of the plasmasphere, accompanied with the He+ ion heating, the frequency bands of H+ and He+ for EMIC waves merged into each other, leading to the disappearance of a usual stop band between the gyrofrequency of He+ ions ((He+)) and the H+ cutoff frequency ((H+co)) in the cold plasma. Moreover, the dispersion relation for EMIC waves theoretically calculated with the observed plasma parameters also demonstrates that EMIC waves can indeed parallel propagate across (He+). Therefore, the paper provides an in situ evidence of the modification of the parallel propagation of EMIC waves by heated He+ ions. C1 [Yuan, Zhigang; Yu, Xiongdong; Wang, Dedong; Huang, Shiyong; Li, Haimeng; Yu, Tao; Qiao, Zheng] Wuhan Univ, Sch Elect Informat, Wuhan, Peoples R China. [Wygant, John R.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Funsten, Herbert O.] Los Alamos Natl Lab, Los Alamos, NM USA. RP Yuan, ZG (reprint author), Wuhan Univ, Sch Elect Informat, Wuhan, Peoples R China. EM y_zgang@vip.163.com FU National Natural Science Foundation of China [41174140, 41374168, 41521063]; Program for New Century Excellent Talents in University [NCET-13-0446]; Keygrant Project of Chinese Ministry of Education [2042015kf0169] FX The Van Allen Probes data are available at the websites http://www.space.umn.edu/rbspefw-data/, http://emfisis.physics.uiowa.edu/data/index, and http://www.rbsp-ect.lanl.gov/data_pub/. This work is supported by the National Natural Science Foundation of China (41174140, 41374168, and 41521063), Program for New Century Excellent Talents in University (NCET-13-0446), and Keygrant Project of Chinese Ministry of Education (2042015kf0169). NR 46 TC 2 Z9 2 U1 0 U2 0 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6711 EP 6717 DI 10.1002/2016JA022573 PG 7 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100047 ER PT J AU Delzanno, GL Borovsky, JE Thomsen, MF Gilchrist, BE Sanchez, E AF Delzanno, Gian Luca Borovsky, Joseph E. Thomsen, Michelle F. Gilchrist, Brian E. Sanchez, Ennio TI Can an electron gun solve the outstanding problem of magnetosphere-ionosphere connectivity? SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Editorial Material DE electron beams; magnetic field line mapping; magnetosphere; ionosphere coupling; spacecraft charging ID SPACECRAFT POTENTIAL CONTROL; MAGNETIC CONJUNCTIONS; EARTHS MAGNETOSPHERE; ACTIVE SPACECRAFT; GEOMAGNETIC-FIELD; ARAKS EXPERIMENTS; CONJUGATE-POINTS; BEAM; CHARGE; PLUME AB Determining the magnetic connectivity between magnetospheric phenomena and ionospheric phenomena is an outstanding problem of magnetospheric and ionospheric physics. Accurately establishing this connectivity could answer a variety of long-standing questions. The most viable option to solve this is by means of a high-power electron beam fired from a magnetospheric spacecraft and spotted at its magnetic footpoint in the ionosphere. This has technical difficulties. Progress has been made on mitigating the major issue of spacecraft charging. The remaining physics issues are identified, together with the need for a synergistic effort in modeling, laboratory experiments, and, ultimately, testing in space. The goal of this commentary is to stimulate awareness and interest on the magnetosphere-ionosphere connectivity problem and possibly accelerate progress toward its solution. C1 [Delzanno, Gian Luca] Los Alamos Natl Lab, Theoret Div, Los Alamos, NM 87545 USA. [Borovsky, Joseph E.] Space Sci Inst, Boulder, CO USA. [Borovsky, Joseph E.; Gilchrist, Brian E.] Univ Michigan, CSSE, Ann Arbor, MI 48109 USA. [Thomsen, Michelle F.] Planetary Sci Inst, Tucson, AZ USA. [Sanchez, Ennio] SRI Int, Ctr Geospace Sci, 333 Ravenswood Ave, Menlo Pk, CA 94025 USA. RP Delzanno, GL (reprint author), Los Alamos Natl Lab, Theoret Div, Los Alamos, NM 87545 USA. EM delzanno@lanl.gov NR 50 TC 0 Z9 0 U1 3 U2 3 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6769 EP 6773 DI 10.1002/2016JA022728 PG 5 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100052 ER PT J AU Shao, XM Lay, EH AF Shao, Xuan-Min Lay, Erin H. TI The origin of infrasonic ionosphere oscillations over tropospheric thunderstorms SO JOURNAL OF GEOPHYSICAL RESEARCH-SPACE PHYSICS LA English DT Article DE ionosphere infrasound; thunderstorm downdraft; lightning sprites ID TOTAL ELECTRON-CONTENT; ACOUSTIC-WAVES; DISTURBANCES; SPRITES; SIGNATURES; CAMPAIGN; WEATHER; STORMS AB Thunderstorms have been observed to introduce infrasonic oscillations in the ionosphere, but it is not clear what processes or which parts of the thunderstorm generate the oscillations. In this paper, we present a new technique that uses an array of ground-based GPS total electron content (TEC) measurements to locate the source of the infrasonic oscillations and compare the source locations with thunderstorm features to understand the possible source mechanisms. The location technique utilizes instantaneous phase differences between pairs of GPS-TEC measurements and an algorithm to best fit the measured and the expected phase differences for assumed source positions and other related parameters. In this preliminary study, the infrasound waves are assumed to propagate along simple geometric raypaths from the source to the measurement locations to avoid extensive computations. The located sources are compared in time and space with thunderstorm development and lightning activity. Sources are often found near the main storm cells, but they are more likely related to the downdraft process than to the updraft process. The sources are also commonly found in the convectively quiet stratiform regions behind active cells and are in good coincidence with extensive lightning discharges and inferred high-altitude sprites discharges. C1 [Shao, Xuan-Min; Lay, Erin H.] Los Alamos Natl Lab, Space & Remote Sensing Grp, Los Alamos, NM 87545 USA. RP Shao, XM (reprint author), Los Alamos Natl Lab, Space & Remote Sensing Grp, Los Alamos, NM 87545 USA. EM xshao@lanl.gov OI Lay, Erin/0000-0002-1310-9035 FU Los Alamos National Laboratory's Laboratory Directed Research and Development; Institute for Geophysics, Planetary Physics and Signatures offices FX We thank Timothy Hamlin for the preparation of OK-LMA lightning data and Kyle Wiens for the display tools for NEXRAD observations. This research was supported by the Los Alamos National Laboratory's Laboratory Directed Research and Development and Institute for Geophysics, Planetary Physics and Signatures offices. Ground-based GPS receiver data used in this study were downloaded from http://geodesy.noaa.gov/CORS/. NEXRAD radar data were downloaded from http://www.roc.noaa.gov/WSR88D/. NR 45 TC 0 Z9 0 U1 4 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9380 EI 2169-9402 J9 J GEOPHYS RES-SPACE JI J. Geophys. Res-Space Phys. PD JUL PY 2016 VL 121 IS 7 BP 6783 EP 6798 DI 10.1002/2015JA022118 PG 16 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DW1SE UT WOS:000383422100054 ER PT J AU Ringstrand, BS Seifert, S Podlesak, DW Firestone, MA AF Ringstrand, Bryan S. Seifert, Sonke Podlesak, David W. Firestone, Millicent A. TI Self-Assembly Directed Organization of Nanodiamond During Ionic Liquid Crystalline Polymer Formation SO MACROMOLECULAR RAPID COMMUNICATIONS LA English DT Article DE ionic liquids; nanodiamonds; nanostructures; poly(ionic liquid)s ID SURFACE FUNCTIONALIZATION; DIAMOND NANOPARTICLES; FLUORESCENT NANODIAMONDS; DETONATION NANODIAMOND; COMPOSITES; PARTICLES; ARCHITECTURE; NANOTUBES; ACID AB The UV-initiated free radical polymerization of a lyotropic mesophase prepared by coassembly of an aqueous mixture of an ionic liquid (IL) monomer, 3-decyl-1-vinylimidazolium chloride, in a dimethyl sulfoxide dispersion of an IL-monomer nanodiamond conjugate yields a well-ordered 2D hexagonally structured network-polymer composite. The IL monomer is covalently bound to carboxylated detonation diamond via ester-linked 3-decyl-1-vinylimidazolium bromide. Successful preparation of the amphiphile-functionalized nanodiamond is determined by ATR/FT-IR, thermogravimetric analysis, and small-angle X-ray scattering (SAXS). Mesophase and composite structure are evaluated by SAXS, revealing a columnar architecture composed of amphiphilic ionic liquid cylinders containing solvent-rich cores. Self-assembly directed site localization of the nanodiamond positions the particles in the alkyl chain continuum upon polymerization. The composite reversibly swells in ethanol allowing structural variation and modulation of the nanoparticle internal packing arrangement. This work demonstrates that through careful molecular design, self-organization and site-directed assembly of nanodiamond into chemically distinct regions of a nanostructured organogel can be achieved. C1 [Ringstrand, Bryan S.; Podlesak, David W.; Firestone, Millicent A.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Seifert, Sonke] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Podlesak, David W.] Chem Div Nucl & Radiochem, MS J514,POB 1663, Los Alamos, NM 87545 USA. [Firestone, Millicent A.] Los Alamos Natl Lab, Mat Phys & Applicat Ctr Integrated Nanotechnol, MS K771,POB 1663, Los Alamos, NM 87545 USA. RP Podlesak, DW; Firestone, MA (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA.; Podlesak, DW (reprint author), Chem Div Nucl & Radiochem, MS J514,POB 1663, Los Alamos, NM 87545 USA.; Firestone, MA (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat Ctr Integrated Nanotechnol, MS K771,POB 1663, Los Alamos, NM 87545 USA. EM podlesak@lanl.gov; restone@lanl.gov FU US Department of Energy, Center for Integrated Nanotechnologies, at Los Alamos National Laboratory [DE-AC52-06NA25396] FX This work was performed in part at the US Department of Energy, Center for Integrated Nanotechnologies, at Los Alamos National Laboratory (Contract DE-AC52-06NA25396). The authors thank Dr. Kirill Velizhanin, (Los Alamos National Laboratory) for assistance with molecular modeling approximations and Dr. Rachel Huber for help with rendering figures. NR 57 TC 1 Z9 1 U1 18 U2 18 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1022-1336 EI 1521-3927 J9 MACROMOL RAPID COMM JI Macromol. Rapid Commun. PD JUL PY 2016 VL 37 IS 14 SI SI BP 1155 EP 1167 DI 10.1002/marc.201600070 PG 13 WC Polymer Science SC Polymer Science GA DW3WA UT WOS:000383572600009 PM 27197942 ER PT J AU Sobes, V Leal, L Arbanas, G Forget, B AF Sobes, Vladimir Leal, Luiz Arbanas, Goran Forget, Benoit TI Resonance Parameter Adjustment Based on Integral Experiments SO NUCLEAR SCIENCE AND ENGINEERING LA English DT Article DE Nuclear data evaluation; differential and integral experimental data; continuous-energy coupled ID MODEL CALIBRATION; SYSTEMS; UNCERTAINTY AB This project seeks to allow coupling of differential and integral data evaluation in a continuous-energy framework and to use the generalized linear least-squares (GLLS) methodology in the TSURFER module of the SCALE code package to update the parameters of a resolved resonance region evaluation. Recognizing that the GLLS methodology in TSURFER is identical to the mathematical description of a Bayesian update in SAMMY, the SAMINT code was created to use the mathematical machinery of SAMMY to update resolved resonance parameters based on integral data. Traditionally, SAMMY used differential experimental data to adjust nuclear data parameters. Integral experimental data, such as in the International Criticality Safety Benchmark Experiments Project, remain a tool for validation of completed nuclear data evaluations. SAMINT extracts information from integral benchmarks to aid the nuclear data evaluation process. Later, integral data can be used to resolve any remaining ambiguity between differential data sets, highlight troublesome energy regions, determine key nuclear data parameters for integral benchmark calculations, and improve the nuclear data covariance matrix evaluation. SAMINT is not intended to bias nuclear data toward specific integral experiments but should be used to supplement the evaluation of differential experimental data. Using GLLS ensures proper weight is given to the differential data. C1 [Sobes, Vladimir; Leal, Luiz; Arbanas, Goran] Oak Ridge Natl Lab, POB 2008,MS-6170, Oak Ridge, TN 37831 USA. [Forget, Benoit] MIT, 77 Massachusetts Ave, Cambridge, MA 02139 USA. RP Sobes, V (reprint author), Oak Ridge Natl Lab, POB 2008,MS-6170, Oak Ridge, TN 37831 USA. EM sobesv@ornl.gov FU U.S. Department of Energy [DE-AC05-00OR22725]; U.S. Nuclear Criticality Safety Program as part of the Oak Ridge National Laboratory Nuclear Data Succession Planning Task FX This manuscript has been authored by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the U.S. Department of Energy. Support for this work has been provided by the U.S. Nuclear Criticality Safety Program as part of the Oak Ridge National Laboratory Nuclear Data Succession Planning Task. The authors would like to thank D. Wiarda for her continuous computer help and advice. NR 19 TC 0 Z9 0 U1 1 U2 1 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5639 EI 1943-748X J9 NUCL SCI ENG JI Nucl. Sci. Eng. PD JUL PY 2016 VL 183 IS 3 BP 347 EP 355 DI 10.13182/NSE15-50 PG 9 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DW0VA UT WOS:000383359900003 ER PT J AU Isotalo, A AF Isotalo, Aarno TI Calculating Time-Integral Quantities in Depletion Calculations SO NUCLEAR SCIENCE AND ENGINEERING LA English DT Article DE Depletion; tally nuclides; Chebyshev rational approximation method (CRAM) ID BURNUP CALCULATIONS; BATEMAN SOLUTIONS; COUPLING SCHEMES; EQUATIONS AB A method referred to as tally nuclides is presented for accurately and efficiently calculating the time-step averages and integrals of any quantities that are weighted sums of atomic densities with constant weights during the step. The method allows all such quantities to be calculated simultaneously as a part of a single depletion solution with existing depletion algorithms. Examples of results that can be extracted include step-average atomic densities and macroscopic reaction rates, the total number of fissions during the step, and the amount of energy released during the step. The method should be applicable with several depletion algorithms, and the integrals or averages should be calculated with an accuracy comparable to that reached by the selected algorithm for end-of-step atomic densities. The accuracy of the method is demonstrated in depletion calculations using the Chebyshev rational approximation method. As an example of a possible use, we demonstrate how the ability to calculate energy release in depletion calculations can be used to determine the accuracy of the normalization in a constant-power burnup calculation during the calculation without a need for a reference solution. C1 [Isotalo, Aarno] Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA. [Isotalo, Aarno] Aalto Univ, Dept Appl Phys, POB 14100, FI-00076 Aalto, Finland. RP Isotalo, A (reprint author), Oak Ridge Natl Lab, POB 2008, Oak Ridge, TN 37831 USA.; Isotalo, A (reprint author), Aalto Univ, Dept Appl Phys, POB 14100, FI-00076 Aalto, Finland. EM aarno.isotalo@aalto.fi FU U.S. Department of Energy [DE-AC05-00OR22725]; Finnish Research Program on Nuclear Power Plant Safety [SAFIR2018]; U.S. Department of Energy, Office of Nuclear Energy, Advanced Modeling and Simulation Office, under the Nuclear Energy Advanced Modeling and Simulation (NEAMS) program FX This manuscript has been authored by UT-Battelle, LLC, under contract DE-AC05-00OR22725 with the U.S. Department of Energy. Funding from SAFIR2018, the Finnish Research Program on Nuclear Power Plant Safety, is acknowledged. This material is based upon work supported by the U.S. Department of Energy, Office of Nuclear Energy, Advanced Modeling and Simulation Office, under the Nuclear Energy Advanced Modeling and Simulation (NEAMS) program. NR 17 TC 0 Z9 0 U1 0 U2 0 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5639 EI 1943-748X J9 NUCL SCI ENG JI Nucl. Sci. Eng. PD JUL PY 2016 VL 183 IS 3 BP 421 EP 429 DI 10.13182/NSE15-119 PG 9 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DW0VA UT WOS:000383359900008 ER PT J AU Kulesza, JA Martz, RL AF Kulesza, Joel A. Martz, Roger L. TI Evaluation of Pulsed Sphere Time-of-Flight and Neutron Attenuation Experimental Benchmarks Using MCNP6's Unstructured Mesh Capabilities SO NUCLEAR TECHNOLOGY LA English DT Article DE Experimental benchmark comparison; MCNP; unstructured mesh AB This paper extends the verification and validation of MCNP6's unstructured mesh (UM) features for neutron transport capabilities by comparing code and experimental results for two different sets of experiments. The first set of experiments comprises time-of-flight spectrum measurements of spheres pulsed by 14-MeV neutrons performed by Lawrence Livermore National Laboratory in the early 1970s. The second set of experiments comprises spontaneous fission neutron attenuation measurements in relatively simple geometries with varying shield thicknesses performed by Ueki et al. in the early 1990s. First, traditional constructive solid geometry (CSG) models are analyzed to ensure agreement with experimental values and to form a basis of comparison with UM results. For the pulsed sphere experiments, a series of UM calculations is performed using first-order tetrahedral elements with various levels of mesh refinement. For the Ueki experiments, purely CSG, purely UM, and hybrid CSG/UM calculations are performed using first-and second-order tetrahedral and hexahedral elements. In the purely UM cases, two different meshing algorithms are used to specify the first-order tetrahedral mesh. The pulsed sphere calculated and experimental time-of-flight spectra agree with p-values >0.999 when compared using chi(2) goodness-of-fit tests. Furthermore, the UM results show discrepancies with the experimental values comparable to the CSG cases. The Ueki neutron attenuation calculated values using track-length and point detector tallies agree with the experimental values within 1 sigma with a single exception that agrees well within 2 sigma. As such, we conclude that the results for the CSG and UM calculations agree among themselves and with the experimental quantities when considering the associated statistical uncertainties. C1 [Kulesza, Joel A.] Univ Michigan, Cooley Lab, 2355 Bonisteel Blvd, Ann Arbor, MI 48105 USA. [Martz, Roger L.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Kulesza, JA (reprint author), Univ Michigan, Cooley Lab, 2355 Bonisteel Blvd, Ann Arbor, MI 48105 USA. EM jkulesza@umich.edu NR 17 TC 0 Z9 0 U1 1 U2 1 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5450 EI 1943-7471 J9 NUCL TECHNOL JI Nucl. Technol. PD JUL PY 2016 VL 195 IS 1 BP 44 EP 54 DI 10.13182/NT15-121 PG 11 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DW0UV UT WOS:000383359300004 ER PT J AU Kulesza, JA Martz, RL AF Kulesza, Joel A. Martz, Roger L. TI Evaluation of the Kobayashi Analytical Benchmark Using MCNP6's Unstructured Mesh Capabilities SO NUCLEAR TECHNOLOGY LA English DT Article DE Kobayashi benchmark; MCNP; unstructured mesh AB This paper provides results for calculations performed using MCNP6's unstructured mesh (UM) capabilities based on the three problems described in the Kobayashi benchmark suite. These calculations are performed to provide a comprehensive and consistent basis for the verification and validation of MCNP6's constructive solid geometry (CSG) and UM neutron transport capabilities relative to a well-known analytic benchmark. First, preexisting MCNP5 CSG models are updated and reexecuted to form a basis of comparison with UM for both the consistency of the numeric results and speed of execution. Next, a series of UM calculations is performed using first-and second-order tetrahedral and hexahedral elements with mesh generated using Abaqus. In addition, a different first-order tetrahedral mesh is generated with Attila4MC in order to investigate the effect on the results. When executed, the results for both CSG and UM agree among themselves and with the benchmark quantities within reasonable statistical fluctuations (at worst, the results agree within 2 sigma or 10% but generally within 1 sigma or 5%) and recognizing from historical work that improved agreement is possible with additional variance-reduction effort. As expected, for the simple geometries herein, we find the CSG calculations completing approximately ten times faster than the comparable fastest UM calculations. We find minor speed differences (similar to 1%) between multigroup and continuous-energy nuclear data and significant speed differences (factor similar to 100) between different element types. As such, the timing results support the recommendation that users run with the simplest UM element type that adequately represents the problem geometry, ideally first-order hexahedra, and with the most convenient nuclear data energy treatment. C1 [Kulesza, Joel A.] Univ Michigan, Cooley Lab, 2355 Bonisteel Blvd, Ann Arbor, MI 48105 USA. [Martz, Roger L.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Kulesza, JA (reprint author), Univ Michigan, Cooley Lab, 2355 Bonisteel Blvd, Ann Arbor, MI 48105 USA. EM jkulesza@umich.edu NR 11 TC 0 Z9 0 U1 0 U2 0 PU AMER NUCLEAR SOC PI LA GRANGE PK PA 555 N KENSINGTON AVE, LA GRANGE PK, IL 60526 USA SN 0029-5450 EI 1943-7471 J9 NUCL TECHNOL JI Nucl. Technol. PD JUL PY 2016 VL 195 IS 1 BP 55 EP 70 DI 10.13182/NT15-122 PG 16 WC Nuclear Science & Technology SC Nuclear Science & Technology GA DW0UV UT WOS:000383359300005 ER PT J AU Yashchuk, VV Tyurin, YN Tyurina, AY AF Yashchuk, Valeriy V. Tyurin, Yury N. Tyurina, Anastasia Y. TI Modeling of surface metrology of state-of-the-art x-ray mirrors as a result of stochastic polishing process SO OPTICAL ENGINEERING LA English DT Article DE surface metrology; time-invariant linear filter; autoregressive moving average; power spectral density; fabrication tolerances; x-ray optics; surface slope profilometry ID OPTICS; ALGORITHM; SYSTEM AB The design and evaluation of the expected performance of optical systems requires sophisticated and reliable information about the surface topography of planned optical elements before they are fabricated. The problem is especially severe in the case of x-ray optics for modern diffraction-limited-electron-ring and free-electron-laser x-ray facilities, as well as x-ray astrophysics missions, such as the X-ray Surveyor under development. Modern x-ray source facilities are reliant upon the availability of optics of unprecedented quality, with surface slope accuracy <0.1 mu rad. The unprecedented high angular resolution and throughput of future x-ray space observatories require high-quality optics of 100 m(2) in total area. The uniqueness of the optics and limited number of proficient vendors make the fabrication extremely time-consuming and expensive, mostly due to the limitations in accuracy and measurement rate of metrology used in fabrication. We continue investigating the possibility of improving metrology efficiency via comprehensive statistical treatment of a compact volume of metrology of surface topography, which is considered the result of a stochastic polishing process. We suggest, verify, and discuss an analytical algorithm for identification of an optimal symmetric time-invariant linear filter model with a minimum number of parameters and smallest residual error. If successful, the modeling could provide feedback to deterministic polishing processes, avoiding time-consuming, whole-scale metrology measurements over the entire optical surface with the resolution required to cover the entire desired spatial frequency range. The modeling also allows forecasting of metrology data for optics made by the same vendor and technology. The forecast data are vital for reliable specification for optical fabrication, evaluated from numerical simulation to be exactly adequate for the required system performance, avoiding both over-and underspecification. (C) The Authors. Published by SPIE under a Creative Commons Attribution 3.0 Unported License. Distribution or reproduction of this work in whole or in part requires full attribution of the original publication C1 [Yashchuk, Valeriy V.] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Tyurin, Yury N.] Moscow MV Lomonosov State Univ, 1 Leninskiye Gory St, Moscow 119991, Russia. [Tyurin, Yury N.; Tyurina, Anastasia Y.] Second Star Algonumer, 19 West St, Needham, MA 02494 USA. RP Yashchuk, VV (reprint author), Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. EM VVYashchuk@lbl.gov FU NASA Small Business Innovation Research grant [15-1 S2.04-9193]; U.S. Department of Energy [DE-AC02-05CH11231]; United States Government FX The authors are very grateful to Daniel J. Merthe, Nikolay A. Artemiev, and Daniele Cocco for their help with high-accuracy surface slope measurements of the LCLS beam split and delay mirror and to the Gary Centers and Wayne McKinney for very useful discussions. This work was supported in part by the NASA Small Business Innovation Research grant to Second Star Algonumerics, Project No. 15-1 S2.04-9193. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, Material Science Division, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231 at the Lawrence Berkeley National Laboratory. This document was prepared as an account of work sponsored by the United States Government. While this document is believed to contain correct information, neither the United States Government nor any agency thereof, nor the Regents of the University of California, nor any of their employees, makes any warranty, express or implied, or assumes any legal responsibility for the accuracy, completeness, or usefulness of any information, apparatus, product, or process disclosed, or represents that its use would not infringe privately owned rights. Reference herein to any specific commercial product, process, or service by its trade name, trademark, manufacturer, or otherwise, does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States Government or any agency thereof, or the Regents of the University of California. The views and opinions of authors expressed herein do not necessarily state or reflect those of the United States Government or any agency thereof or the Regents of the University of California. NR 33 TC 1 Z9 1 U1 0 U2 0 PU SPIE-SOC PHOTO-OPTICAL INSTRUMENTATION ENGINEERS PI BELLINGHAM PA 1000 20TH ST, PO BOX 10, BELLINGHAM, WA 98225 USA SN 0091-3286 EI 1560-2303 J9 OPT ENG JI Opt. Eng. PD JUL PY 2016 VL 55 IS 7 AR 074106 DI 10.1117/1.OE.55.7.074106 PG 11 WC Optics SC Optics GA DV9IN UT WOS:000383254200018 ER PT J AU Rademeyer, C Korber, B Seaman, MS Giorgi, EE Thebus, R Robles, A Sheward, DJ Wagh, K Garrity, J Carey, BR Gao, HM Greene, KM Tang, HL Bandawe, GP Marais, JC Diphoko, TE Hraber, P Tumba, N Moore, PL Gray, GE Kublin, J McElrath, MJ Vermeulen, M Middelkoop, K Bekker, LG Hoelscher, M Maboko, L Makhema, J Robb, ML Karim, SA Karim, QA Kim, JH Hahn, BH Gao, F Swanstrom, R Morris, L Montefiori, DC Williamson, C AF Rademeyer, Cecilia Korber, Bette Seaman, Michael S. Giorgi, Elena E. Thebus, Ruwayhida Robles, Alexander Sheward, Daniel J. Wagh, Kshitij Garrity, Jetta Carey, Brittany R. Gao, Hongmei Greene, Kelli M. Tang, Haili Bandawe, Gama P. Marais, Jinny C. Diphoko, Thabo E. Hraber, Peter Tumba, Nancy Moore, Penny L. Gray, Glenda E. Kublin, James McElrath, M. Juliana Vermeulen, Marion Middelkoop, Keren Bekker, Linda-Gail Hoelscher, Michael Maboko, Leonard Makhema, Joseph Robb, Merlin L. Karim, Salim Abdool Karim, Quarraisha Abdool Kim, Jerome H. Hahn, Beatrice H. Gao, Feng Swanstrom, Ronald Morris, Lynn Montefiori, David C. Williamson, Carolyn TI Features of Recently Transmitted HIV-1 Clade C Viruses that Impact Antibody Recognition: Implications for Active and Passive Immunization SO PLOS PATHOGENS LA English DT Article ID NEUTRALIZING MONOCLONAL-ANTIBODIES; ENVELOPE GLYCOPROTEIN; GLYCOSYLATION SITES; CORECEPTOR TROPISM; VACCINE EFFICACY; LOOP SEQUENCES; ENV CLONES; SUBTYPE-B; TYPE-1; INFECTION AB The development of biomedical interventions to reduce acquisition of HIV-1 infection remains a global priority, however their potential effectiveness is challenged by very high HIV-1 envelope diversity. Two large prophylactic trials in high incidence, clade C epidemic regions in southern Africa are imminent; passive administration of the monoclonal antibody VRC01, and active immunization with a clade C modified RV144-like vaccines. We have created a large representative panel of C clade viruses to enable assessment of antibody responses to vaccines and natural infection in Southern Africa, and we investigated the genotypic and neutralization properties of recently transmitted clade C viruses to determine how viral diversity impacted antibody recognition. We further explore the implications of these findings for the potential effectiveness of these trials. A panel of 200 HIV-1 Envelope pseudoviruses was constructed from clade C viruses collected within the first 100 days following infection. Viruses collected pre-seroconversion were significantly more resistant to serum neutralization compared to post-seroconversion viruses (p = 0.001). Over 13 years of the study as the epidemic matured, HIV-1 diversified (p = 0.0009) and became more neutralization resistant to monoclonal antibodies VRC01, PG9 and 4E10. When tested at therapeutic levels (10ug/ml), VRC01 only neutralized 80% of viruses in the panel, although it did exhibit potent neutralization activity against sensitive viruses (IC50 titres of 0.42 mu g/ml). The Gp120 amino acid similarity between the clade C panel and candidate C-clade vaccine protein boosts (Ce1086 and TV1) was 77%, which is 8% more distant than between CRF01_ AE viruses and the RV144 CRF01_ AE immunogen. Furthermore, two vaccine signature sites, K169 in V2 and I307 in V3, associated with reduced infection risk in RV144, occurred less frequently in clade C panel viruses than in CRF01_ AE viruses from Thailand. Increased resistance of pre-seroconversion viruses and evidence of antigenic drift highlights the value of using panels of very recently transmitted viruses and suggests that interventions may need to be modified over time to track the changing epidemic. Furthermore, high divergence such as that observed in the older clade C epidemic in southern Africa may impact vaccine efficacy, although the correlates of infection risk are yet to be defined in the clade C setting. Findings from this study of acute/early clade C viruses will aid vaccine development, and enable identification of new broad and potent antibodies to combat the HIV-1 C-clade epidemic in southern Africa. C1 [Rademeyer, Cecilia; Thebus, Ruwayhida; Sheward, Daniel J.; Bandawe, Gama P.; Marais, Jinny C.; Williamson, Carolyn] Univ Cape Town, Div Med Virol, Cape Town, South Africa. [Rademeyer, Cecilia; Thebus, Ruwayhida; Sheward, Daniel J.; Bandawe, Gama P.; Marais, Jinny C.; Williamson, Carolyn] Univ Cape Town, Inst Infect Dis & Mol Med, Cape Town, South Africa. [Rademeyer, Cecilia; Thebus, Ruwayhida; Sheward, Daniel J.; Bandawe, Gama P.; Marais, Jinny C.; Williamson, Carolyn] NHLS, Cape Town, South Africa. [Korber, Bette; Giorgi, Elena E.; Wagh, Kshitij; Hraber, Peter] Los Alamos Natl Lab, Los Alamos, NM USA. [Korber, Bette; Giorgi, Elena E.; Wagh, Kshitij; Hraber, Peter] New Mexico Consortium, Los Alamos, NM USA. [Seaman, Michael S.; Robles, Alexander; Garrity, Jetta; Carey, Brittany R.] Beth Israel Deaconess Med Ctr, Boston, MA 02215 USA. [Gao, Hongmei; Greene, Kelli M.; Tang, Haili; Gao, Feng; Montefiori, David C.] Duke Univ, Med Ctr, Dept Surg, Durham, NC 27710 USA. [Diphoko, Thabo E.; Makhema, Joseph] Botswana Harvard AIDS Inst Partnership, Gaborone, Botswana. [Tumba, Nancy; Moore, Penny L.; Morris, Lynn] NHLS, NICD, Johannesburg, South Africa. [Tumba, Nancy; Moore, Penny L.; Morris, Lynn] Univ Witwatersrand, Johannesburg, South Africa. [Moore, Penny L.; Karim, Salim Abdool; Karim, Quarraisha Abdool; Morris, Lynn; Williamson, Carolyn] Univ KwaZulu Natal, Ctr AIDS Programme Res South Africa CAPRISA, Durban, South Africa. [Gray, Glenda E.] Univ Witwatersrand, Fac Hlth Sci, Perinatal HIV Res Unit, Johannesburg, South Africa. [Gray, Glenda E.] South African Med Res Council, Cape Town, South Africa. [Kublin, James; McElrath, M. Juliana] Fred Hutchinson Canc Res Ctr, Vaccine & Infect Dis Div, 1124 Columbia St, Seattle, WA 98104 USA. [Vermeulen, Marion] South African Natl Blood Serv, Weltevreden Pk, South Africa. [Middelkoop, Keren; Bekker, Linda-Gail] Univ Cape Town, Desmond Tutu HIV Ctr, Dept Med, Cape Town, South Africa. [Middelkoop, Keren; Bekker, Linda-Gail] Univ Cape Town, Inst Infect Dis & Mol Med, Cape Town, South Africa. [Hoelscher, Michael] LMU, Klinikum Univ Munich, Dept Infect Dis & Trop Med, Munich, Germany. [Hoelscher, Michael] German Ctr Infect Res DZIF Partner Site Munich, Munich, Germany. [Maboko, Leonard] NIMR Mbeya Med Res Ctr, Mbeya, Tanzania. [Robb, Merlin L.; Kim, Jerome H.] Walter Reed Army Inst Res, US Mil HIV Res Program, Silver Spring, MD USA. [Kim, Jerome H.] Int Vaccine Inst, Seoul, South Korea. [Hahn, Beatrice H.] Univ Penn, Perelman Sch Med, Philadelphia, PA 19104 USA. [Swanstrom, Ronald] Univ North Carolina Chapel Hill, Dept Biochem & Biophys, Chapel Hill, NC USA. RP Williamson, C (reprint author), Univ Cape Town, Div Med Virol, Cape Town, South Africa.; Williamson, C (reprint author), Univ Cape Town, Inst Infect Dis & Mol Med, Cape Town, South Africa.; Williamson, C (reprint author), NHLS, Cape Town, South Africa.; Williamson, C (reprint author), Univ KwaZulu Natal, Ctr AIDS Programme Res South Africa CAPRISA, Durban, South Africa. EM carolyn.williamson@uct.ac.za RI Hoelscher, Michael/D-3436-2012; OI Abdool Karim, Salim/0000-0002-4986-2133; Hraber, Peter/0000-0002-2920-4897 FU Bill & Melinda Gates Foundation [38619, 1032144]; National Institute of Allergy and infectious Disease (NIAID), National Institutes of Health (NIH) [AI51794]; National Research Foundation [67385]; Columbia University-Southern African Fogarty AIDS International Training and Research Programme (AITRP) - Fogarty International Center, NIH [D43TW00231]; South African Government Department of Science and Technology; Medical Research Council, South Africa FX This study is part of the Comprehensive Antibody Vaccine Immune Monitoring Consortium supported by the Bill & Melinda Gates Foundation which established the Collaboration for AIDS Vaccine Discovery (CAVD) (Grant ID: 38619 and 1032144). CAPRISA samples has been supported by the National Institute of Allergy and infectious Disease (NIAID), National Institutes of Health (NIH) (grant # AI51794), the National Research Foundation (grant # 67385), the Columbia University-Southern African Fogarty AIDS International Training and Research Programme (AITRP) funded by the Fogarty International Center, NIH (grant # D43TW00231) the South African Government Department of Science and Technology and the Medical Research Council, South Africa. The opinions expressed herein are those of the authors and do not purport to reflect the official views of the networks that contributed samples. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 72 TC 2 Z9 2 U1 2 U2 2 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1553-7366 EI 1553-7374 J9 PLOS PATHOG JI PLoS Pathog. PD JUL PY 2016 VL 12 IS 7 AR e1005742 DI 10.1371/journal.ppat.1005742 PG 29 WC Microbiology; Parasitology; Virology SC Microbiology; Parasitology; Virology GA DW0XN UT WOS:000383366400027 PM 27434311 ER PT J AU Newland, SH Sinkler, W Mezza, T Bare, SR Raja, R AF Newland, Stephanie H. Sinkler, Wharton Mezza, Thomas Bare, Simon R. Raja, Robert TI Influence of dopant substitution mechanism on catalytic properties within hierarchical architectures SO PROCEEDINGS OF THE ROYAL SOCIETY A-MATHEMATICAL PHYSICAL AND ENGINEERING SCIENCES LA English DT Article DE hierarchically porous; isomorphous substitution; aluminophosphates; Beckmann rearrangement; active-site design ID PHASE BECKMANN REARRANGEMENT; ALUMINOPHOSPHATE MOLECULAR-SIEVES; SURFACTANT-DIRECTED SYNTHESIS; ACTIVE-SITES; CYCLOHEXANONE OXIME; SELECTIVE OXIDATION; EPSILON-CAPROLACTAM; ACID SITES; ZEOLITES; DESIGN AB A range of hierarchically porous (HP) AlPO-5 catalysts, with isomorphously substituted transition metal ions, have been synthesized using an organosilane as a soft template. By employing a range of structural and spectroscopic characterization protocols, the properties of the dopant-substituted species within the HP architectures have been carefully evaluated. The resulting nature of the active site is shown to have a direct impact on the ensuing catalytic properties in the liquid-phase Beckmann rearrangement of cyclic ketones. C1 [Newland, Stephanie H.; Raja, Robert] Univ Southampton, Sch Chem, Southampton SO17 1BJ, Hants, England. [Sinkler, Wharton; Mezza, Thomas; Bare, Simon R.] UOP LLC, Des Plaines, IL 60017 USA. [Bare, Simon R.] SLAC Natl Accelerator Lab, SSRL, Menlo Pk, CA 94025 USA. RP Raja, R (reprint author), Univ Southampton, Sch Chem, Southampton SO17 1BJ, Hants, England. EM r.raja@soton.ac.uk RI Raja, Robert/B-8715-2009 OI Raja, Robert/0000-0002-4161-7053 FU UK Catalysis Hub via UK Catalysis Hub Consortium; EPSRC [EP/K014706/1, EP/K014668/1, EP/K014854/1, EP/K014714/1, EP/M013219/1] FX R.R. and S.H.N. kindly thank the UK Catalysis Hub for resources and support provided via our membership of the UK Catalysis Hub Consortium and supported by EPSRC via grants EP/K014706/1, EP/K014668/1, EP/K014854/1, EP/K014714/1 and EP/M013219/1. NR 63 TC 0 Z9 0 U1 2 U2 2 PU ROYAL SOC PI LONDON PA 6-9 CARLTON HOUSE TERRACE, LONDON SW1Y 5AG, ENGLAND SN 1364-5021 EI 1471-2946 J9 P ROY SOC A-MATH PHY JI Proc. R. Soc. A-Math. Phys. Eng. Sci. PD JUL 1 PY 2016 VL 472 IS 2191 AR 20160095 DI 10.1098/rspa.2016.0095 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DW6TG UT WOS:000383783500007 PM 27493563 ER PT J AU Sheehy, SL Kelliher, DJ Machida, S Rogers, C Prior, CR Volat, L Tahar, MH Ishi, Y Kuriyama, Y Sakamoto, M Uesugi, T Mori, Y AF Sheehy, S. L. Kelliher, D. J. Machida, S. Rogers, C. Prior, C. R. Volat, L. Tahar, M. Haj Ishi, Y. Kuriyama, Y. Sakamoto, M. Uesugi, T. Mori, Y. TI Characterization techniques for fixed-field alternating gradient accelerators and beam studies using the KURRI 150 MeV proton FFAG SO PROGRESS OF THEORETICAL AND EXPERIMENTAL PHYSICS LA English DT Article ID EMMA AB In this paper we describe the methods and tools used to characterize a 150 MeV proton scaling fixed field alternating gradient (FFAG) accelerator at Kyoto University Research Reactor Institute. Many of the techniques used are unique to this class of machine and are thus of relevance to any future FFAG accelerator. For the first time we detail systematic studies undertaken to improve the beam quality of the FFAG. The control of beam quality in this manner is crucial to demonstrating high power operation of FFAG accelerators in future. C1 [Sheehy, S. L.] Univ Oxford, John Adams Inst, Keble Rd, Oxford OX1 3RH, England. [Kelliher, D. J.; Machida, S.; Rogers, C.; Prior, C. R.] STFC Rutherford Appleton Lab, ASTeC, Didcot OX11 0QX, Oxon, England. [Volat, L.] Grenoble Inst Technol, Grenoble, France. [Tahar, M. Haj] Brookhaven Natl Lab, Upton, NY 11973 USA. [Ishi, Y.; Kuriyama, Y.; Sakamoto, M.; Uesugi, T.; Mori, Y.] Kyoto Univ, Inst Res Reactor, Osaka 5900494, Japan. RP Sheehy, SL (reprint author), Univ Oxford, John Adams Inst, Keble Rd, Oxford OX1 3RH, England. EM suzie.sheehy@physics.ox.ac.uk RI Sheehy, Suzie/C-3304-2013 OI Sheehy, Suzie/0000-0002-7653-7205 NR 22 TC 0 Z9 0 U1 2 U2 2 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 2050-3911 J9 PROG THEOR EXP PHYS JI Prog. Theor. Exp. Phys. PD JUL PY 2016 IS 7 AR 073G01 DI 10.1093/ptep/ptw086 PG 31 WC Physics, Multidisciplinary; Physics, Particles & Fields SC Physics GA DV9UL UT WOS:000383287600009 ER PT J AU Smith, KN Mailliard, RB Piazza, PA Fischer, W Korber, BT Fecek, RJ Ratner, D Gupta, P Mullins, JI Rinaldo, CR AF Smith, Kellie N. Mailliard, Robbie B. Piazza, Paolo A. Fischer, Will Korber, Bette T. Fecek, Ronald J. Ratner, Deena Gupta, Phalguni Mullins, James I. Rinaldo, Charles R. TI Effective Cytotoxic T Lymphocyte Targeting of Persistent HIV-1 during Antiretroviral Therapy Requires Priming of Naive CD8(+) T Cells (vol 7, e00473, 2016) SO MBIO LA English DT Correction C1 [Smith, Kellie N.] Univ Pittsburgh, Dept Microbiol & Mol Genet, Pittsburgh, PA USA. [Smith, Kellie N.; Mailliard, Robbie B.; Piazza, Paolo A.; Fecek, Ronald J.; Ratner, Deena; Gupta, Phalguni; Rinaldo, Charles R.] Univ Pittsburgh, Dept Infect Dis & Microbiol, Pittsburgh, PA 15261 USA. [Fischer, Will; Korber, Bette T.] Los Alamos Natl Lab, Theoret Biol & Biophys Grp, Los Alamos, NM USA. [Mullins, James I.] Univ Washington, Dept Microbiol, Seattle, WA 98195 USA. [Rinaldo, Charles R.] Univ Pittsburgh, Sch Med, Dept Pathol, Pittsburgh, PA 15213 USA. RP Rinaldo, CR (reprint author), Univ Pittsburgh, Dept Infect Dis & Microbiol, Pittsburgh, PA 15261 USA.; Rinaldo, CR (reprint author), Univ Pittsburgh, Sch Med, Dept Pathol, Pittsburgh, PA 15213 USA. EM rinaldo@pitt.edu NR 1 TC 0 Z9 0 U1 3 U2 3 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD JUL-AUG PY 2016 VL 7 IS 4 AR e01012 DI 10.1128/mBio.01012-16 PG 1 WC Microbiology SC Microbiology GA DW1YQ UT WOS:000383440500049 ER PT J AU Rouet, FH Li, XYS Ghysels, P Napov, A AF Rouet, Francois-Henry Li, Xiaoye S. Ghysels, Pieter Napov, Artem TI A Distributed-Memory Package for Dense Hierarchically Semi-Separable Matrix Computations Using Randomization SO ACM TRANSACTIONS ON MATHEMATICAL SOFTWARE LA English DT Article DE Design; Algorithms; Performance; HSS matrices; randomized sampling; ULV factorization; parallel algorithms; distributed-memory ID LINEAR-SYSTEMS; RANK; FACTORIZATION; MULTIPLICATION; ALGORITHM; REPRESENTATIONS; EQUATIONS; SOLVER AB We present a distributed-memory library for computations with dense structured matrices. A matrix is considered structured if its off-diagonal blocks can be approximated by a rank-deficient matrix with low numerical rank. Here, we use Hierarchically Semi-Separable (HSS) representations. Such matrices appear in many applications, for example, finite-element methods, boundary element methods, and so on. Exploiting this structure allows for fast solution of linear systems and/or fast computation of matrix-vector products, which are the two main building blocks of matrix computations. The compression algorithm that we use, that computes the HSS form of an input dense matrix, relies on randomized sampling with a novel adaptive sampling mechanism. We discuss the parallelization of this algorithm and also present the parallelization of structured matrix-vector product, structured factorization, and solution routines. The efficiency of the approach is demonstrated on large problems from different academic and industrial applications, on up to 8,000 cores. This work is part of a more global effort, the STRUctured Matrices PACKage (STRUMPACK) software package for computations with sparse and dense structured matrices. Hence, although useful on their own right, the routines also represent a step in the direction of a distributed-memory sparse solver. C1 [Rouet, Francois-Henry; Li, Xiaoye S.; Ghysels, Pieter] Lawrence Berkeley Natl Lab, MS 50F-1650,One Cyclotron Rd, Berkeley, CA 94720 USA. [Napov, Artem] Univ Libre Bruxelles, Serv Metrol Nucl CP 165 84, Ave FD Roosevelt 50, B-1050 Brussels, Belgium. RP Rouet, FH (reprint author), Lawrence Berkeley Natl Lab, MS 50F-1650,One Cyclotron Rd, Berkeley, CA 94720 USA. FU Scientific Discovery through the Advanced Computing (SciDAC) program - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research (and Basic Energy Sciences; Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231] FX Partial support for this work was provided through Scientific Discovery through the Advanced Computing (SciDAC) program funded by the U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research (and Basic Energy Sciences/Biological and Environmental Research/High Energy Physics/Fusion Energy Sciences/Nuclear Physics). This research used resources of the National Energy Research Scientific Computing Center, which is supported by the Office of Science of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 37 TC 1 Z9 1 U1 1 U2 1 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 0098-3500 EI 1557-7295 J9 ACM T MATH SOFTWARE JI ACM Trans. Math. Softw. PD JUL PY 2016 VL 42 IS 4 AR 27 DI 10.1145/2930660 PG 35 WC Computer Science, Software Engineering; Mathematics, Applied SC Computer Science; Mathematics GA DU3TT UT WOS:000382135800001 ER PT J AU Disney, A Reynolds, J Schuman, CD Klibisz, A Young, A Plank, JS AF Disney, Adam Reynolds, John Schuman, Catherine D. Klibisz, Aleksander Young, Aaron Plank, James S. TI DANNA: A neuromorphic software ecosystem SO BIOLOGICALLY INSPIRED COGNITIVE ARCHITECTURES LA English DT Article DE Neuromorphic computing; Genetic algorithms; Visualization AB Architectures for neuromorphic computing have evolved to the point where a significant amount of software design and implementation is necessary for leveraging these architectures to solve real problems. In this paper, we describe the software ecosystem for the DANNA neuromorphic computing model. This ecosystem is composed of four pieces: a simulator, commander, evolutionary optimizer, and visualizer. The ecosystem facilitates developing applications for DANNA, and in turn will help DANNA evolve into a more effective neuromorphic computing model. We describe how we use the software components to perform digit classification using the MNIST dataset. (C) 2016 Elsevier B.V. All rights reserved. C1 [Disney, Adam; Reynolds, John; Klibisz, Aleksander; Young, Aaron; Plank, James S.] Univ Tennessee, Knoxville, TN 37996 USA. [Schuman, Catherine D.] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Disney, A (reprint author), Univ Tennessee, Knoxville, TN 37996 USA. EM adisney1@vols.utk.edu; jreyno40@vols.utk.edu; schumancd@ornl.gov; aklibisz@vols.utk.edu; ayoung48@vols.utk.edu; jplank@vols.utk.edu FU Air Force Research Laboratory [FA8750-16-1-0065] FX This material is based on research sponsored by the Air Force Research Laboratory under agreement number FA8750-16-1-0065. The U.S. Government is authorized to reproduce and distribute reprints for Governmental purposes notwithstanding any copyright notation thereon. The views and conclusions contained herein are those of the authors and should not be interpreted as necessarily representing the official policies or endorsements, either expressed or implied, of the Air Force Research Laboratory or the U.S. Government. NR 14 TC 0 Z9 0 U1 2 U2 2 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2212-683X EI 2212-6848 J9 BIOL INSPIR COGN ARC JI Biol. Inspired Cogn. Archit. PD JUL PY 2016 VL 17 BP 49 EP 56 DI 10.1016/j.bica.2016.07.007 PG 8 WC Computer Science, Artificial Intelligence; Neurosciences SC Computer Science; Neurosciences & Neurology GA DV5YJ UT WOS:000383006300005 ER PT J AU Bauer, SJ Gardner, WP Heath, JE AF Bauer, Stephen J. Gardner, W. Payton Heath, Jason E. TI Helium release during shale deformation: Experimental validation SO GEOCHEMISTRY GEOPHYSICS GEOSYSTEMS LA English DT Article DE physical properties of rocks; structural geology; tectonophysics; hydrology; helium release; shale deformation ID PERMEABILITY; CLAY; ANISOTROPY; STRESS AB This work describes initial experimental results of helium tracer release monitoring during deformation of shale. Naturally occurring radiogenic He-4 is present in high concentration in most shales. During rock deformation, accumulated helium could be released as fractures are created and new transport pathways are created. We present the results of an experimental study in which confined reservoir shale samples, cored parallel and perpendicular to bedding, which were initially saturated with helium to simulate reservoir conditions, are subjected to triaxial compressive deformation. During the deformation experiment, differential stress, axial, and radial strains are systematically tracked. Release of helium is dynamically measured using a helium mass spectrometer leak detector. Helium released during deformation is observable at the laboratory scale and the release is tightly coupled to the shale deformation. These first measurements of dynamic helium release from rocks undergoing deformation show that helium provides information on the evolution of microstructure as a function of changes in stress and strain. C1 [Bauer, Stephen J.] Sandia Natl Labs, Geomech Dept, MS 1033, Albuquerque, NM 87185 USA. [Gardner, W. Payton] Univ Montana, Dept Geosci, Missoula, MT 59812 USA. [Heath, Jason E.] Sandia Natl Labs, Geomech Dept, POB 5800, Albuquerque, NM 87185 USA. RP Bauer, SJ (reprint author), Sandia Natl Labs, Geomech Dept, MS 1033, Albuquerque, NM 87185 USA. EM sjbauer@sandia.gov FU Sandia Laboratory Directed Research and Development (LDRD) [165670]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was funded under the Sandia Laboratory Directed Research and Development (LDRD) project 165670 and title "Appraisal of Hydraulic Fractures Using Natural Tracers." Data in plotted figures may be obtained from SJB upon request ((sjbauer@sandia.gov).). Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 25 TC 1 Z9 1 U1 1 U2 1 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 1525-2027 J9 GEOCHEM GEOPHY GEOSY JI Geochem. Geophys. Geosyst. PD JUL PY 2016 VL 17 IS 7 BP 2612 EP 2622 DI 10.1002/2016GC006352 PG 11 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DV5BI UT WOS:000382940000009 ER PT J AU Macris, N Vuffray, M AF Macris, Nicolas Vuffray, Marc TI The Bethe Free Energy Allows to Compute the Conditional Entropy of Graphical Code Instances: A Proof From the Polymer Expansion SO IEEE TRANSACTIONS ON INFORMATION THEORY LA English DT Article DE Low-density parity-check codes; low-density generator-matrix codes; graphical models; Bethe free energy; loop calculus; polymer expansion; expanders ID ERROR-CORRECTING CODES; BOUNDS AB The main objective of this paper is to explore the precise relationship between the Bethe free energy (or entropy) and the Shannon conditional entropy of graphical error correcting codes. The main result shows that the Bethe free energy associated with a low-density parity-check code used over a binary symmetric channel in a large noise regime is, with high probability, asymptotically exact as the block length grows. To arrive at this result, we develop new techniques for rather general graphical models based on the loop sum as a starting point and the polymer expansion from statistical mechanics. The true free energy is computed as a series expansion containing the Bethe free energy as its zeroth-order term plus a series of corrections. It is easily seen that convergence criteria for such expansions are satisfied for general high-temperature models. We apply these general results to the ensembles of low-density generator-matrix and parity-check codes. While the application to generator-matrix codes follows standard high temperature methods, the case of parity-check codes requires non-trivial new ideas, because the hard constraints correspond to a zero-temperature regime. Nevertheless, one can combine the polymer expansion with expander and counting arguments to show that the difference between the true and Bethe free energies vanishes with high probability in the large block length limit. C1 [Macris, Nicolas] Ecole Polytech Fed Lausanne, Sch Comp & Commun Sci, CH-1015 Lausanne, Switzerland. [Vuffray, Marc] Ecole Polytech Fed Lausanne, CH-1015 Lausanne, Switzerland. [Vuffray, Marc] Los Alamos Natl Lab, Div Theory, Ctr Nonlinear Studies, Los Alamos, NM 87545 USA. RP Macris, N (reprint author), Ecole Polytech Fed Lausanne, Sch Comp & Commun Sci, CH-1015 Lausanne, Switzerland. EM nicolas.macris@epfl.ch; vuffray@lanl.gov OI Vuffray, Marc/0000-0001-7999-9897 FU Swiss National Foundation for Science [200020-140388] FX M. Vuffray was supported by the Swiss National Foundation for Science under Grant 200020-140388. NR 24 TC 0 Z9 0 U1 0 U2 0 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9448 EI 1557-9654 J9 IEEE T INFORM THEORY JI IEEE Trans. Inf. Theory PD JUL PY 2016 VL 62 IS 7 BP 4003 EP 4023 DI 10.1109/TIT.2016.2555843 PG 21 WC Computer Science, Information Systems; Engineering, Electrical & Electronic SC Computer Science; Engineering GA DU3TR UT WOS:000382135600013 ER PT J AU Hodgson, JA Seyler, TH Wang, LQ AF Hodgson, James A. Seyler, Tiffany H. Wang, Lanqing TI Long-Term Stability of Volatile Nitrosamines in Human Urine SO JOURNAL OF ANALYTICAL TOXICOLOGY LA English DT Article ID NITROGEN CHEMILUMINESCENCE DETECTION; COMPREHENSIVE GAS-CHROMATOGRAPHY; SPORADIC ALZHEIMERS-DISEASE; TYPE-2 DIABETES-MELLITUS; N-NITROSAMINES; DRINKING-WATER; MASS-SPECTROMETRY; NONALCOHOLIC STEATOHEPATITIS; CHEMICAL-IONIZATION; MEAT-PRODUCTS AB Volatile nitrosamines (VNAs) are established teratogens and carcinogens in animals and classified as probable (group 2A) and possible (group 2B) carcinogens in humans by the IARC. High levels of VNAs have been detected in tobacco products and in both mainstream and sidestream smoke. VNA exposure may lead to lipid peroxidation and oxidative stress (e.g., inflammation), chronic diseases (e.g., diabetes) and neurodegenerative diseases (e.g., Alzheimer's disease). To conduct epidemiological studies on the effects of VNA exposure, short-term and long-term stabilities of VNAs in the urine matrix are needed. In this report, the stability of six VNAs (N-nitrosodimethylamine, N-nitrosomethylethylamine, N-nitrosodiethylamine, N-nitrosopiperidine, N-nitrosopyrrolidine and N-nitrosomorpholine) in human urine is analyzed for the first time using in vitro blank urine pools fortified with a standard mixture of all six VNAs. Over a 24-day period, analytes were monitored in samples stored at similar to 20A degrees C (collection temperature), 4-10A degrees C (transit temperature) and -20 and -70A degrees C (long-term storage temperatures). All six analytes were stable for 24 days at all temperatures (n = 15). The analytes were then analyzed over a longer time period at -70A degrees C; all analytes were stable for up to 1 year (n = 62). A subset of 44 samples was prepared as a single batch and stored at -20A degrees C, the temperature at which prepared samples are stored. These prepared samples were run in duplicate weekly over 10 weeks, and all six analytes were stable over the entire period (n = 22). C1 [Hodgson, James A.] ORISE, Oak Ridge, TN USA. [Seyler, Tiffany H.; Wang, Lanqing] Ctr Dis Control & Prevent, Tobacco & Volatiles Branch, Div Sci Lab, Natl Ctr Environm Hlth, Atlanta, GA 30329 USA. RP Seyler, TH (reprint author), Ctr Dis Control & Prevent, Tobacco & Volatiles Branch, Div Sci Lab, Natl Ctr Environm Hlth, Atlanta, GA 30329 USA. EM tvh2@cdc.gov FU U.S. Food and Drug Administration, Center for Tobacco Products FX This study was funded by the U.S. Food and Drug Administration, Center for Tobacco Products. The findings and conclusions in this study are those of the authors and do not necessarily represent the views of the U.S. Department of Health and Human Services, or the U.S. Centers for Disease Control and Prevention. Use of trade names and commercial sources is for identification only and does not constitute endorsement by the U.S. Department of Health and Human Services, or the U.S. Centers for Disease Control and Prevention. NR 32 TC 0 Z9 0 U1 9 U2 9 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 0146-4760 EI 1945-2403 J9 J ANAL TOXICOL JI J. Anal. Toxicol. PD JUL-AUG PY 2016 VL 40 IS 6 BP 414 EP 418 DI 10.1093/jat/bkw038 PG 5 WC Chemistry, Analytical; Toxicology SC Chemistry; Toxicology GA DV8GD UT WOS:000383174600003 PM 27274026 ER PT J AU Bernstein, HC McClure, RS Hill, EA Markillie, LM Chrisler, WB Romine, MF McDermott, JE Posewitz, MC Bryant, DA Konopka, AE Fredrickson, JK Beliaev, AS AF Bernstein, Hans C. McClure, Ryan S. Hill, Eric A. Markillie, Lye Meng Chrisler, William B. Romine, Margie F. McDermott, Jason E. Posewitz, Matthew C. Bryant, Donald A. Konopka, Allan E. Fredrickson, James K. Beliaev, Alexander S. TI Unlocking the Constraints of Cyanobacterial Productivity: Acclimations Enabling Ultrafast Growth SO MBIO LA English DT Article ID STRAIN PCC 7002; SYNECHOCOCCUS SP PCC-7002; THERMOSYNECHOCOCCUS-ELONGATUS; OXIDATIVE STRESS; GENE-EXPRESSION; OSCILLATORIA-AGARDHII; CONTINUOUS-CULTURE; OXYGEN EVOLUTION; PHOTOSYSTEM-II; ELECTRON FLOW AB Harnessing the metabolic potential of photosynthetic microbes for next-generation biotechnology objectives requires detailed scientific understanding of the physiological constraints and regulatory controls affecting carbon partitioning between biomass, metabolite storage pools, and bioproduct synthesis. We dissected the cellular mechanisms underlying the remarkable physiological robustness of the euryhaline unicellular cyanobacterium Synechococcus sp. strain PCC 7002 (Synechococcus 7002) and identify key mechanisms that allow cyanobacteria to achieve unprecedented photoautotrophic productivities (similar to 2.5-h doubling time). Ultrafast growth of Synechococcus 7002 was supported by high rates of photosynthetic electron transfer and linked to significantly elevated transcription of precursor biosynthesis and protein translation machinery. Notably, no growth or photosynthesis inhibition signatures were observed under any of the tested experimental conditions. Finally, the ultrafast growth in Synechococcus 7002 was also linked to a 300% expansion of average cell volume. We hypothesize that this cellular adaptation is required at high irradiances to support higher cell division rates and reduce deleterious effects, corresponding to high light, through increased carbon and reductant sequestration. IMPORTANCE Efficient coupling between photosynthesis and productivity is central to the development of biotechnology based on solar energy. Therefore, understanding the factors constraining maximum rates of carbon processing is necessary to identify regulatory mechanisms and devise strategies to overcome productivity constraints. Here, we interrogate the molecular mechanisms that operate at a systems level to allow cyanobacteria to achieve ultrafast growth. This was done by considering growth and photosynthetic kinetics with global transcription patterns. We have delineated putative biological principles that allow unicellular cyanobacteria to achieve ultrahigh growth rates through photophysiological acclimation and effective management of cellular resource under different growth regimes. C1 [Bernstein, Hans C.] Pacific NW Natl Lab, Chem & Biol Signature Sci, Richland, WA 99352 USA. [Bernstein, Hans C.; McClure, Ryan S.; Hill, Eric A.; Chrisler, William B.; Romine, Margie F.; McDermott, Jason E.; Konopka, Allan E.; Fredrickson, James K.; Beliaev, Alexander S.] Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA. [Markillie, Lye Meng] Pacific NW Natl Lab, Environm Mol Sci Lab, Richland, WA 99352 USA. [Posewitz, Matthew C.] Colorado Sch Mines, Dept Chem & Geochem, Golden, CO 80401 USA. [Bryant, Donald A.] Penn State Univ, Dept Biochem & Mol Biol, University Pk, PA 16802 USA. [Bryant, Donald A.] Montana State Univ, Dept Chem & Biochem, Bozeman, MT 59717 USA. [Konopka, Allan E.] Purdue Univ, Dept Biol Sci, W Lafayette, IN 47907 USA. [Bernstein, Hans C.] Washington State Univ, Gene & Linda Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. RP Bernstein, HC (reprint author), Pacific NW Natl Lab, Chem & Biol Signature Sci, Richland, WA 99352 USA.; Bernstein, HC; Beliaev, AS (reprint author), Pacific NW Natl Lab, Div Biol Sci, Richland, WA 99352 USA.; Bernstein, HC (reprint author), Washington State Univ, Gene & Linda Voiland Sch Chem Engn & Bioengn, Pullman, WA 99164 USA. EM Hans.Bernstein@pnnl.gov; alex.beliaev@pnnl.gov OI Romine, Margaret/0000-0002-0968-7641; Bernstein, Hans/0000-0003-2913-7708 FU U.S. Department of Energy [DE-AC05-76RLO 1830]; Genomic Science Program, Office of Biological and Environmental Research (OBER), U.S. Department of Energy (DOE); DOE OBER; Foundational Scientific Focus Area at PNNL; Linus Pauling Distinguished Postdoctoral Fellowship, a Laboratory Directed Research and Development Program of PNNL FX We acknowledge Matthew Melnicki, Victoria Work, and Leo Kucek who assisted with the analyses of turbidostat samples. The Pacific Northwest National Laboratory is operated for the U.S. Department of Energy by Battelle Memorial Institute under contract DE-AC05-76RLO 1830.; This research was supported by the Genomic Science Program, Office of Biological and Environmental Research (OBER), U.S. Department of Energy (DOE), and is a contribution of the Pacific Northwest National Laboratory (PNNL) Foundational and Biofuels Scientific Focus Areas. A significant portion of the research was performed using the Environmental Molecular Sciences Laboratory, a national scientific user facility sponsored by DOE OBER and located at PNNL. The genome annotation and bioinformatics efforts used customized processes and resources developed and supported by the Foundational Scientific Focus Area at PNNL. H.C.B. is grateful for support given by the Linus Pauling Distinguished Postdoctoral Fellowship, a Laboratory Directed Research and Development Program of PNNL. NR 60 TC 3 Z9 3 U1 4 U2 4 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD JUL-AUG PY 2016 VL 7 IS 4 AR e00949-16 DI 10.1128/mBio.00949-16 PG 10 WC Microbiology SC Microbiology GA DW1YQ UT WOS:000383440500038 ER PT J AU Hiras, J Wu, YW Deng, K Nicora, CD Aldrich, JT Frey, D Kolinko, S Robinson, EW Jacobs, JM Adams, PD Northen, TR Simmons, BA Singer, SW AF Hiras, Jennifer Wu, Yu-Wei Deng, Kai Nicora, Carrie D. Aldrich, Joshua T. Frey, Dario Kolinko, Sebastian Robinson, Errol W. Jacobs, Jon M. Adams, Paul D. Northen, Trent R. Simmons, Blake A. Singer, Steven W. TI Comparative Community Proteomics Demonstrates the Unexpected Importance of Actinobacterial Glycoside Hydrolase Family 12 Protein for Crystalline Cellulose Hydrolysis SO MBIO LA English DT Article ID THERMOPHILIC BACTERIAL CONSORTIA; ACIDOTHERMUS-CELLULOLYTICUS 11B; MICROBISPORA-BISPORA; ANGSTROM RESOLUTION; COMPLETE GENOME; ENDOGLUCANASE; DIVERSITY; DECONSTRUCTION; STREPTOMYCES; ALGORITHM AB Glycoside hydrolases (GHs) are key enzymes in the depolymerization of plant-derived cellulose, a process central to the global carbon cycle and the conversion of plant biomass to fuels and chemicals. A limited number of GH families hydrolyze crystalline cellulose, often by a processive mechanism along the cellulose chain. During cultivation of thermophilic cellulolytic microbial communities, substantial differences were observed in the crystalline cellulose saccharification activities of supernatants recovered from divergent lineages. Comparative community proteomics identified a set of cellulases from a population closely related to actinobacterium Thermobispora bispora that were highly abundant in the most active consortium. Among the cellulases from T. bispora, the abundance of a GH family 12 (GH12) protein correlated most closely with the changes in crystalline cellulose hydrolysis activity. This result was surprising since GH12 proteins have been predominantly characterized as enzymes active on soluble polysaccharide substrates. Heterologous expression and biochemical characterization of the suite of T. bispora hydrolytic cellulases confirmed that the GH12 protein possessed the highest activity on multiple crystalline cellulose substrates and demonstrated that it hydrolyzes cellulose chains by a predominantly random mechanism. This work suggests that the role of GH12 proteins in crystalline cellulose hydrolysis by cellulolytic microbes should be reconsidered. IMPORTANCE Cellulose is the most abundant organic polymer on earth, and its enzymatic hydrolysis is a key reaction in the global carbon cycle and the conversion of plant biomass to biofuels. The glycoside hydrolases that depolymerize crystalline cellulose have been primarily characterized from isolates. In this study, we demonstrate that adapting microbial consortia from compost to grow on crystalline cellulose generated communities whose soluble enzymes exhibit differential abilities to hydrolyze crystalline cellulose. Comparative proteomics of these communities identified a protein of glycoside hydrolase family 12 (GH12), a family of proteins previously observed to primarily hydrolyze soluble substrates, as a candidate that accounted for some of the differences in hydrolytic activities. Heterologous expression confirmed that the GH12 protein identified by proteomics was active on crystalline cellulose and hydrolyzed cellulose by a random mechanism, in contrast to most cellulases that act on the crystalline polymer in a processive mechanism. C1 [Hiras, Jennifer; Wu, Yu-Wei; Deng, Kai; Frey, Dario; Kolinko, Sebastian; Adams, Paul D.; Northen, Trent R.; Simmons, Blake A.; Singer, Steven W.] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Hiras, Jennifer; Wu, Yu-Wei; Frey, Dario; Kolinko, Sebastian; Adams, Paul D.; Northen, Trent R.; Simmons, Blake A.; Singer, Steven W.] Lawrence Berkeley Natl Lab, Biosci Directorate, Berkeley, CA 94720 USA. [Deng, Kai] Sandia Natl Labs, Biol & Mat Sci Ctr, Livermore, CA USA. [Nicora, Carrie D.; Jacobs, Jon M.] Pacific Northwest Natl Lab, Div Biol Sci, Richland, WA USA. [Aldrich, Joshua T.; Robinson, Errol W.] Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA USA. [Frey, Dario] Univ Appl Sci Mannheim, Fac Biotechnol, Mannheim, Germany. RP Singer, SW (reprint author), Joint BioEnergy Inst, Emeryville, CA 94608 USA.; Singer, SW (reprint author), Lawrence Berkeley Natl Lab, Biosci Directorate, Berkeley, CA 94720 USA. EM SWSinger@lbl.gov OI Northen, Trent/0000-0001-8404-3259 FU Department of Energy Office of Biological and Environmental Research [DE-AC02-05CH11231, DE-AC05-76RLO 1830] FX This work, including the efforts of Jennifer Hiras, Yu-Wei Wu, Kai Deng, Dario Frey, Sebastian Kolinko, Paul Adams, Trent Northen, Blake Simmons, and Steven Singer, was funded by Department of Energy Office of Biological and Environmental Research (DE-AC02-05CH11231). This work, including the efforts of Carrie Nicora, Joshua Aldrich, Jon Jacobs, and Errol Robinson, was funded by Department of Energy Office of Biological and Environmental Research (DE-AC05-76RLO 1830). NR 52 TC 0 Z9 0 U1 9 U2 9 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD JUL-AUG PY 2016 VL 7 IS 4 AR e01106 DI 10.1128/mBio.01106-16 PG 9 WC Microbiology SC Microbiology GA DW1YQ UT WOS:000383440500059 ER PT J AU James, KL Rios-Hernandez, LA Wofford, NQ Mouttaki, H Sieber, JR Sheik, CS Nguyen, HH Yang, YN Xie, YM Erde, J Rohlin, L Karr, EA Loo, JA Loo, RRO Hurst, GB Gunsalus, RP Szweda, LI McInerney, MJ AF James, Kimberly L. Rios-Hernandez, Luis A. Wofford, Neil Q. Mouttaki, Housna Sieber, Jessica R. Sheik, Cody S. Nguyen, Hong H. Yang, Yanan Xie, Yongming Erde, Jonathan Rohlin, Lars Karr, Elizabeth A. Loo, Joseph A. Loo, Rachel R. Ogorzalek Hurst, Gregory B. Gunsalus, Robert P. Szweda, Luke I. McInerney, Michael J. TI Pyrophosphate-Dependent ATP Formation from Acetyl Coenzyme A in Syntrophus aciditrophicus, a New Twist on ATP Formation SO MBIO LA English DT Article ID ADENYLATE ENERGY-CHARGE; ESCHERICHIA-COLI; CYCLOHEXANE CARBOXYLATE; SKELETAL-MUSCLE; COA SYNTHETASE; BENZOATE; ENZYME; METABOLISM; FATTY; DEGRADATION AB Syntrophus aciditrophicus is a model syntrophic bacterium that degrades key intermediates in anaerobic decomposition, such as benzoate, cyclohexane-1-carboxylate, and certain fatty acids, to acetate when grown with hydrogen-/formate-consuming microorganisms. ATP formation coupled to acetate production is the main source for energy conservation by S. aciditrophicus. However, the absence of homologs for phosphate acetyltransferase and acetate kinase in the genome of S. aciditrophicus leaves it unclear as to how ATP is formed, as most fermentative bacteria rely on these two enzymes to synthesize ATP from acetyl coenzyme A (CoA) and phosphate. Here, we combine transcriptomic, proteomic, metabolite, and enzymatic approaches to show that S. aciditrophicus uses AMP-forming, acetyl-CoA synthetase (Acs1) for ATP synthesis from acetylCoA. acs1 mRNA and Acs1 were abundant in transcriptomes and proteomes, respectively, of S. aciditrophicus grown in pure culture and coculture. Cell extracts of S. aciditrophicus had low or undetectable acetate kinase and phosphate acetyltransferase activities but had high acetyl-CoA synthetase activity under all growth conditions tested. Both Acs1 purified from S. aciditrophicus and recombinantly produced Acs1 catalyzed ATP and acetate formation from acetyl-CoA, AMP, and pyrophosphate. High pyrophosphate levels and a high AMP-to-ATP ratio (5.9 +/- 1.4) in S. aciditrophicus cells support the operation of Acs1 in the acetate-forming direction. Thus, S. aciditrophicus has a unique approach to conserve energy involving pyrophosphate, AMP, acetyl-CoA, and an AMP-forming, acetyl-CoA synthetase. IMPORTANCE Bacteria use two enzymes, phosphate acetyltransferase and acetate kinase, to make ATP from acetyl-CoA, while acetate-forming archaea use a single enzyme, an ADP-forming, acetyl-CoA synthetase, to synthesize ATP and acetate from acetyl-CoA. Syntrophus aciditrophicus apparently relies on a different approach to conserve energy during acetyl-CoA metabolism, as its genome does not have homologs to the genes for phosphate acetyltransferase and acetate kinase. Here, we show that S. aciditrophicus uses an alternative approach, an AMP-forming, acetyl-CoA synthetase, to make ATP from acetyl-CoA. AMP-forming, acetyl-CoA synthetases were previously thought to function only in the activation of acetate to acetyl-CoA. C1 [James, Kimberly L.; Rios-Hernandez, Luis A.; Wofford, Neil Q.; Mouttaki, Housna; Sieber, Jessica R.; Sheik, Cody S.; Karr, Elizabeth A.; McInerney, Michael J.] Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. [Yang, Yanan; Xie, Yongming; Erde, Jonathan; Loo, Joseph A.] Univ Calif Los Angeles, Dept Chem & Biochem, 405 Hilgard Ave, Los Angeles, CA 90024 USA. [Nguyen, Hong H.; Loo, Joseph A.; Loo, Rachel R. Ogorzalek] Univ Calif Los Angeles, Dept Biol Chem, Los Angeles, CA 90024 USA. [Hurst, Gregory B.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN USA. [Rohlin, Lars; Gunsalus, Robert P.] Univ Calif Los Angeles, Dept Microbiol Immunol & Mol Genet, Los Angeles, CA USA. [Szweda, Luke I.] Oklahoma Med Res Fdn, Aging & Metab Res Program, 825 NE 13th St, Oklahoma City, OK 73104 USA. [Rios-Hernandez, Luis A.] Univ Puerto Rico, Dept Biol, Mayaguez, PR USA. [Sieber, Jessica R.] Univ Minnesota, Dept Biol, Duluth, MN 55812 USA. [Sheik, Cody S.] Univ Minnesota, Large Lakes Observ, Duluth, MN 55812 USA. [Sheik, Cody S.] Univ Minnesota, Dept Biol, Duluth, MN 55812 USA. [Yang, Yanan] Agilent Technol, Ctr Excellence, Santa Clara, CA USA. [Xie, Yongming] Zhang Jiang Hitech Pk, Shanghai, Peoples R China. [Rohlin, Lars] EASEL Biotechnol LLC, Culver City, CA USA. RP McInerney, MJ (reprint author), Univ Oklahoma, Dept Microbiol & Plant Biol, Norman, OK 73019 USA. EM mcinerney@ou.edu OI Sheik, Cody/0000-0003-0413-1924 FU HHS \ National Institutes of Health (NIH) [R01GM085402]; U.S. Department of Energy (DOE) [DE-FG02-96ER20214, DE-AC05-00OR22725]; U.S. Department of Energy Office of Science, Office of Biological and Environmental Research program [DE-FC02-02ER63421]; Department of Energy Biosciences Division [DE-FG02-08ER64689] FX This work, including the efforts of Joseph A. Loo and Rachel R. Ogorzalek Loo, was funded by HHS vertical bar National Institutes of Health (NIH) (R01GM085402). This work, including the efforts of Michael J. McInerney, was funded by U.S. Department of Energy (DOE) (DE-FG02-96ER20214). This work, including the efforts of Gregory B. Hurst, was funded by U.S. Department of Energy (DOE) (DE-AC05-00OR22725).; This work, including the efforts of Joseph A Loo, Rachel R. Ogorzalek Loo, and Robert P. Gunsalus, was supported by the U.S. Department of Energy Office of Science, Office of Biological and Environmental Research program under Award Number DE-FC02-02ER63421 for the UCLA-DOE Institute. This research, including the efforts of Robert P. Gunsalus, was funded by the Department of Energy Biosciences Division grant award DE-FG02-08ER64689. NR 33 TC 1 Z9 1 U1 5 U2 5 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD JUL-AUG PY 2016 VL 7 IS 4 AR e01208 DI 10.1128/mBio.01208-16 PG 8 WC Microbiology SC Microbiology GA DW1YQ UT WOS:000383440500070 ER PT J AU North, JA Sriram, J Chourey, K Ecker, CD Sharma, R Wildenthal, JA Hettich, RL Tabita, FR AF North, Justin A. Sriram, Jaya Chourey, Karuna Ecker, Christopher D. Sharma, Ritin Wildenthal, John A. Hettich, Robert L. Tabita, F. Robert TI Metabolic Regulation as a Consequence of Anaerobic 5-Methylthioadenosine Recycling in Rhodospirillum rubrum SO MBIO LA English DT Article ID METHIONINE SALVAGE PATHWAY; RUBISCO-LIKE PROTEIN; CARBOXYLASE/OXYGENASE (RUBISCO)-LIKE PROTEIN; BACILLUS-SUBTILIS; PHOTOSYNTHETIC RUBISCO; EVOLUTIONARY RELATIONSHIPS; MECHANISTIC DIVERSITY; BACTERIAL CHEMOTAXIS; CHLOROBIUM-TEPIDUM; SULFUR METABOLISM AB Rhodospirillum rubrum possesses a novel oxygen-independent, aerobic methionine salvage pathway (MSP) for recycling methionine from 5-methylthioadenosine (MTA), the MTA-isoprenoid shunt. This organism can also metabolize MTA as a sulfur source under anaerobic conditions, suggesting that the MTA-isoprenoid shunt may also function anaerobically as well. In this study, deep proteomics profiling, directed metabolite analysis, and reverse transcriptase quantitative PCR (RT-qPCR) revealed metabolic changes in response to anaerobic growth on MTA versus sulfate as sole sulfur source. The abundance of protein levels associated with methionine transport, cell motility, and chemotaxis increased in the presence of MTA over that in the presence of sulfate. Purine salvage from MTA resulted primarily in hypoxanthine accumulation and a decrease in protein levels involved in GMP-to-AMP conversion to balance purine pools. Acyl coenzyme A (acyl-CoA) metabolic protein levels for lipid metabolism were lower in abundance, whereas poly-beta-hydroxybutyrate synthesis and storage were increased nearly 10-fold. The known R. rubrum aerobic MSP was also shown to be upregulated, to function anaerobically, and to recycle MTA. This suggested that other organisms with gene homologues for the MTA-isoprenoid shunt may also possess a functioning anaerobic MSP. In support of our previous findings that ribulose-1,5-carboxylase/oxygenase (RubisCO) is required for an apparently purely anaerobic MSP, RubisCO transcript and protein levels both increased in abundance by over 10-fold in cells grown anaerobically on MTA over those in cells grown on sulfate, resulting in increased intracellular RubisCO activity. These results reveal for the first time global metabolic responses as a consequence of anaerobic MTA metabolism compared to using sulfate as the sulfur source. IMPORTANCE In nearly all organisms, sulfur-containing byproducts result from many metabolic reactions. Unless these compounds are further metabolized, valuable organic sulfur is lost and can become limiting. To regenerate the sulfur-containing amino acid methionine, organisms typically employ one of several variations of a "universal" methionine salvage pathway (MSP). A common aspect of the universal MSP is a final oxygenation step. This work establishes that the metabolically versatile bacterium Rhodospirillum rubrum employs a novel MSP that does not require oxygen under either aerobic or anaerobic conditions. There is also a separate, dedicated anaerobic MTA metabolic route in R. rubrum. This work reveals global changes in cellular metabolism in response to anaerobic MTA metabolism compared to using sulfate as a sulfur source. We found that cell mobility and transport were enhanced, along with lipid, nucleotide, and carbohydrate metabolism, when cells were grown in the presence of MTA. C1 [North, Justin A.; Sriram, Jaya; Ecker, Christopher D.; Wildenthal, John A.; Tabita, F. Robert] Ohio State Univ, Dept Microbiol, 484 W 12th Ave, Columbus, OH 43210 USA. [Chourey, Karuna; Hettich, Robert L.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN USA. [Sharma, Ritin] Univ Tennessee, ORNL Grad Sch Genome Sci & Technol, Knoxville, TN USA. [Sharma, Ritin] H Lee Moffitt Canc Ctr & Res Inst, Dept Mol Oncol, Tampa, FL USA. RP Tabita, FR (reprint author), Ohio State Univ, Dept Microbiol, 484 W 12th Ave, Columbus, OH 43210 USA. EM tabita.1@osu.edu OI , /0000-0002-9216-3813 FU HHS \ National Institutes of Health (NIH) [GM095742, F32GM109547] FX This work, including the efforts of F Robert Tabita, was funded by HHS vertical bar National Institutes of Health (NIH) (GM095742). This work, including the efforts of Justin A North, was funded by HHS vertical bar National Institutes of Health (NIH) (F32GM109547). NR 61 TC 0 Z9 0 U1 3 U2 3 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD JUL-AUG PY 2016 VL 7 IS 4 AR e00855-16 DI 10.1128/mBio.00855-16 PG 12 WC Microbiology SC Microbiology GA DW1YQ UT WOS:000383440500025 ER PT J AU Schaefer, AL Oda, Y Coutinho, BG Pelletier, DA Weiburg, J Venturi, V Greenberg, EP Harwood, CS AF Schaefer, Amy L. Oda, Yasuhiro Coutinho, Bruna Goncalves Pelletier, Dale A. Weiburg, Justin Venturi, Vittorio Greenberg, E. Peter Harwood, Caroline S. TI A LuxR Homolog in a Cottonwood Tree Endophyte That Activates Gene Expression in Response to a Plant Signal or Specific Peptides SO MBIO LA English DT Article ID BINDING CASSETTE TRANSPORTERS; ORYZAE PV. ORYZAE; POPULUS-DELTOIDES; XANTHOMONAS-ORYZAE; QUORUM; BACTERIA; RHIZOSPHERE; ENDOSPHERE; REGULATORS; MOLECULES AB Homologs of the LuxR acyl-homoserine lactone (AHL) quorum-sensing signal receptor are prevalent in Proteobacteria isolated from roots of the Eastern cottonwood tree, Populus deltoides. Many of these isolates possess an orphan LuxR homolog, closely related to OryR from the rice pathogen Xanthomonas oryzae. OryR does not respond to AHL signals but, instead, responds to an unknown plant compound. We discovered an OryR homolog, PipR, in the cottonwood endophyte Pseudomonas sp. strain GM79. The genes adjacent to pipR encode a predicted ATP-binding cassette (ABC) peptide transporter and peptidases. We purified the putative peptidases, PipA and AapA, and confirmed their predicted activities. A transcriptional pipA-gfp reporter was responsive to PipR in the presence of plant leaf macerates, but it was not influenced by AHLs, similar to findings with OryR. We found that PipR also responded to protein hydrolysates to activate pipA-gfp expression. Among many peptides tested, the tripeptide Ser-His-Ser showed inducer activity but at relatively high concentrations. An ABC peptide transporter mutant failed to respond to leaf macerates, peptone, or Ser-His-Ser, while peptidase mutants expressed higher-than-wild-type levels of pipA-gfp in response to any of these signals. Our studies are consistent with a model where active transport of a peptidelike signal is required for the signal to interact with PipR, which then activates peptidase gene expression. The identification of a peptide ligand for PipR sets the stage to identify plant-derived signals for the OryR family of orphan LuxR proteins. IMPORTANCE We describe the transcription factor PipR from a Pseudomonas strain isolated as a cottonwood tree endophyte. PipR is a member of the LuxR family of transcriptional factors. LuxR family members are generally thought of as quorumsensing signal receptors, but PipR is one of an emerging subfamily of LuxR family members that respond to compounds produced by plants. We found that PipR responds to a peptidelike compound, and we present a model for Pip system signal transduction. A better understanding of plant-responsive LuxR homologs and the compounds to which they respond is of general importance, as they occur in dozens of bacterial species that are associated with economically important plants and, as we report here, they also occur in members of certain root endophyte communities. C1 [Schaefer, Amy L.; Oda, Yasuhiro; Coutinho, Bruna Goncalves; Weiburg, Justin; Greenberg, E. Peter; Harwood, Caroline S.] Univ Washington, Seattle, WA 98195 USA. [Pelletier, Dale A.] Oak Ridge Natl Lab, Oak Ridge, TN USA. [Venturi, Vittorio] Int Ctr Genet Engn & Biotechnol, Trieste, Italy. RP Harwood, CS (reprint author), Univ Washington, Seattle, WA 98195 USA. EM csh5@uw.edu FU Department of Energy (BER) Genomic Science Program [DE-AC05-00OR22725]; Genomic Science Program, U.S. Department of Energy, Office of Science, Biological and Environmental Research, as part of the Plant Microbe Interfaces Scientific Focus Area; U.S. Department of Energy [DE-AC05-00OR22725] FX This work, including the efforts of Amy L. Schaefer, Yasuhiro Oda, Bruna Goncalves Coutinho, Dale A. Pelletier, Justin Weiburg, Everett Peter Greenberg, and Caroline S. Harwood, was funded by Department of Energy (BER) Genomic Science Program (DE-AC05-00OR22725).; This research was sponsored by the Genomic Science Program, U.S. Department of Energy, Office of Science, Biological and Environmental Research, as part of the Plant Microbe Interfaces Scientific Focus Area (http://pmi.ornl.gov). Oak Ridge National Laboratory is managed by UT-Battelle LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725. NR 44 TC 0 Z9 0 U1 12 U2 12 PU AMER SOC MICROBIOLOGY PI WASHINGTON PA 1752 N ST NW, WASHINGTON, DC 20036-2904 USA SN 2150-7511 J9 MBIO JI mBio PD JUL-AUG PY 2016 VL 7 IS 4 AR e01101 DI 10.1128/mBio.01101-16 PG 8 WC Microbiology SC Microbiology GA DW1YQ UT WOS:000383440500058 ER PT J AU Taylor, SG Raby, EY Farinholt, KM Park, G Todd, MD AF Taylor, Stuart G. Raby, Eric Y. Farinholt, Kevin M. Park, Gyuhae Todd, Michael D. TI Active-sensing platform for structural health monitoring: Development and deployment SO STRUCTURAL HEALTH MONITORING-AN INTERNATIONAL JOURNAL LA English DT Article DE embedded sensing; sensor diagnostics; multi-scale sensing; active-sensing; electromechanical impedance ID WIRELESS SENSOR NODE; TURBINE ROTOR BLADE; CRACK DETECTION; DIAGNOSTICS AB Embedded sensing for structural health monitoring is a rapidly expanding field, propelled by algorithmic advances in structural health monitoring and the ever-shrinking size and cost of electronic hardware necessary for its implementation. Although commercial systems are available to perform the relevant tasks, they are usually bulky and/or expensive because of their high degree of general utility to a wider range of applications. As a result, multiple separate devices may be required in order to obtain the same results that could be obtained with a structural health monitoring-specific device. This work presents the development and deployment of a versatile, Wireless Active-Sensing Platform, designed for the particular needs of embedded sensing for multi-scale structural health monitoring. The Wireless Active-Sensing Platform combines a conventional data acquisition ability to record voltage output (e.g. from strain or acceleration transducers) with ultrasonic guided wave-based active-sensing, and a seamlessly integrated impedance measurement mode, enabling impedance-based structural health monitoring and piezoelectric sensor diagnostics to reduce the potential for false positives in damage identification. The motivation, capabilities, and hardware design for the Wireless Active-Sensing Platform are reviewed, and three deployment examples are presented, each demonstrating an important aspect of embedded sensing for structural health monitoring. C1 [Taylor, Stuart G.; Raby, Eric Y.; Farinholt, Kevin M.] Los Alamos Natl Lab, Engn Inst, Los Alamos, NM USA. [Park, Gyuhae] Chonnam Natl Univ, Sch Mech Engn, Gwangju 505707, South Korea. [Todd, Michael D.] Univ Calif San Diego, Jacobs Sch Engn, Dept Struct Engn, La Jolla, CA 92093 USA. RP Park, G (reprint author), Chonnam Natl Univ, Sch Mech Engn, Gwangju 505707, South Korea. EM gpark@jnu.ac.kr OI Raby, Eric/0000-0002-5690-5867 FU Department of Energy through the Laboratory Directed Research and Development program at Los Alamos National Laboratory; Leading Foreign Research Institute Recruitment Program through the National Research Foundation of Korea - Ministry of Education, Science and Technology [2011-0030065]; Defense Acquisition Program Administration; Agency for Defense Development [UD130058JD] FX The author(s) disclosed receipt of the following financial support for the research, authorship, and/or publication of this article: The research was funded by the Department of Energy through the Laboratory Directed Research and Development program at Los Alamos National Laboratory. This research was partially supported by the Leading Foreign Research Institute Recruitment Program through the National Research Foundation of Korea funded by the Ministry of Education, Science and Technology (2011-0030065). This research was also partially supported by the financial support provided by Defense Acquisition Program Administration and Agency for Defense Development under the contract UD130058JD. NR 28 TC 0 Z9 0 U1 2 U2 2 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 1475-9217 EI 1741-3168 J9 STRUCT HEALTH MONIT JI Struct. Health Monit. PD JUL PY 2016 VL 15 IS 4 BP 413 EP 422 DI 10.1177/1475921716642171 PG 10 WC Engineering, Multidisciplinary; Instruments & Instrumentation SC Engineering; Instruments & Instrumentation GA DV5PC UT WOS:000382979100004 ER PT J AU Premke, K Attermeyer, K Augustin, J Cabezas, A Casper, P Deumlich, D Gelbrecht, J Gerke, HH Gessler, A Grossart, HP Hilt, S Hupfer, M Kalettka, T Kayler, Z Lischeid, G Sommer, M Zak, D AF Premke, Katrin Attermeyer, Katrin Augustin, Juergen Cabezas, Alvaro Casper, Peter Deumlich, Detlef Gelbrecht, Joerg Gerke, Horst H. Gessler, Arthur Grossart, Hans-Peter Hilt, Sabine Hupfer, Michael Kalettka, Thomas Kayler, Zachary Lischeid, Gunnar Sommer, Michael Zak, Dominik TI The importance of landscape diversity for carbon fluxes at the landscape level: small-scale heterogeneity matters SO WILEY INTERDISCIPLINARY REVIEWS-WATER LA English DT Article ID DISSOLVED ORGANIC-CARBON; GREENHOUSE-GAS BALANCE; CLIMATE-CHANGE MITIGATION; NITROUS-OXIDE EMISSION; TEMPERATE FOREST SOIL; TERRESTRIAL CARBON; METHANE EMISSIONS; BOREAL LAKES; KETTLE HOLES; HYDROELECTRIC RESERVOIRS AB Landscapes can be viewed as spatially heterogeneous areas encompassing terrestrial and aquatic domains. To date, most landscape carbon (C) fluxes have been estimated by accounting for terrestrial ecosystems, while aquatic ecosystems have been largely neglected. However, a robust assessment of C fluxes on the landscape scale requires the estimation of fluxes within and between both landscape components. Here, we compiled data from the literature on C fluxes across the air-water interface from various landscape components. We simulated C emissions and uptake for five different scenarios which represent a gradient of increasing spatial heterogeneity within a temperate young moraine landscape: (I) a homogeneous landscape with only cropland and large lakes; (II) separation of the terrestrial domain into cropland and forest; (III) further separation into cropland, forest, and grassland; (IV) additional division of the aquatic area into large lakes and peatlands; and (V) further separation of the aquatic area into large lakes, peatlands, running waters, and small water bodies These simulations suggest that C fluxes at the landscape scale might depend on spatial heterogeneity and landscape diversity, among other factors. When we consider spatial heterogeneity and diversity alone, small inland waters appear to play a pivotal and previously underestimated role in landscape greenhouse gas emissions that may be regarded as C hot spots. Approaches focusing on the landscape scale will also enable improved projections of ecosystems' responses to perturbations, e.g., due to global change and anthropogenic activities, and evaluations of the specific role individual landscape components play in regional C fluxes. (C) 2016 The Authors. WIREs Water published by Wiley Periodicals, Inc. C1 [Premke, Katrin; Attermeyer, Katrin; Cabezas, Alvaro; Gelbrecht, Joerg; Hilt, Sabine; Hupfer, Michael; Zak, Dominik] Leibniz Inst Freshwater Ecol & Inland Fisheries I, Chem Analyt & Biogeochem, Berlin, Germany. [Premke, Katrin; Augustin, Juergen; Gessler, Arthur; Kayler, Zachary] Leibniz Ctr Agr Landscape Res ZALF, Inst Landscape Biogeochem, Muncheberg, Germany. [Casper, Peter; Grossart, Hans-Peter] Leibniz Inst Freshwater Ecol & Inland Fisheries I, Expt Limnol, Berlin, Germany. [Deumlich, Detlef; Gerke, Horst H.; Sommer, Michael] Leibniz Ctr Agr Landscape Res ZALF, Inst Soil Landscape, Muncheberg, Germany. [Gessler, Arthur] Swiss Fed Inst Forest Snow & Landscape Res WSL, Birmensdorf, Switzerland. [Grossart, Hans-Peter] Univ Potsdam, Inst Biochem & Biol, Potsdam, Germany. [Kalettka, Thomas; Lischeid, Gunnar] Leibniz Ctr Agr Landscape Res ZALF, Inst Landscape Hydrol, Muncheberg, Germany. [Kayler, Zachary] US Forest Serv, USDA, Northern Res Stn, Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Lischeid, Gunnar; Sommer, Michael] Univ Potsdam, Inst Earth & Environm Sci, Potsdam, Germany. [Zak, Dominik] Aarhus Univ, Dept Biosci, Aarhus, Denmark. RP Premke, K (reprint author), Leibniz Inst Freshwater Ecol & Inland Fisheries I, Chem Analyt & Biogeochem, Berlin, Germany.; Premke, K (reprint author), Leibniz Ctr Agr Landscape Res ZALF, Inst Landscape Biogeochem, Muncheberg, Germany. EM premke@igb-berlin.de RI Gessler, Arthur/C-7121-2008 OI Gessler, Arthur/0000-0002-1910-9589 NR 156 TC 1 Z9 1 U1 13 U2 13 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA EI 2049-1948 J9 WIRES-WATER JI Wiley Interdiscip. Rev.-Water PD JUL-AUG PY 2016 VL 3 IS 4 BP 601 EP 617 DI 10.1002/wat2.1147 PG 17 WC Water Resources SC Water Resources GA DV4DH UT WOS:000382874800009 ER PT J AU Mittal, S AF Mittal, Sparsh TI A Survey of Architectural Techniques for Near-Threshold Computing SO ACM JOURNAL ON EMERGING TECHNOLOGIES IN COMPUTING SYSTEMS LA English DT Article DE Review; classification; near-threshold voltage computing (NT) (NTV) (NTC); low-voltage; voltage scaling; cache; memory; reliability; hard-error ID CACHE; VOLTAGE; OPERATION; SYSTEMS; DESIGN; AREA; SRAM; ECC AB Energy efficiency has now become the primary obstacle in scaling the performance of all classes of computing systems. Low-voltage computing, specifically, near-threshold voltage computing (NTC), which involves operating the transistor very close to and yet above its threshold voltage, holds the promise of providing many-fold improvement in energy efficiency. However, use of NTC also presents several challenges such as increased parametric variation, failure rate, and performance loss. This article surveys several recent techniques that aim to offset these challenges for fully leveraging the potential of NTC. By classifying these techniques along several dimensions, we also highlight their similarities and differences. It is hoped that this article will provide insights into state-of-the-art NTC techniques to researchers and system designers and inspire further research in this field. C1 [Mittal, Sparsh] Oak Ridge Natl Lab, Future Technol Grp, 1 Bethel Valley Rd,Bldg 5100,MS-6173, Oak Ridge, TN 37830 USA. RP Mittal, S (reprint author), Oak Ridge Natl Lab, Future Technol Grp, 1 Bethel Valley Rd,Bldg 5100,MS-6173, Oak Ridge, TN 37830 USA. EM mittals@ornl.gov OI Mittal, Sparsh/0000-0002-2908-993X FU U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research FX Support for this work was provided by the U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research. NR 75 TC 0 Z9 0 U1 1 U2 1 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 1550-4832 EI 1550-4840 J9 ACM J EMERG TECH COM JI ACM J. Emerg. Technol. Comput. Syst. PD JUL PY 2016 VL 12 IS 4 AR 46 DI 10.1145/2821510 PG 26 WC Computer Science, Hardware & Architecture; Engineering, Electrical & Electronic; Nanoscience & Nanotechnology SC Computer Science; Engineering; Science & Technology - Other Topics GA DT4AE UT WOS:000381421500016 ER PT J AU Mittal, S AF Mittal, Sparsh TI A Survey of Techniques for Cache Locking SO ACM TRANSACTIONS ON DESIGN AUTOMATION OF ELECTRONIC SYSTEMS LA English DT Article DE Review; classification; cache locking; worst-case execution time (WCET); hard real-time system; cache partitioning; multitasking; CPU; GPU ID INSTRUCTION CACHES; EMBEDDED SYSTEMS; LEVEL AB Cache memory, although important for boosting application performance, is also a source of execution time variability, and this makes its use difficult in systems requiring worst-case execution time (WCET) guarantees. Cache locking is a promising approach for simplifying WCET estimation and providing predictability, and hence, several commercial processors provide ability for locking cache. However, cache locking also has several disadvantages (e.g., extra misses for unlocked blocks, complex algorithms required for selection of locking contents) and hence, a careful management is required to realize the full potential of cache locking. In this article, we present a survey of techniques proposed for cache locking. We categorize the techniques into several groups to underscore their similarities and differences. We also discuss the opportunities and obstacles in using cache locking. We hope that this article will help researchers gain insight into cache locking schemes and will also stimulate further work in this area. C1 [Mittal, Sparsh] Oak Ridge Natl Lab, 1 Bethel Valley Rd,Bldg 5100, Oak Ridge, TN 37830 USA. RP Mittal, S (reprint author), Oak Ridge Natl Lab, 1 Bethel Valley Rd,Bldg 5100, Oak Ridge, TN 37830 USA. EM mittals@ornl.gov FU U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research FX Support for this work was provided by the U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research. NR 62 TC 0 Z9 0 U1 0 U2 0 PU ASSOC COMPUTING MACHINERY PI NEW YORK PA 2 PENN PLAZA, STE 701, NEW YORK, NY 10121-0701 USA SN 1084-4309 EI 1557-7309 J9 ACM T DES AUTOMAT EL JI ACM Transact. Des. Automat. Electron. Syst. PD JUL PY 2016 VL 21 IS 3 AR 49 DI 10.1145/2858792 PG 24 WC Computer Science, Hardware & Architecture; Computer Science, Software Engineering SC Computer Science GA DT4BD UT WOS:000381424000014 ER PT J AU Koch, V Bzdak, A AF Koch, Volker Bzdak, Adam TI FLUCTUATIONS AND THE QCD PHASE DIAGRAM SO ACTA PHYSICA POLONICA B LA English DT Article ID QUARK; PLASMA; ORDER; TIME AB In this contribution, we will discuss how the study of various fluctuation observables may be used to explore the phase diagram of the strong interaction. We will briefly summarize the present study of experimental and theoretical research in this area. We will then discuss various corrections and issues which need to be understood and applied for a meaningful comparison of experimental measurements with theoretical predictions. C1 [Koch, Volker] Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Bzdak, Adam] AGH Univ Sci & Technol, Fac Phys & Appl Comp Sci, PL-30059 Krakow, Poland. RP Koch, V (reprint author), Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. FU U.S. Department of Energy [DE-AC02-05CH11231]; Polish Ministry of Science and Higher Education (MNiSW); Polish National Science Centre (Narodowe Centrum Nauki) [DEC-2014/15/B/ST2/00175, DEC-2013/09/B/ST2/00497] FX This work is supported by the Director, Office of Energy Research, Office of High Energy and Nuclear Physics, Divisions of Nuclear Physics of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, and by the Polish Ministry of Science and Higher Education (MNiSW), by founding from the Foundation for Polish Science, and by the Polish National Science Centre (Narodowe Centrum Nauki), Grant No. DEC-2014/15/B/ST2/00175 and in part by DEC-2013/09/B/ST2/00497. NR 51 TC 0 Z9 0 U1 0 U2 0 PU JAGIELLONIAN UNIV PRESS PI KRAKOW PA UL MICHALOWSKIEGO 9-2, KRAKOW, 31126, POLAND SN 0587-4254 EI 1509-5770 J9 ACTA PHYS POL B JI Acta Phys. Pol. B PD JUL PY 2016 VL 47 IS 7 BP 1867 EP 1882 DI 10.5506/APhysPolB.47.1867 PG 16 WC Physics, Multidisciplinary SC Physics GA DV3OZ UT WOS:000382833700007 ER PT J AU McLerran, L AF McLerran, Larry TI ANDRZEJ BIALAS: SOME SHORT STORIES SO ACTA PHYSICA POLONICA B LA English DT Article ID HIGH-ENERGIES; NUCLEUS COLLISIONS AB In anecdotal fashion, I discuss some of the contributions of Andrzej Bialas to science and the education of young scientists. C1 [McLerran, Larry] Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA. [McLerran, Larry] Cent China Normal Univ, Wuhan, Peoples R China. RP McLerran, L (reprint author), Brookhaven Natl Lab, Dept Phys, Upton, NY 11973 USA.; McLerran, L (reprint author), Cent China Normal Univ, Wuhan, Peoples R China. FU U.S. Department of Energy [DE-SC0012704] FX This talk was given to celebrate the 80th birthday of in Krakow, Poland, July, 2016. My wife and I thank Andrzej for the friendship and hospitality he has given to both of us during many visits to Poland, and most important, for his friendship. I gratefully acknowledge Michal Praszalowicz, who organized this meeting, and invited me to give this talk. This manuscript has been authorized under Contract No. DE-SC0012704 with the U.S. Department of Energy. NR 5 TC 0 Z9 0 U1 0 U2 0 PU JAGIELLONIAN UNIV PRESS PI KRAKOW PA UL MICHALOWSKIEGO 9-2, KRAKOW, 31126, POLAND SN 0587-4254 EI 1509-5770 J9 ACTA PHYS POL B JI Acta Phys. Pol. B PD JUL PY 2016 VL 47 IS 7 BP 1993 EP 1997 DI 10.5506/APhysPolB.47.1993 PG 5 WC Physics, Multidisciplinary SC Physics GA DV3OZ UT WOS:000382833700014 ER PT J AU Samanta, A Weinan, E AF Samanta, Amit Weinan, E. TI Interfacial diffusion aided deformation during nanoindentation SO AIP ADVANCES LA English DT Article ID DISLOCATION NUCLEATION; INCIPIENT PLASTICITY; MICRO-INDENTATION; DEPTH DEPENDENCE; FREE-ENERGY; MECHANISMS; CRYSTALS; SURFACES; VOLUME; CREEP AB Nanoindentation is commonly used to quantify the mechanical response of material surfaces. Despite its widespread use, a detailed understanding of the deformation mechanisms responsible for plasticity during these experiments has remained elusive. Nanoindentation measurements often show stress values close to a material's ideal strength which suggests that dislocation nucleation and subsequent dislocation activity dominates the deformation. However, low strain-rate exponents and small activation volumes have also been reported which indicates high temperature sensitivity of the deformation processes. Using an order parameter aided temperature accelerated sampling technique called adiabatic free energy dynamics [J. B. Abrams and M. E. Tuckerman, J. Phys. Chem. B, 112, 15742 (2008)], and molecular dynamics we have probed the diffusive mode of deformation during nanoindentation. Localized processes such as surface vacancy and ad-atom pair formation, vacancy diffusion are found to play an important role during indentation. Our analysis suggests a change in the dominant deformation mode from dislocation mediated plasticity to diffusional flow at high temperatures, slow indentation rates and small indenter tip radii. (C) 2016 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/). C1 [Samanta, Amit] Lawrence Livermore Natl Lab, Div Phys, Livermore, CA 94550 USA. [Weinan, E.] Peking Univ, BICMR, Beijing, Peoples R China. [Weinan, E.] Peking Univ, BICMR, Beijing, Peoples R China. [Weinan, E.] Peking Univ, Sch Math Sci, Beijing, Peoples R China. [Weinan, E.] Princeton Univ, Dept Math, Princeton, NJ 08544 USA. [Weinan, E.] Princeton Univ, Program Appl & Computat Math, Princeton, NJ 08544 USA. RP Weinan, E (reprint author), Peking Univ, BICMR, Beijing, Peoples R China.; Weinan, E (reprint author), Peking Univ, Sch Math Sci, Beijing, Peoples R China.; Weinan, E (reprint author), Princeton Univ, Dept Math, Princeton, NJ 08544 USA.; Weinan, E (reprint author), Princeton Univ, Program Appl & Computat Math, Princeton, NJ 08544 USA. EM weinan@math.princeton.edu FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344]; U.S. Department of Energy [DE-SC0009248]; Office of Naval Research [N00014-13-1-0338] FX A. S. wishes to thank Andrew Lange and Ju Li for critical comments. This work was partially performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. The work by A. S and W. E at Princeton was supported by the U.S. Department of Energy (DE-SC0009248) and by the Office of Naval Research (N00014-13-1-0338). NR 26 TC 1 Z9 1 U1 11 U2 11 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2158-3226 J9 AIP ADV JI AIP Adv. PD JUL PY 2016 VL 6 IS 7 AR 075002 DI 10.1063/1.4958299 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DU7OF UT WOS:000382403600002 ER PT J AU Sturtevant, BT Pantea, C Sinha, DN AF Sturtevant, Blake T. Pantea, Cristian Sinha, Dipen N. TI Measured sound speeds and acoustic nonlinearity parameter in liquid water up to 523 K and 14 MPa SO AIP ADVANCES LA English DT Article ID EQUATION-OF-STATE; BIOLOGICAL MEDIA; B/A MEASUREMENT; PRESSURE; FLUIDS AB Sound speed in liquid water at temperatures between 275 and 523 K and pressures up to 14 MPa were experimentally determined using a high temperature/high pressure capable acoustic resonance cell. The measurements enabled the determination of the temperature and pressure dependence of sound speed and thus the parameter of acoustic nonlinearly, B/A, over this entire P-T space. Most of the sound speeds measured in this work were found to be within 0.4% of the IAPWS-IF97 formulation, an international standard for calculating sound speed in water as a function of temperature and pressure. The values for B/A determined at laboratory ambient pressure and at temperatures up to 356 K, were found to be in general agreement with values calculated from the IAPWS-IF97 formulation. Additionally, B/A at 293 K was found to be 4.6, in agreement with established literature values. (C) 2016 Author(s). C1 [Sturtevant, Blake T.; Pantea, Cristian; Sinha, Dipen N.] Los Alamos Natl Lab, Mat Phys & Applicat, Los Alamos, NM 87545 USA. RP Sturtevant, BT (reprint author), Los Alamos Natl Lab, Mat Phys & Applicat, Los Alamos, NM 87545 USA. EM bsturtev@lanl.gov RI Pantea, Cristian/D-4108-2009; OI Pantea, Cristian/0000-0002-0805-8923 FU U.S. DOE [AID 18832] FX This work was supported by the U.S. DOE under award # AID 18832. The authors thank Eric Chisolm of Los Alamos National Laboratory for valuable discussions. NR 23 TC 1 Z9 1 U1 2 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2158-3226 J9 AIP ADV JI AIP Adv. PD JUL PY 2016 VL 6 IS 7 AR 075310 DI 10.1063/1.4959196 PG 11 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DU7OF UT WOS:000382403600078 ER PT J AU Zhang, SJ Zhao, K Yu, XH Zhu, JL Liu, QQ Wang, XC Feng, SM Chen, ZQ Zhao, YS Jin, CQ AF Zhang, Sijia Zhao, Kan Yu, Xiaohui Zhu, Jinlong Liu, Qingqing Wang, Xiancheng Feng, Shaomin Chen, Zhiqiang Zhao, Yusheng Jin, Changqing TI Pressure-induced shift of T-c and structural transition in "122" type pnictide superconductor Ca0.34Na0.66Fe2As2 SO AIP ADVANCES LA English DT Article ID 43 K; IRON; NA1-XFEAS; COMPOUND AB The effect of pressure on superconductivity of "122" type Ca1-xNaxFe2As2 (x=0.66) single crystal is investigated through the temperature dependence of resistance measurement. Optimal Na doped (Ca0.34Na0.66)Fe2As2 shows a superconducting transition with T-c similar to 33 K at ambient pressure. With application of pressure, T-c decreases nearly linearly with dT(c)/d(P) similar to -1.7K/GPa at pressures lower than 2 GPa, and disappears gradually at higher pressure. The disappearance of superconductivity is also companied with the recovery of standard Fermi liquid behaviors of the normal-state transport properties. Moreover, (Ca0.34Na0.66)Fe2As2 exhibits a tetragonal (T) to collapsed-tetragonal (cT) transition at about 3 GPa. The evolution of non-Fermi liquid behaviors and superconductivity under pressure are both related to the interband fluctuations. (C) 2016 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/). C1 [Zhang, Sijia; Zhao, Kan; Yu, Xiaohui; Liu, Qingqing; Wang, Xiancheng; Feng, Shaomin; Jin, Changqing] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Yu, Xiaohui; Zhao, Yusheng] Los Alamos Natl Lab, Los Alamos Neutron Sci Ctr LANSCE, Los Alamos, NM 87545 USA. [Zhu, Jinlong] Univ Nevada, High Pressure Sci & Engn Ctr, Las Vegas, NV 89154 USA. [Chen, Zhiqiang] Brookhaven Natl Lab, Natl Synchrotron Light Source, Upton, NY 11973 USA. RP Zhang, SJ; Jin, CQ (reprint author), Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. EM sjzhang@iphy.ac.cn; jin@iphy.ac.cn FU NSF; MOST of China FX This work is supported by NSF and MOST of China through research projects. NR 47 TC 0 Z9 0 U1 6 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2158-3226 J9 AIP ADV JI AIP Adv. PD JUL PY 2016 VL 6 IS 7 AR 075104 DI 10.1063/1.4958873 PG 8 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DU7OF UT WOS:000382403600029 ER PT J AU Johnson, JR Bell, JF Bender, S Blaney, D Cloutis, E Ehliviann, B Fraeman, A Gasnault, O Kinch, K Le Mouelic, S Maurice, S Rampe, E Vaniman, D Wiens, RC AF Johnson, Jeffrey R. Bell, James F., III Bender, Steve Blaney, Diana Cloutis, Edward Ehliviann, Bethany Fraeman, Abigail Gasnault, Olivier Kinch, Kjartan Le Mouelic, Stephane Maurice, Sylvestre Rampe, Elizabeth Vaniman, David Wiens, Roger C. TI Constraints on iron sulfate and iron oxide mineralogy from ChemCam visible/near-infrared reflectance spectroscopy of Mt. Sharp basal units, Gale Crater, Mars SO AMERICAN MINERALOGIST LA English DT Article DE Mars spectroscopy; Mars remote sensing; visible/near-infrared; IR spectroscopy; ferric sulfates; iron oxides; Invited Centennial article ID PATHFINDER LANDING SITE; YELLOWKNIFE BAY; SPECTRAL CHARACTERISTICS; INSTRUMENT SUITE; CLAY-MINERALS; ROVER; EXPLORATION; SURFACE; ANALOG; ROCKS AB Relative reflectance point spectra (400-840 nm) were acquired by the Chemistry and Camera (ChemCam) instrument on the Mars Science Laboratory (MSL) rover Curiosity in passive mode (no laser) of drill tailings and broken rock fragments near the rover as it entered the lower reaches of Mt. Sharp and of landforms at distances of 2-8 km. Freshly disturbed surfaces are less subject to the spectral masking effects of dust, and revealed spectral features consistent with the presence of iron oxides and ferric sulfates. We present the first detection on Mars of a similar to 433 nm absorption band consistent with small abundances of ferric sulfates, corroborated by jarosite detections by the Chemistry and Mineralogy (CheMin) X-ray diffraction instrument in the Mojave, Telegraph Peak, and Confidence Hills drilled samples. Disturbed materials near the Bonanza King region also exhibited strong 433 nm bands and negative near-infrared spectral slopes consistent with jarosite. ChemCam passive spectra of the Confidence Hills and Mojave drill tailings showed features suggestive of the crystalline hematite identified by CheMin analyses. The Windjana drill sample tailings exhibited flat, low relative reflectance spectra, explained by the occurrence of magnetite detected by CheMin. Passive spectra of Bonanza King were similar, suggesting the presence of spectrally dark and neutral minerals such as magnetite. Long-distance spectra of the "Hematite Ridge" feature (3-5 km from the rover) exhibited features consistent with crystalline hematite. The Bagnold dune field north of the Hematite Ridge area exhibited low relative reflectance and near-infrared features indicative of basaltic materials (olivine, pyroxene). Light-toned layers south of Hematite Ridge lacked distinct spectral features in the 400-840 nm region, and may represent portions of nearby clay minerals and sulfates mapped with orbital near-infrared observations. The presence of ferric sulfates such as jarosite in the drill tailings suggests a relatively acidic environment, likely associated with flow of iron-bearing fluids, associated oxidation, and/or hydrothermal leaching of sedimentary rocks. Combined with other remote sensing data sets, mineralogical constraints from ChemCam passive spectra will continue to play an important role in interpreting the mineralogy and composition of materials encountered as Curiosity traverses further south within the basal layers of the Mt. Sharp complex. C1 [Johnson, Jeffrey R.] Johns Hopkins Univ, Appl Phys Lab, 11101 Johns Hopkins Rd 200-W230, Laurel, MD 20723 USA. [Bell, James F., III] Arizona State Univ, Sch Earth & Space Explorat, POB 871404, Tempe, AZ 85287 USA. [Bender, Steve; Vaniman, David] Planetary Sci Inst, 1700 East Ft Lowell,Suite 106, Tucson, AZ 85719 USA. [Blaney, Diana; Ehliviann, Bethany] Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Cloutis, Edward] Univ Winnipeg, 515 Portage Ave, Winnipeg, MB R3B 2E9, Canada. [Ehliviann, Bethany; Fraeman, Abigail] CALTECH, 1200 E Calif Blvd, Pasadena, CA 91125 USA. [Gasnault, Olivier; Maurice, Sylvestre] Univ Toulouse, Inst Rech Astrophys & Planetol, CNRS, 9 Ave Colonel Roche, F-31400 Toulouse, France. [Kinch, Kjartan] Univ Copenhagen, Niels Bohr Inst, Norregade 10,POB 2177, DK-1017 Copenhagen K, Denmark. [Le Mouelic, Stephane] Univ Nantes, Lab Planetol & Geodynam, 2,Rue Houssiniere,BP 92208 44322, Nantes 3, France. [Wiens, Roger C.] Los Alamos Natl Lab, POB 166, Los Alamos, NM 87545 USA. [Rampe, Elizabeth] Johnson Space Ctr, 2101 NASA Rd 1, Houston, TX 77058 USA. RP Johnson, JR (reprint author), Johns Hopkins Univ, Appl Phys Lab, 11101 Johns Hopkins Rd 200-W230, Laurel, MD 20723 USA. EM jeffrey.r.johnson@jhuapl.edu RI Kinch, Kjartan/C-5742-2015 OI Kinch, Kjartan/0000-0002-4629-8880 FU NASA Mars Science Laboratory Participating Scientist program through the Jet Propulsion Laboratory [1350588]; NASA's Mars Exploration Program; Centre National d'Etudes Spatiales (CNES); Danish Council for Independent Research/Natural Sciences (FNU grant) [12-127126]; Keck Institute for Space Studies; Caltech GPS division Texaco postdoctoral fellowships FX This work was funded by the NASA Mars Science Laboratory Participating Scientist program through the Jet Propulsion Laboratory (contract 1350588). The U.S. portion of ChemCam and MSL rover operations was funded by NASA's Mars Exploration Program. The French contribution to MSL is supported by the Centre National d'Etudes Spatiales (CNES). Work by K. Kinch was supported by the Danish Council for Independent Research/Natural Sciences (FNU grant 12-127126). A. Fraeman is supported by Keck Institute for Space Studies and Caltech GPS division Texaco postdoctoral fellowships. The authors thank W. Farrand and an anonymous reviewer for their helpful suggestions, and to J. Bishop for valuable editorial recommendations. Relative reflectance spectra used in Figures 10, 14, and 15 are available as supplemental material1. NR 89 TC 3 Z9 3 U1 17 U2 17 PU MINERALOGICAL SOC AMER PI CHANTILLY PA 3635 CONCORDE PKWY STE 500, CHANTILLY, VA 20151-1125 USA SN 0003-004X EI 1945-3027 J9 AM MINERAL JI Am. Miner. PD JUL-AUG PY 2016 VL 101 IS 7-8 BP 1501 EP 1514 DI 10.2138/am-2016-5553 PG 14 WC Geochemistry & Geophysics; Mineralogy SC Geochemistry & Geophysics; Mineralogy GA DT4KW UT WOS:000381450500003 ER PT J AU DeAngelis, MT Labotka, TC Fayek, M Cole, DR Anovitz, LM AF DeAngelis, Michael T. Labotka, Theodore C. Fayek, Mostafa Cole, David R. Anovitz, Lawrence M. TI Oxygen diffusion and exchange in dolomite rock at 700 degrees C, 100 MPa SO AMERICAN MINERALOGIST LA English DT Article DE Dolomite; oxygen isotope; exchange; diffusion; contact metamorphism; SIMS ID FLUID-FLOW; ISOTOPE-EXCHANGE; CONTACT AUREOLE; STABLE-ISOTOPES; ALTA AUREOLE; CALCITE; TRANSPORT; UTAH; INFILTRATION; METAMORPHISM AB In contact-metamorphic environments dolomite commonly breaks down to calcite + periclase + CO2 as a result of the infiltration of H2O. The transport and exchange of oxygen in dolomite rock during the breakdown reaction were examined experimentally by reacting a cylindrical core of Reed Dolomite with isotopically enriched water having the composition (HDO0.5O0.5)-O-18-O-16 at 700 degrees C and 100 MPa for 29 days. Reaction products formed along grain boundaries, fractures, and on the outside surface of the core. Some dolomite grains became enriched in Fe as a result of replacement of the host dolomite. Extensive voids are found in the grain boundaries as a result of the similar to 25% loss in solid volume during reaction. There are also pores, similar to 1 mu m in diameter, in the dolomite, notably in the vicinity of the replaced dolomite. The distribution of O-18 in the dolomite and reaction products was used as a tracer of the transport and exchange of 0 during reaction. Electron probe microanalysis (EPMA) and secondary ion mass spectrometry (SIMS) analyses showed pervasive infiltration of fluid along grain boundaries and fractures, growth and isotopic exchange with products of reaction, and diffusion of O-18 into dolomite grains. The fluid infiltrated efficiently along grain boundaries to the dolomite grain surface. The host dolomite shows an enrichment in O-18 along grain boundaries, indicating a diffusive exchange with the fluid. An estimate of the diffusion coefficient of oxygen in dolomite, determined from ion probe spot analyses, gives D approximate to 1 x 10(-12) mm(2)/s. This value is comparable to the oxygen diffusion coefficient for calcite in an H2O-rich fluid. Mass balance of 0 in the experiment (including dolomite fluid exchange, the amounts of neomorphic reaction products, and the fluid components) indicates that the reaction products have a O-18 concentration only about half that of the fluid. Ion probe spot analyses of calcite from both the center and the edge of the core have the fraction F=O-18(O-18+O-16) of 0.14 +/- 0.1, whereas the value calculated for the fluid is 0.31. The measured F values of calcite are intermediate between the initial F values of starting water and dolomite, indicating that the reaction products record a mix of both dolomite- and fluid-derived oxygen. The products reached about 45% of isotopic equilibrium, similar to the extent of the mineral fluid reaction. The Fe-rich, replacement dolomite near the core edge has an elevated value of F = 0.02 +/- 0.002, 10 times the value of F approximate to 0.002 for unreacted dolomite, but less than the value for the calcite. The distribution of O-18 in the minerals indicates that the breakdown and replacement reactions were faster than O diffusion in dolomite. C1 [DeAngelis, Michael T.] Univ Arkansas, Dept Earth Sci, Little Rock, AR 72204 USA. [Labotka, Theodore C.] Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN 37996 USA. [Fayek, Mostafa] Univ Manitoba, Dept Geol Sci, Winnipeg, MB R3T 2N2, Canada. [Cole, David R.] Ohio State Univ, Sch Earth Sci, Columbus, OH 43210 USA. [Anovitz, Lawrence M.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP DeAngelis, MT (reprint author), Univ Arkansas, Dept Earth Sci, Little Rock, AR 72204 USA. EM mtdeangelis@ualr.edu RI Anovitz, Lawrence/P-3144-2016 OI Anovitz, Lawrence/0000-0002-2609-8750 FU National Science Foundation [EAR-0087553]; Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy; U.S. Department of Energy [DE-AC05-00OR22725]; Geosciences Program in the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy [DE-SC0006878]; A.P. Sloan [2013-6-1]; NSERC FX This study is a portion of M.T. DeAngelis's dissertation work at the University of Tennessee, Knoxville. Many thanks to Allan Patchen at the University of Tennessee for help with EPMA analyses, and to Sharon Hull, Brandi Shabaga, and Rong Liu at the University of Manitoba for help with SIMS analyses. We sincerely appreciate the comments from the reviewers of previous versions of the manuscript: John Bowman, Thomas Muller, and Virginia Peterson. Funding for this work was provided by the National Science Foundation grant EAR-0087553 and the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy. Oak Ridge National Laboratory is managed and operated by UT-Battelle for the U.S. Department of Energy under contract DE-AC05-00OR22725. D.R.C. was also supported by research sponsored by the Geosciences Program in the Division of Chemical Sciences, Geosciences, and Biosciences, Office of Basic Energy Sciences, U.S. Department of Energy through grant DE-SC0006878 and by the A.P. Sloan-funded Deep Carbon Observatory under grant 2013-6-1. Partial funding for this work was also provided by a NSERC Discovery Grant to Fayek. Certain commercial equipment, instruments, materials, and software are identified in this paper to foster understanding. Such identification does not imply recommendation or endorsement by the Department of Energy or Oak Ridge National Laboratory, nor does it imply that that materials or equipment identified are necessarily the best available for the purpose. NR 25 TC 0 Z9 0 U1 6 U2 6 PU MINERALOGICAL SOC AMER PI CHANTILLY PA 3635 CONCORDE PKWY STE 500, CHANTILLY, VA 20151-1125 USA SN 0003-004X EI 1945-3027 J9 AM MINERAL JI Am. Miner. PD JUL-AUG PY 2016 VL 101 IS 7-8 BP 1898 EP 1905 DI 10.2138/am-2016-5635 PG 8 WC Geochemistry & Geophysics; Mineralogy SC Geochemistry & Geophysics; Mineralogy GA DT4KW UT WOS:000381450500041 ER PT J AU Stone, KH Schelhas, LT Garten, LM Shyam, B Mehta, A Ndione, PF Ginley, DS Toney, MF AF Stone, Kevin H. Schelhas, Laura T. Garten, Lauren M. Shyam, Badri Mehta, Apurva Ndione, Paul F. Ginley, David S. Toney, Michael F. TI Influence of amorphous structure on polymorphism in vanadia SO APL MATERIALS LA English DT Article ID CRYSTAL-STRUCTURE; PHASE; GLASS; DIOXIDE AB Normally we think of the glassy state as a single phase and therefore crystallization from chemically identical amorphous precursors should be identical. Here we show that the local structure of an amorphous precursor is distinct depending on the initial deposition conditions, resulting in significant differences in the final state material. Using grazing incidence total x-ray scattering, we have determined the local structure in amorphous thin films of vanadium oxide grown under different conditions using pulsed laser deposition (PLD). Here we show that the subsequent crystallization of films deposited using different initial PLD conditions result in the formation of different polymorphs of VO2. This suggests the possibility of controlling the formation of metastable polymorphs by tuning the initial amorphous structure to different formation pathways. (C) 2016 Author(s). C1 [Stone, Kevin H.; Schelhas, Laura T.; Shyam, Badri; Mehta, Apurva; Toney, Michael F.] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Garten, Lauren M.; Ndione, Paul F.; Ginley, David S.] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Shyam, Badri] Washington Coll, Dept Chem, Chestertown, MD 21620 USA. RP Stone, KH (reprint author), SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. EM khstone@slac.stanford.edu FU Center for Next Generation Materials by Design (CMGMD), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-AC36-08GO28308]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-76SF00515] FX The authors would like to thank Ronald Marks for assistance with SSRL beamline 10-2 where the GIPDF measurements were performed and Tim Dunn for assistance with SSRL beamline 11-3 where the in situ x-ray diffraction during crystallization was measured. We would also like to thank Matthew Latimer and Erik Nelson for assistance with SSRL beamlines 4-1 and 4-3 where the XAS data were collected. This work was supported as part of the Center for Next Generation Materials by Design (CMGMD), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences under Contract No. DE-AC36-08GO28308. Use of the Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, was supported by the U.S. Department of Energy, Office of Basic Energy Sciences under Contract No. DE-AC02-76SF00515. NR 24 TC 0 Z9 0 U1 19 U2 19 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 2166-532X J9 APL MATER JI APL Mater. PD JUL PY 2016 VL 4 IS 7 AR 076103 DI 10.1063/1.4958674 PG 6 WC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied SC Science & Technology - Other Topics; Materials Science; Physics GA DU7OL UT WOS:000382404300006 ER PT J AU Melchior, P Sheldon, E Drlica-Wagner, A Rykoff, ES Abbott, TMC Abdalla, FB Allam, S Benoit-Levy, A Brooks, D Buckley-Geer, E Rosell, AC Kind, MC Carretero, J Crocce, M D'Andrea, CB da Costa, LN Desai, S Doel, P Evrard, AE Finley, DA Flaugher, B Frieman, J Gaztanaga, E Gerdes, DW Gruen, D Gruendl, RA Honscheid, K James, DJ Jarvis, M Kuehn, K Li, TS Maia, MAG March, M Marshall, JL Nord, B Ogando, R Plazas, AA Romer, AK Sanchez, E Scarpine, V Sevilla-Noarbe, I Smith, RC Soares-Santos, M Suchyta, E Swanson, MEC Tarle, G Vikram, V Walker, AR Wester, W Zhang, Y AF Melchior, P. Sheldon, E. Drlica-Wagner, A. Rykoff, E. S. Abbott, T. M. C. Abdalla, F. B. Allam, S. Benoit-Levy, A. Brooks, D. Buckley-Geer, E. Carnero Rosell, A. Kind, M. Carrasco Carretero, J. Crocce, M. D'Andrea, C. B. da Costa, L. N. Desai, S. Doel, P. Evrard, A. E. Finley, D. A. Flaugher, B. Frieman, J. Gaztanaga, E. Gerdes, D. W. Gruen, D. Gruendl, R. A. Honscheid, K. James, D. J. Jarvis, M. Kuehn, K. Li, T. S. Maia, M. A. G. March, M. Marshall, J. L. Nord, B. Ogando, R. Plazas, A. A. Romer, A. K. Sanchez, E. Scarpine, V. Sevilla-Noarbe, I. Smith, R. C. Soares-Santos, M. Suchyta, E. Swanson, M. E. C. Tarle, G. Vikram, V. Walker, A. R. Wester, W. Zhang, Y. TI Crowdsourcing quality control for Dark Energy Survey images SO ASTRONOMY AND COMPUTING LA English DT Article DE Surveys Information systems: Crowdsourcing; Human-centered computing: Collaborative filtering ID SCIENCE AB We have developed a crowdsourcing web application for image quality control employed by the Dark Energy Survey. Dubbed the "DES exposure checker", it renders science-grade images directly to a web browser and allows users to mark problematic features from a set of predefined classes. Users can also generate custom labels and thus help identify previously unknown problem classes. User reports are fed back to hardware and software experts to help mitigate and eliminate recognized issues. We report on the implementation of the application and our experience with its over 100 users, the majority of which are professional or prospective astronomers but not data management experts. We discuss aspects of user training and engagement, and demonstrate how problem reports have been pivotal to rapidly correct artifacts which would likely have been too subtle or infrequent to be recognized otherwise. We conclude with a number of important lessons learned, suggest possible improvements, and recommend this collective exploratory approach for future astronomical surveys or other extensive data sets with a sufficiently large user base. We also release open-source code of the web application and host an online demo version at http://des-exp-checker.pmelchionnet. (C) 2016 Elsevier B.V. All rights reserved. C1 [Melchior, P.; Honscheid, K.] Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. [Melchior, P.; Honscheid, K.] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA. [Sheldon, E.] Brookhaven Natl Lab, Bldg 510, Upton, NY 11973 USA. [Drlica-Wagner, A.; Allam, S.; Buckley-Geer, E.; Finley, D. A.; Flaugher, B.; Frieman, J.; Nord, B.; Scarpine, V.; Soares-Santos, M.; Wester, W.] Fermilab Natl Accelerator Lab, POB 500, Batavia, IL 60510 USA. [Rykoff, E. S.] Stanford Univ, Kavli Inst Particle Astrophys & Cosmol, POB 2450, Stanford, CA 94305 USA. [Rykoff, E. S.] SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. [Abbott, T. M. C.; James, D. J.; Smith, R. C.; Walker, A. R.] Natl Opt Astron Observ, Cerro Tololo Interamer Observ, Casilla 603, La Serena, Chile. [Abdalla, F. B.; Benoit-Levy, A.; Brooks, D.; Doel, P.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Abdalla, F. B.] Rhodes Univ, Dept Phys & Elect, POB 94, ZA-6140 Grahamstown, South Africa. [Benoit-Levy, A.] Inst Astrophys Paris, CNRS, UMR 7095, F-75014 Paris, France. [Benoit-Levy, A.] Univ Paris 06, Sorbonne Univ, Inst Astrophys Paris, UMR 7095, F-75014 Paris, France. [Carnero Rosell, A.; da Costa, L. N.; Maia, M. A. G.; Ogando, R.] Lab Interinst E Astron LIneA, Rua Gal Jose Cristino 77, BR-20921400 Rio De Janeiro, RJ, Brazil. [Carnero Rosell, A.; da Costa, L. N.; Maia, M. A. G.; Ogando, R.] Observ Nacl, Rua Gal Jose Cristino 77, BR-20921400 Rio De Janeiro, RJ, Brazil. [Kind, M. Carrasco; Gruendl, R. A.; Sevilla-Noarbe, I.] Univ Illinois, Dept Astron, 1002 W Green St, Urbana, IL 61801 USA. [Kind, M. Carrasco; Gruendl, R. A.; Swanson, M. E. C.] Natl Ctr Supercomp Applicat, 1205 West Clark St, Urbana, IL 61801 USA. [Carretero, J.; Crocce, M.; Gaztanaga, E.] IEEC CSIC, Inst Ciencies Espai, Campus UAB,Carrer Can Magrans S-N, Barcelona 08193, Spain. [Carretero, J.] Barcelona Inst Sci & Technol, IFAE, Campus UAB, Bellaterra 08193, Barcelona, Spain. [D'Andrea, C. B.] Univ Portsmouth, Inst Cosmol & Gravitat, Portsmouth PO1 3FX, Hants, England. [D'Andrea, C. B.] Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England. [Desai, S.] Excellence Cluster Universe, Boltzmannstr 2, D-85748 Garching, Germany. [Desai, S.] Univ Munich, Fac Phys, Scheinerstr 1, D-81679 Munich, Germany. [Evrard, A. E.] Univ Michigan, Dept Astron, Ann Arbor, MI 48109 USA. [Evrard, A. E.; Gerdes, D. W.; Tarle, G.; Zhang, Y.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Frieman, J.] Univ Chicago, Kavli Inst Cosmol Phys, Chicago, IL 60637 USA. [Gruen, D.] Max Planck Inst Extraterr Phys, Giessenbachstr, D-85748 Garching, Germany. [Gruen, D.] Univ Munich, Fak Phys, Univ Sternwarte, Scheinerstr 1, D-81679 Munich, Germany. [Jarvis, M.; March, M.; Suchyta, E.] Univ Pennsylvania, Dept Phys & Astron, Philadelphia, PA 19104 USA. [Kuehn, K.] Australian Astron Observ, N Ryde, NSW 2113, Australia. [Li, T. S.; Marshall, J. L.] Texas A&M Univ, George P & Cynthia Woods Mitchell Inst Fundamenta, College Stn, TX 77843 USA. [Li, T. S.; Marshall, J. L.] Texas A&M Univ, Dept Phys & Astron, College Stn, TX 77843 USA. [Plazas, A. A.] CALTECH, Jet Prop Lab, 4800 Oak Grove Dr, Pasadena, CA 91109 USA. [Romer, A. K.] Univ Sussex, Dept Phys & Astron, Pevensey Bldg, Brighton BN1 9QH, E Sussex, England. [Sanchez, E.; Sevilla-Noarbe, I.] Ctr Invest Energet Medioambient & Tecnol CIEMAT, Madrid, Spain. [Vikram, V.] Argonne Natl Lab, 9700 South Cass Ave, Lemont, IL 60439 USA. RP Melchior, P (reprint author), Ohio State Univ, Ctr Cosmol & Astroparticle Phys, Columbus, OH 43210 USA. EM peter@pmelchior.net RI Ogando, Ricardo/A-1747-2010; Gaztanaga, Enrique/L-4894-2014; OI Ogando, Ricardo/0000-0003-2120-1154; Gaztanaga, Enrique/0000-0001-9632-0815; Abdalla, Filipe/0000-0003-2063-4345 FU U.S. Department of Energy; U.S. National Science Foundation; Ministry of Science and Education of Spain; Science and Technology Facilities Council of the United Kingdom; Higher Education Funding Council for England; National Center for Supercomputing Applications at the University of Illinois at Urbana/Champaign; Kavli Institute of Cosmological Physics at the University of Chicago; Center for Cosmology and Astro/Particle Physics at the Ohio State University; Mitchell Institute for Fundamental Physics and Astronomy at Texas AM University; Financiadora de Estudos e Projetos; Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro; Conselho Nacional de Desenvolvimento Cientifico e Tecnologico; Ministerio da Ciencia, Tecnologia e Inovacao; Deutsche Forschungsgemeinschaft; Argonne National Laboratory; University of California at Santa Cruz; University of Cambridge; Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas Madrid; University of Chicago; University College London; DES/Brazil Consortium; University of Edinburgh; Eidgenossische Technische Hochschule (ETH) Zurich; Fermi National Accelerator Laboratory; University of Illinois at Urbana/Champaign; Institut de Ciencies de l'Espai (IEEC/CSIC); Institut de Fisica d'Altes Energies; Lawrence Berkeley National Laboratory; Ludwig-Maximilians Universitat Munchen; associated Excellence Cluster Universe; University of Michigan; National Optical Astronomy Observatory; University of Nottingham; Ohio State University; University of Pennsylvania; University of Portsmouth; SLAC National Accelerator Laboratory; Stanford University; University of Sussex; Texas AM University; National Science Foundation [AST/1138766, PHYS/1066293]; MINECO [AYA2012/39559, ESP2013/48274, FPA2013/47986]; Centro de Excelencia Severo Ochoa [SEV/2012/0234]; European Research Council under the European Union's Seventh Framework Programme (FP7); ERC [240672, 291329, 306478]; U.S. Department of Energy [DE-FG02/91ER40690]; DOE [DE-AC02/98CH10886] FX Funding for the DES Projects has been provided by the U.S. Department of Energy, the U.S. National Science Foundation, the Ministry of Science and Education of Spain, the Science and Technology Facilities Council of the United Kingdom, the Higher Education Funding Council for England, the National Center for Supercomputing Applications at the University of Illinois at Urbana/Champaign, the Kavli Institute of Cosmological Physics at the University of Chicago, the Center for Cosmology and Astro/Particle Physics at the Ohio State University, the Mitchell Institute for Fundamental Physics and Astronomy at Texas A&M University, Financiadora de Estudos e Projetos, Fundacao Carlos Chagas Filho de Amparo a Pesquisa do Estado do Rio de Janeiro, Conselho Nacional de Desenvolvimento Cientifico e Tecnologico and the Ministerio da Ciencia, Tecnologia e Inovacao, the Deutsche Forschungsgemeinschaft and the Collaborating Institutions in the Dark Energy Survey.; The Collaborating Institutions are Argonne National Laboratory, the University of California at Santa Cruz, the University of Cambridge, Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas Madrid, the University of Chicago, University College London, the DES/Brazil Consortium, the University of Edinburgh, the Eidgenossische Technische Hochschule (ETH) Zurich, Fermi National Accelerator Laboratory, the University of Illinois at Urbana/Champaign, the Institut de Ciencies de l'Espai (IEEC/CSIC), the Institut de Fisica d'Altes Energies, Lawrence Berkeley National Laboratory, the Ludwig-Maximilians Universitat Munchen and the associated Excellence Cluster Universe, the University of Michigan, the National Optical Astronomy Observatory, the University of Nottingham, The Ohio State University, the University of Pennsylvania, the University of Portsmouth, SLAC National Accelerator Laboratory, Stanford University, the University of Sussex, and Texas A&M University.; The DES data management system is supported by the National Science Foundation under Grant Number AST/1138766. The DES participants from Spanish institutions are partially supported by MINECO under grants AYA2012/39559, ESP2013/48274, FPA2013/47986, and Centro de Excelencia Severo Ochoa SEV/2012/0234. Research leading to these results has received funding from the European Research Council under the European Union's Seventh Framework Programme (FP7/2007/2013) including ERC grant agreements 240672, 291329, and 306478.; PM is supported by the U.S. Department of Energy under Contract No. DE-FG02/91ER40690. ES is supported by DOE grant DE-AC02/98CH10886. This work was supported in part by the National Science Foundation under Grant No. PHYS/1066293 and the hospitality of the Aspen Center for Physics. NR 21 TC 1 Z9 1 U1 5 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2213-1337 EI 2213-1345 J9 ASTRON COMPUT JI Astron. Comput. PD JUL PY 2016 VL 16 BP 99 EP 108 DI 10.1016/j.ascom.2016.04.003 PG 10 WC Astronomy & Astrophysics; Computer Science, Interdisciplinary Applications SC Astronomy & Astrophysics; Computer Science GA DU7SE UT WOS:000382414100010 ER PT J AU Besla, G Martinez-Delgado, D van der Marel, RP Beletsky, Y Seibert, M Schlafly, EF Grebel, EK Neyer, F AF Besla, Gurtina Martinez-Delgado, David van der Marel, Roeland P. Beletsky, Yuri Seibert, Mark Schlafly, Edward F. Grebel, Eva K. Neyer, Fabian TI LOW SURFACE BRIGHTNESS IMAGING OF THE MAGELLANIC SYSTEM: IMPRINTS OF TIDAL INTERACTIONS BETWEEN THE CLOUDS IN THE STELLAR PERIPHERY SO ASTROPHYSICAL JOURNAL LA English DT Article DE galaxies: dwarf; galaxies: interactions; Galaxy: kinematics and dynamics; Magellanic Clouds ID NEAR-INFRARED SURVEYS; DARK ENERGY SURVEY; MILKY-WAY; STAR-FORMATION; SMALL COMPANIONS; CARINA DWARF; VMC SURVEY; GALAXY; STREAM; MASS AB We present deep optical images of the Large and Small Magellanic Clouds (LMC and SMC) using a low cost telephoto lens with a wide field of view to explore stellar substructure in the outskirts of the stellar disk of the LMC (< 10 degrees from the LMC center). These data have higher resolution than existing star count maps, and highlight the existence of stellar arcs and multiple spiral arms in the northern periphery, with no comparable counterparts in the south. We compare these data to detailed simulations of the LMC disk outskirts, following interactions with its low mass companion, the SMC. We consider interaction in isolation and with the inclusion of the Milky Way tidal field. The simulations are used to assess the origin of the northern structures, including also the low density stellar arc recently identified in the Dark Energy Survey data by Mackey et al. at similar to 15 degrees. We conclude that repeated close interactions with the SMC are primarily responsible for the asymmetric stellar structures seen in the periphery of the LMC. The orientation and density of these arcs can be used to constrain the LMC's interaction history with and impact parameter of the SMC. More generally, we find that such asymmetric structures should be ubiquitous about pairs of dwarfs and can persist for 1-2 Gyr even after the secondary merges entirely with the primary. As such, the lack of a companion around a Magellanic Irregular does not disprove the hypothesis that their asymmetric structures are driven by dwarf-dwarf interactions. C1 [Besla, Gurtina] Univ Arizona, Steward Observ, 933 North Cherry Ave, Tucson, AZ 85721 USA. [Martinez-Delgado, David; Grebel, Eva K.] Heidelberg Univ, Zentrum Astron, Astron Rech Inst, Monchhofstr 12-14, D-69120 Heidelberg, Germany. [van der Marel, Roeland P.] Space Telescope Sci Inst, 3700 San Martin Dr, Baltimore, MD 21218 USA. [Beletsky, Yuri] Carnegie Inst Sci, Las Campanas Observ, 601 Casilla, La Serena, Chile. [Seibert, Mark] Carnegie Observ, 813 Santa Barbara St, Pasadena, CA 91101 USA. [Schlafly, Edward F.] Lawrence Berkeley Natl Lab, One Cyclotron Rd, Berkeley, CA 94720 USA. [Neyer, Fabian] ETH, Inst Geodesy & Photogrammetry, CH-8093 Zurich, Switzerland. RP Besla, G (reprint author), Univ Arizona, Steward Observ, 933 North Cherry Ave, Tucson, AZ 85721 USA. EM gbesla@email.arizona.edu OI /0000-0002-1891-3794; Schlafly, Edward Ford/0000-0002-3569-7421 FU HST AR grant [12632]; NASA through Space Telescope Science Institute [12632]; NASA contract [NAS 5-26555]; Sonderforschungsbereich (SFB) "The Milky Way System" of the German Research Foundation (DFG) [881]; NASA through Hubble Fellowship - Space Telescope Science Institute [HST-HF2-51367.001-A]; NASA [NAS 5-26555]; FAS Science Division Research Computing Group at Harvard University; National Science Foundation [1228509] FX We thank Dougal Mackey and David Schminovich for useful conversation that have improved this manuscript. GB acknowledges support through HST AR grant # 12632. Support for program # 12632 was provided by NASA through a grant from the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Inc., under NASA contract NAS 5-26555. DMD and EKG acknowledge support by Sonderforschungsbereich (SFB) 881 "The Milky Way System" of the German Research Foundation (DFG), particularly through subproject A2. ES acknowledges support for this work provided by NASA through Hubble Fellowship grant HST-HF2-51367.001-A awarded by the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Inc., for NASA, under contract NAS 5-26555. This paper is based on observations made at the La Silla Paranal Observatory. The simulations in this paper were produced on the Odyssey cluster supported by the FAS Science Division Research Computing Group at Harvard University. Analysis was undertaken on the El Gato cluster at the University of Arizona, which is supported by the National Science Foundation under Grant No. 1228509. NR 76 TC 2 Z9 2 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2016 VL 825 IS 1 AR 20 DI 10.3847/0004-637X/825/1/20 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DU0YD UT WOS:000381930000020 ER PT J AU Dong, RB Dawson, R AF Dong, Ruobing Dawson, Rebekah TI STABILITY AND OCCURRENCE RATE CONSTRAINTS ON THE PLANETARY SCULPTING HYPOTHESIS FOR "TRANSITIONAL" DISKS SO ASTROPHYSICAL JOURNAL LA English DT Article DE circumstellar matter; planet-disk interactions; planets and satellites: formation; protoplanetary disks; stars: pre-main sequence; stars: variables: T Tauri, Herbig Ae/Be ID LOW-MASS PLANETS; POLARIZED SCATTERED-LIGHT; SURFACE-LAYER ACCRETION; 3D PROTOPLANETARY DISKS; MEAN-MOTION RESONANCES; MAIN-SEQUENCE STARS; EXOPLANET IN-ORBIT; INDUCED GAP EDGES; SYSTEM HR 8799; T TAURI DISKS AB Transitional disks, protoplanetary disks with deep and wide central gaps, may be the result of planetary sculpting. By comparing numerical planet-opening-gap models with observed gaps, we find systems of 3-6 giant planets are needed in order to open gaps with the observed depths and widths. We explore the dynamical stability of such multi-planet systems using N-body simulations that incorporate prescriptions for gas effects. We find they can be stable over a typical disk lifetime, with the help of eccentricity damping from the residual gap gas that facilitates planets locking into mean motion resonances. However, in order to account for the occurrence rate of transitional disks, the planet sculpting scenario demands gap-opening-friendly disk conditions, in particular, a disk viscosity alpha less than or similar to 0.001. In addition, the demography of giant planets at similar to 3-30 au separations, poorly constrained by current data, has to largely follow occurrence rates extrapolated outward from radial velocity surveys, not the lower occurrence rates extrapolated inward from direct imaging surveys. Even with the most optimistic occurrence rates, transitional disks cannot be a common phase that most gas disks experience at the end of their life, as popularly assumed, simply because there are not enough planets to open these gaps. Finally, as consequences of demanding almost all giant planets at large separations participate in transitional disk sculpting, the majority of such planets must form early and end up in a chain of mean motion resonances at the end of disk lifetime. C1 [Dong, Ruobing] Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA. [Dong, Ruobing; Dawson, Rebekah] Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. [Dawson, Rebekah] Penn State Univ, Dept Astron & Astrophys, State Coll, PA USA. [Dawson, Rebekah] Penn State Univ, Ctr Exoplanets & Habitable Worlds, State Coll, PA USA. RP Dong, RB (reprint author), Lawrence Berkeley Natl Lab, Div Nucl Sci, Berkeley, CA 94720 USA.; Dong, RB (reprint author), Univ Calif Berkeley, Dept Astron, 601 Campbell Hall, Berkeley, CA 94720 USA. EM rdong2013@berkeley.edu FU NASA - Space Telescope Science Institute [HST-HF-51320.01-A]; NASA [NAS 5-26555]; Miller Institute for Basic Research in Science FX We thank the referee, John E. Chambers, for a constructive report that improved the quality and the clarity of the paper. R.D. thanks Xue-Ning Bai for teaching him about MRI in disks, and Ewine van Dishoeck and Nienke van der Marel for educating him on the topic of ALMA disk observations. We also thank Sean Andrews, Tim Brandt, Sourav Chatterjee, Eugene Chiang, Paul Duffell, Misato Fukagawa, Andrea Isella, John Johnson, Heather Knutson, Chalie Lada, Renu Malhotra, Rebecca Martin, and Ben Montet for insightful discussions. We particularly thank Jeffery Fung and Paul Duffell for kindly sharing the simulation data in Fung et al. (2014) and Duffell & Dong (2015) with us. This project is partially supported by NASA through Hubble Fellowship grant HST-HF-51320.01-A (first R.D.) awarded by the Space Telescope Science Institute, which is operated by the Association of Universities for Research in Astronomy, Inc., for NASA, under contract NAS 5-26555, and by the Miller Institute for Basic Research in Science (second R.D.). Simulations were run on the SAVIO computational cluster provided by Berkeley Research Computing. NR 169 TC 3 Z9 3 U1 1 U2 1 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2016 VL 825 IS 1 AR 77 DI 10.3847/0004-637X/825/1/77 PG 25 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DU0YD UT WOS:000381930000077 ER PT J AU Okura, Y Petri, A May, M Plazas, AA Tamagawa, T AF Okura, Yuki Petri, Andrea May, Morgan Plazas, Andres A. Tamagawa, Toru TI CONSEQUENCES OF CCD IMPERFECTIONS FOR COSMOLOGY DETERMINED BY WEAK LENSING SURVEYS: FROM LABORATORY MEASUREMENTS TO COSMOLOGICAL PARAMETER BIAS SO ASTROPHYSICAL JOURNAL LA English DT Article DE cosmological parameters; cosmology: miscellaneous; cosmology: observations; instrumentation: detectors ID DARK-MATTER; CALIBRATION AB Weak gravitational lensing causes subtle changes in the apparent shapes of galaxies due to the bending of light by the gravity of foreground masses. By measuring the shapes of large numbers of galaxies (millions in recent surveys, up to tens of billions in future surveys) we can infer the parameters that determine cosmology. Imperfections in the detectors used to record images of the sky can introduce changes in the apparent shapes of galaxies, which in turn can bias the inferred cosmological parameters. In this paper we consider the effect of two widely discussed sensor imperfections: tree rings, due to impurity gradients that cause transverse electric fields in the charge-coupled devices (CCDs), and pixel size variation, due to periodic CCD fabrication errors. These imperfections can be observed when the detectors are subject to uniform illumination (flat-field images). We develop methods to determine the spurious shear and convergence (due to the imperfections) from the flat-field images. We calculate how the spurious shear when added to the lensing shear will bias the determination of cosmological parameters. We apply our methods to candidate sensors of the Large Synoptic Survey Telescope (LSST) as a timely and important example, analyzing flat-field images recorded with LSST prototype CCDs in the laboratory. We find that tree rings and periodic pixel size variation present in the LSST CCDs will introduce negligible bias to cosmological parameters determined from the lensing power spectrum, specifically w, Omega(m), and sigma(8). C1 [Okura, Yuki; Tamagawa, Toru] RIKEN Nishina Ctr, Wako, Saitama, Japan. [Okura, Yuki] RIKEN BNL Res Ctr, Upton, NY 11973 USA. [Petri, Andrea] Columbia Univ, New York, NY 10027 USA. [Petri, Andrea; May, Morgan; Plazas, Andres A.] Brookhaven Natl Lab, Upton, NY 11973 USA. [Plazas, Andres A.] CALTECH, Jet Prop Lab, Pasadena, CA 91125 USA. RP Okura, Y (reprint author), RIKEN Nishina Ctr, Wako, Saitama, Japan.; Okura, Y (reprint author), RIKEN BNL Res Ctr, Upton, NY 11973 USA. EM yuki.okura@riken.jp FU US Department of Energy [DEAC02-98CH10886, DE-SC0012704]; Jet Propulsion Laboratory FX We thank G. Bernstein and P. O'Connor for useful comments and discussions, and the Instrumentation Division of Brookhaven for data taking. This work was supported in part by the US Department of Energy under Contract No. DEAC02-98CH10886 and Contract No. DE-SC0012704. A.A.P. is also supported by the Jet Propulsion Laboratory, which is run under a contract for NASA by Caltech. NR 21 TC 0 Z9 0 U1 0 U2 0 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 0004-637X EI 1538-4357 J9 ASTROPHYS J JI Astrophys. J. PD JUL 1 PY 2016 VL 825 IS 1 AR 61 DI 10.3847/0004-637X/825/1/61 PG 10 WC Astronomy & Astrophysics SC Astronomy & Astrophysics GA DU0YD UT WOS:000381930000061 ER PT J AU Mutchek, M Cooney, G Pickenpaugh, G Marriott, J Skone, T AF Mutchek, Michele Cooney, Gregory Pickenpaugh, Gavin Marriott, Joe Skone, Timothy TI Understanding the Contribution of Mining and Transportation to the Total Life Cycle Impacts of Coal Exported from the United States SO ENERGIES LA English DT Article DE coal exports; life cycle analysis; climate change; Powder River Basin; greenhouse gas emissions; power generation; electricity; impact assessment; Asian markets AB The construction of two marine bulk terminals in the Pacific Northwest region of the United States are currently under review and would open up additional thermal coal exports to Asia on the order of almost 100 million additional tonnes per year. The major exporters of coal to Asian markets include Indonesia and Australia. This life cycle analysis (LCA) seeks to understand the role of transportation and mining in the cradle-to-busbar environmental impacts of coal exports from the Powder River Basin (PRB) to Asian countries, when compared to the competitor countries. This LCA shows that: (1) the most significant greenhouse gas (GHG) impacts in the cradle-to-busbar life cycle of coal for power generation come from the combustion of coal in a power plant, even when 90% carbon capture is applied; (2) for non-GHG air impacts, power plant combustion impacts are less dominant and variations in upstream impacts (mining and transportation) are more important; and (3) when comparing impacts between countries, upstream impacts vary for both GHG and non-GHG results, but conclusions that rank countries cannot be made. Future research should include expansion to include non-air impacts, potential consequential effects of coal exports, and a better understanding around the characterization of non-GHG ocean transport impacts. C1 [Mutchek, Michele; Cooney, Gregory; Pickenpaugh, Gavin; Marriott, Joe; Skone, Timothy] Natl Energy Technol Lab, 626 Cochrans Mill Rd,POB 10940, Pittsburgh, PA 15236 USA. RP Skone, T (reprint author), Natl Energy Technol Lab, 626 Cochrans Mill Rd,POB 10940, Pittsburgh, PA 15236 USA. EM Michele.Mutchek@netl.doe.gov; Gregory.Cooney@netl.doe.gov; Gavin.Pickenpaugh@netl.doe.gov; Joseph.Marriott@netl.doe.gov; Timothy.Skone@netl.doe.gov NR 60 TC 0 Z9 0 U1 8 U2 8 PU MDPI AG PI BASEL PA ST ALBAN-ANLAGE 66, CH-4052 BASEL, SWITZERLAND SN 1996-1073 J9 ENERGIES JI Energies PD JUL PY 2016 VL 9 IS 7 AR 559 DI 10.3390/en9070559 PG 20 WC Energy & Fuels SC Energy & Fuels GA DT5CC UT WOS:000381497300081 ER PT J AU Hobbs, BF Xu, QY Ho, J Donohoo, P Kasina, S Ouyang, J Park, SW Eto, J Satyal, V AF Hobbs, Benjamin F. Xu, Qingyu Ho, Jonathan Donohoo, Pearl Kasina, Saamrat Ouyang, Jasmine Park, Sang Woo Eto, Joseph Satyal, Vijay TI Adaptive Transmission Planning Implementing a New Paradigm for Managing Economic Risks in Grid Expansion SO IEEE POWER & ENERGY MAGAZINE LA English DT Article C1 [Hobbs, Benjamin F.; Xu, Qingyu; Kasina, Saamrat; Park, Sang Woo] Johns Hopkins Univ, Baltimore, MD 21211 USA. [Ho, Jonathan] Natl Renewable Energy Lab, Golden, CO USA. [Donohoo, Pearl] Brattle Grp, Washington, DC USA. [Ouyang, Jasmine] Ethree, San Francisco, CA USA. [Eto, Joseph] Lawrence Berkeley Natl Lab, Berkeley, CA USA. [Satyal, Vijay] Western Elect Coordinating Council, Salt Lake City, UT USA. RP Hobbs, BF (reprint author), Johns Hopkins Univ, Baltimore, MD 21211 USA. FU Western Electricity Coordinating Council; U.S. Department of Energy, Office of Electricity Delivery and Energy Reliability; Consortium for Electricity Reliability Technology Solutions of the U.S. Department of Energy FX This material is based upon work supported by the Western Electricity Coordinating Council and by the U.S. Department of Energy, Office of Electricity Delivery and Energy Reliability, through a contract managed by the Lawrence Berkeley National Laboratory. Partial support was also provided by the Consortium for Electricity Reliability Technology Solutions of the U.S. Department of Energy. The project team would like to thank WE CC staff and the members of the Technical Advisory Committee for their advice and input. Reference herein to any specific commercial product, process, or service by trade name, trademark, manufacturer, or otherwise does not necessarily constitute or imply its endorsement, recommendation, or favoring by the United States government or any agency thereof. Our views and opinions expressed herein do not necessarily state or reflect those of the United States government or any agency thereof. NR 6 TC 0 Z9 0 U1 1 U2 1 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1540-7977 EI 1558-4216 J9 IEEE POWER ENERGY M JI IEEE Power Energy Mag. PD JUL-AUG PY 2016 VL 14 IS 4 BP 30 EP 40 DI 10.1109/MPE.2016.2547280 PG 11 WC Engineering, Electrical & Electronic SC Engineering GA DV1MG UT WOS:000382684600003 ER PT J AU Gu, LH Pallardy, SG Yang, B Hosman, KP Mao, JF Ricciuto, D Shi, XY Sun, Y AF Gu, Lianhong Pallardy, Stephen G. Yang, Bai Hosman, Kevin P. Mao, Jiafu Ricciuto, Daniel Shi, Xiaoying Sun, Ying TI Testing a land model in ecosystem functional space via a comparison of observed and modeled ecosystem flux responses to precipitation regimes and associated stresses in a Central US forest SO JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES LA English DT Article DE ecosystem functional space; carbon and water budgets; climate variability indices; land surface modeling; eddy covariance; drought ID CENTRAL UNITED-STATES; WATER-USE EFFICIENCY; EDDY COVARIANCE; CENTRAL MISSOURI; CARBON-DIOXIDE; TEMPERATE FOREST; DECIDUOUS FOREST; OZARK FOREST; DROUGHT; PHOTOSYNTHESIS AB Testing complex land surface models has often proceeded by asking the question: does the model prediction agree with the observation? Such an approach has yet led to high-performance terrestrial models that meet the challenges of climate and ecological studies. Here we test the Community Land Model (CLM) by asking the question: does the model behave like an ecosystem? We pursue its answer by testing CLM in the ecosystem functional space (EFS) at the Missouri Ozark AmeriFlux (MOFLUX) forest site in the Central U.S., focusing on carbon and water flux responses to precipitation regimes and associated stresses. In the observed EFS, precipitation regimes and associated water and heat stresses controlled seasonal and interannual variations of net ecosystem exchange (NEE) of CO2 and evapotranspiration in this deciduous forest ecosystem. Such controls were exerted more strongly by precipitation variability than by the total precipitation amount per se. A few simply constructed climate variability indices captured these controls, suggesting a high degree of potential predictability. While the interannual fluctuation in NEE was large, a net carbon sink was maintained even during an extreme drought year. Although CLM predicted seasonal and interanual variations in evapotranspiration reasonably well, its predictions of net carbon uptake were too small across the observed range of climate variability. Also, the model systematically underestimated the sensitivities of NEE and evapotranspiration to climate variability and overestimated the coupling strength between carbon and water fluxes. We suspect that the modeled and observed trajectories of ecosystem fluxes did not overlap in the EFS and the model did not behave like the ecosystem it attempted to simulate. A definitive conclusion will require comprehensive parameter and structural sensitivity tests in a rigorous mathematical framework. We suggest that future model improvements should focus on better representation and parameterization of process responses to environmental stresses and on more complete and robust representations of carbon-specific processes so that adequate responses to climate variability and a proper degree of coupling between carbon and water exchanges are captured. C1 [Gu, Lianhong; Yang, Bai; Mao, Jiafu; Ricciuto, Daniel; Shi, Xiaoying] Oak Ridge Natl Lab, Environm Sci Div, Oak Ridge, TN 37831 USA. [Gu, Lianhong; Yang, Bai; Mao, Jiafu; Ricciuto, Daniel; Shi, Xiaoying] Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. [Pallardy, Stephen G.; Hosman, Kevin P.] Univ Missouri, Dept Forestry, Columbia, MO USA. [Sun, Ying] Univ Texas Austin, Jackson Sch Geosci, Austin, TX 78712 USA. RP Gu, LH (reprint author), Oak Ridge Natl Lab, Environm Sci Div, Oak Ridge, TN 37831 USA.; Gu, LH (reprint author), Oak Ridge Natl Lab, Climate Change Sci Inst, Oak Ridge, TN 37831 USA. EM lianhong-gu@ornl.gov RI xiao, qiang/S-7367-2016; Gu, Lianhong/H-8241-2014; Mao, Jiafu/B-9689-2012; Ricciuto, Daniel/I-3659-2016 OI Gu, Lianhong/0000-0001-5756-8738; Mao, Jiafu/0000-0002-2050-7373; Ricciuto, Daniel/0000-0002-3668-3021 FU U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research Program, Climate and Environmental Sciences Division; U.S. Department of Energy [DE-AC05-00OR22725]; University of Missouri [DE-FG02-03ER63683] FX This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research Program, Climate and Environmental Sciences Division. ORNL is managed by UT-Battelle, LLC, for the U.S. Department of Energy under contract DE-AC05-00OR22725. U.S. Department of Energy support for the University of Missouri (grant DE-FG02-03ER63683) is gratefully acknowledged. The data used in this study are available from the AmeriFlux network (http://ameriflux.lbl.gov) and from 10.3334/CDIAC/ornIsfa.004. NR 76 TC 0 Z9 0 U1 6 U2 6 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-8953 EI 2169-8961 J9 J GEOPHYS RES-BIOGEO JI J. Geophys. Res.-Biogeosci. PD JUL PY 2016 VL 121 IS 7 BP 1884 EP 1902 DI 10.1002/2015JG003302 PG 19 WC Environmental Sciences; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA DV0BG UT WOS:000382581900012 ER PT J AU Williams, IN Riley, WJ Kueppers, LM Biraud, SC Torn, MS AF Williams, Ian N. Riley, William J. Kueppers, Lara M. Biraud, Sebastien C. Torn, Margaret S. TI Separating the effects of phenology and diffuse radiation on gross primary productivity in winter wheat SO JOURNAL OF GEOPHYSICAL RESEARCH-BIOGEOSCIENCES LA English DT Article DE diffuse radiation; GPP; canopy scaling; phenology; terrestrial carbon cycle; clouds aerosols ID NET ECOSYSTEM EXCHANGE; LIGHT-USE EFFICIENCY; DAILY CANOPY PHOTOSYNTHESIS; LEAF NITROGEN; DECIDUOUS FOREST; STOMATAL CONDUCTANCE; SEASONAL PATTERN; CARBON-DIOXIDE; CLEAR SKIES; TERRESTRIAL AB Gross primary productivity (GPP) has been reported to increase with the fraction of diffuse solar radiation, for a given total irradiance. The correlation between GPP and diffuse radiation suggests effects of diffuse radiation on canopy light-use efficiency, but potentially confounding effects of vegetation phenology have not been fully explored. We applied several approaches to control for phenology, using 8years of eddy-covariance measurements of winter wheat in the U.S. Southern Great Plains. The apparent enhancement of daily GPP due to diffuse radiation was reduced from 260% to 75%, after subsampling over the peak growing season or by subtracting a 15day moving average of GPP, suggesting a role of phenology. The diffuse radiation effect was further reduced to 22% after normalizing GPP by a spectral reflectance index to account for phenological variations in leaf area index LAI and canopy photosynthetic capacity. Canopy photosynthetic capacity covaries with diffuse fraction at a given solar irradiance at this site because both factors are dependent onday of year or solar zenith angle. Using a two-leaf Sun-shaded canopy radiative transfer model, we confirmed that the effects of phenological variations in photosynthetic capacity can appear qualitatively similar to the effects of diffuse radiation on GPP and therefore can be difficult to distinguish using observations. The importance of controlling for phenology when inferring diffuse radiation effects on GPP raises new challenges and opportunities for using radiation measurements to improve carbon cycle models. C1 [Williams, Ian N.; Riley, William J.; Kueppers, Lara M.; Biraud, Sebastien C.; Torn, Margaret S.] Lawrence Berkeley Natl Lab, Climate & Ecosyst Sci Div, Berkeley, CA 94720 USA. RP Williams, IN (reprint author), Lawrence Berkeley Natl Lab, Climate & Ecosyst Sci Div, Berkeley, CA 94720 USA. EM inwilliams@lbl.gov RI Biraud, Sebastien/M-5267-2013; Kueppers, Lara/M-8323-2013; Riley, William/D-3345-2015; Torn, Margaret/D-2305-2015; OI Biraud, Sebastien/0000-0001-7697-933X; Kueppers, Lara/0000-0002-8134-3579; Riley, William/0000-0002-4615-2304; Williams, Ian/0000-0003-0355-1310 FU U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Atmospheric System Research, and Atmospheric Radiation Management Programs [DE-AC02-05CH11231] FX Data were obtained from arm.gov (www.archive.arm.gov) from the following data streams: sgp30co2flx4mmetC1.b1 (http://dx.doi.org/10.5439/1025037), beflux1long (http://dx.doi.org/10.5439/1027285), and sgpmfrsrC1.b1 (http://dx.doLorg/10.5439/1023898). This material is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, Atmospheric System Research, and Atmospheric Radiation Management Programs, under contract DE-AC02-05CH11231. NR 51 TC 0 Z9 0 U1 15 U2 20 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-8953 EI 2169-8961 J9 J GEOPHYS RES-BIOGEO JI J. Geophys. Res.-Biogeosci. PD JUL PY 2016 VL 121 IS 7 BP 1903 EP 1915 DI 10.1002/2015JG003317 PG 13 WC Environmental Sciences; Geosciences, Multidisciplinary SC Environmental Sciences & Ecology; Geology GA DV0BG UT WOS:000382581900013 ER PT J AU MacGregor, JA Fahnestock, MA Catania, GA Aschwanden, A Clow, GD Colgan, WT Gogineni, SP Morlighem, M Nowicki, SMJ Paden, JD Price, SF Seroussi, H AF MacGregor, Joseph A. Fahnestock, Mark A. Catania, Ginny A. Aschwanden, Andy Clow, Gary D. Colgan, William T. Gogineni, S. Prasad Morlighem, Mathieu Nowicki, Sophie M. J. Paden, John D. Price, Stephen F. Seroussi, Helene TI A synthesis of the basal thermal state of the Greenland Ice Sheet SO JOURNAL OF GEOPHYSICAL RESEARCH-EARTH SURFACE LA English DT Article DE Greenland Ice Sheet; ice sheet thermodynamics; remote sensing; radar sounding; Northeast Greenland Ice Stream ID GEOTHERMAL HEAT-FLUX; BORE-HOLE SURVEY; SEA-LEVEL RISE; NORTHEAST GREENLAND; WEST ANTARCTICA; FAST-FLOW; JAKOBSHAVNS-ISBRAE; CLIMATE SCENARIOS; THWAITES GLACIER; SUBGLACIAL LAKES AB The basal thermal state of an ice sheet (frozen or thawed) is an important control upon its evolution, dynamics, and response to external forcings. However, this state can only be observed directly at sparse boreholes or inferred conclusively from the presence of subglacial lakes. Here we synthesize spatially extensive inferences of the basal thermal state of the Greenland Ice Sheet to better constrain this state. Existing inferences include outputs from the eight thermomechanical ice-flow models included in the Sea Level Response to Ice Sheet Evolution (SeaRISE) effort. New remote-sensing inferences of the basal thermal state are derived from Holocene radiostratigraphy, modern surface velocity, and Moderate Resolution Imaging Spectroradiometer (MODIS) imagery. Both thermomechanical modeling and remote inferences generally agree that the Northeast Greenland Ice Stream and large portions of the southwestern ice-drainage systems are thawed at the bed, whereas the bed beneath the central ice divides, particularly their west facing slopes, is frozen. Elsewhere, there is poorer agreement regarding the basal thermal state. Both models and remote inferences rarely represent the borehole-observed basal thermal state accurately near NorthGRIP and DYE-3. This synthesis identifies a large portion of the Greenland Ice Sheet (about one third by area), where additional observations would most improve knowledge of its overall basal thermal state. C1 [MacGregor, Joseph A.; Catania, Ginny A.] Univ Texas Austin, Inst Geophys, 8701 Mopac Blvd, Austin, TX 78712 USA. [MacGregor, Joseph A.; Nowicki, Sophie M. J.] NASA, Goddard Space Flight Ctr, Cryospher Sci Lab, Code 615, Greenbelt, MD 20771 USA. [Fahnestock, Mark A.; Aschwanden, Andy] Univ Alaska Fairbanks, Inst Geophys, Fairbanks, AK 99775 USA. [Catania, Ginny A.] Univ Texas Austin, Dept Geol Sci, Austin, TX USA. [Clow, Gary D.] US Geol Survey, Box 25046, Denver, CO 80225 USA. [Clow, Gary D.] Univ Colorado, Inst Arctic & Alpine Res, Boulder, CO 80309 USA. [Colgan, William T.] York Univ, Dept Earth & Space Sci & Engn, Toronto, ON, Canada. [Gogineni, S. Prasad; Paden, John D.] Univ Kansas, Ctr Remote Sensing Ice Sheets, Lawrence, KS 66045 USA. [Morlighem, Mathieu] Univ Calif Irvine, Dept Earth Syst Sci, Irvine, CA USA. [Price, Stephen F.] Los Alamos Natl Lab, Fluid Dynam Grp, Los Alamos, NM USA. [Seroussi, Helene] CALTECH, Jet Prop Lab, Pasadena, CA USA. RP MacGregor, JA (reprint author), Univ Texas Austin, Inst Geophys, 8701 Mopac Blvd, Austin, TX 78712 USA.; MacGregor, JA (reprint author), NASA, Goddard Space Flight Ctr, Cryospher Sci Lab, Code 615, Greenbelt, MD 20771 USA. EM joseph.a.macgregor@nasa.gov RI Colgan, William/H-1570-2014; Catania, Ginny/B-9787-2008 OI Colgan, William/0000-0001-6334-1660; FU NSF [ARC 1107753, 1108058, ANT 0424589]; NASA [NNX12AB71G, NNX13AM16G, NNX13AK27G, NNX13AD53A]; U.S. Geological Survey Climate and Land Use Change Program; U.S. Department of Energy Office of Science's Biological and Environmental Research Program; NASA Cryospheric Sciences and Modeling Analysis and Prediction Programs, under Caltech's Jet Propulsion Laboratory FX NSF (ARC 1107753 and 1108058 and ANT 0424589) and NASA (NNX12AB71G, NNX13AM16G, NNX13AK27G, and NNX13AD53A) supported this work. We thank the organizations (Program for Arctic Regional Climate Assessment, Center for Remote Sensing of Ice Sheets, Operation IceBridge, and SeaRISE) and innumerable individuals that both supported and performed the development, collection, and processing of the radar data and numerical models used in this study. G.D. Clow was supported by the U.S. Geological Survey Climate and Land Use Change Program. S.F. Price was supported by the U.S. Department of Energy Office of Science's Biological and Environmental Research Program. H. Seroussi was supported by NASA Cryospheric Sciences and Modeling Analysis and Prediction Programs, under a contract with Caltech's Jet Propulsion Laboratory. We thank A.N. Mabrey for analyzing the MOG surface texture, I. Joughin for providing the updated composite surface-velocity field, H. Thomsen for the borehole-temperature data, and L.C. Andrews for the valuable discussions. We thank the Editor, Associate Editor, M. Luthi, and two anonymous reviews for their constructive reviews that substantially improved this manuscript. A mask of the likely basal thermal state of the GrIS (Figure 11) will be archived at the National Snow and Ice Data Center. NR 100 TC 4 Z9 4 U1 8 U2 8 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9003 EI 2169-9011 J9 J GEOPHYS RES-EARTH JI J. Geophys. Res.-Earth Surf. PD JUL PY 2016 VL 121 IS 7 BP 1328 EP 1350 DI 10.1002/2015JF003803 PG 23 WC Geosciences, Multidisciplinary SC Geology GA DV0AZ UT WOS:000382581200008 PM 28163988 ER PT J AU Donnelly, B Perfect, E McKay, LD Lemiszki, PJ DiStefano, VH Anovitz, LM McFarlane, J Hale, RE Cheng, CL AF Donnelly, B. Perfect, E. McKay, L. D. Lemiszki, P. J. DiStefano, V. H. Anovitz, L. M. McFarlane, J. Hale, R. E. Cheng, C. -L. TI Capillary pressure - saturation relationships for gas shales measured using a water activity meter SO JOURNAL OF NATURAL GAS SCIENCE AND ENGINEERING LA English DT Article DE Water activity meter; Capillary pressure; Volumetric water content; Porosity; Shale; Brooks and Corey ID TIGHT-GAS; SPONTANEOUS IMBIBITION; FRACTAL ANALYSIS; OIL; FLOW; WETTABILITY; HYSTERESIS; RESERVOIRS; BEHAVIOR; SAMPLES AB Hydraulic fracturing of gas shale formations involves pumping a large volume of fracking fluid into a hydrocarbon reservoir to fracture the rock and thus increase its permeability. The majority of the fracking fluid introduced is never recovered and the fate of this lost fluid, often called "leak off," has become the source of much debate. Information on the capillary pressure - saturation relationship for each wetting phase is needed to simulate leak off using numerical reservoir models. The petroleum industry commonly employs air water capillary pressure - saturation curves to predict these relationships for mixed wet reservoirs. Traditional methods of measuring this curve are unsuitable for gas shales due to high capillary pressures associated with the small pores present. A possible alternative method is the water activity meter which is used widely in the soil sciences for such measurements. However, its application to lithified material has been limited. This study utilized a water activity meter to measure air - water capillary pressures (ranging from 1.3 to 219.6 MPa) at several water saturation levels in both the wetting and drying directions. Water contents were measured gravimetrically. Seven types of gas producing shale with different porosities (2.5-13.6%) and total organic carbon contents (0.4-13.5%) were investigated. Nonlinear regression was used to fit the resulting capillary pressure water saturation data pairs for each shale type to the Brooks and Corey equation. Data for six of the seven shale types investigated were successfully fitted (median R-2 = 0.93), indicating this may be a viable method for parameterizing capillary pressure - saturation relationships for inclusion in numerical reservoir models. As expected, the different shale types had statistically different Brooks and Corey parameters. However, there were no significant differences between the Brooks and Corey parameters for the wetting and drying measurements, suggesting that hysteresis may not need to be taken into account in leak off simulations. (C) 2016 Elsevier B.V. All rights reserved. C1 [Donnelly, B.; Perfect, E.; McKay, L. D.] Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN 37996 USA. [Lemiszki, P. J.] Dept Environm & Conservat, Tennessee Div Geol, Knoxville, TN 37921 USA. [DiStefano, V. H.] Univ Tennessee, Bredesen Ctr Interdisciplinary Res & Grad Educ, Knoxville, TN 37996 USA. [DiStefano, V. H.; Anovitz, L. M.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [McFarlane, J.] Oak Ridge Natl Lab, Energy & Transportat Sci Div, Oak Ridge, TN 37831 USA. [Hale, R. E.] Oak Ridge Natl Lab, Reactor & Nucl Syst Div, Oak Ridge, TN 37831 USA. [Cheng, C. -L.] Univ Texas Rio Grande Valley, Dept Environm & Earth Sci, Edinburg, TX 78539 USA. [Cheng, C. -L.] Univ Texas Rio Grande Valley, Dept Civil Engn, Edinburg, TX 78539 USA. RP Perfect, E (reprint author), Univ Tennessee, Dept Earth & Planetary Sci, Knoxville, TN 37996 USA. EM eperfect@utk.edu RI Anovitz, Lawrence/P-3144-2016; OI Anovitz, Lawrence/0000-0002-2609-8750; Cheng, Chu-Lin/0000-0002-1900-463X FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; BDY Environmental LLC, Nashville, TN through a Faculty Achievement Award FX The authors wish to thank Consol Energy Inc. (Pittsburgh, PA) for providing the Chattanooga and Marcellus shale samples. E. Perfect acknowledges funding from David E. Jackson of BDY Environmental LLC, Nashville, TN through a Faculty Achievement Award. Work by V.H. DiStefano and L.M. Anovitz was supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. NR 68 TC 1 Z9 1 U1 14 U2 15 PU ELSEVIER SCI LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND SN 1875-5100 EI 2212-3865 J9 J NAT GAS SCI ENG JI J. Nat. Gas Sci. Eng. PD JUL PY 2016 VL 33 BP 1342 EP 1352 DI 10.1016/j.jngse.2016.05.014 PG 11 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DT6KV UT WOS:000381594000118 ER PT J AU Montgomery, CL Keereetaweep, J Johnson, HM Grillo, SL Chapman, KD Koulen, P AF Montgomery, Christa L. Keereetaweep, Jantana Johnson, Heather M. Grillo, Stephanie L. Chapman, Kent D. Koulen, Peter TI Changes in Retinal N-Acylethanolamines and their Oxylipin Derivatives During the Development of Visual Impairment in a Mouse Model for Glaucoma SO LIPIDS LA English DT Article DE Acylethanolamides; Anandamide; Contrast sensitivity; DBA/2; Intraocular pressure; Lipoxin; Lipoxygenase; Neuroprotection; N-Linoleoylethanolamine; N-Oleylethanolamine; Optokinetic reflex; Optomotor; Visual acuity ID ACID AMIDE HYDROLASE; CANNABINOID CB1 RECEPTORS; GANGLION-CELL DEATH; OXIDATIVE STRESS; ENDOCANNABINOIDS; PALMITOYLETHANOLAMINE; LIPOXYGENASES; PATHWAYS; TISSUES; LIPIDS AB Neurons are especially susceptible to oxidative damage, which is increasingly implicated in neurodegenerative disease. Certain N-acylethanolamines (NAEs) have been shown to protect neurons from oxidative stress. Since glaucoma may be considered a neurodegenerative disorder and the survival of retinal neurons could also be influenced by N-acylethanolamines, our goal was to quantify changes in certain N-acylethanolamine species and their oxylipin derivatives in the retina of a mouse model for glaucoma. We also sought to identify relationships between these and parameters of glaucoma disease development, specifically intraocular pressure, visual acuity, and contrast sensitivity. Five N-acylethanolamine species and three NAE oxylipin derivatives were quantified in retina from young and aged DBA/2Crl mice. N-Acylethanolamines and NAE-oxylipins in retinal extracts were quantified against deuterated standards by isotope dilution gas chromatography-mass spectrometry. Levels (nmol/g dry weight) of N-arachidonoylethanolamine (anandamide; NAE 20:4) were significantly (p = 0.008) decreased in aged (2.875 +/- 0.6702) compared to young animals (5.175 +/- 0.971). Conversely, the anandamide oxylipin, 15(S)-HETE ethanolamide (15(S)-HETE EA), was significantly (p = 0.042) increased in aged (0.063 +/- 0.009) compared to young animals (0.039 +/- 0.011). Enzymatic depletion of the anandamide pool by 15-lipoxygenase and consequent accumulation of 15(S)-HETE ethanolamine may contribute to decreased visual function in glaucomatous mice. Since N-acylethanolamines effectively attenuate glaucoma pathogenesis and associated visual impairment, our data provides additional rationale and novel targets for glaucoma therapies. C1 [Montgomery, Christa L.; Johnson, Heather M.; Grillo, Stephanie L.; Koulen, Peter] Univ Missouri, Sch Med, Dept Ophthalmol, Vis Res Ctr, Kansas City, MO 64108 USA. [Keereetaweep, Jantana; Chapman, Kent D.; Koulen, Peter] Univ North Texas, Dept Biol Sci, Ctr Plant Lipid Res, Denton, TX 76203 USA. [Koulen, Peter] Univ Missouri, Sch Med, Dept Basic Med Sci, Kansas City, MO 64108 USA. Brookhaven Natl Lab, Dept Biol, 50 Bell Ave, Upton, NY 11973 USA. RP Koulen, P (reprint author), Univ Missouri, Sch Med, Dept Ophthalmol, Vis Res Ctr, Kansas City, MO 64108 USA.; Koulen, P (reprint author), Univ North Texas, Dept Biol Sci, Ctr Plant Lipid Res, Denton, TX 76203 USA.; Koulen, P (reprint author), Univ Missouri, Sch Med, Dept Basic Med Sci, Kansas City, MO 64108 USA. EM koulenp@umkc.edu FU National Eye Institute [EY022774]; National Institute on Aging [AG010485, AG022550, AG027956]; National Center for Research Resources; National Institute of General Medical Sciences of the National Institutes of Health [RR027093]; US Department of Energy, Office of Science, Basic Energy Sciences program [DE-FG02-05ER15647]; Felix and Carmen Sabates Missouri Endowed Chair in Vision Research, a Challenge Grant from Research to Prevent Blindness; Vision Research Foundation of Kansas City FX The present study was supported in part by grants from the National Eye Institute (EY022774), the National Institute on Aging (AG010485, AG022550 and AG027956), the National Center for Research Resources and National Institute of General Medical Sciences (RR027093) of the National Institutes of Health (PK). The content of the present study is the sole responsibility of the authors and does not necessarily represent the official views of the National Institutes of Health. Lipid analysis was supported by a grant from the US Department of Energy, Office of Science, Basic Energy Sciences program (DE-FG02-05ER15647; KDC). K.D.C. is grateful to the US National Science Foundation for providing individual research and development leave to assist in the supervision of this research and the preparation of this manuscript by agreement under the Intergovernmental Personnel Act. Additional partial support was provided by the Felix and Carmen Sabates Missouri Endowed Chair in Vision Research, a Challenge Grant from Research to Prevent Blindness and the Vision Research Foundation of Kansas City (PK) and is gratefully acknowledged. The authors thank Margaret, Richard and Sara Koulen for their generous support and encouragement. NR 36 TC 0 Z9 0 U1 1 U2 1 PU SPRINGER HEIDELBERG PI HEIDELBERG PA TIERGARTENSTRASSE 17, D-69121 HEIDELBERG, GERMANY SN 0024-4201 EI 1558-9307 J9 LIPIDS JI Lipids PD JUL PY 2016 VL 51 IS 7 BP 857 EP 866 DI 10.1007/s11745-016-4161-x PG 10 WC Biochemistry & Molecular Biology; Nutrition & Dietetics SC Biochemistry & Molecular Biology; Nutrition & Dietetics GA DR8UB UT WOS:000380171800007 PM 27221132 ER PT J AU Yu, L Bonnell, E Homa, D Pickrell, G Wang, AB Ohodnicki, PR Woodruff, S Chorpening, B Buric, M AF Yu, Li Bonnell, Elizabeth Homa, Daniel Pickrell, Gary Wang, Anbo Ohodnicki, P. R., Jr. Woodruff, Steven Chorpening, Benjamin Buric, Michael TI Observation of temperature dependence of the IR hydroxyl absorption bands in silica optical fiber SO OPTICAL FIBER TECHNOLOGY LA English DT Article DE Fused silica; Glass; Fiber optics; Hydroxyl absorption band ID OH-GROUPS; VIBRATIONAL-MODES; FUSED-SILICA; GLASS; HYDROGEN; SPECTRA; SENSORS; SILANOL; REGION; WATER AB This study reports on the temperature dependent behavior of silica based optical fibers upon exposure to high temperatures in hydrogen and ambient air. The hydroxyl absorption bands in the wavelength range of 1000-2500 nm of commercially available multimode fibers with pure silica and germanium doped cores were examined in the temperature range of 20-800 degrees C. Two hydroxyl-related infrared absorption bands were observed: similar to 2200 nm assigned to the combination of the vibration mode of Si-OH bending and the fundamental hydroxyl stretching mode, and similar to 1390 nm assigned to the first overtone of the hydroxyl stretching. The absorption in the 2200 nm band decreased in intensity, while the 1390 nm absorption band shifted to longer wavelengths with an increase in temperature. The observed phenomena were reversible with temperature and suspected to be due, in part, to the conversion of the OH spectral components into each other and structural relaxation. (C) 2016 Elsevier Inc. All rights reserved. C1 [Yu, Li; Bonnell, Elizabeth; Homa, Daniel; Pickrell, Gary; Wang, Anbo; Ohodnicki, P. R., Jr.; Woodruff, Steven; Chorpening, Benjamin; Buric, Michael] Natl Energy Technol Lab, 3610 Collins Ferry Rd, Morgantown, WV 26507 USA. [Yu, Li; Wang, Anbo] Virginia Polytech Inst & State Univ, Ctr Photon Technol, Bradley Dept Elect & Comp Engn, 460 Turner St,Suite 303, Blacksburg, VA 24061 USA. [Bonnell, Elizabeth; Homa, Daniel; Pickrell, Gary] Virginia Polytech Inst & State Univ, Dept Mat Sci & Engn, 213 Holden Hall, Blacksburg, VA 24061 USA. [Ohodnicki, P. R., Jr.] Carnegie Mellon Univ, Dept Mat Sci & Engn, Pittsburgh, PA 15213 USA. RP Yu, L (reprint author), Virginia Polytech Inst & State Univ, Ctr Photon Technol, Bradley Dept Elect & Comp Engn, 460 Turner St,Suite 303, Blacksburg, VA 24061 USA. EM yuli@vt.edu NR 33 TC 2 Z9 2 U1 8 U2 8 PU ELSEVIER SCIENCE INC PI NEW YORK PA 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA SN 1068-5200 EI 1095-9912 J9 OPT FIBER TECHNOL JI Opt. Fiber Technol. PD JUL PY 2016 VL 30 BP 1 EP 7 DI 10.1016/j.yofte.2016.01.004 PG 7 WC Engineering, Electrical & Electronic; Optics; Telecommunications SC Engineering; Optics; Telecommunications GA DU5OO UT WOS:000382261300001 ER PT J AU Bongard, MW Barr, JL Fonck, RJ Reusch, JA Thome, KE AF Bongard, M. W. Barr, J. L. Fonck, R. J. Reusch, J. A. Thome, K. E. TI On virial analysis at low aspect ratio SO PHYSICS OF PLASMAS LA English DT Article ID SPHERICAL TORUS PLASMAS; EQUILIBRIUM RECONSTRUCTION; CROSS-SECTION; TOKAMAK; PARAMETERS; PROFILE; SHAPE; LI AB The validity of virial analysis to infer global MHD equilibrium poloidal beta beta(p) and internal inductance l(i) from external magnetics measurements is examined for low aspect ratio configurations with A < 2. Numerical equilibrium studies at varied aspect ratio are utilized to validate the technique at finite aspect ratio. The effect of applying high-A approximations to low-A experimental data is quantified and demonstrates significant over-estimation of stored energy (factors of 2-10) in spherical tokamak geometry. Experimental approximations to equilibrium-dependent volume integral terms in the analysis are evaluated at low-A. Highly paramagnetic configurations are found to be inadequately represented through the virial mean radius parameter R-T. Alternate formulations for inferring beta(p) and l(i) that are independent of R-T to avoid this difficulty are presented for the static isotropic limit. These formulations are suitable for fast estimation of tokamak stored energy components at low aspect ratio using virial analysis. Published by AIP Publishing. C1 [Bongard, M. W.; Barr, J. L.; Fonck, R. J.; Reusch, J. A.; Thome, K. E.] Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. [Thome, K. E.] Oak Ridge Associated Univ, Oak Ridge, TN 37831 USA. RP Bongard, MW (reprint author), Univ Wisconsin, Dept Engn Phys, Madison, WI 53706 USA. OI Thome, Kathreen/0000-0002-4801-3922 FU U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences [DE-FG02-96ER54375] FX This material was based upon work supported by the U.S. Department of Energy, Office of Science, Office of Fusion Energy Sciences, under Award No. DE-FG02-96ER54375. Data from this publication are publicly available in openly documented, machine-readable formats.24 Disclaimer: any opinions, findings, and conclusions or recommendations expressed in this publication are those of the author(s) and do not necessarily reflect the views of the U.S. Department of Energy. NR 24 TC 0 Z9 0 U1 1 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 072508 DI 10.1063/1.4959808 PG 8 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800043 ER PT J AU Chung, M Qin, H Davidson, RC AF Chung, Moses Qin, Hong Davidson, Ronald C. TI Envelope Hamiltonian for charged-particle dynamics in general linear coupled systems SO PHYSICS OF PLASMAS LA English DT Article AB We report the discovery of an envelope Hamiltonian describing the charged-particle dynamics in general linear coupled lattices. Published by AIP Publishing. C1 [Chung, Moses] Ulsan Natl Inst Sci & Technol, Dept Phys, Ulsan 689798, South Korea. [Qin, Hong; Davidson, Ronald C.] Princeton Univ, Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. [Qin, Hong] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. RP Chung, M (reprint author), Ulsan Natl Inst Sci & Technol, Dept Phys, Ulsan 689798, South Korea. EM mchung@unist.ac.kr FU National Research Foundation of Korea - Korean Government (MSIP: Ministry of Science, ICT and Future Planning) [NRF-2015R1D1A1A01061074]; UNIST (Ulsan National Institute of Science and Technology) [1.150124.01]; U.S. Department of Energy [DE-AC02-09CH11466] FX This work was supported by the National Research Foundation of Korea (NRF-2015R1D1A1A01061074) grant funded by the Korean Government (MSIP: Ministry of Science, ICT and Future Planning) and by the 2015 UMI Research Fund (1.150124.01) of UNIST (Ulsan National Institute of Science and Technology). This work was also supported by the U.S. Department of Energy Grant No. DE-AC02-09CH11466. NR 13 TC 0 Z9 0 U1 2 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 074507 DI 10.1063/1.4959112 PG 4 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800112 ER PT J AU Clark, DS Weber, CR Smalyuk, VA Robey, HF Kritcher, AL Milovich, JL Salmonson, JD AF Clark, D. S. Weber, C. R. Smalyuk, V. A. Robey, H. F. Kritcher, A. L. Milovich, J. L. Salmonson, J. D. TI Mitigating the impact of hohlraum asymmetries in National Ignition Facility implosions using capsule shims SO PHYSICS OF PLASMAS LA English DT Article ID NOVA AB Current indirect drive implosion experiments on the National Ignition Facility (NIF) [Moses et al., Phys. Plasmas 16, 041006 (2009)] are believed to be strongly impacted by long wavelength perturbations driven by asymmetries in the hohlraum x-ray flux. To address this perturbation source, active efforts are underway to develop modified hohlraum designs with reduced asymmetry imprint. An alternative strategy, however, is to modify the capsule design to be more resilient to a given amount of hohlraum asymmetry. In particular, the capsule may be deliberately misshaped, or "shimmed," so as to counteract the expected asymmetries from the hohlraum. Here, the efficacy of capsule shimming to correct the asymmetries in two recent NIF implosion experiments is assessed using two-dimensional radiation hydrodynamics simulations. Despite the highly time-dependent character of the asymmetries and the high convergence ratios of these implosions, simulations suggest that shims could be highly effective at counteracting current asymmetries and result in factors of a few enhancements in neutron yields. For higher compression designs, the yield improvement could be even greater. Published by AIP Publishing. C1 [Clark, D. S.; Weber, C. R.; Smalyuk, V. A.; Robey, H. F.; Kritcher, A. L.; Milovich, J. L.; Salmonson, J. D.] Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94550 USA. RP Clark, DS (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94550 USA. FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 50 TC 1 Z9 1 U1 4 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 072707 DI 10.1063/1.4958812 PG 11 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800053 ER PT J AU Gerashchenko, S Livescu, D AF Gerashchenko, S. Livescu, D. TI Viscous effects on the Rayleigh-Taylor instability with background temperature gradient SO PHYSICS OF PLASMAS LA English DT Article ID INERTIAL CONFINEMENT FUSION; NUMERICAL SIMULATIONS; LINEAR-STABILITY; HEAT-TRANSFER; PLASMAS; GROWTH; FLUIDS; MODEL; INTERFACE; DYNAMICS AB The growth rate of the compressible Rayleigh-Taylor instability is studied in the presence of a background temperature gradient, Theta, using a normal mode analysis. The effect of Theta variation is examined for three interface types corresponding to the combinations of the viscous properties of the fluids (inviscid-inviscid, viscous-viscous, and viscous-inviscid) at different Atwood numbers, At, and when at least one of the fluids' viscosity is non-zero, as a function of the Grashof number. For the general case, the resulting ordinary differential equations are solved numerically; however, dispersion relations for the growth rate are presented for several limiting cases. An analytical solution is found for the inviscid-inviscid interface and the corresponding dispersion equation for the growth rate is obtained in the limit of large Theta. For the viscous-inviscid case, a dispersion relation is derived in the incompressible limit and Theta = 0. Compared to Theta = 0 case, the role of Theta < 0 (hotter light fluid) is destabilizing and becomes stabilizing when Theta > 0 (colder light fluid). The most pronounced effect of Theta not equal 0 is found at low At and/or at large perturbation wavelengths relative to the domain size for all interface types. On the other hand, at small perturbation wavelengths relative to the domain size, the growth rate for the Theta < 0 case exceeds the infinite domain incompressible constant density result. The results are applied to two practical examples, using sets of parameters relevant to Inertial Confinement Fusion coasting stage and solar corona plumes. The role of viscosity on the growth rate reduction is discussed together with highlighting the range of wavenumbers most affected by viscosity. The viscous effects further increase in the presence of background temperature gradient, when the viscosity is temperature dependent. Published by AIP Publishing. C1 [Gerashchenko, S.] Los Alamos Natl Lab, MPA CMMS CNLS, Los Alamos, NM 87545 USA. [Livescu, D.] Los Alamos Natl Lab, CCS 2, Los Alamos, NM 87545 USA. RP Livescu, D (reprint author), Los Alamos Natl Lab, CCS 2, Los Alamos, NM 87545 USA. EM livescu@lanl.gov OI Livescu, Daniel/0000-0003-2367-1547 FU LDRD program at Los Alamos National Laboratory [20150568ER]; U.S. Department of Energy NNSA [DE-AC52-06NA25396] FX The authors would like to thank H. Yu and R. McClarren for help with the early stages of this paper. This work was made possible in part by funding from the LDRD program at Los Alamos National Laboratory through Project No. 20150568ER. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC for the U.S. Department of Energy NNSA under Contract No. DE-AC52-06NA25396. Computational resources were provided by the LANL Institutional Computing (IC) Program. NR 48 TC 0 Z9 0 U1 4 U2 4 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 072121 DI 10.1063/1.4959810 PG 14 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800026 ER PT J AU Haines, BM Grim, GP Fincke, JR Shah, RC Forrest, CJ Silverstein, K Marshall, FJ Boswell, M Fowler, MM Gore, RA Hayes-Sterbenz, AC Jungman, G Klein, A Rundberg, RS Steinkamp, MJ Wilhelmy, JB AF Haines, Brian M. Grim, Gary P. Fincke, James R. Shah, Rahul C. Forrest, Chad J. Silverstein, Kevin Marshall, Frederic J. Boswell, Melissa Fowler, Malcolm M. Gore, Robert A. Hayes-Sterbenz, Anna C. Jungman, Gerard Klein, Andreas Rundberg, Robert S. Steinkamp, Michael J. Wilhelmy, Jerry B. TI Detailed high-resolution three-dimensional simulations of OMEGA separated reactants inertial confinement fusion experiments SO PHYSICS OF PLASMAS LA English DT Article ID DIRECT-DRIVE IMPLOSIONS; LASER; DISPERSION; UNIFORMITY; REDUCTION; SHELL; MIX AB We present results from the comparison of high-resolution three-dimensional (3D) simulations with data from the implosions of inertial confinement fusion capsules with separated reactants performed on the OMEGA laser facility. Each capsule, referred to as a "CD Mixcap," is filled with tritium and has a polystyrene (CH) shell with a deuterated polystyrene (CD) layer whose burial depth is varied. In these implosions, fusion reactions between deuterium and tritium ions can occur only in the presence of atomic mix between the gas fill and shell material. The simulations feature accurate models for all known experimental asymmetries and do not employ any adjustable parameters to improve agreement with experimental data. Simulations are performed with the RAGE radiation-hydrodynamics code using an Implicit Large Eddy Simulation (ILES) strategy for the hydrodynamics. We obtain good agreement with the experimental data, including the DT/TT neutron yield ratios used to diagnose mix, for all burial depths of the deuterated shell layer. Additionally, simulations demonstrate good agreement with converged simulations employing explicit models for plasma diffusion and viscosity, suggesting that the implicit sub-grid model used in ILES is sufficient to model these processes in these experiments. In our simulations, mixing is driven by short-wavelength asymmetries and longer-wavelength features are responsible for developing flows that transport mixed material towards the center of the hot spot. Mix material transported by this process is responsible for most of the mix (DT) yield even for the capsule with a CD layer adjacent to the tritium fuel. Consistent with our previous results, mix does not play a significant role in TT neutron yield degradation; instead, this is dominated by the displacement of fuel from the center of the implosion due to the development of turbulent instabilities seeded by long-wavelength asymmetries. Through these processes, the long-wavelength asymmetries degrade TT yield more than the DT yield and thus bring DT/TT neutron yield ratios into agreement with experiment. Finally, we present a detailed comparison of the flows in 2D and 3D simulations. Published by AIP Publishing. C1 [Haines, Brian M.; Fincke, James R.; Shah, Rahul C.; Boswell, Melissa; Fowler, Malcolm M.; Gore, Robert A.; Hayes-Sterbenz, Anna C.; Jungman, Gerard; Klein, Andreas; Rundberg, Robert S.; Steinkamp, Michael J.; Wilhelmy, Jerry B.] Los Alamos Natl Lab, MS T087, Los Alamos, NM 87545 USA. [Grim, Gary P.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Forrest, Chad J.; Silverstein, Kevin; Marshall, Frederic J.] Univ Rochester, Laser Energet Lab, 250 E River Rd, Rochester, NY 14623 USA. RP Haines, BM (reprint author), Los Alamos Natl Lab, MS T087, Los Alamos, NM 87545 USA. EM bmhaines@lanl.gov OI klein, andreas/0000-0003-2358-2691; Haines, Brian/0000-0002-3889-7074 FU U.S. Department of Energy NNSA [DE-AC52-06NA25396] FX The authors would like to thank C. Aldrich, J. Campbell, G. Hale, T. Masser, M. McKay, R. Rauenzahn, and C. Snell for useful discussions and code debugging assistance. Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the U.S. Department of Energy NNSA under Contract No. DE-AC52-06NA25396. NR 54 TC 0 Z9 0 U1 8 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 072709 DI 10.1063/1.4959117 PG 13 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800055 ER PT J AU Lan, T Liu, HQ Liu, J Jie, YX Wang, YL Gao, X Qin, H AF Lan, T. Liu, H. Q. Liu, J. Jie, Y. X. Wang, Y. L. Gao, X. Qin, H. TI Design of geometric phase measurement in EAST Tokamak SO PHYSICS OF PLASMAS LA English DT Article ID BERRY TOPOLOGICAL PHASE; OPTICAL-FIBER; PURE FARADAY; POLARIMETRY; SYSTEM; ITER AB The optimum scheme for geometric phase measurement in EAST Tokamak is proposed in this paper. The theoretical values of geometric phase for the probe beams of EAST Polarimeter-Interferometer (POINT) system are calculated by path integration in parameter space. Meanwhile, the influences of some controllable parameters on geometric phase are evaluated. The feasibility and challenge of distinguishing geometric effect in the POINT signal are also assessed in detail. Published by AIP Publishing. C1 [Lan, T.; Liu, J.; Wang, Y. L.; Qin, H.] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Lan, T.; Liu, J.; Wang, Y. L.; Qin, H.] Univ Sci & Technol China, Sch Nucl Sci & Technol, Hefei 230026, Anhui, Peoples R China. [Lan, T.; Liu, H. Q.; Jie, Y. X.; Gao, X.] Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Anhui, Peoples R China. [Qin, H.] Princeton Univ, Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. RP Liu, HQ (reprint author), Chinese Acad Sci, Inst Plasma Phys, Hefei 230031, Anhui, Peoples R China. EM hqliu@ipp.ac.cn OI lan, ting/0000-0001-9853-1982; liu, hai qing/0000-0001-6892-358X; Liu, Jian/0000-0001-7484-401X; Wang, Yulei/0000-0001-9863-5917 FU National Magnetic Confinement Fusion Program of China [2012GB101002, 2014GB106002]; National Nature Science Foundation of China [11375237, 11305171, 11575185, 11575186]; ITER-China Program [2015GB111003, 2014GB124005] FX This work was supported by the National Magnetic Confinement Fusion Program of China with Contract Nos: 2012GB101002 and 2014GB106002, the National Nature Science Foundation of China with Contract Nos. 11375237; 11305171; 11575185; and 11575186, ITER-China Program with Contract Nos. 2015GB111003 and 2014GB124005. NR 26 TC 1 Z9 1 U1 7 U2 8 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 072109 DI 10.1063/1.4958310 PG 6 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800014 ER PT J AU Lee, WW AF Lee, W. W. TI Magnetohydrodynamics for collisionless plasmas from the gyrokinetic perspective SO PHYSICS OF PLASMAS LA English DT Article ID PARTICLE SIMULATION; EQUATIONS; TOKAMAKS AB The effort to obtain a set of MagnetoHydroDynamic (MHD) equations for a magnetized collisionless plasma was started nearly 60 years ago by Chew et al. [Proc. R. Soc. London, Ser. A 236(1204), 112-118 (1956)]. Many attempts have been made ever since. Here, we will show the derivation of a set of these equations from the gyrokinetic perspective, which we call it gyrokinetic MHD, and it is different from the conventional ideal MHD. However, this new set of equations still has conservation properties and, in the absence of fluctuations, recovers the usual MHD equilibrium. Furthermore, the resulting equations allow for the plasma pressure balance to be further modified by finite-Larmor-radius effects in regions with steep pressure gradients. The present work is an outgrowth of the paper on "Alfven Waves in Gyrokinetic Plasmas" by Lee and Qin [Phys. Plasmas 10, 3196 (2003)]. Published by AIP Publishing. C1 [Lee, W. W.] Princeton Univ, Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. RP Lee, WW (reprint author), Princeton Univ, Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. FU U.S. DoE [DE-AC02-09CH11466] FX The author wishes to thank Professor Russell Kulsrud of Princeton University for his interest in this work and his critical comments, also to Dr. Peter Porazik and Dr. Stuart Hudson of PPPL for useful discussions. This work was partially supported by U.S. DoE, Grant DE-AC02-09CH11466. NR 22 TC 0 Z9 0 U1 2 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 070705 DI 10.1063/1.4960029 PG 5 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800005 ER PT J AU Ogawa, S Cambon, B Leoncini, X Vittot, M del Castillo-Negrete, D Dif-Pradalier, G Garbet, X AF Ogawa, Shun Cambon, Benjamin Leoncini, Xavier Vittot, Michel del Castillo-Negrete, Diego Dif-Pradalier, Guilhem Garbet, Xavier TI Full particle orbit effects in regular and stochastic magnetic fields SO PHYSICS OF PLASMAS LA English DT Article ID PRESERVING NONTWIST MAPS; GUIDING-CENTER MOTION; ADIABATIC-INVARIANT; SEPARATRIX; CHAOS; SYSTEMS; TRANSITION; TRANSPORT; PHYSICS AB We present a numerical study of charged particle motion in a time-independent magnetic field in cylindrical geometry. The magnetic field model consists of an unperturbed reversed-shear (non-monotonic q-profile) helical part and a perturbation consisting of a superposition of modes. Contrary to most of the previous studies, the particle trajectories are computed by directly solving the full Lorentz force equations of motion in a six-dimensional phase space using a sixth-order, implicit, symplectic Gauss-Legendre method. The level of stochasticity in the particle orbits is diagnosed using averaged, effective Poincare sections. It is shown that when only one mode is present, the particle orbits can be stochastic even though the magnetic field line orbits are not stochastic (i.e., fully integrable). The lack of integrability of the particle orbits in this case is related to separatrix crossing and the breakdown of the global conservation of the magnetic moment. Some perturbation consisting of two modes creates resonance overlapping, leading to Hamiltonian chaos in magnetic field lines. Then, the particle orbits exhibit a nontrivial dynamics depending on their energy and pitch angle. It is shown that the regions where the particle motion is stochastic decrease as the energy increases. The non-monotonicity of the q-profile implies the existence of magnetic ITBs (internal transport barriers) which correspond to shearless flux surfaces located in the vicinity of the q-profile minimum. It is shown that depending on the energy, these magnetic ITBs might or might not confine particles. That is, magnetic ITBs act as an energy-dependent particle confinement filter. Magnetic field lines in reversed-shear configurations exhibit topological bifurcations (from homoclinic to heteroclinic) due to separatrix reconnection. We show that a similar but more complex scenario appears in the case of particle orbits that depend in a non-trivial way on the energy and pitch angle of the particles. Published by AIP Publishing. C1 [Ogawa, Shun; Cambon, Benjamin; Leoncini, Xavier; Vittot, Michel] Univ Toulon & Var, Aix Marseille Univ, CNRS, CPT, Marseille, France. [Ogawa, Shun; Dif-Pradalier, Guilhem; Garbet, Xavier] CEA, IRFM, F-13108 St Paul Les Durance, France. [del Castillo-Negrete, Diego] Oak Ridge Natl Lab, Oak Ridge, TN 37831 USA. RP Ogawa, S (reprint author), Univ Toulon & Var, Aix Marseille Univ, CNRS, CPT, Marseille, France.; Ogawa, S (reprint author), CEA, IRFM, F-13108 St Paul Les Durance, France. EM shun.ogawa@cpt.univ-mrs.fr RI Dif-Pradalier, Guilhem/K-7442-2015; OI del-Castillo-Negrete, Diego/0000-0001-7183-801X; Dif-Pradalier, Guilhem/0000-0003-4869-7049; Garbet, Xavier/0000-0001-5730-1259 FU A*MIDEX project - "investissements d'Avenir" French Government program [ANR-11-IDEX-0001-02]; Office of Fusion Energy Sciences of the U.S. Department of Energy at Oak Ridge National Laboratory for the U.S. Department of Energy [DE-AC05-00OR22725] FX This work has been carried out thanks to the support of the A*MIDEX project (No. ANR-11-IDEX-0001-02) funded by the "investissements d'Avenir" French Government program, managed by the French National Research Agency (ANR). D.d.C.-N. acknowledges support from the Office of Fusion Energy Sciences of the U.S. Department of Energy at Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy under Contract No. DE-AC05-00OR22725. NR 32 TC 1 Z9 1 U1 2 U2 2 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 072506 DI 10.1063/1.4958653 PG 12 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800041 ER PT J AU Perkins, RJ Hosea, JC Bertelli, N Taylor, G Wilson, JR AF Perkins, R. J. Hosea, J. C. Bertelli, N. Taylor, G. Wilson, J. R. TI Resonance in fast-wave amplitude in the periphery of cylindrical plasmas and application to edge losses of wave heating power in tokamaks SO PHYSICS OF PLASMAS LA English DT Article ID GENERATION AB Heating magnetically confined plasmas using waves in the ion-cyclotron range of frequencies typically requires coupling these waves over a steep density gradient. This process has produced an unexpected and deleterious phenomenon on the National Spherical Torus eXperiment (NSTX): a prompt loss of wave power along magnetic field lines in front of the antenna to the divertor. Understanding this loss may be key to achieving effective heating and expanding the operational space of NSTX-Upgrade. Here, we propose that a new type of mode, which conducts a significant fraction of the total wave power in the low-density peripheral plasma, is driving these losses. We demonstrate the existence of such modes, which are distinct from surface modes and coaxial modes, in a cylindrical cold-plasma model when a half wavelength structure fits into the region outside the core plasma. The latter condition generalizes the previous hypothesis regarding the occurrence of the edge losses and may explain why full-wave simulations predict these losses in some cases but not others. If valid, this condition implies that outer gap control is a potential strategy for mitigating the losses in NSTX-Upgrade in addition to raising the magnetic field or influencing the edge density. Published by AIP Publishing. C1 [Perkins, R. J.; Hosea, J. C.; Bertelli, N.; Taylor, G.; Wilson, J. R.] Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. RP Perkins, RJ (reprint author), Princeton Plasma Phys Lab, Princeton, NJ 08540 USA. OI wilson, james/0000-0003-3627-1278; Perkins, Rory/0000-0002-7216-0201 FU DOE [DE-AC02-09CH11466] FX This work was supported by DOE Contract No. DE-AC02-09CH11466. The digital data for this paper can be found in http://arks.princeton.edu/ark:/88435/dsp018p58pg29j. We gratefully acknowledge R. I. Pinsker and S. J. Zweben for useful discussions and S. M. Kaye and P. T. Bonoli for critically reading the manuscript. NR 18 TC 0 Z9 0 U1 3 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 070702 DI 10.1063/1.4954899 PG 5 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800002 ER PT J AU Reiman, AH AF Reiman, Allan H. TI Pressure driven currents near magnetic islands in 3D MHD equilibria: Effects of pressure variation within flux surfaces and of symmetry SO PHYSICS OF PLASMAS LA English DT Article ID NEOCLASSICAL TEARING MODES; HYDROMAGNETIC EQUILIBRIA; PLASMA EQUILIBRIUM; TOROIDAL PLASMA; STELLARATORS; SEPARATRIX; EQUATIONS; FIELDS AB In toroidal, magnetically confined plasmas, the heat and particle transport is strongly anisotropic, with transport along the field lines sufficiently strong relative to cross-field transport that the equilibrium pressure can generally be regarded as constant on the flux surfaces in much of the plasma. The regions near small magnetic islands, and those near the X-lines of larger islands, are exceptions, having a significant variation of the pressure within the flux surfaces. It is shown here that the variation of the equilibrium pressure within the flux surfaces in those regions has significant consequences for the pressure driven currents. It is further shown that the consequences are strongly affected by the symmetry of the magnetic field if the field is invariant under combined reflection in the poloidal and toroidal angles. (This symmetry property is called "stellarator symmetry.") In non-stellarator-symmetric equilibria, the pressure-driven currents have logarithmic singularities at the X-lines. In stellarator-symmetric MHD equilibria, the singular components of the pressure-driven currents vanish. These equilibria are to be contrasted with equilibria having B . del p = 0; where the singular components of the pressure-driven currents vanish regardless of the symmetry. They are also to be contrasted with 3D MHD equilibrium solutions that are constrained to have simply nested flux surfaces, where the pressure-driven current goes like 1/x near rational surfaces, where x is the distance from the rational surface, except in the case of quasi-symmetric flux surfaces. For the purpose of calculating the pressure-driven currents near magnetic islands, we work with a closed subset of the MHD equilibrium equations that involves only perpendicular force balance, and is decoupled from parallel force balance. It is not correct to use the parallel component of the conventional MHD force balance equation, B . del p = 0; near magnetic islands. Small but nonzero values of B . del p are important in this region, and small non-MHD contributions to the parallel force balance equation cannot be neglected there. Two approaches are pursued to solve our equations for the pressure driven currents. First, the equilibrium equations are applied to an analytically tractable magnetic field with an island, obtaining explicit expressions for the rotational transform and magnetic coordinates, and for the pressure-driven current and its limiting behavior near the X-line. The second approach utilizes an expansion about the X-line to provide a more general calculation of the pressure-driven current near an X-line and of the rotational transform near a separatrix. The study presented in this paper is motivated, in part, by tokamak experiments with nonaxisymmetric magnetic perturbations, where significant differences are observed between the behavior of stellarator-symmetric and non-stellarator-symmetric configurations with regard to stabilization of edge localized modes by resonant magnetic perturbations. Implications for the coupling between neoclassical tearing modes, and for magnetic island stability calculations, are also discussed. Published by AIP Publishing. C1 [Reiman, Allan H.] Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. RP Reiman, AH (reprint author), Princeton Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. FU DOE [DEAC02-76CH03073] FX I am grateful to Per Helander for his comments on an earlier version of this manuscript. This work was supported by DOE Contract No. DEAC02-76CH03073. NR 45 TC 0 Z9 0 U1 6 U2 6 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 072502 DI 10.1063/1.4954900 PG 14 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800037 ER PT J AU Ruby, JJ Pak, A Field, JE Ma, T Spears, BK Benedetti, LR Bradley, DK Hopkins, LFB Casey, DT Doppner, T Eder, D Fittinghoff, D Grim, G Hatarik, R Hinkel, DE Izumi, N Kilkenny, JD Khan, SF Knauer, JP Kritcher, AL Merrill, FE Moody, JD Nagel, SR Park, HS Salmonson, JD Sayre, DB Callahan, DA Hsing, WW Hurricane, OA Patel, PK Edwards, MJ AF Ruby, J. J. Pak, A. Field, J. E. Ma, T. Spears, B. K. Benedetti, L. R. Bradley, D. K. Hopkins, L. F. Berzak Casey, D. T. Doeppner, T. Eder, D. Fittinghoff, D. Grim, G. Hatarik, R. Hinkel, D. E. Izumi, N. Kilkenny, J. D. Khan, S. F. Knauer, J. P. Kritcher, A. L. Merrill, F. E. Moody, J. D. Nagel, S. R. Park, H. -S. Salmonson, J. D. Sayre, D. B. Callahan, D. A. Hsing, W. W. Hurricane, O. A. Patel, P. K. Edwards, M. J. TI Spatially resolved X-ray emission measurements of the residual velocity during the stagnation phase of inertial confinement fusion implosion experiments SO PHYSICS OF PLASMAS LA English DT Article ID IGNITION; GAIN AB A technique for measuring residual motion during the stagnation phase of an indirectly driven inertial confinement experiment has been implemented. This method infers a velocity from spatially and temporally resolved images of the X-ray emission from two orthogonal lines of sight. This work investigates the accuracy of recovering spatially resolved velocities from the X-ray emission data. A detailed analytical and numerical modeling of the X-ray emission measurement shows that the accuracy of this method increases as the displacement that results from a residual velocity increase. For the typical experimental configuration, signal-to-noise ratios, and duration of X-ray emission, it is estimated that the fractional error in the inferred velocity rises above 50% as the velocity of emission falls below 24 mu m/ns. By inputting measured parameters into this model, error estimates of the residual velocity as inferred from the X-ray emission measurements are now able to be generated for experimental data. Details of this analysis are presented for an implosion experiment conducted with an unintentional radiation flux asymmetry. The analysis shows a bright localized region of emission that moves through the larger emitting volume at a relatively higher velocity towards the location of the imposed flux deficit. This technique allows for the possibility of spatially resolving velocity flows within the so-called central hot spot of an implosion. This information would help to refine our interpretation of the thermal temperature inferred from the neutron time of flight detectors and the effect of localized hydrodynamic instabilities during the stagnation phase. Across several experiments, along a single line of sight, the average difference in magnitude and direction of the measured residual velocity as inferred from the X-ray and neutron time of flight detectors was found to be similar to 13 mu m/ns and similar to 14 degrees, respectively. Published by AIP Publishing. C1 [Ruby, J. J.; Pak, A.; Field, J. E.; Ma, T.; Spears, B. K.; Benedetti, L. R.; Bradley, D. K.; Hopkins, L. F. Berzak; Casey, D. T.; Doeppner, T.; Eder, D.; Fittinghoff, D.; Grim, G.; Hatarik, R.; Hinkel, D. E.; Izumi, N.; Khan, S. F.; Kritcher, A. L.; Moody, J. D.; Nagel, S. R.; Park, H. -S.; Salmonson, J. D.; Sayre, D. B.; Callahan, D. A.; Hsing, W. W.; Hurricane, O. A.; Patel, P. K.; Edwards, M. J.] Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94550 USA. [Kilkenny, J. D.] Gen Atom, POB 85608, San Diego, CA 92186 USA. [Knauer, J. P.] Laser Energet Lab, 250 East River Rd,POB 278871, Rochester, NY 14623 USA. [Merrill, F. E.] Los Alamos Natl Lab, POB 1663, Los Alamos, NM 87545 USA. RP Pak, A (reprint author), Lawrence Livermore Natl Lab, POB 808, Livermore, CA 94550 USA. EM pak5@llnl.gov RI Patel, Pravesh/E-1400-2011 FU U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX The authors sincerely thank the NIF operations staff who supported this work. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 23 TC 1 Z9 1 U1 7 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 072701 DI 10.1063/1.4956468 PG 13 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800047 ER PT J AU Wang, ZY Lin, Y Wang, XY Tummel, K Chen, L AF Wang, Zhenyu Lin, Yu Wang, Xueyi Tummel, Kurt Chen, Liu TI 3D electrostatic gyrokinetic electron and fully kinetic ion simulation of lower-hybrid drift instability of Harris current sheet SO PHYSICS OF PLASMAS LA English DT Article ID COLLISIONLESS MAGNETIC RECONNECTION; 3-DIMENSIONAL PARTICLE SIMULATIONS; NEUTRAL SHEET; NONLINEAR EVOLUTION; TURBULENCE; PLASMA; ONSET; RESISTIVITY; EIGENMODES; EQUATIONS AB The eigenmode stability properties of three-dimensional lower-hybrid-drift-instabilities (LHDI) in a Harris current sheet with a small but finite guide magnetic field have been systematically studied by employing the gyrokinetic electron and fully kinetic ion (GeFi) particle-in-cell (PIC) simulation model with a realistic ion-to-electron mass ratio m(i)/m(e). In contrast to the fully kinetic PIC simulation scheme, the fast electron cyclotron motion and plasma oscillations are systematically removed in the GeFi model, and hence one can employ the realistic m(i)/m(e). The GeFi simulations are bench-marked against and show excellent agreement with both the fully kinetic PIC simulation and the analytical eigenmode theory. Our studies indicate that, for small wavenumbers, k(y), along the current direction, the most unstable eigenmodes are peaked at the location where (k) over right arrow. (B) over right arrow = 0, consistent with previous analytical and simulation studies. Here, (B) over right arrow is the equilibrium magnetic field and (k) over right arrow is the wavevector perpendicular to the nonuniformity direction. As k(y) increases, however, the most unstable eigenmodes are found to be peaked at (k) over right arrow. (B) over right arrow not equal 0. In addition, the simulation results indicate that varying m(i)/m(e), the current sheet width, and the guide magnetic field can affect the stability of LHDI. Simulations with the varying mass ratio confirm the lower hybrid frequency and wave number scalings. Published by AIP Publishing. C1 [Wang, Zhenyu; Lin, Yu; Wang, Xueyi] Auburn Univ, Dept Phys, Auburn, AL 36849 USA. [Tummel, Kurt; Chen, Liu] Univ Calif Irvine, Dept Phys & Astron, Irvine, CA 92697 USA. [Tummel, Kurt] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Chen, Liu] Zhejiang Univ, Inst Fus Theory & Simulat, Hangzhou 310058, Zhejiang, Peoples R China. RP Wang, ZY (reprint author), Auburn Univ, Dept Phys, Auburn, AL 36849 USA. EM zzw0008@tigermail.auburn.edu RI chen, liu/I-2297-2013 FU NSF [ATM-0646442, ATM-0852682, PHY-0903794]; NASA [NNX10AK97G]; DoE [DE-SC0010486]; U.S. NSF; DoE; ITER-CN; China Scholarship Council; [NSFC 41028003]; [NSFC 40890163]; [NSFC 11235009]; [NSFC-11235009] FX This work was supported by NSF Grant Nos. ATM-0646442 and ATM-0852682 and PHY-0903794 and NASA Grant No. NNX10AK97G and DoE Grant No. DE-SC0010486 to Auburn University, and Grant Nos. NSFC 41028003, NSFC 40890163, and NSFC 11235009. Research at UC Irvine was supported by U.S. NSF and DoE grants, and the authors acknowledge support from ITER-CN grants and the NSFC-11235009 grant. Z. Wang was supported in part by the scholarship from China Scholarship Council. High performance computing resources were provided by Auburn University and Alabama Supercomputing Center. NR 50 TC 0 Z9 0 U1 3 U2 3 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 072104 DI 10.1063/1.4954830 PG 10 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800009 ER PT J AU Zhang, RL Qin, H Davidson, RC Liu, J Xiao, JY AF Zhang, Ruili Qin, Hong Davidson, Ronald C. Liu, Jian Xiao, Jianyuan TI On the structure of the two-stream instability-complex G-Hamiltonian structure and Krein collisions between positive-and negative-action modes SO PHYSICS OF PLASMAS LA English DT Article ID MAXWELL-VLASOV EQUATIONS; SYSTEM AB The two-stream instability is probably the most important elementary example of collective instabilities in plasma physics and beam-plasma systems. For a warm plasma with two charged particle species, the instability diagram of the two-stream instability based on a 1D warm-fluid model exhibits an interesting band structure that has not been explained. We show that the band structure for this instability is the consequence of the Hamiltonian nature of the warm two-fluid system. Interestingly, the Hamiltonian nature manifests as a complex G-Hamiltonian structure in wave-number space, which directly determines the instability diagram. Specifically, it is shown that the boundaries between the stable and unstable regions are locations for Krein collisions between eigenmodes with different Krein signatures. In terms of physics, this rigorously implies that the system is destabilized when a positive-action mode resonates with a negative-action mode, and that this is the only mechanism by which the system can be destabilized. It is anticipated that this physical mechanism of destabilization is valid for other collective instabilities in conservative systems in plasma physics, accelerator physics, and fluid dynamics systems, which admit infinite-dimensional Hamiltonian structures. Published by AIP Publishing. C1 [Zhang, Ruili; Qin, Hong; Liu, Jian; Xiao, Jianyuan] Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China. [Zhang, Ruili; Qin, Hong; Liu, Jian; Xiao, Jianyuan] Univ Sci & Technol China, Sch Nucl Sci & Technol, Hefei 230026, Anhui, Peoples R China. [Zhang, Ruili; Liu, Jian; Xiao, Jianyuan] Chinese Acad Sci, Key Lab Geospace Environm, Hefei 230026, Anhui, Peoples R China. [Qin, Hong; Davidson, Ronald C.] Princeton Univ, Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. RP Qin, H (reprint author), Univ Sci & Technol China, Dept Modern Phys, Hefei 230026, Anhui, Peoples R China.; Qin, H (reprint author), Univ Sci & Technol China, Sch Nucl Sci & Technol, Hefei 230026, Anhui, Peoples R China.; Qin, H (reprint author), Princeton Univ, Plasma Phys Lab, POB 451, Princeton, NJ 08543 USA. EM hongqin@princeton.edu OI Liu, Jian/0000-0001-7484-401X FU National Natural Science Foundation of China [NSFC-11505186, 11575185, 11575186]; ITER-China Program [2015GB111003, 2014GB124005]; Fundamental Research Funds for the Central Universities [WK2030040068]; China Postdoctoral Science Foundation [2015M581994]; CAS Program for Interdisciplinary Collaboration Team; Geo-Algorithmic Plasma Simulator (GAPS) Project; U.S. Department of Energy [DE-AC02-09CH11466] FX This research was supported by the National Natural Science Foundation of China (NSFC-11505186, 11575185, and 11575186), ITER-China Program (2015GB111003 and 2014GB124005), the Fundamental Research Funds for the Central Universities (No. WK2030040068), the China Postdoctoral Science Foundation (No. 2015M581994), the CAS Program for Interdisciplinary Collaboration Team, the Geo-Algorithmic Plasma Simulator (GAPS) Project, and the U.S. Department of Energy (DE-AC02-09CH11466). NR 26 TC 0 Z9 0 U1 8 U2 9 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 1070-664X EI 1089-7674 J9 PHYS PLASMAS JI Phys. Plasmas PD JUL PY 2016 VL 23 IS 7 AR 072111 DI 10.1063/1.4954832 PG 7 WC Physics, Fluids & Plasmas SC Physics GA DU8FD UT WOS:000382447800016 ER PT J AU Peris, D Langdon, QK Moriarty, RV Sylvester, K Bontrager, M Charron, G Leducq, JB Landry, CR Libkind, D Hittinger, CT AF Peris, David Langdon, Quinn K. Moriarty, Ryan V. Sylvester, Kayla Bontrager, Martin Charron, Guillaume Leducq, Jean-Baptiste Landry, Christian R. Libkind, Diego Hittinger, Chris Todd TI Complex Ancestries of Lager-Brewing Hybrids Were Shaped by Standing Variation in the Wild Yeast Saccharomyces eubayanus SO PLOS GENETICS LA English DT Article ID NEW-ZEALAND EVIDENCE; GENOME SEQUENCE; POPULATION-STRUCTURE; MIGRATORY BIRDS; DOMESTICATION; EVOLUTION; CEREVISIAE; DIVERSITY; WINE; FERMENTATION AB Lager-style beers constitute the vast majority of the beer market, and yet, the genetic origin of the yeast strains that brew them has been shrouded in mystery and controversy. Unlike alestyle beers, which are generally brewed with Saccharomyces cerevisiae, lagers are brewed at colder temperatures with allopolyploid hybrids of Saccharomyces eubayanus x S. cerevisiae. Since the discovery of S. eubayanus in 2011, additional strains have been isolated from South America, North America, Australasia, and Asia, but only interspecies hybrids have been isolated in Europe. Here, using genome sequence data, we examine the relationships of these wild S. eubayanus strains to each other and to domesticated lager strains. Our results support the existence of a relatively low-diversity (pi = 0.00197) lineage of S. eubayanus whose distribution stretches across the Holarctic ecozone and includes wild isolates from Tibet, new wild isolates from North America, and the S. eubayanus parents of lager yeasts. This Holarctic lineage is closely related to a population with higher diversity (pi = 0.00275) that has been found primarily in South America but includes some widely distributed isolates. A second diverse South American population (pi = 0.00354) and two early-diverging Asian subspecies are more distantly related. We further show that no single wild strain from the Holarctic lineage is the sole closest relative of lager yeasts. Instead, different parts of the genome portray different phylogenetic signals and ancestry, likely due to outcrossing and incomplete lineage sorting. Indeed, standing genetic variation within this wild Holarctic lineage of S. eubayanus is responsible for genetic variation still segregating among modern lager-brewing hybrids. We conclude that the relationships among wild strains of S. eubayanus and their domesticated hybrids reflect complex biogeographical and genetic processes. C1 [Peris, David; Langdon, Quinn K.; Moriarty, Ryan V.; Sylvester, Kayla; Bontrager, Martin; Hittinger, Chris Todd] Univ Wisconsin, JF Crow Inst Study Evolut, Genet Lab, Genome Ctr Wisconsin,Wisconsin Energy Inst, Madison, WI USA. [Peris, David; Moriarty, Ryan V.; Sylvester, Kayla; Hittinger, Chris Todd] Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI USA. [Charron, Guillaume; Leducq, Jean-Baptiste; Landry, Christian R.] Univ Laval, IBIS, Dept Biol, PROTEO, Pavillon Charles Eugene Marchand, Quebec City, PQ, Canada. [Libkind, Diego] Ctr Reg Univ Bariloche, Inst Andino Patagon Tecnol Biol & Geoambientales, Lab Microbiol Aplicada Biotecnol & Bioinformat, IPATEC CONICET UNComahue, San Carlos De Bariloche, Rio Negro, Argentina. RP Hittinger, CT (reprint author), Univ Wisconsin, JF Crow Inst Study Evolut, Genet Lab, Genome Ctr Wisconsin,Wisconsin Energy Inst, Madison, WI USA.; Hittinger, CT (reprint author), Univ Wisconsin, DOE Great Lakes Bioenergy Res Ctr, Madison, WI USA. EM cthittinger@wisc.edu OI Charron, Guillaume/0000-0001-5971-3337; Peris, David/0000-0001-9912-8802 FU National Science Foundation [DGE-1256259, DEB-1253634]; Predoctoral Training Program in Genetics - National Institutes of Health [5 T32 GM007133-40]; Natural Sciences and Engineering Research Council of Canada (NSERC); ANPCyT [PICT2011-1814, PICT2014-2542]; UNComahue [B171]; CONICET [11220130100392CO]; NSF-CONICET; USDA National Institute of Food and Agriculture [1003258]; DOE Great Lakes Bioenergy Research Center (DOE Office of Science BER) [DE-FC02-07ER64494]; Pew Charitable Trusts; Alexander von Humboldt Foundation FX This material is based upon work supported by the National Science Foundation Graduate Research Fellowship under Grant No. DGE-1256259 to QKL and MB; QKL and MB were also supported by the Predoctoral Training Program in Genetics, funded by the National Institutes of Health (5 T32 GM007133-40). CRL was funded by a Discovery grant from the Natural Sciences and Engineering Research Council of Canada (NSERC). CRL holds the Canada Research Chair in Evolutionary Cell and Systems Biology. DL was funded by ANPCyT (PICT2011-1814, and PICT2014-2542), UNComahue (B171), CONICET (11220130100392CO), and NSF-CONICET Bilateral Cooperation Projects. This material is based upon work supported by the National Science Foundation under Grant No. DEB-1253634 to CTH, by USDA National Institute of Food and Agriculture Hatch Project 1003258, and funded in part by the DOE Great Lakes Bioenergy Research Center (DOE Office of Science BER DE-FC02-07ER64494). CTH is a Pew Scholar in the Biomedical Sciences and an Alfred Toepfer Faculty Fellow, supported by the Pew Charitable Trusts and the Alexander von Humboldt Foundation, respectively. The funders had no role in study design, data collection and analysis, decision to publish, or preparation of the manuscript. NR 59 TC 4 Z9 4 U1 13 U2 15 PU PUBLIC LIBRARY SCIENCE PI SAN FRANCISCO PA 1160 BATTERY STREET, STE 100, SAN FRANCISCO, CA 94111 USA SN 1553-7404 J9 PLOS GENET JI PLoS Genet. PD JUL PY 2016 VL 12 IS 7 AR e1006155 DI 10.1371/journal.pgen.1006155 PG 20 WC Genetics & Heredity SC Genetics & Heredity GA DS8RI UT WOS:000381050100023 PM 27385107 ER PT J AU Sparks, AM Kolden, CA Talhelm, AF Smith, AMS Apostol, KG Johnson, DM Boschetti, L AF Sparks, Aaron M. Kolden, Crystal A. Talhelm, Alan F. Smith, Alistair M. S. Apostol, Kent G. Johnson, Daniel M. Boschetti, Luigi TI Spectral Indices Accurately Quantify Changes in Seedling Physiology Following Fire: Towards Mechanistic Assessments of Post-Fire Carbon Cycling SO REMOTE SENSING LA English DT Article DE fire; remote sensing; severity; carbon; recovery; mortality ID NORMALIZED BURN RATIO; UNITED-STATES; WILDFIRE SEVERITY; REFLECTANCE; PHOTOSYNTHESIS; ECOSYSTEMS; MORTALITY; BIOMASS; NDVI; HYPOTHESIS AB Fire activity, in terms of intensity, frequency, and total area burned, is expected to increase with a changing climate. A challenge for landscape-level assessment of fire effects, often termed burn severity, is that current remote sensing assessments provide very little information regarding tree/vegetation physiological performance and recovery, limiting our understanding of fire effects on ecosystem services such as carbon storage/cycling. In this paper, we evaluated whether spectral indices common in vegetation stress and burn severity assessments could accurately quantify post-fire physiological performance (indicated by net photosynthesis and crown scorch) of two seedling species, Larix occidentalis and Pinus contorta. Seedlings were subjected to increasing fire radiative energy density (FRED) doses through a series of controlled laboratory surface fires. Mortality, physiology, and spectral reflectance were assessed for a month following the fires, and then again at one year post-fire. The differenced Normalized Difference Vegetation Index (dNDVI) spectral index outperformed other spectral indices used for vegetation stress and burn severity characterization in regard to leaf net photosynthesis quantification, indicating that landscape-level quantification of tree physiology may be possible. Additionally, the survival of the majority of seedlings in the low and moderate FRED doses indicates that fire-induced mortality is more complex than the currently accepted binary scenario, where trees survive with no impacts below a certain temperature and duration threshold, and mortality occurs above the threshold. C1 [Sparks, Aaron M.; Kolden, Crystal A.; Smith, Alistair M. S.; Johnson, Daniel M.; Boschetti, Luigi] Univ Idaho, Coll Nat Resources, Moscow, ID 83844 USA. [Sparks, Aaron M.; Kolden, Crystal A.; Smith, Alistair M. S.] Univ Idaho, IFIRE, Moscow, ID 83844 USA. [Talhelm, Alan F.] US EPA, Oak Ridge Inst Sci Educ, Natl Ctr Environm Assessment, Res Triangle Pk, NC 27711 USA. [Apostol, Kent G.] Univ Arizona, Coll Agr & Life Sci, Payson, AZ 85541 USA. RP Sparks, AM (reprint author), Univ Idaho, Coll Nat Resources, Moscow, ID 83844 USA.; Sparks, AM (reprint author), Univ Idaho, IFIRE, Moscow, ID 83844 USA. EM spar5010@vandals.uidaho.edu; ckolden@uidaho.edu; atalhelm@uidaho.edu; alistair@uidaho.edu; kapostol@gmail.com; danjohnson@uidaho.edu; luigi@uidaho.edu RI Boschetti, Luigi/C-6198-2008; Johnson, Daniel/E-6789-2011; OI Boschetti, Luigi/0000-0001-6525-4413; Johnson, Daniel/0000-0001-5890-3147; Smith, Alistair/0000-0003-0071-9958; Kolden, Crystal/0000-0001-7093-4552 FU National Aeronautics and Space Administration (NASA) [NNX11AO24G]; National Science Foundation [IOS-1146751, DEB-1251441, IIA-1301792]; National Science Foundation under Hazards SEES award [DMS-1520873]; Idaho Space Grant Consortium FX Seedlings were grown at the University of Idaho's Center for Forest Nursery and Seedling Research and combustion experiments were conducted within the Idaho Fire Initiative for Research and Education (IFIRE) combustion laboratory. This work was partially funded by the National Aeronautics and Space Administration (NASA) under award NNX11AO24G and the National Science Foundation under award IOS-1146751 to Dan Johnson. Partial support for Alan Talhelm was provided by the National Science Foundation under award DEB-1251441. Partial funding for this research for Aaron Sparks, Alistair Smith, and Crystal Kolden was provided by the National Science Foundation under Hazards SEES award DMS-1520873. Alistair Smith received partial support from the National Science Foundation award IIA-1301792. Aaron Sparks was additionally funded through the Idaho Space Grant Consortium. The views expressed in this paper are those of the authors and do not necessarily represent the views or policies of the U.S. Environmental Protection Agency. NR 62 TC 4 Z9 4 U1 7 U2 8 PU MDPI AG PI BASEL PA ST ALBAN-ANLAGE 66, CH-4052 BASEL, SWITZERLAND SN 2072-4292 J9 REMOTE SENS-BASEL JI Remote Sens. PD JUL PY 2016 VL 8 IS 7 AR UNSP 572 DI 10.3390/rs8070572 PG 13 WC Remote Sensing SC Remote Sensing GA DU5AR UT WOS:000382224800042 ER PT J AU Hoffman, AS Debefve, LM Bendjeriou-Sedjerari, A Ouldchikh, S Bare, SR Basset, JM Gates, BC AF Hoffman, A. S. Debefve, L. M. Bendjeriou-Sedjerari, A. Ouldchikh, S. Bare, Simon R. Basset, J. -M. Gates, B. C. TI Transmission and fluorescence X-ray absorption spectroscopy cell/flow reactor for powder samples under vacuum or in reactive atmospheres SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID IN-SITU; CATALYSTS; CELL; SILICA; EXAFS; COMPLEXES; CHEMISTRY; MODEL AB X-ray absorption spectroscopy is an element-specific technique for probing the local atomic-scale environment around an absorber atom. It is widely used to investigate the structures of liquids and solids, being especially valuable for characterization of solid-supported catalysts. Reported cell designs are limited in capabilities-to fluorescence or transmission and to static or flowing atmospheres, or to vacuum. Our goal was to design a robust and widely applicable cell for catalyst characterizations under all these conditions-to allow tracking of changes during genesis and during operation, both under vacuum and in reactive atmospheres. Herein, we report the design of such a cell and a demonstration of its operation both with a sample under dynamic vacuum and in the presence of gases flowing at temperatures up to 300 degrees C, showing data obtained with both fluorescence and transmission detection. The cell allows more flexibility in catalyst characterization than any reported. Published by AIP Publishing. C1 [Hoffman, A. S.; Debefve, L. M.; Gates, B. C.] Univ Calif Davis, Dept Chem Engn, Davis, CA 95616 USA. [Bendjeriou-Sedjerari, A.; Ouldchikh, S.; Basset, J. -M.] KAUST, KCC, Thuwal 239556900, Saudi Arabia. [Bare, Simon R.] SSRL, SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA. RP Gates, BC (reprint author), Univ Calif Davis, Dept Chem Engn, Davis, CA 95616 USA. EM bcgates@ucdavis.edu OI Bare, Simon/0000-0002-4932-0342; basset, jean marie/0000-0003-3166-8882 FU King Abdullah University of Science and Technology; U.S. Department of Energy, Office of Science, Basic Energy Sciences [FG02-04ER15513, DE-AC02-76SF00515]; Chevron FX We thank A. Cobb and J. Roach of the University of California, Davis, Biological and Agricultural Engineering Machine Shop, for design consultation and cell fabrication, and R. Davis of the Stanford Synchrotron Radiation Lightsource (SSRL) for helpful discussions. We thank SSRL for beam time (beamline 4-1). The work was funded by the King Abdullah University of Science and Technology and by the U.S. Department of Energy, Office of Science, Basic Energy Sciences (Grant No. FG02-04ER15513). Use of SSRL, SLAC National Accelerator Laboratory, is supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences (Grant No. DE-AC02-76SF00515). A. S. Hoffman was supported by a fellowship from Chevron. NR 25 TC 1 Z9 1 U1 5 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JUL PY 2016 VL 87 IS 7 AR 073108 DI 10.1063/1.4958824 PG 7 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA DU8FL UT WOS:000382448600011 PM 27475549 ER PT J AU Merritt, EC Doss, FW AF Merritt, E. C. Doss, F. W. TI Wavelet analysis methods for radiography of multidimensional growth of planar mixing layers SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID SHEAR-LAYER; TRANSFORM; CONVERGENT; PLASMAS; SYSTEM AB The counter-propagating shear campaign is examining instability growth and its transition to turbulence in the high-energy-density physics regime using a laser-driven counter-propagating flow platform. In these experiments, we observe consistent complex break-up of and structure growth in a tracer layer placed at the shear flow interface during the instability growth phase. We present a wavelet-transform based analysis technique capable of characterizing the scale-and directionality-resolved average intensity perturbations in static radiographs of the experiment. This technique uses the complete spatial information available in each radiograph to describe the structure evolution. We designed this analysis technique to generate a two-dimensional power spectrum for each radiograph from which we can recover information about structure widths, amplitudes, and orientations. The evolution of the distribution of power in the spectra for an experimental series is a potential metric for quantifying the structure size evolution as well as a system's evolution towards isotropy. Published by AIP Publishing. C1 [Merritt, E. C.; Doss, F. W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Merritt, EC (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM emerritt@lanl.gov FU U.S. Department of Energy; [DE-AC52-06NA25396] FX The authors would like to extend their gratitude for their contributions to the rest of the LANL counter-propagating Shear team: Kirk Flippo, John Kline, Eric Loomis (P-24), Carlos Di Stefano (XTD-IDA), Susan Kurien (T-5), and Barbara DeVolder (XCP-6). This work was supported by the U.S. Department of Energy and performed by Los Alamos National Laboratory, operated by Los Alamos National Security under Contract No. DE-AC52-06NA25396. NR 32 TC 1 Z9 1 U1 1 U2 1 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JUL PY 2016 VL 87 IS 7 AR 075103 DI 10.1063/1.4955097 PG 12 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA DU8FL UT WOS:000382448600053 PM 27475591 ER PT J AU Opachich, YP Koch, JA Haugh, MJ Romano, E Lee, JJ Huffman, E Weber, FA Bowers, JW Benedetti, LR Wilson, M Prisbrey, ST Wehrenberg, CE Baumann, TF Lenhardt, JM Cook, A Arsenlis, A Park, HS Remington, BA AF Opachich, Y. P. Koch, J. A. Haugh, M. J. Romano, E. Lee, J. J. Huffman, E. Weber, F. A. Bowers, J. W. Benedetti, L. R. Wilson, M. Prisbrey, S. T. Wehrenberg, C. E. Baumann, T. F. Lenhardt, J. M. Cook, A. Arsenlis, A. Park, H. -S. Remington, B. A. TI A multi-wavelength, high-contrast contact radiography system for the study of low-density aerogel foams SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID NATIONAL IGNITION FACILITY; RAY AB A multi-wavelength, high contrast contact radiography system has been developed to characterize density variations in ultra-low density aerogel foams. These foams are used to generate a ramped pressure drive in materials strength experiments at the National Ignition Facility and require precision characterization in order to reduce errors in measurements. The system was used to characterize density variations in carbon and silicon based aerogels to similar to 10.3% accuracy with similar to 30 mu m spatial resolution. The system description, performance, and measurement results collected using a 17.8 mg/cc carbon based JX-6 (C20H30) aerogel are discussed in this manuscript. Published by AIP Publishing. C1 [Opachich, Y. P.; Koch, J. A.; Haugh, M. J.; Romano, E.; Lee, J. J.; Huffman, E.; Weber, F. A.; Bowers, J. W.] Natl Secur Technol LLC, Livermore, CA 94550 USA. [Bowers, J. W.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Benedetti, L. R.; Wilson, M.; Prisbrey, S. T.; Wehrenberg, C. E.; Baumann, T. F.; Lenhardt, J. M.; Cook, A.; Arsenlis, A.; Park, H. -S.; Remington, B. A.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. RP Opachich, YP (reprint author), Natl Secur Technol LLC, Livermore, CA 94550 USA. EM opachiyp@nv.doe.gov OI Haugh, Michael/0000-0002-9613-9220 FU National Security Technologies, LLC [DE-AC52-06NA25946]; U.S. Department of Energy; DOE Public Access Plan [DOE/NV/259469-2663]; U.S. Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This manuscript has been authored by the National Security Technologies, LLC, under Contract No. DE-AC52-06NA25946 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, world-wide license to publish or reproduce the published form of this manuscript, or allow others to do so, for the United States Government purposes. The U.S. Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan), No. DOE/NV/259469-2663. This work was done under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 12 TC 1 Z9 1 U1 4 U2 5 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JUL PY 2016 VL 87 IS 7 AR 073706 DI 10.1063/1.4958826 PG 5 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA DU8FL UT WOS:000382448600026 PM 27475564 ER PT J AU Weber, JKR Tamalonis, A Benmore, CJ Alderman, OLG Sendelbach, S Hebden, A Williamson, MA AF Weber, J. K. R. Tamalonis, A. Benmore, C. J. Alderman, O. L. G. Sendelbach, S. Hebden, A. Williamson, M. A. TI Aerodynamic levitator for in situ x-ray structure measurements on high temperature and molten nuclear fuel materials SO REVIEW OF SCIENTIFIC INSTRUMENTS LA English DT Article ID URANIUM-DIOXIDE; SURFACE-TENSION; AL-27 NMR; LIQUID; SPECTROSCOPY; SYNCHROTRON; DYNAMICS; RAMAN AB An aerodynamic levitator with carbon dioxide laser beam heating was integrated with a hermetically sealed controlled atmosphere chamber and sample handling mechanism. The system enabled containment of radioactive samples and control of the process atmosphere chemistry. The chamber was typically operated at a pressure of approximately 0.9 bars to ensure containment of the materials being processed. Samples 2.5-3 mm in diameter were levitated in flowing gas to achieve containerless conditions. Levitated samples were heated to temperatures of up to 3500 degrees C with a partially focused carbon dioxide laser beam. Sample temperature was measured using an optical pyrometer. The sample environment was integrated with a high energy (100 keV) x-ray synchrotron beamline to enable in situ structure measurements to be made on levitated samples as they were heated, melted, and supercooled. The system was controlled from outside the x-ray beamline hutch by using a LabVIEW program. Measurements have been made on hot solid and molten uranium dioxide and binary uranium dioxide-zirconium dioxide compositions. Published by AIP Publishing. C1 [Weber, J. K. R.; Tamalonis, A.; Alderman, O. L. G.; Sendelbach, S.] Mat Dev Inc, Arlington Hts, IL 60004 USA. [Weber, J. K. R.; Benmore, C. J.; Alderman, O. L. G.] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Hebden, A.; Williamson, M. A.] Argonne Natl Lab, Nucl Engn Div, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Weber, JKR (reprint author), Mat Dev Inc, Arlington Hts, IL 60004 USA.; Weber, JKR (reprint author), Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. OI Weber, Richard/0000-0002-2145-1279; Benmore, Chris/0000-0001-7007-7749 FU MDI from U.S. Department of Energy [DE-SC0007564, DE-SC0015241]; Argonne National Laboratory [6F-30221, 6F-30241, 6F-30581]; [DE-AC02-06CH11357] FX Work was supported under the following contracts: MDI, Contract Nos. DE-SC0007564 and DE-SC0015241 from the U.S. Department of Energy and Contract Nos. 6F-30221, 6F-30241, and 6F-30581 from Argonne National Laboratory. APS, U.S. DOE, Argonne National Laboratory was supported under Contract No. DE-AC02-06CH11357. We thank Douglas Robinson for helping with the beamline experiments at APS and John Vacca and Bruce Glagola for their advice about radiation safety for the beamline installation. NR 34 TC 2 Z9 2 U1 8 U2 12 PU AMER INST PHYSICS PI MELVILLE PA 1305 WALT WHITMAN RD, STE 300, MELVILLE, NY 11747-4501 USA SN 0034-6748 EI 1089-7623 J9 REV SCI INSTRUM JI Rev. Sci. Instrum. PD JUL PY 2016 VL 87 IS 7 AR 073902 DI 10.1063/1.4955210 PG 9 WC Instruments & Instrumentation; Physics, Applied SC Instruments & Instrumentation; Physics GA DU8FL UT WOS:000382448600028 PM 27475566 ER PT J AU Denton, MH Henderson, MG Jordanova, VK Thomsen, MF Borovsky, JE Woodroffe, J Hartley, DP Pitchford, D AF Denton, M. H. Henderson, M. G. Jordanova, V. K. Thomsen, M. F. Borovsky, J. E. Woodroffe, J. Hartley, D. P. Pitchford, D. TI An improved empirical model of electron and ion fluxes at geosynchronous orbit based on upstream solar wind conditions SO SPACE WEATHER-THE INTERNATIONAL JOURNAL OF RESEARCH AND APPLICATIONS LA English DT Article ID LOW-ENERGY ELECTRONS; INNER MAGNETOSPHERE; PLASMA SHEET; MAGNETIC-FIELD; SPACECRAFT; STORM; SATELLITE; TRANSPORT; ACCESS AB A new empirical model of the electron fluxes and ion fluxes at geosynchronous orbit (GEO) is introduced, based on observations by Los Alamos National Laboratory (LANL) satellites. The model provides flux predictions in the energy range similar to 1eV to similar to 40keV, as a function of local time, energy, and the strength of the solar wind electric field (the negative product of the solar wind speed and the z component of the magnetic field). Given appropriate upstream solar wind measurements, the model provides a forecast of the fluxes at GEO with a similar to 1h lead time. Model predictions are tested against in-sample observations from LANL satellites and also against out-of-sample observations from the Compact Environmental Anomaly Sensor II detector on the AMC-12 satellite. The model does not reproduce all structure seen in the observations. However, for the intervals studied here (quiet and storm times) the normalized root-mean-square deviation < similar to 0.3. It is intended that the model will improve forecasting of the spacecraft environment at GEO and also provide improved boundary/input conditions for physical models of the magnetosphere. C1 [Denton, M. H.; Borovsky, J. E.] Space Sci Inst, Ctr Space Plasma Phys, Boulder, CO 80301 USA. [Denton, M. H.] New Mexico Consortium, Los Alamos, NM 87544 USA. [Henderson, M. G.; Jordanova, V. K.; Woodroffe, J.] Los Alamos Natl Lab, ISR 1, Los Alamos, NM USA. [Thomsen, M. F.] Planetary Sci Inst, Tucson, AZ USA. [Borovsky, J. E.] Univ Michigan, Climate & Space Engn, Ann Arbor, MI 48109 USA. [Hartley, D. P.] Univ Iowa, Dept Phys & Astron, Iowa City, IA 52242 USA. [Pitchford, D.] SES Engn, Betzdorf, Luxembourg. RP Denton, MH (reprint author), Space Sci Inst, Ctr Space Plasma Phys, Boulder, CO 80301 USA.; Denton, MH (reprint author), New Mexico Consortium, Los Alamos, NM 87544 USA. EM mdenton@spacescience.org RI Henderson, Michael/A-3948-2011 OI Henderson, Michael/0000-0003-4975-9029 FU Space Hazards Induced near Earth by Large, Dynamic Storms (SHIELDS) project - U.S. Department of Energy through the LANL/LDRD Program [DE-AC52-06NA25396]; Space Science Institute by the NASA Heliophysics LWS program [NNX14AN90G, NNX16AB75G]; NASA Heliophysics GI program [NNX14AC15G]; NSF GEM program [1502947] FX The authors gratefully acknowledge the OMNI database for the solar wind and geophysical parameters used in this study. We also acknowledge use of the list of satellites at GEO maintained by Eric Johnston at www.satsig.net. This work was partially supported by the Space Hazards Induced near Earth by Large, Dynamic Storms (SHIELDS) project, funded by the U.S. Department of Energy through the LANL/LDRD Program under contract DE-AC52-06NA25396. This work was supported at the Space Science Institute by the NASA Heliophysics LWS program via grants NNX14AN90G and NNX16AB75G, the NASA Heliophysics GI program via grant NNX14AC15G, and the NSF GEM program award number 1502947. M.H.D. wishes to thank J. Denton for help with the Kp version of the model and comments on the current manuscript. MPA data are available by contacting the PI, Mike Henderson, at mghenderson@lanl.gov. The model, written in FORTRAN, is available from M.H.D. at mdenton@spacescience.org, or via download at http://gemelli.spacescience.org/mdenton/. NR 41 TC 2 Z9 2 U1 4 U2 4 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 1542-7390 J9 SPACE WEATHER JI Space Weather PD JUL PY 2016 VL 14 IS 7 BP 511 EP 523 DI 10.1002/2016SW001409 PG 13 WC Astronomy & Astrophysics; Geochemistry & Geophysics; Meteorology & Atmospheric Sciences SC Astronomy & Astrophysics; Geochemistry & Geophysics; Meteorology & Atmospheric Sciences GA DV5SS UT WOS:000382990100005 ER PT J AU Gaukler, SM Ruff, JS Potts, WK AF Gaukler, Shannon Marie Ruff, James Steven Potts, Wayne K. TI Paroxetine exposure skews litter sex ratios in mice suggesting a Trivers-Willard process SO BEHAVIORAL ECOLOGY LA English DT Article DE adaptive sex allocation; cost of reproduction hypothesis; fitness assay; paroxetine; SSRI ID HOUSE MICE; RED DEER; COMPETITIVE ABILITY; BREEDING SUCCESS; MUS-MUSCULUS; ALBINO-RAT; WILD BIRD; MANIPULATION; ADJUSTMENT; HYPOTHESIS AB While conducting a toxicity assessment of the antidepressant paroxetine (PaxilA (R)), in wild-derived mice (Mus musculus), we observed that exposed dams (P-0) produced female biased litters (32:68 M:F). Though numerous experimental manipulations have induced sex ratio bias in mice, none have assessed the fitness of the offspring from these litters relative to controls. Here, we retrospectively analyze experimentally derived fitness data gathered for the purpose of toxicological assessment in light of 2 leading hypothesis (Trivers-Willard hypothesis [TWH] and cost of reproduction hypothesis [CRH]), seeking to test if this facultative sex ratio adjustment fits into an adaptive framework. Control F-1 males were heavier than F-1 females, but no differences in mass were detected between exposed F-1 males and females, suggesting that exposed dams did not save energy by producing fewer males, despite producing 29.2% lighter litters relative to controls. F-1 offspring of both treatments were released into seminatural enclosures where fitness was quantified. In enclosures, the relative reproductive success of F-1-exposed males (compared with controls) was reduced by similar to 20% compared with the relative reproductive success of F-1-exposed females. Thus, exposed dams increased their fitness by adjusting litters toward females who were less negatively affected by the exposure than males. Collectively, these data provide less support that the observed sex ratio bias results in energetic savings (CRH), and more support for the TWH because fitness was increased by biasing litters toward female offspring. These mammalian data are unique in their ability to support the TWH through the use of relevant fitness data. C1 [Gaukler, Shannon Marie; Ruff, James Steven; Potts, Wayne K.] Univ Utah, Dept Biol, 257 South 1400 East, Salt Lake City, UT 84112 USA. [Gaukler, Shannon Marie] Los Alamos Natl Lab, ENV ES, Environm Stewardship Grp, Mailstop J978,POB 1663, Los Alamos, NM 87545 USA. RP Gaukler, SM (reprint author), Univ Utah, Dept Biol, 257 South 1400 East, Salt Lake City, UT 84112 USA.; Gaukler, SM (reprint author), Los Alamos Natl Lab, ENV ES, Environm Stewardship Grp, Mailstop J978,POB 1663, Los Alamos, NM 87545 USA. EM sgaukler@lanl.gov FU University of Utah's Technology Commercialization Program; National Institutes of Health [R01-GM109500]; National Science Foundation [DEB 09-18969]; National Science Foundation GK-12 Educational Outreach Fellowship [DGE 08-41233] FX This project was supported by the University of Utah's Technology Commercialization Program and was partially conducted under the support of the National Institutes of Health (R01-GM109500) and National Science Foundation (DEB 09-18969) to (W.P.), and by a National Science Foundation GK-12 Educational Outreach Fellowship (DGE 08-41233) to (S.G.). NR 53 TC 1 Z9 1 U1 7 U2 7 PU OXFORD UNIV PRESS INC PI CARY PA JOURNALS DEPT, 2001 EVANS RD, CARY, NC 27513 USA SN 1045-2249 EI 1465-7279 J9 BEHAV ECOL JI Behav. Ecol. PD JUL-AUG PY 2016 VL 27 IS 4 BP 1113 EP 1121 DI 10.1093/beheco/arw017 PG 9 WC Behavioral Sciences; Biology; Ecology; Zoology SC Behavioral Sciences; Life Sciences & Biomedicine - Other Topics; Environmental Sciences & Ecology; Zoology GA DT1EU UT WOS:000381225300023 PM 27418753 ER PT J AU Shah, I Setzer, RW Jack, J Houck, KA Judson, RS Knudsen, TB Liu, J Martin, MT Reif, DM Richard, AM Thomas, RS Crofton, KM Dix, DJ Kavlock, RJ AF Shah, Imran Setzer, R. Woodrow Jack, John Houck, Keith A. Judson, Richard S. Knudsen, Thomas B. Liu, Jie Martin, Matthew T. Reif, David M. Richard, Ann M. Thomas, Russell S. Crofton, Kevin M. Dix, David J. Kavlock, Robert J. TI Using ToxCast (TM) Data to Reconstruct Dynamic Cell State Trajectories and Estimate Toxicological Points of Departure SO ENVIRONMENTAL HEALTH PERSPECTIVES LA English DT Article ID TOXICITY; 21ST-CENTURY; ADVERSE; SYSTEMS; VISION AB BACKGROUND: High-content imaging (HCI) allows simultaneous measurement of multiple cellular phenotypic changes and is an important tool for evaluating the biological activity of chemicals. OBJECTIVES: Our goal was to analyze dynamic cellular changes using HCI to identify the "tipping point" at which the cells did not show recovery towards a normal phenotypic state. METHODS: HCI was used to evaluate the effects of 967 chemicals (in concentrations ranging from 0.4 to 200 mu M) on HepG2 cells over a 72-hr exposure period. The HCI end points included p53, c-Jun, histone H2A. x, alpha-tubulin, histone H3, alpha tubulin, mitochondrial membrane potential, mitochondrial mass, cell cycle arrest, nuclear size, and cell number. A computational model was developed to interpret HCI responses as cell-state trajectories. RESULTS: Analysis of cell-state trajectories showed that 336 chemicals produced tipping points and that HepG2 cells were resilient to the effects of 334 chemicals up to the highest concentration (200 mu M) and duration (72 hr) tested. Tipping points were identified as concentration-dependent transitions in system recovery, and the corresponding critical concentrations were generally between 5 and 15 times (25th and 75th percentiles, respectively) lower than the concentration that produced any significant effect on HepG2 cells. The remaining 297 chemicals require more data before they can be placed in either of these categories. CONCLUSIONS: These findings show the utility of HCI data for reconstructing cell state trajectories and provide insight into the adaptation and resilience of in vitro cellular systems based on tipping points. Cellular tipping points could be used to define a point of departure for risk-based prioritization of environmental chemicals. C1 [Shah, Imran; Setzer, R. Woodrow; Houck, Keith A.; Judson, Richard S.; Knudsen, Thomas B.; Martin, Matthew T.; Richard, Ann M.; Thomas, Russell S.; Crofton, Kevin M.; Dix, David J.; Kavlock, Robert J.] US EPA, Natl Ctr Computat Toxicol, Off Res & Dev, Res Triangle Pk, NC 27711 USA. [Jack, John] North Carolina State Univ, Dept Stat, Raleigh, NC USA. [Liu, Jie] US DOE, ORISE, Oak Ridge, TN USA. [Reif, David M.] North Carolina State Univ, Dept Biol Sci, Raleigh, NC USA. [Dix, David J.] US EPA, Off Sci Coordinat & Policy, Washington, DC 20460 USA. [Kavlock, Robert J.] US EPA, Off Res & Dev, Washington, DC 20460 USA. [Liu, Jie] US FDA, Ctr Food Safety & Appl Nutr, Off Food Addit Safety, College Pk, MD USA. RP Shah, I (reprint author), US EPA, 109 TW Alexander Dr B205-01, Res Triangle Pk, NC 27711 USA. EM Shah.Imran@epa.gov FU U.S. Environmental Protection Agency (EPA) [EP-D-13-013] FX Cell culture, chemical exposure, and HCI imaging were conducted by Apredica, Watertown, Massachusetts, under U.S. Environmental Protection Agency (EPA) contract EP-D-13-013. NR 28 TC 3 Z9 3 U1 3 U2 4 PU US DEPT HEALTH HUMAN SCIENCES PUBLIC HEALTH SCIENCE PI RES TRIANGLE PK PA NATL INST HEALTH, NATL INST ENVIRONMENTAL HEALTH SCIENCES, PO BOX 12233, RES TRIANGLE PK, NC 27709-2233 USA SN 0091-6765 EI 1552-9924 J9 ENVIRON HEALTH PERSP JI Environ. Health Perspect. PD JUL PY 2016 VL 124 IS 7 BP 910 EP 919 DI 10.1289/ehp.1409029 PG 10 WC Environmental Sciences; Public, Environmental & Occupational Health; Toxicology SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Toxicology GA DS4KF UT WOS:000380749300011 PM 26473631 ER PT J AU Mansouri, K Abdelaziz, A Rybacka, A Roncaglioni, A Tropsha, A Varnek, A Zakharov, A Worth, A Richard, AM Grulke, CM Trisciuzzi, D Fourches, D Horvath, D Benfenati, E Muratov, E Wedebye, EB Grisoni, F Mangiatordi, GF Incisivo, GM Hong, HX Ng, HW Tetko, IV Balabin, I Kancherla, J Shen, J Burton, J Nicklaus, M Cassotti, M Nikolov, NG Nicolotti, O Andersson, PL Zang, QD Politi, R Beger, RD Todeschini, R Huang, RL Farag, S Rosenberg, SA Slavov, S Hu, X Judson, RS AF Mansouri, Kamel Abdelaziz, Ahmed Rybacka, Aleksandra Roncaglioni, Alessandra Tropsha, Alexander Varnek, Alexandre Zakharov, Alexey Worth, Andrew Richard, Ann M. Grulke, Christopher M. Trisciuzzi, Daniela Fourches, Denis Horvath, Dragos Benfenati, Emilio Muratov, Eugene Wedebye, Eva Bay Grisoni, Francesca Mangiatordi, Giuseppe F. Incisivo, Giuseppina M. Hong, Huixiao Ng, Hui W. Tetko, Igor V. Balabin, Ilya Kancherla, Jayaram Shen, Jie Burton, Julien Nicklaus, Marc Cassotti, Matteo Nikolov, Nikolai G. Nicolotti, Orazio Andersson, Patrik L. Zang, Qingda Politi, Regina Beger, Richard D. Todeschini, Roberto Huang, Ruili Farag, Sherif Rosenberg, Sine A. Slavov, Svetoslav Hu, Xin Judson, Richard S. TI CERAPP: Collaborative Estrogen Receptor Activity Prediction Project SO ENVIRONMENTAL HEALTH PERSPECTIVES LA English DT Article ID ENDOCRINE-DISRUPTING CHEMICALS; COMPUTATIONAL TOXICOLOGY RESOURCE; QUANTITATIVE STRUCTURE-ACTIVITY; THROUGHPUT SCREENING ASSAYS; RELATIONSHIP QSDAR MODELS; ENVIRONMENTAL CHEMICALS; DECISION FOREST; PARTITION-COEFFICIENTS; BINARY CLASSIFICATION; BIOLOGICAL-ACTIVITY AB BACKGROUND: Humans are exposed to thousands of man-made chemicals in the environment. Some chemicals mimic natural endocrine hormones and, thus, have the potential to be endocrine disruptors. Most of these chemicals have never been tested for their ability to interact with the estrogen receptor (ER). Risk assessors need tools to prioritize chemicals for evaluation in costly in vivo tests, for instance, within the U.S. EPA Endocrine Disruptor Screening Program. OBJECTIVES: We describe a large-scale modeling project called CERAPP (Collaborative Estrogen Receptor Activity Prediction Project) and demonstrate the efficacy of using predictive computational models trained on high-throughput screening data to evaluate thousands of chemicals for ER-related activity and prioritize them for further testing. METHODS: CERAPP combined multiple models developed in collaboration with 17 groups in the United States and Europe to predict ER activity of a common set of 32,464 chemical structures. Quantitative structure-activity relationship models and docking approaches were employed, mostly using a common training set of 1,677 chemical structures provided by the U.S. EPA, to build a total of 40 categorical and 8 continuous models for binding, agonist, and antagonist ER activity. All predictions were evaluated on a set of 7,522 chemicals curated from the literature. To overcome the limitations of single models, a consensus was built by weighting models on scores based on their evaluated accuracies. RESULTS: Individual model scores ranged from 0.69 to 0.85, showing high prediction reliabilities. Out of the 32,464 chemicals, the consensus model predicted 4,001 chemicals (12.3%) as high priority actives and 6,742 potential actives (20.8%) to be considered for further testing. CONCLUSION: This project demonstrated the possibility to screen large libraries of chemicals using a consensus of different in silico approaches. This concept will be applied in future projects related to other end points. C1 [Mansouri, Kamel; Richard, Ann M.; Grulke, Christopher M.; Kancherla, Jayaram; Judson, Richard S.] US EPA, Natl Ctr Computat Toxicol, 109 TW Alexander Dr, Res Triangle Pk, NC 27711 USA. [Mansouri, Kamel] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Abdelaziz, Ahmed; Tetko, Igor V.] German Res Ctr Environm Hlth GmbH, Helmholtz Zentrum Muenchen, Inst Struct Biol, Neuherberg, Germany. [Rybacka, Aleksandra; Andersson, Patrik L.] Umea Univ, Dept Chem, Umea, Sweden. [Roncaglioni, Alessandra; Benfenati, Emilio; Incisivo, Giuseppina M.] Ist Ric Farmacol Mario Negri, IRCCS, Environm Chem & Toxicol Lab, Milan, Italy. [Tropsha, Alexander; Fourches, Denis; Muratov, Eugene; Politi, Regina; Farag, Sherif] Univ North Carolina Chapel Hill, Lab Mol Modeling, Chapel Hill, NC USA. [Varnek, Alexandre; Horvath, Dragos] Univ Strasbourg, Lab Chemoinformat, Strasbourg, France. [Zakharov, Alexey; Nicklaus, Marc] NCI, NIH, US Dept HHS, Bethesda, MD 20892 USA. [Worth, Andrew; Burton, Julien] European Commiss Ispra, Joint Res Ctr, IHCP, Ispra, Italy. [Trisciuzzi, Daniela; Mangiatordi, Giuseppe F.; Nicolotti, Orazio] Univ Bari, Dept Pharmacy Drug Sci, Bari, Italy. [Wedebye, Eva Bay; Nikolov, Nikolai G.; Rosenberg, Sine A.] Tech Univ Denmark, Natl Food Inst, Div Toxicol & Risk Assessment, Copenhagen, Denmark. [Grisoni, Francesca; Cassotti, Matteo; Todeschini, Roberto] Univ Milano Bicocca, Milano Chemometr & QSAR Res Grp, Milan, Italy. [Hong, Huixiao; Ng, Hui W.] US FDA, Div Bioinformat & Biostat, Natl Ctr Toxicol Res, USDA, Jefferson, AZ USA. [Tetko, Igor V.] BigChem GmbH, Neuherberg, Germany. [Balabin, Ilya] Lockheed Martin, High Performance Comp, Res Triangle Pk, NC USA. [Shen, Jie] Res Inst Fragrance Mat Inc, Woodcliff Lake, NJ USA. [Zang, Qingda; Slavov, Svetoslav] Integrated Lab Syst Inc, Res Triangle Pk, NC USA. [Beger, Richard D.] USDA, Div Syst Biol, Natl Ctr Toxicol Res, Jefferson, AZ USA. [Huang, Ruili; Hu, Xin] NIH, Natl Ctr Adv Translat Sci, DHHS, Bldg 10, Bethesda, MD 20892 USA. RP Judson, RS (reprint author), US EPA, Natl Ctr Computat Toxicol, 109 TW Alexander Dr, Res Triangle Pk, NC 27711 USA. EM judson.richard@epa.gov RI Tetko, Igor/B-1540-2010; Varnek, Alexandre/E-7076-2017; Kancherla, Jayaram/P-7756-2015; OI Tetko, Igor/0000-0002-6855-0012; Varnek, Alexandre/0000-0003-1886-925X; Kancherla, Jayaram/0000-0001-5855-5031; Mansouri, Kamel/0000-0002-6426-8036 FU NIGMS NIH HHS [T32 GM067553] NR 101 TC 17 Z9 17 U1 13 U2 15 PU US DEPT HEALTH HUMAN SCIENCES PUBLIC HEALTH SCIENCE PI RES TRIANGLE PK PA NATL INST HEALTH, NATL INST ENVIRONMENTAL HEALTH SCIENCES, PO BOX 12233, RES TRIANGLE PK, NC 27709-2233 USA SN 0091-6765 EI 1552-9924 J9 ENVIRON HEALTH PERSP JI Environ. Health Perspect. PD JUL PY 2016 VL 124 IS 7 BP 1023 EP 1033 DI 10.1289/ehp.1510267 PG 11 WC Environmental Sciences; Public, Environmental & Occupational Health; Toxicology SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Toxicology GA DS4KF UT WOS:000380749300025 PM 26908244 ER PT J AU Leung, MCK Phuong, J Baker, NC Sipes, NS Klinefelter, GR Martin, MT McLaurin, KW Setzer, RW Darney, SP Judson, RS Knudsen, TB AF Leung, Maxwell C. K. Phuong, Jimmy Baker, Nancy C. Sipes, Nisha S. Klinefelter, Gary R. Martin, Matthew T. McLaurin, Keith W. Setzer, R. Woodrow Darney, Sally Perreault Judson, Richard S. Knudsen, Thomas B. TI Systems Toxicology of Male Reproductive Development: Profiling 774 Chemicals for Molecular Targets and Adverse Outcomes SO ENVIRONMENTAL HEALTH PERSPECTIVES LA English DT Article ID TESTICULAR DYSGENESIS SYNDROME; INTERLEUKIN-6 SIGNAL BLOCKADE; GERM-CELL DIFFERENTIATION; RECEPTOR TYROSINE KINASE; GENOME-WIDE ASSOCIATION; LARGE GENE LISTS; FETAL TESTIS; DI(N-BUTYL) PHTHALATE; NUCLEAR RECEPTORS; DIETHYLHEXYL PHTHALATE AB BACKGROUND: Trends in male reproductive health have been reported for increased rates of testicular germ cell tumors, low semen quality, cryptorchidism, and hypospadias, which have been associated with prenatal environmental chemical exposure based on human and animal studies. OBJECTIVE: In the present study we aimed to identify significant correlations between environmental chemicals, molecular targets, and adverse outcomes across a broad chemical landscape with emphasis on developmental toxicity of the male reproductive system. METHODS: We used U.S. EPA's animal study database (ToxRefDB) and a comprehensive literature analysis to identify 774 chemicals that have been evaluated for adverse effects on male reproductive parameters, and then used U.S. EPA's in vitro high-throughput screening (HTS) database (ToxCastDB) to profile their bioactivity across approximately 800 molecular and cellular features. RESULTS: A phenotypic hierarchy of testicular atrophy, sperm effects, tumors, and malformations, a composite resembling the human testicular dysgenesis syndrome (TDS) hypothesis, was observed in 281 chemicals. A subset of 54 chemicals with male developmental consequences had in vitro bioactivity on molecular targets that could be condensed into 156 gene annotations in a bipartite network. CONCLUSION: Computational modeling of available in vivo and in vitro data for chemicals that produce adverse effects on male reproductive end points revealed a phenotypic hierarchy across animal studies consistent with the human TDS hypothesis. We confirmed the known role of estrogen and androgen signaling pathways in rodent TDS, and importantly, broadened the list of molecular targets to include retinoic acid signaling, vascular remodeling proteins, G-protein coupled receptors (GPCRs), and cytochrome P450s. C1 [Leung, Maxwell C. K.; Sipes, Nisha S.; McLaurin, Keith W.] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Leung, Maxwell C. K.; Phuong, Jimmy; Sipes, Nisha S.; Martin, Matthew T.; McLaurin, Keith W.; Setzer, R. Woodrow; Judson, Richard S.; Knudsen, Thomas B.] US EPA, Natl Ctr Computat Toxicol, Res Triangle Pk, NC 27711 USA. [Baker, Nancy C.] Lockheed Martin, Res Triangle Pk, NC USA. [Klinefelter, Gary R.; Darney, Sally Perreault] US EPA, Natl Hlth & Environm Effects Res Lab, Res Triangle Pk, NC 27711 USA. [Darney, Sally Perreault] NIEHS, Environm Hlth Perspect, NIH, US Dept HHS, POB 12233, Res Triangle Pk, NC 27709 USA. RP Leung, MCK; Knudsen, TB (reprint author), US EPA, 109 TW Alexander Dr, Res Triangle Pk, NC 27711 USA. EM leung.max-well@epa.gov; knudsen.thomas@epa.gov OI Leung, Maxwell/0000-0003-1530-3306 NR 98 TC 2 Z9 2 U1 9 U2 13 PU US DEPT HEALTH HUMAN SCIENCES PUBLIC HEALTH SCIENCE PI RES TRIANGLE PK PA NATL INST HEALTH, NATL INST ENVIRONMENTAL HEALTH SCIENCES, PO BOX 12233, RES TRIANGLE PK, NC 27709-2233 USA SN 0091-6765 EI 1552-9924 J9 ENVIRON HEALTH PERSP JI Environ. Health Perspect. PD JUL PY 2016 VL 124 IS 7 BP 1050 EP 1061 DI 10.1289/ehp.1510385 PG 12 WC Environmental Sciences; Public, Environmental & Occupational Health; Toxicology SC Environmental Sciences & Ecology; Public, Environmental & Occupational Health; Toxicology GA DS4KF UT WOS:000380749300028 PM 26662846 ER PT J AU Nakamura, YK Metea, C Karstens, L Asquith, M Gruner, H Moscibrocki, C Lee, I Brislawn, CJ Jansson, JK Rosenbaum, JT Lin, P AF Nakamura, Yukiko K. Metea, Christina Karstens, Lisa Asquith, Mark Gruner, Henry Moscibrocki, Cathleen Lee, Iris Brislawn, Colin J. Jansson, Janet K. Rosenbaum, James T. Lin, Phoebe TI Gut Microbial Alterations Associated With Protection From Autoimmune Uveitis SO INVESTIGATIVE OPHTHALMOLOGY & VISUAL SCIENCE LA English DT Article DE microbiome; uveitis; antibiotics; regulatory T cells ID DISEASE; MODEL; MICE AB PURPOSE. To investigate the contribution of the gut microbiota to the pathogenesis of uveitis. METHODS. Experimental autoimmune uveitis (EAU) in B10.RIII mice was induced using interphotoreceptor binding protein peptide. Mice were treated with oral or intraperitoneal (IP) antibiotics. Effector (Teff) and regulatory (Treg) T lymphocytes were identified using flow cytometry; 16S rRNA gene sequencing and qPCR were performed on gastrointestinal (GI) contents. RESULTS. Broad-spectrum (four antibiotics given simultaneously) oral, but not IP, antibiotics reduced mean uveitis clinical scores significantly compared with water-treated animals (0.5 vs. 3.0, P < 0.0001 for oral; 3.4 vs. 3.4, P > 0.99 for IP). Both oral metronidazole (P = 0.02) and vancomycin (P < 0.0001) alone decreased inflammation, whereas neomycin (P = 0.7) and ampicillin (P = 0.4) did not change mean uveitis scores. Oral broad-spectrum antibiotics increased Tregs in the GI lamina propria of EAU animals at 1 week, and in extraintestinal lymphoid tissues later, whereas Teff and inflammatory cytokines were reduced. 16S sequencing of GI contents revealed altered microbiota in immunized mice compared with nonimmunized mice, and microbial diversity clustering in EAU mice treated with uveitis-protective antibiotics. Experimental autoimmune uveitis mice also demonstrated gut microbial diversity clustering associated with clinical score severity. CONCLUSIONS. Oral antibiotics modulate the severity of inducible EAU by increasing Tregs in the gut and extraintestinal tissues, as well as decreasing effector T cells and cytokines. 16S sequencing suggests that there may be protective and, conversely, potentially uveitogenic, gut microbiota. These findings may lead to a better understanding of how uveitis can be treated or prevented by modulating the gut microbiome. C1 [Nakamura, Yukiko K.; Metea, Christina; Gruner, Henry; Moscibrocki, Cathleen; Lee, Iris; Rosenbaum, James T.; Lin, Phoebe] Oregon Hlth & Sci Univ, Casey Eye Inst, 3375 SW Terwilliger Blvd, Portland, OR 97239 USA. [Karstens, Lisa] Oregon Hlth & Sci Univ, Dept Med Informat & Clin Epidemiol, Portland, OR 97201 USA. [Asquith, Mark; Rosenbaum, James T.] Oregon Hlth & Sci Univ, Dept Med, Div Rheumatol, Portland, OR 97201 USA. [Brislawn, Colin J.; Jansson, Janet K.] Pacific Northwest Natl Lab, Richland, WA USA. [Rosenbaum, James T.] Devers Eye Inst, Portland, OR USA. RP Lin, P (reprint author), Oregon Hlth & Sci Univ, Casey Eye Inst, 3375 SW Terwilliger Blvd, Portland, OR 97239 USA. EM linp@ohsu.edu OI Brislawn, Colin/0000-0002-9109-1950; Karstens, Lisa/0000-0001-6188-4397 FU NEI NIH HHS [P30 EY010572, K08 EY022948]; NICHD NIH HHS [K12 HD043488] NR 28 TC 2 Z9 2 U1 2 U2 2 PU ASSOC RESEARCH VISION OPHTHALMOLOGY INC PI ROCKVILLE PA 12300 TWINBROOK PARKWAY, ROCKVILLE, MD 20852-1606 USA SN 0146-0404 EI 1552-5783 J9 INVEST OPHTH VIS SCI JI Invest. Ophthalmol. Vis. Sci. PD JUL PY 2016 VL 57 IS 8 BP 3747 EP 3758 DI 10.1167/iovs.16-19733 PG 12 WC Ophthalmology SC Ophthalmology GA DT8GW UT WOS:000381729000024 PM 27415793 ER PT J AU Montgomery, BL AF Montgomery, Beronda L. TI Mechanisms and fitness implications of photomorphogenesis during chromatic acclimation in cyanobacteria SO JOURNAL OF EXPERIMENTAL BOTANY LA English DT Review DE Chromatic acclimation; cyanobacteria; cyanobacteriochromes; light sensing; photomorphogenesis; photosensing ID FAR-RED LIGHT; SP PCC 6803; FREMYELLA-DIPLOSIPHON CELLS; CELLULAR MORPHOLOGY; RED/GREEN CYANOBACTERIOCHROMES; THERMOSYNECHOCOCCUS-ELONGATUS; REVERSIBLE PHOTOCONVERSION; MARINE SYNECHOCOCCUS; ACARYOCHLORIS-MARINA; RESPONSE REGULATOR AB Cyanobacteria are oxygenic photosynthetic prokaryotes possessing diverse photoreceptors that initiate light-dependent signaling cascades that allow the organisms to optimize fitness by tuning their metabolism, growth and development to dynamic photoenvironments.Photosynthetic organisms absorb photons and convert light energy to chemical energy through the process of photosynthesis. Photosynthetic efficiency is tuned in response to the availability of light, carbon dioxide and nutrients to promote maximal levels of carbon fixation, while simultaneously limiting the potential for light-associated damage or phototoxicity. Given the central dependence on light for energy production, photosynthetic organisms possess abilities to tune their growth, development and metabolism to external light cues in the process of photomorphogenesis. Photosynthetic organisms perceive light intensity and distinct wavelengths or colors of light to promote organismal acclimation. Cyanobacteria are oxygenic photosynthetic prokaryotes that exhibit abilities to alter specific aspects of growth, including photosynthetic pigment composition and morphology, in responses to changes in available wavelengths and intensity of light. This form of photomorphogenesis is known as chromatic acclimation and has been widely studied. Recent insights into the photosensory photoreceptors found in cyanobacteria and developments in our understanding of the molecular mechanisms initiated by light sensing to affect the changes characteristic of chromatic acclimation are discussed. I consider cyanobacterial responses to light, the broad diversity of photoreceptors encoded by these organisms, specific mechanisms of photomorphogenesis, and associated fitness implications in chromatically acclimating cyanobacteria. C1 [Montgomery, Beronda L.] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. [Montgomery, Beronda L.] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. RP Montgomery, BL (reprint author), Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA.; Montgomery, BL (reprint author), Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. EM montg133@msu.edu NR 134 TC 2 Z9 2 U1 9 U2 12 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0022-0957 EI 1460-2431 J9 J EXP BOT JI J. Exp. Bot. PD JUL PY 2016 VL 67 IS 14 BP 4079 EP 4090 DI 10.1093/jxb/erw206 PG 12 WC Plant Sciences SC Plant Sciences GA DU2SE UT WOS:000382060300007 PM 27217547 ER PT J AU Chelliah, K Raman, GG Muehleisen, RT AF Chelliah, Kanthasamy Raman, Ganesh G. Muehleisen, Ralph T. TI Enhanced nearfield acoustic holography for larger distances of reconstructions using fixed parameter Tikhonov regularization SO JOURNAL OF THE ACOUSTICAL SOCIETY OF AMERICA LA English DT Article ID FIELD; SUPERPOSITION AB This paper evaluates the performance of various regularization parameter choice methods applied to different approaches of nearfield acoustic holography when a very nearfield measurement is not possible. For a fixed grid resolution, the larger the hologram distance, the larger the error in the naive nearfield acoustic holography reconstructions. These errors can be smoothed out by using an appropriate order of regularization. This study shows that by using a fixed/manual choice of regularization parameter, instead of automated parameter choice methods, reasonably accurate reconstructions can be obtained even when the hologram distance is 16 times larger than the grid resolution. (C) 2016 Acoustical Society of America. C1 [Chelliah, Kanthasamy; Raman, Ganesh G.] IIT, Dept Mech Aerosp & Mat Engn, Chicago, IL 60616 USA. [Muehleisen, Ralph T.] Argonne Natl Lab, Div Energy Syst, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Chelliah, K (reprint author), IIT, Dept Mech Aerosp & Mat Engn, Chicago, IL 60616 USA. EM kchellia@iit.edu FU U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Office of Building Technology [DE-AC02-06CH11357] FX This work was supported by the U.S. Department of Energy, Office of Energy Efficiency and Renewable Energy, Office of Building Technology under Contract No. DE-AC02-06CH11357. NR 14 TC 0 Z9 0 U1 1 U2 1 PU ACOUSTICAL SOC AMER AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0001-4966 EI 1520-8524 J9 J ACOUST SOC AM JI J. Acoust. Soc. Am. PD JUL PY 2016 VL 140 IS 1 BP 114 EP 120 DI 10.1121/1.4954757 PG 7 WC Acoustics; Audiology & Speech-Language Pathology SC Acoustics; Audiology & Speech-Language Pathology GA DU7PG UT WOS:000382406500035 PM 27475137 ER PT J AU Park, J Stump, BW Hayward, C Arrowsmith, SJ Che, IY Drob, DP AF Park, Junghyun Stump, Brian W. Hayward, Chris Arrowsmith, Stephen J. Che, Il-Young Drob, Douglas P. TI Detection of regional infrasound signals using array data: Testing, tuning, and physical interpretation SO JOURNAL OF THE ACOUSTICAL SOCIETY OF AMERICA LA English DT Article ID OCEAN WAVES; PROPAGATION; LOCATION; NOISE; MICROBAROMS; EXPLOSIONS; MORPHOLOGY; NETWORK; EVENTS; SYSTEM AB This work quantifies the physical characteristics of infrasound signal and noise, assesses their temporal variations, and determines the degree to which these effects can be predicted by time-varying atmospheric models to estimate array and network performance. An automated detector that accounts for both correlated and uncorrelated noise is applied to infrasound data from three seismo-acoustic arrays in South Korea (BRDAR, CHNAR, and KSGAR), cooperatively operated by Korea Institute of Geoscience and Mineral Resources (KIGAM) and Southern Methodist University (SMU). Arrays located on an island and near the coast have higher noise power, consistent with both higher wind speeds and seasonably variable ocean wave contributions. On the basis of the adaptive F-detector quantification of time variable environmental effects, the time-dependent scaling variable is shown to be dependent on both weather conditions and local site effects. Significant seasonal variations in infrasound detections including daily time of occurrence, detection numbers, and phase velocity/azimuth estimates are documented. These time-dependent effects are strongly correlated with atmospheric winds and temperatures and are predicted by available atmospheric specifications. This suggests that commonly available atmospheric specifications can be used to predict both station and network detection performance, and an appropriate forward model improves location capabilities as a function of time. (C) 2016 Acoustical Society of America. C1 [Park, Junghyun; Stump, Brian W.; Hayward, Chris] Southern Methodist Univ, Roy M Huffington Dept Earth Sci, POB 750395, Dallas, TX 75275 USA. [Arrowsmith, Stephen J.] Sandia Natl Labs, 1515 Eubank SE,Mail Stop 0404, Albuquerque, NM 87123 USA. [Che, Il-Young] Korea Inst Geosci & Mineral Resources, 124 Gwahak Ro, Deajeon 34132, South Korea. [Drob, Douglas P.] Naval Res Lab, Div Space Sci, Washington, DC 20375 USA. RP Park, J (reprint author), Southern Methodist Univ, Roy M Huffington Dept Earth Sci, POB 750395, Dallas, TX 75275 USA. EM junghyunp@smu.edu FU Air Force Research Laboratory; National Nuclear Security Administration [FA8718-08-C-0008]; Chief of Naval Research through Naval Research Laboratory base program FX This work was funded by the Air Force Research Laboratory and the National Nuclear Security Administration, under Award No. FA8718-08-C-0008. D.P.D. acknowledges support from the Chief of Naval Research through the Naval Research Laboratory base program. The MERRA/GEOS-5 data utilized in the G2S atmospheric specifications were provided by the Global Modeling and Assimilation Office at NASA Goddard Space Flight Center through the online data portal in the NASA Center for Climate Simulation. The NOAA GFS analysis fields, also utilized in the G2S specifications, were obtained from NOAA's National Operational Model Archive and Distribution System, which is maintained at NOAA's National Climatic Data Center. NR 60 TC 0 Z9 0 U1 6 U2 6 PU ACOUSTICAL SOC AMER AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0001-4966 EI 1520-8524 J9 J ACOUST SOC AM JI J. Acoust. Soc. Am. PD JUL PY 2016 VL 140 IS 1 BP 239 EP 259 DI 10.1121/1.4954759 PG 21 WC Acoustics; Audiology & Speech-Language Pathology SC Acoustics; Audiology & Speech-Language Pathology GA DU7PG UT WOS:000382406500048 ER PT J AU Gueguen, P Johnson, P Roux, P AF Gueguen, Philippe Johnson, Paul Roux, Philippe TI Nonlinear dynamics induced in a structure by seismic and environmental loading SO JOURNAL OF THE ACOUSTICAL SOCIETY OF AMERICA LA English DT Article ID STRONG GROUND MOTION; RANDOM DECREMENT TECHNIQUE; SAN-ANDREAS FAULT; TEMPORAL-CHANGES; EARTHQUAKE; FREQUENCY; CONCRETE; IDENTIFICATION; DECONVOLUTION; PERTURBATION AB In this study, it is shown that under very weak dynamic and quasi-static deformation that is orders of magnitude below the yield deformation of the equivalent stress-strain curve (around 10(-3)), the elastic parameters of a civil engineering structure (resonance frequency and damping) exhibit nonlinear softening and recovery. These observations bridge the gap between laboratory and seismic scales where elastic nonlinear behavior has been previously observed. Under weak seismic or atmospheric loading, modal frequencies are modified by around 1% and damping by more than 100% for strain levels between 10(-7) and 10(-4). These observations support the concept of universal behavior of nonlinear elastic behavior in diverse systems, including granular materials and damaged solids that scale from millimeter dimensions to the scale of structures to fault dimensions in the Earth. (C) 2016 Acoustical Society of America. C1 [Gueguen, Philippe; Roux, Philippe] Univ Grenoble Alpes, ISTerre, CNRS IFSTTAR, BP 53, F-38041 Grenoble 9, France. [Johnson, Paul] Los Alamos Natl Lab, Geophys Grp, Los Alamos, NM 87545 USA. RP Gueguen, P (reprint author), Univ Grenoble Alpes, ISTerre, CNRS IFSTTAR, BP 53, F-38041 Grenoble 9, France. EM philippe.gueguen@ujf-grenoble.fr RI Gueguen, Philippe/A-3852-2012; roux, philippe/B-8538-2014 FU U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division; European Research Council [227507] FX All of the data used in this study came from the UCLA Factor building array downloaded from the IRIS (http://www.iris.edu) datacenter, mseed code FABI.FE.HNN and FABA.XE.HNN. P.G. acknowledges LabEx OSUG@2020 (Investissements d'avenir - ANR10LABX56). P.J. acknowledges support by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, Chemical Sciences, Geosciences, and Biosciences Division. P.R. acknowledges the European Research Council through the advanced grant "Whisper" 227507. NR 50 TC 0 Z9 0 U1 6 U2 7 PU ACOUSTICAL SOC AMER AMER INST PHYSICS PI MELVILLE PA STE 1 NO 1, 2 HUNTINGTON QUADRANGLE, MELVILLE, NY 11747-4502 USA SN 0001-4966 EI 1520-8524 J9 J ACOUST SOC AM JI J. Acoust. Soc. Am. PD JUL PY 2016 VL 140 IS 1 BP 582 EP 590 DI 10.1121/1.4958990 PG 9 WC Acoustics; Audiology & Speech-Language Pathology SC Acoustics; Audiology & Speech-Language Pathology GA DU7PG UT WOS:000382406500077 PM 27475180 ER PT J AU Hamilton, MT Kupar, CA Kelley, MD Finger, JW Tuberville, TD AF Hamilton, Matthew T. Kupar, Caitlin A. Kelley, Meghan D. Finger, John W., Jr. Tuberville, Tracey D. TI Blood and Plasma Biochemistry Reference Intervals for Wild Juvenile American Alligators (Alligator mississippiensis) SO JOURNAL OF WILDLIFE DISEASES LA English DT Article DE Alligator mississippiensis; American alligator; point-of-care; reference intervals; stress ID CROCODYLUS-POROSUS; RESTRAINT; POND AB American alligators (Alligator mississippiensis) are one of the most studied crocodilian species in the world, yet blood and plasma biochemistry information is limited for juvenile alligators in their northern range, where individuals may be exposed to extreme abiotic and biotic stressors. We collected blood samples over a 2-yr period from 37 juvenile alligators in May, June, and July to establish reference intervals for 22 blood and plasma analytes. We observed no effect of either sex or blood collection time on any analyte investigated. However, our results indicate a significant correlation between a calculated body condition index and aspartate aminotransferase and creatine kinase. Glucose, total protein, and potassium varied significantly between sampling sessions. In addition, glucose and potassium were highly correlated between the two point-of-care devices used, although they were significantly lower with the i-STAT 1 CG8+ cartridge than with the Vetscan VS2 Avian/Reptile Rotor. The reference intervals presented herein should provide baseline data for evaluating wild juvenile alligators in the northern portion of their range. C1 [Hamilton, Matthew T.; Kupar, Caitlin A.; Finger, John W., Jr.; Tuberville, Tracey D.] Univ Georgia, Savannah River Ecol Lab, PO Drawer E, Aiken, SC 29802 USA. [Hamilton, Matthew T.; Kupar, Caitlin A.] Univ Georgia, Warnell Sch Forestry & Nat Resources, 180 E Green St, Athens, GA 30602 USA. [Kelley, Meghan D.; Finger, John W., Jr.] Auburn Univ, Dept Biol Sci, 101 Rouse Life Sci, Auburn, AL 36849 USA. RP Hamilton, MT (reprint author), Univ Georgia, Savannah River Ecol Lab, PO Drawer E, Aiken, SC 29802 USA.; Hamilton, MT (reprint author), Univ Georgia, Warnell Sch Forestry & Nat Resources, 180 E Green St, Athens, GA 30602 USA. EM hamiltmatt@gmail.com OI Finger, John/0000-0003-0661-7821 FU Department of Energy [DE-FC09-07SR22506]; Savannah River Nuclear Solutions-Area Closures Project FX We thank Dan Quinn, Megan Winzeler, Nick Bossenbroek, David Haskins, and Erin Abernathy for assisting with alligator sampling and processing. We extend a special thanks to Jessica Hoover from Abaxis for donating 25-CG8+ cartridges for this research. This work was supported by the Department of Energy under Award DE-FC09-07SR22506 to the University of Georgia Research Foundation, and by the Savannah River Nuclear Solutions-Area Closures Project. All procedures were approved by the University of Georgia's Institutional Animal Care and Use Committee (Animal Use Protocol A2013 12-008-Y2-A0). Animals used in this study were collected under permits 04-2014 and 05-2015 issued by South Carolina Department of Natural Resources. NR 20 TC 1 Z9 1 U1 6 U2 6 PU WILDLIFE DISEASE ASSOC, INC PI LAWRENCE PA 810 EAST 10TH ST, LAWRENCE, KS 66044-8897 USA SN 0090-3558 EI 1943-3700 J9 J WILDLIFE DIS JI J. Wildl. Dis. PD JUL PY 2016 VL 52 IS 3 BP 631 EP 635 DI 10.7589/2015-10-275 PG 5 WC Veterinary Sciences SC Veterinary Sciences GA DT5NA UT WOS:000381528700023 PM 27224213 ER PT J AU Evans, JE Friedrich, H Bals, S Bradley, RS Dahmen, T De Backer, A de Jonge, N Elbaum, M Goris, B Houben, L Leary, RK Midgley, PA Slusallek, P Trampert, P Van Aert, S Van Tendeloo, G Withers, PJ Wolf, SG AF Evans, James E. Friedrich, Heiner Bals, Sara Bradley, Robert S. Dahmen, Tim De Backer, Annick de Jonge, Niels Elbaum, Michael Goris, Bart Houben, Lothar Leary, Rowan K. Midgley, Paul A. Slusallek, Philipp Trampert, Patrick Van Aert, Sandra Van Tendeloo, Gustaaf Withers, Philip J. Wolf, Sharon G. TI Advanced tomography techniques for inorganic, organic, and biological materials SO MRS BULLETIN LA English DT Article ID FOCUSED ION-BEAM; CORRELATIVE CRYO-LIGHT; ATOM-PROBE TOMOGRAPHY; X-RAY TOMOGRAPHY; ELECTRON TOMOGRAPHY; CRYOELECTRON TOMOGRAPHY; 3-DIMENSIONAL STRUCTURE; HETEROGENEOUS CATALYSTS; MICROSCOPY; RESOLUTION AB Three-dimensional (3D) tomography using electrons and x-rays has pushed and expanded our understanding of the micro-and nanoscale spatial organization of inorganic, organic, and biological materials. While a significant impact on the field of materials science has already been realized from tomography applications, new advanced methods are quickly expanding the versatility of this approach to better link structure, composition, and function of complex 3D assemblies across multiple scales. In this article, we highlight several frontiers where new developments in tomography are empowering new science across biology, chemistry, and physics. The five articles that appear in this issue of MRS Bulletin describe some of these latest developments in detail, including analytical electron tomography, atomic resolution electron tomography, advanced recording schemes in scanning transmission electron microscopy (STEM) tomography, cryo-STEM tomography of whole cells, and multiscale correlative tomography. C1 [Evans, James E.] Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA. [Evans, James E.] Pacific Northwest Natl Lab, Richland, WA 99354 USA. [Friedrich, Heiner] Eindhoven Univ Technol, Dept Chem Engn & Chem, Eindhoven, Netherlands. [Friedrich, Heiner] Eindhoven Univ Technol, Lab Mat & Interface Chem, Eindhoven, Netherlands. Eindhoven Univ Technol, Ctr Multiscale Electron Microscopy, Eindhoven, Netherlands. [Bals, Sara; De Backer, Annick; Goris, Bart; Van Aert, Sandra; Van Tendeloo, Gustaaf] Univ Antwerp, Electron Microscopy Materials Res Lab, Campus Groenenborger, Antwerp, Belgium. [Bals, Sara; De Backer, Annick; Goris, Bart; Van Aert, Sandra] Univ Antwerp, Electron Microscopy Materials Res Grp, Antwerp, Belgium. [Bals, Sara] Lawrence Berkeley Natl Lab, Natl Ctr Electron Microscopy, Berkeley, CA 94720 USA. [Bradley, Robert S.] Univ Manchester, Manchester, Lancs, England. [Bradley, Robert S.] Henry Moseley X Ray Imaging Facil HMXIF, Manchester, Lancs, England. [Dahmen, Tim; Slusallek, Philipp; Trampert, Patrick] German Res Ctr Artificial Intelligence, Saarbrucken, Germany. [de Jonge, Niels] Leibniz Inst New Materials, Saarbrucken, Germany. [de Jonge, Niels] Univ Saarland, Expt Phys, Saarbrucken, Germany. [de Jonge, Niels] Philips Res, Eindhoven, Netherlands. [Elbaum, Michael] Weizmann Inst Sci, Dept Materials & Interfaces, Rehovot, Israel. [Houben, Lothar; Wolf, Sharon G.] Weizmann Inst Sci, Dept Chem Res Support, Rehovot, Israel. [Houben, Lothar] Forschungszentrum Julich GmbH, Julich, Germany. [Leary, Rowan K.; Midgley, Paul A.] Univ Cambridge, Dept Materials Sci & Met, Cambridge, England. [Leary, Rowan K.] Univ Cambridge, Clare Coll, Cambridge, England. [Midgley, Paul A.] Univ Cambridge, Mat Sci, Cambridge, England. [Midgley, Paul A.] Univ Cambridge, Dept Materials Sci & Met, Wolfson Electron Microscopy Suite, Cambridge, England. [Slusallek, Philipp] Univ Saarland, Saarbrucken, Germany. [Slusallek, Philipp] Univ Saarland, Comp Graph, Saarbrucken, Germany. [Van Tendeloo, Gustaaf] Wuhan Univ China, Wuhan, Hubei, Peoples R China. [Withers, Philip J.] Univ Manchester, Sch Mat, Mat, Manchester, Lancs, England. [Wolf, Sharon G.] Weizmann Inst Sci, Electron Microscopy Unit, Rehovot, Israel. RP Evans, JE (reprint author), Pacific Northwest Natl Lab, Environm Mol Sci Lab, Richland, WA 99354 USA.; Evans, JE (reprint author), Pacific Northwest Natl Lab, Richland, WA 99354 USA. EM james.evans@pnnl.gov; h.friedrich@tue.nl; sara.bals@uantwerpen.be; rob.bradley@geotek.co.uk; tim.dahmen@dfki.de; annick.debacker@uantwerpen.be; niels.dejonge@leibniz-inm.de; michael.elbaum@weizmann.ac.il; bart.goris@uantwerpen.be; lothar.houben@weizmann.ac.il; rkl26@cam.ac.uk; pam33@cam.ac.uk; slusallek@dfki.de; patrick.trampert@dfki.de; sandra.vanaert@uantwerpen.be; staf.vantendeloo@uantwerpen.be; p.j.withers@manchester.ac.uk; sharon.wolf@weizmann.ac.il RI de Jonge, Niels/B-5677-2008; Van Aert, Sandra/B-7913-2017 OI Van Aert, Sandra/0000-0001-9603-8764 FU Department of Energy's Office of Biological and Environmental Research Mesoscale to Molecules Project [66382] FX J.E.E. acknowledges support from the Department of Energy's Office of Biological and Environmental Research Mesoscale to Molecules Project #66382. NR 59 TC 0 Z9 0 U1 8 U2 13 PU CAMBRIDGE UNIV PRESS PI NEW YORK PA 32 AVENUE OF THE AMERICAS, NEW YORK, NY 10013-2473 USA SN 0883-7694 EI 1938-1425 J9 MRS BULL JI MRS Bull. PD JUL PY 2016 VL 41 IS 7 BP 516 EP 524 DI 10.1557/mrs.2016.134 PG 9 WC Materials Science, Multidisciplinary; Physics, Applied SC Materials Science; Physics GA DU9AH UT WOS:000382508100011 ER PT J AU Morgan, BE Greenough, JA AF Morgan, B. E. Greenough, J. A. TI Large-eddy and unsteady RANS simulations of a shock-accelerated heavy gas cylinder SO SHOCK WAVES LA English DT Article DE Richtmyer-Meshkov instability; Turbulent mixing; Large-eddy simulation ID RICHTMYER-MESHKOV INSTABILITY; RAYLEIGH-TAYLOR INSTABILITY; ATWOOD NUMBERS; TURBULENCE; FLOW; REFINEMENT; RESOLUTION AB Two-dimensional numerical simulations of the Richtmyer-Meshkov unstable "shock-jet" problem are conducted using both large-eddy simulation (LES) and unsteady Reynolds-averaged Navier-Stokes (URANS) approaches in an arbitrary Lagrangian-Eulerian hydrodynamics code. Turbulence statistics are extracted from LES by running an ensemble of simulations with multimode perturbations to the initial conditions. Detailed grid convergence studies are conducted, and LES results are found to agree well with both experiment and high-order simulations conducted by Shankar et al. (Phys Fluids 23, 024102, 2011). URANS results using a k-L approach are found to be highly sensitive to initialization of the turbulence lengthscale L and to the time at which L becomes resolved on the computational mesh. It is observed that a gradient diffusion closure for turbulent species flux is a poor approximation at early times, and a new closure based on the mass-flux velocity is proposed for low-Reynolds-number mixing. C1 [Morgan, B. E.; Greenough, J. A.] Lawrence Livermore Natl Lab, 7000 East Ave,L-170, Livermore, CA 94550 USA. RP Morgan, BE (reprint author), Lawrence Livermore Natl Lab, 7000 East Ave,L-170, Livermore, CA 94550 USA. EM morgan65@llnl.gov; greenough1@llnl.gov FU US Department of Energy by Lawrence Livermore National Laboratory [DE-AC52-07NA27344] FX This work was performed under the auspices of the US Department of Energy by Lawrence Livermore National Laboratory under Contract No. DE-AC52-07NA27344. NR 52 TC 0 Z9 0 U1 6 U2 6 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0938-1287 EI 1432-2153 J9 SHOCK WAVES JI Shock Waves PD JUL PY 2016 VL 26 IS 4 BP 355 EP 383 DI 10.1007/s00193-015-0566-3 PG 29 WC Mechanics SC Mechanics GA DU7NM UT WOS:000382401300002 ER PT J AU Campbell, MF Haylett, DR Davidson, DF Hanson, RK AF Campbell, M. F. Haylett, D. R. Davidson, D. F. Hanson, R. K. TI AEROFROSH: a shock condition calculator for multi-component fuel aerosol-laden flows SO SHOCK WAVES LA English DT Article DE Shock tube; Aerosol; Evaporation; Diesel fuel ID IGNITION DELAY TIMES; VAPOR-DROPLET FLOWS; RELAXATION ZONE; WATER DROPLETS; COMPRESSIBLE FLOWS; PHASE-TRANSITION; DIESEL IGNITION; PRESSURE FUELS; METHYL OLEATE; DUSTY GASES AB This article introduces an algorithm that determines the thermodynamic conditions behind incident and reflected shocks in aerosol-laden flows. Importantly, the algorithm accounts for the effects of droplet evaporation on post-shock properties. Additionally, this article describes an algorithm for resolving the effects of multiple-component-fuel droplets. This article presents the solution methodology and compares the results to those of another similar shock calculator. It also provides examples to show the impact of droplets on post-shock properties and the impact that multi-component fuel droplets have on shock experimental parameters. Finally, this paper presents a detailed uncertainty analysis of this algorithm's calculations given typical experimental uncertainties. C1 [Campbell, M. F.] Sandia Natl Labs, Livermore, CA 94551 USA. [Haylett, D. R.] Lawrence Livermore Natl Lab, Livermore, CA 94551 USA. [Davidson, D. F.; Hanson, R. K.] Stanford Univ, Stanford, CA 94305 USA. RP Campbell, MF (reprint author), Sandia Natl Labs, Livermore, CA 94551 USA. EM mfcampb@sandia.gov FU Army Research Office; Division of Chemical Sciences, Geosciences, and Biosciences; Office of Basic Energy Sciences (BES); U.S. Department of Energy (DOE); National Defense Science and Engineering Graduate (NDSEG) Fellowship [32 CFR 168a]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work was supported by the Army Research Office with Dr. Ralph Anthenien as contract monitor. M.F.C. is supported by the Division of Chemical Sciences, Geosciences, and Biosciences, the Office of Basic Energy Sciences (BES), the U.S. Department of Energy (DOE). Also, during a portion of this work, M.F.C. was supported by a National Defense Science and Engineering Graduate (NDSEG) Fellowship, 32 CFR 168a. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 85 TC 0 Z9 0 U1 5 U2 5 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0938-1287 EI 1432-2153 J9 SHOCK WAVES JI Shock Waves PD JUL PY 2016 VL 26 IS 4 BP 429 EP 447 DI 10.1007/s00193-015-0582-3 PG 19 WC Mechanics SC Mechanics GA DU7NM UT WOS:000382401300007 ER PT J AU Velmurugan, J Mollison, E Barth, S Marshall, D Milne, L Creevey, CJ Lynch, B Meally, H McCabe, M Milbourne, D AF Velmurugan, Janaki Mollison, Ewan Barth, Susanne Marshall, David Milne, Linda Creevey, Christopher J. Lynch, Bridget Meally, Helena McCabe, Matthew Milbourne, Dan TI An ultra-high density genetic linkage map of perennial ryegrass (Lolium perenne) using genotyping by sequencing (GBS) based on a reference shotgun genome assembly SO ANNALS OF BOTANY LA English DT Article DE Lolium perenne; perennial ryegrass; genome assembly; genotyping by sequencing; GBS; single nucleotide polymorphism; linkage mapping; presence/absence variation ID GENERATION; RECOMBINATION; DISCOVERY; IDENTIFICATION; CONSTRUCTION; DIVERSITY; ALIGNMENT; MARKERS; BARLEY; TOOL AB Background and Aims High density genetic linkage maps that are extensively anchored to assembled genome sequences of the organism in question are extremely useful in gene discovery. To facilitate this process in perennial ryegrass ( Lolium perenne L.), a high density single nucleotide polymorphism ( SNP)- and presence/ absence variant ( PAV)- based genetic linkage map has been developed in an F2 mapping population that has been used as a reference population in numerous studies. To provide a reference sequence to which to align genotyping by sequencing ( GBS) reads, a shotgun assembly of one of the grandparents of the population, a tenth- generation inbred line, was created using Illumina- based sequencing. Methods The assembly was based on paired-end Illumina reads, scaffolded by mate pair and long jumping distance reads in the range of 3-40 kb, with > 200-fold initial genome coverage. A total of 169 individuals from an F-2 mapping population were used to construct PstI-based GBS libraries tagged with unique 4-9 nucleotide barcodes, resulting in 284 million reads, with approx. 1 center dot 6 million reads per individual. A bioinformatics pipeline was employed to identify both SNPs and PAVs. A core genetic map was generated using high confidence SNPs, to which lower confidence SNPs and PAVs were subsequently fitted in a straightforward binning approach. Key Results The assembly comprises 424 750 scaffolds, covering 1 center dot 11 Gbp of the 2 center dot 5 Gbp perennial ryegrass genome, with a scaffold N50 of 25 212 bp and a contig N50 of 3790 bp. It is available for download, and access to a genome browser has been provided. Comparison of the assembly with available transcript and gene model data sets for perennial ryegrass indicates that approx. 570 Mbp of the gene-rich portion of the genome has been captured. An ultra-high density genetic linkage map with 3092 SNPs and 7260 PAVs was developed, anchoring just over 200 Mb of the reference assembly. Conclusions The combined genetic map and assembly, combined with another recently released genome assembly, represent a significant resource for the perennial ryegrass genetics community. C1 [Velmurugan, Janaki; Mollison, Ewan; Barth, Susanne; Meally, Helena; Milbourne, Dan] TEAGASC, Crops Environm & Land Use Programme, Oak Pk Res Ctr, Carlow, Ireland. [Velmurugan, Janaki; Lynch, Bridget] Univ Coll Dublin, Sch Agr & Food Sci, Dublin, Ireland. [Mollison, Ewan; Marshall, David; Milne, Linda] James Hutton Inst, Informat & Computat Sci Grp, Errol Rd, Dundee, Scotland. [Mollison, Ewan] Univ Dundee, James Hutton Inst, Div Plant Sci, Errol Rd, Dundee, Scotland. [Creevey, Christopher J.; McCabe, Matthew] TEAGASC, Anim & Grassland Res & Innovat Ctr, Grange, Ireland. [Creevey, Christopher J.] Aberystwyth Univ, Inst Biol Environm & Rural Sci, Aberystwyth SY23 3FG, Dyfed, Wales. RP Milbourne, D (reprint author), TEAGASC, Crops Environm & Land Use Programme, Oak Pk Res Ctr, Carlow, Ireland. EM dan.milbourne@teagasc.ie FU Teagasc FX The authors wish to acknowledge Trinity College Dublin (Elaine Kenny), University College Dublin (Alison Murphy) and the Oslo Sequencing Centre (Lex Nederbragt and Gregor Gilfillan) for their technical expertise in the sequencing for the assembly described herein. We also thank Dr Tom Ruttink, ILVO, Belgium for access to Lolium perenne OGA assembled transcript data, and Dr Stephen Byrne for useful discussions that contributed to the revised draft of the manuscript. This study was funded by Teagasc core funding and Teagasc PhD Walsh Fellowships to J.V. and E.M. NR 50 TC 0 Z9 0 U1 17 U2 19 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0305-7364 EI 1095-8290 J9 ANN BOT-LONDON JI Ann. Bot. PD JUL PY 2016 VL 118 IS 1 BP 71 EP 87 DI 10.1093/aob/mcw081 PG 17 WC Plant Sciences SC Plant Sciences GA DT1GD UT WOS:000381228800006 PM 27268483 ER PT J AU Yung, MM Starace, AK Mukarakate, C Crow, AM Leshnov, MA Magrini, KA AF Yung, Matthew M. Starace, Anne K. Mukarakate, Calvin Crow, Allison M. Leshnov, Marissa A. Magrini, Kimberly A. TI Biomass Catalytic Pyrolysis on Ni/ZSM-5: Effects of Nickel Pretreatment and Loading SO ENERGY & FUELS LA English DT Article; Proceedings Paper CT 65th Canadian Chemical Engineering Conference CY OCT 04-07, 2015 CL Calgary, CANADA SP Canadian Soc Chem Engn, Principal Tech Org Profess Chem Engineers, Chem Inst Canada ID HZSM-5 ZEOLITE CATALYST; FLUIDIZED-BED REACTOR; BIO-OIL; MOLECULAR CHARACTERIZATION; TRANSPORTATION FUELS; VAPORS; HYDROCARBONS; LIQUIDS; GC/MS; WOOD AB In this work, Ni/ZSM-5 catalysts with varied nickel loadings were evaluated for their ability to produce aromatic hydrocarbons by upgrading of pine pyrolysis vapors. The effect of catalyst pretreatment by hydrogen reduction was also investigated. Results indicate that the addition of nickel increases the yield of aromatic hydrocarbons while simultaneously increasing the conversion of oxygenates, relative to ZSM-5, and these effects are more pronounced with increasing nickel loading. Additionally, while initial activity differences were observed between the oxidized and reduced forms of nickel on ZSM-5 (i.e., NiO/ZSM-5 versus Ni/ZSM-5), the activity of both catalysts converges with increasing time on stream. These reaction results coupled with characterization of pristine and spent catalysts suggest that the catalysts reach similar active states during catalytic pyrolysis, regardless of pretreatment, as NiO undergoes in situ reduction to Ni by biomass pyrolysis vapors. This reduction of NiO to Ni was confirmed by reaction results and characterization by NH3 temperature-programmed desorption, temperature programmed reduction, and X-ray diffraction. This finding is significant in that the ability to reduce or eliminate the need for a pre-reaction H-2 reduction of Ni-modified zeolite catalysts could reduce process complexity and operating costs in a biorefinery-based vapor-phase upgrading process to produce biomass-derived fuels and chemicals. The ability to monitor catalyst activity in real time with a molecular beam mass spectrometer used to measure uncondensed, hot pyrolysis vapors allows for an improved understanding of the mechanism for improved activity with Ni addition to ZSM-5, which is attributed to the ability to prevent deactivation by deposition of coke and capping of zeolite micropores. C1 [Yung, Matthew M.; Starace, Anne K.; Mukarakate, Calvin; Crow, Allison M.; Leshnov, Marissa A.; Magrini, Kimberly A.] Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. RP Yung, MM (reprint author), Natl Renewable Energy Lab, Natl Bioenergy Ctr, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM matthew.yung@nrel.gov NR 42 TC 0 Z9 0 U1 11 U2 11 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD JUL PY 2016 VL 30 IS 7 BP 5259 EP 5268 DI 10.1021/acs.energyfuels.6b00239 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DS2BO UT WOS:000380523200008 ER PT J AU Starace, AK Evans, RJ Lee, DD Carpenter, DL AF Starace, Anne K. Evans, Robert J. Lee, David D. Carpenter, Daniel L. TI Effects of Torrefaction Temperature on Pyrolysis Vapor Products of Woody and Herbaceous Feedstocks SO ENERGY & FUELS LA English DT Article ID MICROWAVE TORREFACTION; BIOMASS; TRANSFORMATION AB A variety of hardwood, softwood, and herbaceous feedstocks (oak, southern yellow pine mix, loblolly pine, pinyon-juniper mix, and switchgrass) were each torrefied at 200, 250, and 300 degrees C. Each of the feedstocks was pyrolyzed and the resulting vapors were analyzed with a molecular beam mass spectrometer (py-MBMS). Compositional analysis was used to measure the total lignin content of three of the feedstocks (southern yellow pine, softwood; oak, hardwood; and switchgrass, herbaceous) before and after torrefaction at 300 degrees C, and large differences in the fraction of lignin lost during torrefaction were found between feedstocks, with oak having the largest decrease in lignin during torrefaction and switchgrass having the least. It is hypothesized that these differences in the thermal degradation are due to, in part, the different ratios of S, G, and H lignins in the feedstocks. Additionally, the torrefaction of kraft lignin was studied using thermogravirnetric analysis coupled with Fourier transform infrared spectroscopy (TGA-FTIR) and attenuated total reflectance Fourier transform infrared spectroscopy (ATR-FTIR). C1 [Starace, Anne K.; Evans, Robert J.; Lee, David D.; Carpenter, Daniel L.] Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. RP Starace, AK (reprint author), Natl Renewable Energy Lab, 15013 Denver West Pkwy, Golden, CO 80401 USA. EM anne.starace@nrel.gov FU U.S. Department of Energy [DE-AC36-08GO28308]; National Renewable Energy Laboratory; U.S. DOE Office of Energy Efficiency and Renewable Energy Bioenergy Technologies Office FX This work was supported by the U.S. Department of Energy under Contract No. DE-AC36-08GO28308 with the National Renewable Energy Laboratory. Funding was provided by U.S. DOE Office of Energy Efficiency and Renewable Energy Bioenergy Technologies Office. The U.S. Government retains and the publisher, by accepting the article for publication, acknowledges that the U.S. Government retains a nonexclusive, paid up, irrevocable, worldwide license to publish or reproduce the published form of this work, or allow others to do so, for U.S. Government purposes. We would like to thank Justin Sluiter and Ryan Ness for performing the compositional analysis and Mike Griffin for performing additional ATR-FTIR. measurements. We also thank INL for providing the feedstocks. NR 29 TC 2 Z9 2 U1 4 U2 4 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD JUL PY 2016 VL 30 IS 7 BP 5677 EP 5683 DI 10.1021/acs.energyfuels.6b00267 PG 7 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DS2BO UT WOS:000380523200053 ER PT J AU Tolbert, AK Ma, T Kalluri, UC Ragauskas, AJ AF Tolbert, Allison K. Ma, Tao Kalluri, Udaya C. Ragauskas, Arthur J. TI Determining the Syringyl/Guaiacyl Lignin Ratio in the Vessel and Fiber Cell Walls of Transgenic Populus Plants SO ENERGY & FUELS LA English DT Article ID ION MASS-SPECTROMETRY; ULTRAVIOLET MICROSCOPY; TOF-SIMS; SYRINGYL; SUGAR; WOOD; NMR AB Observation of the spatial lignin distribution throughout the plant cell wall provides insight into the physicochemical characteristics of lignocellulosic biomass. The distribution of syringyl (S) and guaiacyl (G) lignin in cell walls of a genetically modified Populus deltoides and its corresponding empty vector control were analyzed with time-of-flight secondary ion mass spectrometry (ToF-SIMS) and then mapped to determine the S/G lignin ratio of the sample surface and specific regions of interest (ROIs). The surface characterizations of transgenic cross-sections within 1 cm vertical distance of each other on the stem possess similar S/G lignin ratios. The analysis of the ROIs determined that there was a 50% decrease in the S/G lignin ratio of the transgenic xylem fiber cell walls. C1 [Tolbert, Allison K.; Ma, Tao; Kalluri, Udaya C.; Ragauskas, Arthur J.] Georgia Inst Technol, Sch Chem & Biochem, Atlanta, GA 30332 USA. [Tolbert, Allison K.; Ma, Tao; Kalluri, Udaya C.; Ragauskas, Arthur J.] Oak Ridge Natl Lab, BioEnergy Sci Ctr BESC, Oak Ridge, TN 37830 USA. [Ragauskas, Arthur J.] Oak Ridge Natl Lab, Univ Tennessee UT Oak Ridge Natl Lab ORNL Joint I, Biosci Div, Oak Ridge, TN 37831 USA. RP Ragauskas, AJ (reprint author), Oak Ridge Natl Lab, POB 2008 MS6341, Oak Ridge, TN 37831 USA. EM aragausk@utk.edu OI KALLURI, UDAYA/0000-0002-5963-8370; Ragauskas, Arthur/0000-0002-3536-554X FU U.S. Department of Energy [DE-AC05-00OR22725]; Office of Biological and Environmental Research in the U.S. Department of Energy; Bioenergy Research Center; U.S. Department of Energy; Paper Science and Enegineering (PSE) fellowship program at the Renewable Bioproducts Institute at Georgia Institute of Technology FX This manuscript has been authored by University of Tennessee (UT)-Battelle, LLC under Contract DE-AC05-00OR22725 with the U.S. Department of Energy. The BioEnergy Science Center is supported by the Office of Biological and Environmental Research in the U.S. Department of Energy. Mass spectrometry analysis was carried out by the U.S. Department of Energy Office of Biological and Environmental Research supported by the Bioenergy Research Center proteomics pipeline. The publisher, by accepting the article for publication, acknowledges that the United States Government retains a non-exclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript or allow others to do so for United States Government purposes. The U.S. Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). Allison K. Tolbert is grateful for the financial support from the Paper Science and Enegineering (PSE) fellowship program at the Renewable Bioproducts Institute at Georgia Institute of Technology. NR 22 TC 1 Z9 1 U1 5 U2 7 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD JUL PY 2016 VL 30 IS 7 BP 5716 EP 5720 DI 10.1021/acs.energyfuels.6b00560 PG 5 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DS2BO UT WOS:000380523200057 ER PT J AU Koronaios, P Stevenson, C Warman, S Enick, R Luebke, D AF Koronaios, P. Stevenson, C. Warman, S. Enick, R. Luebke, D. TI Thermally Stable Silicone Solvents for the Selective Absorption of CO2 from Warm Gas Streams That Also Contain H-2 and H2O SO ENERGY & FUELS LA English DT Article ID CARBON-DIOXIDE; KINETIC ASPECTS; CROSS-LINKING; SOLUBILITY; HYDROGEN; POLYDIMETHYLSILOXANE; TEMPERATURES; DEGRADATION; METHYL; DIMETHYLPOLYSILOXANES AB Polydimethylsiloxane (PDMS) is a promising hydrophobic, CO2-selective solvent for the absorption of CO2 from a hot or warm water-rich, H-2-rich, postwater gas shift reactor (WGSR) stream in an integrated gasification combined cycle (IGCC) power plant. In this work, there are three hydrophobic silicones that are more thermally stable than PDMS, including an iron-stabilized PDMS (PDMS-Fe), poly(dimethyl-co-methylphenyl)siloxane (PDMMPS), and poly(dimethyl-co-diphenyl)siloxane (PDMDPS). PDMDPS is an extremely poor CO2 solvent, which is undesirable for the proposed separation, and a poor hydrogen solvent, which is a desirable trait. PDMDPS and PDMMPS absorb about the same amount of H-2. Although PDMMPS is a much better CO2 solvent than PDMDPS, PDMMPS is a slightly poorer CO2 solvent than PDMS or PDMS-Fe. PDMS-Fe and PDMS are comparable hydrophobic solvents that exhibit the greatest solvent strength for CO2 however, PDMS-Fe and PDMS absorb slightly more hydrogen than PDMDPS and PDMMPS. If the absorption/regeneration process is designed such that the solvent is exposed to temperatures no greater than 230 degrees C, PDMS is recommended due to its low cost. For higher temperatures, the extremely low solubility of CO2 in PDMDPS precludes its use as a CO2-selective solvent. The ferrosilicone additive in PDMS-Fe is designed to inhibit polymer degradation in an oxidizing environment, but it offers no additional stability in the oxygen-free closed system associated with the IGCC. PDMMPS absorbs less H-2 than PDMS or PDMS-Fe but is a slightly poorer CO2 solvent than PDMS or PDMS-Fe. However, PDMMPS is thermally stable in closed systems to 300 degrees C. Therefore, PDMMPS is recommended for prolonged high temperature use as the precombustion carbon capture absorber solvent at absorption/regeneration temperatures above 230 degrees C. Although these hydrophobic silicones exhibit promising attributes for a warm or hot precombustion carbon capture process, the diminishing CO2 solubility and increasing CO2 solubility that occur with increasing temperature will challenge the economic viability of this proposed CO2-selective absorption process. C1 [Koronaios, P.; Stevenson, C.; Warman, S.; Enick, R.] Univ Pittsburgh, Dept Chem & Petr Engn, 940 Benedum Hall,3700 OHara St, Pittsburgh, PA 15261 USA. [Enick, R.] Natl Energy Technol Lab, 626 Cochrans Mill Rd,POB 10940, Pittsburgh, PA 15236 USA. [Luebke, D.] LumiShield Technol, 1816 Pkwy View Dr, Pittsburgh, PA 15205 USA. RP Enick, R (reprint author), Univ Pittsburgh, Dept Chem & Petr Engn, 940 Benedum Hall,3700 OHara St, Pittsburgh, PA 15261 USA.; Enick, R (reprint author), Natl Energy Technol Lab, 626 Cochrans Mill Rd,POB 10940, Pittsburgh, PA 15236 USA. EM rme@pitt.edu FU National Energy Technology Laboratory's Regional University Alliance (NETL-RUA), a collaboration initiative of the NETL [DE-FE0004000] FX As part of the National Energy Technology Laboratory's Regional University Alliance (NETL-RUA), a collaboration initiative of the NETL, this technical effort was performed under the RES contract DE-FE0004000. We would like to thank Christopher Cleary of Clearco Products Co., Inc. for his helpful discussions concerning the silicone oils. We are appreciative of the helpful discussions with Dr. Robert J. Perry from GE Global Research on the stability of silicone polymers. We would also like to thank Jared Ciferno of the US DOE NETL for helpful discussions concerning absorption of CO, at warm and hot temperatures using hydrophobic solvents. NR 46 TC 1 Z9 1 U1 5 U2 5 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 0887-0624 EI 1520-5029 J9 ENERG FUEL JI Energy Fuels PD JUL PY 2016 VL 30 IS 7 BP 5901 EP 5910 DI 10.1021/acs.energyfuels.6b00140 PG 10 WC Energy & Fuels; Engineering, Chemical SC Energy & Fuels; Engineering GA DS2BO UT WOS:000380523200079 ER PT J AU Pandey, A Wheeler, R Shyam, A Stoughton, TB AF Pandey, A. Wheeler, R. Shyam, A. Stoughton, T. B. TI Onset of Plasticity via Relaxation Analysis (OPRA) SO EXPERIMENTAL MECHANICS LA English DT Article DE Yield stress; Elastic limit; Yield surface; Microtesting; Mobile dislocation ID STRESS-RELAXATION; INTERNAL-STRESS; CRYSTAL PLASTICITY; MICROMETER-SCALE; METALS; ALUMINUM; DEFORMATION; CREEP AB In crystalline metals and alloys, plasticity occurs due to the movement of mobile dislocations and the yield stress for engineering applications is traditionally quantified based on strain. The onset of irreversible plasticity or "yielding" is generally identified by a deviation from linearity in the stress-strain plot or by some standard convention such as 0.2 % offset strain relative to the "linear elastic response". In the present work, we introduce a new methodology for the determination of the true yield point based on stress relaxation. We show experimentally that this determination is self-consistent in nature and, as such, provides an objective observation of the very onset of plastic flow. Our designation for yielding is no longer related to the shape of the stress-strain curve but instead reflects the earliest signature of the activation of concerted irreversible dislocation motion in a test specimen under increasing load. C1 [Pandey, A.; Shyam, A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Pandey, A.] Rolls Royce LG Fuel Cell Syst Inc, North Canton, OH 44720 USA. [Wheeler, R.] MicroTesting Solut LLC, Columbus, OH 43026 USA. [Stoughton, T. B.] Gen Motors Res & Dev Ctr, Warren, MI 48090 USA. RP Pandey, A (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.; Pandey, A (reprint author), Rolls Royce LG Fuel Cell Syst Inc, North Canton, OH 44720 USA. EM dramitpandey@gmail.com OI Shyam, Amit/0000-0002-6722-4709 FU U.S Department of Energy, Office of Fossil Energy, Solid State Energy Conversion Alliance (SECA) Program FX Research sponsored by the U.S Department of Energy, Office of Fossil Energy, Solid State Energy Conversion Alliance (SECA) Program. Some of the instruments used in this investigation, which are part of the High Temperature Materials Laboratory at ORNL had been acquired with support from the U.S Department of Energy's Vehicle Technologies Program. NR 47 TC 0 Z9 0 U1 3 U2 3 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0014-4851 EI 1741-2765 J9 EXP MECH JI Exp. Mech. PD JUL PY 2016 VL 56 IS 6 BP 1095 EP 1107 DI 10.1007/s11340-016-0152-3 PG 13 WC Materials Science, Multidisciplinary; Mechanics; Materials Science, Characterization & Testing SC Materials Science; Mechanics GA DT8SX UT WOS:000381765600014 ER PT J AU Pandey, A Wheeler, R Shyam, A Stoughton, TB AF Pandey, A. Wheeler, R. Shyam, A. Stoughton, T. B. TI Onset of Plasticity via Relaxation Analysis (OPRA) (vol 56, pg 1109, 2016) SO EXPERIMENTAL MECHANICS LA English DT Correction C1 [Pandey, A.; Shyam, A.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Pandey, A.] Rolls Royce LG Fuel Cell Syst Inc, North Canton, OH 44720 USA. [Wheeler, R.] MicroTesting Solut LLC, Columbus, OH 43026 USA. [Stoughton, T. B.] Gen Motors Res & Dev Ctr, Warren, MI 48090 USA. RP Pandey, A (reprint author), Rolls Royce LG Fuel Cell Syst Inc, North Canton, OH 44720 USA. EM dramitpandey@gmail.com NR 1 TC 1 Z9 1 U1 0 U2 0 PU SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013 USA SN 0014-4851 EI 1741-2765 J9 EXP MECH JI Exp. Mech. PD JUL PY 2016 VL 56 IS 6 BP 1109 EP 1109 DI 10.1007/s11340-016-0166-x PG 1 WC Materials Science, Multidisciplinary; Mechanics; Materials Science, Characterization & Testing SC Materials Science; Mechanics GA DT8SX UT WOS:000381765600015 ER PT J AU Chang, YH Dobbe, R Bhushan, P Gray, JW Tomlin, CJ AF Chang, Young Hwan Dobbe, Roel Bhushan, Palak Gray, Joe W. Tomlin, Claire J. TI Reconstruction of Gene Regulatory Networks Based on Repairing Sparse Low-Rank Matrices SO IEEE-ACM TRANSACTIONS ON COMPUTATIONAL BIOLOGY AND BIOINFORMATICS LA English DT Article DE System identification; gene regulatory network; repairing ID EXPRESSION DATA; INFERENCE; IMAGE; IDENTIFICATION; MODELS AB With the growth of high-throughput proteomic data, in particular time series gene expression data from various perturbations, a general question that has arisen is how to organize inherently heterogenous data into meaningful structures. Since biological systems such as breast cancer tumors respond differently to various treatments, little is known about exactly how these gene regulatory networks (GRNs) operate under different stimuli. Challenges due to the lack of knowledge not only occur in modeling the dynamics of a GRN but also cause bias or uncertainties in identifying parameters or inferring the GRN structure. This paper describes a new algorithm which enables us to estimate bias error due to the effect of perturbations and correctly identify the common graph structure among biased inferred graph structures. To do this, we retrieve common dynamics of the GRN subject to various perturbations. We refer to the task as "repairing" inspired by "image repairing" in computer vision. The method can automatically correctly repair the common graph structure across perturbed GRNs, even without precise information about the effect of the perturbations. We evaluate the method on synthetic data sets and demonstrate an application to the DREAM data sets and discuss its implications to experiment design. C1 [Chang, Young Hwan; Dobbe, Roel; Bhushan, Palak; Tomlin, Claire J.] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Gray, Joe W.] Oregon Hlth & Sci Univ, Dept Biomed Engn, Portland, OR 97239 USA. [Gray, Joe W.] Oregon Hlth & Sci Univ, Ctr Spatial Syst Biomed, Portland, OR 97239 USA. [Tomlin, Claire J.] Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. RP Chang, YH (reprint author), Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. EM yhchang@berkeley.edu; dobbe@berkeley.edu; palak@berkeley.edu; grayjo@ohsu.edu; tomlin@eecs.berkeley.edu FU NIH NCI under the ICBP program [5U54CA112970-08]; NIH NCI under PS-OC program [5U54CA112970-08] FX This research was supported by the NIH NCI under the ICBP and PS-OC programs (5U54CA112970-08). NR 38 TC 0 Z9 0 U1 2 U2 2 PU IEEE COMPUTER SOC PI LOS ALAMITOS PA 10662 LOS VAQUEROS CIRCLE, PO BOX 3014, LOS ALAMITOS, CA 90720-1314 USA SN 1545-5963 EI 1557-9964 J9 IEEE ACM T COMPUT BI JI IEEE-ACM Trans. Comput. Biol. Bioinform. PD JUL-AUG PY 2016 VL 13 IS 4 BP 767 EP 777 DI 10.1109/TCBB.2015.2465952 PG 11 WC Biochemical Research Methods; Computer Science, Interdisciplinary Applications; Mathematics, Interdisciplinary Applications; Statistics & Probability SC Biochemistry & Molecular Biology; Computer Science; Mathematics GA DT5FI UT WOS:000381506500015 PM 27990101 ER PT J AU McDermott, SD Fox, PJ Cholis, I Lee, SK AF McDermott, Samuel D. Fox, Patrick J. Cholis, Ilias Lee, Samuel K. TI Wavelet-based techniques for the gamma-ray sky SO JOURNAL OF COSMOLOGY AND ASTROPARTICLE PHYSICS LA English DT Article DE dark matter theory; gamma ray detectors ID ANNIHILATING DARK-MATTER; FERMI-LAT OBSERVATIONS; GALACTIC-CENTER; EXCESS; EMISSION; BUBBLES; SPHERE; TELESCOPE; GALAXY; SIGNAL AB We demonstrate how the image analysis technique of wavelet decomposition can be applied to the gamma-ray sky to separate emission on different angular scales. New structures on scales that differ from the scales of the conventional astrophysical foreground and background uncertainties can be robustly extracted, allowing a model-independent characterization with no presumption of exact signal morphology. As a test case, we generate mock gamma-ray data to demonstrate our ability to extract extended signals without assuming a fixed spatial template. For some point source luminosity functions, our technique also allows us to differentiate a diffuse signal in gamma-rays from dark matter annihilation and extended gamma-ray point source populations in a data-driven way. C1 [McDermott, Samuel D.] SUNY Stony Brook, CN Yang Inst Theoret Phys, Stony Brook, NY 11794 USA. [Fox, Patrick J.] Fermilab Natl Accelerator Lab, Theoret Phys Dept, MS 106, Batavia, IL 60510 USA. [Cholis, Ilias] Johns Hopkins Univ, Dept Phys & Astron, 3400 N Charles St, Baltimore, MD 21218 USA. [Cholis, Ilias] Fermilab Natl Accelerator Lab, Ctr Particle Astrophys, POB 500, Batavia, IL 60510 USA. [Lee, Samuel K.] Broad Inst, 75 Ames St, Cambridge, MA 02142 USA. [Lee, Samuel K.] Princeton Univ, Princeton Ctr Theoret Sci, Jadwin Hall, Princeton, NJ 08544 USA. RP McDermott, SD (reprint author), SUNY Stony Brook, CN Yang Inst Theoret Phys, Stony Brook, NY 11794 USA. EM samuel.mcdermott@stonybrook.edu; pjfox@fnal.gov; icholis1@jhu.edu; lee.samuel.k@gmail.com OI Cholis, Ilias/0000-0002-3805-6478 FU National Science Foundation [PHY-1066293]; NSF [PHY1316617]; NASA [NNX15AB18G] FX We would like to thank T. Brandt, E. Charles, V. Gluscevic, D. Hooper, M. Lisanti, P. Luthy, M. Luty, J. Mardon, S. Murgia, B. Safdi, N. Shaviv, T. Slatyer, J. Thaler, C. Weniger, W. Xue, and G. Zweig for useful discussions. SDM also thanks the CTP at MIT and the astronomy group at IAS for feedback and hospitality while this work was underway. The work of SDM was performed in part at the Aspen Center for Physics, which is supported by National Science Foundation grant PHY-1066293, and at the Galileo Galilei Insitute. SDM is supported by NSF PHY1316617. IC is supported by NASA NNX15AB18G. PJF and IC would like to thank the Korea Institute for Advanced Study for their hospitality provided during the completion of this work. This work has made use of the SciPy [115], iPython [116], HEALPix [117], and healpy packages. NR 118 TC 1 Z9 1 U1 3 U2 4 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1475-7516 J9 J COSMOL ASTROPART P JI J. Cosmol. Astropart. Phys. PD JUL PY 2016 IS 7 AR 045 DI 10.1088/1475-7516/2016/07/045 PG 27 WC Astronomy & Astrophysics; Physics, Particles & Fields SC Astronomy & Astrophysics; Physics GA DT9NY UT WOS:000381830000046 ER PT J AU Du, ZY Arias, T Meng, W Chye, ML AF Du, Zhi-Yan Arias, Tatiana Meng, Wei Chye, Mee-Len TI Plant acyl-CoA-binding proteins: An emerging family involved in plant development and stress responses SO PROGRESS IN LIPID RESEARCH LA English DT Review DE Acyl-CoA metabolism; Lipid transport; Long-chain acyl-CoA esters; Phylogenetics; Stress tolerance; Subcellular localization; Temporal and spatial expression ID LIPID-TRANSFER PROTEINS; ACID BETA-OXIDATION; ENHANCES FREEZING TOLERANCE; ENDOPLASMIC-RETICULUM BODY; EPIDERMAL BARRIER FUNCTION; INNATE IMMUNE-RESPONSE; END RULE PATHWAY; FATTY-ACID; ARABIDOPSIS-THALIANA; BRASSICA-NAPUS AB Acyl-CoA-binding protein (ACBP) was first identified in mammals as a neuropeptide, and was demonstrated to belong to an important house-keeping protein family that extends across eukaryotes and some prokaryotes. In plants, the Arabidopsis ACBP family consists of six AtACBPs (AtACBP1 to AtACBP6), and has been investigated using gene knock-out mutants and overexpression lines. Herein, recent findings on the AtACBPs are examined to provide an insight on their functions in various plant developmental processes, such as embryo and seed development, seed dormancy and germination, seedling development and cuticle formation, as well as their roles under various environmental stresses. The significance of the AtACBPs in acyl-CoA/lipid metabolism, with focus on their interaction with long to very-long-chain (VLC) aryl-CoA esters and their potential role in the formation of lipid droplets in seeds and vegetative tissues are discussed. In addition, recent findings on the rice ACBP family are presented. The similarities and differences between ACBPs from Arabidopsis and rice, that represent eudicot and monocot model plants, respectively, are analyzed and the evolution of plant ACBPs by phylogenetic analysis reviewed. Finally, we propose potential uses of plant ACBPs in phytoremediation and in agriculture related to the improvement of environmental stress tolerance and seed oil production. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Du, Zhi-Yan; Arias, Tatiana; Chye, Mee-Len] Univ Hong Kong, Sch Biol Sci, Pokfulam, Hong Kong, Peoples R China. [Meng, Wei] Northeast Forestry Univ, Coll Life Sci, Harbin, Peoples R China. [Du, Zhi-Yan] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. [Du, Zhi-Yan] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. [Arias, Tatiana] Corp Invest Biol, Cra 72 A 78 B 141, Medellin, Colombia. RP Chye, ML (reprint author), Univ Hong Kong, Sch Biol Sci, Pokfulam, Hong Kong, Peoples R China. EM mlchye@hkucc.hku.hk RI Chye, Mee Len/A-2740-2010; OI /0000-0003-3505-3674 FU Research Grants Council of the Hong Kong Special Administrative Region, China [HKU765813M, HKU17105615M]; Wilson and Amelia Wong Endowment Fund FX This work was supported by the Research Grants Council of the Hong Kong Special Administrative Region, China (projects no. HKU765813M and HKU17105615M) and the Wilson and Amelia Wong Endowment Fund. We thank Ziwei Ye and Terry S.C. Lung for critical comments on the manuscript. NR 202 TC 0 Z9 0 U1 9 U2 10 PU PERGAMON-ELSEVIER SCIENCE LTD PI OXFORD PA THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND SN 0163-7827 J9 PROG LIPID RES JI Prog. Lipid Res. PD JUL PY 2016 VL 63 BP 165 EP 181 DI 10.1016/j.plipres.2016.06.002 PG 17 WC Biochemistry & Molecular Biology; Nutrition & Dietetics SC Biochemistry & Molecular Biology; Nutrition & Dietetics GA DT9PO UT WOS:000381835000011 PM 27368137 ER PT J AU Hammel, M Amlanjyoti, D Reyes, FE Chen, JH Parpana, R Tang, HYH Larabell, CA Tainer, JA Adhya, S AF Hammel, Michal Amlanjyoti, Dhar Reyes, Francis E. Chen, Jian-Hua Parpana, Rochelle Tang, Henry Y. H. Larabell, Carolyn A. Tainer, John A. Adhya, Sankar TI HU multimerization shift controls nucleoid compaction SO SCIENCE ADVANCES LA English DT Article ID X-RAY-SCATTERING; BINDING PROTEIN HU; ESCHERICHIA-COLI; DNA-BINDING; BIOLOGICAL MACROMOLECULES; CRYSTAL-STRUCTURE; GENE-EXPRESSION; BENT DNA; SAXS; TRANSCRIPTION AB Molecular mechanisms controlling functional bacterial chromosome (nucleoid) compaction and organization are surprisingly enigmatic but partly depend on conserved, histone-like proteins HU alpha alpha and HU alpha beta and their interactions that span the nanoscale and mesoscale from protein-DNA complexes to the bacterial chromosome and nucleoid structure. We determined the crystal structures of these chromosome-associated proteins in complex with native duplex DNA. Distinct DNA binding modes of HU alpha alpha and HU alpha beta elucidate fundamental features of bacterial chromosome packing that regulate gene transcription. By combining crystal structures with solution x-ray scattering results, we determined architectures of HU-DNA nucleoproteins in solution under near-physiological conditions. These macromolecular conformations and interactions result in contraction at the cellular level based on in vivo imaging of native unlabeled nucleoid by soft x-ray tomography upon HU beta and ectopic HU alpha 38 expression. Structural characterization of charge-altered HU alpha alpha-DNA complexes reveals an HU molecular switch that is suitable for condensing nucleoid and reprogramming noninvasive Escherichia coli into an invasive form. Collective findings suggest that shifts between networking and cooperative and noncooperative DNA-dependent HU multimerization control DNA compaction and supercoiling independently of cellular topoisomerase activity. By integrating x-ray crystal structures, x-ray scattering, mutational tests, and x-ray imaging that span from protein-DNA complexes to the bacterial chromosome and nucleoid structure, we show that defined dynamic HU interaction networks can promote nucleoid reorganization and transcriptional regulation as efficient general microbial mechanisms to help synchronize genetic responses to cell cycle, changing environments, and pathogenesis. C1 [Hammel, Michal; Reyes, Francis E.; Parpana, Rochelle; Tang, Henry Y. H.; Larabell, Carolyn A.; Tainer, John A.] Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging, Berkeley, CA 94720 USA. [Amlanjyoti, Dhar; Adhya, Sankar] NCI, Mol Biol Lab, Ctr Canc Res, NIH, Bldg 37, Bethesda, MD 20892 USA. [Chen, Jian-Hua; Larabell, Carolyn A.] Univ Calif San Francisco, Dept Anat, San Francisco, CA 94143 USA. [Tainer, John A.] Univ Texas MD Anderson Canc Ctr, Dept Mol & Cellular Oncol, 1515 Holcombe Blvd, Houston, TX 77030 USA. RP Hammel, M; Tainer, JA (reprint author), Lawrence Berkeley Natl Lab, Mol Biophys & Integrated Bioimaging, Berkeley, CA 94720 USA.; Tainer, JA (reprint author), Univ Texas MD Anderson Canc Ctr, Dept Mol & Cellular Oncol, 1515 Holcombe Blvd, Houston, TX 77030 USA. EM mhammel@lbl.gov; jatainer@lbl.gov FU NCI NIH HHS [P01 CA092584]; NIGMS NIH HHS [P41 GM103445, R01 GM105404] NR 57 TC 1 Z9 1 U1 6 U2 7 PU AMER ASSOC ADVANCEMENT SCIENCE PI WASHINGTON PA 1200 NEW YORK AVE, NW, WASHINGTON, DC 20005 USA SN 2375-2548 J9 SCI ADV JI Sci. Adv. PD JUL PY 2016 VL 2 IS 7 AR e1600650 DI 10.1126/sciadv.1600650 PG 11 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DT9GQ UT WOS:000381805300035 PM 27482541 ER PT J AU Tokunaga, TK Kim, Y Conrad, ME Bill, M Hobson, C Williams, KH Dong, W Wan, J Robbins, MJ Long, PE Faybishenko, B Christensen, JN Hubbard, SS AF Tokunaga, Tetsu K. Kim, Yongman Conrad, Mark E. Bill, Markus Hobson, Chad Williams, Kenneth H. Dong, Wenming Wan, Jiamin Robbins, Mark J. Long, Philip E. Faybishenko, Boris Christensen, John N. Hubbard, Susan S. TI Deep Vadose Zone Respiration Contributions to Carbon Dioxide Fluxes from a Semiarid Floodplain SO VADOSE ZONE JOURNAL LA English DT Article ID DISSOLVED ORGANIC-MATTER; URANIUM-CONTAMINATED AQUIFER; GAS-DIFFUSION COEFFICIENT; SOIL CO2 EFFLUX; UNSATURATED ZONE; GRADIENT-METHOD; GROUNDWATER; TEMPERATURE; SEDIMENT; TRANSFORMATIONS AB Although CO2 fluxes from soils are often assumed to originate within shallow soil horizons (<1-m depth), relatively little is known about respiration rates at greater depths. We compared measured and calculated CO2 fluxes at the Rifle floodplain along the Colorado River and measured CO2 production rates of floodplain sediments to determine the relative importance of deeper vadose zone respiration. Calculations based on measured CO2 gradients and estimated effective diffusion coefficients yielded fluxes that are generally consistent with measurements obtained at the soil surface (326 g C m(-2) yr(-1)). Carbon dioxide production from the 2.0- to 3.5-m depth interval was calculated to contribute 17% of the total floodplain respiration, with rates that were larger than some parts of the shallower vadose zone and underlying aquifer. Microbial respiration rates determined from laboratory incubation tests of the sediments support this conclusion. The deeper unsaturated zone typically maintains intermediate water and air saturations, lacks extreme temperatures and salinities, and is annually resupplied with organic carbon from snowmelt-driven recharge and by water table decline. This combination of favorable conditions supports deeper unsaturated zone microbial respiration throughout the year. C1 [Tokunaga, Tetsu K.] Lawrence Berkeley Natl Lab, Earth & Environm Sci Area, Berkeley, CA 94720 USA. RP Tokunaga, TK (reprint author), Lawrence Berkeley Natl Lab, Earth & Environm Sci Area, Berkeley, CA 94720 USA. RI Kim, Yongman/D-1130-2015; Wan, Jiamin/H-6656-2014; Hubbard, Susan/E-9508-2010; Tokunaga, Tetsu/H-2790-2014 OI Kim, Yongman/0000-0002-8857-1291; Tokunaga, Tetsu/0000-0003-0861-6128 FU DOE Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; U.S. Department of Energy (DOE) Subsurface Biogeochemical Research Program FX This work was conducted as part of the Genomes to Watershed Scientific Focus Area at Lawrence Berkeley National Laboratory, and was supported by the U.S. Department of Energy (DOE) Subsurface Biogeochemical Research Program, DOE Office of Science, Office of Biological and Environmental Research, under Contract Number DE-AC02-05CH11231. The invaluable support provided by the late Richard Dayvault of S.M. Stoller Corporation is gratefully acknowledged and remembered. We also thank Ben Potter (Stoller Corp., thermistor datalogging), Roelof Versteeg (Subsurface Insights, thermistor data), Rocky Cain (Cascade Drilling), and Craig Goodknight (Stoller, sediment logging). We thank the anonymous reviewers and Associate Editor Jorg Bachmann for their very helpful comments. NR 71 TC 0 Z9 0 U1 7 U2 8 PU SOIL SCI SOC AMER PI MADISON PA 677 SOUTH SEGOE ROAD, MADISON, WI 53711 USA SN 1539-1663 J9 VADOSE ZONE J JI Vadose Zone J. PD JUL PY 2016 VL 15 IS 7 DI 10.2136/vzj2016.02.0014 PG 25 WC Environmental Sciences; Soil Science; Water Resources SC Environmental Sciences & Ecology; Agriculture; Water Resources GA DT2HP UT WOS:000381301700001 ER PT J AU Xi, JX Si, XHA Kim, J Zhang, Y Jacob, RE Kabilan, S Corley, RA AF Xi, Jinxiang Si, Xiuhua A. Kim, Jongwon Zhang, Yu Jacob, Richard E. Kabilan, Senthil Corley, Richard A. TI Anatomical Details of the Rabbit Nasal Passages and Their Implications in Breathing, Air Conditioning, and Olfaction SO ANATOMICAL RECORD-ADVANCES IN INTEGRATIVE ANATOMY AND EVOLUTIONARY BIOLOGY LA English DT Article DE New Zealand white rabbit; nasal morphology; respiration; olfaction; lateral recess ID FLUID-DYNAMICS; MORPHOMETRIC-ANALYSIS; PARTICLE DEPOSITION; PARANASAL SINUSES; LARYNGEAL AIRWAYS; 5-YEAR-OLD CHILD; HUMAN NOSE; FLOW; AEROSOLS; CAVITY AB The rabbit is commonly used as a laboratory animal for inhalation toxicology tests and detail knowledge of the rabbit airway morphometry is needed for outcome analysis or theoretical modeling. The objective of this study is to quantify the morphometric dimension of the nasal airway of a New Zealand white rabbit and to relate the morphology and functions through analytical and computational methods. Images of high-resolution MRI scans of the rabbit were processed to measure the axial distribution of the cross-sectional areas, perimeter, and complexity level. The lateral recess, which has functions other than respiration or olfaction, was isolated from the nasal airway and its dimension was quantified separately. A low Reynolds number turbulence model was implemented to simulate the airflow, heat transfer, vapor transport, and wall shear stress. Results of this study provide detailed morphological information of the rabbit that can be used in the studies of olfaction, inhalation toxicology, drug delivery, and physiology-based pharmacokinetics modeling. For the first time, we reported a spiral nasal vestibule that splits into three paths leading to the dorsal meatus, maxilloturbinate, and ventral meatus, respectively. Both non-dimensional functional analysis and CFD simulations suggested that the airflow in the rabbit nose is laminar and the unsteady effect is only significantly during sniffing. Due to the large surface-to-volume ratio, the maxilloturbinate is highly effective in warming and moistening the inhaled air to body conditions. The unique anatomical structure and respiratory airflow pattern may have important implications for designing new odorant detectors or electronic noses. (C) 2016 Wiley Periodicals, Inc. C1 [Xi, Jinxiang; Zhang, Yu] Cent Michigan Univ, Sch Engn & Technol, 1200 South Franklin St, Mt Pleasant, MI 48859 USA. [Si, Xiuhua A.] Calif Baptist Univ, Dept Mech Engn, Riverside, CA USA. [Kim, Jongwon] Univ Georgia, Coll Engn, Athens, GA 30602 USA. [Jacob, Richard E.; Kabilan, Senthil; Corley, Richard A.] Pacific Northwest Natl Lab, Syst Toxicol & Exposure Sci, Richland, WA USA. RP Xi, JX (reprint author), Cent Michigan Univ, Sch Engn & Technol, 1200 South Franklin St, Mt Pleasant, MI 48859 USA. EM xi1j@cmich.edu FU Central Michigan University Early Career Award [P622911]; National Heart, Lung, and Blood Institute of the National Institutes of Health [NHLBI R01 HL073598]; U.S. Environmental Protection Agency [EP-C-09-006] FX Grant sponsor: Central Michigan University Early Career Award; Grant number: P622911 (to J.X.); Grant sponsor: National Heart, Lung, and Blood Institute of the National Institutes of Health; Grant number: NHLBI R01 HL073598 (to R.A.C.); Grant sponsor: U.S. Environmental Protection Agency; Grant number: EP-C-09-006 (to R.A.C.). NR 63 TC 1 Z9 1 U1 5 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1932-8486 EI 1932-8494 J9 ANAT REC JI Anat. Rec. PD JUL PY 2016 VL 299 IS 7 BP 853 EP 868 DI 10.1002/ar.23367 PG 16 WC Anatomy & Morphology SC Anatomy & Morphology GA DT7BM UT WOS:000381640700004 PM 27145450 ER PT J AU Giannakidis, A Gullberg, GT Pennell, DJ Firmin, DN AF Giannakidis, Archontis Gullberg, Grant T. Pennell, Dudley J. Firmin, David N. TI Value of Formalin Fixation for the Prolonged Preservation of Rodent Myocardial Microanatomical Organization: Evidence by MR Diffusion Tensor Imaging SO ANATOMICAL RECORD-ADVANCES IN INTEGRATIVE ANATOMY AND EVOLUTIONARY BIOLOGY LA English DT Article DE magnetic resonance diffusion tensor imaging; rat myocardial microanatomy; formalin; fixation; diffusivity; diffusion anisotropy; helix angle; inter-voxel diffusion coherence ID MAGNETIC-RESONANCE; FIBER-ORIENTATION; TISSUE; IMMUNOHISTOCHEMISTRY; INFARCTION; BRAIN; HEART; MODEL; SHEEP AB Previous ex vivo diffusion tensor imaging (DTI) studies on formalin-fixed myocardial tissue assumed that, after some initial changes in the first 48 hr since the start of fixation, DTI parameters remain stable over time. Prolonged preservation of cardiac tissue in formalin prior to imaging has been seen many times in the DTI literature as it is considered orderly. Our objective is to define the effects of the prolonged cardiac tissue exposure to formalin on tissue microanatomical organization, as this is assessed by DTI parameters. DTI experiments were conducted on eight excised rodent hearts that were fixed by immersion in formalin. The samples were randomly divided into two equinumerous groups corresponding to shorter (similar to 2 weeks) and more prolonged (similar to 6-8 weeks) durations of tissue exposure to formalin prior to imaging. We found that when the duration of cardiac tissue exposure to formalin before imaging increased, water diffusion became less restricted, helix angle (HA) histograms flattened out and exhibited heavier tails (even though the classic HA transmural variation was preserved), and a significant loss of inter-voxel primary diffusion orientation integrity was introduced. The prolonged preservation of cardiac tissue in formalin profoundly affected its microstructural organization, as this was assessed by DTI parameters. The accurate interpretation of diffusivity profiles necessitates awareness of the pitfalls of prolonged cardiac tissue exposure duration to formalin. The acquired knowledge works to the advantage of a proper experimental design of DTI studies of fixed hearts. (C) 2016 Wiley Periodicals, Inc. C1 [Giannakidis, Archontis; Pennell, Dudley J.; Firmin, David N.] Royal Brompton Hosp, NIHR Cardiovasc Biomed Res Unit, London, England. [Giannakidis, Archontis; Pennell, Dudley J.; Firmin, David N.] Imperial Coll London, Natl Heart & Lung Inst, London, England. [Giannakidis, Archontis; Gullberg, Grant T.] Lawrence Berkeley Natl Lab, Life Sci, Berkeley, CA USA. [Gullberg, Grant T.] Univ Calif San Francisco, Dept Radiol & Biomed Imaging, San Francisco, CA 94143 USA. RP Giannakidis, A (reprint author), Royal Brompton Hosp, Cardiovasc Biomed Res Unit, Sydney St, London SW3 6NP, England. EM A.Giannakidis@rbht.nhs.uk OI Pennell, Dudley/0000-0001-5523-1314 FU National Institutes of Health [R01 EB007219]; Office of Science, Office of Biological and Environmental Research, Biological Systems Science Division of the U.S. Department of Energy [DE-AC02-05CH11231]; NIHR Cardiovascular Biomedical Research Unit of Royal Brompton and Harefield NHS Foundation Trust and Imperial College London FX Grant sponsors: National Institutes of Health; Grant number: R01 EB007219; Director, Office of Science, Office of Biological and Environmental Research, Biological Systems Science Division of the U.S. Department of Energy; Grant number: DE-AC02-05CH11231; Grant sponsor: NIHR Cardiovascular Biomedical Research Unit of Royal Brompton and Harefield NHS Foundation Trust and Imperial College London. NR 41 TC 1 Z9 1 U1 0 U2 0 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1932-8486 EI 1932-8494 J9 ANAT REC JI Anat. Rec. PD JUL PY 2016 VL 299 IS 7 BP 878 EP 887 DI 10.1002/ar.23359 PG 10 WC Anatomy & Morphology SC Anatomy & Morphology GA DT7BM UT WOS:000381640700006 PM 27111575 ER PT J AU Ralph, FM Prather, KA Cayan, D Spackman, JR DeMott, P Dettinger, M Fairall, C Leung, R Rosenfeld, D Rutledge, S Waliser, D White, AB Cordeira, J Martin, A Helly, J Intrieri, J AF Ralph, F. M. Prather, K. A. Cayan, D. Spackman, J. R. DeMott, P. Dettinger, M. Fairall, C. Leung, R. Rosenfeld, D. Rutledge, S. Waliser, D. White, A. B. Cordeira, J. Martin, A. Helly, J. Intrieri, J. TI CALWATER FIELD STUDIES DESIGNED TO QUANTIFY THE ROLES OF ATMOSPHERIC RIVERS AND AEROSOLS IN MODULATING US WEST COAST PRECIPITATION IN A CHANGING CLIMATE SO BULLETIN OF THE AMERICAN METEOROLOGICAL SOCIETY LA English DT Article ID WATER-VAPOR SIGNATURE; SIERRA BARRIER JETS; UNITED-STATES; OROGRAPHIC PRECIPITATION; NORTHERN CALIFORNIA; AIR-POLLUTION; PACIFIC; STORM; WINTER; SATELLITE C1 [Ralph, F. M.; Prather, K. A.; Cayan, D.; Dettinger, M.; Martin, A.; Helly, J.] Univ Calif San Diego, Scripps Inst Oceanog, 9500 Gilman Dr,Ste 0224, La Jolla, CA 92093 USA. [Cayan, D.; Dettinger, M.] US Geol Survey, La Jolla, CA USA. [Spackman, J. R.] Sci & Technol Corp, Boulder, CO USA. [Spackman, J. R.; Fairall, C.; White, A. B.; Intrieri, J.] NOAA, Earth Syst Res Lab, Boulder, CO USA. [DeMott, P.; Rutledge, S.] Colorado State Univ, Ft Collins, CO 80523 USA. [Leung, R.] Pacific Northwest Natl Lab, Dept Energy, Richland, WA USA. [Rosenfeld, D.] Hebrew Univ Jerusalem, Jerusalem, Israel. [Waliser, D.] NASA, Jet Prop Lab, Pasadena, CA USA. [Cordeira, J.] Plymouth State Univ, Plymouth, NH USA. [Helly, J.] Univ Calif San Diego, San Diego Super Comp Ctr, La Jolla, CA 92093 USA. RP Ralph, FM (reprint author), Univ Calif San Diego, Scripps Inst Oceanog, 9500 Gilman Dr,Ste 0224, La Jolla, CA 92093 USA. EM mralph@ucsd.edu RI Rosenfeld, Daniel/F-6077-2016; Prather, Kimberly/A-3892-2008 OI Rosenfeld, Daniel/0000-0002-0784-7656; Prather, Kimberly/0000-0003-3048-9890 FU California Energy Commission (CEC); NOAA's Physical Sciences Division; NOAA; DOE; NSF; California's Department of Water Resources; UC San Diego's Scripps Institution of Oceanography; Center for Western Weather and Water Extremes; Science and Technology Corporation FX The CalWater-1 study from 2009 to 2011 was sponsored primarily by the California Energy Commission (CEC) and NOAA's Physical Sciences Division. The programmatic leadership of Guido Franco and Joe O'Hagan of CEC were central to the success of the experiment. Major field deployments for CalWater-2 (2014-16) are sponsored primarily by NOAA, DOE, and NSF, with additional facilities provided by NASA. The entire CalWater program of field studies leverages the unique ground-based extreme precipitation-observing network sponsored by California's Department of Water Resources. Planning has been heavily sponsored by UC San Diego's Scripps Institution of Oceanography and by the Center for Western Weather and Water Extremes, as well as Science and Technology Corporation. The knowledge and major effort of innumerable engineering, aircraft, ship, and technical support staff were vital to the development and execution of CalWater over the last several years. NR 63 TC 6 Z9 6 U1 14 U2 17 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0003-0007 EI 1520-0477 J9 B AM METEOROL SOC JI Bull. Amer. Meteorol. Soc. PD JUL PY 2016 VL 97 IS 7 BP 1209 EP 1228 DI 10.1175/BAMS-D-14-00043.1 PG 20 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DT7GF UT WOS:000381654400013 ER PT J AU Theurich, G DeLuca, C Campbell, T Liu, F Saint, K Vertenstein, M Chen, J Oehmke, R Doyle, J Whitcomb, T Wallcraft, A Iredell, M Black, T da Silva, AM Clune, T Ferraro, R Li, P Kelley, M Aleinov, I Balaji, V Zadeh, N Jacob, R Kirtman, B Giraldo, F McCarren, D Sandgathe, S Peckham, S Dunlap, R AF Theurich, Gerhard DeLuca, C. Campbell, T. Liu, F. Saint, K. Vertenstein, M. Chen, J. Oehmke, R. Doyle, J. Whitcomb, T. Wallcraft, A. Iredell, M. Black, T. da Silva, A. M. Clune, T. Ferraro, R. Li, P. Kelley, M. Aleinov, I. Balaji, V. Zadeh, N. Jacob, R. Kirtman, B. Giraldo, F. McCarren, D. Sandgathe, S. Peckham, S. Dunlap, R. TI THE EARTH SYSTEM PREDICTION SUITE Toward a Coordinated US Modeling Capability SO BULLETIN OF THE AMERICAN METEOROLOGICAL SOCIETY LA English DT Article ID ATMOSPHERIC SIMULATIONS; COUPLING TECHNOLOGIES; COAMPS-TC; CLIMATE; COMMUNITY; DESIGN; FRAMEWORK; ARCHITECTURE; DISSIPATION; WEATHER C1 [Theurich, Gerhard; Chen, J.] Sci Applicat Int Corp, Mclean, VA USA. [DeLuca, C.; Oehmke, R.; Dunlap, R.] NOAA ESRL, Boulder, CO USA. [DeLuca, C.; Oehmke, R.; Dunlap, R.] CIRES, Boulder, CO USA. [Campbell, T.; Wallcraft, A.] Naval Res Lab, Stennis Space Ctr, MS USA. [Liu, F.; Saint, K.] Cherokee Serv Grp, Ft Collins, CO USA. [Vertenstein, M.] Natl Ctr Atmospher Res, Boulder, CO USA. [Doyle, J.; Whitcomb, T.] Naval Res Lab, Monterey, CA USA. [Iredell, M.; Black, T.] NOAA NWS NCEP Environm Modeling Ctr, College Pk, MD USA. [da Silva, A. M.; Clune, T.] NASA, Goddard Space Flight Ctr, Greenbelt, MD USA. [Ferraro, R.; Li, P.] NASA, Jet Prop Lab, Pasadena, CA USA. [Kelley, M.; Aleinov, I.] NASA, Goddard Space Flight Ctr, New York, NY USA. [Balaji, V.; Zadeh, N.] Geophys Fluid Dynam Lab, Princeton, NJ USA. [Balaji, V.] Princeton Univ, Princeton, NJ 08544 USA. [Zadeh, N.] Engil Inc, Princeton, NJ USA. [Jacob, R.] Argonne Natl Lab, Lemont, IL USA. [Kirtman, B.] Univ Miami, Miami, FL USA. [Giraldo, F.] Naval Postgrad Sch, Monterey, CA USA. [McCarren, D.] Naval Meteorol & Oceanog, Naval Meteorol & Oceanog Command, Silver Spring, MD USA. [Sandgathe, S.] Univ Washington, Appl Phys Lab, Seattle, WA 98105 USA. [Peckham, S.] Univ Colorado, Boulder, CO 80309 USA. RP DeLuca, C (reprint author), NOAA CIRES, 325 Broadway, Boulder, CO 80305 USA. EM cecelia.deluca@noaa.gov FU National Aeronautics and Space Administration's Computational Modeling Algorithms and Cyberinfrastructure program [NNX12AP51G, NNX16AB20G]; National Aeronautics and Space Administration's Modeling Analysis and Prediction program [NNX11AL82G]; National Oceanic and Atmospheric Administration Climate Program Office; National Weather Service [NA15OAR4310103, NA12OAR4320137]; Department of Defense Office of Naval Research [N00014-13-1-0508, N00014-13-1-0845]; High Performance Computing Modernization Program [PP-CWO-KY06-001-P3]; National Science Foundation [1343811]; Oak Ridge Leadership Computing Facility, located in the National Center for Computational Sciences at Oak Ridge National Laboratory - Office of Science (BER) of the Department of Energy; NASA Center for Climate Simulation; NOAA Environmental Security Computer Center; Cooperative Institute for Climate Science, Princeton University from the National Oceanic and Atmospheric Administration, U.S. Department of Commerce [NA080AR4320752] FX The National Aeronautics and Space Administration's Computational Modeling Algorithms and Cyberinfrastructure program provides support for ESMF, the Cupid Integrated Development Environment, and integration of ESMF and the NUOPC Layer with ModelE (NNX12AP51G, NNX16AB20G). The National Aeronautics and Space Administration's Modeling Analysis and Prediction program supports ESMF and the integration of ESMF and the NUOPC Layer with the GEOS-5 model (NNX11AL82G). The National Oceanic and Atmospheric Administration Climate Program Office provides support for ESMF and the development of the Climate Forecast System using NUOPC Layer tools. The National Weather Service supports ESMF and NUOPC Layer development, and development of the Next Generation Global Prediction System using NUOPC Layer tools (NA15OAR4310103, NA12OAR4320137). The Department of Defense Office of Naval Research supports ESMF and NUOPC development, including adaption for emerging computer architectures, and the integration of the NUOPC Layer into the Community Earth System Model and Navy models (N00014-13-1-0508, N00014-13-1-0845). The High Performance Computing Modernization Program provides support for development of asynchronous I/O capabilities in ESMF (PP-CWO-KY06-001-P3). The National Science Foundation provided support for early development of ESMF and support for integration of hydrology and land components into NEMS (1343811). Computing resources for testing infrastructure and implementing it in applications were provided by the National Center for Atmospheric Research Computational and Information Systems Laboratory (CISL), sponsored by the National Science Foundation and other agencies; the Oak Ridge Leadership Computing Facility, located in the National Center for Computational Sciences at Oak Ridge National Laboratory, which is supported by the Office of Science (BER) of the Department of Energy; the NASA Center for Climate Simulation; and the NOAA Environmental Security Computer Center. V. Balaji is supported by the Cooperative Institute for Climate Science, Princeton University, under Award NA080AR4320752 from the National Oceanic and Atmospheric Administration, U.S. Department of Commerce. The statements, findings, conclusions, and recommendations are those of the authors and do not necessarily reflect the views of Princeton University, the National Oceanic and Atmospheric Administration, or the U.S. Department of Commerce. The authors thank Richard Rood and Anthony Craig for their insightful comments on the original manuscript, Donald Anderson for his guidance and advocacy, and Matthew Rothstein for his contributions to understanding the performance of NUOPC modeling applications. NR 75 TC 1 Z9 1 U1 1 U2 3 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 0003-0007 EI 1520-0477 J9 B AM METEOROL SOC JI Bull. Amer. Meteorol. Soc. PD JUL PY 2016 VL 97 IS 7 BP 1229 EP 1247 DI 10.1175/BAMS-D-14-00164.1 PG 19 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DT7GF UT WOS:000381654400014 ER PT J AU Lewis, JW Xue, LT AF Lewis, John W. Xue Litai TI China's security agenda transcends the South China Sea SO BULLETIN OF THE ATOMIC SCIENTISTS LA English DT Article DE Xi Jinping; China; South China Sea; Spratlys; Paracels; theater commands; strategic rivalry; strategic security mechanism AB In 2013, China's president, Xi Jinping, launched a massive reclamation and construction campaign on seven reefs in the Spratly Islands in the South China Sea. Beijing insisted that its actions were responsible and in accord with international law, but foreign critics questioned Xi's real intentions. Recently available internal documents involving China's leader reveal his views about war, the importance of oceans in protecting and rejuvenating the nation, and the motives underlying his moves in the South China Sea. Central to those motives is China's rivalry with the United States and the grand strategy needed to determine its outcome. To this end, Xi created five externally oriented and proactive military theater commands, one of which would protect newly built assets in the South China Sea and the sea lanes - sometimes referred to as the Maritime Silk Road - that pass through this sea to Eurasia and beyond. Simultaneously, China's actions in the Spratlys complicated and worsened the US-China rivalry, and security communities in both countries recognized that these actions could erupt into armed crises - despite decades of engagement to prevent them. A permanent problem-solving mechanism may allow the two countries to move toward a positive shared future. C1 [Lewis, John W.] Stanford Univ, Stanford, CA 94305 USA. [Lewis, John W.] Stanford Univ, Ctr Int Secur, Stanford, CA 94305 USA. [Lewis, John W.] Stanford Univ, Cooperat Project Peace & Cooperat Asian Pacific R, Stanford, CA 94305 USA. [Lewis, John W.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Lewis, John W.] Lawrence Livermore Natl Lab, Livermore, CA 94550 USA. [Lewis, John W.] US Dept Def, Ft Belvoir, VA 22060 USA. [Lewis, John W.] Senate Select Comm Intelligence, Washington, DC USA. [Lewis, John W.] Ctr East Asian Studies, Washington, DC USA. [Lewis, John W.] Ctr Int Secur & Arms Control, Washington, DC USA. [Lewis, John W.] Northeast Asia US Forum Int Policy, Washington, DC USA. [Xue Litai] Stanford Univ, Ctr Int Secur & Cooperat, Project Peace & Cooperat Asian Pacific Reg, Stanford, CA 94305 USA. RP Lewis, JW (reprint author), Stanford Univ, Stanford, CA 94305 USA.; Lewis, JW (reprint author), Stanford Univ, Ctr Int Secur, Stanford, CA 94305 USA.; Lewis, JW (reprint author), Stanford Univ, Cooperat Project Peace & Cooperat Asian Pacific R, Stanford, CA 94305 USA.; Lewis, JW (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA.; Lewis, JW (reprint author), Lawrence Livermore Natl Lab, Livermore, CA 94550 USA.; Lewis, JW (reprint author), US Dept Def, Ft Belvoir, VA 22060 USA.; Lewis, JW (reprint author), Senate Select Comm Intelligence, Washington, DC USA.; Lewis, JW (reprint author), Ctr East Asian Studies, Washington, DC USA.; Lewis, JW (reprint author), Ctr Int Secur & Arms Control, Washington, DC USA.; Lewis, JW (reprint author), Northeast Asia US Forum Int Policy, Washington, DC USA. EM jwlewis@stanford.edu NR 5 TC 0 Z9 0 U1 16 U2 20 PU SAGE PUBLICATIONS LTD PI LONDON PA 1 OLIVERS YARD, 55 CITY ROAD, LONDON EC1Y 1SP, ENGLAND SN 0096-3402 EI 1938-3282 J9 B ATOM SCI JI Bull. Atom. Scient. PD JUL PY 2016 VL 72 IS 4 BP 212 EP 221 DI 10.1080/00963402.2016.1194056 PG 10 WC International Relations; Social Issues SC International Relations; Social Issues GA DS6MZ UT WOS:000380897400003 ER PT J AU Lin, L Stamm, B AF Lin, Lin Stamm, Benjamin TI A POSTERIORI ERROR ESTIMATES FOR DISCONTINUOUS GALERKIN METHODS USING NON-POLYNOMIAL BASIS FUNCTIONS PART I: SECOND ORDER LINEAR PDE SO ESAIM-MATHEMATICAL MODELLING AND NUMERICAL ANALYSIS-MODELISATION MATHEMATIQUE ET ANALYSE NUMERIQUE LA English DT Article DE Discontinuous Galerkin method; a posteriori error estimation; non-polynomial basis functions; partial differential equations ID FINITE-ELEMENT-METHOD; ELLIPTIC PROBLEMS; LAGRANGE MULTIPLIERS; HELMHOLTZ PROBLEMS; PLANE-WAVES; EQUATIONS AB We present the first systematic work for deriving a posteriori error estimates for general non-polynomial basis functions in an interior penalty discontinuous Galerkin (DG) formulation for solving second order linear PDEs. Our residual type upper and lower bound error estimates measure the error in the energy norm. The main merit of our method is that the method is parameter-free, in the sense that all but one solution-dependent constants appearing in the upper and lower bound estimates are explicitly computable by solving local eigenvalue problems, and the only non-computable constant can be reasonably approximated by a computable one without affecting the overall effectiveness of the estimates in practice. As a side product of our formulation, the penalty parameter in the interior penalty formulation can be automatically determined as well. We develop an efficient numerical procedure to compute the error estimators. Numerical results for a variety of problems in 1D and 2D demonstrate that both the upper bound and lower bound are effective. C1 [Lin, Lin] Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA. [Lin, Lin] Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. [Stamm, Benjamin] Univ Paris 06, Sorbonne Univ, CNRS, Lab Jacques Louis Lions,UMR 7598,UMR 7598, F-75005 Paris, France. RP Lin, L (reprint author), Univ Calif Berkeley, Dept Math, Berkeley, CA 94720 USA.; Lin, L (reprint author), Lawrence Berkeley Natl Lab, Computat Res Div, Berkeley, CA 94720 USA. EM linlin@math.berkeley.edu; stamm@ann.jussieu.fr OI Stamm, Benjamin /0000-0003-3375-483X FU Laboratory Directed Research and Development (LDRD) from Berkeley Lab [DE-AC02-05CH11231]; Scientific Discovery through Advanced Computing (SciDAC) program; Center for Applied Mathematics for Energy Research Applications (CAMERA) - U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences FX This work was partially supported by Laboratory Directed Research and Development (LDRD) funding from Berkeley Lab, provided by the Director, Office of Science, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231, by the Scientific Discovery through Advanced Computing (SciDAC) program, and by the Center for Applied Mathematics for Energy Research Applications (CAMERA) funded by U.S. Department of Energy, Office of Science, Advanced Scientific Computing Research and Basic Energy Sciences (L. L.). L. L. would like to thank the hospitality of the Jacques-Louis Lions Laboratory (LJLL) during his visit. We sincerely thank Yvon Maday for thoughtful suggestions and critical reading of the paper. NR 29 TC 0 Z9 0 U1 2 U2 2 PU EDP SCIENCES S A PI LES ULIS CEDEX A PA 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A, FRANCE SN 0764-583X EI 1290-3841 J9 ESAIM-MATH MODEL NUM JI ESAIM-Math. Model. Numer. Anal.-Model. Math. Anal. Numer. PD JUL-AUG PY 2016 VL 50 IS 4 BP 1193 EP 1222 DI 10.1051/m2an/2015069 PG 30 WC Mathematics, Applied SC Mathematics GA DS1QQ UT WOS:000380371800011 ER PT J AU Al Hosni, M Caspari, E Pevzner, R Daley, TM Gurevich, B AF Al Hosni, Mohammed Caspari, Eva Pevzner, Roman Daley, Thomas M. Gurevich, Boris TI Case History: Using time-lapse vertical seismic profiling data to constrain velocity-saturation relations: the Frio brine pilot CO2 injection SO GEOPHYSICAL PROSPECTING LA English DT Article; Proceedings Paper CT 3rd International Workshop on Rock Physics (IWRP) CY APR 13-17, 2015 CL Perth, AUSTRALIA DE VSP; Rock physics; Time lapse; Monitoring ID GASSMANNS EQUATIONS; CORE MEASUREMENTS; ROCK PHYSICS; STORAGE; GERMANY; KETZIN; SITE; SEQUESTRATION; PRESSURE; POROSITY AB CO2 sequestration projects benefit from quantitative assessment of saturation distribution and plume extent for field development and leakage prevention. In this work, we carry out quantitative analysis of time-lapse seismic by using rock physics and seismic modelling tools. We investigate the suitability of Gassmann's equation for a CO2 sequestration project with 1600 tons of CO2 injected into high-porosity, brine-saturated sandstone. We analyze the observed time delays and amplitude changes in a time-lapse vertical seismic profile dataset. Both reflected and transmitted waves are analyzed qualitatively and quantitatively. To interpret the changes obtained from the vertical seismic profile, we perform a 2.5D elastic, finite-difference modelling study. The results show a P-wave velocity reduction of 750 m/s in the proximity of the injection well evident by the first arrivals (travel-time delays and amplitude change) and reflected wave amplitude changes. These results do not match with our rock physics model using Gassmann's equation predictions even when taking uncertainty in CO2 saturation and grain properties into account. We find that time-lapse vertical seismic profile data integrated with other information (e.g., core and well log) can be used to constrain the velocity-saturation relation and verify the applicability of theoretical models such as Gassmann's equation with considerable certainty. The study shows that possible nonelastic factors are in play after CO2 injection (e.g., CO2-brine-rock interaction and pressure effect) as Gassmann's equation underestimated the velocity reduction in comparison with field data for all three sets of time-lapse vertical seismic profile attributes. Our work shows the importance of data integration to validate the applicability of theoretical models such as Gassmann's equation for quantitative analysis of time-lapse seismic data. C1 [Al Hosni, Mohammed; Pevzner, Roman; Gurevich, Boris] Curtin Univ, Dept Explorat Geophys, GPO Box U1987, Perth, WA 6845, Australia. [Al Hosni, Mohammed; Pevzner, Roman; Gurevich, Boris] Cooperat Res Ctr Greenhouse Gas Technol CO2CRC, Barton, ACT 2600, Australia. [Gurevich, Boris] ARRC, CSIRO Energy, 26 Dick Perry Ave, Kensington, WA 6151, Australia. [Daley, Thomas M.] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Caspari, Eva] Univ Lausanne, Appl & Environm Geophys Grp, CH-1015 Lausanne, Switzerland. RP Al Hosni, M (reprint author), Curtin Univ, Dept Explorat Geophys, GPO Box U1987, Perth, WA 6845, Australia.; Al Hosni, M (reprint author), Cooperat Res Ctr Greenhouse Gas Technol CO2CRC, Barton, ACT 2600, Australia. EM m.alhosni@postgrad.curtin.edu.au RI Daley, Thomas/G-3274-2015 OI Daley, Thomas/0000-0001-9445-0843 NR 45 TC 1 Z9 1 U1 1 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0016-8025 EI 1365-2478 J9 GEOPHYS PROSPECT JI Geophys. Prospect. PD JUL PY 2016 VL 64 IS 4 SI SI BP 987 EP 1000 DI 10.1111/1365-2478.12386 PG 14 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DS6UB UT WOS:000380917200014 ER PT J AU Liljegren, JC Brown, DF Lunden, MM Silcott, D AF Liljegren, James C. Brown, David F. Lunden, Melissa M. Silcott, David TI PARTICLE DEPOSITION ONTO PEOPLE IN A TRANSIT VENUE SO HEALTH SECURITY LA English DT Article ID BACILLUS-ANTHRACIS; SIMULANT; RESUSPENSION; SURFACES; TRACKING; REMOVAL; INDOORS AB Following the release of an aerosolized biological agent in a transit venue, material deposited on waiting passengers and subsequently shed from their clothing may significantly magnify the scope and consequences of such an attack. Published estimates of the relevant particle deposition and resuspension parameters for complex indoor environments such as a transit facility are nonexistent. In this study, measurements of particle deposition velocity onto cotton fabric samples affixed to stationary and walking people in a large multimodal transit facility were obtained for tracer particle releases carried out as part of a larger study of subway airflows and particulate transport. Deposition velocities onto cotton and wool were also obtained using a novel automated sampling mechanism deployed at locations in the transit facility and throughout the subway. The data revealed higher deposition velocities than have been previously reported for people exposed in test chambers or office environments. The relatively high rates of deposition onto people in a transit venue obtained in this study suggest it is possible that fomite transport by subway and commuter/regional rail passengers could present a significant mechanism for rapidly dispersing a biological agent throughout a metropolitan area and beyond. C1 [Liljegren, James C.; Brown, David F.] Argonne Natl Lab, Global Secur Sci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Lunden, Melissa M.] Lawrence Berkeley Natl Lab, Environm Energy Technol Div, Berkeley, CA USA. [Lunden, Melissa M.] Aclima Inc, San Francisco, CA USA. [Silcott, David] S3I LLC, Reisterstown, MD USA. RP Liljegren, JC (reprint author), Argonne Natl Lab, Global Secur Sci, 9700 South Cass Ave,Bldg 221, Argonne, IL 60439 USA. EM jcliljegren@anl.gov FU Department of Homeland Security, Science and Technology Directorate, Chemical and Biological Division; Department of Homeland Security, Office of Health Affairs, Health Threats Resilience Division; [DE-AC02-06CH11357] FX We wish to thank an anonymous reviewer for bringing the work of Harper et al to our attention. This work was supported by the Department of Homeland Security, Science and Technology Directorate, Chemical and Biological Division, and by the Department of Homeland Security, Office of Health Affairs, Health Threats Resilience Division. The submitted manuscript has been created by UChicago Argonne, LLC, Operator of Argonne National Laboratory ("Argonne"). Argonne, a US Department of Energy Office of Science laboratory, is operated under Contract No. DE-AC02-06CH11357. The US government retains for itself, and others acting on its behalf, a paid-up nonexclusive, irrevocable worldwide license in said article to reproduce, prepare derivative works, distribute copies to the public, and perform publicly and display publicly, by or on behalf of the government. NR 24 TC 0 Z9 0 U1 1 U2 1 PU MARY ANN LIEBERT, INC PI NEW ROCHELLE PA 140 HUGUENOT STREET, 3RD FL, NEW ROCHELLE, NY 10801 USA SN 2326-5094 EI 2326-5108 J9 HEALTH SECUR JI Health Secur. PD JUL-AUG PY 2016 VL 14 IS 4 BP 237 EP 249 DI 10.1089/hs.2016.0010 PG 13 WC Public, Environmental & Occupational Health SC Public, Environmental & Occupational Health GA DS4SS UT WOS:000380772200006 PM 27400030 ER PT J AU Berdnikov, VV Somov, SV Pentchev, L Somov, A AF Berdnikov, V. V. Somov, S. V. Pentchev, L. Somov, A. TI Calibration of cathode strip gains in multiwire drift chambers of the GlueX experiment SO INSTRUMENTS AND EXPERIMENTAL TECHNIQUES LA English DT Article ID ANODE AB A technique for calibrating cathode strip gains in multiwire drift chambers of the GlueX experiment is described. The accuracy of the technique is estimated based on Monte Carlo generated data with known gain coefficients in the strip signal channels. One of the four detector sections has been calibrated using cosmic rays. Results of drift chamber calibration on the accelerator beam upon inclusion in the GlueX experimental setup are presented. C1 [Berdnikov, V. V.; Somov, S. V.] Natl Res Nucl Univ MEPhI, Moscow Engn Phys Inst, Kashirskoe Sh 31, Moscow 115409, Russia. [Pentchev, L.; Somov, A.] Thomas Jefferson Natl Accelerator Facil, 12000 Jefferson Ave, Newport News, VA 23606 USA. RP Berdnikov, VV (reprint author), Natl Res Nucl Univ MEPhI, Moscow Engn Phys Inst, Kashirskoe Sh 31, Moscow 115409, Russia. EM vvberdnikov@gmail.com FU Jefferson Science Associated, LLC under U.S. DOE [DOE_AC05_06OR23177] FX The work was done by the National Research Nuclear University MEPhI in cooperation with the Thomas Jefferson Accelerator Facility as a part of the GlueX experiment under financing from Jefferson Science Associated, LLC, which supports the work of the Thomas Jefferson Accelerator Facility for the United States Department of Energy under U.S. DOE contract no. DOE_AC05_06OR23177. NR 4 TC 0 Z9 0 U1 0 U2 0 PU MAIK NAUKA/INTERPERIODICA/SPRINGER PI NEW YORK PA 233 SPRING ST, NEW YORK, NY 10013-1578 USA SN 0020-4412 EI 1608-3180 J9 INSTRUM EXP TECH+ JI Instrum. Exp. Tech. PD JUL PY 2016 VL 59 IS 4 BP 513 EP 518 DI 10.1134/S0020441216030027 PG 6 WC Engineering, Multidisciplinary; Instruments & Instrumentation SC Engineering; Instruments & Instrumentation GA DS3LZ UT WOS:000380685800005 ER PT J AU Yuzawa, S Keasling, JD Katz, L AF Yuzawa, Satoshi Keasling, Jay D. Katz, Leonard TI Insights into polyketide biosynthesis gained from repurposing antibiotic-producing polyketide synthases to produce fuels and chemicals SO JOURNAL OF ANTIBIOTICS LA English DT Review ID MASS-SPECTROMETRY; ALPHA-LIPOMYCIN; BETA-LIPOMYCIN; GENE-CLUSTER; STEREOCHEMISTRY; ORGANIZATION; BORRELIDIN; ASSIGNMENT; MODULE; ACID AB Complex polyketides comprise a large number of natural products that have broad application in medicine and agriculture. They are produced in bacteria and fungi from enzyme complexes named type I polyketide synthases (PKSs) that are composed of multifunctional polypeptides containing discrete enzymatic domains organized into modules. The modular nature of PKSs has enabled a multitude of efforts to engineer the PKS genes to produce novel polyketides with enhanced or new properties. We have repurposed PKSs, employing up to three modules to produce a number of short-chain molecules that could have applications as fuels or industrial chemicals. Examining the enzymatic functions in vitro of these repurposed PKSs, we have uncovered a number of expanded substrate specificities and requirements of various PKS domains not previously reported and determined an unexpected difference in the order of enzymatic reactions within a module. In addition, we were able to efficiently change the stereochemistry of side chains in selected PKS products. C1 [Yuzawa, Satoshi; Keasling, Jay D.; Katz, Leonard] Univ Calif Berkeley, QB3 Inst, Berkeley, CA 94720 USA. [Keasling, Jay D.] Joint BioEnergy Inst, Emeryville, CA 94608 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Bioengn, Berkeley, CA 94720 USA. [Keasling, Jay D.; Katz, Leonard] Synthet Biol Res Ctr, Emeryville, CA 94608 USA. [Keasling, Jay D.] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Keasling, Jay D.] Lawrence Berkeley Natl Lab, Biol Syst & Engn Div, Berkeley, CA 94720 USA. RP Katz, L (reprint author), Univ Calif Berkeley, QB3 Inst, 5885 Hollis St,4th Floor, Berkeley, CA 94608 USA. EM katzl@berkeley.edu FU Joint BioEnergy Institute; Office of Science, Office of Biological and Environmental Research of the US Department of Energy [DE-AC02-05CH11231]; Department of Energy, ARPA-E Electrofuels Program [DE-0000206-1577]; National Science Foundation [EEC-0540879, MCB-1341894, DGE 1106400, 1106400] FX This work was supported by the Joint BioEnergy Institute, which is funded by the Office of Science, Office of Biological and Environmental Research of the US Department of Energy (Contract No. DE-AC02-05CH11231), by the Department of Energy, ARPA-E Electrofuels Program (Contract No. DE-0000206-1577) and by the National Science Foundation (Award No. EEC-0540879 to the Synthetic Biology Engineering Research Center, Award No. MCB-1341894, and Grant Nos. DGE 1106400 and 1106400 of the Graduate Research Fellowship Program). NR 28 TC 2 Z9 2 U1 8 U2 15 PU JAPAN ANTIBIOTICS RESEARCH ASSOC PI TOKYO PA 2 20 8 KAMIOSAKI SHINAGAWA KU, TOKYO, 141, JAPAN SN 0021-8820 J9 J ANTIBIOT JI J. Antibiot. PD JUL PY 2016 VL 69 IS 7 SI SI BP 494 EP 499 DI 10.1038/ja.2016.64 PG 6 WC Biotechnology & Applied Microbiology; Immunology; Microbiology; Pharmacology & Pharmacy SC Biotechnology & Applied Microbiology; Immunology; Microbiology; Pharmacology & Pharmacy GA DS5UL UT WOS:000380848100004 PM 27245558 ER PT J AU Burleyson, CD Feng, Z Hagos, SM Fast, J Machado, LAT Martin, ST AF Burleyson, Casey D. Feng, Zhe Hagos, Samson M. Fast, Jerome Machado, Luiz A. T. Martin, Scot T. TI Spatial Variability of the Background Diurnal Cycle of Deep Convection around the GoAmazon2014/5 Field Campaign Sites SO JOURNAL OF APPLIED METEOROLOGY AND CLIMATOLOGY LA English DT Article ID BOUNDARY-LAYER EXPERIMENT; AMERICAN MONSOON SYSTEM; SOUTH-AMERICA; TROPICAL PRECIPITATION; GLOBAL PRECIPITATION; PASSIVE MICROWAVE; EASTERN AMAZONIA; CLOUD SYSTEMS; RIVER BREEZE; SQUALL LINES AB The isolation of the Amazon rain forest makes it challenging to observe precipitation forming there, but it also creates a natural laboratory to study anthropogenic impacts on clouds and precipitation in an otherwise pristine environment. Observations were collected upwind and downwind of Manaus, Brazil, during the "Observations and Modeling of the Green Ocean Amazon 2014-2015" experiment (GoAmazon2014/5). Besides aircraft, most of the observations were point measurements made in a spatially heterogeneous environment, making it hard to distinguish anthropogenic signals from naturally occurring spatial variability. In this study, 15 years of satellite data are used to examine the spatial and temporal variability of deep convection around the GoAmazon2014/5 sites using cold cloud tops (infrared brightness temperatures colder than 240 K) as a proxy for deep convection. During the rainy season, convection associated with the inland propagation of the previous day's sea-breeze front is in phase with the diurnal cycle of deep convection near Manaus but is out of phase a few hundred kilometers to the east and west. Convergence between the river breezes and the easterly trade winds generates afternoon convection up to 10% more frequently (on average; similar to 4 mm day(-1) more intense rainfall) at the GoAmazon2014/5 sites east of the Negro River (T0e, T0t/k, and T1) relative to the T3 site, which was located west of the river. In general, the annual and diurnal cycles of precipitation during 2014 were similar to climatological values that are based on satellite data from 2000 to 2013. C1 [Burleyson, Casey D.; Feng, Zhe; Hagos, Samson M.; Fast, Jerome; Machado, Luiz A. T.; Martin, Scot T.] Pacific Northwest Natl Lab, POB 999,MS K9-24, Richland, WA 99352 USA. RP Burleyson, CD (reprint author), Pacific Northwest Natl Lab, POB 999,MS K9-24, Richland, WA 99352 USA. EM casey.burleyson@pnnl.gov RI Martin, Scot/G-1094-2015 OI Martin, Scot/0000-0002-8996-7554 FU U.S. Department of Energy (DOE) Office of Science, Biological and Environmental Research as part of the Atmospheric System Research (ASR) program; Office of Biological and Environmental Research; DOe [DE-AC06-76RLO 1830] FX This research is based on work supported by the U.S. Department of Energy (DOE) Office of Science, Biological and Environmental Research as part of the Atmospheric System Research (ASR) program. We acknowledge the logistical support during GoAmazon2014/5 from the ARM Climate Research Facility, a DOE Office of Science user facility sponsored by the Office of Biological and Environmental Research. The work was conducted under 001030/2012-4 of the Brazilian National Council for Scientific and Technological Development (CNPq). The Pacific Northwest National Laboratory is operated for DOE by Battelle Memorial Institute under Contract DE-AC06-76RLO 1830. We thank Aaron Funk and Courtney Schumacher for providing the gridded SIPAM radar data. Special thanks are given to Larry Berg, Jennifer Comstock, Laura Riihimaki, and Hailong Wang for their suggestions on improving this work. David Fitzjarrald and two anonymous reviewers provided valuable feedback. NR 55 TC 3 Z9 3 U1 4 U2 5 PU AMER METEOROLOGICAL SOC PI BOSTON PA 45 BEACON ST, BOSTON, MA 02108-3693 USA SN 1558-8424 EI 1558-8432 J9 J APPL METEOROL CLIM JI J. Appl. Meteorol. Climatol. PD JUL PY 2016 VL 55 IS 7 BP 1579 EP 1598 DI 10.1175/JAMC-D-15-0229.1 PG 20 WC Meteorology & Atmospheric Sciences SC Meteorology & Atmospheric Sciences GA DS4NK UT WOS:000380757600004 ER PT J AU Frash, LP Carey, JW Lei, Z Rougier, E Ickes, T Viswanathan, HS AF Frash, Luke P. Carey, J. William Lei, Zhou Rougier, Esteban Ickes, Timothy Viswanathan, Hari S. TI High-stress triaxial direct-shear fracturing of Utica shale and in situ X-ray microtomography with permeability measurement SO JOURNAL OF GEOPHYSICAL RESEARCH-SOLID EARTH LA English DT Article DE microtomography; CO2 sequestration; induced seismicity; shear stimulation; caprock; FDEM ID DISCRETE ELEMENT METHOD; FLUID-FLOW; HYDRAULIC FRACTURE; ROCK FRACTURE; PRESSURE; SIMULATIONS; EVOLUTION; FAILURE; MEDIA AB The challenge of characterizing subsurface fluid flow has motivated extensive laboratory studies, yet fluid flow through rock specimens in which fractures are created and maintained at high-stress conditions remains underinvestigated at this time. The studies of this type that do exist do not include in situ fracture geometry measurements acquired at stressed conditions, which would be beneficial for interpreting the flow behavior. Therefore, this study investigates the apparent permeability induced by direct-shear fracture stimulation through Utica shale (a shale gas resource and potential caprock material) at high triaxial stress confinement and for the first time relates these values to simultaneously acquired in situ X-ray radiography and microtomography images. Change in fracture geometry and apparent permeability was also investigated at additional reduced stress states. Finite element and combined finite-discrete element modeling were used to evaluate the in situ observed fracturing process. Results from this study indicate that the increase in apparent permeability through fractures created at high-stress (22.2MPa) was minimal relative to the intact rock (less than 1 order of magnitude increase), while fractures created at low stress (3.4MPa) were significantly more permeable (2 to 4 orders of magnitude increase). This study demonstrates the benefit of in situ X-ray observation coupled with apparent permeability measurement to analyze fracture creation in the subsurface. Our results show that the permeability induced by fractures through shale at high stress can be minor and therefore favorable in application to CO2 sequestration caprock integrity but unfavorable for hydrocarbon recovery from unconventional reservoirs. C1 [Frash, Luke P.; Carey, J. William; Lei, Zhou; Rougier, Esteban; Viswanathan, Hari S.] Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. [Ickes, Timothy] Los Alamos Natl Lab, Appl Engn Technol, Los Alamos, NM USA. RP Frash, LP (reprint author), Los Alamos Natl Lab, Earth & Environm Sci Div, Los Alamos, NM 87545 USA. EM lfrash@lanl.gov OI Frash, Luke/0000-0002-5424-4698; Lei, Zhou/0000-0002-4965-5556 FU Los Alamos National Laboratory LDRD [200140002DR]; DOE-Fossil Energy [FWP FE-406/408/409-14-FY15, FE-374-14-FY15, FE-10-003] FX Support provided by the Los Alamos National Laboratory LDRD 200140002DR and DOE-Fossil Energy (FWP FE-406/408/409-14-FY15, FE-374-14-FY15, and FE-10-003) is gratefully acknowledged. We also thank Chesapeake Energy (Steve Chipera) for providing Utica shale samples and mineralogical analyses. LA-UR-15-27278. Data used in the production of this document are available upon request to the corresponding author. NR 64 TC 1 Z9 1 U1 10 U2 11 PU AMER GEOPHYSICAL UNION PI WASHINGTON PA 2000 FLORIDA AVE NW, WASHINGTON, DC 20009 USA SN 2169-9313 EI 2169-9356 J9 J GEOPHYS RES-SOL EA JI J. Geophys. Res.-Solid Earth PD JUL PY 2016 VL 121 IS 7 BP 5493 EP 5508 DI 10.1002/2016JB012850 PG 16 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DT6XF UT WOS:000381627500035 ER PT J AU Chan, MK Harrison, N McDonald, RD Ramshaw, BJ Modic, KA Barisic, N Greven, M AF Chan, M. K. Harrison, N. McDonald, R. D. Ramshaw, B. J. Modic, K. A. Barisic, N. Greven, M. TI Single reconstructed Fermi surface pocket in an underdoped single-layer cuprate superconductor SO NATURE COMMUNICATIONS LA English DT Article ID HIGH-TEMPERATURE SUPERCONDUCTORS; T-C SUPERCONDUCTOR; DENSITY-WAVE ORDER; QUANTUM OSCILLATIONS; CHARGE ORDER; NORMAL-STATE; SPECTROSCOPIC EVIDENCE; PHASE-DIAGRAM; PSEUDOGAP; BI2SR2CACU2O8+DELTA AB The observation of a reconstructed Fermi surface via quantum oscillations in hole-doped cuprates opened a path towards identifying broken symmetry states in the pseudogap regime. However, such an identification has remained inconclusive due to the multi-frequency quantum oscillation spectra and complications accounting for bilayer effects in most studies. We overcome these impediments with high-resolution measurements on the structurally simpler cuprate HgBa2CuO4+delta (Hg1201), which features one CuO2 plane per primitive unit cell. We find only a single oscillatory component with no signatures of magnetic breakdown tunnelling to additional orbits. Therefore, the Fermi surface comprises a single quasi-two-dimensional pocket. Quantitative modelling of these results indicates that a biaxial charge density wave within each CuO2 plane is responsible for the reconstruction and rules out crisscrossed charge stripes between layers as a viable alternative in Hg1201. Lastly, we determine that the characteristic gap between reconstructed pockets is a significant fraction of the pseudogap energy. C1 [Chan, M. K.; Harrison, N.; McDonald, R. D.; Ramshaw, B. J.; Modic, K. A.] Los Alamos Natl Lab, Pulsed Field Facil, Natl High Magnet Field Lab, Mail Stop E536, Los Alamos, NM 87545 USA. [Chan, M. K.; Barisic, N.; Greven, M.] Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. [Barisic, N.] Tech Univ Wien, Wiedner Haupstr 8-10, A-1040 Vienna, Austria. RP Chan, MK; Harrison, N (reprint author), Los Alamos Natl Lab, Pulsed Field Facil, Natl High Magnet Field Lab, Mail Stop E536, Los Alamos, NM 87545 USA.; Chan, MK (reprint author), Univ Minnesota, Sch Phys & Astron, Minneapolis, MN 55455 USA. EM mkchan@lanl.gov; nharrison@lanl.gov OI Harrison, Neil/0000-0001-5456-7756; Chan, Mun/0000-0002-8808-9040 FU US Department of Energy BES 'Science at 100T' [LANLF100]; National Science Foundation [DMR-1157490]; State of Florida; U.S. Department of Energy; Department of Energy, Office of Basic Energy Sciences [DE-SC0006858]; FWF project [P2798] FX The work performed at Los Alamos National Laboratory, was supported by the US Department of Energy BES 'Science at 100T' grant number LANLF100. The National High Magnetic Field Laboratory - PFF facility is funded by the National Science Foundation Cooperative Agreement Number DMR-1157490, the State of Florida and the U.S. Department of Energy. Work at the University of Minnesota was supported by the Department of Energy, Office of Basic Energy Sciences, under Award Number DE-SC0006858. N.B. acknowledges the support of FWF project P2798. We thank Ruixing Liang, W.N. Hardy and D.A. Bonn at UBC, Canada, for generously supplying the Y123 crystal measured as part of this work. We aknowledge fruitful discussion with S.E. Sebastian. We also thank the Pulsed Field Facility, Los Alamos National Lab engineering and technical staff for experimental assistance. NR 62 TC 4 Z9 4 U1 16 U2 20 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2016 VL 7 AR 12244 DI 10.1038/ncomms12244 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DS5RX UT WOS:000380841100001 PM 27448102 ER PT J AU Sun, JP Matsuura, K Ye, GZ Mizukami, Y Shimozawa, M Matsubayashi, K Yamashita, M Watashige, T Kasahara, S Matsuda, Y Yan, JQ Sales, BC Uwatoko, Y Cheng, JG Shibauchi, T AF Sun, J. P. Matsuura, K. Ye, G. Z. Mizukami, Y. Shimozawa, M. Matsubayashi, K. Yamashita, M. Watashige, T. Kasahara, S. Matsuda, Y. Yan, J-Q. Sales, B. C. Uwatoko, Y. Cheng, J-G. Shibauchi, T. TI Dome-shaped magnetic order competing with high-temperature superconductivity at high pressures in FeSe SO NATURE COMMUNICATIONS LA English DT Article ID PHASE-DIAGRAM; THIN-FILMS; CRYSTAL; DENSITY; FIELDS; SRTIO3 AB The coexistence and competition between superconductivity and electronic orders, such as spin or charge density waves, have been a central issue in high transition-temperature (T-c) superconductors. Unlike other iron-based superconductors, FeSe exhibits nematic ordering without magnetism whose relationship with its superconductivity remains unclear. Moreover, a pressure-induced fourfold increase of Tc has been reported, which poses a profound mystery. Here we report high-pressure magnetotransport measurements in FeSe up to similar to 15 GPa, which uncover the dome shape of magnetic phase superseding the nematic order. Above similar to 6GPa the sudden enhancement of superconductivity (T-c <= 38.3 K) accompanies a suppression of magnetic order, demonstrating their competing nature with very similar energy scales. Above the magnetic dome, we find anomalous transport properties suggesting a possible pseudogap formation, whereas linear-in-temperature resistivity is observed in the normal states of the high-T-c phase above 6 GPa. The obtained phase diagram highlights unique features of FeSe among iron-based superconductors, but bears some resemblance to that of high-T-c cuprates. C1 [Sun, J. P.; Ye, G. Z.; Cheng, J-G.] Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China. [Sun, J. P.; Ye, G. Z.; Cheng, J-G.] Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China. [Matsuura, K.; Mizukami, Y.; Shibauchi, T.] Univ Tokyo, Dept Adv Mat Sci, Kashiwa, Chiba 2778561, Japan. [Ye, G. Z.] Yunnan Univ, Sch Phys Sci & Technol, Kunming 650091, Peoples R China. [Shimozawa, M.; Yamashita, M.; Uwatoko, Y.] Univ Tokyo, Inst Solid State Phys, Kashiwa, Chiba 2778581, Japan. [Matsubayashi, K.] Univ Electrocommun, Dept Engn Sci, Chofu, Tokyo 1828585, Japan. [Watashige, T.; Kasahara, S.; Matsuda, Y.] Kyoto Univ, Dept Phys, Sakyo Ku, Kyoto 6068502, Japan. [Yan, J-Q.; Sales, B. C.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Yan, J-Q.] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. RP Cheng, JG (reprint author), Chinese Acad Sci, Beijing Natl Lab Condensed Matter Phys, Beijing 100190, Peoples R China.; Cheng, JG (reprint author), Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China.; Shibauchi, T (reprint author), Univ Tokyo, Dept Adv Mat Sci, Kashiwa, Chiba 2778561, Japan.; Yan, JQ (reprint author), Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA.; Yan, JQ (reprint author), Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. EM jqyan@utk.edu; jgcheng@iphy.ac.cn; shibauchi@k.u-tokyo.ac.jp RI Shibauchi, Takasada/B-9349-2008; Cheng, Jinguang/A-8342-2012; Matsubayashi, Kazuyuki/F-7696-2013; Kasahara, Shigeru/H-3064-2014 OI Shibauchi, Takasada/0000-0001-5831-4924; Kasahara, Shigeru/0000-0002-6007-9617 FU National Basic Research Program of China [2014CB921500]; National Science Foundation of Chin [11574377, 11304371]; Strategic Priority Research Program of the Chinese Academy of Sciences [XDB07020100]; Opening Project of Wuhan National High Magnetic Field Center [2015KF22]; Huazhong University of Science and Technology; US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division FX We thank T. Terashima, X.J. Zhou, T. Xiang, R. Yu, Q.M. Zhang, G. Chen, and J.-S. Zhou for very helpful discussions. We also thank Bosen Wang for his technical help. Work at IOP CAS was supported by the National Basic Research Program of China (Grant No. 2014CB921500), National Science Foundation of China (Grant No. 11574377, 11304371), and the Strategic Priority Research Program of the Chinese Academy of Sciences (Grant No. XDB07020100) as well as the Opening Project of Wuhan National High Magnetic Field Center (Grant No. 2015KF22), Huazhong University of Science and Technology. Work in Japan was supported by Grant-in-Aids for Scientific Research (A), (B), (S), and on Innovative Areas 'Topological Materials Science'. Work at ORNL was supported by the US Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. NR 43 TC 10 Z9 10 U1 31 U2 47 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2016 VL 7 AR 12146 DI 10.1038/ncomms12146 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DS5GQ UT WOS:000380810100001 PM 27431724 ER PT J AU Zhu, Y Yan, JW Liu, WJ Liu, L Sheng, Y Sun, Y Li, YY Scheller, HV Jiang, MY Hou, XL Ni, L Zhang, AY AF Zhu, Yuan Yan, Jingwei Liu, Weijuan Liu, Lei Sheng, Yu Sun, Yue Li, Yanyun Scheller, Henrik Vibe Jiang, Mingyi Hou, Xilin Ni, Lan Zhang, Aying TI Phosphorylation of a NAC Transcription Factor by a Calcium/Calmodulin-Dependent Protein Kinase Regulates Abscisic Acid-Induced Antioxidant Defense in Maize SO PLANT PHYSIOLOGY LA English DT Article ID CA2+/CALMODULIN-DEPENDENT PROTEIN; DROUGHT TOLERANCE; INTRACELLULAR ACCOMMODATION; MEDICAGO-TRUNCATULA; SIGNAL-TRANSDUCTION; CALMODULIN-BINDING; CALCIUM-CALMODULIN; NODULE DEVELOPMENT; FUNGAL SYMBIOSES; LOTUS-JAPONICUS AB Calcium/calmodulin-dependent protein kinase (CCaMK) has been shown to play an important role in abscisic acid (ABA)-induced antioxidant defense and enhance the tolerance of plants to drought stress. However, its downstream molecular events are poorly understood. Here, we identify a NAC transcription factor, ZmNAC84, in maize (Zea mays), which physically interacts with ZmCCaMK in vitro and in vivo. ZmNAC84 displays a partially overlapping expression pattern with ZmCCaMK after ABA treatment, and H2O2 is required for ABA-induced ZmNAC84 expression. Functional analysis reveals that ZmNAC84 is essential for ABA-induced antioxidant defense in a ZmCCaMK-dependent manner. Furthermore, ZmCCaMK directly phosphorylates Ser-113 of ZmNAC84 in vitro, and Ser-113 is essential for the ABA-induced stimulation of antioxidant defense by ZmCCaMK. Moreover, overexpression of ZmNAC84 in tobacco (Nicotiana tabacum) can improve drought tolerance and alleviate drought-induced oxidative damage of transgenic plants. These results define a mechanism for ZmCCaMK function in ABA-induced antioxidant defense, where ABA-produced H2O2 first induces expression of ZmCCaMK and ZmNAC84 and activates ZmCCaMK. Subsequently, the activated ZmCCaMK phosphorylates ZmNAC84 at Ser-113, thereby inducing antioxidant defense by activating downstream genes. C1 [Zhu, Yuan; Yan, Jingwei; Liu, Weijuan; Liu, Lei; Sheng, Yu; Sun, Yue; Li, Yanyun; Jiang, Mingyi; Hou, Xilin; Ni, Lan; Zhang, Aying] Nanjing Agr Univ, Coll Life Sci, Nanjing 210095, Jiangsu, Peoples R China. [Scheller, Henrik Vibe] Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Phys Biosci Div, Berkeley, CA 94720 USA. [Jiang, Mingyi] Nanjing Agr Univ, Natl Key Lab Crop Genet & Germplasm Enhancement, Nanjing 210095, Jiangsu, Peoples R China. [Hou, Xilin] Jiangsu Polytech Coll Agr & Forestry, Engn & Technol Ctr Modern Hort, Zhenjiang 212400, Jiangsu, Peoples R China. RP Zhang, AY (reprint author), Nanjing Agr Univ, Coll Life Sci, Nanjing 210095, Jiangsu, Peoples R China. EM ayzhang@njau.edu.cn RI Scheller, Henrik/A-8106-2008 OI Scheller, Henrik/0000-0002-6702-3560 FU National Natural Science Foundation of China [31371547, 31071344, J1210056]; Fundamental Research Funds for the Central Universities [KYZ201637, KYZ201402, KYZ201157]; Program for New Century Excellent Talents in University [NCET-10-0498]; Priority Academic Program Development of Jiangsu Higher Education Institutions; DOE Joint BioEnergy Institute by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231] FX This study was supported by grants from the National Natural Science Foundation of China (31371547, 31071344, and J1210056), the Fundamental Research Funds for the Central Universities (KYZ201637, KYZ201402, and KYZ201157), the Program for New Century Excellent Talents in University (NCET-10-0498), the Priority Academic Program Development of Jiangsu Higher Education Institutions, and as part of the DOE Joint BioEnergy Institute (http://www.jbei.org) by the U.S. Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the U.S. Department of Energy. NR 63 TC 4 Z9 4 U1 12 U2 15 PU AMER SOC PLANT BIOLOGISTS PI ROCKVILLE PA 15501 MONONA DRIVE, ROCKVILLE, MD 20855 USA SN 0032-0889 EI 1532-2548 J9 PLANT PHYSIOL JI Plant Physiol. PD JUL PY 2016 VL 171 IS 3 BP 1651 EP 1664 DI 10.1104/pp.16.00168 PG 14 WC Plant Sciences SC Plant Sciences GA DT2IF UT WOS:000381303300013 PM 27208250 ER PT J AU Lopez-Igual, R Wilson, A Leverenz, RL Melnicki, MR de Carbon, CB Sutter, M Turmo, A Perreau, F Kerfeld, CA Kirilovsky, D AF Lopez-Igual, Rocio Wilson, Adjele Leverenz, Ryan L. Melnicki, Matthew R. de Carbon, Celine Bourcier Sutter, Markus Turmo, Aiko Perreau, Francois Kerfeld, Cheryl A. Kirilovsky, Diana TI Different Functions of the Paralogs to the N-Terminal Domain of the Orange Carotenoid Protein in the Cyanobacterium Anabaena sp PCC 7120 SO PLANT PHYSIOLOGY LA English DT Article ID SP-STRAIN PCC-7120; HETEROCYST DIFFERENTIATION; CELL-DIFFERENTIATION; ENERGY-DISSIPATION; NITROGEN-FIXATION; LIGHT; PHOTOPROTECTION; PHYCOBILISOME; PHOTOSYNTHESIS; MECHANISM AB The photoactive Orange Carotenoid Protein (OCP) is involved in cyanobacterial photoprotection. Its N-terminal domain (NTD) is responsible for interaction with the antenna and induction of excitation energy quenching, while the C-terminal domain is the regulatory domain that senses light and induces photoactivation. In most nitrogen-fixing cyanobacterial strains, there are one to four paralogous genes coding for homologs to the NTD of the OCP. The functions of these proteins are unknown. Here, we study the expression, localization, and function of these genes in Anabaena sp. PCC 7120. We show that the four genes present in the genome are expressed in both vegetative cells and heterocysts but do not seem to have an essential role in heterocyst formation. This study establishes that all four Anabaena NTD-like proteins can bind a carotenoid and the different paralogs have distinct functions. Surprisingly, only one paralog (All4941) was able to interact with the antenna and to induce permanent thermal energy dissipation. Two of the other Anabaena paralogs (All3221 and Alr4783) were shown to be very good singlet oxygen quenchers. The fourth paralog (All1123) does not seem to be involved in photoprotection. Structural homology modeling allowed us to propose specific features responsible for the different functions of these soluble carotenoid-binding proteins. C1 [Lopez-Igual, Rocio; Wilson, Adjele; de Carbon, Celine Bourcier; Kirilovsky, Diana] Univ Paris 11, Univ Paris Saclay, CEA, CNRS,Inst Integrat Biol Cell, F-91198 Gif Sur Yvette, France. [Lopez-Igual, Rocio; Wilson, Adjele; de Carbon, Celine Bourcier; Kirilovsky, Diana] CEA, Inst Biol & Technol Saclay iBiTec S, F-91191 Gif Sur Yvette, France. [Leverenz, Ryan L.; Sutter, Markus; Turmo, Aiko; Kerfeld, Cheryl A.] Michigan State Univ, MSU DOE Plant Res Lab, E Lansing, MI 48824 USA. [Leverenz, Ryan L.; Sutter, Markus; Turmo, Aiko; Kerfeld, Cheryl A.] Michigan State Univ, Dept Biochem & Mol Biol, E Lansing, MI 48824 USA. [Melnicki, Matthew R.; Kerfeld, Cheryl A.] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Melnicki, Matthew R.; Sutter, Markus; Kerfeld, Cheryl A.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Perreau, Francois] INRA, Inst Jean Pierre Bourgin, UMR 1318, ERL CNRS 3559,Saclay Plant Sci, F-78026 Versailles, France. [Lopez-Igual, Rocio] CNRS, Unite Mixte Rech 3525, Dept Genomes & Genet, Inst Pasteur,Unite Plasticite Genome Bacterien, F-75015 Paris, France. RP Kirilovsky, D (reprint author), Univ Paris 11, Univ Paris Saclay, CEA, CNRS,Inst Integrat Biol Cell, F-91198 Gif Sur Yvette, France.; Kirilovsky, D (reprint author), CEA, Inst Biol & Technol Saclay iBiTec S, F-91191 Gif Sur Yvette, France. EM diana.kirilovsky@cea.fr OI kerfeld, cheryl/0000-0002-9977-8482; Lopez-Igual, Rocio/0000-0002-2369-1583 FU Lidex BIG [ANR-11-IDEX-0003-02] FX We thank Sandrine Cot for technical assistance. We are indebted to Dr. Enrique Flores and Dr. Antonia Herrero (IBVF, Sevilla, Spain) for the generous gift of strain Anabaena sp. PCC 7120 and pRL277 plasmid and to Prof. Peter C. Wolk (Michigan State University) for the gift of E. coli strain ED8654. We thank Dr. Sebastian Aguilar (Pasteur Institut, Paris, France) for help with statistical analysis of qPCR data. We thank Laetitia Besse (beneficiary from a research grant supported by the Lidex BIG, ANR-11-IDEX-0003-02) for her expertise in live cell imaging and her help on image acquisitions. NR 58 TC 2 Z9 2 U1 4 U2 7 PU AMER SOC PLANT BIOLOGISTS PI ROCKVILLE PA 15501 MONONA DRIVE, ROCKVILLE, MD 20855 USA SN 0032-0889 EI 1532-2548 J9 PLANT PHYSIOL JI Plant Physiol. PD JUL PY 2016 VL 171 IS 3 BP 1852 EP 1866 DI 10.1104/pp.16.00502 PG 15 WC Plant Sciences SC Plant Sciences GA DT2IF UT WOS:000381303300029 PM 27208286 ER PT J AU Heuskin, AC Osseiran, AI Tang, J Costes, SV AF Heuskin, A. C. Osseiran, A. I. Tang, J. Costes, S. V. TI Simulating Space Radiation-Induced Breast Tumor Incidence Using Automata SO RADIATION RESEARCH LA English DT Article ID ATOMIC-BOMB SURVIVORS; CARCINOMA IN-SITU; IONIZING-RADIATION; CELLULAR SENESCENCE; CHROMOSOMAL INSTABILITY; MULTISTAGE MODELS; MENSTRUAL-CYCLE; DOSE-RESPONSE; CANCER-RISK; DNA-DAMAGE AB Estimating cancer risk from space radiation has been an ongoing challenge for decades primarily because most of the reported epidemiological data on radiation-induced risks are derived from studies of atomic bomb survivors who were exposed to an acute dose of gamma rays instead of chronic high-LET cosmic radiation. In this study, we introduce a formalism using cellular automata to model the long-term effects of ionizing radiation in human breast for different radiation qualities. We first validated and tuned parameters for an automata-based two-stage clonal expansion model simulating the age dependence of spontaneous breast cancer incidence in an unexposed U. S. population. We then tested the impact of radiation perturbation in the model by modifying parameters to reflect both targeted and nontargeted radiation effects. Targeted effects (TE) reflect the immediate impact of radiation on a cell's DNA with classic end points being gene mutations and cell death. They are well known and are directly derived from experimental data. In contrast, nontargeted effects (NTE) are persistent and affect both damaged and undamaged cells, are nonlinear with dose and are not well characterized in the literature. In this study, we introduced TE in our model and compared predictions against epidemiologic data of the atomic bomb survivor cohort. TE alone are not sufficient for inducing enough cancer. NTE independent of dose and lasting; 100 days postirradiation need to be added to accurately predict dose dependence of breast cancer induced by gamma rays. Finally, by integrating experimental relative biological effectiveness (RBE) for TE and keeping NTE (i. e., radiation-induced genomic instability) constant with dose and LET, the model predicts that RBE for breast cancer induced by cosmic radiation would be maximum at 220 keV/ lm. This approach lays the groundwork for further investigation into the impact of chronic low-dose exposure, inter-individual variation and more complex space radiation scenarios. (C) 2016 by Radiation Research Society C1 [Heuskin, A. C.; Osseiran, A. I.; Costes, S. V.] Lawrence Berkeley Natl Lab, Div Life Sci, 1 Cyclotron Rd,MS 977, Berkeley, CA 94720 USA. [Tang, J.] Exogen Biotechnol Inc, Berkeley, CA USA. [Heuskin, A. C.] Univ Namur, Res Ctr Phys Matter & Radiat PMR, NAmur Res Inst Life Sci NARILIS, Namur, Belgium. RP Costes, SV (reprint author), Lawrence Berkeley Natl Lab, Div Life Sci, 1 Cyclotron Rd,MS 977, Berkeley, CA 94720 USA. EM svcostes@lbl.gov FU Belgian American Education Foundation; Fulbright Commission; Walloon region of Belgium; National Aeronautics and Space Administration [NNL15AA08I] FX We thank Dr. Louise Viger for her constructive feedback on the manuscript. Support was provided by the Belgian American Education Foundation, the Fulbright Commission and the Walloon region of Belgium (ACH, postdoctoral fellow), as well as the National Aeronautics and Space Administration (grant no. NNL15AA08I awarded to SVC, JT and AO). NR 64 TC 0 Z9 0 U1 1 U2 1 PU RADIATION RESEARCH SOC PI LAWRENCE PA 810 E TENTH STREET, LAWRENCE, KS 66044 USA SN 0033-7587 EI 1938-5404 J9 RADIAT RES JI Radiat. Res. PD JUL PY 2016 VL 186 IS 1 BP 27 EP 38 DI 10.1667/RR14338.1 PG 12 WC Biology; Biophysics; Radiology, Nuclear Medicine & Medical Imaging SC Life Sciences & Biomedicine - Other Topics; Biophysics; Radiology, Nuclear Medicine & Medical Imaging GA DS5PT UT WOS:000380835200003 PM 27333083 ER PT J AU Pelly, S Winglee, K Xia, FF Stevens, RL Bishai, WR Lamichhane, G AF Pelly, Shaaretha Winglee, Kathryn Xia, Fangfang Stevens, Rick L. Bishai, William R. Lamichhane, Gyanu TI REMap: Operon map of M-tuberculosis based on RNA sequence data SO TUBERCULOSIS LA English DT Article DE Operon; Mycobacterium tuberculosis; RNAseq ID NITRATE REDUCTASE NARGHJI; POLYMORPHIC NUCLEOTIDE; GENE; IDENTIFICATION; PROMOTER; UNITS; TRANSCRIPTOME; PERSISTENCE; EXPRESSION; PREDICTION AB A map of the transcriptional organization of genes of an organism is a basic tool that is necessary to understand and facilitate a more accurate genetic manipulation of the organism. Operon maps are largely generated by computational prediction programs that rely on gene conservation and genome architecture and may not be physiologically relevant. With the widespread use of RNA sequencing (RNAseq), the prediction of operons based on actual transcriptome sequencing rather than computational genomics alone is much needed. Here, we report a validated operon map of Mycobacterium tuberculosis, developed using RNAseq data from both the exponential and stationary phases of growth. At least 58.4% of M. tuberculosis genes are organized into 749 operons. Our prediction algorithm, REMap (RNA Expression Mapping of operons), considers the many cases of transcription coverage of intergenic regions, and avoids dependencies on functional annotation and arbitrary assumptions about gene structure. As a result, we demonstrate that REMap is able to more accurately predict operons, especially those that contain long intergenic regions or functionally unrelated genes, than previous operon prediction programs. The REMap algorithm is publicly available as a user-friendly tool that can be readily modified to predict operons in other bacteria. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Pelly, Shaaretha; Winglee, Kathryn; Bishai, William R.; Lamichhane, Gyanu] Johns Hopkins Univ, Sch Med, Ctr TB Res, 1550 Orleans St, Baltimore, MD 21287 USA. [Xia, Fangfang; Stevens, Rick L.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. [Xia, Fangfang; Stevens, Rick L.] Univ Chicago, Chicago, IL 60637 USA. [Bishai, William R.] Johns Hopkins Univ, Sch Med, Ctr TB Res, Howard Hughes Med Inst, 1550 Orleans St, Baltimore, MD 21231 USA. RP Lamichhane, G (reprint author), Johns Hopkins Univ, Sch Med, Ctr TB Res, 1550 Orleans St, Baltimore, MD 21287 USA. EM lamichhane@jhu.edu OI Lamichhane, Gyanu/0000-0002-2214-0114 FU National Institutes of Health [DP2OD008459] FX This work was supported by the National Institutes of Health award DP2OD008459 to GL. NR 49 TC 0 Z9 0 U1 1 U2 1 PU CHURCHILL LIVINGSTONE PI EDINBURGH PA JOURNAL PRODUCTION DEPT, ROBERT STEVENSON HOUSE, 1-3 BAXTERS PLACE, LEITH WALK, EDINBURGH EH1 3AF, MIDLOTHIAN, SCOTLAND SN 1472-9792 J9 TUBERCULOSIS JI Tuberculosis PD JUL PY 2016 VL 99 BP 70 EP 80 DI 10.1016/j.tube.2016.04.010 PG 11 WC Immunology; Microbiology; Respiratory System SC Immunology; Microbiology; Respiratory System GA DS4MV UT WOS:000380756100011 PM 27450008 ER PT J AU Zhou, Y Bukusoglu, E Martinez-Gonzalez, JA Rahimi, M Roberts, TF Zhang, R Wang, XG Abbott, NL de Pablo, JJ AF Zhou, Ye Bukusoglu, Emre Martinez-Gonzalez, Jose A. Rahimi, Mohammad Roberts, Tyler F. Zhang, Rui Wang, Xiaoguang Abbott, Nicholas L. de Pablo, Juan J. TI Structural Transitions in Cholesteric Liquid Crystal Droplets SO ACS NANO LA English DT Article DE ChLC; liquid crystal; Landau-de Gennes model; chirality AB Confinement of cholesteric liquid crystals (ChLC) into droplets leads to a delicate interplay between elasticity, chirality, and surface energy. In this work, we rely on a combination of theory and experiments to understand the rich morphological behavior that arises from that balance. More specifically, a systematic study of micrometer-sized ChLC droplets is presented as a function of chirality and surface energy (or anchoring). With increasing chirality, a continuous transition is observed from a twisted bipolar structure to a radial spherical structure, all within a narrow range of chirality. During such a transition, a bent structure is predicted by simulations and confirmed by experimental observations. Simulations are also able to capture the dynamics of the quenching process observed in experiments. Consistent with published work, it is found that nanoparticles are attracted to defect regions on the surface of the droplets. For weak anchoring conditions at the nanoparticle surface, ChLC droplets adopt a morphology similar to that of the equilibrium helical phase observed for ChLCs in the bulk. As the anchoring strength increases, a planar bipolar structure arises, followed by a morphological transition to a bent structure. The influence of chirality and surface interactions are discussed in the context of the potential use of ChLC droplets as stimuli-responsive materials for reporting molecular adsorbates. C1 [Zhou, Ye; Martinez-Gonzalez, Jose A.; Rahimi, Mohammad; Roberts, Tyler F.; Zhang, Rui; de Pablo, Juan J.] Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA. [Bukusoglu, Emre; Wang, Xiaoguang; Abbott, Nicholas L.] Univ Wisconsin, Dept Chem & Biol Engn, Madison, WI 53706 USA. [de Pablo, Juan J.] Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. RP de Pablo, JJ (reprint author), Univ Chicago, Inst Mol Engn, Chicago, IL 60637 USA.; de Pablo, JJ (reprint author), Argonne Natl Lab, 9700 S Cass Ave, Argonne, IL 60439 USA. EM depablo@uchicago.edu OI Martinez-Gonzalez, Jose Adrian/0000-0001-7257-8889; Wang, Xiaoguang/0000-0002-4079-9596 FU Department of Energy, Basic Energy Sciences, Division of Materials Research, Biomaterials Program [DE-SC0004025] FX The authors acknowledge support from the Department of Energy, Basic Energy Sciences, Division of Materials Research, Biomaterials Program under Grant No. DE-SC0004025. NR 27 TC 5 Z9 5 U1 35 U2 45 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2016 VL 10 IS 7 BP 6484 EP 6490 DI 10.1021/acsnano.6b01088 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DS2FD UT WOS:000380576600010 PM 27249186 ER PT J AU Amani, M Burke, RA Ji, X Zhao, P Lien, DH Taheri, P Ahn, GH Kirya, D Ager, JW Yablonovitch, E Kong, J Dubey, M Jayey, A AF Amani, Matin Burke, Robert A. Ji, Xiang Zhao, Peida Lien, Der-Hsien Taheri, Peyman Ahn, Geun Ho Kirya, Daisuke Ager, Joel W., III Yablonovitch, Eli Kong, Jing Dubey, Madan Jayey, Ali TI High Luminescence Efficiency in MoS2 Grown by Chemical Vapor Deposition SO ACS NANO LA English DT Article DE transition metal dichalcogenide; MoS2; chemical vapor deposition; quantum yield; radiative lifetime; biexcitonic recombination ID TRANSITION-METAL DICHALCOGENIDES; MONOLAYER MOLYBDENUM-DISULFIDE; ATOMIC LAYERS; DOUBLE HETEROSTRUCTURES; SPONTANEOUS EMISSION; BAND-GAP; PHOTOLUMINESCENCE; TRANSPORT; GRAPHENE; WS2 AB One of the major challenges facing the rapidly growing field of two-dimensional (2D) transition metal dichalcogenides (TMDCs) is the development of growth techniques to enable large area synthesis of high-quality materials. Chemical vapor deposition (CVD) is one of the leading techniques for the synthesis of TMDCs; however, the quality of the material produced is limited by defects formed during the growth process. A very useful nondestructive technique that can be utilized to probe defects in semiconductors is the room-temperature photoluminescence (PL) quantum yield (QY). It was recently demonstrated that a PL QY near 100% can be obtained in MoS2 and WS2 monolayers prepared by micromechanical exfoliation by treating samples with an organic superacid: bis(trifluoromethane)sulfonimide (TFSI). Here we have performed a thorough exploration of this chemical treatment on CVD-grown MoS2 samples. We find that the as-grown monolayers must be transferred to a secondary substrate, which releases strain, to obtain high QY by TFSI treatment. Furthermore, we find that the sulfur precursor temperature during synthesis of the MoS2 plays a critical role in the effectiveness of the treatment. By satisfying the aforementioned conditions we show that the PL QY of CVD-grown monolayers can be improved from similar to 0.1% in the as-grown case to similar to 30% after treatment, with enhancement factors ranging from 100 to 1500x depending on the initial monolayer quality. We also found that after TFSI treatment the PL emission from MoS2 films was visible by eye despite the low absorption (5-10%). The discovery of an effective passivation strategy will speed the development of scalable high-performance optoelectronic and electronic devices based on MoS2. C1 [Amani, Matin; Zhao, Peida; Lien, Der-Hsien; Taheri, Peyman; Ahn, Geun Ho; Kirya, Daisuke; Yablonovitch, Eli; Jayey, Ali] Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Amani, Matin; Zhao, Peida; Lien, Der-Hsien; Ahn, Geun Ho; Kirya, Daisuke; Ager, Joel W., III; Yablonovitch, Eli; Jayey, Ali] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Burke, Robert A.; Dubey, Madan] US Army Res Lab, 2800 Powder Mill Rd, Adelphi, MD 20783 USA. [Ji, Xiang; Kong, Jing] MIT, Elect Engn & Comp Sci, 77 Mass Ave, Cambridge, MA 02139 USA. RP Jayey, A (reprint author), Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA.; Jayey, A (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM ajavey@berkeley.edu FU Electronic Materials Program - Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231]; NSF Center for Energy Efficient Electronics Science (E3S); U.S. Army Research Lab; Center for Excitonics, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences (BES) [DE-SC0001088]; NWO-Rubicon; Office of Science of the U.S. Department of Energy [DE-SC0004993] FX M.A., J.W.A., and A.J. were supported by the Electronic Materials Program, funded by Director, Office of Science, Office of Basic Energy Sciences, Materials Sciences and Engineering Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. P.Z., E.Y., J.K., and A.J. acknowledge support from the NSF Center for Energy Efficient Electronics Science (E3S). R.A.B. and M.D. acknowledge support from the U.S. Army Research Lab Director's Strategic Initiative program on interfaces in stacked 2D atomic layers and materials. X.J. acknowledges support from the Center for Excitonics, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Basic Energy Sciences (BES), under award number DE-SC0001088. P.T. was supported by a fellowship awarded by NWO-Rubicon. Raman spectroscopy was performed in collaboration with the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award Number DE-SC0004993. NR 41 TC 9 Z9 9 U1 69 U2 119 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2016 VL 10 IS 7 BP 6535 EP 6541 DI 10.1021/acsnano.6603443 PG 7 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DS2FD UT WOS:000380576600016 PM 27291297 ER PT J AU Schiros, T Nordlund, D Palova, L Zhao, LY Levendorf, M Jaye, C Reichman, D Park, J Hybertsen, M Pasupathy, A AF Schiros, Theanne Nordlund, Dennis Palova, Lucia Zhao, Liuyan Levendorf, Mark Jaye, Cherno Reichman, David Park, Jiwoong Hybertsen, Mark Pasupathy, Abhay TI Atomistic Interrogation of B-N Co-dopant Structures and Their Electronic Effects in Graphene SO ACS NANO LA English DT Article DE graphene; doping; X-ray spectroscopy; scanning tunneling microscopy; chemical bonding; atomic design; electronic structure; work function ID NITROGEN-DOPED GRAPHENE; CHEMICAL-VAPOR-DEPOSITION; HEXAGONAL BORON-NITRIDE; X-RAY-ABSORPTION; SCANNING TUNNELING MICROSCOPE; THIN-FILMS; MONOLAYER GRAPHENE; BAND-GAP; SPECTROSCOPY; CARBON AB Chemical doping has been demonstrated to be an effective method for producing high-quality, large-area graphene with controlled carrier concentrations and an atomically tailored work function. The emergent optoelectronic properties and surface reactivity of carbon nanostructures are dictated by the microstructure of atomic dopants. Co doping of graphene with boron and nitrogen offers the possibility to further tune the electronic properties of graphene at the atomic level, potentially creating p- and n-type domains in a single carbon sheet, opening a gap between valence and conduction bands in the 2-D semimetal. Using a suite of high-resolution synchrotron-based X-ray techniques, scanning tunneling microscopy, and density functional theory based computation we visualize and characterize B-N dopant bond structures and their electronic effects at the atomic level in single-layer graphene grown on a copper substrate. We find there is a thermodynamic driving force for B and N atoms to cluster into BNC structures in graphene, rather than randomly distribute into isolated B and N graphitic dopants, although under the present growth conditions, kinetics limit segregation of large B N domains. We observe that the doping effect of these BNC structures, which open a small band gap in graphene, follows the B:N ratio (B > N, p-type; B < N, n-type; B=N, neutral). We attribute this to the comparable electron-withdrawing and-donating effects, respectively, of individual graphitic B and N dopants, although local electrostatics also play a role in the work function change. C1 [Schiros, Theanne] Columbia Univ, MRSEC, New York, NY 10027 USA. [Palova, Lucia; Reichman, David] Columbia Univ, Dept Chem, New York, NY 10027 USA. [Zhao, Liuyan; Pasupathy, Abhay] Columbia Univ, Dept Phys, New York, NY 10027 USA. [Schiros, Theanne] SUNY Fashion Inst Technol, Department Sci & Math, New York, NY 10001 USA. [Nordlund, Dennis] SLAC Natl Accelerator Lab, Stanford Synchrotron Radiat Lightsource, Menlo Pk, CA 94025 USA. [Levendorf, Mark; Park, Jiwoong] Cornell Univ, Dept Chem, Ithaca, NY 10065 USA. [Jaye, Cherno] NIST, Mat Measurement Lab, Gaithersburg, MD 20899 USA. [Hybertsen, Mark] Brookhaven Natl Lab, Ctr Funct Nanomat, Upton, NY 11973 USA. RP Schiros, T (reprint author), Columbia Univ, MRSEC, New York, NY 10027 USA.; Schiros, T (reprint author), SUNY Fashion Inst Technol, Department Sci & Math, New York, NY 10001 USA. EM ts2526@columbia.edu FU NSF MRSEC program through Columbia in the Center for Precision Assembly of Superstratic and Superatomic Solids [DMR-1420634]; U.S. DOE Office of Science Facilities, at Brookhaven National Laboratory [DE-SC0012704]; Office of Naval Research [N00014-14-1-0501]; Air Force Office of Scientific Research (AFOSR) [FA9530-11-1-0010] FX Research was supported by the NSF MRSEC program through Columbia in the Center for Precision Assembly of Superstratic and Superatomic Solids (DMR-1420634). NEXAFS, XPS, and photoemission threshold (work function) experiments were performed at beamline 10-1 at the Stanford Synchrotron Radiation Laboratory, a national user facility operated by Stanford University on behalf of the U.S. Department of Energy, Office of Basic Energy Sciences (T.S., D.N.). Additional NEXAFS experiments were also carried out at beamline U7A at the National Synchrotron Light Source, and theory and computations were carried out in part at the Center for Functional Nanomaterials, both of which are U.S. DOE Office of Science Facilities, at Brookhaven National Laboratory; under Contract No. DE-SC0012704 (M.H., C.J., T.S.). STM experiments were supported by the Office of Naval Research (award number N00014-14-1-0501) and by the Air Force Office of Scientific Research (AFOSR) (award number FA9530-11-1-0010) (L.Z., A.N.P.). Theoretical calculations were performed by L.P., D.R., and M.H. Sample growth was performed by M.L. and J.P. NR 69 TC 0 Z9 0 U1 27 U2 49 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2016 VL 10 IS 7 BP 6574 EP 6584 DI 10.1021/acsnano.6b01318 PG 11 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DS2FD UT WOS:000380576600020 PM 27327863 ER PT J AU Wang, K Huang, B Tian, M Ceballos, F Lin, MW Mahjouri-Samani, M Boulesbaa, A Puretzky, AA Rouleau, CM Yoon, M Zhao, H Xiao, K Duscher, G Geohegan, DB AF Wang, Kai Huang, Bing Tian, Mengkun Ceballos, Frank Lin, Ming-Wei Mahjouri-Samani, Masoud Boulesbaa, Abdelaziz Puretzky, Alexander A. Rouleau, Christopher M. Yoon, Mina Zhao, Hui Xiao, Kai Duscher, Gerd Geohegan, David B. TI Interlayer Coupling in Twisted WSe2/WS2 Bilayer Heterostructures Revealed by Optical Spectroscopy SO ACS Nano LA English DT Article DE van der Waals heterostructures; interlayer coupling; twist angle; charge transfer ID SINGLE-LAYER MOS2; MOLYBDENUM-DISULFIDE; MONOLAYER MOS2; ELECTRONIC-STRUCTURE; CHARGE-TRANSFER; MONO; WS2; PHOTOLUMINESCENCE; EVOLUTION; PIEZOELECTRICITY AB van der Waals (vdW) heterostructures are promising building blocks for future ultrathin electronics. Fabricating vdW heterostructures by stamping monolayers at arbitrary angles provides an additional range of flexibility to tailor the resulting properties than could be expected by direct growth. Here, we report fabrication and comprehensive characterizations of WSe2/WS2 bilayer heterojunctions with various twist angles that were synthesized by artificially stacking monolayers of WS2 and WSe2 grown by chemical vapor deposition. After annealing the WSe2/WS2 bilayers, Raman spectroscopy reveals interlayer coupling with the appearance of a mode at 309.4 cm(-1) that is sensitive to the number of WSe2 layers. This interlayer coupling is associated with substantial quenching of the intralayer photoluminescence. In addition, microabsorption spectroscopy of WSe2/WS2 bilayers revealed spectral broadening and shifts as well as a net similar to 10% enhancement in integrated absorption strength across the visible spectrum with respect to the sum of the individual monolayer spectra. The observed broadening of the WSe2 A exciton absorption band in the bilayers suggests fast charge separation between the layers, which was supported by direct femtosecond pump-probe spectroscopy. Density functional calculations of the band structures of the bilayers at different twist angles and interlayer distances found robust type II heterojunctions at all twist angles, and predicted variations in band gap for particular atomistic arrangements. Although interlayer excitons were indicated using femtosecond pump-probe spectroscopy, photoluminescence and absorption spectroscopies did not show any evidence of them, suggesting that the interlayer exciton transition is very weak. However, the interlayer coupling for the WSe2/WS2 bilayer heterojunctions indicated by substantial PL quenching, enhanced absorption, and rapid charge transfer was found to be insensitive to the relative twist angle, indicating that stamping provides a robust approach to realize reliable optoelectronics. C1 [Wang, Kai; Huang, Bing; Lin, Ming-Wei; Mahjouri-Samani, Masoud; Boulesbaa, Abdelaziz; Puretzky, Alexander A.; Rouleau, Christopher M.; Yoon, Mina; Xiao, Kai; Geohegan, David B.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Huang, Bing] Beijing Computat Sci Res Ctr, Beijing 100094, Peoples R China. [Huang, Bing] Univ Utah, Dept Mat Sci & Engn, Salt Lake City, UT 84112 USA. [Tian, Mengkun; Duscher, Gerd] Univ Tennessee, Dept Mat Sci & Engn, Knoxville, TN 37996 USA. [Zhao, Hui] Univ Kansas, Dept Phys & Astron, Lawrence, KS 66045 USA. RP Wang, K; Geohegan, DB (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. EM wangk@ornl.gov; geohegandb@ornl.gov RI Zhao, Hui/A-2703-2009; Wang, Kai/H-4361-2011; Geohegan, David/D-3599-2013; Duscher, Gerd/G-1730-2014 OI Zhao, Hui/0000-0003-4552-3836; Wang, Kai/0000-0002-6405-7837; Geohegan, David/0000-0003-0273-3139; Duscher, Gerd/0000-0002-2039-548X FU U.S. Department of Energy, Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division; U.S. Department of Energy [DE-AC05-00OR22725] FX Research was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences (BES), Materials Sciences and Engineering Division, and performed in part as a user project at the Center for Nanophase Materials Sciences (CNMS), which is a DOE Office of Science User Facility. Characterization techniques and spectroscopic facilities at CNMS developed through the CNMS theme science program. K.W. thanks Dr. Ying-Zhong Ma for his suggestion on exciton dynamics studies. This article has been authored by UT-Battelle, LLC, under Contract No. DE-AC05-00OR22725 with the U.S. Department of Energy. The United States Government retains and the publisher, by accepting the article for publication, acknowledges that the United States Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this article, or allow others to do so, for United States Government purposes. The Department of Energy will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan (http://energy.gov/downloads/doe-public-access-plan). NR 60 TC 6 Z9 6 U1 51 U2 79 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2016 VL 10 IS 7 BP 6612 EP 6622 DI 10.1021/acsnano.6b01486 PG 11 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DS2FD UT WOS:000380576600023 PM 27309275 ER PT J AU Holt, AP Bocharova, V Cheng, SW Kisliuk, AM White, BT Saito, T Uhrig, D Mahalik, JP Kumar, R Imel, AE Etampawala, T Martin, H Sikes, N Sumpter, BG Dadmun, MD Sokolov, AP AF Holt, Adam P. Bocharova, Vera Cheng, Shiwang Kisliuk, Alexander M. White, B. Tyler Saito, Tomonori Uhrig, David Mahalik, J. P. Kumar, Rajeev Imel, Adam E. Etampawala, Thusitha Martin, Halie Sikes, Nicole Sumpter, Bobby G. Dadmun, Mark D. Sokolov, Alexei P. TI Controlling Interfacial Dynamics: Covalent Bonding versus Physical Adsorption in Polymer Nanocomposites SO ACS NANO LA English DT Article DE polymer nanocomposites; polymer-grafted nanoparticles; glass transition; segmental dynamics; interfacial dynamics; self-consistent field theory ID MOLECULAR-DYNAMICS; GLASS-TRANSITION; SPHERICAL NANOPARTICLES; IMMOBILIZED POLYMER; SEGMENTAL DYNAMICS; COOPERATIVE MOTION; MODEL; FILMS; FRAGILITY; BRUSHES AB It is generally believed that the strength of the polymer-nanoparticle interaction controls the modification of near-interface segmental mobility in polymer nanocomposites (PNCs). However, little is known about the effect of covalent bonding on the segmental dynamics and glass transition of matrix-free polymer-grafted nanoparticles (PGNs), especially when compared to PNCs. In this article, we directly compare the static and dynamic properties of poly(2-vinylpyridine)/silica-based nanocomposites with polymer chains either physically adsorbed (PNCs) or covalently bonded (PGNs) to identical silica nanoparticles (R-NP = 12.5 nm) for three different molecular weight (MW) systems. Interestingly, when the MW of the matrix is as low as 6 kg/mol (R-NP/R-g = 5.4) or as high as 140 kg/mol (R-NP/R-g = 1.13), both small-angle X-ray scattering and broadband dielectric spectroscopy show similar static and dynamic properties for PNCs and PGNs. However, for the intermediate MW of 18 kg/mol (R-NP/R-g = 3.16), the difference between physical adsorption and covalent bonding can be clearly identified in the static and dynamic properties of the interfacial layer. We ascribe the differences in the interfacial properties of PNCs and PGNs to changes in chain stretching, as quantified by self-consistent field theory calculations. These results demonstrate that the dynamic suppression at the interface is affected by the chain stretching; that is, it depends on the anisotropy of the segmental conformations, more so than the strength of the interaction, which suggests that the interfacial dynamics can be effectively tuned by the degree of stretching-a parameter accessible from the MW or grafting density. C1 [Holt, Adam P.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Imel, Adam E.; Etampawala, Thusitha; Martin, Halie; Dadmun, Mark D.; Sokolov, Alexei P.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Bocharova, Vera; Cheng, Shiwang; Kisliuk, Alexander M.; White, B. Tyler; Saito, Tomonori; Dadmun, Mark D.; Sokolov, Alexei P.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Uhrig, David; Mahalik, J. P.; Kumar, Rajeev; Sumpter, Bobby G.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Mahalik, J. P.; Kumar, Rajeev; Sumpter, Bobby G.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Sikes, Nicole] Columbus State Univ, Dept Chem, Columbus, GA USA. RP Holt, AP (reprint author), Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA.; Bocharova, V (reprint author), Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. EM aholt19@vols.utk.edu; bocharovav@ornl.gov RI Kumar, Rajeev/Q-2255-2015; Sumpter, Bobby/C-9459-2013; OI Kumar, Rajeev/0000-0001-9494-3488; Sumpter, Bobby/0000-0001-6341-0355; Dadmun, Mark/0000-0003-4304-6087 FU U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy; NSF-REU summer program at the University of Tennessee [CHE-1262767] FX We thank Ken Schweizer and Eileen Buenning for many useful and insightful discussions. This work was supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. We also acknowledge the support of the Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy, who sponsors the Center for Nanophase Materials Sciences (CNMS) at Oak Ridge National Laboratory. N.S. thanks the NSF-REU summer program (CHE-1262767) at the University of Tennessee for the opportunity to work on this project. NR 55 TC 10 Z9 10 U1 42 U2 60 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2016 VL 10 IS 7 BP 6843 EP 6852 DI 10.1021/acsnano.6b02501 PG 10 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DS2FD UT WOS:000380576600049 PM 27337392 ER PT J AU Tosun, M Chan, L Amani, M Roy, T Ahn, GH Taheri, P Carraro, C Ager, JW Maboudian, R Javey, A AF Tosun, Mahmut Chan, Leslie Amani, Matin Roy, Tania Ahn, Geun Ho Taheri, Peyman Carraro, Carlo Ager, Joel W. Maboudian, Roya Javey, Ali TI Air-Stable n-Doping of WSe2 by Anion Vacancy Formation with Mild Plasma Treatment SO ACS Nano LA English DT Article DE transition metal dichalcogenides; defect engineering; air stable doping; WSe2; vacancy formation ID TRANSITION-METAL DICHALCOGENIDES; FIELD-EFFECT TRANSISTORS; PROBE FORCE MICROSCOPY; MOS2 TRANSISTORS; 2-DIMENSIONAL SEMICONDUCTORS; LAYER MOS2; CONTACTS; DEFECTS; PHOTOLUMINESCENCE; DIODES AB Transition metal dichalcogenides (TMDCs) have been extensively explored for applications in electronic and optoelectronic devices due to their unique material properties. However, the presence of large contact resistances is still a fundamental challenge in the field. In this work, we study defect engineering by using a mild plasma treatment (He or H-2) as an approach to reduce the contact resistance to WSe2. Material characterization by X-ray photoelectron spectroscopy, photoluminescence, and Kelvin probe force microscopy confirm defect-induced n-doping, up to degenerate level, which is attributed to the creation of anion (Se) vacancies. The plasma treatment is adopted in the fabrication process flow of WSe2 n-type metal-oxide-semiconductor field-effect transistors to selectively create anion vacancies at the metal contact regions. Due to lowering the metal contact resistance, improvements in the device performance metrics such as a 20x improvement in ON current and a nearly ideal subthreshold swing value of 66 mV/dec are observed. This work demonstrates that defect engineering at the contact regions can be utilized as a reliable scheme to realize high-performance electronic and optoelectronic TMDC devices. C1 [Tosun, Mahmut; Amani, Matin; Roy, Tania; Ahn, Geun Ho; Taheri, Peyman; Javey, Ali] Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Tosun, Mahmut; Chan, Leslie; Amani, Matin; Roy, Tania; Ahn, Geun Ho; Taheri, Peyman; Carraro, Carlo; Maboudian, Roya; Javey, Ali] Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94720 USA. [Chan, Leslie; Carraro, Carlo; Maboudian, Roya] Univ Calif Berkeley, Dept Chem & Biomol Engn, Berkeley, CA 94720 USA. [Tosun, Mahmut; Amani, Matin; Roy, Tania; Ahn, Geun Ho; Ager, Joel W.; Javey, Ali] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Javey, A (reprint author), Univ Calif Berkeley, Elect Engn & Comp Sci, Berkeley, CA 94720 USA.; Javey, A (reprint author), Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94720 USA.; Javey, A (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. EM ajavey@eecs.berkeley.edu FU Office of Science, Office of Basic Energy Sciences, Material Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231] FX This work was funded by the Director, Office of Science, Office of Basic Energy Sciences, Material Sciences and Engineering Division of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. We thank Mayur Savla of Bruker Nano for the PeakForce KPFM measurements performed using the Dimension Icon AFM. NR 34 TC 2 Z9 2 U1 25 U2 37 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2016 VL 10 IS 7 BP 6853 EP 6860 DI 10.1021/acsnano.6b02521 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DS2FD UT WOS:000380576600050 PM 27294286 ER PT J AU Pinchetti, V Meinardi, F Camellini, A Sirigu, G Christodoulou, S Bae, WK De Donato, F Manna, L Zavelani-Rossi, M Moreels, I Klimov, VI Brovelli, S AF Pinchetti, Valerio Meinardi, Francesco Camellini, Andrea Sirigu, Gianluca Christodoulou, Sotirios Bae, Wan Ki De Donato, Francesco Manna, Liberato Zavelani-Rossi, Margherita Moreels, Iwan Klimov, Victor I. Brovelli, Sergio TI Effect of Core/Shell Interface on Carrier Dynamics and Optical Gain Properties of Dual-Color Emitting CdSe/CdS Nanocrystals SO ACS Nano LA English DT Article DE nanocrystal quantum dots; core/shell heterostructures; dual emission; interface structure; exciton dynamics; amplified spontaneous emission ID IN-BULK NANOCRYSTALS; HETEROSTRUCTURED QUANTUM DOTS; CORE-SHELL INTERFACE; SEMICONDUCTOR NANOCRYSTALS; AUGER RECOMBINATION; SEEDED GROWTH; ELECTRONIC-STRUCTURE; REDOX POTENTIALS; 2-COLOR QUANTUM; EMISSION AB Two-color emitting colloidal semiconductor nanocrystals (NCs) are of interest for applications in multimodal imaging, sensing, lighting, and integrated photonics. Dual color emission from core- and shell-related optical transitions has been recently obtained using so-called dot-in-bulk (DiB) CdSe/CdS NCs comprising a quantum-confined CdSe core embedded into an ultrathick (similar to 7-9 nm) CdS shell. The physical mechanism underlying this behavior is still under debate. While a large shell volume appears to be a necessary condition for dual emission, comparison between various types of thick-shell CdSe/CdS NCs indicates a critical role of the interface "sharpness" and the presence of potential barriers. To elucidate the effect of the interface morphology on the dual emission, we perform side-by-side studies of CdSe/CdS DiB-NCs with nominally identical core and shell dimensions but different structural properties of the core/shell interface arising from the crystal structure of the starting CdSe cores (zincblende vs wurtzite). While both structures exhibit dual emission under comparable pump intensities, NCs with a zincblende core show a faster growth of shell luminescence with excitation fluence and a more readily realized regime of amplified spontaneous emission (ASE) even under "slow" nanosecond excitation. These distinctions can be linked to the structure of the core/shell interface: NCs grown from the zincblende cores contain a similar to 3.5 nm thick zincblende CdS interlayer, which separates the core from the wurtzite CdS shell and creates a potential barrier for photoexcited shell holes inhibiting their relaxation into the core. This helps maintain a higher population of shell states and simplifies the realization of dual emission and ASE involving shell-based optical transitions. C1 [Pinchetti, Valerio; Meinardi, Francesco; Brovelli, Sergio] Univ Milano Bicocca, Dipartimento Sci Mat, Via Cozzi 55, IT-20125 Milan, Italy. [Camellini, Andrea; Sirigu, Gianluca] Politecn Milan, Dipartimento Fis, Piazza Leonardo da Vinci 32, IT-20133 Milan, Italy. [Christodoulou, Sotirios; De Donato, Francesco; Manna, Liberato; Moreels, Iwan] Ist Italiano Tecnol, Via Morego 30, IT-16163 Genoa, Italy. [Zavelani-Rossi, Margherita] Politecn Milan, Dipartimento Energia, Via Ponzio 34-3, IT-20133 Milan, Italy. [Zavelani-Rossi, Margherita] Inst Photon & Nanotechnol IFN CNR, Piazza Leonardo da Vinci 32, IT-20133 Milan, Italy. [Bae, Wan Ki; Klimov, Victor I.] Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. RP Brovelli, S (reprint author), Univ Milano Bicocca, Dipartimento Sci Mat, Via Cozzi 55, IT-20125 Milan, Italy.; Moreels, I (reprint author), Ist Italiano Tecnol, Via Morego 30, IT-16163 Genoa, Italy.; Klimov, VI (reprint author), Los Alamos Natl Lab, Div Chem, Los Alamos, NM 87545 USA. EM iwan.moreels@iit.it; klimov@lanl.gov; sergio.brovelli@unimib.it RI Manna, Liberato/G-2339-2010; Zavelani-Rossi, Margherita/H-2121-2012; Moreels, Iwan/E-5230-2011; OI Manna, Liberato/0000-0003-4386-7985; Zavelani-Rossi, Margherita/0000-0001-9910-0391; Moreels, Iwan/0000-0003-3998-7618; Klimov, Victor/0000-0003-1158-3179 FU Fondazione Cariplo [2012-0844, 2012-0824]; Chemical Sciences, Biosciences and Geosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy; European Community [324603] FX Financial support from Fondazione Cariplo is acknowledged by S.B. and F.M. through grant no. 2012-0844 and by G.S and M.Z.-R. through grant no. 2012-0824. V.I.K. and W.K.B. were supported by the Chemical Sciences, Biosciences and Geosciences Division, Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy. S.B. wishes to thank the European Community's Seventh Framework Programme (FP7/2007-2013) under grant agreement no. 324603 for financial support (EDONHIST). G.S. and M.Z.-R. acknowledge COST Action MP1302-NanoSpectroscopy. NR 61 TC 10 Z9 10 U1 16 U2 31 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2016 VL 10 IS 7 BP 6877 EP 6887 DI 10.1021/acsnano.6b02635 PG 11 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DS2FD UT WOS:000380576600053 PM 27276033 ER PT J AU Carrillo, JMY Seibers, Z Kumar, R Matheson, MA Ankner, JR Goswami, M Bhaskaran-Nair, K Shelton, WA Sumpter, BG Kilbey, SM AF Carrillo, Jan-Michael Y. Seibers, Zach Kumar, Rajeev Matheson, Michael A. Ankner, John R. Goswami, Monojoy Bhaskaran-Nair, Kiran Shelton, William A. Sumpter, Bobby G. Kilbey, S. Michael, II TI Petascale Simulations of the Morphology and the Molecular Interface of Bulk Heterojunctions SO ACS Nano LA English DT Article DE bulk heterojunction; organic photovoltaics; petascale simulations; neutron reflectometry; molecular dynamics simulations; coupled-cluster methods; donor/acceptor interface ID COUPLED-CLUSTER METHOD; CONNECTED TRIPLE EXCITATIONS; VERTICAL PHASE-SEPARATION; SOLAR-CELLS; ORGANIC PHOTOVOLTAICS; COPOLYMER COMPATIBILIZERS; METATHESIS POLYMERIZATION; ELECTRON-ATTACHMENT; GRIGNARD METATHESIS; P3HTPCBM INTERFACE AB Understanding how additives interact and segregate within bulk heterojunction (BHJ) thin films is critical for exercising control over structure at multiple length scales and delivering improvements in photovoltaic performance. The morphological evolution of poly(3-hexylthiophene) (P3HT) and phenyl-C-61- butyric acid methyl ester (PCBM) blends that are commensurate with the size of a BHJ thin film is examined using petascale coarse-grained molecular dynamics simulations. Comparisons between two-component and three-component systems containing short P3HT chains as additives undergoing thermal annealing demonstrate that the short chains alter the morphology in apparently useful ways: they efficiently migrate to the P3HT/PCBM interface, increasing the P3HT domain size and interfacial area. Simulation results agree with depth profiles determined from neutron reflectometry measurements that reveal PCBM enrichment near substrate and air interfaces but a decrease in that PCBM enrichment when a small amount of short P3HT chains are integrated into the BHJ blend. Atomistic simulations of the P3HT/PCBM blend interfaces show a nonmonotonic dependence of the interfacial thickness as a function of number of repeat units in the oligomeric P3HT additive, and the thiophene rings orient parallel to the interfacial plane as they approach the PCBM domain. Using the nanoscale geometries of the P3HT oligomers, LUMO and HOMO energy levels calculated by density functional theory are found to be invariant across the donor/acceptor interface. These connections between additives, processing, and morphology at all length scales are generally useful for efforts to improve device performance. C1 [Carrillo, Jan-Michael Y.; Kumar, Rajeev; Goswami, Monojoy; Sumpter, Bobby G.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Carrillo, Jan-Michael Y.; Kumar, Rajeev; Goswami, Monojoy; Sumpter, Bobby G.] Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA. [Matheson, Michael A.] Oak Ridge Natl Lab, Natl Ctr Computat Sci, Oak Ridge, TN 37831 USA. [Ankner, John R.] Oak Ridge Natl Lab, Spallat Neutron Source, Oak Ridge, TN 37831 USA. [Seibers, Zach] Univ Tennessee, Dept Energy Sci & Engn, Knoxville, TN 37996 USA. [Kilbey, S. Michael, II] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Kilbey, S. Michael, II] Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. [Bhaskaran-Nair, Kiran; Shelton, William A.] Louisiana State Univ, Ctr Computat & Technol, Baton Rouge, LA 70803 USA. [Bhaskaran-Nair, Kiran; Shelton, William A.] Louisiana State Univ, Cain Dept Chem Engn, Baton Rouge, LA 70803 USA. RP Carrillo, JMY (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.; Carrillo, JMY (reprint author), Oak Ridge Natl Lab, Comp Sci & Math Div, Oak Ridge, TN 37831 USA.; Kilbey, SM (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA.; Kilbey, SM (reprint author), Univ Tennessee, Dept Chem & Biomol Engn, Knoxville, TN 37996 USA. EM carrillojy@ornl.gov; mkilbey@utk.edu RI Kumar, Rajeev/Q-2255-2015; Sumpter, Bobby/C-9459-2013 OI Kumar, Rajeev/0000-0001-9494-3488; Sumpter, Bobby/0000-0001-6341-0355 FU Office of Science of the U.S. Department of Energy (DoE) [DE-AC05-00OR22725]; ORNL by the Scientific User Facilities Division, Office of Basic Energy Sciences (BES), U.S. DoE; National Science Foundation [EPS 1004083, 1512221]; U.S. DoE, BES, Materials Science and Engineering Division (MSED); U.S. DoE under EPSCoR Grant [DE-SC0012432]; Louisiana Board of Regents FX We thank C. Rycroft for assistance with radical Voronoi analysis using MPI and Voro++, A.V. Dobrynin for assistance with the development of the substrate-BHJ interactions, T.D. Nguyen and W.M. Brown for assistance with LAMMPS MD code, and M. Chen for assistance with NWChem code. This research used resources of the Oak Ridge Leadership Computing Facility at the Oak Ridge National Laboratory (ORNL), which is supported by the Office of Science of the U.S. Department of Energy (DoE) under Contract No. DE-AC05-00OR22725. This research was conducted in part at the Center for Nanophase Materials Sciences (CNMS) and at the Spoliation Neutron Source (SNS), which are sponsored at ORNL by the Scientific User Facilities Division, Office of Basic Energy Sciences (BES), U.S. DoE. Experimental work of Z.S. and S.M.K. was sponsored by National Science Foundation under Award No. EPS 1004083 and Award No. 1512221. M.G. and J.-M.Y.C. acknowledge support by the U.S. DoE, BES, Materials Science and Engineering Division (MSED). The computational work conducted by K.B.-N. and W.A.S. is supported by the U.S. DoE under EPSCoR Grant No. DE-SC0012432 with additional support from the Louisiana Board of Regents. NR 80 TC 1 Z9 1 U1 5 U2 13 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2016 VL 10 IS 7 BP 7008 EP 7022 DI 10.1021/acsnano.6b03009 PG 15 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DS2FD UT WOS:000380576600067 PM 27299676 ER PT J AU Yoon, SJ Guo, Z Claro, PCD Sheychenko, EV Huang, LB AF Yoon, Seog Joon Guo, Zhi Claro, Paula C. dos Santos Sheychenko, Elena V. Huang, Libai TI Direct Imaging of Long-Range Exciton Transport in Quantum Dot Superlattices by Ultrafast Microscopy SO ACS Nano LA English DT Article DE energy transfer; femtosecond transient absorption spectroscopy; pump-probe microscopy; exciton diffusion; quantum dot solids ID FORSTER ENERGY-TRANSFER; PUMP-PROBE MICROSCOPY; SELF-ORGANIZATION; CHARGE-TRANSPORT; SOLAR-CELLS; THIN-FILMS; SOLIDS; NANOCRYSTALS; NANOWIRES; CARRIER AB Long-range charge and exciton transport in quantum dot (QD) solids is a crucial challenge in utilizing QDs for optoelectronic applications. Here, we present a direct visualization of exciton diffusion in highly ordered CdSe QDs superlattices by mapping exciton population using ultrafast transient absorption microscopy. A temporal resolution of similar to 200 fs and a spatial precision of similar to 50 nm of this technique provide a direct assessment of the upper limit for exciton transport in QD solids. An exciton diffusion length of similar to 125 nm has been visualized in the 3 ns experimental time window and an exciton diffusion coefficient of (2.5 +/- 0.2) x 10(-2) cm(2) s(-1) has been measured for superlattices constructed from 3.6 nm CdSe QDs with center-to-center distance of 6.7 nm. The measured exciton diffusion constant is in good agreement with FOrster resonance energy transfer theory. We have found that exciton diffusion is greatly enhanced in the superlattices over the disordered films with an order of magnitude higher diffusion coefficient, pointing toward the role of disorder in limiting transport. This study provides important understandings on energy transport mechanisms in both the spatial and temporal domains in QD solids. C1 [Yoon, Seog Joon] Univ Notre Dame, Radiat Lab, Notre Dame, IN 46556 USA. [Yoon, Seog Joon] Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA. [Guo, Zhi; Huang, Libai] Purdue Univ, Dept Chem, W Lafayette, IN 47907 USA. [Claro, Paula C. dos Santos; Sheychenko, Elena V.] Argonne Natl Lab, Ctr Nanoscale Mat, Argonne, IL 60439 USA. RP Huang, LB (reprint author), Purdue Univ, Dept Chem, W Lafayette, IN 47907 USA. EM libai-huang@purdue.edu FU National Science Foundation [NSF-CHE-1555005]; Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy [DE-FC02-04ER15533]; Materials Science of Actinides, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science [DE-SC0001089] FX L.H. acknowledges support from National Science Foundation through grant NSF-CHE-1555005. The authors acknowledge the support from the Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences of the U.S. Department of Energy through grant DE-FC02-04ER15533 for funding the part of work carried out at the Radiation Laboratory at University of Notre Dame. This is document no. NDRL 5907 from Notre Dame Radiation Laboratory. Small angle X-ray scattering studies are sponsored by the Materials Science of Actinides, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, under award No. DE-SC0001089. The authors thank Yong-Siou Chen for his assistance in TEM imaging. NR 45 TC 3 Z9 3 U1 27 U2 32 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2016 VL 10 IS 7 BP 7208 EP 7215 DI 10.1021/acsnano.6b03700 PG 8 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DS2FD UT WOS:000380576600088 PM 27387010 ER PT J AU Nyein, HYY Gao, W Shahpar, Z Emaminejad, S Challa, S Chen, K Fahad, HM Tai, LC Ota, H Davis, RW Javey, A AF Nyein, Hnin Yin Yin Gao, Wei Shahpar, Ziba Emaminejad, Sam Challa, Samyuktha Chen, Kevin Fahad, Hossain M. Tai, Li-Chia Ota, Hiroki Davis, Ronald W. Javey, Ali TI A Wearable Electrochemical Platform for Noninvasive Simultaneous Monitoring of Ca2+ and pH SO ACS Nano LA English DT Article DE wearable biosensors; flexible electronics; multiplexed sensing; system integration; in situ analysis ID SELECTIVE ELECTRODE; CALCIUM SENSOR; SWEAT; SKIN; ION; PERSPIRATION; EXERCISE; POLYMER AB Homeostasis of ionized calcium in biofluids is critical for human biological functions and organ systems. Measurement of ionized calcium for clinical applications is not easily accessible due to its strict procedures and dependence on pH. pH balance in body fluids greatly affects metabolic reactions and biological transport systems. Here, we demonstrate a wearable electrochemical device for continuous monitoring of ionized calcium and pH of body fluids using a disposable and flexible array of Ca2+ and pH sensors that interfaces with a flexible printed circuit board. This platform enables real-time quantitative analysis of these sensing elements in body fluids such as sweat, urine, and tears. Accuracy of Ca2+ concentration and pH measured by the wearable sensors is validated through inductively coupled plasma-mass spectrometry technique and a commercial pH meter, respectively. Our results show that the wearable sensors have high repeatability and selectivity to the target ions. Real-time on-body assessment of sweat is also performed, and our results indicate that calcium concentration increases with decreasing pH. This platform can be used in noninvasive continuous analysis of ionized calcium and pH in body fluids for disease diagnosis such as primary hyperparathyroidism and kidney stones. C1 [Nyein, Hnin Yin Yin; Gao, Wei; Shahpar, Ziba; Emaminejad, Sam; Chen, Kevin; Fahad, Hossain M.; Tai, Li-Chia; Ota, Hiroki; Javey, Ali] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. [Nyein, Hnin Yin Yin; Gao, Wei; Emaminejad, Sam; Chen, Kevin; Fahad, Hossain M.; Ota, Hiroki; Javey, Ali] Univ Calif Berkeley, Berkeley Sensor & Actuator Ctr, Berkeley, CA 94720 USA. [Nyein, Hnin Yin Yin; Gao, Wei; Emaminejad, Sam; Chen, Kevin; Tai, Li-Chia; Ota, Hiroki; Javey, Ali] Lawrence Berkeley Natl Lab, Mat Sci Div, Berkeley, CA 94720 USA. [Emaminejad, Sam; Challa, Samyuktha; Davis, Ronald W.] Stanford Sch Med, Stanford Genome Technol Ctr, Palo Alto, CA 94304 USA. RP Javey, A (reprint author), Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA. EM ajavey@berkeley.edu RI Gao, Wei/A-1347-2011 OI Gao, Wei/0000-0002-8503-4562 FU NSF Nanomanufacturing Systems for Mobile Computing and Energy Technologies (NASCENT) Center; National Institutes of Health [P01 HG000205]; Office of Science, Office of Basic Energy Sciences, Material Sciences and Engineering Division of the U.S. Department of Energy [DE-AC02-05CH11231]; Robert N. Noyce Fellowship in Microelectronics FX This work at the University of California, Berkeley was supported by NSF Nanomanufacturing Systems for Mobile Computing and Energy Technologies (NASCENT) Center and at Stanford University was supported by the National Institutes of Health grant no. P01 HG000205. The sensor fabrication was performed in the Electronic Materials (E-MAT) laboratory funded by the Director, Office of Science, Office of Basic Energy Sciences, Material Sciences and Engineering Division of the U.S. Department of Energy under contract no. DE-AC02-05CH11231. K.C. acknowledges support from the Robert N. Noyce Fellowship in Microelectronics. The authors thank H.W.W.N. for her assistance. NR 43 TC 6 Z9 6 U1 42 U2 65 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1936-0851 EI 1936-086X J9 ACS NANO JI ACS Nano PD JUL PY 2016 VL 10 IS 7 BP 7216 EP 7224 DI 10.1021/acsnano.6b04005 PG 9 WC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary SC Chemistry; Science & Technology - Other Topics; Materials Science GA DS2FD UT WOS:000380576600089 PM 27380446 ER PT J AU Pinard, MA Kurian, JJ Aggarwal, M Agbandje-McKenna, M McKenna, R AF Pinard, Melissa A. Kurian, Justin J. Aggarwal, Mayank Agbandje-McKenna, Mavis McKenna, Robert TI Cryoannealing-induced space-group transition of crystals of the carbonic anhydrase psCA3 SO ACTA CRYSTALLOGRAPHICA SECTION F-STRUCTURAL BIOLOGY COMMUNICATIONS LA English DT Article DE beta-carbonic anhydrase; Pseudomonas aeruginosa; cryoannealing; crystal packing ID PSEUDOMONAS-AERUGINOSA PAO1; PH-DEPENDENT ACTIVITY; X-RAY-DIFFRACTION; MYCOBACTERIUM-TUBERCULOSIS; CRYOCRYSTALLOGRAPHY; MOSAICITY; ENZYME AB Cryoannealing has been demonstrated to improve the diffraction quality and resolution of crystals of the beta-carbonic anhydrase psCA3 concomitant with a change in space group. After initial flash-cooling in a liquid-nitrogen cryostream an X-ray diffraction data set from a psCA3 crystal was indexed in space group P2(1)2(1)2 and was scaled to 2.6 angstrom resolution, but subsequent cryoannealing studies revealed induced protein rearrangements in the crystal contacts, which transformed the space group to I222, with a corresponding improvement of 0.7 angstrom in resolution. Although the change in diffraction resolution was significant, only minor changes in the psCA3 structure, which retained its catalytic 'open' conformation, were observed. These findings demonstrate that cryoannealing can be successfully utilized to induce higher diffraction-quality crystals while maintaining enzymatically relevant conformations and may be useful as an experimental tool for structural studies of other enzymes where the initial diffraction quality is poor. C1 [Pinard, Melissa A.; Kurian, Justin J.; Agbandje-McKenna, Mavis; McKenna, Robert] Univ Florida, Coll Med, Dept Biochem & Mol Biol, 1200 Newell Dr,POB 100245, Gainesville, FL 32610 USA. [Aggarwal, Mayank] Oak Ridge Natl Lab, Div Biol & Soft Matter, Oak Ridge, TN 37831 USA. RP McKenna, R (reprint author), Univ Florida, Coll Med, Dept Biochem & Mol Biol, 1200 Newell Dr,POB 100245, Gainesville, FL 32610 USA. EM rmckenna@ufl.edu FU NSF; NIH/NIGMS via NSF [DMR-1332208]; NIGMS [GM-103485]; DOE [DE-AC05-00OR22725]; US Department of Energy FX The authors would like to thank the UF Center for Structural Biology for support of the X-ray facility. We would also like to thank the MacCHESS staff for their help during X-ray diffraction data collection at the Cornell High Energy Synchrotron (CHESS) Facility, Ithaca. CHESS is supported by the NSF and NIH/NIGMS via NSF award DMR-1332208, and the MacCHESS resource is supported by NIGMS award GM-103485. This manuscript has been authored by UT-Battelle LLC under DOE Contract No. DE-AC05-00OR22725 with the US Department of Energy. The publisher, by accepting the article, acknowledges that the US Government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US Government purposes. NR 26 TC 1 Z9 1 U1 3 U2 3 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 2053-230X J9 ACTA CRYSTALLOGR F JI Acta Crystallogr. F-Struct. Biol. Commun. PD JUL PY 2016 VL 72 BP 573 EP 577 DI 10.1107/S2053230X16009286 PN 7 PG 5 WC Biochemical Research Methods; Biochemistry & Molecular Biology; Biophysics; Crystallography SC Biochemistry & Molecular Biology; Biophysics; Crystallography GA DS0MF UT WOS:000380289200010 PM 27380376 ER PT J AU Calle, L Canadell, JG Patra, P Ciais, P Ichii, K Tian, HQ Kondo, M Piao, SL Arneth, A Harper, AB Ito, A Kato, E Koven, C Sitch, S Stocker, BD Vivoy, N Wiltshire, A Zaehle, S Poulter, B AF Calle, Leonardo Canadell, Josep G. Patra, Prabir Ciais, Philippe Ichii, Kazuhito Tian, Hanqin Kondo, Masayuki Piao, Shilong Arneth, Almut Harper, Anna B. Ito, Akihiko Kato, Etsushi Koven, Charlie Sitch, Stephen Stocker, Benjamin D. Vivoy, Nicolas Wiltshire, Andy Zaehle, Soenke Poulter, Benjamin TI Regional carbon fluxes from land use and land cover change in Asia, 1980-2009 SO Environmental Research Letters LA English DT Article DE land use change; deforestation; DGVM; carbon budget ID TERRESTRIAL ECOSYSTEMS; TROPICAL REGIONS; SECONDARY LANDS; USE TRANSITIONS; SOUTHEAST-ASIA; FIRE EMISSIONS; CO2 EMISSIONS; FOREST COVER; WOOD-HARVEST; DEFORESTATION AB We present a synthesis of the land-atmosphere carbon flux from land use and land cover change (LULCC) in Asia using multiple data sources and paying particular attention to deforestation and forest regrowth fluxes. The data sources are quasi-independent and include the U.N. Food andAgriculture Organization-Forest Resource Assessment (FAO-FRA2015; country-level inventory estimates), the Emission Database for Global Atmospheric Research (EDGARv4.3), the 'Houghton' bookkeeping model that incorporates FAO-FRA data, an ensemble of 8 state-of-the-art Dynamic Global Vegetation Models (DGVM), and 2 recently published independent studies using primarily remote sensing techniques. The estimates are aggregated spatially to Southeast, East, and South Asia and temporally for three decades, 1980-1989, 1990-1999 and 2000-2009. Since 1980, net carbon emissions from LULCC in Asia were responsible for 20%-40% of global LULCC emissions, with emissions from Southeast Asia alone accounting for 15%-25% of global LULCC emissions during the same period. In the 2000s and for all Asia, three estimates (FAO-FRA, DGVM, Houghton) were in agreement of a net source of carbon to the atmosphere, with mean estimates ranging between 0.24 to 0.41 Pg Cyr(-1), whereas EDGARv4.3 suggested a net carbon sink of -0.17 Pg Cyr(-1). Three of 4 estimates suggest that LULCC carbon emissions declined by at least 34% in the preceding decade (1990-2000). Spread in the estimates is due to the inclusion of different flux components and their treatments, showing the importance to include emissions from carbon rich peatlands and land management, such as shifting cultivation and wood harvesting, which appear to be consistently underreported. C1 [Calle, Leonardo; Poulter, Benjamin] Montana State Univ, Dept Ecol, Bozeman, MT 59717 USA. [Calle, Leonardo; Poulter, Benjamin] Montana State Univ, Inst Ecosyst, Bozeman, MT 59717 USA. [Canadell, Josep G.] CSIRO Oceans & Atmospher Res, Global Carbon Project, GPO Box 3023, Canberra, ACT 2601, Australia. [Patra, Prabir; Ichii, Kazuhito; Kondo, Masayuki] Japan Agcy Marine Earth Sci & Technol JAMSTEC, Dept Environm Geochem Cycle Research, 3173-25 Showa Machi, Yokohama, Kanagawa, Japan. [Ciais, Philippe; Piao, Shilong; Vivoy, Nicolas] UVSQ, CNRS, CEA, LSCE, Gif Sur Yvette, France. [Ichii, Kazuhito; Ito, Akihiko] Natl Inst Environm Studies, Ctr Global Environm Res, Tsukuba, Ibaraki 3050053, Japan. [Tian, Hanqin] Auburn Univ, Int Ctr Climate & Global Change Res, Auburn, AL 36849 USA. [Tian, Hanqin] Auburn Univ, Sch Forestry & Wildlife Sci, Auburn, AL 36849 USA. [Piao, Shilong] CNRS, Lab Glaciol & Geophys Environm, F-38041 Grenoble, France. [Piao, Shilong] Univ Grenoble Alpes, F-38041 Grenoble, France. [Arneth, Almut] Karlsruhe Inst Technol, Inst Meteorol & Climate Res Atmospher Environm Re, D-82467 Garmisch Partenkirchen, Germany. [Harper, Anna B.] Univ Exeter, Coll Engn Math & Phys Sci, Exeter, Devon, England. [Kato, Etsushi] Inst Appl Energy, Minato Ku, Tokyo 1050003, Japan. [Koven, Charlie] Lawrence Berkeley Natl Lab, Div Earth Sci, Berkeley, CA USA. [Sitch, Stephen] Univ Exeter, Dept Geog, Exeter EX4 4QF, Devon, England. [Stocker, Benjamin D.] Imperial Coll London, Dept Life Sci, Silwood Pk, Ascot SL5 7PY, Berks, England. [Stocker, Benjamin D.] Univ Bern, Climate & Environm Phys, Bern, Switzerland. [Stocker, Benjamin D.] Univ Bern, Oeschger Ctr Climate Change Res, Bern, Switzerland. [Wiltshire, Andy] Met Off Hadley Ctr, Exeter EX1 3PB, Devon, England. [Zaehle, Soenke] Max Planck Inst Biogeochem, Biogeochem Integrat Dept, Hans Knoll Str 10, D-07745 Jena, Germany. RP Calle, L (reprint author), Montana State Univ, Dept Ecol, Bozeman, MT 59717 USA.; Calle, L (reprint author), Montana State Univ, Inst Ecosyst, Bozeman, MT 59717 USA. EM Leonardo.Calle@msu.montana.edu RI Ichii, Kazuhito/D-2392-2010; Stocker, Benjamin/K-3194-2015; Canadell, Josep/E-9419-2010; Koven, Charles/N-8888-2014; Zaehle, Sonke/C-9528-2017; Patra, Prabir/B-5206-2009 OI Ichii, Kazuhito/0000-0002-8696-8084; Stocker, Benjamin/0000-0003-2697-9096; Canadell, Josep/0000-0002-8788-3218; Koven, Charles/0000-0002-3367-0065; Zaehle, Sonke/0000-0001-5602-7956; Patra, Prabir/0000-0001-5700-9389 FU Asia Pacific Network for Global Change Research (Patra/Canadell) [ARCP2013-01CMY]; National Science Foundation East Asia Pacific Summer Institute (EAPSI) Fellowship; Environment Research and Technology Development Funds from the Ministry of the Environment of Japan [2-1401]; Australian Climate Change Science Program; ERTDF by the Ministry of the Environment, Japan [S-10]; DOE-BER through BGC-Feedbacks SFA and NGEE-Tropics; Joint UK DECC/Defra Met Office Hadley Centre Climate Programme [GA01101]; EU FP7 through project LUC4C [603542] FX This work was supported by the Asia Pacific Network for Global Change Research (ARCP2013-01CMY-Patra/Canadell). LC was supported by the National Science Foundation East Asia Pacific Summer Institute (EAPSI) Fellowship. KI and PP were supported by the Environment Research and Technology Development Funds (2-1401) from the Ministry of the Environment of Japan. JGC thanks the support from the Australian Climate Change Science Program. AI and EK were supported by ERTDF (S-10) by the Ministry of the Environment, Japan. CK is supported by DOE-BER through BGC-Feedbacks SFA and NGEE-Tropics. AW was supported by the Joint UK DECC/Defra Met Office Hadley Centre Climate Programme (GA01101) and EU FP7 Funding through project LUC4C (603542). NR 56 TC 0 Z9 0 U1 35 U2 49 PU IOP PUBLISHING LTD PI BRISTOL PA TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND SN 1748-9326 J9 ENVIRON RES LETT JI Environ. Res. Lett. PD JUL PY 2016 VL 11 IS 7 AR 074011 DI 10.1088/1748-9326/11/7/074011 PG 12 WC Environmental Sciences; Meteorology & Atmospheric Sciences SC Environmental Sciences & Ecology; Meteorology & Atmospheric Sciences GA DS5JD UT WOS:000380817000011 ER PT J AU Huang, C Li, FX Zhou, D Guo, JH Pan, ZH Liu, Y Liu, YL AF Huang, Can Li, Fangxing Zhou, Dao Guo, Jiahui Pan, Zhuohong Liu, Yong Liu, Yilu TI Data quality issues for synchrophasor applications Part I: a review SO Journal of Modern Power Systems and Clean Energy LA English DT Review DE Synchrophasor system; Synchrophasor application; Data quality; Data accuracy; Data loss; Latency ID POWER-SYSTEMS; PROTECTION AB Synchrophasor systems, providing low-latency, high-precision, and time-synchronized measurements to enhance power grid performances, are deployed globally. However, the synchrophasor system as a physical network, involves communication constraints and data quality issues, which will impact or even disable certain synchrophasor applications. This work investigates the data quality issue for synchrophasor applications. In Part I, the standards of synchrophasor systems and the classifications and data quality requirements of synchrophasor applications are reviewed. Also, the actual events of synchronization signal accuracy, synchrophasor data loss, and latency are counted and analyzed. The review and statistics are expected to provide an overall picture of data accuracy, loss, and latency issues for synchrophasor applications. C1 [Huang, Can; Li, Fangxing; Zhou, Dao; Guo, Jiahui; Pan, Zhuohong; Liu, Yong; Liu, Yilu] Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37996 USA. [Liu, Yong] Univ Tennessee, Engn Res Ctr, Knoxville, TN USA. [Liu, Yilu] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Li, FX (reprint author), Univ Tennessee, Dept Elect Engn & Comp Sci, Knoxville, TN 37996 USA. EM chuang16@vols.utk.edu; fli6@utk.edu; dao@vols.utk.edu; jguo7@vols.utk.edu; leekey2@gmail.com; yliu66@vols.utk.edu; liu@utk.edu OI Li, Fangxing/0000-0003-1060-7618 FU U.S. National Science Foundation (U.S. NSF) through the U.S. NSF/Department of Energy (DOE) Engineering Research Center Program [EEC-1041877] FX This work was supported in part by the U.S. National Science Foundation (U.S. NSF) through the U.S. NSF/Department of Energy (DOE) Engineering Research Center Program under Award EEC-1041877 for CURENT. The authors would also like to thank the editors and reviewers for their insightful comments and suggestions on improving the quality of this work. NR 32 TC 1 Z9 1 U1 3 U2 3 PU STATE GRID ELECTRIC POWER RESEARCH INST PI NANJING PA NO 19 CHENGXIN AVE, JIANGNING DISTRICT, NANJING, 211106, PEOPLES R CHINA SN 2196-5625 EI 2196-5420 J9 J MOD POWER SYST CLE JI J. Mod. Power Syst. Clean Energy PD JUL PY 2016 VL 4 IS 3 SI SI BP 342 EP 352 DI 10.1007/s40565-016-0217-4 PG 11 WC Engineering, Electrical & Electronic SC Engineering GA DS3VB UT WOS:000380709700004 ER PT J AU Huang, C Li, FX Zhan, LW Xu, Y Hu, QR Zhou, D Liu, YL AF Huang, Can Li, Fangxing Zhan, Lingwei Xu, Yao Hu, Qinran Zhou, Dao Liu, Yilu TI Data quality issues for synchrophasor applications Part II: problem formulation and potential solutions SO Journal of Modern Power Systems and Clean Energy LA English DT Article DE GPS loss; Synchronization signal loss; Synchrophasor data loss; Estimation; Forecasting ID POWER-SYSTEM; COMMUNICATION; STATE AB This work investigates the data quality issue for synchrophasor applications, and pays particular attention to synchronization signal loss and synchrophasor data loss events. First, the historical synchronization signal loss events are analyzed and the potential reasons and solutions are discussed. Then, the scenario of a small amount of synchrophasor data loss is studied and a Lagrange interpolating polynomial method is used to adaptively estimate the incomplete and missing data. The performance of proposed method is demonstrated with simulation results. Specifically, the proposed method considers the trade-off between the estimation accuracy and the hardware cost, and could be efficiently employed in reality. C1 [Huang, Can; Li, Fangxing; Zhan, Lingwei; Xu, Yao; Hu, Qinran; Zhou, Dao; Liu, Yilu] Univ Tennessee, Dept Elect Engn & Comp Sci, Elect Engn, Knoxville, TN 37996 USA. [Huang, Can] NARI Grp Corp, State Grid Elect Power Res Inst, Nanjing, Jiangsu, Peoples R China. [Li, Fangxing] ABB Elect Syst Consulting, Raleigh, NC USA. [Zhan, Lingwei] Gen Elect Grid Solut, Philadelphia, PA USA. [Xu, Yao] Lamar Univ, Beaumont, TX USA. [Hu, Qinran] Harvard Univ, Cambridge, MA USA. [Liu, Yilu] Oak Ridge Natl Lab, Oak Ridge, TN USA. RP Li, FX (reprint author), Univ Tennessee, Dept Elect Engn & Comp Sci, Elect Engn, Knoxville, TN 37996 USA. EM chuang16@vols.utk.edu; fli6@utk.edu; lzhan@vols.utk.edu; yxu4@lamar.edu; qinranhu@g.harvard.edu; dao@vols.utk.edu; liu@utk.edu OI Li, Fangxing/0000-0003-1060-7618; Zhan, Lingwei/0000-0003-0021-6234 FU U.S. National Science Foundation (U.S. NSF) through the U.S. NSF/Department of Energy (DOE) Engineering Research Center Program [EEC-1041877] FX This work was supported in part by the U.S. National Science Foundation (U.S. NSF) through the U.S. NSF/Department of Energy (DOE) Engineering Research Center Program under Award EEC-1041877 for CURENT. The authors would also like to thank the editors and reviewers for their insightful comments and suggestions on improving the quality of this work. NR 43 TC 1 Z9 1 U1 2 U2 2 PU STATE GRID ELECTRIC POWER RESEARCH INST PI NANJING PA NO 19 CHENGXIN AVE, JIANGNING DISTRICT, NANJING, 211106, PEOPLES R CHINA SN 2196-5625 EI 2196-5420 J9 J MOD POWER SYST CLE JI J. Mod. Power Syst. Clean Energy PD JUL PY 2016 VL 4 IS 3 SI SI BP 353 EP 361 DI 10.1007/s40565-016-0213-8 PG 9 WC Engineering, Electrical & Electronic SC Engineering GA DS3VB UT WOS:000380709700005 ER PT J AU Villa-Aleman, E Wellons, MS AF Villa-Aleman, Eliel Wellons, Matthew S. TI Characterization of uranium tetrafluoride (UF4) with Raman spectroscopy SO JOURNAL OF RAMAN SPECTROSCOPY LA English DT Article DE uranium tetrafluoride; nuclear forensics; in situ SEM; Raman spectroscopy ID VIBRATIONAL-SPECTRA; SIZE PARTICLES AB The Raman spectrum of uranium tetrafluoride (UF4) is unambiguously characterized with multiple Raman excitation laser sources for the first time. Across different laser excitation wavelengths, UF4 demonstrates 16 distinct Raman bands within the 50-400cm(-1) region. The observed Raman bands are representative of various F-F vibrational modes. UF4 also shows intense fluorescent bands in the 325-750nm spectral region. Comparison of the UF4 spectrum with the ZrF4 spectrum, its crystalline analog, demonstrates a similar Raman band structure consistent with group theory predictions for expected Raman bands. Additionally, a demonstration of combined scanning electron microscopy and in situ Raman spectroscopy microanalytical measurements of UF4 particulates shows that despite the inherent weak intensity of Raman bands, identification and characterization are possible for micron-sized particulates with modern instrumentation. The published well-characterized UF4 spectrum is extremely relevant to nuclear materials and nuclear safeguard applications. Published 2016. This article is a U.S. Government work and is in the public domain in the USA. Journal of Raman Spectroscopy published by John Wiley & Sons Ltd. C1 [Villa-Aleman, Eliel; Wellons, Matthew S.] Savannah River Natl Lab, Nonproliferat Technol Sect, Aiken, SC 29808 USA. RP Villa-Aleman, E (reprint author), Savannah River Natl Lab, Nonproliferat Technol Sect, Aiken, SC 29808 USA. EM eliel.villa-aleman@srnl.doe.gov FU Office of Defense Nuclear Nonproliferation Research and Development within US Department of Energy's National Nuclear Security Administration; Savannah River National Laboratory, Laboratory Directed R&D (LDRD) project [SRNL-2015-00142] FX The authors wish to thankMichael Summer and Ross Smith for their contributing efforts on the collection of SEM images and Raman spectra of UF4, Sheldon Nichols for his contributing efforts on the collection of XRD data and Dr. Lindsay Roy on her consultations regarding the current state of computational modeling of uranium materials. This work was funded by the Office of Defense Nuclear Nonproliferation Research and Development within the US Department of Energy's National Nuclear Security Administration and the Savannah River National Laboratory, Laboratory Directed R&D funding (LDRD) project #SRNL-2015-00142. NR 28 TC 0 Z9 0 U1 10 U2 16 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0377-0486 EI 1097-4555 J9 J RAMAN SPECTROSC JI J. Raman Spectrosc. PD JUL PY 2016 VL 47 IS 7 BP 865 EP 870 DI 10.1002/jrs.4909 PG 6 WC Spectroscopy SC Spectroscopy GA DS1RU UT WOS:000380376100016 ER PT J AU McMasters, RL de Monte, F Beck, JV Nallapaneni, SC Amos, DE AF McMasters, Robert L. de Monte, Filippo Beck, James V. Nallapaneni, Satish C. Amos, Donald E. TI Diffusion Penetration Time for Transient Heat Conduction SO JOURNAL OF THERMOPHYSICS AND HEAT TRANSFER LA English DT Article; Proceedings Paper CT 15th AIAA Aviation Technology, Integration, and Operations Conference CY JUN 22-26, 2015 CL Dallas, TX SP AIAA AB The time duration for processes involving transient thermal diffusion can be a critical piece of information related to thermal processes in engineering applications. Analytical solutions must be used to calculate these types of time durations because the boundary conditions in such cases can be effectively like semi-infinite conditions. This research involves an investigation into analytical solutions for six geometries, including one-dimensional cases for Cartesian, cylindrical, and spherical coordinates. The fifth case involves a heated surface on the inside of a hole bored through an infinite body, which is a one-dimensional problem in cylindrical coordinates. The sixth case involves two-dimensional conduction from a point heat source on the surface of a slab subjected to insulated boundary conditions elsewhere. The mathematical modeling for this case is done in cylindrical coordinates. For each geometric configuration, a relationship is developed to determine the time required for a temperature rise to occur at a nonheated point in the body in response to a sudden change at a heated boundary. A range of time values is computed for each configuration based on the amount of temperature rise used as a criterion. Plots are given for each case, showing the relationships between the temperature rise at the point of interest and the amount of time required to reach that temperature. It was found that a dimensionless parameter, defined herein as dimensionless penetration time, remains reasonably constant between the various geometries studied. The definition of this term is the dimensionless time required to bring about a desired temperature rise, with the characteristic length being the distance between the point of heating and the point of interest. C1 [McMasters, Robert L.] Virginia Mil Inst, Dept Mech Engn, Lexington, VA 24450 USA. [de Monte, Filippo] Univ Aquila, Dept Ind & Informat Engn & Econ, Via G Gronchi 18, I-67100 Laquila, Italy. [Beck, James V.; Nallapaneni, Satish C.] Michigan State Univ, Dept Mech Engn, E Lansing, MI 48824 USA. [Amos, Donald E.] Sandia Natl Labs, Dept Adv Sci Comp Res, Albuquerque, NM 87110 USA. RP McMasters, RL (reprint author), Virginia Mil Inst, Dept Mech Engn, Lexington, VA 24450 USA. NR 11 TC 0 Z9 0 U1 3 U2 3 PU AMER INST AERONAUTICS ASTRONAUTICS PI RESTON PA 1801 ALEXANDER BELL DRIVE, STE 500, RESTON, VA 22091-4344 USA SN 0887-8722 EI 1533-6808 J9 J THERMOPHYS HEAT TR JI J. Thermophys. Heat Transf. PD JUL-SEP PY 2016 VL 30 IS 3 BP 614 EP 621 DI 10.2514/1.T4819 PG 8 WC Thermodynamics; Engineering, Mechanical SC Thermodynamics; Engineering GA DS1NZ UT WOS:000380364100014 ER PT J AU Martin, AA Lin, T Toth, M Westphal, AJ Vicenzi, EP Beeman, J Silver, EH AF Martin, Aiden A. Lin, Ting Toth, Milos Westphal, Andrew J. Vicenzi, Edward P. Beeman, Jeffrey Silver, Eric H. TI Exposure and analysis of microparticles embedded in silica aerogel keystones using NF3-mediated electron beam-induced etching and energy-dispersive X-ray spectroscopy SO METEORITICS & PLANETARY SCIENCE LA English DT Article ID COMET 81P/WILD 2; TOF-SIMS ANALYSIS; STARDUST AEROGEL; DUST PARTICLES; MICROSCOPY; CRATERS; SPACECRAFT; MINERALOGY; DENSITY; MISSION AB In 2006, NASA's Stardust spacecraft delivered to Earth dust particles collected from the coma of comet 81P/Wild 2, with the goal of furthering the understanding of solar system formation. Stardust cometary samples were collected in a low-density, nanoporous silica aerogel making their study technically challenging. This article demonstrates the identification, exposure, and elemental composition analysis of particles analogous to those collected by NASA's Stardust mission using in-situ SEM techniques. Backscattered electron imaging is shown by experimental observation and Monte Carlo simulation to be suitable for locating particles of a range of sizes relevant to Stardust (down to submicron diameters) embedded within silica aerogel. Selective removal of the silica aerogel encapsulating an embedded particle is performed by cryogenic NF3-mediated electron beam-induced etching. The porous, low-density nature of the aerogel results in an enhanced etch rate compared with solid material, making it an effective, nonmechanical method for the exposure of particles. After exposure, elemental composition of the particle was analyzed by energy-dispersive X-ray spectroscopy using a high spectral resolution microcalorimeter. Signals from fluorine contamination are shown to correspond to nonremoved silica aerogel and only in residual concentrations. C1 [Martin, Aiden A.; Toth, Milos] Univ Technol, Sch Phys & Adv Mat, 15 Broadway, Ultimo, NSW 2007, Australia. [Lin, Ting; Silver, Eric H.] Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. [Westphal, Andrew J.] Univ Calif Berkeley, Space Sci Lab, Berkeley, CA 94720 USA. [Vicenzi, Edward P.] Smithsonian Inst, Museum Conservat Inst, 4210 Silver Hill Rd, Camp Springs, MD 20746 USA. [Beeman, Jeffrey] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. RP Silver, EH (reprint author), Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA. EM esilver@cfa.harvard.edu FU NASA [NNX11AF61Gno1]; FEI Company; John Stocker Postgraduate Scholarship from Science and Industry Endowment Fund FX This work was partly funded by NASA Grant NNX11AF61Gno1 and FEI Company. A.A.M. is the recipient of a John Stocker Postgraduate Scholarship from the Science and Industry Endowment Fund. NR 44 TC 0 Z9 0 U1 2 U2 2 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1086-9379 EI 1945-5100 J9 METEORIT PLANET SCI JI Meteorit. Planet. Sci. PD JUL PY 2016 VL 51 IS 7 BP 1223 EP 1232 DI 10.1111/maps.12655 PG 10 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DS0GU UT WOS:000380274300002 ER PT J AU Gilbert, DA Grutter, AJ Arenholz, E Liu, K Kirby, BJ Borchers, JA Maranville, BB AF Gilbert, Dustin A. Grutter, Alexander J. Arenholz, Elke Liu, Kai Kirby, B. J. Borchers, Julie A. Maranville, Brian B. TI Structural and magnetic depth profiles of magneto-ionic heterostructures beyond the interface limit SO NATURE COMMUNICATIONS LA English DT Article ID NEUTRON-SCATTERING LENGTHS; ELECTRIC-FIELD CONTROL; ROOM-TEMPERATURE; EXCHANGE BIAS; MAGNETORESISTANCE; FERROMAGNETISM; REFLECTOMETRY; REVERSAL; COBALT AB Electric field control of magnetism provides a promising route towards ultralow power information storage and sensor technologies. The effects of magneto-ionic motion have been prominently featured in the modification of interface characteristics. Here, we demonstrate magnetoelectric coupling moderated by voltage-driven oxygen migration beyond the interface in relatively thick AlOx/GdOx/Co(15 nm) films. Oxygen migration and Co magnetization are quantitatively mapped with polarized neutron reflectometry under electro-thermal conditioning. The depth-resolved profiles uniquely identify interfacial and bulk behaviours and a semi-reversible control of the magnetization. Magnetometry measurements suggest changes in the microstructure which disrupt long-range ferromagnetic ordering, resulting in an additional magnetically soft phase. X-ray spectroscopy confirms changes in the Co oxidation state, but not in the Gd, suggesting that the GdOx transmits oxygen but does not source or sink it. These results together provide crucial insight into controlling magnetism via magneto-ionic motion, both at interfaces and throughout the bulk of the films. C1 [Gilbert, Dustin A.; Grutter, Alexander J.; Kirby, B. J.; Borchers, Julie A.; Maranville, Brian B.] NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. [Arenholz, Elke] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. [Liu, Kai] Univ Calif Davis, Dept Phys, Davis, CA 95616 USA. RP Gilbert, DA; Grutter, AJ (reprint author), NIST, Ctr Neutron Res, Gaithersburg, MD 20899 USA. EM dustin.gilbert@nist.gov; alexander.grutter@nist.gov RI Liu, Kai/B-1163-2008; Gilbert, Dustin/G-1683-2011 OI Liu, Kai/0000-0001-9413-6782; Gilbert, Dustin/0000-0003-3747-3883 FU U.S. Department of Commerce; National Research Council; National Science Foundation [DMR-1543582, ECCS-1232275]; Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy [DEAC02-05CH11231] FX We thank Professor Geoffrey Beach from the Massachusetts Institute of Technology for discussions. Work at NIST has been supported by the U.S. Department of Commerce. D.A.G. and A.J.G. acknowledge support from the National Research Council Research Associateship Program. Work at UCD has been supported by the National Science Foundation (DMR-1543582 and ECCS-1232275). Work at the ALS has been supported by the Director, Office of Science, Office of Basic Energy Sciences of the U.S. Department of Energy (DEAC02-05CH11231). NR 55 TC 2 Z9 2 U1 24 U2 34 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2016 VL 7 AR 12264 DI 10.1038/ncomms12264 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DS5SH UT WOS:000380842100001 PM 27447691 ER PT J AU Jiang, MP Trigo, M Savic, I Fahy, S Murray, ED Bray, C Clark, J Henighan, T Kozina, M Chollet, M Glownia, JM Hoffmann, MC Zhu, D Delaire, O May, AF Sales, BC Lindenberg, AM Zalden, P Sato, T Merlin, R Reis, DA AF Jiang, M. P. Trigo, M. Savic, I. Fahy, S. Murray, E. D. Bray, C. Clark, J. Henighan, T. Kozina, M. Chollet, M. Glownia, J. M. Hoffmann, M. C. Zhu, D. Delaire, O. May, A. F. Sales, B. C. Lindenberg, A. M. Zalden, P. Sato, T. Merlin, R. Reis, D. A. TI The origin of incipient ferroelectricity in lead telluride SO Nature Communications LA English DT Article ID IV-VI COMPOUNDS; LATTICE THERMAL-CONDUCTIVITY; CRYSTAL-STRUCTURE; PBTE; SEMICONDUCTORS; SCATTERING; MODEL AB The interactions between electrons and lattice vibrations are fundamental to materials behaviour. In the case of group IV-VI, V and related materials, these interactions are strong, and the materials exist near electronic and structural phase transitions. The prototypical example is PbTe whose incipient ferroelectric behaviour has been recently associated with large phonon anharmonicity and thermoelectricity. Here we show that it is primarily electron-phonon coupling involving electron states near the band edges that leads to the ferroelectric instability in PbTe. Using a combination of nonequilibrium lattice dynamics measurements and first principles calculations, we find that photoexcitation reduces the Peierls-like electronic instability and reinforces the paraelectric state. This weakens the long-range forces along the cubic direction tied to resonant bonding and low lattice thermal conductivity. Our results demonstrate how free-electron-laser-based ultrafast X-ray scattering can be utilized to shed light on the microscopic mechanisms that determine materials properties. C1 [Jiang, M. P.; Trigo, M.; Bray, C.; Clark, J.; Henighan, T.; Kozina, M.; Lindenberg, A. M.; Zalden, P.; Reis, D. A.] SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA. [Jiang, M. P.; Trigo, M.; Henighan, T.; Kozina, M.; Lindenberg, A. M.; Zalden, P.; Reis, D. A.] SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA. [Jiang, M. P.; Henighan, T.] Stanford Univ, Dept Phys, Stanford, CA 94305 USA. [Savic, I.; Fahy, S.; Murray, E. D.] Tyndall Natl Inst, Lee Maltings Complex, Cork T12R 5CP, Ireland. [Savic, I.; Fahy, S.; Murray, E. D.] Univ Coll Cork, Dept Phys, Coll Rd, Cork, Ireland. [Murray, E. D.; Reis, D. A.] Imperial Coll London, Dept Phys & Mat, London SW7 2AZ, England. [Bray, C.; Kozina, M.] Stanford Univ, Dept Appl Phys, Stanford, CA 94305 USA. [Chollet, M.; Glownia, J. M.; Hoffmann, M. C.; Zhu, D.] SLAC Natl Accelerator Lab, Linac Coherent Light Source, Menlo Pk, CA 94025 USA. [Delaire, O.] Duke Univ, Dept Mech Engn & Mat Sci, Durham, NC 27708 USA. [Delaire, O.; May, A. F.; Sales, B. C.] Oak Ridge Natl Lab, Mat Sci & Technol Div, Oak Ridge, TN 37831 USA. [Lindenberg, A. M.; Zalden, P.] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA. [Sato, T.] RIKEN SPring 8 Ctr, Kouto 1-1-1, Sayo, Hyogo 6795148, Japan. [Sato, T.] Univ Tokyo, Sch Sci, Dept Chem, Bunkyo Ku, 7-3-1 Hongo, Tokyo 1130033, Japan. [Merlin, R.] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. RP Jiang, MP; Reis, DA (reprint author), SLAC Natl Accelerator Lab, Stanford PULSE Inst, Menlo Pk, CA 94025 USA.; Jiang, MP; Reis, DA (reprint author), SLAC Natl Accelerator Lab, Stanford Inst Mat & Energy Sci, Menlo Pk, CA 94025 USA.; Jiang, MP (reprint author), Stanford Univ, Dept Phys, Stanford, CA 94305 USA.; Reis, DA (reprint author), Imperial Coll London, Dept Phys & Mat, London SW7 2AZ, England. EM mpjiang@stanford.edu; dreis@stanford.edu RI Savic, Ivana/J-8556-2014; Hoffmann, Matthias/B-3893-2009; May, Andrew/E-5897-2011; Murray, Eamonn/J-8476-2014; OI Savic, Ivana/0000-0003-1503-3828; Hoffmann, Matthias/0000-0002-3596-9853; May, Andrew/0000-0003-0777-8539; Murray, Eamonn/0000-0003-1526-663X; Merlin, Roberto/0000-0002-5584-0248; Kozina, Michael/0000-0002-4747-345X FU Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division [DE-AC02-76SF00515]; Science Foundation Ireland; Marie Curie Action COFUND [11/SIRG/E2113]; Science Foundation Ireland [12/1A/1601]; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, through the Office of Science Early Career Research Program; U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division; Volkswagen Foundation; U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE AC02-76SF00515] FX This work is supported by the Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, under Contract DE-AC02-76SF00515. I.S. acknowledges support by Science Foundation Ireland and Marie Curie Action COFUND under Starting Investigator Research Grant 11/SIRG/E2113. S.F. and E.D.M. acknowledge support by Science Foundation Ireland under Grant No. 12/1A/1601. O.D. acknowledges support from the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division, through the Office of Science Early Career Research Program. A.F.M. and B.C.S. were supported by the U.S. Department of Energy, Office of Science, Basic Energy Sciences, Materials Sciences and Engineering Division. J.C. acknowledges financial support from the Volkswagen Foundation. Portions of this research were carried out at the Linac Coherent Light Source (LCLS) at the SLAC National Accelerator Laboratory. LCLS is an Office of Science User Facility operated for the U.S. Department of Energy Office of Science by Stanford University. Preliminary experiments were performed at SACLA with the approval of the Japan Synchrotron Radiation Research Institute (JASRI) (Proposal No. 2013A8038) and at the Stanford Synchrotron Radiation Light source, SLAC National Accelerator Laboratory, which like the LCLS is supported by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Contract No. DE AC02-76SF00515. NR 39 TC 2 Z9 2 U1 22 U2 29 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2016 VL 7 AR 12291 DI 10.1038/ncomms12291 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DS5ST UT WOS:000380843300001 PM 27447688 ER PT J AU Jin, HB Jiao, F Daily, MD Chen, YL Yan, F Ding, YH Zhang, X Robertson, EJ Baer, MD Chen, CL AF Jin, Haibao Jiao, Fang Daily, Michael D. Chen, Yulin Yan, Feng Ding, Yan-Huai Zhang, Xin Robertson, Ellen J. Baer, Marcel D. Chen, Chun-Long TI Highly stable and self-repairing membrane-mimetic 2D nanomaterials assembled from lipid-like peptoids SO Nature Communications LA English DT Article ID MECHANICAL CALCULATIONS; BIOMIMETIC MEMBRANES; FORCE-FIELD; NANOSHEETS; POLYMERS; NANOSTRUCTURES; FRAMEWORKS; PROTEINS; CHANNELS; BILAYERS AB An ability to develop sequence-defined synthetic polymers that both mimic lipid amphiphilicity for self-assembly of highly stable membrane-mimetic 2D nanomaterials and exhibit protein-like functionality would revolutionize the development of biomimetic membranes. Here we report the assembly of lipid-like peptoids into highly stable, crystalline, free-standing and self-repairing membrane-mimetic 2D nanomaterials through a facile crystallization process. Both experimental and molecular dynamics simulation results show that peptoids assemble into membranes through an anisotropic formation process. We further demonstrated the use of peptoid membranes as a robust platform to incorporate and pattern functional objects through large side-chain diversity and/or co-crystallization approaches. Similar to lipid membranes, peptoid membranes exhibit changes in thickness upon exposure to external stimuli; they can coat surfaces in single layers and self-repair. We anticipate that this new class of membrane-mimetic 2D nanomaterials will provide a robust matrix for development of biomimetic membranes tailored to specific applications. C1 [Jin, Haibao; Jiao, Fang; Daily, Michael D.; Chen, Yulin; Yan, Feng; Ding, Yan-Huai; Zhang, Xin; Baer, Marcel D.; Chen, Chun-Long] Pacific Northwest Natl Lab, Div Phys Sci, Richland, WA 99352 USA. [Jiao, Fang] East China Normal Univ, Sch Chem & Mol Engn, Shanghai 200241, Peoples R China. [Yan, Feng] Linyi Univ, Coll Chem & Chem Engn, Linyi 276005, Shandong, Peoples R China. [Ding, Yan-Huai] Xiangtan Univ, Inst Rheol Mech, Xiangtan 411105, Hunan, Peoples R China. [Robertson, Ellen J.] Lawrence Berkeley Natl Lab, Mol Foundry, Berkeley, CA 94720 USA. [Daily, Michael D.] Univ Texas Med Branch, Dept Biochem & Mol Biol, Galveston, TX 77555 USA. RP Chen, CL (reprint author), Pacific Northwest Natl Lab, Div Phys Sci, Richland, WA 99352 USA. EM Chunlong.Chen@pnnl.gov RI Zhang, Xin/I-9221-2014 OI Zhang, Xin/0000-0003-2000-858X FU Materials Synthesis and Simulation Across Scales (MS3) Initiative through the LDRD fund at Pacific Northwest National Laboratory (PNNL); US Department of Energy, Office of Basic Energy Sciences, Biomolecular Materials Program at PNNL; Molecular Foundry - Office of Science [DE-AC02-05CH11231]; China Scholarship Council; Department of Energy [DE-AC05-76RL01830]; DARPA Fold F(x) programme FX We thank R. Zuckermann, J.J. DeYoreo and C.J. Mundy for helpful discussions, and thank Caroline Proulx and Jing Sun for helping with X-ray diffraction measurements. This work was primarily supported by the Materials Synthesis and Simulation Across Scales (MS3) Initiative through the LDRD fund at Pacific Northwest National Laboratory (PNNL). In situ AFM studies and MD simulations were supported by the US Department of Energy, Office of Basic Energy Sciences, Biomolecular Materials Program at PNNL. X-ray diffraction work was conducted at the Advanced Light Source with support from the Molecular Foundry, at the Lawrence Berkeley National Laboratory, both of which are supported by the Office of Science, under Contrast No. DE-AC02-05CH11231. Peptoid synthesis was partially supported by the DARPA Fold F(x) programme. F.J. gratefully acknowledges financial support from China Scholarship Council. PNNL is a multiprogram national laboratory operated for Department of Energy by Battelle under Contracts No. DE-AC05-76RL01830. NR 36 TC 1 Z9 1 U1 34 U2 59 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2016 VL 7 AR 12252 DI 10.1038/ncomms12252 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DS4IQ UT WOS:000380745100001 PM 27402325 ER PT J AU Kampman, N Busch, A Bertier, P Snippe, J Hangx, S Pipich, V Di, Z Rother, G Harrington, JF Evans, JP Maskell, A Chapman, HJ Bickle, MJ AF Kampman, N. Busch, A. Bertier, P. Snippe, J. Hangx, S. Pipich, V. Di, Z. Rother, G. Harrington, J. F. Evans, J. P. Maskell, A. Chapman, H. J. Bickle, M. J. TI Observational evidence confirms modelling of the long-term integrity of CO2-reservoir caprocks SO Nature Communications LA English DT Article ID FLUID-ROCK INTERACTION; NATURAL CO2 RESERVOIR; CARBON-DIOXIDE; HYDROGEN-SULFIDE; STORAGE; GAS; TRANSPORT; IMPACT; SEQUESTRATION; DIFFUSION AB Storage of anthropogenic CO2 in geological formations relies on a caprock as the primary seal preventing buoyant super-critical CO2 escaping. Although natural CO2 reservoirs demonstrate that CO2 may be stored safely for millions of years, uncertainty remains in predicting how caprocks will react with CO2-bearing brines. This uncertainty poses a significant challenge to the risk assessment of geological carbon storage. Here we describe mineral reaction fronts in a CO2 reservoir-caprock system exposed to CO2 over a timescale comparable with that needed for geological carbon storage. The propagation of the reaction front is retarded by redox-sensitive mineral dissolution reactions and carbonate precipitation, which reduces its penetration into the caprock to similar to 7cm in similar to 10(5) years. This distance is an order-of-magnitude smaller than previous predictions. The results attest to the significance of transport-limited reactions to the long-term integrity of sealing behaviour in caprocks exposed to CO2. C1 [Kampman, N.; Busch, A.; Snippe, J.] Shell Global Solut Int, Kessler Pk 1, NL-2288 GS Rijswijk, Netherlands. [Kampman, N.; Maskell, A.; Chapman, H. J.; Bickle, M. J.] Univ Cambridge, Dept Earth Sci, Downing St, Cambridge CB2 3EQ, England. [Bertier, P.] Rhein Westfal TH Aachen, Clay & Interface Mineral, Bunsenstr 8, D-52072 Aachen, Germany. [Hangx, S.] Univ Utrecht, High Pressure & Temp Lab, POB 80 021, NL-3508 TA Utrecht, Netherlands. [Pipich, V.; Di, Z.] Forschungszentrum Julich, JCNS, Outstn Heinz Maier Leibnitz Zentrum MLZ, 1 Lichtenbergstr, D-85747 Garching, Germany. [Rother, G.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. [Harrington, J. F.] British Geol Survey, Ctr Environm Sci, Nottingham NG12 5GG, England. [Evans, J. P.] Utah State Univ, Dept Geol, 4505 Old Main Hill, Logan, UT 84322 USA. RP Bickle, MJ (reprint author), Univ Cambridge, Dept Earth Sci, Downing St, Cambridge CB2 3EQ, England. EM mb72@esc.cam.ac.uk RI Bertier, Pieter/K-3960-2016; Rother, Gernot/B-7281-2008; OI Bertier, Pieter/0000-0003-1770-412X; Rother, Gernot/0000-0003-4921-6294; Busch, Andreas/0000-0002-3279-5202 FU NERC [NE/F004699/1]; Shell Global Solutions, Center for Nanoscale Controls on Geologic CO2 (NCGC), an Energy Frontier Research Center - U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES) [DE-AC02-05CH11231]; DECC FX We thank DOSECC for carrying out the drilling, Morgan Schaller for coordinating activities on the drill site, the core logging team from Utah State University and staff at the Godwin Laboratory, Cambridge for O- and C-isotopic analyses. Funding was provided by NERC to the CRIUS consortium (NE/F004699/1), Shell Global Solutions, for GR as part of the Center for Nanoscale Controls on Geologic CO2 (NCGC), an Energy Frontier Research Center funded by the U.S. Department of Energy (DOE), Office of Science, Basic Energy Sciences (BES), under Award #DE-AC02-05CH11231, and DECC, which provided a CCS Innovation grant for completion of this work. Data from the British Geological Survey is published with the permission of the Executive Director, British Geological Survey (NERC). NR 53 TC 4 Z9 4 U1 11 U2 13 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2016 VL 7 AR 12268 DI 10.1038/ncomms12268 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DS2DB UT WOS:000380536100001 PM 27464840 ER PT J AU Poplawsky, JD Guo, W Paudel, N Ng, A More, K Leonard, D Yan, YF AF Poplawsky, Jonathan D. Guo, Wei Paudel, Naba Ng, Amy More, Karren Leonard, Donovan Yan, Yanfa TI Structural and compositional dependence of the CdTexSe1-x alloy layer photoactivity in CdTe-based solar cells SO Nature Communications LA English DT Article ID ATOM-PROBE TOMOGRAPHY; PSEUDOBINARY SYSTEM; 1ST-PRINCIPLES CALCULATION; CADMIUM TELLURIDE; GRAIN-BOUNDARIES; PHASE-DIAGRAM; THIN-FILMS; CDS AB The published external quantum efficiency data of the world-record CdTe solar cell suggests that the device uses bandgap engineering, most likely with a CdTexSe1-x alloy layer to increase the short-circuit current and overall device efficiency. Here atom probe tomography, transmission electron microscopy and electron beam-induced current are used to clarify the dependence of Se content on the photoactive properties of CdTexSe1-x alloy layers in bandgap-graded CdTe solar cells. Four solar cells were prepared with 50, 100, 200 and 400 nm-thick CdSe layers to reveal the formation, growth, composition, structure and photoactivity of the CdTexSe1-x alloy with respect to the degree of Se diffusion. The results show that the CdTexSe1-x layer photoactivity is highly dependent on the crystalline structure of the alloy (zincblende versus wurtzite), which is also dependent on the Se and Te concentrations. C1 [Poplawsky, Jonathan D.; Guo, Wei; More, Karren; Leonard, Donovan] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA. [Poplawsky, Jonathan D.; Guo, Wei; More, Karren; Leonard, Donovan] Oak Ridge Natl Lab, Dept Phys & Astron, Oak Ridge, TN 37831 USA. [Paudel, Naba; Yan, Yanfa] Univ Toledo, Dept Phys & Astron, McMaster Hall,2nd Floor Room 2017, Toledo, OH 43606 USA. [Ng, Amy] Vanderbilt Univ, Dept Chem, Stevenson Ctr 7330, Nashville, TN 37235 USA. [Ng, Amy] US Naval Res Lab, Mat Sci & Technol Div, 4555 Overlook Ave SW, Washington, DC 20375 USA. RP Poplawsky, JD (reprint author), Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.; Poplawsky, JD (reprint author), Oak Ridge Natl Lab, Dept Phys & Astron, Oak Ridge, TN 37831 USA. EM poplawskyjd@ornl.gov FU US Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy, Foundational Program to Advance Cell Efficiency [DE-FOA-0000492]; ORNL's Laboratory Directed Research and Development program FX This research was supported by the US Department of Energy (DOE) Office of Energy Efficiency and Renewable Energy, Foundational Program to Advance Cell Efficiency, grant number DE-FOA-0000492, and performed in part at ORNL's Center for Nanophase Materials Sciences, which is a DOE Office of Science User Facility. J.P. was supported in part by ORNL's Laboratory Directed Research and Development program. We thank Dorothy Coffey and Shawn Reeves for specimen preparation. NR 41 TC 1 Z9 1 U1 15 U2 25 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2016 VL 7 AR 12537 DI 10.1038/ncomms12537 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DS2DX UT WOS:000380540000001 PM 27460872 ER PT J AU Wagner, MR Lundberg, DS del Rio, TG Tringe, SG Dangl, JL Mitchell-Olds, T AF Wagner, Maggie R. Lundberg, Derek S. del Rio, Tijana G. Tringe, Susannah G. Dangl, Jeffery L. Mitchell-Olds, Thomas TI Host genotype and age shape the leaf and root microbiomes of a wild perennial plant SO Nature Communications LA English DT Article ID RHIZOSPHERE MICROBIOME; ECOSYSTEM GENETICS; FUNGAL PATHOGEN; PHYLLOSPHERE; ARABIDOPSIS; COMMUNITY; DIVERSITY; EVOLUTION; BACTERIA; TRAITS AB Bacteria living on and in leaves and roots influence many aspects of plant health, so the extent of a plant's genetic control over its microbiota is of great interest to crop breeders and evolutionary biologists. Laboratory-based studies, because they poorly simulate true environmental heterogeneity, may misestimate or totally miss the influence of certain host genes on the microbiome. Here we report a large-scale field experiment to disentangle the effects of genotype, environment, age and year of harvest on bacterial communities associated with leaves and roots of Boechera stricta (Brassicaceae), a perennial wild mustard. Host genetic control of the microbiome is evident in leaves but not roots, and varies substantially among sites. Microbiome composition also shifts as plants age. Furthermore, a large proportion of leaf bacterial groups are shared with roots, suggesting inoculation from soil. Our results demonstrate how genotype-by-environment interactions contribute to the complexity of microbiome assembly in natural environments. C1 [Wagner, Maggie R.; Mitchell-Olds, Thomas] Duke Univ, Dept Biol, Program Genet & Genom, Durham, NC 27708 USA. [Lundberg, Derek S.; Dangl, Jeffery L.] Univ N Carolina, Carolina Ctr Genome Sci, Dept Biol, Curriculum Genet & Mol Biol, Chapel Hill, NC 27599 USA. [del Rio, Tijana G.; Tringe, Susannah G.] Dept Energy Joint Genome Inst, Walnut Creek, CA 94598 USA. [Dangl, Jeffery L.] Univ N Carolina, Howard Hughes Med Inst, Dept Microbiol & Immunol, Chapel Hill, NC 27599 USA. [Wagner, Maggie R.] N Carolina State Univ, Dept Plant Pathol, Raleigh, NC 27695 USA. [Lundberg, Derek S.] Max Planck Inst Dev Biol, D-72076 Tubingen, Germany. RP Wagner, MR (reprint author), Duke Univ, Dept Biol, Program Genet & Genom, Durham, NC 27708 USA.; Wagner, MR (reprint author), N Carolina State Univ, Dept Plant Pathol, Raleigh, NC 27695 USA. EM maggie.r.wagner@gmail.com RI Mitchell-Olds, Thomas/K-8121-2012; OI Mitchell-Olds, Thomas/0000-0003-3439-9921; Wagner, Maggie/0000-0002-6924-7226 FU National Science Foundation [DEB-1311440, EF-0723447]; NIH Training Grant [5T32 GM007754-32, T32 GM07092-34]; American Philosophical Society Lewis and Clark Fund for Exploration and Field Research; National Institutes of Health [R01 GM086496]; NSF Microbial Systems Biology grant [IOS-0958245]; NSF INSPIRE Track II grant [IOS-1343020]; DOE Plant Feedstocks grant [DOE-SC0010423]; Howard Hughes Medical Institute; Gordon and Betty Moore Foundation [GBMF3030]; JGI Director's Discretionary Grand Challenge Program; JGI community Sequencing Project; Office of Science of the US Department of Energy [DE-AC02-05CH11231] FX We thank P. Busby, S. Herrera Paredes, J. Wernegreen and D. Weigel for valuable discussion and critical comments on the manuscript; D. Coleman-Derr for assistance with sample handling and sequencing; S. Herrera Paredes and S. Yourstone for use of their custom scripts; and J.T. Anderson, K. Ghattas, L. Heil, R. Keith, C.-R. Lee, J. Lipkowitz, A. Manzaneda, T. Park, M. Rozen and C. Rushworth for assistance in the greenhouse and field. M.R.W. was supported by a Graduate Research Fellowship and a Doctoral Dissertation Improvement Grant DEB-1311440 from the National Science Foundation, NIH Training Grant 5T32 GM007754-32, and the American Philosophical Society Lewis and Clark Fund for Exploration and Field Research. T.M.-O. was supported by grant R01 GM086496 from the National Institutes of Health and EF-0723447 from the National Science Foundation. J.L.D. was supported by NSF Microbial Systems Biology grant IOS-0958245, NSF INSPIRE Track II grant IOS-1343020 and DOE Plant Feedstocks grant DOE-SC0010423. D.S.L. was supported by NIH Training Grant T32 GM07092-34. J.L.D. is an Investigator of the Howard Hughes Medical Institute and support was provided by the Howard Hughes Medical Institute and the Gordon and Betty Moore Foundation (in part via Grant GBMF3030 to J.L.D.). This work was also funded by the JGI Director's Discretionary Grand Challenge Program, and a JGI community Sequencing Project (S.G.T., J.L.D. and T.M.-O.). Work conducted by the US Department of Energy Joint Genome Institute, a DOE Office of Science User Facility, is supported by the Office of Science of the US Department of Energy under Contract No. DE-AC02-05CH11231. NR 70 TC 6 Z9 6 U1 45 U2 83 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2016 VL 7 AR 12151 DI 10.1038/ncomms12151 PG 15 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DS4IJ UT WOS:000380744400001 PM 27402057 ER PT J AU Wang, QS Shen, Y Pan, BY Zhang, XW Ikeuchi, K Iida, K Christianson, AD Walker, HC Adroja, DT Abdel-Hafiez, M Chen, XJ Chareev, DA Vasiliev, AN Zhao, J AF Wang, Qisi Shen, Yao Pan, Bingying Zhang, Xiaowen Ikeuchi, K. Iida, K. Christianson, A. D. Walker, H. C. Adroja, D. T. Abdel-Hafiez, M. Chen, Xiaojia Chareev, D. A. Vasiliev, A. N. Zhao, Jun TI Magnetic ground state of FeSe SO Nature Communications LA English DT Article ID PHASE-DIAGRAM; SUPERCONDUCTIVITY; FILMS; EXCITATIONS AB Elucidating the nature of the magnetism of a high-temperature superconductor is crucial for establishing its pairing mechanism. The parent compounds of the cuprate and iron-pnictide superconductors exhibit Neel and stripe magnetic order, respectively. However, FeSe, the structurally simplest iron-based superconductor, shows nematic order (T-s = 90 K), but not magnetic order in the parent phase, and its magnetic ground state is intensely debated. Here we report inelastic neutron-scattering experiments that reveal both stripe and Neel spin fluctuations over a wide energy range at 110 K. On entering the nematic phase, a substantial amount of spectral weight is transferred from the Neel to the stripe spin fluctuations. Moreover, the total fluctuating magnetic moment of FeSe is similar to 60% larger than that in the iron pnictide BaFe2As2. Our results suggest that FeSe is a novel S = 1 nematic quantum-disordered paramagnet interpolating between the Neel and stripe magnetic instabilities. C1 [Wang, Qisi; Shen, Yao; Pan, Bingying; Zhang, Xiaowen; Zhao, Jun] Fudan Univ, State Key Lab Surface Phys, Shanghai 200433, Peoples R China. [Wang, Qisi; Shen, Yao; Pan, Bingying; Zhang, Xiaowen; Zhao, Jun] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China. [Ikeuchi, K.; Iida, K.] Comprehens Res Org Sci & Soc, Res Ctr Neutron Sci & Technol, Tokai, Ibaraki 3191106, Japan. [Christianson, A. D.] Oak Ridge Natl Lab, Quantum Condensed Matter Div, Oak Ridge, TN 37831 USA. [Christianson, A. D.] Univ Tennessee, Dept Phys & Astron, Knoxville, TN 37996 USA. [Walker, H. C.; Adroja, D. T.] STFC, Rutherford Appleton Lab, ISIS Facil, Didcot OX11 0QX, Oxon, England. [Abdel-Hafiez, M.; Chen, Xiaojia] Ctr High Pressure Sci & Technol Adv Res, Shanghai 201203, Peoples R China. [Abdel-Hafiez, M.] Fayoum Univ, Fac Sci, Dept Phys, Al Fayyum 63514, Egypt. [Chareev, D. A.] Russian Acad Sci, Inst Expt Mineral, Chernogolovka 142432, Russia. [Chareev, D. A.; Vasiliev, A. N.] Ural Fed Univ, Inst Phys & Technol, Ekaterinburg 620002, Russia. [Vasiliev, A. N.] Moscow MV Lomonosov State Univ, Low Temp Phys & Supercond Dept, Moscow 119991, Russia. [Vasiliev, A. N.] Natl Univ Sci & Technol MISiS, Moscow 119049, Russia. [Zhao, Jun] Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China. RP Zhao, J (reprint author), Fudan Univ, State Key Lab Surface Phys, Shanghai 200433, Peoples R China.; Zhao, J (reprint author), Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China.; Zhao, J (reprint author), Collaborat Innovat Ctr Adv Microstruct, Nanjing 210093, Jiangsu, Peoples R China. EM zhaoj@fudan.edu.cn RI Chareev, Dmitriy/B-8504-2009; BL18, ARCS/A-3000-2012; Vasiliev, Alexander/A-7562-2008; christianson, andrew/A-3277-2016; Zhao, Jun/A-2492-2010; Walker, Helen/C-4201-2011 OI Chareev, Dmitriy/0000-0002-9380-2680; christianson, andrew/0000-0003-3369-5884; Zhao, Jun/0000-0002-0421-8934; Walker, Helen/0000-0002-7859-5388 FU Ministry of Science and Technology of China (973 project) [2015CB921302]; National Natural Science Foundation of China [11374059]; Shanghai Pujiang Scholar Program [13PJ1401100]; Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy; Ministry of Education and Science of the Russian Federation [2-2014-036]; Russian Foundation for Basic Research [13-02-00174, 14-02-92002, 14-02-92693]; Act 211 Government of the Russian Federation [02.A03.21.0006] FX We gratefully acknowledge H. Cao for the neutron diffraction experimental support, and Q. Si, R. Yu, A. Kreisel, P. Hirschfeld, B. M. Andersen and R. Valenti for discussions. This work was supported by the Ministry of Science and Technology of China (973 project: 2015CB921302), the National Natural Science Foundation of China (No. 11374059) and the Shanghai Pujiang Scholar Program (No. 13PJ1401100). Research at the Spallation Neutron Source of Oak Ridge National Laboratory was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy. A.N.V. was supported in part by the Ministry of Education and Science of the Russian Federation in the framework of the Increase Competitiveness Program of NUST 'MISiS' (No. 2-2014-036). D.A.C. and A.N.V. also acknowledge the support of the Russian Foundation for Basic Research through grants 13-02-00174, 14-02-92002, 14-02-92693 and Act 211 Government of the Russian Federation (No. 02.A03.21.0006). NR 28 TC 8 Z9 8 U1 33 U2 47 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2016 VL 7 AR 12182 DI 10.1038/ncomms12182 PG 7 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DS5GX UT WOS:000380810800001 PM 27431986 ER PT J AU Rinehart, AJ McKenna, SA Dewers, TA AF Rinehart, Alex J. McKenna, Sean A. Dewers, Thomas A. TI Using Wavelet Covariance Models for Simultaneous Picking of Overlapping P- and S-Wave Arrival Times in Noisy Single-Component Data SO SEISMOLOGICAL RESEARCH LETTERS LA English DT Article ID SEISMOGRAMS; STRATEGIES AB We present a method for automatically identifying overlapping elastice-waveelastice-wave phase arrivals in single-component data. The algorithm applies to traditional near-source seismic, microseismicity and picoseismicity monitoring, and acoustic emission monitoring; we use acoustic emissions examples as a worst-case demonstration. These signals have low signal-to-noise and, because of small geometric dimensions, overlapping P-and S-wave arrivals. Our method uses the statistics of temporal covariance across many wavelet scales. We use a nonnormalized rectilinity function of the scale covariance. The workflow begins by denoising signals and making a rough first-arrival estimate. We then perform a continuous Daubechies wavelet transform over tens to hundreds of scales on the signal and find a moving covariance across transform scales. The nonnormalized rectilinity is calculated for each of the covariance matrices, and we sharpen changes in the rectilinity values with a maximization filter. We then estimate phase arrival times using thresholds of the filtered rectilinity. Overall, we have a high success rate for both P-and S-wave arrivals. Remaining challenges include estimation of arrival times of long duration, cigar-shape events, and culling complex high-magnitude electrical noise. By using higher-order Daubechies wavelet transforms, the scale covariance metric reflects variations in higher-moment statistics (skewness and kurtosis) and changes in short-term versus long-term means, as well as the covariance across timescales of the signal. For single- component data, it is necessary to preserve both amplitude and correlation information of the signal; this necessitates using the nonnormalized rectilinity function. C1 [Rinehart, Alex J.] New Mexico Bur Geol, Aquifer Mapping Program, 801 Leroy Pl, Socorro, NM 87801 USA. [McKenna, Sean A.] IBM Research Ireland, Constrained Resources & Environm Analyt Dept, Bldg 3,Damastown Ind Estate, Dublin 15, Ireland. [Dewers, Thomas A.] Sandia Natl Labs, Geomech Dept, POB 5800,MS 0735, Albuquerque, NM 87185 USA. RP Rinehart, AJ (reprint author), New Mexico Bur Geol, Aquifer Mapping Program, 801 Leroy Pl, Socorro, NM 87801 USA. EM arinehart@nmbg.nmt.edu; seanmcke@ie.ibm.com; tdewers@sandia.gov FU Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-SC0001114]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This material is based upon work supported as part of the Center for Frontiers of Subsurface Energy Security, an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences under Award Number DE-SC0001114. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 19 TC 0 Z9 0 U1 3 U2 3 PU SEISMOLOGICAL SOC AMER PI ALBANY PA 400 EVELYN AVE, SUITE 201, ALBANY, CA 94706-1375 USA SN 0895-0695 EI 1938-2057 J9 SEISMOL RES LETT JI Seismol. Res. Lett. PD JUL PY 2016 VL 87 IS 4 BP 893 EP 900 DI 10.1785/0220150130 PG 8 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DP4TU UT WOS:000378490100012 ER PT J AU Gibbons, SJ Kvaerna, T Harris, DB Dodge, DA AF Gibbons, Steven J. Kvaerna, Tormod Harris, David B. Dodge, Douglas A. TI Iterative Strategies for Aftershock Classification in Automatic Seismic Processing Pipelines SO SEISMOLOGICAL RESEARCH LETTERS LA English DT Article ID EMPIRICAL SIGNAL DETECTORS; WAVE-FORM CORRELATION; EARTHQUAKE SEQUENCE; MONITORING-SYSTEM; EVENT LOCATION; 7.8 GORKHA; NETWORK; TIME; NEPAL; MOTION AB Aftershock sequences following very large earthquakes present enormous challenges to near-real-time generation of seismic bulletins. The increase in analyst resources needed to relocate an inflated number of events is compounded by failures of phaseassociation algorithms and a significant deterioration in the quality of underlying, fully automatic event bulletins. Current processing pipelines were designed a generation ago, and, due to computational limitations of the time, are usually limited to single passes over the raw data. With current processing capability, multiple passes over the data are feasible. Processing the raw data at each station currently generates parametric data streams that are then scanned by a phase-association algorithm to form event hypotheses. We consider the scenario in which a large earthquake has occurred and propose to define a region of likely aftershock activity in which events are detected and accurately located, using a separate specially targeted semiautomatic process. This effort may focus on so-called pattern detectors, but here we demonstrate a more general grid-search algorithm that may cover wider source regions without requiring waveform similarity. Given many well-located aftershocks within our source region, we may remove all associated phases from the original detection lists prior to a new iteration of the phase-association algorithm. We provide a proof-of-concept example for the 2015 Gorkha sequence, Nepal, recorded on seismic arrays of the International Monitoring System. Even with very conservative conditions for defining event hypotheses within the aftershock source region, we can automatically remove about half of the original detections that could have been generated by Nepal earthquakes and reduce the likelihood of false associations and spurious event hypotheses. Further reductions in the number of detections in the parametric data streams are likely, using correlation and subspace detectors and/ or empirical matched field processing. C1 [Gibbons, Steven J.; Kvaerna, Tormod] NORSAR, POB 53, N-2027 Kjeller, Norway. [Harris, David B.] Deschutes Signal Proc LLC, 81211 East Wapinitia Rd, Maupin, OR 97037 USA. [Dodge, Douglas A.] Lawrence Livermore Natl Lab, 7000 East Ave,Mail Stop 046, Livermore, CA 94550 USA. RP Gibbons, SJ (reprint author), NORSAR, POB 53, N-2027 Kjeller, Norway. EM steven@norsar.no; tormod@norsar.no; oregondsp@gmail.com; dodge1@llnl.gov OI Gibbons, Steven J./0000-0002-7822-0244 FU Air Force Research Laboratory [FA9453-13-C-0270]; Norwegian Ministry of Foreign Affairs; U.S. Department of Energy by Lawrence Livermore National Laboratory (LLNL), Lawrence Livermore National Security, LLC [DE-AC52-07NA27344] FX This work was supported in part by the Air Force Research Laboratory under Contract Number FA9453-13-C-0270 and in part by the Norwegian Ministry of Foreign Affairs. It was also performed in part under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory (LLNL) under Contract DE-AC52-07NA27344, Lawrence Livermore National Security, LLC. This is LLNL Contribution LLNL-JRNL-683501. All maps were generated by the Generic Mapping Tool (GMT) package (Wessel and Smith, 1995). NR 35 TC 0 Z9 0 U1 3 U2 4 PU SEISMOLOGICAL SOC AMER PI ALBANY PA 400 EVELYN AVE, SUITE 201, ALBANY, CA 94706-1375 USA SN 0895-0695 EI 1938-2057 J9 SEISMOL RES LETT JI Seismol. Res. Lett. PD JUL PY 2016 VL 87 IS 4 BP 919 EP 929 DI 10.1785/0220160047 PG 11 WC Geochemistry & Geophysics SC Geochemistry & Geophysics GA DP4TU UT WOS:000378490100015 ER PT J AU Sun, SQ Wang, D Russell, TP Zhang, LQ AF Sun, Shuquan Wang, Dong Russell, Thomas P. Zhang, Liqun TI Nanomechanical Mapping of a Deformed Elastomer: Visualizing a Self-Reinforcement Mechanism SO ACS MACRO LETTERS LA English DT Article ID STRAIN-INDUCED CRYSTALLIZATION; ATOMIC-FORCE MICROSCOPY; X-RAY-DIFFRACTION; NATURAL-RUBBER; UNIAXIAL DEFORMATION; ELECTRON-MICROSCOPY; SYNTHETIC RUBBERS; ORIENTATION; MORPHOLOGY; SULFUR AB Mapping the structure evolution and mechanical properties of elastic polymers or biomaterials during bulk deformation has been difficult, yet this information has long been thought to be key for understanding the structure-mechanical property relationship necessary to guide the design of new materials. Here we use a nanomechanical mapping to assess the structural evolution and mechanical properties of a deformed isoprene rubber (IR) to elucidate a self-reinforcement mechanism in this material. A hierarchical nanofibrillar structure, ranging from several to a hundred nanometers in size, comprised of fibers oriented parallel to the stretching direction was found. The nanofibers, connected by oriented amorphous tie chains, form a network structure that is responsible for significantly enhanced stress, a key factor giving rise to the self-reinforcement of IR and, more than likely, most elastomers that undergo strained-induced crystallization. C1 [Sun, Shuquan; Wang, Dong; Zhang, Liqun] Beijing Univ Chem Technol, Coll Mat Sci & Engn, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China. [Russell, Thomas P.] Univ Massachusetts, Dept Polymer Sci & Engn, Amherst, MA 01003 USA. [Russell, Thomas P.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Russell, Thomas P.] Beijing Univ Chem Technol, Beijing Adv Innovat Ctr Soft Matter Sci & Engn, Beijing 100029, Peoples R China. RP Wang, D; Zhang, LQ (reprint author), Beijing Univ Chem Technol, Coll Mat Sci & Engn, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China. EM dwang@mail.buct.edu.cn; zhanglq@mail.buct.edu.cn RI zhang, liqun/S-7337-2016 OI zhang, liqun/0000-0003-0291-4351 FU National 973 Basic Research Program of China [2015CB654700(2015CB654704)]; Foundation for Innovative Research Groups of the NSF of China [51221002]; Major International Cooperation of the National Nature Science Foundation of China [51320105012] FX We would like to thank Prof. Ken Nakajima, Dr. So Fujinami, and Dr. Xiaobin Liang for valuable discussions on the JKR analysis and assistance with the experiments. We gratefully acknowledge financial support from the National 973 Basic Research Program of China 2015CB654700(2015CB654704), the Foundation for Innovative Research Groups of the NSF of China (51221002), and the Major International Cooperation(51320105012) of the National Nature Science Foundation of China. NR 44 TC 1 Z9 1 U1 16 U2 20 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2161-1653 J9 ACS MACRO LETT JI ACS Macro Lett. PD JUL PY 2016 VL 5 IS 7 BP 839 EP 843 DI 10.1021/acsmacrolett.6b00278 PG 5 WC Polymer Science SC Polymer Science GA DS0OG UT WOS:000380296000013 ER PT J AU Gmernicki, KR Hong, E Maroon, CR Mahurin, SM Sokolov, AP Saito, T Long, BK AF Gmernicki, Kevin R. Hong, Eunice Maroon, Christopher R. Mahurin, Shannon M. Sokolov, Alexei P. Saito, Tomonori Long, Brian K. TI Accessing Siloxane Functionalized Polynorbornenes via Vinyl-Addition Polymerization for CO2 Separation Membranes SO ACS MACRO LETTERS LA English DT Article ID GAS SEPARATION; SURFACE FLUORINATION; TRANSPORT-PROPERTIES; TRIBLOCK COPOLYMER; BLOCK-COPOLYMERS; ION-BEAM; POLYIMIDE; PERMEABILITY; FILMS; POLYSTYRENE AB The vinyl addition polymerization of norbornyl-based monomers bearing polar functional groups is often problematic, leading to low molecular weight polymers in poor yield. Herein, we provide proof-of-principle evidence that addition-type homopolymers of siloxane substituted norbornyl-based monomers may be readily synthesized using the catalyst trans-[Ni(C6F5)(2)(SbPh3)(2)]. Polymerizations using this catalyst reached moderate to high conversion in just 5 min of polymerization and produced siloxane-substituted polymers with molecular weights exceeding 100 kg/mol. These polymers showed excellent thermal stability (T-d >= 362 degrees C) and were cast into membranes that displayed high CO2 permeability and enhanced CO2/N-2 selectivity as compared to related materials. C1 [Gmernicki, Kevin R.; Hong, Eunice; Maroon, Christopher R.; Sokolov, Alexei P.; Long, Brian K.] Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. [Mahurin, Shannon M.; Sokolov, Alexei P.; Saito, Tomonori] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA. RP Long, BK (reprint author), Univ Tennessee, Dept Chem, Knoxville, TN 37996 USA. EM long@utk.edu FU UTK/ORNL Science Alliance Joint Directed Research and Development program; Laboratory Directed Research and Development Program of Oak Ridge National Laboratory FX The authors acknowledge the UTK/ORNL Science Alliance Joint Directed Research and Development program for their financial support of this work. T.S., S.M.M., and A.P.S. were sponsored by the Laboratory Directed Research and Development Program of Oak Ridge National Laboratory, managed by UT-Battelle, LLC, for the U.S. Department of Energy. The authors would like to thank Prof. Benny Freeman and Dr. Kevin Stevens for their advice, guidance, and assistance in the construction of the permeation instrument used herein. The authors would like to thank Albemarle Corp. for generously providing the MAO used in this study. NR 28 TC 1 Z9 1 U1 11 U2 14 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2161-1653 J9 ACS MACRO LETT JI ACS Macro Lett. PD JUL PY 2016 VL 5 IS 7 BP 879 EP 883 DI 10.1021/acsmacrolett.6b00435 PG 5 WC Polymer Science SC Polymer Science GA DS0OG UT WOS:000380296000021 ER PT J AU Bassalo, MC Garst, AD Halweg-Edwards, AL Grau, WC Domaille, DW Mutalik, VK Arkin, AP Gill, RT AF Bassalo, Marcelo C. Garst, Andrew D. Halweg-Edwards, Andrea L. Grau, William C. Domaille, Dylan W. Mutalik, Vivek K. Arkin, Adam P. Gill, Ryan T. TI Rapid and Efficient One-Step Metabolic Pathway Integration in E-coli SO ACS SYNTHETIC BIOLOGY LA English DT Article DE genome integration; metabolic pathways; CRISPR; synthetic biology; genome editing ID GENE-EXPRESSION; RECA PROTEIN; GENOME; SYSTEMS; REPLACEMENT; COMPLEX; CLONING; K-12 AB Methods for importing heterologous genes into genetically tractable hosts are among the most desired tools of synthetic biology. Easy plug-and-play construction methods to rapidly test genes and pathways stably in the host genome would expedite synthetic biology and metabolic engineering applications. Here, we describe a CRISPR-based strategy that allows highly efficient, single step integration of large pathways in Escherichia coli. This strategy allows high efficiency integration in a broad range of homology arm sizes and genomic positions, with efficiencies ranging from 70 to 100% in 7 distinct loci. To demonstrate the large size capability, we integrated a 10 kb construct to implement isobutanol production in a single day. The ability to efficiently integrate entire metabolic pathways in a rapid and markerless manner will facilitate testing and engineering of novel pathways using the E. coli genome as a stable testing platform. C1 [Bassalo, Marcelo C.] Univ Colorado, Dept Mol Cellular & Dev Biol, Boulder, CO 80303 USA. [Bassalo, Marcelo C.; Garst, Andrew D.; Halweg-Edwards, Andrea L.; Grau, William C.; Domaille, Dylan W.; Gill, Ryan T.] Univ Colorado, Dept Chem & Biol Engn, Boulder, CO 80303 USA. [Grau, William C.] Univ Colorado, Dept Chem & Biochem, Boulder, CO 80303 USA. [Mutalik, Vivek K.; Arkin, Adam P.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Mutalik, Vivek K.; Arkin, Adam P.] Dept Bioengn, Berkeley, CA 94720 USA. RP Gill, RT (reprint author), Univ Colorado, Dept Chem & Biol Engn, Boulder, CO 80303 USA. EM rtg@colorado.edu OI Mutalik, Vivek/0000-0001-7934-0400; Arkin, Adam/0000-0002-4999-2931 FU US Department of Energy [DE-SC0008812]; CAPES foundation [0315133] FX Special thanks for G. Pines for advice on this work. We also thank G.S. Teixeira for assistance with yeast cloning approaches. We would like to thank J. Dragavon at the Colorado BioFrontiers Advanced Light Microscopy Core for assistance with fluorescence microscopy. We also thank the Flow Cytometry Shared Resource in University of Colorado Anschutz Medical Campus. This work was supported by the US Department of Energy (Grant DE-SC0008812) and CAPES foundation (Grant #0315133). NR 36 TC 4 Z9 5 U1 16 U2 26 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2161-5063 J9 ACS SYNTH BIOL JI ACS Synth. Biol. PD JUL PY 2016 VL 5 IS 7 BP 561 EP 568 DI 10.1021/acssynbio.5b00187 PG 8 WC Biochemical Research Methods SC Biochemistry & Molecular Biology GA DR8XZ UT WOS:000380183000004 PM 27072506 ER PT J AU Kosina, SM Danielewicz, MA Mohammed, M Ray, J Suh, Y Yilmaz, S Singh, AK Arkin, AP Deutschbauer, AM Northen, TR AF Kosina, Suzanne M. Danielewicz, Megan A. Mohammed, Mujahid Ray, Jayashree Suh, Yumi Yilmaz, Suzan Singh, Anup K. Arkin, Adam P. Deutschbauer, Adam M. Northen, Trent R. TI Exometabolomics Assisted Design and Validation of Synthetic Obligate Mutualism SO ACS SYNTHETIC BIOLOGY LA English DT Article DE microbial synthetic biology; synthetic obligate mutualism; exometabolomics; mutant fitness profiling; cross feeding; mass spectrometry ID ESCHERICHIA-COLI; ZYMOMONAS-MOBILIS; MUTANT LIBRARIES; DETERMINANTS; PRODUCTIVITY; EVOLUTION; CONSORTIA; BACTERIA; REVEALS; GENES AB Synthetic microbial ecology has the potential to enhance the productivity and resiliency of biotechnology processes compared to approaches using single isolates. Engineering microbial consortia is challenging; however, one approach that has attracted significant attention is the creation of synthetic obligate mutualism using auxotrophic mutants that depend on each other for exchange or cross-feeding of metabolites. Here, we describe the integration of mutant library fitness profiling with mass spectrometry based exometabolomics as a method for constructing synthetic mutualism based on cross-feeding. Two industrially important species lacking known ecological interactions, Zymomonas mobilis and Escherichia coli, were selected as the test species. Amino acid exometabolites identified in the spent medium of Z. mobilis were used to select three corresponding E. coli auxotrophs (proA, pheA and IlvA), as potential E. coli counterparts for the coculture. A pooled mutant fitness assay with a Z. mobilis transposon mutant library was used to identify mutants with improved growth in the presence of E. coli. An auxotroph mutant in a gene (ZMO0748) with sequence similarity to cysteine synthase A (cysK), was selected as the Z. mobilis counterpart for the coculture. Exometabolomic analysis of spent E. coli medium identified glutathione related metabolites as potentially available for rescue of the Z. mobilis cysteine synthase mutant. Three sets of cocultures between the Z. mobilis auxotroph and each of the three E. coli auxotrophs were monitored by optical density for growth and analyzed by flow cytometry to confirm high cell counts for each species. Taken together, our methods provide a technological framework for creating synthetic mutualisms combining existing screening based methods and exometabolomics for both the selection of obligate mutualism partners and elucidation of metabolites involved in auxotroph rescue. C1 [Kosina, Suzanne M.; Danielewicz, Megan A.; Mohammed, Mujahid; Ray, Jayashree; Suh, Yumi; Arkin, Adam P.; Deutschbauer, Adam M.; Northen, Trent R.] Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. [Arkin, Adam P.] Univ Calif Berkeley, Berkeley, CA 94720 USA. [Yilmaz, Suzan; Singh, Anup K.] Sandia Natl Labs, Livermore, CA 94550 USA. RP Northen, TR (reprint author), Lawrence Berkeley Natl Lab, Berkeley, CA 94720 USA. EM trnorthen@lbl.gov OI Arkin, Adam/0000-0002-4999-2931; Northen, Trent/0000-0001-8404-3259 FU U.S. Department of Energy, Office of Science, Office of Biological & Environmental Research [DE-AC02-05CH11231] FX This material by ENIGMA-Ecosystems and Networks Integrated with Genes and Molecular Assemblies (hap://enigma.1131.gov), a Scientific Focus Area Program at Lawrence Berkeley National Laboratory is based upon work supported by the U.S. Department of Energy, Office of Science, Office of Biological & Environmental Research under contract number DE-AC02-05CH11231. We thank Morgan N. Price (Lawrence Berkeley National Laboratory) for processing the Z. mobilis mutant fitness assay data. NR 46 TC 1 Z9 1 U1 15 U2 22 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2161-5063 J9 ACS SYNTH BIOL JI ACS Synth. Biol. PD JUL PY 2016 VL 5 IS 7 BP 569 EP 576 DI 10.1021/acssynbio.5b00236 PG 8 WC Biochemical Research Methods SC Biochemistry & Molecular Biology GA DR8XZ UT WOS:000380183000005 PM 26885935 ER PT J AU Jensen, HM TerAvest, MA Kokish, MG Ajo-Franklin, CM AF Jensen, Heather M. TerAvest, Michaela A. Kokish, Mark G. Ajo-Franklin, Caroline M. TI CymA and Exogenous Flavins Improve Extracellular Electron Transfer and Couple It to Cell Growth in Mtr-Expressing Escherichia coli SO ACS SYNTHETIC BIOLOGY LA English DT Article DE synthetic biology; dissimilatory metal-reducing bacteria; bioelectrochemical systems; energy conservation; multiheme cytochrome c ID SHEWANELLA-ONEIDENSIS MR-1; PSEUDOMONAS-PUTIDA KT2440; DISSIMILATORY IRON REDUCTION; RESPIRATORY FLEXIBILITY; TRANSFER MECHANISMS; PUTREFACIENS MR-1; MINERALS; METABOLISM; REDUCTASES; BACTERIUM AB Introducing extracellular electron transfer pathways into heterologous organisms offers the opportunity to explore fundamental biogeochemical processes and to biologically alter redox states of exogenous metals for various applications. While expression of the MtrCAB electron nanoconduit from Shewanella oneidensis MR-1 permits extracellular electron transfer in Escherichia coli, the low electron flux and absence of growth in these cells limits their practicality for such applications. Here we investigate how the rate of electron transfer to extracellular Fe(111) and cell survival in engineered E. coli are affected by mimicking different features of the S. oneidensis pathway: the number of electron nanoconduits, the link between the quinol pool and MtrA, and the presence of flavin-dependent electron transfer. While increasing the number of pathways does not significantly improve the extracellular electron transfer rate or cell survival, using the native inner membrane component, CymA, significantly improves the reduction rate of extracellular acceptors and increases cell viability. Strikingly, introducing both CymA and riboflavin to Mtr-expressing E. coli also allowed these cells to couple metal reduction to growth, which is the first time an increase in biomass of an engineered E. coli has been observed under Fe2O3 (s) reducing conditions. Overall, this work provides engineered E. coli strains for modulating extracellular metal reduction and elucidates critical factors for engineering extracellular electron transfer in heterologous organisms. C1 [Jensen, Heather M.; Ajo-Franklin, Caroline M.] Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA. [Kokish, Mark G.; Ajo-Franklin, Caroline M.] Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA. [Jensen, Heather M.; Kokish, Mark G.] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA. [Ajo-Franklin, Caroline M.] Synthet Biol Inst, Berkeley, CA 94720 USA. [TerAvest, Michaela A.] Univ Calif Berkeley, Calif Inst Quantitat Biosci, Berkeley, CA 94720 USA. [Jensen, Heather M.] Joint BioEnergy Inst, Emeryville, CA USA. [TerAvest, Michaela A.] Michigan State Univ, E Lansing, MI 48824 USA. [Kokish, Mark G.] Northwestern Univ, Evanston, IL USA. RP Ajo-Franklin, CM (reprint author), Lawrence Berkeley Natl Lab, Phys Biosci Div, Berkeley, CA 94720 USA.; Ajo-Franklin, CM (reprint author), Lawrence Berkeley Natl Lab, Div Mat Sci, Berkeley, CA 94720 USA.; Ajo-Franklin, CM (reprint author), Synthet Biol Inst, Berkeley, CA 94720 USA. EM cajo-franklin@lbl.gov FU Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-O5CH11231]; Physical Biosciences Program, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231]; Office of Naval Research [N000141310551]; Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy [DE-AC02-05CH11231.] FX Work at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-O5CH11231. CMAF and HMJ acknowledge support from the Physical Biosciences Program, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. CMAF and MAT acknowledge support from Office of Naval Research, Award number N000141310551. This work was supported in part by previous breakthroughs obtained through the Laboratory Directed Research and Development Program of Lawrence Berkeley National Laboratory under U.S. Department of Energy Contract No. DE-AC02-05CH11231. NR 50 TC 1 Z9 1 U1 13 U2 19 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 2161-5063 J9 ACS SYNTH BIOL JI ACS Synth. Biol. PD JUL PY 2016 VL 5 IS 7 BP 679 EP 688 DI 10.1021/acssynbio.5b00279 PG 10 WC Biochemical Research Methods SC Biochemistry & Molecular Biology GA DR8XZ UT WOS:000380183000017 PM 27000939 ER PT J AU Hameed, A Khoshkbarforoushha, A Ranjan, R Jayaraman, PP Kolodziej, J Balaji, P Zeadally, S Malluhi, QM Tziritas, N Vishnu, A Khan, SU Zomaya, A AF Hameed, Abdul Khoshkbarforoushha, Alireza Ranjan, Rajiv Jayaraman, Prem Prakash Kolodziej, Joanna Balaji, Pavan Zeadally, Sherali Malluhi, Qutaibah Marwan Tziritas, Nikos Vishnu, Abhinav Khan, Samee U. Zomaya, Albert TI A survey and taxonomy on energy efficient resource allocation techniques for cloud computing systems SO COMPUTING LA English DT Article DE Cloud computing; Energy efficiency; Energy efficient resource allocation; Energy consumption; Power management ID DATA CENTERS; PERFORMANCE MANAGEMENT; POWER; NETWORKS; CHALLENGES AB In a cloud computing paradigm, energy efficient allocation of different virtualized ICT resources (servers, storage disks, and networks, and the like) is a complex problem due to the presence of heterogeneous application (e.g., content delivery networks, MapReduce, web applications, and the like) workloads having contentious allocation requirements in terms of ICT resource capacities (e.g., network bandwidth, processing speed, response time, etc.). Several recent papers have tried to address the issue of improving energy efficiency in allocating cloud resources to applications with varying degree of success. However, to the best of our knowledge there is no published literature on this subject that clearly articulates the research problem and provides research taxonomy for succinct classification of existing techniques. Hence, the main aim of this paper is to identify open challenges associated with energy efficient resource allocation. In this regard, the study, first, outlines the problem and existing hardware and software-based techniques available for this purpose. Furthermore, available techniques already presented in the literature are summarized based on the energy-efficient research dimension taxonomy. The advantages and disadvantages of the existing techniques are comprehensively analyzed against the proposed research dimension taxonomy namely: resource adaption policy, objective function, allocation method, allocation operation, and interoperability. C1 [Hameed, Abdul; Khan, Samee U.] North Dakota State Univ, Fargo, ND USA. [Khoshkbarforoushha, Alireza] Australian Natl Univ, Canberra, ACT, Australia. [Ranjan, Rajiv; Jayaraman, Prem Prakash] CSIRO, Canberra, ACT, Australia. [Kolodziej, Joanna] Cracow Univ Technol, Krakow, Poland. [Balaji, Pavan] Argonne Natl Lab, Lemont, IL USA. [Zeadally, Sherali] Univ Dist Columbia, Washington, DC USA. [Malluhi, Qutaibah Marwan] Qatar Univ, Doha, Qatar. [Tziritas, Nikos] Chinese Acad Sci, Beijing, Peoples R China. [Vishnu, Abhinav] Pacific NW Natl Lab, Richland, WA 99352 USA. [Zomaya, Albert] Univ Sydney, Sydney, NSW, Australia. RP Ranjan, R (reprint author), CSIRO, Canberra, ACT, Australia. EM rajiv.ranjan@csiro.au RI Ranjan, Rajiv/F-4700-2011; OI Kolodziej, Joanna/0000-0002-5181-8713 NR 76 TC 1 Z9 1 U1 6 U2 9 PU SPRINGER WIEN PI WIEN PA SACHSENPLATZ 4-6, PO BOX 89, A-1201 WIEN, AUSTRIA SN 0010-485X EI 1436-5057 J9 COMPUTING JI Computing PD JUL PY 2016 VL 98 IS 7 SI SI BP 751 EP 774 DI 10.1007/s00607-014-0407-8 PG 24 WC Computer Science, Theory & Methods SC Computer Science GA DR7ZL UT WOS:000380118100003 ER PT J AU Rathnayake, AS Feaster, KA White, J Barnes, CL Teat, SJ Atwood, JL AF Rathnayake, Asanka S. Feaster, Kyle A. White, Joshua Barnes, Charles L. Teat, Simon J. Atwood, Jerry L. TI Investigating Reaction Conditions To Control the Self-Assembly of Cobalt-Seamed Nanocapsules SO CRYSTAL GROWTH & DESIGN LA English DT Article ID COORDINATION; CAPSULES; COMPLEXES; CHEMISTRY AB The synthesis and X-ray crystallographic structure of the first cobalt-seamed hexameric nanocapsule, [Co-24(C-pentylpyrogallol[4]arene)(6)], is presented. The overall metalligand arrangement of this novel capsule is similar to that of previously reported copper- and nickel-seamed hexameric nanocapsules. However, the title nanocapsule encloses a larger void space than those found in previous hexameric nanocapsules C1 [Rathnayake, Asanka S.; Feaster, Kyle A.; White, Joshua; Barnes, Charles L.; Atwood, Jerry L.] Univ Missouri, Dept Chem, 601 South Coll Ave, Columbia, MO 65211 USA. [Teat, Simon J.] Lawrence Berkeley Natl Lab, Adv Light Source, 1 Cyclotron Rd,MS6R2100, Berkeley, CA 94720 USA. RP Atwood, JL (reprint author), Univ Missouri, Dept Chem, 601 South Coll Ave, Columbia, MO 65211 USA. EM atwoodj@missouri.edu NR 13 TC 1 Z9 1 U1 4 U2 4 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1528-7483 EI 1528-7505 J9 CRYST GROWTH DES JI Cryst. Growth Des. PD JUL PY 2016 VL 16 IS 7 BP 3562 EP 3564 DI 10.1021/acs.cgd.6b00306 PG 3 WC Chemistry, Multidisciplinary; Crystallography; Materials Science, Multidisciplinary SC Chemistry; Crystallography; Materials Science GA DQ8JJ UT WOS:000379456700002 ER PT J AU Slater, NH Buckley, BR Elsegood, MRJ Teat, SJ Kimber, MC AF Slater, Natasha H. Buckley, Benjamin R. Elsegood, Mark R. J. Teat, Simon J. Kimber, Marc C. TI Controlling the Assembly of C2-Symmetric Molecular Tectons Using a Thiocarbamate Appended Carbocyclic Cleft Molecule Analogous to Troger's Base SO CRYSTAL GROWTH & DESIGN LA English DT Article ID RAY CRYSTALLOGRAPHIC ANALYSIS; ENANTIOMER RECOGNITION; CHIRAL CENTER; CROWN-ETHERS; SUBUNIT; DERIVATIVES; NETWORKS; PATTERNS AB By way of appending the C-2-symmetric carbocyclic cleft diol with thiocarbamates with varying substituents, significant control of the hydrogen bonded network can be achieved. Smaller alkyl substituents lead to the formation of stacked columns of components with the apex of one molecule suitably aligned in the cleft of a second. Aryl substituents, however, lead to the formation of ribbons via an H-bonding network. Additionally, the packing of these ribbons into networks is considerably different between the enantiopure and racemic clefts, with the latter giving rise to channels within the crystal structure. C1 [Slater, Natasha H.; Buckley, Benjamin R.; Elsegood, Mark R. J.; Kimber, Marc C.] Univ Loughborough, Dept Chem, Loughborough LE11 3TU, Leics, England. [Teat, Simon J.] Berkeley Lab, ALS, 1 Cyclotron Rd,MS2-400, Berkeley, CA 94720 USA. RP Elsegood, MRJ; Kimber, MC (reprint author), Univ Loughborough, Dept Chem, Loughborough LE11 3TU, Leics, England. EM M.RJ.Elsegood@lboro.ac.uk; M.C.Kimber@lboro.ac.uk OI Kimber, Marc/0000-0003-2943-1974 FU Loughborough University; Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy [DE-AC02-05CH11231] FX We gratefully acknowledge financial support from Loughborough University (studentship for NHS). We also thank Dr. Mark Edgar (Loughborough) for assistance with NMR assignments. The Advanced Light Source is supported by the Director, Office of Science, Office of Basic Energy Sciences, of the U.S. Department of Energy under Contract No. DE-AC02-05CH11231. NR 32 TC 1 Z9 1 U1 3 U2 6 PU AMER CHEMICAL SOC PI WASHINGTON PA 1155 16TH ST, NW, WASHINGTON, DC 20036 USA SN 1528-7483 EI 1528-7505 J9 CRYST GROWTH DES JI Cryst. Growth Des. PD JUL PY 2016 VL 16 IS 7 BP 3846 EP 3852 DI 10.1021/acs.cgd.6b00388 PG 7 WC Chemistry, Multidisciplinary; Crystallography; Materials Science, Multidisciplinary SC Chemistry; Crystallography; Materials Science GA DQ8JJ UT WOS:000379456700036 ER PT J AU Ekdahl, C Coleman, JE McCuistian, BT AF Ekdahl, Carl Coleman, Joshua E. McCuistian, Brian Trent TI Beam Breakup in an Advanced Linear Induction Accelerator SO IEEE TRANSACTIONS ON PLASMA SCIENCE LA English DT Article DE Electron beam instabilities; linear induction accelerators (LIAs) ID RADIOGRAPHY AB Two linear induction accelerators (LIAs) have been in operation for a number of years at the Los Alamos Dual Axis Radiographic Hydrodynamic Test (DARHT) facility. A new multipulse LIA is being developed. We have computationally investigated the beam breakup (BBU) instability in this advanced LIA. In particular, we have explored the consequences of the choice of beam injector energy and the grouping of LIA cells. We find that within the limited range of options presently under consideration for the LIA architecture, there is little adverse effect on the BBU growth. The computational tool that we used for this investigation was the beam dynamics code linear accelerator model for DARHT (LAMDA). To confirm that LAMDA was appropriate for this task, we first validated it through comparisons with the experimental BBU data acquired on the DARHT accelerators. C1 [Ekdahl, Carl; Coleman, Joshua E.; McCuistian, Brian Trent] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. RP Ekdahl, C (reprint author), Los Alamos Natl Lab, Los Alamos, NM 87545 USA. EM cekdahl@lanl.gov; jecoleman@lanl.gov; trentmc@lanl.gov FU National Nuclear Security Administration within the U.S. Department of Energy [DE-AC52-06NA25396] FX This work was supported by the National Nuclear Security Administration within the U.S. Department of Energy under Contract DE-AC52-06NA25396. NR 34 TC 0 Z9 0 U1 0 U2 0 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0093-3813 EI 1939-9375 J9 IEEE T PLASMA SCI JI IEEE Trans. Plasma Sci. PD JUL PY 2016 VL 44 IS 7 BP 1094 EP 1102 DI 10.1109/TPS.2016.2571123 PG 9 WC Physics, Fluids & Plasmas SC Physics GA DR6TQ UT WOS:000380034600007 ER PT J AU Fan, Y Sun, B Agarwal, S Zhang, L AF Fan, Ying Sun, Bo Agarwal, Sheetal Zhang, Lei TI Review of Transporter-Related Postmarketing Requirement or Postmarketing Commitment Studies SO JOURNAL OF CLINICAL PHARMACOLOGY LA English DT Article DE transporters; new molecular entity (NME); postmarketing requirement (PMR); postmarketing commitment (PMC); drug-drug interaction (DDI); regulatory; labeling ID DRUG-INTERACTION; POLYMORPHISMS; CONSORTIUM AB The objectives of this report are to summarize the content and status of transporter-related postmarketing requirement (PMR)/postmarketing commitment (PMC) studies in new drug applications (NDAs) approved by the U.S. Food and Drug Administration (FDA) and to discuss the reasons for requesting such studies and the impact of PMR/PMC study results on labeling to guide the optimal use of the drugs. Multiple data sources were searched to collect information on transporter-related PMR/PMC studies between January 1999 and May 2015. A total of 40 transporter-related PMR/PMC study requests were issued for 35 NDAs. Among these PMR/PMC studies, 27 requested studies related to P-glycoprotein. As of May 31, 2015, 34 transporter-related PMR/PMC studies (85%) are considered "fulfilled" (per the FDA's PMR/PMC website), and 22 (65%) resulted in labeling updates. The majority of the PMR/PMC studies are for drugs in the therapeutic areas of anti-infectives, oncology, and neurology. The results from PMR/PMC studies are important for dosing optimization and are often included in the updated labeling. Because a significant lag time is anticipated between drug approval and PMR/PMC fulfillment, NDA applicants are encouraged to include transporter-related assessments in clinical drug development programs for drug products. C1 [Fan, Ying; Sun, Bo; Agarwal, Sheetal; Zhang, Lei] US FDA, Off Clin Pharmacol, Off Translat Sci, Ctr Drug Evaluat & Res, 10903 New Hampshire Ave, Silver Spring, MD 20993 USA. [Fan, Ying] US FDA, Off Bioequivalence, Off Gener Drugs, Ctr Drug Evaluat & Res, Silver Spring, MD USA. [Sun, Bo] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. [Sun, Bo] Shanghai Jiao Tong Univ, Sch Med, Shanghai Gen Hosp, Dept Pharm, Shanghai, Peoples R China. RP Zhang, L (reprint author), US FDA, Off Clin Pharmacol, Off Translat Sci, Ctr Drug Evaluat & Res, 10903 New Hampshire Ave, Silver Spring, MD 20993 USA. EM leik.zhang@fda.hhs.gov FU National Key Clinical Specialty Construction Project of China FX Dr. Bo Sun was supported in part by an appointment to the research participation program at the CDER administered by the Oak Ridge Institute for Science and Education (ORISE) through an interagency agreement between the U.S. Dept. of Energy and the U.S. FDA. She was also supported by the National Key Clinical Specialty Construction Project of China. NR 30 TC 1 Z9 1 U1 1 U2 1 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0091-2700 EI 1552-4604 J9 J CLIN PHARMACOL JI J. Clin. Pharmacol. PD JUL PY 2016 VL 56 SU 7 SI SI BP S193 EP S204 DI 10.1002/jcph.770 PG 12 WC Pharmacology & Pharmacy SC Pharmacology & Pharmacy GA DR6ZW UT WOS:000380050800015 PM 27385175 ER PT J AU Vaidyanathan, J Yoshida, K Arya, V Zhang, L AF Vaidyanathan, Jayabharathi Yoshida, Kenta Arya, Vikram Zhang, Lei TI Comparing Various In Vitro Prediction Criteria to Assess the Potential of a New Molecular Entity to Inhibit Organic Anion Transporting Polypeptide 1B1 SO JOURNAL OF CLINICAL PHARMACOLOGY LA English DT Article DE Transporters; Drug-Drug Interactions; Pharmacokinetics and drug metabolism; Clinical Pharmacology (CPH); Organic Anion Transporting Polypeptide (OATP); Inhibition ID DRUG-DRUG INTERACTIONS; HEPATIC-UPTAKE; CYCLOSPORINE-A; PHARMACOKINETICS; ATORVASTATIN; METABOLISM; HUMANS; CERIVASTATIN; ROSUVASTATIN; ITRACONAZOLE AB Evaluation of organic anion transporting polypeptide (OATP) 1B1-mediated drug-drug interactions (DDIs) is an integral part of drug development and is recommended by regulatory agencies. In this study we compared various prediction methods and cutoff criteria based on in vitro inhibition data to assess the potential of a new molecular entity to inhibit OATP1B1 in vivo. In vitro (eg, IC50, f(u,p)) and in vivo (eg, dose, C-max, change in area under the curve [AUC]) data for 11 substrates and 61 inhibitors for OATP1B1 were obtained from literature and Drugs@FDA, which include 107 clinical (in vivo) DDI studies. Substrate dependency and variability of IC50 values were noted. In addition to the ratio of unbound or total systemic concentration (I-max,I-u and I-max) to IC50, maximum unbound inhibitor concentration at the inlet to the liver (I-u,I-in,I-max) was used for the estimation of "R value" where R = 1 + I-u,I-in,I-max/IC50. Based on our analyses, I-max/K-i >= 0.1, R >= 1.04, or R >= 1.1 seem to be appropriate for reducing the false-negative (FN) predictions. However, as compared with R >= 1.1, I-max/K-i >= 0.1 and R >= 1.04 resulted in higher false positives (FPs) and lower true negatives (TNs). R >= 1.1,I-max,I-u/K-i >= 0.02, and R >= 1.25 alone, or combined criterion of I-max/K-i >= 0.1 and R >= 1.25, were reasonable to determine the need to perform clinical DDI studies with OATP1B1 substrates with similar positive and negative predictive values. Possible reasons of FP or FN from different decision criteria should be considered when interpreting prediction results, and the variability in IC50 determination needs to be understood and minimized. C1 [Vaidyanathan, Jayabharathi; Yoshida, Kenta; Arya, Vikram; Zhang, Lei] US FDA, Off Clin Pharmacol, Off Translat Sci, Ctr Drug Evaluat & Res, Silver Spring, MD 20993 USA. [Yoshida, Kenta] Oak Ridge Inst Sci & Educ, Oak Ridge, TN USA. RP Zhang, L (reprint author), US FDA, Off Clin Pharmacol, Off Translat Sci, Ctr Drug Evaluat & Res, Silver Spring, MD 20993 USA. EM leik.zhang@fda.hhs.gov NR 46 TC 2 Z9 2 U1 4 U2 4 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0091-2700 EI 1552-4604 J9 J CLIN PHARMACOL JI J. Clin. Pharmacol. PD JUL PY 2016 VL 56 SU 7 SI SI BP S59 EP S72 DI 10.1002/jcph.723 PG 14 WC Pharmacology & Pharmacy SC Pharmacology & Pharmacy GA DR6ZW UT WOS:000380050800005 PM 27385179 ER PT J AU Wierer, JJ Tansu, N Fischer, AJ Tsao, JY AF Wierer, Jonathan J., Jr. Tansu, Nelson Fischer, Arthur J. Tsao, Jeffrey Y. TI III-nitride quantum dots for ultra-efficient solid-state lighting SO LASER & PHOTONICS REVIEWS LA English DT Article DE Quantum Dots; Solid-state lighting; light-emitting diodes; LEDs; laser diodes; LDs; efficiency droop; III-nitride; InGaN; GaN; phosphor-converted; PC-LEDs; Auger recombination ID CURRENT INJECTION EFFICIENCY; EMITTING-DIODES; TEMPERATURE-DEPENDENCE; LASER; WELL; THRESHOLD; GROWTH; GAIN; BLUE AB III-nitride light-emitting diodes (LEDs) and laser diodes (LDs) are ultimately limited in performance due to parasitic Auger recombination. For LEDs, the consequences are poor efficiencies at high current densities; for LDs, the consequences are high thresholds and limited efficiencies. Here, we present arguments for III-nitride quantum dots (QDs) as active regions for both LEDs and LDs, to circumvent Auger recombination and achieve efficiencies at higher current densities that are not possible with quantum wells. QD-based LDs achieve gain and thresholds at lower carrier densities before Auger recombination becomes appreciable. QD-based LEDs achieve higher efficiencies at higher currents because of higher spontaneous emission rates and reduced Auger recombination. The technical challenge is to control the size distribution and volume of the QDs to realize these benefits. If constructed properly, III-nitride light-emitting devices with QD active regions have the potential to outperform quantum well light-emitting devices, and enable an era of ultra-efficient solid-state lighting. C1 [Wierer, Jonathan J., Jr.; Tansu, Nelson] Lehigh Univ, Ctr Photon & Nanoelect, Dept Elect & Comp Engn, Bethlehem, PA 18015 USA. [Fischer, Arthur J.; Tsao, Jeffrey Y.] Sandia Natl Labs, POB 5800, Albuquerque, NM 87185 USA. RP Wierer, JJ (reprint author), Lehigh Univ, Ctr Photon & Nanoelect, Dept Elect & Comp Engn, Bethlehem, PA 18015 USA. EM jwierer@lehigh.edu RI Wierer, Jonathan/G-1594-2013 OI Wierer, Jonathan/0000-0001-6971-4835 FU Sandia's Laboratory Directed Research and Development program; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX The authors would like to thank Ben Leung for his useful suggestions on the manuscript. Work at Sandia National Laboratories was supported by Sandia's Laboratory Directed Research and Development program. Sandia National Laboratories is a multiprogram laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 58 TC 0 Z9 0 U1 16 U2 24 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1863-8880 EI 1863-8899 J9 LASER PHOTONICS REV JI Laser Photon. Rev. PD JUL PY 2016 VL 10 IS 4 BP 612 EP 622 DI 10.1002/lpor.201500332 PG 11 WC Optics; Physics, Applied; Physics, Condensed Matter SC Optics; Physics GA DR5QZ UT WOS:000379958800006 ER PT J AU Khromova, I Kuzel, P Brener, I Reno, JL Seu, UCC Elissalde, C Maglione, M Mounaix, P Mitrofanov, O AF Khromova, Irina Kuzel, Petr Brener, Igal Reno, John L. Seu, U-Chan Chung Elissalde, Catherine Maglione, Mario Mounaix, Patrick Mitrofanov, Oleg TI Splitting of magnetic dipole modes in anisotropic TiO2 micro-spheres SO LASER & PHOTONICS REVIEWS LA English DT Article DE Terahertz spectroscopy; Mie scattering; dielectric metamaterials; magnetic dipole ID DIELECTRIC METAMATERIALS; FANO RESONANCES; MIE RESONATORS; METASURFACES; WAVES; PHASE AB Monocrystalline titanium dioxide (TiO2) micro-spheres support two orthogonal magnetic dipole modes at terahertz (THz) frequencies due to strong dielectric anisotropy. For the first time, we experimentally detected the splitting of the first Mie mode in spheres of radii 10-20m through near-field time-domain THz spectroscopy. By fitting the Fano lineshape model to the experimentally obtained spectra of the electric field detected by the sub-wavelength aperture probe, we found that the magnetic dipole resonances in TiO2 spheres have narrow linewidths of only tens of gigahertz. Anisotropic TiO2 micro-resonators can be used to enhance the interplay of magnetic and electric dipole resonances in the emerging THz all-dielectric metamaterial technology. C1 [Khromova, Irina] Kings Coll London, Dept Phys, London WC2R 2LS, England. [Khromova, Irina; Mitrofanov, Oleg] UCL, Dept Elect & Elect Engn, London WC1E 7JE, England. [Khromova, Irina] ITMO Univ, St Petersburg 199034, Russia. [Kuzel, Petr] Acad Sci Czech Republic, Inst Phys, Prague 18221 8, Czech Republic. [Brener, Igal; Reno, John L.; Mitrofanov, Oleg] Sandia Natl Labs, Ctr Integrated Nanotechnol, POB 5800, Albuquerque, NM 87185 USA. [Brener, Igal; Reno, John L.] Sandia Natl Labs, Albuquerque, NM 87185 USA. [Seu, U-Chan Chung; Elissalde, Catherine; Maglione, Mario] Univ Bordeaux, ICMCB, CRNS, UPR 9048, 87 Ave Docteur Schweitzer, F-33608 Pessac, France. [Mounaix, Patrick] Univ Bordeaux, CNRS, IMS, UMR 5218, 351 Cours Liberat, F-33405 Talence, France. RP Khromova, I (reprint author), Kings Coll London, Dept Phys, London WC2R 2LS, England.; Khromova, I (reprint author), UCL, Dept Elect & Elect Engn, London WC1E 7JE, England.; Khromova, I (reprint author), ITMO Univ, St Petersburg 199034, Russia. EM irina.khromova@kcl.ac.uk RI Kuzel, Petr/G-6006-2014; Mitrofanov, Oleg/C-1938-2008 OI Mitrofanov, Oleg/0000-0003-3510-2675 FU Royal Society [UF130493]; RFBR [16-07-01166, 14-22-02064-ofi-m]; Czech Science Foundation [14-25639S]; LabEx AMADEus in the framework of IdEx Bordeaux [ANR-10-LABX-42, ANR-10-IDEX-03-02]; Investissements d Avenir programme of the French government; Government of the Russian Federation [074-U01, GZ 3.561.2014/K]; U.S. Department of Energy's National Nuclear Security Administration [DE-AC04-94AL85000] FX This work is supported by the Royal Society [Grant No. UF130493], RFBR [16-07-01166 and 14-22-02064-ofi-m], the Czech Science Foundation (project 14-25639S), LabEx AMADEus (ANR-10-LABX-42) in the framework of IdEx Bordeaux (ANR-10-IDEX-03-02)/i.e./ the Investissements d Avenir programme of the French government managed by the Agence Nationale de la Recherche, and partially supported by the Government of the Russian Federation [Grant No. 074-U01 and GZ 3.561.2014/K]. This work was performed at UCL and, in part, at the Center for Integrated Nanotechnologies, a U.S. Department of Energy, Office of Basic Energy Sciences user facility. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000. NR 29 TC 1 Z9 1 U1 12 U2 29 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1863-8880 EI 1863-8899 J9 LASER PHOTONICS REV JI Laser Photon. Rev. PD JUL PY 2016 VL 10 IS 4 BP 681 EP 687 DI 10.1002/lpor.201600084 PG 7 WC Optics; Physics, Applied; Physics, Condensed Matter SC Optics; Physics GA DR5QZ UT WOS:000379958800014 ER PT J AU Rautengarten, C Ebert, B Liu, LF Stonebloom, S Smith-Moritz, AM Pauly, M Orellana, A Scheller, HV Heazlewood, JL AF Rautengarten, Carsten Ebert, Berit Liu, Lifeng Stonebloom, Solomon Smith-Moritz, Andreia M. Pauly, Markus Orellana, Ariel Scheller, Henrik Vibe Heazlewood, Joshua L. TI The Arabidopsis Golgi-localized GDP-L-fucose transporter is required for plant development SO NATURE COMMUNICATIONS LA English DT Article ID DE-NOVO SYNTHESIS; GALACTOSE TRANSPORTER; RHAMNOGALACTURONAN-II; SUGAR TRANSPORTERS; N-GLYCANS; UDP-GALACTOSE; MUR1 GENE; THALIANA; XYLOGLUCAN; EXPRESSION AB Nucleotide sugar transport across Golgi membranes is essential for the luminal biosynthesis of glycan structures. Here we identify GDP-fucose transporter 1 (GFT1), an Arabidopsis nucleotide sugar transporter that translocates GDP-L-fucose into the Golgi lumen. Using proteo-liposome-based transport assays, we show that GFT preferentially transports GDP-L-fucose over other nucleotide sugars in vitro, while GFT1-silenced plants are almost devoid of L-fucose in cell wall-derived xyloglucan and rhamnogalacturonan II. Furthermore, these lines display reduced L-fucose content in N-glycan structures accompanied by severe developmental growth defects. We conclude that GFT1 is the major nucleotide sugar transporter for import of GDP-L-fucose into the Golgi and is required for proper plant growth and development. C1 [Rautengarten, Carsten; Ebert, Berit; Stonebloom, Solomon; Smith-Moritz, Andreia M.; Scheller, Henrik Vibe; Heazlewood, Joshua L.] Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Phys Biosci Div, Berkeley, CA 94702 USA. [Rautengarten, Carsten; Ebert, Berit; Heazlewood, Joshua L.] Univ Melbourne, Sch BioSci, ARC Ctr Excellence Plant Cell Walls, Melbourne, Vic 3010, Australia. [Ebert, Berit] Univ Copenhagen, Dept Plant & Environm Sci, Fac Sci, DK-1871 Copenhagen, Denmark. [Liu, Lifeng; Pauly, Markus; Scheller, Henrik Vibe] Univ Calif Berkeley, Dept Plant & Microbial Biol, Berkeley, CA 94720 USA. [Orellana, Ariel] Univ Andres Bello, Fac Ciencias Biol, Ctr Biotecnol Vegetal, Santiago 8370146, RM, Chile. [Orellana, Ariel] Fondo Areas Prioritarias Ctr Genome Regulat, Santiago 8370146, RM, Chile. RP Heazlewood, JL (reprint author), Lawrence Berkeley Natl Lab, Joint BioEnergy Inst, Phys Biosci Div, Berkeley, CA 94702 USA.; Heazlewood, JL (reprint author), Univ Melbourne, Sch BioSci, ARC Ctr Excellence Plant Cell Walls, Melbourne, Vic 3010, Australia. EM jheazlewood@unimelb.edu.au RI Heazlewood, Joshua/A-2554-2008; Orellana, Ariel/E-2166-2014; Pauly, Markus/B-5895-2008; Scheller, Henrik/A-8106-2008 OI Heazlewood, Joshua/0000-0002-2080-3826; Orellana, Ariel/0000-0002-9243-808X; Pauly, Markus/0000-0002-3116-2198; Scheller, Henrik/0000-0002-6702-3560 FU US Department of Energy, Office of Science, Office of Biological and Environmental Research [DE-AC02-05CH11231]; Australian Research Council Future Fellowship [FT130101165]; Danish Strategic Research Council (Set4Future) [11-116795]; Fondecyt [1151335]; FONDAP-CRG [15090007]; Basal Program [PB-16]; NSF-RCN grant [0090281]; Lawrence Berkeley National Laboratory; US Department of Energy FX This work was supported by the US Department of Energy, Office of Science, Office of Biological and Environmental Research, through contract DE-AC02-05CH11231 between Lawrence Berkeley National Laboratory and the US Department of Energy. J.L.H. is supported by an Australian Research Council Future Fellowship (FT130101165). Part of the work was supported by the Danish Strategic Research Council (Set4Future 11-116795). A.O. is supported by Fondecyt 1151335, FONDAP-CRG 15090007 and Basal Program PB-16. The substrates obtained from Carbosource Services (Athens, GA) were supported in part by NSF-RCN grant #0090281. We also thank the Biological Optical Microscopy Platform (BOMP) at the University of Melbourne for technical support. NR 53 TC 2 Z9 2 U1 13 U2 20 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2016 VL 7 AR 12119 DI 10.1038/ncomms12119 PG 10 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DS0MW UT WOS:000380292100001 PM 27381418 ER PT J AU Struzhkin, VV Kim, DY Stavrou, E Muramatsu, T Mao, HK Pickard, CJ Needs, RJ Prakapenka, VB Goncharov, AF AF Struzhkin, Viktor V. Kim, Duck Young Stavrou, Elissaios Muramatsu, Takaki Mao, Ho-kwang Pickard, Chris J. Needs, Richard J. Prakapenka, Vitali B. Goncharov, Alexander F. TI Synthesis of sodium polyhydrides at high pressures SO NATURE COMMUNICATIONS LA English DT Article ID GENERALIZED GRADIENT APPROXIMATION; METALLIC HYDROGEN; LITHIUM; H-3(-); SUPERCONDUCTIVITY; TRANSITION; COMPLEXES; MOLECULES; HYDRIDE; SYSTEM AB The only known compound of sodium and hydrogen is archetypal ionic NaH. Application of high pressure is known to promote states with higher atomic coordination, but extensive searches for polyhydrides with unusual stoichiometry have had only limited success in spite of several theoretical predictions. Here we report the first observation of the formation of polyhydrides of Na (NaH3 and NaH7) above 40GPa and 2,000 K. We combine synchrotron X-ray diffraction and Raman spectroscopy in a laser-heated diamond anvil cell and theoretical random structure searching, which both agree on the stable structures and compositions. Our results support the formation of multicenter bonding in a material with unusual stoichiometry. These results are applicable to the design of new energetic solids and high-temperature superconductors based on hydrogen-rich materials. C1 [Struzhkin, Viktor V.; Kim, Duck Young; Stavrou, Elissaios; Muramatsu, Takaki; Mao, Ho-kwang; Goncharov, Alexander F.] Carnegie Inst Sci, Geophys Lab, 5251 Broad Branch Rd NW, Washington, DC 20015 USA. [Kim, Duck Young; Mao, Ho-kwang] Ctr High Pressure Sci & Technol Adv Res, Shanghai 201203, Peoples R China. [Stavrou, Elissaios] Lawrence Livermore Natl Lab, Div Mat Sci, 7000 East Ave,L-350, Livermore, CA 94550 USA. [Pickard, Chris J.] UCL, Dept Phys & Astron, Gower St, London WC1E 6BT, England. [Pickard, Chris J.] Univ Cambridge, Dept Mat Sci & Met, 27 Charles Babbage Rd, Cambridge CB3 0FS, England. [Needs, Richard J.] Cavendish Lab, Condensed Matter Theory Grp, JJ Thomson Ave, Cambridge CB3 0HE, England. [Prakapenka, Vitali B.] Univ Chicago, Ctr Adv Radiat Sources, Chicago, IL 60637 USA. [Goncharov, Alexander F.] Chinese Acad Sci, Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Anhui, Peoples R China. RP Struzhkin, VV (reprint author), Carnegie Inst Sci, Geophys Lab, 5251 Broad Branch Rd NW, Washington, DC 20015 USA. EM vstruzhkin@carnegiescience.edu FU DOE/BES [DE-FG02-02ER45955, DE-FG02-99ER45775]; Energy Frontier Research in Extreme Environments Center (EFree), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science [DE-SC0001057]; Engineering and Physical Sciences Research Council (EPSRC) of the UK; DARPA [W31P4Q1310005, W31P4Q1210008]; Engineering and Physical Sciences Research Council (EPSRC) of the U.K. [EP/J017639/1]; EPSRC [EP/G007489/2]; U.S. Department of Energy by Lawrence Livermore National Security, LLC [DE- AC52-07NA27344]; NSFC [21473211]; National Science Foundation-Earth Sciences [EAR-1128799]; Department of Energy-Geosciences [DE-FG02-94ER14466]; U.S. Department of Energy, Office of Basic Energy Sciences [DE-AC02-06CH11357]; U.S. Department of Energy, Office of Science [DE-AC02-06CH11357] FX High-pressure experiments were supported by DOE/BES under contract no. DE-FG02-02ER45955 and DE-FG02-99ER45775. D.Y.K. and T.M. acknowledge salary support by Energy Frontier Research in Extreme Environments Center (EFree), an Energy Frontier Research Center funded by the U.S. Department of Energy, Office of Science under Award Number DE-SC0001057. C.J.P. and R.J.N. were supported by the Engineering and Physical Sciences Research Council (EPSRC) of the UK. E.S. and A.F.G. acknowledge support of DARPA under contracts nos'. W31P4Q1310005 and W31P4Q1210008. R.J.N. acknowledges financial support from the Engineering and Physical Sciences Research Council (EPSRC) of the U.K. [EP/J017639/1]. C.J.P. acknowledges financial support from EPSRC [EP/G007489/2]. E.S. has performed parts of the work under the auspices of the U.S. Department of Energy by Lawrence Livermore National Security, LLC under Contract DE- AC52-07NA27344. A.F.G. acknowledges support of NSFC (no. 21473211). Portions of this work were performed at GeoSoilEnviroCARS (Sector 13), Advanced Photon Source (APS) and Argonne National Laboratory. GeoSoilEnviroCARS is supported by the National Science Foundation-Earth Sciences (EAR-1128799) and Department of Energy-Geosciences (DE-FG02-94ER14466). Use of the Advanced Photon Source was supported by the U.S. Department of Energy, Office of Science and Office of Basic Energy Sciences under contract no. DE-AC02-06CH11357. We thank K. Zhuravlev and S. Tkachev for help with XRD and Raman measurements at GSECARS. NR 48 TC 2 Z9 2 U1 23 U2 41 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2016 VL 7 AR 12267 DI 10.1038/ncomms12267 PG 8 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DS2DA UT WOS:000380536000001 PM 27464650 ER PT J AU Tan, GJ Shi, FY Hao, SQ Zhao, LD Chi, H Zhang, XM Uher, C Wolverton, C Dravid, VP Kanatzidis, MG AF Tan, Gangjian Shi, Fengyuan Hao, Shiqiang Zhao, Li-Dong Chi, Hang Zhang, Xiaomi Uher, Ctirad Wolverton, Chris Dravid, Vinayak P. Kanatzidis, Mercouri G. TI Non-equilibrium processing leads to record high thermoelectric figure of merit in PbTe-SrTe SO NATURE COMMUNICATIONS LA English DT Article ID PERFORMANCE BULK THERMOELECTRICS; LATTICE THERMAL-CONDUCTIVITY; 2ND VALENCE-BAND; EFFICIENCY; TELLURIDE; NANOSTRUCTURES; SEMICONDUCTORS; TEMPERATURES; CONVERGENCE; ENHANCEMENT AB The broad-based implementation of thermoelectric materials in converting heat to electricity hinges on the achievement of high conversion efficiency. Here we demonstrate a thermoelectric figure of merit ZT of 2.5 at 923 K by the cumulative integration of several performance-enhancing concepts in a single material system. Using non-equilibrium processing we show that hole-doped samples of PbTe can be heavily alloyed with SrTe well beyond its thermodynamic solubility limit of <1 mol%. The much higher levels of Sr alloyed into the PbTe matrix widen the bandgap and create convergence of the two valence bands of PbTe, greatly boosting the power factors with maximal values over 30 mu Wcm (-1) K (-2). Exceeding the 5 mol% solubility limit leads to endotaxial SrTe nanostructures which produce extremely low lattice thermal conductivity of 0.5 Wm (-1) K (-1) but preserve high hole mobilities because of the matrix/precipitate valence band alignment. The best composition is hole-doped PbTe-8% SrTe. C1 [Tan, Gangjian; Zhao, Li-Dong; Kanatzidis, Mercouri G.] Northwestern Univ, Dept Chem, Evanston, IL 60208 USA. [Shi, Fengyuan; Hao, Shiqiang; Zhang, Xiaomi; Wolverton, Chris; Dravid, Vinayak P.] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA. [Zhao, Li-Dong] Beihang Univ, Sch Mat Sci & Engn, Beijing 100191, Peoples R China. [Chi, Hang; Uher, Ctirad] Univ Michigan, Dept Phys, Ann Arbor, MI 48109 USA. [Kanatzidis, Mercouri G.] Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. RP Kanatzidis, MG (reprint author), Northwestern Univ, Dept Chem, Evanston, IL 60208 USA.; Kanatzidis, MG (reprint author), Argonne Natl Lab, Div Mat Sci, Argonne, IL 60439 USA. EM m-kanatzidis@northwestern.edu RI Wolverton, Christopher/B-7542-2009; Dravid, Vinayak/B-6688-2009; Chi, Hang/F-1537-2011; OI Chi, Hang/0000-0002-1299-1150; Tan, Gangjian/0000-0002-9087-4048 FU Department of Energy, Office of Science Basic Energy Sciences [DE-SC0014520] FX This work was supported by the Department of Energy, Office of Science Basic Energy Sciences under grant DE-SC0014520. Transmission electron microscopy work was partially performed in the EPIC facility of the NUANCE Center at Northwestern University. Access to facilities of high performance computational resources at the Northwestern University is acknowledged. NR 58 TC 14 Z9 14 U1 42 U2 72 PU NATURE PUBLISHING GROUP PI LONDON PA MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1 9XW, ENGLAND SN 2041-1723 J9 NAT COMMUN JI Nat. Commun. PD JUL PY 2016 VL 7 AR 12167 DI 10.1038/ncomms12167 PG 9 WC Multidisciplinary Sciences SC Science & Technology - Other Topics GA DR9DA UT WOS:000380196100001 PM 27456303 ER PT J AU Erdemir, A AF Erdemir, Ali TI From Curiosity to Presidency SO TRIBOLOGY & LUBRICATION TECHNOLOGY LA English DT Editorial Material C1 [Erdemir, Ali] Argonne Natl Lab, Lemont, IL 60439 USA. RP Erdemir, A (reprint author), Argonne Natl Lab, Lemont, IL 60439 USA. EM erdemir@anl.gov NR 0 TC 0 Z9 0 U1 0 U2 0 PU SOC TRIBOLOGISTS & LUBRICATION ENGINEERS PI PARK RIDGE PA 840 BUSSE HIGHWAY, PARK RIDGE, IL 60068 USA SN 1545-858X J9 TRIBOL LUBR TECHNOL JI Tribol. Lubr. Technol. PD JUL PY 2016 VL 72 IS 7 BP 4 EP 4 PG 1 WC Engineering, Mechanical SC Engineering GA DP4DI UT WOS:000378445200001 ER PT J AU Blanco-Gomez, A Castillo-Lluva, S Saez-Freire, MD Hontecillas-Prieto, L Mao, JH Castellanos-Martin, A Perez-Losada, J AF Blanco-Gomez, Adrian Castillo-Lluva, Sonia del Mar Saez-Freire, Maria Hontecillas-Prieto, Lourdes Mao, Jian Hua Castellanos-Martin, Andres Perez-Losada, Jesus TI Missing heritability of complex diseases: Enlightenment by genetic variants from intermediate phenotypes SO BIOESSAYS LA English DT Review DE complex diseases; heritability; intermediate phenotype or endophenotype; missing heritability ID GENOME-WIDE ASSOCIATION; SYSTEMIC-LUPUS-ERYTHEMATOSUS; INFLAMMATORY-BOWEL-DISEASE; LONG-QT SYNDROME; RARE VARIANTS; MENDELIAN RANDOMIZATION; PSYCHIATRIC GENETICS; COMMON VARIANTS; BREAST-CANCER; LOCI AB Diseases of complex origin have a component of quantitative genetics that contributes to their susceptibility and phenotypic variability. However, after several studies, a major part of the genetic component of complex phenotypes has still not been found, a situation known as "missing heritability.'' Although there have been many hypotheses put forward to explain the reasons for the missing heritability, its definitive causes remain unknown. Complex diseases are caused by multiple intermediate phenotypes involved in their pathogenesis and, very often, each one of these intermediate phenotypes also has a component of quantitative inheritance. Here we propose that at least part of the missing heritability can be explained by the genetic component of intermediate phenotypes that is not detectable at the level of the main complex trait. At the same time, the identification of the genetic component of intermediate phenotypes provides an opportunity to identify part of the missing heritability of complex diseases. C1 [Blanco-Gomez, Adrian; Castillo-Lluva, Sonia; del Mar Saez-Freire, Maria; Hontecillas-Prieto, Lourdes; Castellanos-Martin, Andres; Perez-Losada, Jesus] Univ Salamanca, CSIC, Inst Biol Mol & Celular Canc CIC IBMC, Salamanca, Spain. [Blanco-Gomez, Adrian; Castillo-Lluva, Sonia; del Mar Saez-Freire, Maria; Hontecillas-Prieto, Lourdes; Castellanos-Martin, Andres; Perez-Losada, Jesus] Inst Invest Biomed Salamanca IBSAL, Salamanca, Spain. [Mao, Jian Hua] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Div Life Sci, Berkeley, CA 94720 USA. [Castillo-Lluva, Sonia] Univ Complutense Madrid, Dept Bioquim & Biol Mol 1, Fac Biol, Madrid, Spain. [Hontecillas-Prieto, Lourdes] Inst Biomed Sevilla IBiS, Dept Patol Mol, Seville, Spain. [Castellanos-Martin, Andres] IRB, Barcelona, Spain. RP Castellanos-Martin, A; Perez-Losada, J (reprint author), Univ Salamanca, CSIC, Inst Biol Mol & Celular Canc CIC IBMC, Salamanca, Spain.; Castellanos-Martin, A; Perez-Losada, J (reprint author), Inst Invest Biomed Salamanca IBSAL, Salamanca, Spain. EM jperezlosada@usal.es OI Castillo-LLuva, Sonia/0000-0001-5357-7178 FU FEDER; MICINN [PLE2009-119, SAF2014-56989-R]; Instituto de Salud Carlos III [PI07/0057, PI10/00328, PIE14/00066]; Junta de Castilla y Leon [CSI034U13, BIO/SA31/15]; Proyectos integrados IBSAL [IBY15/00003]; Eugenio Rodriguez Pascual; "Fundacion Inbiomed" (Instituto Oncologico Obra Social de la Caja Guipozcoa-San Sebastian, Kutxa); Fundacion Sandra Ibarra de Solidaridad frente al Cancer; Fundacion Eugenio Rodriguez Pascual; FIS [PI07/0057]; JAEdoc Fellowship (CSIC)/FSE; National Institutes of Health; National Cancer Institute [R01 CA116481]; Low-Dose Scientific Focus Area; Office of Biological & Environmental Research; US Department of Energy [DE-AC02-05CH11231]; [Q3718001E (2009-2010) y GRS 612/A/11 (2011-2012)] FX JPL was partially supported by FEDER and MICINN (PLE2009-119, SAF2014-56989-R), Instituto de Salud Carlos III (PI07/0057, PI10/00328, PIE14/00066), Junta de Castilla y Leon (CSI034U13, BIO/SA31/15), "Proyectos integrados IBSAL 2015" (IBY15/00003), the "Eugenio Rodriguez Pascual", the "Fundacion Inbiomed" (Instituto Oncologico Obra Social de la Caja Guipozcoa-San Sebastian, Kutxa), and the "Fundacion Sandra Ibarra de Solidaridad frente al Cancer". CR-C is funded by Q3718001E (2009-2010) y GRS 612/A/11 (2011-2012) and "the Fundacion Eugenio Rodriguez Pascual". AC was supported by FIS (PI07/0057) and MICINN (PLE2009-119). SCLL was funded by a JAEdoc Fellowship (CSIC)/FSE. JHM was supported by the National Institutes of Health, a National Cancer Institute grant (R01 CA116481), and the Low-Dose Scientific Focus Area, Office of Biological & Environmental Research, US Department of Energy (DE-AC02-05CH11231). We thank Dr. Elena de la Casa Esperon for their useful comments on the manuscript, Emma Keck from the University of Salamanca for her help in English editing and Rocio Puras Pardo for figure construction. We apologize to the many colleagues whose work could not be cited due to space restrictions. NR 78 TC 1 Z9 1 U1 6 U2 8 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 0265-9247 EI 1521-1878 J9 BIOESSAYS JI Bioessays PD JUL PY 2016 VL 38 IS 7 BP 664 EP 673 DI 10.1002/bies.201600084 PG 10 WC Biochemistry & Molecular Biology; Biology SC Biochemistry & Molecular Biology; Life Sciences & Biomedicine - Other Topics GA DR6YZ UT WOS:000380048500010 PM 27241833 ER PT J AU Lei, DS Rames, M Zhang, X Zhang, L Zhang, SL Ren, G AF Lei, Dongsheng Rames, Matthew Zhang, Xing Zhang, Lei Zhang, Shengli Ren, Gang TI Insights into the Tunnel Mechanism of Cholesteryl Ester Transfer Protein through All-atom Molecular Dynamics Simulations SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE cholesterol; cholesterol metabolism; cholesterol regulation; cholesterol-binding protein; lipid metabolism; lipid transport; lipid-protein interaction; lipoprotein metabolism; molecular dynamics ID HIGH-DENSITY-LIPOPROTEINS; LIPID-TRANSFER; HEART-DISEASE; ELECTRON-MICROSCOPY; SURFACE-LIPIDS; CETP; PARTICLES; BINDING; IMPLICIT; MODEL AB Cholesteryl ester transfer protein (CETP) mediates cholesteryl ester (CE) transfer from the atheroprotective high density lipoprotein (HDL) cholesterol to the atherogenic low density lipoprotein cholesterol. In the past decade, this property has driven the development of CETP inhibitors, which have been evaluated in large scale clinical trials for treating cardiovascular diseases. Despite the pharmacological interest, little is known about the fundamental mechanism of CETP in CE transfer. Recent electron microscopy (EM) experiments have suggested a tunnel mechanism, and molecular dynamics simulations have shown that the flexible N-terminal distal end of CETP penetrates into the HDL surface and takes up a CE molecule through an open pore. However, it is not known whether a CE molecule can completely transfer through an entire CETP molecule. Here, we used all-atom molecular dynamics simulations to evaluate this possibility. The results showed that a hydrophobic tunnel inside CETP is sufficient to allow a CE molecule to completely transfer through the entire CETP within a predicted transfer time and at a rate comparable with those obtained through physiological measurements. Analyses of the detailed interactions revealed several residues that might be critical for CETP function, which may provide important clues for the effective development of CETP inhibitors and treatment of cardiovascular diseases. C1 [Lei, Dongsheng; Rames, Matthew; Zhang, Xing; Ren, Gang] Lawrence Berkeley Natl Lab, Mol Foundry, Lawrence, CA 94720 USA. [Lei, Dongsheng; Zhang, Xing; Zhang, Lei; Zhang, Shengli] Xi An Jiao Tong Univ, Dept Appl Phys, Xian 710049, Shaanxi, Peoples R China. RP Ren, G (reprint author), Lawrence Berkeley Natl Lab, Mol Foundry, Lawrence, CA 94720 USA.; Zhang, SL (reprint author), Xi An Jiao Tong Univ, Dept Appl Phys, Xian 710049, Shaanxi, Peoples R China. EM zhangsl@xjtu.edu.cn; gren@lbl.gov RI Zhang, Lei/G-6427-2012 OI Zhang, Lei/0000-0002-4880-824X FU National Institutes of Health from the NHLBI [1R01HL115153]; National Natural Science Foundation of China [11074196, 11374237]; Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy [DE-AC02-05CH11231] FX This work was supported by National Institutes of Health Grant 1R01HL115153 from the NHLBI (to G. R.) and National Natural Science Foundation of China Grants 11074196 and 11374237 (to S. Z.). The work performed at the Molecular Foundry was supported by the Office of Science, Office of Basic Energy Sciences, of the United States Department of Energy under Contract DE-AC02-05CH11231. The authors declare that they have no conflicts of interest with the contents of this article. The content is solely the responsibility of the authors and does not necessarily represent the official views of the National Institutes of Health. NR 51 TC 1 Z9 1 U1 4 U2 5 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD JUL 1 PY 2016 VL 291 IS 27 BP 14034 EP 14044 DI 10.1074/jbc.M116.715565 PG 11 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DR5XG UT WOS:000379975100012 PM 27143480 ER PT J AU Wang, WJ Yan, RY Nocek, BP Vuong, TV Di Leo, R Xu, XH Cui, H Gatenholm, P Toriz, G Tenkanen, M Savchenko, A Master, ER AF Wang, Weijun Yan, Ruoyu Nocek, Boguslaw P. Vuong, Thu V. Di Leo, Rosa Xu, Xiaohui Cui, Hong Gatenholm, Paul Toriz, Guillermo Tenkanen, Maija Savchenko, Alexei Master, Emma R. TI Biochemical and Structural Characterization of a Five-domain GH115-Glucuronidase from the Marine Bacterium Saccharophagus degradans 2-40(T) SO JOURNAL OF BIOLOGICAL CHEMISTRY LA English DT Article DE carbohydrate; crystal structure; enzyme catalysis; enzyme structure; protein domain; GH115-glucuronidase; carbohydrate degradation; catalytic apparatus; enzyme domain composition ID PLANT-CELL WALL; THERMOTOGA-MARITIMA MSB8; ALPHA-GLUCURONIDASE; DENSITY MODIFICATION; FAMILY GH115; SCHIZOPHYLLUM-COMMUNE; INVERTING CHARACTER; CRYSTAL-STRUCTURES; XYLAN; POLYSACCHARIDES AB Glucuronic acid (GlcAp) and/or methylglucuronic acid (MeGlcAp) decorate the major forms of xylan in hardwood and coniferous softwoods as well as many cereal grains. Accordingly, the complete utilization of glucuronoxylans or conversion to sugar precursors requires the action of main chain xylanases as well as -glucuronidases that release the - (12)-linked (Me)GlcAp side groups. Herein, a family GH115 enzymefrom the marine bacterium Saccharophagus degradans 2-40(T), SdeAgu115A, demonstrated activity toward glucuronoxylan and oligomers thereof with preference toward MeGlcAp linked to internal xylopyranosyl residues. Unique biochemical characteristics of NaCl activation were also observed. The crystal structure of SdeAgu115A revealed a five-domain architecture, with an additional insertion C+ domain that had significant impact on the domain arrangement of SdeAgu115A monomer and its dimerization. The participation of domain C+ in substrate binding was supported by reduced substrate inhibition upon introducing W773A, W689A, and F696A substitutions within this domain. In addition to Asp-335, the catalytic essentiality of Glu-216 was revealed by site-specific mutagenesis. A primary sequence analysis suggested that the SdeAgu115A architecture is shared by more than half of GH115 members, thus defining a distinct archetype for GH115 enzymes. C1 [Wang, Weijun; Yan, Ruoyu; Vuong, Thu V.; Di Leo, Rosa; Xu, Xiaohui; Cui, Hong; Savchenko, Alexei; Master, Emma R.] Univ Toronto, Dept Chem Engn & Appl Chem, 200 Coll St, Toronto, ON M5S 3E5, Canada. [Nocek, Boguslaw P.] Argonne Natl Lab, Struct Biol Ctr, Biosci Div, 9700 S Cass Ave, Argonne, IL 60439 USA. [Gatenholm, Paul; Toriz, Guillermo] Chalmers, Dept Chem & Chem Engn, Wallenberg Wood Sci Ctr, Kemivagen 4, S-41296 Gothenburg, Sweden. [Gatenholm, Paul; Toriz, Guillermo] Chalmers, Biopolymer Technol, Kemivagen 4, S-41296 Gothenburg, Sweden. [Toriz, Guillermo] Univ Guadalajara, Dept Wood Cellulose & Paper Res, Guadalajara 44100, Mexico. [Tenkanen, Maija] Univ Helsinki, Dept Food & Environm Sci, POB 27, FIN-00014 Helsinki, Finland. RP Savchenko, A; Master, ER (reprint author), Univ Toronto, Dept Chem Engn & Appl Chem, 200 Coll St, Toronto, ON M5S 3E5, Canada. EM alexei.savchenko@utoronto.ca; emma.master@utoronto.ca FU United States Department of Energy, Office of Biological and Environmental Research [DE-AC02-06CH11357] FX We thank G. Brown and Professor A. Yakunin (University of Toronto) for technical support and Dr. Masoud Vedadi and Dr. Guillermo Senisterra (Structural Genomics Consortium, Toronto, Canada) for circular dichroism spectra acquisition. We also thank K. Parikka for preparing figures of xylan structures. Structural results shown in this report are derived from work performed at Argonne National Laboratory, Structural Biology Center at the Advanced Photon Source. Argonne National Laboratory is operated by UChicago Argonne, LLC, for the United States Department of Energy, Office of Biological and Environmental Research, under contract DE-AC02-06CH11357. NR 65 TC 1 Z9 1 U1 3 U2 3 PU AMER SOC BIOCHEMISTRY MOLECULAR BIOLOGY INC PI BETHESDA PA 9650 ROCKVILLE PIKE, BETHESDA, MD 20814-3996 USA SN 0021-9258 EI 1083-351X J9 J BIOL CHEM JI J. Biol. Chem. PD JUL 1 PY 2016 VL 291 IS 27 BP 14120 EP 14133 DI 10.1074/jbc.M115.702944 PG 14 WC Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DR5XG UT WOS:000379975100020 PM 27129264 ER PT J AU Dajnowicz, S Seaver, S Hanson, BL Fisher, SZ Langan, P Kovalevsky, AY Mueser, TC AF Dajnowicz, Steven Seaver, Sean Hanson, B. Leif Fisher, S. Zoe Langan, Paul Kovalevsky, Andrey Y. Mueser, Timothy C. TI Visualizing the Bohr effect in hemoglobin: neutron structure of equine cyanomethemoglobin in the R state and comparison with human deoxyhemoglobin in the T state SO ACTA CRYSTALLOGRAPHICA SECTION D-STRUCTURAL BIOLOGY LA English DT Article DE neutron crystallography; cyanomethemoglobin; alkaline Bohr effect; H/D exchange ID SURFACE HISTIDYL RESIDUES; NORMAL ADULT HEMOGLOBIN; X-RAY-DIFFRACTION; CRYSTAL-STRUCTURES; HYDROGEN-EXCHANGE; CRYSTALLOGRAPHY; BINDING; RESOLUTION; IDENTIFICATION; PROTEINS AB Neutron crystallography provides direct visual evidence of the atomic positions of deuterium-exchanged H atoms, enabling the accurate determination of the protonation/deuteration state of hydrated biomolecules. Comparison of two neutron structures of hemoglobins, human deoxyhemoglobin (T state) and equine cyanomethemoglobin (R state), offers a direct observation of histidine residues that are likely to contribute to the Bohr effect. Previous studies have shown that the T-state N-terminal and C-terminal salt bridges appear to have a partial instead of a primary overall contribution. Four conserved histidine residues [alpha His72(EF1), alpha His103(G10), alpha His89(FG1), alpha His112(G19) and beta His97(FG4)] can become protonated/deuterated from the R to the T state, while two histidine residues [alpha His20(B1) and beta His117(G19)] can lose a proton/deuteron. alpha His103(G10), located in the alpha(1):beta(1) dimer interface, appears to be a Bohr group that undergoes structural changes: in the R state it is singly protonated/deuterated and hydrogen-bonded through a water network to beta Asn108(G10) and in the T state it is doubly protonated/deuterated with the network uncoupled. The very long-term H/D exchange of the amide protons identifies regions that are accessible to exchange as well as regions that are impermeable to exchange. The liganded relaxed state (R state) has comparable levels of exchange (17.1% non-exchanged) compared with the deoxy tense state (T state; 11.8% non-exchanged). Interestingly, the regions of non-exchanged protons shift from the tetramer interfaces in the T-state interface (alpha(1):beta(2) and alpha(2):beta(1)) to the cores of the individual monomers and to the dimer interfaces (alpha(1):beta(1) and alpha(2):beta(2)) in the R state. The comparison of regions of stability in the two states allows a visualization of the conservation of fold energy necessary for ligand binding and release. C1 [Dajnowicz, Steven; Seaver, Sean; Hanson, B. Leif; Langan, Paul; Kovalevsky, Andrey Y.; Mueser, Timothy C.] Univ Toledo, Dept Chem & Biochem, 2801 W Bancroft St, Toledo, OH 43606 USA. [Fisher, S. Zoe] European Spallat Source, Sci Act Div, Sci Directorate, POB 176, S-22100 Lund, Sweden. [Langan, Paul; Kovalevsky, Andrey Y.] Oak Ridge Natl Lab, Biol & Soft Matter Div, Oak Ridge, TN USA. RP Mueser, TC (reprint author), Univ Toledo, Dept Chem & Biochem, 2801 W Bancroft St, Toledo, OH 43606 USA. EM timothy.mueser@utoledo.edu RI Langan, Paul/N-5237-2015; Hanson, Bryant Leif/F-8007-2010; OI Langan, Paul/0000-0002-0247-3122; Hanson, Bryant Leif/0000-0003-0345-3702; Kovalevsky, Andrey/0000-0003-4459-9142 FU Office of Biological and Environmental Research of the US Department of Energy; PCS; NIH-NIGMS [1R01GM071939-01]; NSF [446218]; University of Toledo FX The Protein Crystallography Station (PCS), located at Los Alamos Neutron Scattering Center (LANSCE), is funded by the Office of Biological and Environmental Research of the US Department of Energy. AYK, SZF and PL were supported by PCS. PL was partly supported by an NIH-NIGMS-funded consortium (1R01GM071939-01) between LANL and LBNL to develop computational tools for neutron protein crystallography. TCM, SS and BLH were supported by NSF (446218). SD was supported by The University of Toledo. NR 42 TC 1 Z9 1 U1 9 U2 15 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 2059-7983 J9 ACTA CRYSTALLOGR D JI Acta Crystallogr. Sect. D-Struct. Biol. PD JUL PY 2016 VL 72 BP 892 EP 903 DI 10.1107/S2059798316009049 PN 7 PG 12 WC Biochemical Research Methods; Biochemistry & Molecular Biology; Biophysics; Crystallography SC Biochemistry & Molecular Biology; Biophysics; Crystallography GA DR4ZM UT WOS:000379912500008 PM 27377386 ER PT J AU Yoon, JH Rasch, PJ Wang, HL Vinoj, V Ganguly, D AF Yoon, Jin-Ho Rasch, Philip J. Wang, Hailong Vinoj, V. Ganguly, Dilip TI The role of carbonaceous aerosols on short-term variations of precipitation over North Africa SO ATMOSPHERIC SCIENCE LETTERS LA English DT Article DE Sahel rainfall; aerosol indirect effect; cloud lifetime effect ID COMMUNITY ATMOSPHERE MODEL; SEA-SURFACE TEMPERATURE; ASIAN SUMMER MONSOON; SAHEL RAINFALL; MICROPHYSICS PARAMETERIZATION; CLIMATE VARIABILITY; CLOUD MICROPHYSICS; HYDROLOGICAL CYCLE; 20TH-CENTURY; ATLANTIC AB Subtropical North Africa has been subject to extensive droughts in the late 20th century, linked to changes in the sea surface temperature (SST). However, climate models forced by observed SSTs cannot reproduce the magnitude of the observed rainfall reduction. Here, we propose aerosol indirect effects (AIE) as an important positive feedback mechanism. Model results are presented using two sets of sensitivity experiments designed to distinguish the role of aerosol direct/semi-direct and indirect effects on regional precipitation. Changes in cloud properties due to the presence of carbonaceous aerosols are proposed as a key mechanism to explain the reduced rainfall over subtropical North Africa. C1 [Yoon, Jin-Ho] Gwangju Inst Sci & Technol, Sch Earth Sci & Environm Engn, 123 Cheomdan Gwagi Ro, Gwangju 61005, South Korea. [Rasch, Philip J.; Wang, Hailong] Pacific Northwest Natl Lab, Richland, WA USA. [Vinoj, V.] Indian Inst Technol, Sch Earth Ocean & Climate Sci, Bhubaneswar, Odisha, India. [Ganguly, Dilip] Indian Inst Technol Delhi, Ctr Atmospher Sci, New Delhi, India. RP Yoon, JH (reprint author), Gwangju Inst Sci & Technol, Sch Earth Sci & Environm Engn, 123 Cheomdan Gwagi Ro, Gwangju 61005, South Korea. EM yjinho@gist.ac.kr RI Wang, Hailong/B-8061-2010; OI Wang, Hailong/0000-0002-1994-4402; Vinoj, V./0000-0001-8573-6073 FU US Department of Energy, Office of Science, Biological and Environmental Research (BER) through the Earth System Modelling programme; US Department of Energy [DE-AC06-76RLO1830]; Korean Polar Research Institute [PE16100] FX We would like to acknowledge support from the US Department of Energy, Office of Science, Biological and Environmental Research (BER) through the Earth System Modelling programme. Comments from anonymous reviewers are helpful in improving the manuscript. We also thank Drs Carl Berkowitz and Zhao Chun at Pacific Northwest National Laboratory (PNNL) for providing helpful comments on an earlier version of the manuscript. PNNL is operated for the US Department of Energy by Battelle Memorial Institute under contract DE-AC06-76RLO1830. JHYoon was also partly supported by the funding from the Korean Polar Research Institute through the grant of PE16100. NR 70 TC 0 Z9 0 U1 2 U2 5 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1530-261X J9 ATMOS SCI LETT JI Atmos. Sci. Lett. PD JUL PY 2016 VL 17 IS 7 BP 407 EP 414 DI 10.1002/asl.672 PG 8 WC Geochemistry & Geophysics; Meteorology & Atmospheric Sciences SC Geochemistry & Geophysics; Meteorology & Atmospheric Sciences GA DR3VJ UT WOS:000379830400005 ER PT J AU Barrows, CW Murphy-Mariscal, ML Hernandez, RR AF Barrows, Cameron W. Murphy-Mariscal, Michelle L. Hernandez, Rebecca R. TI At a Crossroads: The Nature of Natural History in the Twenty-First Century SO BIOSCIENCE LA English DT Article DE ecology; education; field-based research; natural history; survey ID CLIMATE-CHANGE; SCIENCE; COMMUNITIES AB The relevance of natural history is challenged and marginalized today more than ever. We addressed the hypothesis that natural history is still relevant to the field of ecology by assessing the attitudes and perceptions related to natural history by early-career scientists and environmental-science professionals across 31 universities in California. Early-career scientists surveyed agreed that natural history is relevant to science (93%), and approximately 70% believed it "essential" for conducting field-based research; however, 54% felt inadequately trained to teach a natural-history course and would benefit from additional training in natural history (more than 80%). Of the 185 professionals surveyed, all felt that natural history is relevant to science and "essential" or "desirable" in their vocation (93%). Our results indicate a disconnection between the value and relevance of natural history in twenty-first-century ecological science and opportunities for gaining those skills and knowledge through education and training. C1 [Barrows, Cameron W.] Univ Calif Riverside, Ctr Conservat Biol, Riverside, CA 92521 USA. [Murphy-Mariscal, Michelle L.] Western Riverside Cty Multiple Species Habitat Co, Biol Monitoring Program, Riverside, CA USA. [Hernandez, Rebecca R.] Univ Calif Berkeley, Energy & Resources Grp, Berkeley, CA 94720 USA. [Hernandez, Rebecca R.] Lawrence Berkeley Natl Lab, Climate & Carbon Sci Program Area, Berkeley, CA USA. [Hernandez, Rebecca R.] Univ Calif Davis, Dept Land Air & Water Resources, Davis, CA 95616 USA. RP Barrows, CW (reprint author), Univ Calif Riverside, Ctr Conservat Biol, Riverside, CA 92521 USA. EM cbarrows@ucr.edu NR 26 TC 1 Z9 3 U1 7 U2 7 PU OXFORD UNIV PRESS PI OXFORD PA GREAT CLARENDON ST, OXFORD OX2 6DP, ENGLAND SN 0006-3568 EI 1525-3244 J9 BIOSCIENCE JI Bioscience PD JUL PY 2016 VL 66 IS 7 BP 592 EP 599 DI 10.1093/biosci/biw043 PG 8 WC Biology SC Life Sciences & Biomedicine - Other Topics GA DR7JD UT WOS:000380075000010 ER PT J AU Freedman, LP Gibson, MC Bradbury, ARM Buchberg, AM Davis, D Dolled-Filhart, MP Lund-Johansen, F Rimm, DL AF Freedman, Leonard P. Gibson, Mark C. Bradbury, Andrew R. M. Buchberg, Arthur M. Davis, Darryl Dolled-Filhart, Marisa P. Lund-Johansen, Fridtjof Rimm, David L. TI The need for improved education and training in research antibody usage and validation practices SO BIOTECHNIQUES LA English DT Letter ID REPRODUCIBILITY C1 [Freedman, Leonard P.; Gibson, Mark C.] Global Biol Stand Inst, 1020 19th St,NW,Suite 550, Washington, DC 20036 USA. [Bradbury, Andrew R. M.] Los Alamos Natl Lab, Los Alamos, NM 87545 USA. [Buchberg, Arthur M.] Amer Assoc Canc Res, Philadelphia, PA USA. [Davis, Darryl] Janssen R&D LLC, Spring House, PA USA. [Dolled-Filhart, Marisa P.] Merck, Rahway, NJ USA. [Lund-Johansen, Fridtjof] Oslo Univ Hosp, N-0450 Oslo, Norway. [Rimm, David L.] Yale Univ, New Haven, CT USA. RP Freedman, LP (reprint author), Global Biol Stand Inst, 1020 19th St,NW,Suite 550, Washington, DC 20036 USA. EM lfreedman@gbsi.org OI Bradbury, Andrew/0000-0002-5567-8172 NR 18 TC 2 Z9 2 U1 5 U2 5 PU BIOTECHNIQUES OFFICE PI NEW YORK PA 52 VANDERBILT AVE, NEW YORK, NY 10017 USA SN 0736-6205 EI 1940-9818 J9 BIOTECHNIQUES JI Biotechniques PD JUL PY 2016 VL 61 IS 1 BP 16 EP 18 DI 10.2144/000114431 PG 3 WC Biochemical Research Methods; Biochemistry & Molecular Biology SC Biochemistry & Molecular Biology GA DR2OG UT WOS:000379743200003 PM 27401669 ER PT J AU Lambert, CG Mazurie, AJ Lauve, NR Hurwitz, NG Young, SS Obenchain, RL Hengartner, NW Perkins, DJ Tohen, M Kerner, B AF Lambert, C. G. Mazurie, A. J. Lauve, N. R. Hurwitz, N. G. Young, S. S. Obenchain, R. L. Hengartner, N. W. Perkins, D. J. Tohen, M. Kerner, B. TI Hypothyroidism risk compared among nine common bipolar disorder therapies in a large US Cohort SO BIPOLAR DISORDERS LA English DT Meeting Abstract CT 18th Annual Conference of the International-Society-for-Bipolar-Disorders / 8th Biennial Conference of the International-Society-for-Affective-Disorders CY JUL 13-16, 2016 CL Amsterdam, NETHERLANDS SP Int Soc Bipolar Disorders, Int Soc Affect Disorders C1 [Lambert, C. G.] Univ New Mexico, Hlth Sci Ctr, Ctr Global Hlth, Div Translat Informat,Dept Internal Med, Albuquerque, NM 87131 USA. [Mazurie, A. J.] Montana State Univ, Bioinformat Core, Bozeman, MT 59717 USA. [Lauve, N. R.] Univ New Mexico, Comp Sci, Albuquerque, NM 87131 USA. [Hurwitz, N. G.] New Mexico Behav Hlth Inst, Las Vegas, NV USA. [Young, S. S.] CGStat LLC, Raleigh, NC USA. [Obenchain, R. L.] Risk Benefit Stat LLC, Bella Vista, CA USA. [Hengartner, N. W.] Los Alamos Natl Lab, Theoret Biol Grp, Div Theoret, Los Alamos, NM USA. [Perkins, D. J.] Univ New Mexico, Hlth Sci Ctr, Dept Internal Med, Ctr Global Hlth, Albuquerque, NM 87131 USA. [Tohen, M.] Univ New Mexico, Hlth Sci Ctr, Dept Psychiat & Behav Sci, Albuquerque, NM 87131 USA. [Kerner, B.] Univ Calif Los Angeles, Semel Inst Neurosci & Human Behav, David Geffen Sch Med, Los Angeles, CA 90024 USA. NR 0 TC 0 Z9 0 U1 1 U2 1 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1398-5647 EI 1399-5618 J9 BIPOLAR DISORD JI Bipolar Disord. PD JUL PY 2016 VL 18 SU 1 SI SI MA RC-14 BP 65 EP 65 PG 1 WC Clinical Neurology; Neurosciences; Psychiatry SC Neurosciences & Neurology; Psychiatry GA DR5KI UT WOS:000379941500154 ER PT J AU Troia, MJ McManamay, RA AF Troia, Matthew J. McManamay, Ryan A. TI Filling in the GAPS: evaluating completeness and coverage of open-access biodiversity databases in the United States SO ECOLOGY AND EVOLUTION LA English DT Article DE Biodiversity; Global Biodiversity Information Facility; museum collections; National Rivers and Streams Assessment; National Water Quality Assessment; North American Breeding Bird Survey; Regional Environmental Monitoring and Assessment Program; species distribution modeling; Wallacean shortfall ID SPECIES DISTRIBUTION MODELS; FRESH-WATER FISHES; TERRESTRIAL BIODIVERSITY; INFORMATION FACILITY; RICHNESS PATTERNS; GLOBAL DIVERSITY; NICHE; BIAS; SIZE; HOMOGENIZATION AB Primary biodiversity data constitute observations of particular species at given points in time and space. Open-access electronic databases provide unprecedented access to these data, but their usefulness in characterizing species distributions and patterns in biodiversity depend on how complete species inventories are at a given survey location and how uniformly distributed survey locations are along dimensions of time, space, and environment. Our aim was to compare completeness and coverage among three open-access databases representing ten taxonomic groups (amphibians, birds, freshwater bivalves, crayfish, freshwater fish, fungi, insects, mammals, plants, and reptiles) in the contiguous United States. We compiled occurrence records from the Global Biodiversity Information Facility (GBIF), the North American Breeding Bird Survey (BBS), and federally administered fish surveys (FFS). We aggregated occurrence records by 0.1 degrees x0.1 degrees grid cells and computed three completeness metrics to classify each grid cell as well-surveyed or not. Next, we compared frequency distributions of surveyed grid cells to background environmental conditions in a GIS and performed Kolmogorov-Smirnov tests to quantify coverage through time, along two spatial gradients, and along eight environmental gradients. The three databases contributed >13.6million reliable occurrence records distributed among >190,000 grid cells. The percent of well-surveyed grid cells was substantially lower for GBIF (5.2%) than for systematic surveys (BBS and FFS; 82.5%). Still, the large number of GBIF occurrence records produced at least 250 well-surveyed grid cells for six of nine taxonomic groups. Coverages of systematic surveys were less biased across spatial and environmental dimensions but were more biased in temporal coverage compared to GBIF data. GBIF coverages also varied among taxonomic groups, consistent with commonly recognized geographic, environmental, and institutional sampling biases. This comprehensive assessment of biodiversity data across the contiguous United States provides a prioritization scheme to fill in the gaps by contributing existing occurrence records to the public domain and planning future surveys. C1 [Troia, Matthew J.; McManamay, Ryan A.] Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. RP Troia, MJ (reprint author), Oak Ridge Natl Lab, Div Environm Sci, Oak Ridge, TN 37831 USA. EM troiamj@gmail.com FU United States Department of Energy's Office of Energy Efficiency and Renewable Energy, Wind and Water Power Technologies Program FX This research was sponsored by the United States Department of Energy's Office of Energy Efficiency and Renewable Energy, Wind and Water Power Technologies Program. NR 74 TC 0 Z9 0 U1 13 U2 25 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 2045-7758 J9 ECOL EVOL JI Ecol. Evol. PD JUL PY 2016 VL 6 IS 14 BP 4654 EP 4669 DI 10.1002/ece3.2225 PG 16 WC Ecology; Evolutionary Biology SC Environmental Sciences & Ecology; Evolutionary Biology GA DR6TE UT WOS:000380033400004 PM 27547303 ER PT J AU Joe, JC Hendrickson, K Wong, M Kane, SL Solan, D Carlisle, JE Koehler, D Ames, DP Beazer, R AF Joe, Jeffrey C. Hendrickson, Kelsie Wong, Maria Kane, Stephanie L. Solan, David Carlisle, Juliet E. Koehler, David Ames, Daniel P. Beazer, Robert TI Political efficacy and familiarity as predictors of attitudes towards electric transmission lines in the United States SO ENERGY RESEARCH & SOCIAL SCIENCE LA English DT Article DE High voltage overhead transmission lines; Political efficacy; Familiarity; Place attachment ID WIND ENERGY LANDSCAPES; PUBLIC-ATTITUDES; OPINION LEADERSHIP; PLACE ATTACHMENT; DECISION-MAKING; FIT INDEXES; POWER; PERCEPTIONS; HABITUATION; TECHNOLOGY AB Public opposition to the construction (i.e., siting) of new high voltage overhead transmission lines is not a new or isolated phenomenon. Past research has posited a variety of reasons, applied general theories, and has provided empirical evidence to explain public opposition. The existing literature, while clarifying many elements of the issue, does not yet fully explain the complexities underlying this public opposition phenomenon. The current study demonstrated how two overlooked factors, people's sense of political efficacy and their familiarity (i.e., prior exposure) with transmission lines, explained attitudes of support and opposition to siting new power lines. (C) 2016 Elsevier Ltd. All rights reserved. C1 [Joe, Jeffrey C.] Idaho Natl Lab, POB 1625,Mail Stop 3818, Idaho Falls, ID 83415 USA. [Hendrickson, Kelsie; Wong, Maria] Idaho State Univ, Dept Psychol, 921 S 8th Ave,Stop 8112, Pocatello, ID 83209 USA. [Kane, Stephanie L.] Washington State Univ, Off Inst Res, Pullman, WA 99164 USA. [Solan, David; Koehler, David] Boise State Univ, Energy Policy Inst, 1910 Univ Dr, Boise, ID 83725 USA. [Carlisle, Juliet E.] Univ Idaho, Dept Polit Sci, Moscow, ID 83843 USA. [Ames, Daniel P.] Brigham Young Univ, Dept Civil & Environm Engn, 368 Clyde Bldg, Provo, UT 84602 USA. [Beazer, Robert] Idaho State Univ, Dept Geosci, Pocatello, ID 83209 USA. RP Joe, JC (reprint author), Idaho Natl Lab, POB 1625,Mail Stop 3818, Idaho Falls, ID 83415 USA. EM Jeffrey.Joe@inl.gov; hendkel2@isu.edu; wongmari@isu.edu; slkane@wsu.edu; davidsolan@boisestate.edu; carlisle@uidaho.edu; davekoehler@boisestate.edu; dan.ames@byu.edu; beazrobe@isu.edu NR 67 TC 0 Z9 0 U1 5 U2 6 PU ELSEVIER SCIENCE BV PI AMSTERDAM PA PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS SN 2214-6296 EI 2214-6326 J9 ENERGY RES SOC SCI JI Energy Res. Soc. Sci. PD JUL PY 2016 VL 17 BP 127 EP 134 DI 10.1016/j.erss.2016.04.010 PG 8 WC Environmental Studies SC Environmental Sciences & Ecology GA DQ8CJ UT WOS:000379436400012 ER PT J AU Myers, TW Brown, KE Chavez, DE Scharff, RJ Veauthier, JM AF Myers, Thomas W. Brown, Kathryn E. Chavez, David E. Scharff, R. Jason Veauthier, Jacqueline M. TI Correlating the Structural, Electronic, and Explosive Sensitivity Properties of CuII Tetrazine Complexes SO EUROPEAN JOURNAL OF INORGANIC CHEMISTRY LA English DT Article DE Energetic materials; Explosives; Copper; Nitrogen heterocycles; Ligand design; Coordination modes ID IGNITABLE PRIMARY EXPLOSIVES; ENERGETIC MATERIALS; PYROTECHNIC COMPOSITIONS; PERCHLORATE; NITROGEN; NITRATE; SALTS; LEAD; 1,2,4,5-TETRAZINES; CRYSTAL AB The synthesis and characterization of explosive coordination complexes of Cu-II with nitrogen-rich tetrazine ligands and nitrate counter-anions have been achieved. The complexes adopt a variety of coordination geometries including monomeric and dimeric architectures with five and six coordinate Cu-II centers. The thermal stabilities of the complexes correlate to the strength of the Cu-nitrate interaction such that more strongly bound nitrates exhibit higher thermal stability. Exchanging amine groups on the coordinating ligands with 3,3-dinitroazetidine groups led to changes in the solid-state structures and increases to the impact sensitivity of the resulting complexes relative to the corresponding amine derivatives. C1 [Myers, Thomas W.; Brown, Kathryn E.; Chavez, David E.; Scharff, R. Jason; Veauthier, Jacqueline M.] Los Alamos Natl Lab, M Div, MS C920, Los Alamos, NM 87544 USA. [Myers, Thomas W.; Brown, Kathryn E.; Chavez, David E.; Scharff, R. Jason; Veauthier, Jacqueline M.] Los Alamos Natl Lab, Div Chem, MS C920, Los Alamos, NM 87544 USA. RP Myers, TW (reprint author), Los Alamos Natl Lab, M Div, MS C920, Los Alamos, NM 87544 USA.; Myers, TW (reprint author), Los Alamos Natl Lab, Div Chem, MS C920, Los Alamos, NM 87544 USA. EM twmyers@lanl.gov OI Scharff, Robert/0000-0002-1708-8964; Veauthier, Jacqueline/0000-0003-2206-7786 FU U.S. Department of Energy; National Nuclear Security Administration of the U.S. Department of Energy [DE-AC52-06NA25396] FX The authors thank A. M. Giambra, H. Tian, and M. Sandstrom for assistance with elemental, thermal and explosive sensitivity analyses. In addition we thank K. Ramos and G. K. Windler for assistance with explosive single crystal XRD. For financial support of this work, we acknowledge the U.S. Department of Energy through the LANL LDRD Program and the Director's Post-Doctoral Fellowship Program (PD fellowship to T.W. M.). Los Alamos National Laboratory is operated by Los Alamos National Security, LLC, for the National Nuclear Security Administration of the U.S. Department of Energy (contract number DE-AC52-06NA25396). NR 31 TC 2 Z9 2 U1 5 U2 11 PU WILEY-V C H VERLAG GMBH PI WEINHEIM PA POSTFACH 101161, 69451 WEINHEIM, GERMANY SN 1434-1948 EI 1099-0682 J9 EUR J INORG CHEM JI Eur. J. Inorg. Chem. PD JUL PY 2016 IS 19 BP 3178 EP 3183 DI 10.1002/ejic.201600344 PG 6 WC Chemistry, Inorganic & Nuclear SC Chemistry GA DR5CB UT WOS:000379919500015 ER PT J AU Liu, X Thadesar, PA Taylor, CL Kunz, M Tamura, N Bakir, MS Sitaraman, SK AF Liu, Xi Thadesar, Paragkumar A. Taylor, Christine L. Kunz, Martin Tamura, Nobumichi Bakir, Muhannad S. Sitaraman, Suresh K. TI Experimental Stress Characterization and Numerical Simulation for Copper Pumping Analysis of Through-Silicon Vias SO IEEE TRANSACTIONS ON COMPONENTS PACKAGING AND MANUFACTURING TECHNOLOGY LA English DT Article DE Copper pumping; finite-element analysis; synchrotron X-ray diffraction; through-silicon vias (TSVs) ID TSV; WAFER AB In this paper, a 3-D thermomechanical model of through-silicon vias (TSVs) has been analyzed and verified with in situ microscale strain measurements by synchrotron X-ray microdiffraction. Thereafter, a comprehensive stress/strain analysis on copper pumping and back-end-of-line (BEOL) cracking issues has been carried out. In addition, a design-of-experiments-based approach has been used to understand the effect of various parameters on copper pumping and BEOL stress. The results show that the smaller TSV diameter and thinner silicon die help reduce the copper pumping and thus mitigate BEOL stress. C1 [Liu, Xi; Taylor, Christine L.; Sitaraman, Suresh K.] Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. [Liu, Xi; Thadesar, Paragkumar A.; Bakir, Muhannad S.] Georgia Inst Technol, Sch Elect & Comp Engn, Atlanta, GA 30332 USA. [Kunz, Martin; Tamura, Nobumichi] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Liu, X (reprint author), Georgia Inst Technol, George W Woodruff Sch Mech Engn, Atlanta, GA 30332 USA. EM xi.liu@gatech.edu; pthadesar3@gatech.edu; c.taylor@gatech.edu; mkunz@lbl.gov; ntamura@lbl.gov; muhannad.bakir@mirc.gatech.edu; suresh.sitaraman@me.gatech.edu FU Semiconductor Research Corporation [2012-KJ-2255]; Advanced Light Source within Office of Science, Office of Basic Energy Sciences; Lawrence Berkeley National Laboratory through U.S. Department of Energy [DE-AC02-05CH11231] FX This work was supported in part by Semiconductor Research Corporation under Contract 2012-KJ-2255, in part by Advanced Light Source within the Office of Science, Office of Basic Energy Sciences, and in part by the Lawrence Berkeley National Laboratory through the U.S. Department of Energy under Contract DE-AC02-05CH11231. Recommended for publication by Associate Editor D. Goyal upon evaluation of reviewers' comments. NR 22 TC 0 Z9 0 U1 5 U2 6 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 2156-3950 EI 2156-3985 J9 IEEE T COMP PACK MAN JI IEEE Trans. Compon. Pack. Manuf. Technol. PD JUL PY 2016 VL 6 IS 7 BP 995 EP 1001 DI 10.1109/TCPMT.2015.2507164 PG 7 WC Engineering, Manufacturing; Engineering, Electrical & Electronic; Materials Science, Multidisciplinary SC Engineering; Materials Science GA DR5WS UT WOS:000379973700004 ER PT J AU Gaunkar, NGP Nlebedim, IC Bulu, I Mina, M Hadimani, RL Song, YQ Jiles, DC AF Gaunkar, N. G. Prabhu Nlebedim, I. C. Bulu, I. Mina, M. Hadimani, R. L. Song, Y. Q. Jiles, D. C. TI Broadband Analysis of Response From Magnetic Cores Used in Inductive Sensors for Pulsed Nuclear Magnetic Resonance Applications SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article; Proceedings Paper CT 13th Joint Magnetism and Magnetic Materials (MMM)/Intermag Conference CY JAN 11-15, 2016 CL San Diego, CA SP Amer Inst Phys, IEEE Magnet soc DE Inductive sensors; magnetic core; nuclear magnetic resonance (NMR); ringing ID NMR; SPECTROSCOPY; SUPPRESSION; SYSTEM AB Inductive sensors used in oil-field well-logging instruments can detect the presence of oil/water in earth formations. The inductive sensor acts as both a signal transmitter and receiver and, at the same time, contributes its own intrinsic signal to each measurement. Often, this contribution can mask the actual measured signal. It is thus vital to reduce the contribution of the inductive sensor signal from the measured signal. Since the major contributor to the signal from the inductive sensor is the magnetic core, the focus of this paper is to identify its signal characteristics and minimize the interference due to the magnetic core material. On the basis of a signal analysis, Mu 125 is identified as a suitable core material for inductive sensors due to its lower signal amplitude and shorter decay time at each resonant frequency. C1 [Gaunkar, N. G. Prabhu; Nlebedim, I. C.; Mina, M.; Hadimani, R. L.; Jiles, D. C.] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. [Nlebedim, I. C.] US DOE, Ames Lab, Ames, IA 50011 USA. [Bulu, I.; Song, Y. Q.] Schlumberger Doll Res Div, Cambridge, MA 02139 USA. RP Gaunkar, NGP (reprint author), Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. EM neelampg@iastate.edu NR 19 TC 0 Z9 0 U1 3 U2 4 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 EI 1941-0069 J9 IEEE T MAGN JI IEEE Trans. Magn. PD JUL PY 2016 VL 52 IS 7 AR 2800404 DI 10.1109/TMAG.2016.2527794 PG 4 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA DR5EC UT WOS:000379924800043 ER PT J AU Lin, H Gao, Y Wang, XJ Nan, TX Liu, M Lou, J Yang, GM Zhou, ZY Yang, X Wu, J Li, M Hu, ZQ Sun, NX AF Lin, Hwaider Gao, Yuan Wang, Xinjun Nan, Tianxiang Liu, Ming Lou, Jing Yang, Guomin Zhou, Ziyao Yang, Xi Wu, Jing Li, Ming Hu, Zhongqiang Sun, Nian Xiang TI Integrated Magnetics and Multiferroics for Compact and Power-Efficient Sensing, Memory, Power, RF, and Microwave Electronics SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article; Proceedings Paper CT 13th Joint Magnetism and Magnetic Materials (MMM)/Intermag Conference CY JAN 11-15, 2016 CL San Diego, CA SP Amer Inst Phys, IEEE Magnet soc DE Magnetoelectric (ME); magnetometer; multiferroic; tunable RF ID ELECTRIC-FIELD CONTROL; MAGNETOELECTRIC COMPOSITES; FERROMAGNETIC-RESONANCE; PT HETEROSTRUCTURES; ROOM-TEMPERATURE; BANDPASS FILTER; PATCH ANTENNAS; FERRITE FILMS; PHASE-SHIFTER; VOLTAGE AB The coexistence of electric polarization and magnetization in multiferroic materials provides great opportunities for realizing magnetoelectric (ME) coupling, including electric field control of magnetism, or vice versa, through a strain-mediated ME coupling in layered magnetic/ferroelectric multiferroic heterostructures. Strong ME coupling has been the enabling factor for different multiferroic devices, which, however, has been elusive, particularly at RF/microwave frequencies. In this paper, most recent progress on new integrated multiferroic devices for sensing RF and microwave electronics will be presented, including novel RF Nano-electromechanical systems ME resonators with picotesla sensitivity for dc magnetic fields and novel gigahertz magnetic and multiferroic integrated inductors with a wide operation frequency range of 0.3 similar to 3 GHz, a high quality factor close to 20, and a voltage tunable inductance of 50%similar to 150%. At the same time, we will also demonstrate other tunable RF devices, including integrated non-reciprocal tunable bandpass filter with ultrawideband isolation more than 13 dB. These novel magnetics and multiferroic devices show great promise for applications, such as compact, lightweight, and power-efficient sensing, memory, RF, and microwave integrated electronics. C1 [Lin, Hwaider; Gao, Yuan; Wang, Xinjun; Lou, Jing; Wu, Jing; Li, Ming; Sun, Nian Xiang] Northeastern Univ, Dept Elect & Comp Engn, WM Keck Lab Integrated Ferro, Boston, MA 02115 USA. [Nan, Tianxiang] Univ Wisconsin, Madison, WI 53706 USA. [Liu, Ming] Xi An Jiao Tong Univ, Xian 710049, Peoples R China. [Yang, Guomin] Fudan Univ, Shanghai 200433, Peoples R China. [Zhou, Ziyao] Argonne Natl Lab, Lemont, IL 60439 USA. [Yang, Xi] Beijing Inst Technol, Beijing 100083, Peoples R China. [Hu, Zhongqiang] Air Force Res Lab, Wright Patterson AFB, OH 45433 USA. RP Sun, NX (reprint author), Northeastern Univ, Dept Elect & Comp Engn, WM Keck Lab Integrated Ferro, Boston, MA 02115 USA. EM nian@ece.neu.edu RI Gao, Yuan/E-4277-2016; Liu, Ming/B-4143-2009; OI Gao, Yuan/0000-0002-2444-1180; Liu, Ming/0000-0002-6310-948X; Hu, Zhongqiang/0000-0002-7534-0427 NR 79 TC 1 Z9 1 U1 25 U2 35 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 EI 1941-0069 J9 IEEE T MAGN JI IEEE Trans. Magn. PD JUL PY 2016 VL 52 IS 7 AR 4002208 DI 10.1109/TMAG.2016.2514982 PG 8 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA DR5EC UT WOS:000379924800100 ER PT J AU Ni, Y Zhang, Z Nlebedim, IC Jiles, DC AF Ni, Y. Zhang, Z. Nlebedim, I. C. Jiles, D. C. TI Ultrahigh Sensitivity of Anomalous Hall Effect Sensor Based on Cr-Doped Bi2Te3 Topological Insulator Thin Films SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article; Proceedings Paper CT 13th Joint Magnetism and Magnetic Materials (MMM)/Intermag Conference CY JAN 11-15, 2016 CL San Diego, CA SP Amer Inst Phys, IEEE Magnet soc DE Anomalous Hall effect (AHE) sensor; sensitivity; thin films; topological insulators (TIs) AB Anomalous Hall effect (AHE) was recently discovered in magnetic element-doped topological insulators (TIs), which promises low power consumption and high efficiency spintronics and electronics. This discovery broadens the family of Hall sensors. In this paper, AHE sensors based on Cr-doped Bi2Te3 topological insulator thin films are studied with two thicknesses (15 and 65 nm). It is found, in both cases, that ultrahigh Hall sensitivity can be obtained in Cr-doped Bi2Te3. Hall sensitivity reaches 1666 Omega/T in the sensor with the 15 nm TI thin film, which is higher than that of the conventional semiconductor HE sensor. The AHE of 65 nm sensors is even stronger, which causes the sensitivity increasing to 2620 Omega/T. Furthermore, after comparing Cr-doped Bi2Te3 with the previously studied Mn-doped Bi2Te3 TI Hall sensor, the sensitivity of the present AHE sensor shows about 60 times higher in 65 nm sensors. The implementation of AHE sensors based on a magnetic-doped TI thin film indicates that the TIs are good candidates for ultrasensitive AHE sensors. C1 [Ni, Y.; Zhang, Z.; Nlebedim, I. C.; Jiles, D. C.] Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. [Nlebedim, I. C.] US DOE, Ames Lab, Ames, IA 50011 USA. RP Zhang, Z (reprint author), Iowa State Univ, Dept Elect & Comp Engn, Ames, IA 50011 USA. EM zhenn.zhang@gmail.com NR 21 TC 0 Z9 0 U1 15 U2 21 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 EI 1941-0069 J9 IEEE T MAGN JI IEEE Trans. Magn. PD JUL PY 2016 VL 52 IS 7 AR 4002304 DI 10.1109/TMAG.2016.2519512 PG 4 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA DR5EC UT WOS:000379924800101 ER PT J AU Poudel, N Gooch, M Lorenz, B Chu, CW Kim, J Cheong, SW AF Poudel, Narayan Gooch, Melissa Lorenz, Bernd Chu, Ching-Wu Kim, Jaewook Cheong, Sang-Wook TI Pressure Effect on Ferroelectric Properties of GdMn2O5 and TmMn2O5 SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article; Proceedings Paper CT 13th Joint Magnetism and Magnetic Materials (MMM)/Intermag Conference CY JAN 11-15, 2016 CL San Diego, CA SP Amer Inst Phys, IEEE Magnet soc DE Exchange striction; ferroelectric (FE); multiferroic; pressure effect ID MULTIFERROIC HOMN2O5; POLARIZATION AB The pressure effect on the ferroelectric (FE) properties of the multiferroic compounds GdMn2O5 and TmMn2O5 was studied up to 18.2 kbars. A new FE phase was observed at a higher temperature in GdMn2O5 above a critical pressure, P-c approximate to 10 kbars. Our results indicate that pressure decouples the Gd moment from Mn spin system and splits the FE phase. Thermal expansion measurements reveal a large increase of the c-axis at the ambient-pressure FE transition. The pressure-induced contraction of the c lattice parameter is considered to be the origin of the decoupling of both spin systems above P-c. From the dielectric and FE properties of GdMn2O5, a pressure-temperature phase diagram can be derived. While a new phase was discovered for GdMn2O5, no significant change in polarization was observed for TmMn2O5 up to 16.6 kbars. C1 [Poudel, Narayan; Gooch, Melissa; Lorenz, Bernd; Chu, Ching-Wu] Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA. [Poudel, Narayan; Gooch, Melissa; Lorenz, Bernd; Chu, Ching-Wu] Univ Houston, Dept Phys, Houston, TX 77204 USA. [Chu, Ching-Wu] Lawrence Berkeley Natl Lab, 1 Cyclotron Rd, Berkeley, CA 94720 USA. [Kim, Jaewook; Cheong, Sang-Wook] Rutgers State Univ, Rutgers Ctr Emergent Mat, Piscataway, NJ 08854 USA. [Kim, Jaewook; Cheong, Sang-Wook] Rutgers State Univ, Dept Phys & Astron, POB 849, Piscataway, NJ 08854 USA. RP Poudel, N (reprint author), Univ Houston, Texas Ctr Superconduct, Houston, TX 77204 USA.; Poudel, N (reprint author), Univ Houston, Dept Phys, Houston, TX 77204 USA. EM npoudel@uh.edu NR 21 TC 0 Z9 0 U1 11 U2 11 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 EI 1941-0069 J9 IEEE T MAGN JI IEEE Trans. Magn. PD JUL PY 2016 VL 52 IS 7 AR 2501204 DI 10.1109/TMAG.2016.2528169 PG 4 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA DR5EC UT WOS:000379924800036 ER PT J AU Sterwerf, C Meinert, M Arenholz, E Schmalhorst, JM Reiss, G AF Sterwerf, Christian Meinert, Markus Arenholz, Elke Schmalhorst, Jan-Michael Reiss, Guenter TI Room Temperature Exchange Bias in BiFeO3/Co-Fe Bilayers SO IEEE TRANSACTIONS ON MAGNETICS LA English DT Article; Proceedings Paper CT 13th Joint Magnetism and Magnetic Materials (MMM)/Intermag Conference CY JAN 11-15, 2016 CL San Diego, CA SP Amer Inst Phys, IEEE Magnet soc DE Antiferromagnet; BiFeO3; exchange bias; magnetic coupling; magnetic films; reactive sputtering ID DICHROISM AB Thin highly epitaxial BiFeO3 films were prepared on SrTiO3 (100) substrates by reactive magnetron cosputtering. Detailed magneto-optic Kerr effect (MOKE) measurements on BiFeO3/Co-Fe bilayers were performed to investigate the exchange bias as a function of film thicknesses and Co-Fe stoichiometries. We found a maximum exchange bias of H-eb = 92 Oe and a coercive field of H-c = 89 Oe for a 12.5 nm-thick BiFeO3 film with a 2 nm-thick Co layer. The unidirectional anisotropy is clearly visible in in-plane rotational MOKE measurements. Anisotropic magnetoresistance measurements reveal a strongly increasing coercivity with decreasing temperature, but no significant change in the exchange bias field. C1 [Sterwerf, Christian; Meinert, Markus; Schmalhorst, Jan-Michael; Reiss, Guenter] Univ Bielefeld, Dept Phys, Ctr Spinelect Mat & Devices, D-33615 Bielefeld, Germany. [Arenholz, Elke] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA. RP Sterwerf, C (reprint author), Univ Bielefeld, Dept Phys, Ctr Spinelect Mat & Devices, D-33615 Bielefeld, Germany. EM csterwerf@physik.uni-bielefeld.de RI Meinert, Markus/E-8794-2011; Reiss, Gunter/A-3423-2010 OI Meinert, Markus/0000-0002-7813-600X; Reiss, Gunter/0000-0002-0918-5940 NR 16 TC 0 Z9 0 U1 12 U2 19 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 0018-9464 EI 1941-0069 J9 IEEE T MAGN JI IEEE Trans. Magn. PD JUL PY 2016 VL 52 IS 7 AR 4800204 DI 10.1109/TMAG.2015.2510544 PG 4 WC Engineering, Electrical & Electronic; Physics, Applied SC Engineering; Physics GA DR5EC UT WOS:000379924800115 ER PT J AU Guggilam, SS Dall'Anese, E Chen, YC Dhople, SV Giannakis, GB AF Guggilam, Swaroop S. Dall'Anese, Emiliano Chen, Yu Christine Dhople, Sairaj V. Giannakis, Georgios B. TI Scalable Optimization Methods for Distribution Networks With High PV Integration SO IEEE TRANSACTIONS ON SMART GRID LA English DT Article DE Distribution networks; linearization; optimization; PV systems ID RESIDENTIAL DISTRIBUTION-SYSTEMS; ALTERNATING DIRECTION METHOD; PHOTOVOLTAIC INVERTERS; OPTIMAL DISPATCH; REACTIVE POWER; MULTIPLIERS; GRIDS AB This paper proposes a suite of algorithms to determine the active- and reactive-power setpoints for photovoltaic (PV) inverters in distribution networks. The objective is to optimize the operation of the distribution feeder according to a variety of performance objectives and ensure voltage regulation. In general, these algorithms take a form of the widely studied ac optimal power flow (OPF) problem. For the envisioned application domain, nonlinear power-flow constraints render pertinent OPF problems nonconvex and computationally intensive for large systems. To address these concerns, we formulate a quadratic constrained quadratic program (QCQP) by leveraging a linear approximation of the algebraic power-flow equations. Furthermore, simplification from QCQP to a linearly constrained quadratic program is provided under certain conditions. The merits of the proposed approach are demonstrated with simulation results that utilize realistic PV-generation and load-profile data for illustrative distribution-system test feeders. C1 [Guggilam, Swaroop S.; Dhople, Sairaj V.; Giannakis, Georgios B.] Univ Minnesota, Dept Elect & Comp Engn, Minneapolis, MN 55455 USA. [Guggilam, Swaroop S.; Dhople, Sairaj V.; Giannakis, Georgios B.] Univ Minnesota, Digital Technol Ctr, Minneapolis, MN 55455 USA. [Dall'Anese, Emiliano] Natl Renewable Energy Lab, Golden, CO 80401 USA. [Chen, Yu Christine] Univ British Columbia, Dept Elect & Comp Engn, Vancouver, BC V6T 1Z4, Canada. RP Guggilam, SS (reprint author), Univ Minnesota, Dept Elect & Comp Engn, Minneapolis, MN 55455 USA.; Guggilam, SS (reprint author), Univ Minnesota, Digital Technol Ctr, Minneapolis, MN 55455 USA. EM guggi022@umn.edu; emiliano.dallanese@nrel.gov; chen@ece.ubc.ca; sdhople@umn.edu; georgios@umn.edu FU National Science Foundation under Grant CCF [1423316]; National Science Foundation under Grant CyberSEES [1442686]; National Science Foundation under Grant CAREER Award [ECCS-1453921]; Institute of Renewable Energy and Environment, University of Minnesota [RL-0010-13]; Laboratory Directed Research and Development Program at the National Renewable Energy Laboratory FX The work of S. S. Guggilam, S. V. Dhople, and G. B. Giannakis were supported in part by the National Science Foundation under Grant CCF 1423316, Grant CyberSEES 1442686, and Grant CAREER Award ECCS-1453921, and in part by the Institute of Renewable Energy and the Environment, University of Minnesota, under Grant RL-0010-13. The work of E. Dall'Anese was supported by the Laboratory Directed Research and Development Program at the National Renewable Energy Laboratory. Paper no. TSG-01151-2015. NR 34 TC 0 Z9 0 U1 3 U2 3 PU IEEE-INST ELECTRICAL ELECTRONICS ENGINEERS INC PI PISCATAWAY PA 445 HOES LANE, PISCATAWAY, NJ 08855-4141 USA SN 1949-3053 EI 1949-3061 J9 IEEE T SMART GRID JI IEEE Trans. Smart Grid PD JUL PY 2016 VL 7 IS 4 BP 2061 EP 2070 DI 10.1109/TSG.2016.2543264 PG 10 WC Engineering, Electrical & Electronic SC Engineering GA DR1WY UT WOS:000379696800031 ER PT J AU Rimal, P Han, ST Hong, SJ Kim, HS Cho, KY Lee, I AF Rimal, Pradip Han, Seung Tek Hong, Soon-Jik Kim, Hyo-Seob Cho, Kuk Young Lee, Ilsueuk TI Effects of Bi2Se3 Amount in Thermoelectric Performance of Bi-2(TeSe)(3) Materials Fabricated by High-Energy Ball Milling SO INTERNATIONAL JOURNAL OF APPLIED CERAMIC TECHNOLOGY LA English DT Article DE Bi-2(TeSe)(3) materials; high-energy ball milling; microstructure; thermoelectric properties ID FIGURE-OF-MERIT; BISMUTH-TELLURIDE; GAS-ATOMIZATION; HOT EXTRUSION; ALLOYS; ENHANCEMENT; GENERATION; TRANSPORT AB Amount of Bi2Se3 has significant role in controlling thermoelectric properties of n-type Bi-2(TeSe)(3) material. In this study, effects of Se alloying amount in Bi-2(TeSe)(3) thermoelectric materials fabricated by high-energy ball milling and spark plasma sintering were studied and compared with other fabrication methods. Amount of Bi2Se3 (5%, 10%, 15%, and 20%) did not have any significant effect over fabricated powder size, grains of consolidated bulks, and mechanical properties; however, electrical properties and thermoelectric efficiency were noticeably influenced. Both carrier concentration and carrier mobility decreased with increase in Se amount. In total, 20% Se alloying was effective in improving thermoelectric figure of merit ZT value by almost 40% compared with only 5% Se alloying. C1 [Rimal, Pradip; Han, Seung Tek; Hong, Soon-Jik] Kongju Natl Univ, Div Adv Mat Engn, Cheonan 330717, South Korea. [Kim, Hyo-Seob] Iowa State Univ, Met Dev, Ames Lab, Ames, IA 50011 USA. [Cho, Kuk Young] Hanyang Univ, Dept Mat Sci & Chem Engn, Ansan 15588, South Korea. [Lee, Ilsueuk] Korea Inst Ind Technol KITECH, Korea Natl Cleaner Prod Ctr, Seoul 06211, South Korea. RP Hong, SJ (reprint author), Kongju Natl Univ, Div Adv Mat Engn, Cheonan 330717, South Korea. EM hongsj@kongju.ac.kr FU Korea Institute of Energy Technology Evaluation and Planning (KETEP) - Korea Government Ministry of Knowledge Economy [20115010100020]; National Research Foundation of Korea (NRF) - Ministry of Education, Science and Technology [NRF-2015R1D1A1A09060920] FX This work was supported by the Korea Institute of Energy Technology Evaluation and Planning (KETEP) grant funded by the Korea Government Ministry of Knowledge Economy (N0. 20115010100020). This work was supported by the Basic Science Research Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Education, Science and Technology (NRF-2015R1D1A1A09060920). NR 29 TC 1 Z9 1 U1 11 U2 17 PU WILEY-BLACKWELL PI HOBOKEN PA 111 RIVER ST, HOBOKEN 07030-5774, NJ USA SN 1546-542X EI 1744-7402 J9 INT J APPL CERAM TEC JI Int. J. Appl. Ceram. Technol. PD JUL-AUG PY 2016 VL 13 IS 4 BP 711 EP 717 DI 10.1111/ijac.12534 PG 7 WC Materials Science, Ceramics SC Materials Science GA DR5MA UT WOS:000379945900013 ER PT J AU Erickson, BA Ju, X Nibler, JW Beaudry, CM Blake, TA AF Erickson, B. A. Ju, X. Nibler, J. W. Beaudry, C. M. Blake, T. A. TI High-resolution infrared studies of perdeutero-spiropentane, C5D8 SO JOURNAL OF MOLECULAR SPECTROSCOPY LA English DT Article DE Spiropentane; C5H8 and C5D8; High-resolution infrared spectrum; Rovibrational constants; Molecular structure: DFT study; Anharmonic frequencies ID SPECTROSCOPY; BANDS; C5H8 AB Perdeutero-spiropentane (C5D8) has been synthesized, and infrared and Raman spectra are reported for the first time. Wavenumber assignments are made for most of the fundamental vibrational states. Gas phase infrared spectra were recorded at a resolution (0.002 cm(-1)) sufficient to resolve individual rovibrational lines and show evidence of strong Coriolis and/or Fermi resonance interactions for most bands. However a detailed rovibrational analysis of the fundamental v(15) (b(2)) parallel band proved possible, and a fit of more than 1600 lines yielded a band origin of 1053.84465(10) cm(-1) and ground state constants (in units of cm(-1)): B-0 = 0.1120700(9), D-j = 1.51(3) x 10(-8), DJK = 3.42(15) x 10(-8). We note that the B-0 value is significantly less than a value of B-a = 0.1140 cm(-1) calculated using structural parameters from an earlier electron diffraction (ED) study, whereas one expects Ba to be lower than Bo because of thermal averaging over higher vibrational levels. A similar discrepancy was noted in an earlier study of C5H8 (Price et al., 2011). The structural and spectroscopic results are in good accord with values computed at the anharmonic level using the B3LYP density functional method with a cc-pVTZ basis set. (C) 2016 Elsevier Inc. All rights reserved. C1 [Erickson, B. A.; Ju, X.; Nibler, J. W.; Beaudry, C. M.] Oregon State Univ, Dept Chem, Corvallis, OR 97332 USA. [Blake, T. A.] Pacific Northwest Natl Lab, POB 999,Mail Stop K8-88, Richland, WA 99352 USA. RP Nibler, JW (reprint author), Oregon State Univ, Dept Chem, Corvallis, OR 97332 USA. EM Niblerj@chem.orst.edu FU Camille and Henry Dreyfus Senior Scientist Mentor Award; U.S. Department of Energy [DE-AC05-76RL01830] FX J. Nibler acknowledges a Camille and Henry Dreyfus Senior Scientist Mentor Award which provided support of B. Erickson. The infrared spectra were recorded at the Pacific Northwest National Laboratory (PNNL) located in Richland, WA, USA. The Pacific Northwest National Laboratory is operated by Battelle Memorial Institute for the U.S. Department of Energy under Contract No. DE-AC05-76RL01830. NR 20 TC 0 Z9 0 U1 1 U2 1 PU ACADEMIC PRESS INC ELSEVIER SCIENCE PI SAN DIEGO PA 525 B ST, STE 1900, SAN DIEGO, CA 92101-4495 USA SN 0022-2852 EI 1096-083X J9 J MOL SPECTROSC JI J. Mol. Spectrosc. PD JUL PY 2016 VL 325 BP 13 EP 19 DI 10.1016/j.jms.2016.05.003 PG 7 WC Physics, Atomic, Molecular & Chemical; Spectroscopy SC Physics; Spectroscopy GA DR4RE UT WOS:000379889100003 ER PT J AU Kim, J Shi, XB Casa, D Qian, J Huang, XR Gog, T AF Kim, Jungho Shi, Xianbo Casa, Diego Qian, Jun Huang, XianRong Gog, Thomas TI Collimating Montel mirror as part of a multi-crystal analyzer system for resonant inelastic X-ray scattering SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE X-ray optics; multilayer mirror; X-ray collimation; resonant inelastic X-ray scattering ID GRADED MULTILAYER MIRROR; NSLS-II; EXCITATIONS; TESTS AB Advances in resonant inelastic X-ray scattering (RIXS) have come in lockstep with improvements in energy resolution. Currently, the best energy resolution at the Ir L-3-edge stands at similar to 25 meV, which is achieved using a diced Si(844) spherical crystal analyzer. However, spherical analyzers are limited by their intrinsic reflection width. A novel analyzer system using multiple flat crystals provides a promising way to overcome this limitation. For the present design, an energy resolution at or below 10 meV was selected. Recognizing that the angular acceptance of flat crystals is severely limited, a collimating element is essential to achieve the necessary solid-angle acceptance. For this purpose, a laterally graded, parabolic, multilayer Montel mirror was designed for use at the Ir L-3-absorption edge. It provides an acceptance larger than 10 mrad, collimating the reflected X-ray beam to smaller than 100 mrad, in both vertical and horizontal directions. The performance of this mirror was studied at beamline 27-ID at the Advanced Photon Source. X-rays from a diamond (111) monochromator illuminated a scattering source of diameter 5 mm, generating an incident beam on the mirror with a well determined divergence of 40 mrad. A flat Si(111) crystal after the mirror served as the divergence analyzer. From X-ray measurements, ray-tracing simulations and optical metrology results, it was established that the Montel mirror satisfied the specifications of angular acceptance and collimation quality necessary for a high-resolution RIXS multi-crystal analyzer system. C1 [Kim, Jungho; Shi, Xianbo; Casa, Diego; Qian, Jun; Huang, XianRong; Gog, Thomas] Argonne Natl Lab, Adv Photon Source, 9700 South Cass Ave, Argonne, IL 60439 USA. RP Kim, J (reprint author), Argonne Natl Lab, Adv Photon Source, 9700 South Cass Ave, Argonne, IL 60439 USA. EM jhkim@aps.anl.gov FU US DOE [DE-AC02-06CH11357] FX The authors would like to thank M. G. Honnicke for the initial design of the Montel mirror. Use of the Advanced Photon Source, an Office of Science User Facility operated for the US DOE Office of Science by Argonne National Laboratory, was supported by the US DOE under Contract No. DE-AC02-06CH11357. NR 15 TC 1 Z9 1 U1 6 U2 6 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD JUL PY 2016 VL 23 BP 880 EP 886 DI 10.1107/S1600577516007426 PN 4 PG 7 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DR5PJ UT WOS:000379954600005 PM 27359136 ER PT J AU Crawford, AM Kurecka, P Yim, TK Kozemchak, C Deb, A Dostal, L Sun, CJ Brewe, DL Barrea, R Penner-Hahn, JE AF Crawford, Andrew M. Kurecka, Patrick Yim, Tsz Kwan Kozemchak, Claire Deb, Aniruddha Dostal, Lubomir Sun, Cheng-Jun Brewe, Dale L. Barrea, Raul Penner-Hahn, James E. TI Development of a single-cell X-ray fluorescence flow cytometer SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE flow cytometry; X-ray fluorescence; single cell; metallome; homeostasis ID RED-BLOOD-CELLS; SACCHAROMYCES-CEREVISIAE; IRON HOMEOSTASIS; TRACE METALS; HUMAN PLASMA; ICP-MS; ZINC; COPPER; YEAST; MAGNESIUM AB An X-ray fluorescence flow cytometer that can determine the total metal content of single cells has been developed. Capillary action or pressure was used to load cells into hydrophilic or hydrophobic capillaries, respectively. Once loaded, the cells were transported at a fixed vertical velocity past a focused X-ray beam. X-ray fluorescence was then used to determine the mass of metal in each cell. By making single-cell measurements, the population heterogeneity for metals in the mu M to mM concentration range on fL sample volumes can be directly measured, a measurement that is difficult using most analytical methods. This approach has been used to determine the metal composition of 936 individual bovine red blood cells (bRBC), 31 individual 3T3 mouse fibroblasts (NIH3T3) and 18 Saccharomyces cerevisiae (yeast) cells with an average measurement frequency of similar to 4 cells min(-1). These data show evidence for surprisingly broad metal distributions. Details of the device design, data analysis and opportunities for further sensitivity improvement are described. C1 [Crawford, Andrew M.; Kurecka, Patrick; Yim, Tsz Kwan; Kozemchak, Claire; Deb, Aniruddha; Dostal, Lubomir; Penner-Hahn, James E.] Univ Michigan, Dept Chem, Ann Arbor, MI 48109 USA. [Deb, Aniruddha; Penner-Hahn, James E.] Univ Michigan, Dept Biophys, Ann Arbor, MI 48109 USA. [Sun, Cheng-Jun; Brewe, Dale L.] Argonne Natl Lab, Xray Sci Div, 9700 South Cass Ave, Argonne, IL 60439 USA. [Barrea, Raul] Depaul Univ, Dept Phys, Chicago, IL 60604 USA. RP Penner-Hahn, JE (reprint author), Univ Michigan, Dept Chem, Ann Arbor, MI 48109 USA.; Penner-Hahn, JE (reprint author), Univ Michigan, Dept Biophys, Ann Arbor, MI 48109 USA. EM jeph@umich.edu FU National Science Foundation [NSF-IDBR-0852802]; National Institutes of Health [9 P41 GM103622]; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357]; US Department of Energy, Basic Energy Sciences; Canadian Light Source; University of Washington; Advanced Photon Source FX This research was funded in part by the National Science Foundation under (NSF-IDBR-0852802 to JEPH). LD was supported by the National Institutes of Health (9 P41 GM103622). This research used resources of the Advanced Photon Source, a US Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. Sector 20 facilities at the APS is supported by the US Department of Energy, Basic Energy Sciences, the Canadian Light Source and its funding partners, the University of Washington, and the Advanced Photon Source. The staff of the LSA Scientific Instruments Shop provided valuable collaboration on sample holder design. The authors would like to thank Erik Guetschow for assistance with the syphon pump. NR 37 TC 1 Z9 1 U1 3 U2 7 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD JUL PY 2016 VL 23 BP 901 EP 908 DI 10.1107/S1600577516008006 PN 4 PG 8 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DR5PJ UT WOS:000379954600007 PM 27359138 ER PT J AU Feng, H Zhang, WG Qian, Y Liu, WL Yu, LZ Yoo, SJ Wang, J Wang, JJ Eng, C Liu, CJ Tappero, R AF Feng, Huan Zhang, Weiguo Qian, Yu Liu, Wenliang Yu, Lizhong Yoo, Shinjae Wang, Jun Wang, Jia-Jun Eng, Christopher Liu, Chang-Jun Tappero, Ryan TI Synchrotron X-ray microfluorescence measurement of metal distributions in Phragmites australis root system in the Yangtze River intertidal zone SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE Yangtze River intertidal zone; metal uptake; Phragmites australis; Fe nanoparticles ID URBAN BROWNFIELD SITE; TYPHA-LATIFOLIA ROOT; IRON PLAQUE; IMPERATA-CYLINDRICA; ASTER-TRIPOLIUM; AQUATIC PLANTS; WETLAND PLANTS; RICE ROOTS; FE-PLAQUE; IN-SITU AB This study investigates the distributions of Br, Ca, Cl, Cr, Cu, K, Fe, Mn, Pb, Ti, V and Zn in Phragmites australis root system and the function of Fe nanoparticles in scavenging metals in the root epidermis using synchrotron X-ray microfluorescence, synchrotron transmission X-ray microscope measurement and synchrotron X-ray absorption near-edge structure techniques. The purpose of this study is to understand the mobility of metals in wetland plant root systems after their uptake from rhizosphere soils. Phragmites australis samples were collected in the Yangtze River intertidal zone in July 2013. The results indicate that Fe nanoparticles are present in the root epidermis and that other metals correlate significantly with Fe, suggesting that Fe nanoparticles play an important role in metal scavenging in the epidermis. C1 [Feng, Huan; Qian, Yu] Montclair State Univ, Dept Earth & Environm Studies, Montclair, NJ 07043 USA. [Zhang, Weiguo; Liu, Wenliang; Yu, Lizhong] East China Normal Univ, State Key Lab Estuarine & Coastal Res, Shanghai 200062, Peoples R China. [Yoo, Shinjae] Brookhaven Natl Lab, Computat Sci Ctr, Upton, NY 11973 USA. [Wang, Jun; Wang, Jia-Jun; Eng, Christopher; Tappero, Ryan] Brookhaven Natl Lab, Photon Sci Directorate, Upton, NY 11973 USA. [Liu, Chang-Jun] Brookhaven Natl Lab, Biol Sci Dept, Upton, NY 11973 USA. RP Feng, H (reprint author), Montclair State Univ, Dept Earth & Environm Studies, Montclair, NJ 07043 USA. EM fengh@mail.montclair.edu FU State Key Laboratory of Estuarine and Coastal Research Open Research Fund [SKLEC-KF201304]; China Scholarship Council; Margaret and Herman Sokol Foundation; US Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Visiting Faculty Program (VFP); US Department of Energy, Office of Science, Office of Basic Energy Sciences [DE-AC02-98CH10886]; US Department of Energy - Geosciences [DE-FG02-92ER14244]; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357]; National Synchrotron Light Source II, Brookhaven National Laboratory, under DOE [DE-SC0012704]; National Science Foundation [MCB-1051675]; Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences of the US Department of Energy [DEAC0298CH10886] FX We would like to thank Dr S. M. Heald (Co-editor of Journal of Synchrotron Radiation), Dr A. Weight (Managing Editor of Journal of Synchrotron Radiation) and two anonymous reviewers for their constructive comments and suggestions which have improved the quality of an early version of this manuscript. This work was supported in part by the State Key Laboratory of Estuarine and Coastal Research Open Research Fund (SKLEC-KF201304) (HF, WZ, LY, WL, YQ), the China Scholarship Council (YQ), and the Margaret and Herman Sokol Foundation (HF). This project was also supported in part by the US Department of Energy, Office of Science, Office of Workforce Development for Teachers and Scientists (WDTS) under the Visiting Faculty Program (VFP) (HF). Use of the NSLS was supported by the US Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. DE-AC02-98CH10886. NSLS X27A was supported in part by the US Department of Energy - Geosciences (DE-FG02-92ER14244 to The University of Chicago - CARS). This research used resources of the Advanced Photon Source, a US Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under Contract No. DE-AC02-06CH11357. Use of APS beamline 8BM is partially supported by the National Synchrotron Light Source II, Brookhaven National Laboratory, under DOE Contract No. DE-SC0012704. The part of work carried out at Biology Department, Brookhaven National Laboratory, was supported in part by the National Science Foundation through grant MCB-1051675 and by the Division of Chemical Sciences, Geosciences and Biosciences, Office of Basic Energy Sciences of the US Department of Energy through Grant DEAC0298CH10886 to CJL. NR 47 TC 0 Z9 0 U1 10 U2 20 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD JUL PY 2016 VL 23 BP 937 EP 946 DI 10.1107/S1600577516008146 PN 4 PG 10 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DR5PJ UT WOS:000379954600011 PM 27359142 ER PT J AU Monteforte, M Estandarte, AK Chen, B Harder, R Huang, MH Robinson, IK AF Monteforte, Marianne Estandarte, Ana K. Chen, Bo Harder, Ross Huang, Michael H. Robinson, Ian K. TI Novel silica stabilization method for the analysis of fine nanocrystals using coherent X-ray diffraction imaging SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE Bragg coherent X-ray diffraction; nanocrystals; stabilization method; three-dimensional reconstruction; strain ID NANOPARTICLES; DEPOSITION AB High-energy X-ray Bragg coherent diffraction imaging (BCDI) is a well established synchrotron-based technique used to quantitatively reconstruct the three-dimensional morphology and strain distribution in nanocrystals. The BCDI technique has become a powerful analytical tool for quantitative investigations of nanocrystals, nanotubes, nanorods and more recently biological systems. BCDI has however typically failed for fine nanocrystals in sub-100 nm size regimes - a size routinely achievable by chemical synthesis - despite the spatial resolution of the BCDI technique being 20-30 nm. The limitations of this technique arise from the movement of nanocrystals under illumination by the highly coherent beam, which prevents full diffraction data sets from being acquired. A solution is provided here to overcome this problem and extend the size limit of the BCDI technique, through the design of a novel stabilization method by embedding the fine nanocrystals into a silica matrix. Chemically synthesized FePt nanocrystals of maximum dimension 20 nm and AuPd nanocrystals in the size range 60-65 nm were investigated with BCDI measurement at beamline 34-ID-C of the APS, Argonne National Laboratory. Novel experimental methodologies to elucidate the presence of strain in fine nanocrystals are a necessary pre-requisite in order to better understand strain profiles in engineered nanocrystals for novel device development. C1 [Monteforte, Marianne; Estandarte, Ana K.; Chen, Bo; Robinson, Ian K.] UCL, London Ctr Nanotechnol, Gower St, London WC1E 6BT, England. [Harder, Ross] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA. [Huang, Michael H.] Natl Tsing Hua Univ, Guangfu Rd, Hsinchu 300, Taiwan. RP Monteforte, M (reprint author), UCL, London Ctr Nanotechnol, Gower St, London WC1E 6BT, England. EM marianne.monteforte.10@ucl.ac.uk OI Robinson, Ian/0000-0003-4897-5221 FU Diamond Light Source, an EPSRC [EP/I022562/1]; ERC [227711] FX This work was sponsored by a studentship to MM from the Diamond Light Source, an EPSRC grant EP/I022562/1, Phase modulation technology for X-ray imaging, and an ERC Advanced Grant 227711, Exploration of strains in synthetic nanocrystals. NR 15 TC 2 Z9 2 U1 4 U2 8 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD JUL PY 2016 VL 23 BP 953 EP 958 DI 10.1107/S1600577516006408 PN 4 PG 6 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DR5PJ UT WOS:000379954600013 PM 27359144 ER PT J AU Newman, JA Zhang, SJ Sullivan, SZ Dow, XY Becker, M Sheedlo, MJ Stepanov, S Carlsen, MS Everly, RM Das, C Fischetti, RF Simpson, GJ AF Newman, Justin A. Zhang, Shijie Sullivan, Shane Z. Dow, Ximeng Y. Becker, Michael Sheedlo, Michael J. Stepanov, Sergey Carlsen, Mark S. Everly, R. Michael Das, Chittaranjan Fischetti, Robert F. Simpson, Garth J. TI Guiding synchrotron X-ray diffraction by multimodal video-rate protein crystal imaging SO JOURNAL OF SYNCHROTRON RADIATION LA English DT Article DE nonlinear optical microscopy; protein crystal; synchronous digitization ID THROUGHPUT MACROMOLECULAR CRYSTALLOGRAPHY; SERIAL FEMTOSECOND CRYSTALLOGRAPHY; RADIATION-DAMAGE; FLUORESCENCE; BEAM; DETECTOR AB Synchronous digitization, in which an optical sensor is probed synchronously with the firing of an ultrafast laser, was integrated into an optical imaging station for macromolecular crystal positioning prior to synchrotron X-ray diffraction. Using the synchronous digitization instrument, second-harmonic generation, two-photon-excited fluorescence and bright field by laser transmittance were all acquired simultaneously with perfect image registry at up to video-rate (15 frames s(-1)). A simple change in the incident wavelength enabled simultaneous imaging by two-photon-excited ultraviolet fluorescence, one-photon-excited visible fluorescence and laser transmittance. Development of an analytical model for the signal-to-noise enhancement afforded by synchronous digitization suggests a 15.6-fold improvement over previous photon-counting techniques. This improvement in turn allowed acquisition on nearly an order of magnitude more pixels than the preceding generation of instrumentation and reductions of well over an order of magnitude in image acquisition times. These improvements have allowed detection of protein crystals on the order of 1 mu m in thickness under cryogenic conditions in the beamline. These capabilities are well suited to support serial crystallography of crystals approaching 1 mu m or less in dimension. C1 [Newman, Justin A.; Zhang, Shijie; Sullivan, Shane Z.; Dow, Ximeng Y.; Sheedlo, Michael J.; Carlsen, Mark S.; Everly, R. Michael; Das, Chittaranjan; Simpson, Garth J.] Purdue Univ, Dept Chem, 560 Oval Dr, W Lafayette, IN 47906 USA. [Becker, Michael; Stepanov, Sergey; Fischetti, Robert F.] Argonne Natl Lab, Xray Sci Div, GM CA APS, 9700 S Cass Ave, Argonne, IL 60439 USA. RP Simpson, GJ (reprint author), Purdue Univ, Dept Chem, 560 Oval Dr, W Lafayette, IN 47906 USA. EM gsimpson@purdue.edu FU NIH grant from the NIGMS [R01GM-103401, R01GM-103910]; Federal funds from the National Cancer Institute [ACB-12002]; National Institute of General Medical Sciences [AGM-12006]; DOE Office of Science by Argonne National Laboratory [DE-AC02-06CH11357] FX JAN, SZ, SZS, XYD, MSC, RME and GJS gratefully acknowledge support from the NIH grant Nos. R01GM-103401 and R01GM-103910 from the NIGMS. MJS and CD also acknowledge support from R01GM-103401. GM/CA@APS has been funded in whole or in part with Federal funds from the National Cancer Institute (ACB-12002) and the National Institute of General Medical Sciences (AGM-12006). This research used resources of the Advanced Photon Source, a US Department of Energy (DOE) Office of Science User Facility operated for the DOE Office of Science by Argonne National Laboratory under contract No. DE-AC02-06CH11357. NR 32 TC 1 Z9 1 U1 3 U2 3 PU INT UNION CRYSTALLOGRAPHY PI CHESTER PA 2 ABBEY SQ, CHESTER, CH1 2HU, ENGLAND SN 1600-5775 J9 J SYNCHROTRON RADIAT JI J. Synchrot. Radiat. PD JUL PY 2016 VL 23 BP 959 EP 965 DI 10.1107/S1600577516005919 PN 4 PG 7 WC Instruments & Instrumentation; Optics; Physics, Applied SC Instruments & Instrumentation; Optics; Physics GA DR5PJ UT WOS:000379954600014 PM 27359145 ER EF